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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 181 records · Page 10
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Plasma surface ionization wave interactions with single channels

Abstract The study of plasma surface ionization waves (SIWs) in recent years has primarily focused on planar surfaces and periodic two dimensional structures. In application, substrates are likely to have non-planar morphology such as cracks, pores, and steps. Additionally, targets for the applications of medicine or catalysis may have targets with heterogeneous composition. This classification of targets are brought under the umbrella of complex interfaces. In this work, plasma SIWs were incident on a complex target consisting of a single channel cut into glass slides. The SIW velocities for the in-channel portion of the wave and radially propagating portion of the wave were tracked. It was found that surface wave velocities are not significantly affected by channel geometry, but primarily increase with pulse energy. A third propagation direction for the SIW is characterized in the azimuthal direction relative to the radial portion of the wave. Channel geometry is found to greatly effect the area treated by the plasma but not the propagation velocity of the surface wave. Surface wave morphology and the impact on application is also discussed. A simple model was introduced to understand the mechanisms behind SIW escape from a channel. It was found that the ratio of pulse energy to a geometry dependent minimum energy can predict the escape angle of a SIW from single channels.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Causality, intermittence, and crossphase evolution during confinement transitions in the TJ-II stellarator

In this work, we study spontaneous electron to ion root transitions in TJ-II using Langmuir probes. By scanning the probe position on a shot to shot basis, we reconstruct a spatiotemporal map of the evolution of important turbulent quantities in the plasma edge region. We pay particular attention to the evolution of the cross phase between transport-relevant variables, showing the spatiotemporal evolution of this quantity for the first time, revealing the outward propagation of the changes associated with the transition. Additionally, we also compute the intermittence parameter, which allows us to conclude that the turbulence, although its amplitude increases, condenses in a reduced number of dominant modes and becomes less bursty. The causal relationship between variables is studied using the transfer entropy, clarifying the interactions between the main variables and offering a rather complete picture of the complex evolution of the plasma across the confinement transition.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS2013

Uplift of Ionospheric Oxygen Ions During Extreme Magnetic Storms

Research reported earlier in literature was conducted relating to estimation of the ionospheric electrical field, which may have occurred during the September 1859 Carrington geomagnetic storm event, with regard to modern-day consequences. In this research, the NRL SAMI2 ionospheric code has been modified and applied the estimated electric field to the dayside ionosphere. The modeling was done at 15-minute time increments to track the general ionospheric changes. Although it has been known that magnetospheric electric fields get down into the ionosphere, it has been only in the last ten years that scientists have discovered that intense magnetic storm electric fields do also. On the dayside, these dawn-to-dusk directed electric fields lift the plasma (electrons and ions) up to higher altitudes and latitudes. As plasma is removed from lower altitudes, solar UV creates new plasma, so the total plasma in the ionosphere is increased several-fold. Thus, this complex process creates super-dense plasmas at high altitudes (from 700 to 1,000 km and higher).

Tsurutani, Bruce T.↗
DOE OSTI2021

From thermal catalysis to plasma catalysis: a review of surface processes and their characterizations

The use of atmospheric pressure plasma to enhance catalytic chemical reactions involves complex surface processes induced by the interactions of plasma-generated fluxes with catalyst surfaces. Industrial implementation of plasma catalysis necessitates optimizing the design and realization of plasma catalytic reactors that enable chemical reactions that are superior to conventional thermal catalysis approaches. This requires the fundamental understanding of essential plasma-surface interaction mechanisms of plasma catalysis from the aspect of experimental investigation and theoretical analysis or computational modeling. In addition, experimental results are essential to validate the relative theoretical models and hypotheses of plasma catalysis that was rarely understood so far, compared to conventional thermal catalysis. This overview focuses on two important application areas, nitrogen fixation and methane reforming, and presents a comparison of important aspects of the state of knowledge of these applications when performed using either plasma-catalysis or conventional thermal catalysis. We discuss the potential advantage of plasma catalysis over thermal catalysis from the aspects of plasma induced synergistic effect and in situ catalyst regeneration. In-situ/operando surface characterization of catalysts in plasma catalytic reactors is a significant challenge since the high pressure of realistic plasma catalysis systems preclude the application of many standard surface characterization techniques that operate in a low-pressure environment. Here, we present a review of the status of experimental approaches to probe gas-surface interaction mechanisms of plasma catalysis, including an appraisal of demonstrated approaches for integrating surface diagnostic tools into plasma catalytic reactors.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Fractional Laplacian spectral approach to turbulence in a dusty plasma monolayer

