Heterometal incorporation in NH2-MIL-125(Ti) and its participation in the photoinduced charge-separated excited state
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Ion evaporation from aqueous nanodrops is measured for the first time using charge detection mass spectrometry, and the origin of solute ion dependent charging of large (MDa) macromolecules is revealed.
Understanding the physical and chemical processes occurring in concentrated electrolyte solutions is required to achieve redox flow batteries with high energy density. Highly concentrated electrolyte solutions are often studied in which collective crowded interactions between molecules and ions become predominant. In this work, experimental and computational methods were used to examine non-aqueous electrolyte solutions in two different states of charge as a function of redoxmer concentration. As the latter increases and the ionic association strengthens, the electric conductivity passes through a maximum and the solution increasingly gels, which is seen through a rapid non-linear increase in viscosity. We establish that the structural rigidity of ionic networks is closely connected with this loss of fluidity and show that charging generally yields softer ionic assemblies with weaker attractive forces and improved dynamical properties.
We report a flux-integrated cross section measurement of muon neutrino interactions on water and hydrocarbon via charged current reactions without charged pions in the final state with the WAGASCI-BabyMIND detector, which was installed in the T2K near detector hall in 2018. The detector is located 1.5° off-axis and is exposed to a more energetic neutrino flux than ND280, another T2K near detector, which is located at a different off-axis position. The total flux-integrated cross section is measured to be 1.26 ± 0.18(stat+syst) × 10 −39 cm 2 /nucleon on CH and 1.44 ± 0.21(stat+syst) × 10 −39 cm 2 /nucleon on H 2 O. These results are compared to model predictions provided by the neut v5.3.2 and genie v2.8.0 Monte Carlo generators and the measurements are compatible with these models. Differential cross sections in muon momentum and cosine of the muon scattering angle are also reported. This is the first such measurement reported with the WAGASCI-BabyMIND detector and utilizes the 2020 and 2021 datasets.
Background: Energetic quarks in nuclear deep-inelastic scattering propagate through the nuclear medium. Processes that are believed to occur inside nuclei include quark energy loss through medium-stimulated gluon bremsstrahlung and intranuclear interactions of forming hadrons. More data are required to gain a more complete understanding of these effects. Purpose: To test the theoretical models of parton transport and hadron formation, we compared their predictions for the nuclear and kinematic dependence of pion production in nuclei. Methods: We have measured charged-pion production in semi-inclusive deep-inelastic scattering off D, C, Fe, and Pb using the CLAS detector and the CEBAF 5.014-GeV electron beam. We report results on the nuclear-to-deuterium multiplicity ratio for π + and π - as a function of energy transfer, four-momentum transfer, and pion energy fraction or transverse momentum—the first three-dimensional study of its kind. Results: The π + multiplicity ratio is found to depend strongly on the pion fractional energy z and reaches minimum values of 0.67 ± 0.03, 0.43 ± 0.02, and 0.27 ± 0.01 for the C, Fe, and Pb targets, respectively. The z dependencies of the multiplicity ratios for π + and π - are equal within uncertainties for C and Fe targets but show differences at the level of 10% for the Pb-target data. The results are qualitatively described by the GIBUU transport model, as well as with a model based on hadron absorption, but are in tension with calculations based on nuclear fragmentation functions. Conclusions: These precise results will strongly constrain the kinematic and flavor dependence of nuclear effects in hadron production, probing an unexplored kinematic region. They will help to reveal how the nucleus reacts to a fast quark, thereby shedding light on its color structure and transport properties and on the mechanisms of the hadronization process.
We study the separability of the Dirac equation in the background of four dimensional charged rotating asymptotically flat black hole solution of supergravity and the low energy string theory known as STU black hole. In particular, we analyze in detail the separability conditions in the pairwise equal charge STU black hole space-time. While in the latter case the minimally coupled Dirac equation is not separable, the introduction of a specific torsion term ensures the separability. The source of the torsion is the Kalb-Ramond field, which is an integral part of string theory, but further aspects of its properties and coupling to fermionic fields remain to be studied. To derive the torsion, two different approaches are used in conformally related frames, showing that the torsion is not unique. The correspondingly modified Dirac equations in the Einstein and string frames are shown to be separable. Furthermore, the massless radial and angular wave equations are examined; they show close similarity with corresponding equations for the standard Kerr background. A generalization of the Teukolsky equation for the pairwise equal case is conjectured. We also briefly analyze a technically sophisticated radial equation in the massive case.
A reversible density driven insulator to metal to insulator transition in high-spin MnS 2 is experimentally observed, leading with a colossal electrical resistance drop of $10^8$ Omega by 12 GPa. Density functional theory simulations reveal the metallization to be unexpectedly driven by previously unoccupied $S_{2}^{-2}$ $\sigma^{*}_{3p}$ antibonding states crossing the Fermi level. This is a unique variant of the charge transfer insulator to metal transition for negative charge transfer insulators having anions with an unsaturated valence. By 36 GPa the emergence of the low-spin insulating arsenopyrite ($P2_1/c$) is confirmed, and the bulk metallicity is broken with the system returning to an insulative electronic state.
Understanding electron neutrino interactions is crucial for measurements of neutrino oscillations and searches for new physics in neutrino experiments. We present the first measurement of the flux-averaged $𝜈_𝑒$ + $\bar{𝜈}_𝑒$ charged-current single charged-pion production cross section on argon using the MicroBooNE detector and data from the NuMI neutrino beam. The total cross section is measured to be [0.93 ± 0.13(stat) ± 0.27(syst)] × 10 −39 cm 2 /nucleon at a mean $𝜈_𝑒$ + $\bar{𝜈}_𝑒$ energy of 730 MeV. Differential cross sections are also reported in electron energy, electron and pion angles, and electron-pion opening angle.
