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At least 181 records · Page 10

On the Reconstruction of Palaeo-Ice Sheets: Recent Advances and Future Challenges

Reconstructing the growth and decay of palaeo-ice sheets is critical to understanding mechanisms of global climate change and associated sea-level fluctuations in the past, present and future. The significance of palaeo-ice sheets is further underlined by the broad range of disciplines concerned with reconstructing their behaviour, many of which have undergone a rapid expansion since the 1980s. In particular, there has been a major increase in the size and qualitative diversity of empirical data used to reconstruct and date ice sheets, and major improvements in our ability to simulate their dynamics in numerical ice sheet models. These developments have made it increasingly necessary to forge interdisciplinary links between sub-disciplines and to link numerical modelling with observations and dating of proxy records. The aim of this paper is to evaluate recent developments in the methods used to reconstruct ice sheets and outline some key challenges that remain, with an emphasis on how future work might integrate terrestrial and marine evidence together with numerical modelling. Our focus is on pan-ice sheet reconstructions of the last deglaciation, but regional case studies are used to illustrate methodological achievements, challenges and opportunities. Whilst various disciplines have made important progress in our understanding of ice-sheet dynamics, it is clear that data-model integration remains under-used, and that uncertainties remain poorly quantified in both empirically-based and numerical ice-sheet reconstructions. The representation of past climate will continue to be the largest source of uncertainty for numerical modelling. As such, palaeo-observations are critical to constrain and validate modelling. State-of-the-art numerical models will continue to improve both in model resolution and in the breadth of inclusion of relevant processes, thereby enabling more accurate and more direct comparison with the increasing range of palaeo-observations. Thus, the capability is developing to use all relevant palaeo-records to more strongly constrain deglacial (and to a lesser extent pre-LGM) ice sheet evolution. In working towards that goal, the accurate representation of uncertainties is required for both constraint data and model outputs. Close cooperation between modelling and data-gathering communities is essential to ensure this capability is realised and continues to progress.

Ice sheet reconstruction↗

Confronting the water potential information gap

Water potential directly controls the function of leaves, roots and microbes, and gradients in water potential drive water flows throughout the soil–plant–atmosphere continuum. Notwithstanding its clear relevance for many ecosystem processes, soil water potential is rarely measured in situ, and plant water potential observations are generally discrete, sparse, and not yet aggregated into accessible databases. These gaps limit our conceptual understanding of biophysical responses to moisture stress and inject large uncertainty into hydrologic and land-surface models. Here, we outline the conceptual and predictive gains that could be made with more continuous and discoverable observations of water potential in soils and plants. We discuss improvements to sensor technologies that facilitate in situ characterization of water potential, as well as strategies for building new networks that aggregate water potential data across sites. Here, we end by highlighting novel opportunities for linking more representative site-level observations of water potential to remotely sensed proxies. Together, these considerations offer a road map for clearer links between ecohydrological processes and the water potential gradients that have the ‘potential’ to substantially reduce conceptual and modelling uncertainties.

58 GEOSCIENCES↗

Solar measurements from the Airglow-Solar Spectrometer Instrument (ASSI) on the San Marco 5 satellite

The analysis of the solar spectral irradiance from the Airglow-Solar Spectrometer Instrument (ASSI) on the San Marco 5 satellite is the focus for this research grant. A pre-print copy of the paper describing the calibrations of and results from the San Marco ASSI is attached to this report. The calibration of the ASSI included (1) transfer of photometric calibration from a rocket experiment and the Solar Mesosphere Explorer (SME), (2) use of the on-board radioactive calibration sources, (3) validation of the ASSI sensitivity over its field of view, and (4) determining the degradation of the spectrometers. We have determined that the absolute values for the solar irradiance needs adjustment in the current proxy models of the solar UV irradiance, and the amount of solar variability from the proxy models are in reasonable agreement with the ASSI measurements. This research grant also has supported the development of a new solar EUV irradiance proxy model. We expected that the magnetic flux is responsible for most of the heating, via Alfen waves, in the chromosphere, transition region, and corona. From examining time series of solar irradiance data and magnetic fields at different levels, we did indeed find that the chromospheric emissions correlate best with the large magnetic field levels.

