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DOE OSTI2024

Undulator radiation of single electrons: coherence length and quantum-optical properties

The aims of the CLARA experiment at the Fermilab Integrable Optics Test Accelerator (IOTA) were to directly measure the coherence length of undulator radiation emitted by a single electron and to test whether the radiation is in a pure classical Glauber coherent state or in a quantum mixture of coherent and Fock states. We used a Mach-Zehnder interferometer (MZI) to study visible radiation generated by 150-MeV electrons circulating in the ring. The relative delay between the two arms of the MZI was adjusted by varying the length of one of them with a resolution of 10 nm. The intensity of the circulating beam spanned several orders of magnitude, down to single electrons. A pair of single-photon avalanche diodes (SPADs) was placed at the output of the MZI arms to detect photocounts with high efficiency and timing resolution. We describe the observed interference patterns and photocount rates as a function of interferometer delay and discuss their implications.

43 PARTICLE ACCELERATORS↗

DOE OSTI2024

Undulator Radiation of Single Electrons: Coherence Length and Quantum-Optical Properties

43 PARTICLE ACCELERATORS↗

NASA NTRS2012

Real Time In Situ Observations of Equiaxed Dendrite Coherency in Al-Cu Alloys Using High-Brilliance, 3rd Generation Synchrotron Sources

In the last decade synchrotron X-ray sources have fast become the tool of choice for performing in-situ high resolution imaging during alloy solidification. This paper presents the results of an experimental campaign carried out at the European Synchrotron Radiation Facility, using a Bridgman furnace, to monitor phenomena during solidification of Al-Cu alloys - specifically the onset of equiaxed dendrite coherency. Conventional experimental methods for determining coherency involve measuring the change in viscosity or measuring the change in thermal conductivity across the solidifying melt Conflicts arise when comparing the results of these experimental techniques to find a relationship between cooling rate and coherency fraction. It has been shown that the ratio of average velocity to the average grain diameter has an inversely proportional relationship to coherency fraction. In-situ observation therefore makes it possible to measure these values directly from acquired images sequences and make comparisons with published results.

Murphy, Andrew G.↗

DOE OSTI2024

Witnessing Entanglement and Quantum Correlations in Condensed Matter: A Review

The detection and certification of entanglement and quantum correlations in materials is of fundamental and far-reaching importance, and has seen significant recent progress. It impacts both the understanding of the basic science of quantum many-body phenomena as well as the identification of systems suitable for novel technologies. Frameworks suitable to condensed matter that connect measurements to entanglement and coherence have been developed in the context of quantum information theory. These take the form of entanglement witnesses and quantum correlation measures. Here, the underlying theory of these quantities, their relation to condensed matter experimental techniques, and their application to real materials are comprehensively reviewed. In addition, their usage in, e.g., protocols, the relative advantages and disadvantages of witnesses and measures, and future prospects in, e.g., correlated electrons, entanglement dynamics, and entangled spectroscopic probes, are presented. Consideration is given to the interdisciplinary nature of this emerging research and substantial ongoing progress by providing an accessible and practical treatment from fundamentals to application. Particular emphasis is placed on quantities accessible to collective measurements, including by susceptibility and spectroscopic techniques. This includes the magnetic susceptibility witness, one-tangle, concurrence and two-tangle, two-site quantum discord, and quantum coherence measures such as the quantum Fisher information.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2023