This work presents an analytical investigation of anomalous diffusion and turbulence in a dusty plasma monolayer, where energy transport across scales leads to the spontaneous formation of spatially disordered patterns. Many-body simulations of 10,000-particle dusty plasma monolayers are used to demonstrate how the global dynamics depend on the statistical properties of the dust assembly for realistic laboratory conditions. We find that disorder due to variations in the dust size distribution and charge-driven nonlocal interactions resulting in anomalous dust diffusion are key factors for the onset of instabilities. The resulting dynamics exhibit features of inertial turbulence over slightly more than half a decade of scales proportional or smaller than the Debye shielding length. These processes are examined analytically using a recently developed Fractional Laplacian Spectral (FLS) technique, which identifies the active energy channels as a function of scale, disorder concentration, and features of the nonlocal-interactions. The predictions from the theoretical (spectral) analysis demonstrate agreement with the results from the many-body (kinetic) simulations, thus providing a powerful tool for the study of active turbulence.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2026

Partially Ionized Plasma Physics and Technological Applications

Partially ionized plasma physics has attracted increased attention recently due to numerous technological applications made possible by the increased sophistication of computer modelling, the depth of the theoretical analysis, and the technological applications to a vast field of manufacturing for computer components. Partially ionized plasma is characterized by a significant presence of neutral particles in contrast to the fully ionized plasma. The theoretical analysis is based upon solutions of the kinetic Boltzmann equation, yielding the non-Maxwellian electron energy distribution function (EEDF), thereby emphasizing the difference with a fully ionized plasma. The impact of the effect on discharges in inert and molecular gases is described in detail, yielding the complex nonlinear phenomena resulting in plasma selforganization. A few examples of such phenomena are given, including the non-monotonic EEDFs in the discharge afterglow in a mixture of argon with the molecular gas NF3; the explosive generation of cold electron populations in capacitive discharges, hysteresis of EEDF in inductively coupled plasmas. Recently, highly advanced computer codes were developed in order to address the outstanding challenges in plasma technology. These developments are briefly described in general terms.

non-Maxwellian electron energy distribution functi↗
DOE OSTI2020

High-resolution X-ray spectroscopy of the stellar wind in Vela X-1 during a flare

In this work, we present a ~130 ks observation of the prototypical wind-accreting, high-mass X-ray binary Vela X-1 collected with XMM-Newton at orbital phases between 0.12 and 0.28. A strong flare took place during the observation that allows us to investigate the reaction of the clumpy stellar wind to the increased X-ray irradiation. To examine the wind’s reaction to the flare, we performed both time-averaged and time-resolved analyses of the RGS spectrum and examined potential spectral changes. We focused on the high-resolution XMM-Newton RGS spectra and divided the observation into pre-flare, flare, and post-flare phases. We modeled the time-averaged and time-resolved spectra with phenomenological components and with the self-consistent photoionization models calculated via CLOUDY and XSTAR in the pre-flare phase, where strong emission lines due to resonant transitions of highly ionized ions are seen. In the spectra, we find emission lines corresponding to K-shell transitions in highly charged ions of oxygen, neon, magnesium, and silicon as well as radiative recombination continua (RRC) of oxygen. Additionally, we observe potential absorption lines of magnesium at a lower ionization stage and features identified as iron L lines. The, CLOUDY and XSTAR photoionization models provide contradictory results, either pointing towards uncertainties in theory or possibly a more complex multi-phase plasma, or both. We are able to demonstrate the existence of a plethora of variable narrow features, including the firm detection of oxygen lines and RRC that RGS enables to observe in this source for the first time. We show that Vela X-1 is an ideal source for future high-resolution missions, such as XRISM and Athena.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

Brewster angle-cavity ringdown spectroscopy for low temperature plasma measurements in multiphases