This data set includes modeling results from The 2030 National Charging Network: Estimating U.S. Light-Duty Demand for Electric Vehicle Charging Infrastructure, including region-specific (i.e., national, state, and core-based statistical area cities and towns) electric vehicle supply equipment port count requirements in 2025 and 2030 for multiple scenarios described in the study.
Resonant neutrino–nucleus processes constitute a significant portion of neutrino interactions in the few-GeV energy region. Charged-current interactions with a muon and one single charged pion in the final state (CC1$\pi$) are primarily sensitive to resonant processes, while also receiving contributions from non-resonant processes and being strongly affected by nuclear effects and final-state interactions. A precise understanding of this channel is essential for improving neutrino interaction models and reducing systematic uncertainties in oscillation measurements. The Short-Baseline Near Detector (SBND) at Fermilab has collected the largest neutrino–argon dataset to date, providing an excellent opportunity to study CC1$\pi$ interactions on argon. This analysis aims to improve existing single-differential cross-section measurements by reporting results in a variety of kinematic variables and to perform the first double-differential CC1$\pi$ cross-section measurement on argon, using novel techniques for pion energy reconstruction.
Low collision energy charge transfer and dissociative charge transfer between rare gas ions and molecular nitrogen, measuring nitrogen ion kinetic energy distributions
The CHARGE-2 sounding rocket payload has measured the transient and steady-state charging of a spacecraft in LEO during the emission of a low-power electron beam. The electron beam successfully escaped the emitting spacecraft above 240 km, rather than being degraded by the spacecraft's potentials. These potentials were limited to about half of the 1-kV beam accelerating potential at all latitudes, suggesting that the electron beam was able to escape at altitudes down to 160 km. Electrons created from beam-plasma interactions become increasingly important in the return current below 240 km, and increased with decreasing altitude.
As part of ongoing research at Marshall Space Flight Center, Cadmium-Zinc- Telluride (CdZnTe) pixilated detectors are being developed for use at the focal plane of the High Energy Replicated Optics (HERO) telescope. HERO requires a 64x64 pixel array with a spatial resolution of around 200 microns (with a 6m focal length) and high energy resolution (< 2% at 60keV). We are currently testing smaller arrays as a necessary first step towards this goal. In this presentation, we compare charge sharing and charge loss measurements between two devices that differ both electronically and geometrically. The first device consists of a 1-mm-thick piece of CdZnTe that is sputtered with a 4x4 array of pixels with pixel pitch of 750 microns (inter-pixel gap is 100 microns). The signal is read out using discrete ultra-low-noise preamplifiers, one for each of the 16 pixels. The second detector consists of a 2-mm-thick piece of CdZnTe that is sputtered with a 16x16 array of pixels with a pixel pitch of 300 microns (inter-pixel gap is 50 microns). Instead of using discrete preamplifiers, the crystal is bonded to an ASIC that provides all of the front-end electronics to each of the 256 pixels. what degree the bias voltage (i.e. the electric field) and hence the drift and diffusion coefficients affect our measurements. Further, we compare the measured results with simulated results and discuss to
Recent JPL absolute excitation and charge exchange cross sections, and measurements of lifetimes of metastable levels in highly-charged ions (HCIs) are reported. These data provide benchmark comparisons to results of theoretical calculations. Theoretical approaches can then be used to calculate the vast array of data which cannot be measured due to experimental constraints. Applications to the X-ray emission from comets are given.
Today's presentation is a short tutorial on auroral charging of spacecraft and the characteristics of the space plasma environment that are required to predict charging.
Low noise CCDs fully-depleted up to 675 micrometers have been identified as a unique tool for Dark Matter searches and low energy neutrino physics. The charge collection efficiency (CCE) for these detectors is a critical parameter for the performance of future experiments. We present here a new technique to characterize CCE in back-illuminated CCDs based on soft X-rays. This technique is used to characterize two different detector designs. The results demonstrate the importance of the backside processing for detection near threshold, showing that a recombination layer of a few microns significantly distorts the low energy spectrum. The studies demonstrate that the region of partial charge collection can be reduced to less than 1 micrometer thickness with adequate backside processing.
The study of neutrino oscillations is a main priority for particle physics as the most immediately tractable lever on physics beyond the Standard Model. In particular, more insight into violation of the combined symmetry of charge-conjugation plus parity could yield clues to the origin of matter-antimatter asymmetry, and in some theoretical frameworks the neutrino mass could give insights into dark matter. NOvA is a long-baseline accelerator neutrino experiment with both a near and far detector that seeks to measure several of the parameters of the neutrino mixing matrix, as well as carry out a broad program of additional physics. NOvA has innovated and developed a variety of techniques in the space of neutrino physics, including expanding the use of machine learning techniques in reconstruction. NOvA has also set the stage for the next generation US-based long baseline experiment, DUNE. This dissertation details the creation of a new neutrino interaction vertex reconstruction package for NOvA, which offers enormous improvements in accuracy above the previous vertexer it replaces. This is accomplished using a Convolutional Visual Network trained on large datasets of simulated events. The vertexer is validated thoroughly against data. This dissertation also presents a cross-section measurement for $\nu_\mu + N \rightarrow \mu^- + 1\pi^\pm + X$ (where X does not include additional charged pions) binned in pion kinetic energy, a challenging measurement in general and for NOvA in particular. Measurements like this provide crucial inputs for neutrino interaction models utilized by neutrino oscillation experiments. This measurement in particular is important to the energy ranges relevant for DUNE in a band not well-covered by any other experiment.
This presentation, part of the 2020 Vehicle Technologies Office Annual Merit Review and Peer Evaluation Meeting, discusses the development of a multiport, >1 MW charging system for medium- and heavy-duty electric vehicles.