Hard x-ray – optical four-wave mixing using a split-and-delay line

New, hard x-ray free electron lasers (FEL) produce intense femtosecond-to-attosecond pulses at angstrom wavelengths, giving access to the fundamental spatial and temporal scales of matter. These revolutionary light sources open the door to applying the suite of nonlinear, optical spectroscopy methods at hard x-ray photon energies. Nonlinear spectroscopy with hard x-rays can allow for measuring the coherence properties of short wavelength excitations with atomic specificity and for understanding how high energy excitations couple to other degrees of freedom in atomic, molecular or condensed-phase systems. As a step in this direction, here we present hard x-ray, optical four-wave mixing (4WM) measurements done at 9.8 keV at the split-and-delay line at the x-ray correlation spectroscopy (XCS) hutch of the Linac Coherent Light Source (LCLS). In this work, we create an x-ray transient grating (TG) from a pair of crossing x-ray beams and diffract optical laser pulses at 400 nm from the TG. The key technical advance here is being able to independently vary the delays of the x-ray pulses. Measurements were made in 3 different solid samples: bismuth germinate (BGO), zinc oxide (ZnO) and yttrium aluminum garnet (YAG). The resulting phase-matched, 4WM signal is measured in two different ways: by varying the x-ray, x-ray pulse delay which can reveal both material and light source coherence properties and also by varying the optical laser delay with respect to the x-ray TG to study how the x-ray excitation couples to the optical properties. Although no coherent 4WM signal was seen in these measurements, the absence of this signal gives important information on experimental requirements for detecting this in future work. Also, our laser-delay scans, although not a new measurement, were applied to different materials than in past work and reveal new examples x-ray induced lattice dynamics in solids. This work represents a key step towards extending nonlinear optics and time-resolved spectroscopy into the hard x-ray regime.

47 OTHER INSTRUMENTATION↗

NASA NTRS1992

Elliptic jets, part 2. Dynamics of coherent structures: Pairing

The dynamics of the jet column mode of vortex pairing in the near field of an elliptic jet was investigated. Hot-wire measurements and flow visualization were used to examine the details of the pairing mechanism of nonplanar vortical elliptic structures and its effect on such turbulence measures as coherent velocities, incoherent turbulence intensities, incoherent and coherent Reynolds, stresses, turbulence production, and mass entrainment. It was found that pairing of elliptic vortices in the jet column does not occur uniformly around the entire perimeter, unlike in a circular jet. Merger occurs only in the initial major-axis plane. In the initial minor-axis plane, the trailing vortex rushes through the leading vortex without pairing and then breaks down violently, producing considerably greater entrainment and mixing than in circular or plane jets.

Husain, Hyder S.↗

NASA NTRS1991

Elliptic jets. II - Dynamics of coherent structures: Pairing

The dynamics of the jet column mode of vortex pairing in the near field of an elliptic jet was investigated. Hot-wire measurements and flow visualization were used to examine the details of the pairing mechanism of nonplanar vortical elliptic structures and its effect on such turbulence measures as coherent velocities, incoherent turbulence intensities, incoherent and coherent Reynolds, stresses, turbulence production, and mass entrainment. It was found that pairing of elliptic vortices in the jet column does not occur uniformly around the entire perimeter, unlike in a circular jet. Merger occurs only in the initial major-axis plane. In the inital minor-axis plane, the trailing vortex rushes through the leading vortex without pairing and then breaks down violently, producing considerably greater entrainment and mixing than in circular or plane jets.

Husain, Hyder S.↗

NASA NTRS1992

Determining the coherence of micropulses

A technique based on analysis of the cross spectra of single-use data from pulsars is described which can be used to measure the coherence properties of, and search for coherent periodicities in, pulsar signals. Several simulated pulsar models are constructed and analyzed to test the technique. From an analysis of 2000 consecutive pulses from PSR 2016 + 28 it is concluded that the micropulse coherence time of 430 MHz is less than the spin period for this object. This could could be consistent with a coherent model if the random phase jitter in such a model is 35 percent or more of the micropulse quasi-periodicity. The subpulse separation of roughly 10 ms is coherent across 4-5 pulse periods and is reasonably consistent with a model of subpulse drift that allows for variation about some mean drift rate. A two-component shot-noise model can reproduce much of the structure seen in the individual pulses as well as the spectra of PSR 2016 + 28.

Strohmayer, T. E.↗

NASA NTRS1996

Coherent Lidar Design and Performance Verification

This final report summarizes the investigative results from the 3 complete years of funding and corresponding publications are listed. The first year saw the verification of beam alignment for coherent Doppler lidar in space by using the surface return. The second year saw the analysis and computerized simulation of using heterodyne efficiency as an absolute measure of performance of coherent Doppler lidar. A new method was proposed to determine the estimation error for Doppler lidar wind measurements without the need for an independent wind measurement. Coherent Doppler lidar signal covariance, including wind shear and turbulence, was derived and calculated for typical atmospheric conditions. The effects of wind turbulence defined by Kolmogorov spatial statistics were investigated theoretically and with simulations. The third year saw the performance of coherent Doppler lidar in the weak signal regime determined by computer simulations using the best velocity estimators. Improved algorithms for extracting the performance of velocity estimators with wind turbulence included were also produced.