Woods, Thomas N.↗

CHARGED-CURRENT DOUBLE-DIFFERENTIAL CROSS SECTION MEASUREMENT OF ELECTRON NEUTRINOS IN LOW RECOIL REGION ON HYDROCARBON AT ∼7 GEV

Measuring neutrino mixing angles, especially the CP violation phase and mass hierarchy, is one of the priorities of the neutrino community and long baseline neutrino oscillation programs, such as T2K and NOvA, provided the most precise measurements to date. One of the dominating uncertainties of the measurements is the neutrino interaction model due to the difficulty of modeling the nuclear effects from first principles. As a result, neutrino scattering experiments such as MINERvA were conducted to provide data as input to reduce this uncertainty. This thesis presents a charged-current double-differential cross section measurement of electron neutrinos using the MINERvA detector in terms of available energy (a proxy of energy transfer), three-momentum transfer, and/or transverse momentum of the final state electron. This measurement focuses on the transition region between quasi-elastic and resonance processes, where the multi-nucleon knockout process dominates. The result is compared to a modified GENIE model and similar measurements using muon neutrino samples. In addition, this measurement reproduces the photon-like excess seen by previous MINERvA electron neutrino measurements.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Use of High-Resolution WRF Simulations to Forecast Lightning Threat

Recent observational studies have confirmed the existence of a robust statistical relationship between lightning flash rates and the amount of large precipitating ice hydrometeors aloft in storms. This relationship is exploited, in conjunction with the capabilities of cloud-resolving forecast models such as WRF, to forecast explicitly the threat of lightning from convective storms using selected output fields from the model forecasts. The simulated vertical flux of graupel at -15C and the shape of the simulated reflectivity profile are tested in this study as proxies for charge separation processes and their associated lightning risk. Our lightning forecast method differs from others in that it is entirely based on high-resolution simulation output, without reliance on any climatological data. short [6-8 h) simulations are conducted for a number of case studies for which three-dmmensional lightning validation data from the North Alabama Lightning Mapping Array are available. Experiments indicate that initialization of the WRF model on a 2 km grid using Eta boundary conditions, Doppler radar radial velocity fields, and METAR and ACARS data y&eld satisfactory simulations. __nalyses of the lightning threat fields suggests that both the graupel flux and reflectivity profile approaches, when properly calibrated, can yield reasonable lightning threat forecasts, although an ensemble approach is probably desirable in order to reduce the tendency for misplacement of modeled storms to hurt the accuracy of the forecasts. Our lightning threat forecasts are also compared to other more traditional means of forecasting thunderstorms, such as those based on inspection of the convective available potential energy field.

McCaul, E. W., Jr.↗

Usefulness of AIRS-Derived OLR, Temperature, Water Vapor and Cloudiness Anomaly Trends for GCM Validation

Mainly due to their global nature, satellite observations can provide a very useful basis for GCM validations. In particular, satellite sounders such as AIRS provide 3-D spatial information (most useful for GCMs), so the question arises: can we use AIRS datasets for climate variability assessments? We show that the recent (September 2002 February 2010) CERES-observed negative trend in OLR of approx.-0.1 W/sq m/yr averaged over the globe is found in the AIRS OLR data as well. Most importantly, even minute details (down to 1 x 1 degree GCM-scale resolution) of spatial and temporal anomalies and trends of OLR as observed by CERES and computed based on AIRS-retrieved surface and atmospheric geophysical parameters over this time period are essentially the same. The correspondence can be seen even in the very large spatial variations of these trends with local values ranging from -2.6 W/sq m/yr to +3.0 W/sq m/yr in the tropics, for example. This essentially perfect agreement of OLR anomalies and trends derived from observations by two different instruments, in totally independent and different manners, implies that both sets of results must be highly accurate, and indirectly validates the anomalies and trends of other AIRS derived products as well. These products show that global and regional anomalies and trends of OLR, water vapor and cloud cover over the last 7+ years are strongly influenced by EI-Nino-La Nina cycles . We have created climate parameter anomaly datasets using AIRS retrievals which can be compared directly with coupled GCM climate variability assessments. Moreover, interrelationships of these anomalies and trends should also be similar between the observed and GCM-generated datasets, and, in cases of discrepancies, GCM parameterizations could be improved based on the relationships observed in the data. First, we assess spatial "trends" of variability of climatic parameter anomalies [since anomalies relative to the seasonal cycle are good proxies of climate variability] at the common 1x1 degree GCM grid-scale by creating spatial anomaly "trends" based on the first 7+ years of AIRS Version 5 Leve13 data. We suggest that modelers should compare these with their (coupled) GCM's performance covering the same period. We evaluate temporal variability and interrelations of climatic anomalies on global to regional e.g., deep Tropical Hovmoller diagrams, El-Nino-related variability scales, and show the effects of El-Nino-La Nina activity on tropical anomalies and trends of water vapor cloud cover and OLR. For GCMs to be trusted highly for long-term climate change predictions, they should be able to reproduce findings similar to these. In summary, the AIRS-based climate variability analyses provide high quality, informative and physically plausible interrelationships among OLR, temperature, humidity and cloud cover both on the spatial and temporal scales. GCM validations can use these results even directly, e. g., by creating 1x1 degree trendmaps for the same period in coupled climate simulations.