Here we report on the development of a Brewster angle-cavity ringdown spectroscopy (BA-CRDS) system for low temperature plasma diagnostics. The system can measure gas species in solutions, with a detection limit (minimum detectable absorbance) of 9.1 × 10 -5 , which is equivalent to a detection limit of 0.04 parts per billion for measuring OH radicals in water at 308 nm. With higher reflectivity ringdown mirrors and improved design of a Brewster angle cell, the detection limit can potentially be up to 10 -6 or lower. In this exploratory study, the absorption cross sections of HgBr 2 and H 2 O 2 in the aqueous phase at 256 nm are measured to be (1.8 ± 0.1) × 10 -18 cm 2 and (5.2 ± 0.5) × 10 -20 cm 2 , respectively. Furthermore, temporal profiles of absorbance from distilled water, HgBr 2 , and H 2 O 2 solutions when interacting with a helium atmospheric plasma jet are individually characterized at different plasma powers, gas flow rates, and/or solute concentrations. The observed linear temporal profiles of absorbance from the plasma-interacted water suggest formation of H 2 O 2 from plasma-generated OH radicals, while the nonlinear temporal profiles from the plasma-treated HgBr 2 solutions reveal possible removal of HgBr 2 by OH radicals. Our results demonstrate that the new BA-CRDS system is a powerful tool for quantification of reactive plasma species in multiphases or other complex settings.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Model predictive control of KSTAR equilibrium parameters enabled by TRANSP

Due to the complex behavior of tokamak plasmas and the importance of optimizing performance while avoiding instabilities and machine limits, plasma control algorithms are becoming increasingly dependent on sophisticated model-based control approaches. It is anticipated that the use of integrated modeling codes in the model-based control design process will reduce the amount of experimental time needed to implement new control algorithms by facilitating development of control-oriented models and enabling higher-fidelity closed-loop simulations. In this work, a reduced model is developed from a series of TRANSP simulations and is used to develop a model predictive control (MPC) algorithm for controlling important equilibrium parameters in KSTAR [1] discharges. The control algorithm uses the KSTAR neutral beam injection system and the target plasma current and plasma boundary as actuators, and optimizes the plasma stored energy, loop voltage, and internal inductance while avoiding constraints that could lead to disruptions. Higher fidelity testing of the control algorithm is performed using a flexible framework for enabling external processes to actively control plasma parameters in TRANSP simulations. Furthermore, closed-loop simulations demonstrate the ability of the control algorithm to respond to disturbances in density and confinement, handle actuator failures, and move the discharge to high non-inductive fraction conditions.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Time-resolved tracking of cellulose biosynthesis and assembly during cell wall regeneration in live Arabidopsis protoplasts

Cellulose, the most abundant polysaccharide on earth composing plant cell walls, is synthesized by coordinated action of multiple enzymes in cellulose synthase complexes embedded within the plasma membrane. Multiple chains of cellulose fibrils form intertwined extracellular matrix networks. It remains largely unknown how newly synthesized cellulose is assembled into an intricate fibril network on cell surfaces. Here, we have established an in vivo time-resolved imaging platform to continuously visualize cellulose biosynthesis and fibril network assembly onArabidopsis thalianaprotoplast surfaces as the primary cell wall regenerates. Our observations provide the basis for a model of cellulose fibril network development in protoplasts driven by an interplay of multiscale dynamics that includes rapid diffusion and coalescence of nascent cellulose fibrils, processive elongation of single fibrils, and cellulose fibrillar network rearrangement during maturation. This study provides fresh insights into the dynamic and mechanistic aspects of cell wall synthesis at the single-cell level.

Science & Technology - Other Topics↗
DOE OSTI2023

Species mix & distribution function dependence of energetic-ion driven magnetospheric instabilities on DIII-D (Final Report)

Energetic ions drive a rich variety of instabilities in the complex multi-species plasma of Earth’s magnetosphere. This experiment exploited the highly flexible, high power particle beam injection capability and sophisticated diagnostic suite of the DIII-D tokamak to advance understanding of two particular instabilities of significant interest to the magnetospheric research community that have closely-related counterparts in beam-heated tokamak plasmas: electromagnetic ion cyclotron waves (EMIC) [1], observed at frequencies somewhat below the ion cyclotron frequencies of bulk ion species, and equatorial noise [2], observed at energetic-ion cyclotron harmonics. In the magnetic fusion energy domain, such waves are called ICE (Ion Cyclotron Emission). Recent substantial advances in diagnostic capability in the ion cyclotron range of frequencies in DIII-D, including measurement of wave polarization, spa)al structure and amplitude created an exciting opportunity to challenge and drive advances in theoretical understanding of these phenomena.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

ezAlign: A Tool for Converting Coarse-Grained Molecular Dynamics Structures to Atomistic Resolution for Multiscale Modeling