Frehlich, Rod↗

NASA NTRS1989

Spectral analysis, digital integration, and measurement of low backscatter in coherent laser radar

A method of surface acoustic wave (SAW) spectral analysis and digital integration that has been used previously in coherent CW laser work with CO2 lasers at 10.6 microns is described. Expressions are derived for the signal to noise ratio in the measured voltage spectrum with an approximation for the general case and rigorous treatment for the low signal case. The atmospheric backscatter data accumulated by the airborne LATAS (laser true airspeed) coherent laser radar system are analyzed.

Vaughan, J. M.↗

NASA NTRS1986

Airborne Doppler lidar measurements

This paper describes recent measurements using coherent Doppler lidars operating at a wavelength of 10.6 microns aboard the NASA Ames Convair 990. The purpose of the measurements was to obtain data on the atmospheric wind fields and the distribution of the backscatter coefficient at 10.6 microns. A decription of the instruments is provided detailing the modifications incorporated following the 1981 test flights of the systems. The measurement program is outlined, and preliminary results are discussed.

Bilbro, James W.↗

NASA NTRS1994

On the theory of quantum measurement

Many so called paradoxes of quantum mechanics are clarified when the measurement equipment is treated as a quantized system. Every measurement involves nonlinear processes. Self consistent formulations of nonlinear quantum optics are relatively simple. Hence optical measurements, such as the quantum nondemolition (QND) measurement of photon number, are particularly well suited for such a treatment. It shows that the so called 'collapse of the wave function' is not needed for the interpretation of the measurement process. Coherence of the density matrix of the signal is progressively reduced with increasing accuracy of the photon number determination. If the QND measurement is incorporated into the double slit experiment, the contrast ratio of the fringes is found to decrease with increasing information on the photon number in one of the two paths.

Haus, Hermann A.↗

DOE OSTI2021

Observation of Quasiparticle Pair Production and Quantum Entanglement in Atomic Quantum Gases Quenched to an Attractive Interaction

We report observation of quasiparticle pair-production and characterize quantum entanglement created by a modulational instability in an atomic superfluid. By quenching the atomic interaction to attractive and then back to weakly repulsive, we produce correlated quasiparticles and monitor their evolution in a superfluid through evaluating the in situ density noise power spectrum, which essentially measures a 'homodyne' interference between ground state atoms and quasiparticles of opposite momenta. We observe large amplitude growth in the power spectrum and subsequent coherent oscillations in a wide spatial frequency band within our resolution limit, demonstrating coherent quasiparticle generation and evolution. Here, the spectrum is observed to oscillate below a quantum limit set by the Peres-Horodecki separability criterion of continuous-variable states, thereby confirming quantum entanglement between interaction quench-induced quasiparticles.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

NASA NTRS1986

Analysis and measurement of electromagnetic scattering by pyramidal and wedge absorbers

By modifying the reflection coefficients in the Uniform Geometrical Theory of Diffraction a solution that approximates the scattering from a dielectric wedge is found. This solution agrees closely with the exact solution of Rawlins which is only valid for a few minor cases. This modification is then applied to the corner diffraction coefficient and combined with an equivalent current and geometrical optics solutions to model scattering from pyramid and wedge absorbers. Measured results from 12 inch pyramid absorbers from 2 to 18 GHz are compared to calculations assuming the returns add incoherently and assuming the returns add coherently. The measured results tend to be between the two curves. Measured results from the 8 inch wedge absorber are also compared to calculations with the return being dominated by the wedge diffraction. The procedures for measuring and specifying absorber performance are discussed and calibration equations are derived to calculate a reflection coefficient or a reflectivity using a reference sphere. Shaping changes to the present absorber designs are introduced to improve performance based on both high and low frequency analysis. Some prototypes were built and tested.