Molnar, Gyula I.↗

The Goes-R Geostationary Lightning Mapper (GLM): Algorithm and Instrument Status

The Geostationary Operational Environmental Satellite (GOES-R) is the next series to follow the existing GOES system currently operating over the Western Hemisphere. Superior spacecraft and instrument technology will support expanded detection of environmental phenomena, resulting in more timely and accurate forecasts and warnings. Advancements over current GOES capabilities include a new capability for total lightning detection (cloud and cloud-to-ground flashes) from the Geostationary Lightning Mapper (GLM), and improved capability for the Advanced Baseline Imager (ABI). The Geostationary Lighting Mapper (GLM) will map total lightning activity (in-cloud and cloud-to-ground lighting flashes) continuously day and night with near-uniform spatial resolution of 8 km with a product refresh rate of less than 20 sec over the Americas and adjacent oceanic regions. This will aid in forecasting severe storms and tornado activity, and convective weather impacts on aviation safety and efficiency. In parallel with the instrument development (a prototype and 4 flight models), a GOES-R Risk Reduction Team and Algorithm Working Group Lightning Applications Team have begun to develop the Level 2 algorithms, cal/val performance monitoring tools, and new applications. Proxy total lightning data from the NASA Lightning Imaging Sensor on the Tropical Rainfall Measuring Mission (TRMM) satellite and regional test beds are being used to develop the pre-launch algorithms and applications, and also improve our knowledge of thunderstorm initiation and evolution. A joint field campaign with Brazilian researchers in 2010-2011 will produce concurrent observations from a VHF lightning mapping array, Meteosat multi-band imagery, Tropical Rainfall Measuring Mission (TRMM) Lightning Imaging Sensor (LIS) overpasses, and related ground and in-situ lightning and meteorological measurements in the vicinity of Sao Paulo. These data will provide a new comprehensive proxy data set for algorithm and application development.

Goodman, Steven J.↗

The GOES-R Series Geostationary Lightning Mapper (GLM)

The Geostationary Operational Environmental Satellite (GOES-R) is the next series to follow the existing GOES system currently operating over the Western Hemisphere. Superior spacecraft and instrument technology will support expanded detection of environmental phenomena, resulting in more timely and accurate forecasts and warnings. Advancements over current GOES capabilities include a new capability for total lightning detection (cloud and cloud-to-ground flashes) from the Geostationary Lightning Mapper (GLM), which will have just completed Critical Design Review and move forward into the construction phase of instrument development. The GLM will operate continuously day and night with near-uniform spatial resolution of 8 km with a product refresh rate of less than 20 sec over the Americas and adjacent oceanic regions. This will aid in forecasting severe storms and tornado activity, and convective weather impacts on aviation safety and efficiency. In parallel with the instrument development (an engineering development unit and 4 flight models), a GOES-R Risk Reduction Team and Algorithm Working Group Lightning Applications Team have begun to develop the Level 2 algorithms, cal/val performance monitoring tools, and new applications. Proxy total lightning data from the NASA Lightning Imaging Sensor (LIS) on the Tropical Rainfall Measuring Mission (TRMM) satellite and regional ground-based lightning networks are being used to develop the pre-launch algorithms, test data sets, and applications, as well as improve our knowledge of thunderstorm initiation and evolution. In this presentation we review the planned implementation of the instrument and suite of operational algorithms

Goodman, Steven J.↗

Improved Assessment of Recent Trends in NOx and VOC Emissions and Ozone Production Sensitivity Regimes Using Satellite Data