Soft condensed matter is challenging to study due to the vast time and length scales that are necessary to accurately represent complex systems and capture their underlying physics. Multiscale simulations are necessary to study processes that have disparate time and/or length scales, which abound throughout biology and other complex systems. Herein we present ezAlign, an open-source software for converting coarse-grained molecular dynamics structures to atomistic representation, allowing multiscale modeling of biomolecular systems. The ezAlign v1.1 software package is publicly available for download at github.com/LLNL/ezAlign. Its underlying methodology is based on a simple alignment of an atomistic template molecule, followed by position-restraint energy minimization, which forces the atomistic molecule to adopt a conformation consistent with the coarse-grained molecule. The molecules are then combined, solvated, minimized, and equilibrated with position restraints. Validation of the process was conducted on a pure POPC membrane and compared with other popular methods to construct atomistic membranes. Additional examples, including surfactant self-assembly, membrane proteins, and more complex bacterial and human plasma membrane models, are also presented. By providing these examples, parameter files, code, and an easy-to-follow recipe to add new molecules, this work will aid future multiscale modeling efforts.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS1994

Pickup protons and pressure-balanced structures: Voyager 2 observations in merged interaction regions near 35 AU

Five pressure-balanced structures, each with a scale of the order of a few hundredths of an astonomical unit (AU), were identified in two merged interaction regions (MIRs) near 35 AU in the Voyager 2 plasma and magnetic field data. They include a tangential discountinuity, simple and complex magnetic holes, slow correlated variations among the plasma and magnetic field parameters, and complex uncorrelated variations among the parameters. The changes in the magnetic pressure in these events are balanced by changes in the pressure of interstellar pickup protons. Thus the pickup protons probably play a major role in the dynamics of the MIRs. The solar wind proton and electron pressures are relatively unimportant in the MIRs at 35 AU and beyond. The region near 35 AU is transition region: the Sun is the source of the magnetic field, but the interstellar medium in source of pickups protons. Relative to the solar wind proton guyroadius, the thicknesses of the discontinuities and simple magnetic holes observed near 35 AU are at least an order of magnitude greater than those observed at 1 AU. However, the thicknesses of the tangential discontinuity and simple magnetic holes observed near 35 AU (in units of the pickup proton Larmor radius) are comparable to those observed at 1 AU (in units of the solar wind proton gyroradius). Thus the gyroradius of interstellar pickup protons controls the thickness of current sheets near 35 AU. We determine the interstellar pickup proton pressure in the PBSs. Using a model for the pickup proton temperature, we estimate that the average interstellar pickup proton pressure, temperature, and density in the MIRs at 35 AU are (0.53 +/- 0.14) x 10(exp -12) erg/cu cm, (5.8 +/- 0.4) x 10(exp 6) K and (7 +/- 2) x 10(exp -4)/cu cm.

Burlaga, L. F.↗
NASA NTRS2022

Direct Observations of a Complex Coronal Web Driving Highly Structured Slow Solar Wind

The solar wind is formed by continuous streams of charged particles that escape into the heliosphere from the Sun. Fast wind with speeds more than 500 km s -1 emerges from the interiors of coronal holes. Near the ecliptic plane, fast wind from low-latitude coronal holes is interspersed with a highly structured slow solar wind. The source regions and drivers of this slow wind are poorly understood. Here we report observations from an off-point campaign of the GOES Solar Ultraviolet Imager that reveal a spatially complex web of magnetized plasma structures, over a low-latitude coronal hole active region system, that persistently interact and reconnect in the middle corona. SOHO coronagraphic images show concurrent emergence of slow wind streams over these coronal web structures. With advanced global MHD coronal models, we demonstrate that the observed coronal web is a direct imprint of the magnetic separatrix web (S-web). By revealing a highly dynamic portion of S-web, our observations open a window into important middle coronal processes that appear to play key role in driving structured slow solar wind.