Dewitt, B. T.↗

DOE OSTI2024

Superconducting Qubits above 20 GHz Operating over 200 mK

Current state-of-the-art superconducting microwave qubits are cooled to extremely low temperatures to avoid sources of decoherence. Higher qubit operating temperatures would significantly increase the cooling power available, which is desirable for scaling up the number of qubits in quantum computing architectures and integrating qubits in experiments requiring increased heat dissipation. To operate superconducting qubits at higher temperatures, it is necessary to address both quasiparticle decoherence (which becomes significant for aluminum junctions above 160 mK) and dephasing from thermal microwave photons (which are problematic above 50 mK). Using low-loss niobium-trilayer junctions, which have reduced sensitivity to quasiparticles due to the higher superconducting transition temperature of niobium, we fabricate transmons with higher frequencies than previously studied, up to 24 GHz. We measure decoherence and dephasing times of about 1 μs, corresponding to average qubit quality factors of approximately 10 5 , and find that decoherence is unaffected by quasiparticles up to 1 K. Without relaxation from quasiparticles, we are able to explore dephasing from purely thermal sources, finding that our qubits can operate up to approximately 250 mK while maintaining similar performance. The thermal resilience of these qubits creates new options for scaling up quantum processors, enables hybrid quantum experiments with high heat-dissipation budgets, and introduces a material platform for even-higher-frequency qubits.

Josephson junctions↗

NASA NTRS1993

Coherent anti-Stokes Raman spectroscopy temperature measurements in a hydrogen-fueled supersonic combustor

Coherent anti-Stokes Raman spectroscopy (CARS) thermometry has been used to obtain static temperature cross sections in a three-dimensional supersonic combustor flowfield. Data were obtained in three spanwise planes downstream of a single normal fuel injector which was located downstream of a rearward-facing step. The freestream flow was nominally Mach 2 and was combustion heated to a total temperature of 1440 K (yielding a static temperature of about 800 K in the freestream) to simulate the inflow to a combustor operating at a flight Mach number of about 5.4. Since a broadband probe laser was used an instantaneous temperature sample was obtained with each laser shot at a repetition rate of 10 Hz. Thus root-mean-square (rms) temperatures and temperature probability density functions (pdf's) were obtained in addition to mean temperatures.

Smith, Michael W.↗

DOE OSTI2023

Linear Modelling from Betatron Phase Measurements at the Fermilab Recycler NOvA ring

Utilizing the measurement of coherent betatron oscillation phase has emerged as fast and precise approach for identifying and rectifying errors in implementing a desired lattice in CESR (Cornell Electron Storage Ring). One key advantage of betatron phase measurement over β measurement is its sensitivity to phase variations between widely separated points. This methodology has been successfully implemented for the Recycler NOvA Ring at Fermilab, with the adoption of TAO (Tool for Accelerator Optics) developed by Cornell University. By employing this technique, a linear model of the Recycler NOvA ring is established, enabling the correction of quadrupole errors.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS2018

Multibaseline TanDEM-X Mangrove Height Estimation: The Selection of the Vertical Wavenumber

We generated a large-scale mangrove forest height map using multiple TanDEM-X (TDX) interferometric synthetic aperture radar (InSAR) acquisitions with various spatial baselines in order to improve the height estimation accuracy across a wide range of forest heights. The forest height inversion using InSAR data is strongly dependent upon the vertical wavenumber (i.e., perpendicular baseline). First, we investigated the role of the vertical wavenumber in forest height inversion from InSAR data using the sensitivity of the interferometric (volume) coherence to forest height. We used corrected but lower resolution and accuracy Shuttle Radar Topography Mission (SRTM) mangrove height maps as a priori information over Akanda and Pongara National Parks in Gabon to estimate lower and upper boundaries of the vertical wavenumber over test sites from the measured coherence-to-height sensitivity. Only TDX acquisitions within the boundaries of the vertical wavenumber were selected and combined for multibaseline mangrove height inversion. Mangrove forest height was obtained with multibaseline TDX acquisitions and was validated against the reference height derived from field measurement data providing improvements in multibaseline inversion over existing height estimates (i.e., SRTM height) and single-baseline inversions (multibaseline inversion: r(exp 2) = 0.98, root mean square error (RMSE) of 2.73 m; SRTM height: r(exp 2) = 0.86, RMSE = 7.21 m; single-baseline inversions: r(exp 2) = 0.08-0.97, RMSE = 3.86-11.10 m). As a result, to accurately estimate forest heights over a wide range (3-60 m), multibaseline InSAR acquisitions (at least three different baselines) are needed to exclude biases associated with the vertical wavenumber in forest height inversion.

vertical wavenumber.↗