This presentation highlights results from a NASA Aura Science Team and Atmospheric Composition Modeling and Analysis Program (ACMAP) project which study the capability to observe and model trends in ozone (O3) production regimes using spaceborne sensors. Ultraviolet– visible (UV–Vis) tropospheric column satellite retrievals of formaldehyde (HCHO) (a proxy for volatile organic compound [VOC] reactivity) and nitrogen dioxide (NO2) (a proxy for nitrogen oxides [NOx]) are frequently used to investigate the sensitivity of O3 production to emissions of NOx and VOCs. There are challenges that come from using satellite-derived ratios of HCHO and NO2 (FNR) to study O3 production sensitivity with the largest uncertainties associated with specific spaceborne sensor’s retrieval biases and errors. This study quantifies the differences and improvements in satellite retrievals of O3 production sensitivity regimes using FNRs when moving from legacy polar orbiting satellites such as the Ozone Monitoring Instrument (OMI) onboard NASA’s Aura satellite and Ozone Mapping and Profiler Suite Nadir Mapper (OMPS-NM) onboard the NASA/NOAA Suomi-NPP platform to newer, higher spatiotemporal resolution satellite sensors TROPOspheric Monitoring Instrument (TROPOMI) and eventually the recently launched NASA geostationary sensor Tropospheric Emissions: Monitoring of Pollution (TEMPO). Furthermore, we investigate how using retrievals of NO2 and HCHO from these different satellites to constrain model predictions impacts the ability to accurately simulate O3 chemistry including chemical production regimes. To this end, we have conducted inverse model simulations, using the WRF-CMAQ-DDM data assimilation system at 12 km × 12 km, to constrain emissions of NOx and VOCs over the contiguous United States (CONUS) when assimilating OMI and TROPOMI retrievals of NO2 and HCHO. Two advantages of this are that we a) account for each satellite’s errors/biases in the emission estimation and b) update the prior profile to ensure that only radiance information is used for optimizing the emissions. This presentation will demonstrate: a) the varying accuracy of different satellite retrieved FNRs and ability to capture known sub-annual emission trends (e.g., seasonal, weekend/weekday) and emission anomalies during the COVID-19 lockdown of 2020, b) the differences and improvements in top-down emission estimates of NOx and VOCs when constrained by newer satellite sensors compared to legacy systems, and c) multi-sensor optimized emission estimates of summer-time NOx and VOCs between 2019-2021.

Data↗

Learning perturbation-inducible cell states from observability analysis of transcriptome dynamics

Abstract A major challenge in biotechnology and biomanufacturing is the identification of a set of biomarkers for perturbations and metabolites of interest. Here, we develop a data-driven, transcriptome-wide approach to rank perturbation-inducible genes from time-series RNA sequencing data for the discovery of analyte-responsive promoters. This provides a set of biomarkers that act as a proxy for the transcriptional state referred to as cell state. We construct low-dimensional models of gene expression dynamics and rank genes by their ability to capture the perturbation-specific cell state using a novel observability analysis. Using this ranking, we extract 15 analyte-responsive promoters for the organophosphate malathion in the underutilized host organism Pseudomonas fluorescens SBW25. We develop synthetic genetic reporters from each analyte-responsive promoter and characterize their response to malathion. Furthermore, we enhance malathion reporting through the aggregation of the response of individual reporters with a synthetic consortium approach, and we exemplify the library’s ability to be useful outside the lab by detecting malathion in the environment. The engineered host cell, a living malathion sensor, can be optimized for use in environmental diagnostics while the developed machine learning tool can be applied to discover perturbation-inducible gene expression systems in the compendium of host organisms.

59 BASIC BIOLOGICAL SCIENCES↗

Sources, Sinks, and Transatlantic Transport of North African Dust Aerosol: A Multimodel Analysis and Comparison With Remote Sensing Data