Solar physics↗
DOE OSTI2024

Direct HCN synthesis via plasma-assisted conversion of methane and nitrogen

Hydrogen cyanide (HCN) is synthesized from ammonia (NH 3 ) and methane (CH 4 ) at ~1200°C over a Pt catalyst. Ammonia synthesis entails several complex, highly emitting processes. Plasma-assisted HCN synthesis directly from CH 4 and nitrogen (N 2 ) could be pivotal for on-demand HCN production. Here, we evaluate the potential of dielectric barrier discharge (DBD) N 2 /CH 4 plasma for decentralized catalyst-free selective HCN production. We demonstrate a single-step conversion of methane and nitrogen to HCN with a 72% yield at <300°C. HCN is favored at low CH 4 concentrations with ethane (C 2 H 6 ) as the secondary product. We propose a first-principles microkinetic model with few electron impact reactions. The model accurately predicts primary product yields and elucidates that methyl radical (·CH 3 ) is a common intermediate in HCN and C 2 H 6 synthesis. Compared to current industrial processes, N 2 /CH 4 DBD plasma can achieve minimal CO 2 emissions.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1998

Spatial Distribution of Ionospheric Plasma and Field Structures in the High-Latitude F Region

Ion density and velocity measurements from the Dynamics Explorer 2 (DE 2) spacecraft are used to obtain the average magnetic local time versus invariant latitude distribution of irregularities in the high-latitude F region ionosphere. To study the small-scale structure and its relationship to background conditions in the ionosphere, we have formed a reduced database using 2-s (approx. = 16 km) segments of the ion density and velocity data. The background gradients associated with each 2-s segment and the spectral characteristics, such as power at 6 Hz (approx. = 1.3 km) and spectral index, are among the reduced parameters used in this study. The relationship between the observed plasma structure and its motion is complex and dependent on the externally applied fields as well as locally generated plasma structure. The evolution of plasma structures also depends critically on the conductivity of the underlying ionosphere. Observations indicate an enhancement of irregularity amplitudes in two spatially isolated regions in both the ion density and the velocity. Convective properties seem to play a more important role in winter hemisphere where smaller-scale structures are maintained outside the source regions. (Delta)V irregularity amplitudes are enhanced in the cusp and the polar cap during northward interplanetary magnetic field regardless of season. The power in (Delta)V is usually higher than that associated with local polarization electric fields, suggesting that the observed structure in (Delta)N/N is strongly influenced by (Delta)V structure applied to large density gradients.

Kivanc, O.↗
NASA NTRS1995

A Fully Integrated Micro-Magnometer/Microspacecraft for Multipoint Measurements: The Free-Flyer Magnometer

In the decades since the advent of in situ plasma measurements on board spacecraft, the instrumentation has grown bigger, heavier, and more complex as our understanding of space plasmas improves and our appetite for more information increases...There has thus been a recent interest in the miniaturization of both spacecraft and the instrument payload... This paper describes the results and status of an ongoing design study to understand the problems and trade space of fully integrating an instrument into a micro-spacecraft.

plasma plasma measurement space plasma↗
DOE OSTI2024

The magnetic gradient scale length explains why certain plasmas require close external magnetic coils

Abstract The separation between the last closed flux surface of a plasma and the external coils that magnetically confine it is a limiting factor in the construction of fusion-capable plasma devices. This plasma-coil separation must be large enough so that components such as a breeding blanket and neutron shielding can fit between the plasma and the coils. Plasma-coil separation affects reactor size, engineering complexity, and particle loss due to field ripple. For some plasmas it can be difficult to produce the desired flux surface shaping with distant coils, and for other plasmas it is infeasible altogether. Here, we seek to understand the underlying physics that limits plasma-coil separation and explain why some configurations require close external coils. In this paper, we explore the hypothesis that the limiting plasma-coil separation is set by the shortest scale length of the magnetic field as expressed by the ∇ B tensor. We tested this hypothesis on a database of > 40 stellarator and tokamak configurations. Within this database, the coil-to-plasma distance compared to the minor radius varies by over an order of magnitude. The magnetic scale length is well correlated to the coil-to-plasma distance of actual coil designs generated using the REGCOIL method (Landreman 2017 Nucl. Fusion 57 046003). Additionally, this correlation reveals a general trend that larger plasma-coil separation is possible with a small number of field periods.

Physics↗