This study evaluates model-simulated dust aerosols over North Africa and the North Atlantic from five global models that participated in the Aerosol Comparison between Observations and Models phase II model experiments. The model results are compared with satellite aerosol optical depth (AOD) data from Moderate Resolution Imaging Spectroradiometer (MODIS), Multiangle Imaging Spectroradiometer (MISR), and Sea-viewing Wide Field-of-view Sensor, dust optical depth (DOD) derived from MODIS and MISR, AOD and coarse-mode AOD (as a proxy of DOD) from ground-based Aerosol Robotic Network Sun photometer measurements, and dust vertical distributions/centroid height from Cloud Aerosol Lidar with Orthogonal Polarization and Atmospheric Infrared Sounder satellite AOD retrievals. We examine the following quantities of AOD and DOD: (1) the magnitudes over land and over ocean in our study domain, (2) the longitudinal gradient from the dust source region over North Africa to the western North Atlantic, (3) seasonal variations at different locations, and (4) the dust vertical profile shape and the AOD centroid height (altitude above or below which half of the AOD is located). The different satellite data show consistent features in most of these aspects; however, the models display large diversity in all of them, with significant differences among the models and between models and observations. By examining dust emission, removal, and mass extinction efficiency in the five models, we also find remarkable differences among the models that all contribute to the discrepancies of model-simulated dust amount and distribution. This study highlights the challenges in simulating the dust physical and optical processes, even in the best known dust environment, and stresses the need for observable quantities to constrain the model processes.

Africa↗

SPoRT's Participation in the GOES-R Proving Ground Activity

The next generation geostationary satellite, GOES-R, will carry two new instruments with unique atmospheric and surface observing capabilities, the Advanced Baseline Imager (ABI) and the Geostationary Lightning Mapper (GLM), to study short-term weather processes. The ABI will bring enhanced multispectral observing capabilities with frequent refresh rates for regional and full disk coverage to geostationary orbit to address many existing and new forecast challenges. The GLM will, for the first time, provide the continuous monitoring of total lightning flashes over a hemispherical region from space. NOAA established the GOES-R Proving Ground activity several years ago to demonstrate the new capabilities of these instruments and to prepare forecasters for their day one use. Proving Ground partners work closely with algorithm developers and the end user community to develop and transition proxy data sets representing GOES-R observing capabilities. This close collaboration helps to maximize refine algorithms leading to the delivery of a product that effectively address a forecast challenge. The NASA Short-term Prediction Research and Transition (SPoRT) program has been a participant in the NOAA GOES-R Proving Ground activity by developing and disseminating selected GOES-R proxy products to collaborating WFOs and National Centers. Established in 2002 to demonstrate the weather and forecasting application of real-time EOS measurements, the SPoRT program has grown to be an end-to-end research to operations activity focused on the use of advanced NASA modeling and data assimilation approaches, nowcasting techniques, and unique high-resolution multispectral data from EOS satellites to improve short-term weather forecasts on a regional and local scale. Participation in the Proving Ground activities extends SPoRT s activities and taps its experience and expertise in diagnostic weather analysis, short-term weather forecasting, and the transition of research and experimental data to operational decision support systems like NAWIPS, AWIPS, AWIPS2, and Google Earth. Recent SPoRT Proving Ground activities supporting the development and use of a pseudo GLM total lightning product and the transition of the AWG s Convective Initiation (CI) product, both of which were available in AWIPS and AWIPS II environments, by forecasters during the Hazardous Weather Testbed (HWT) Spring Experiment. SPoRT is also providing a suite of SEVIRI and MODIS RGB image products, and a high resolution composite SST product to several National Centers for use in there ongoing demonstration activities. Additionally, SPoRT has involved numerous WFOs in the evaluation of a GOES-MODIS hybrid product which brings ABI-like data sets in front of the forecaster for everyday use. An overview of this activity will be presented at the conference.

Jedlovec, Gary↗

Development of lean, efficient, and fast physics-framed deep-learning-based proxy models for subsurface carbon storage

In this work, we present deep-learning-based surrogate models for CCUS developed with four different algorithms and a physics-framed two-phase flow problem involving displacement of water by CO 2 . The deep-learning models were trained using 3D datasets describing the pressure plume, CO 2 saturation plume, and water extraction rate generated by numerical simulation. The hyperparameters defining the architecture of the neural networks were optimized to determine the slimmest network size and training parameters that give the most efficient performance at the least training cost. To develop a robust model that closely mimics the governing physical laws, the discretized form of the two-phase fluid transport equation was used to formulate the supervised deep-learning task. The algorithms investigated in this study predicted the data to above 95% accuracy, with the multi-layer perceptron model demonstrating the best performance by balancing training speed, prediction time, and prediction accuracy with lean network capacity. Furthermore, the surrogate models simultaneously predict reservoir pressure and CO 2 saturation in every grid block, including the surface well extraction rate and bottomhole pressure, at all simulation times for a given static model realization in just a few seconds on a standard desktop computer. A key outcome of this study is that limits can be placed on network design parameters to avoid over designing neural networks, with associated efficiencies in training and prediction times. This is very useful because large volumes of data may be generated in CCUS projects and over-design of neural network architectures imposes penalties that are antithetical to the goal of near-real time forecasting.

58 GEOSCIENCES↗

Temperature Changes in the United States

Temperature is among the most important climatic elements used in decision-making. For example, builders and insurers use temperature data for planning and risk management while energy companies and regulators use temperature data to predict demand and set utility rates. Temperature is also a key indicator of climate change: recent increases are apparent over the land, ocean, and troposphere, and substantial changes are expected for this century. This chapter summarizes the major observed and projected changes in near-surface air temperature over the United States, emphasizing new data sets and model projections since the Third National Climate Assessment (NCA3). Changes are depicted using a spectrum of observations, including surface weather stations, moored ocean buoys, polar-orbiting satellites, and temperature-sensitive proxies. Projections are based on global models and downscaled products from CMIP5 (Coupled Model Intercomparison Project Phase 5) using a suite of Representative Concentration Pathways (RCPs; see Ch. 4: Projections for more on RCPs and future scenarios).

Vose, R. S.↗

Seasonal and Non-seasonal Sea Level Variations by Exchange of Water with Land Hydrology

The global ocean exchanges a large amount of water, seasonally or non-seasonally, with land hydrology. Apart from the long-term melting of ice sheets and glaciers, the water is exchanged directly as land runoff R, and indirectly via atmosphere in the form of precipitation minus evapo-transpiration P-E. On land, the hydrological budget balance is soil moisture S = P-E-R. The runoff R has been difficult to monitor; but now by combining the following two data sets one can obtain a global estimate, subject to the spatial and temporal resolutions afforded by the data: (1) The space gravity mission GRACE yields monthly S estimate on a spatial scale larger than approx. 1000 km over the last 2.5 years; (2) The atmospheric circulation model output, such as from NCEP, provides proxy estimates for P-E at monthly and approx. 200 km resolutions. We will discuss these estimates and the effects on the global ocean water budget and hence sea level.

Chao, Benjamin F.↗

[Space Weather Impact on the Electricity Market]

Forbes & St. Cyr (2004, hereafter "FISC") have provided evidence that the electricity market can be impacted by space weather. Our analysis indicated that the estimated market impact for PJM was 3.7 % or approximately $500 million dollars over the 19 month sample period. Kappenman has taken exception to this estimate and contends that we have exaggerated the magnitude of the problem that space weather poses to PJM. There are four specific issues: (1) he claims that we have ignored relevant literature; (2) he asserts that Dst is not an appropriate proxy for GICs in PJM; (3) he charges that our findings are inconsistent with the impact of the 17 September 2000 storm; and (4) he alleges that our discussion of October 2003 storms is misleading. In our article, we have explained our methodology, multivariate regression analysis, with a particular focus on how it compares to correlation analysis. We have also explained the limitations of our analysis. We noted that "...While the Dstlprice relationship was found to be robust, the precise estimate should be treated with a relatively high degree of caution given that econometric modeling is not an exact science as well as the fact that the measure of space weather may be a poor proxy for GICs" (paragraph 96). We have also noted that additional research using local magnetometer data are needed (paragraph 97). We did not claim that that our findings for PJM are representative of the impact of space weather on other power grids. On the contrary, we noted that ... "Only analysis of other power grids will tell. " (paragraph 97). Kappenman inaccurately asserts that we have indicated that our findings . . . "imply much higher total costs are likely across the US and elsewhere in the world." He also inaccurately asserts that we have claimed that " . . . Dst is the most suited proxy for GIC in the PJM grid.. ." Moreover, he inaccurately refers to our analysis as a correlation study that uses Dst as quasi-binary indicator.

SaintCyr, O. Chris↗

Variability of Marine Aerosol Fine-Mode Fraction and Estimates of Anthropogenic Aerosol Component Over Cloud-Free Oceans from the Moderate Resolution Imaging Spectroradiometer (MODIS)

In this study, we examine seasonal and geographical variability of marine aerosol fine-mode fraction (f(sub m)) and its impacts on deriving the anthropogenic component of aerosol optical depth (tau(sub a)) and direct radiative forcing from multispectral satellite measurements. A proxy of f(sub m), empirically derived from the Moderate Resolution Imaging Spectroradiometer (MODIS) Collection 5 data, shows large seasonal and geographical variations that are consistent with the Goddard Chemistry Aerosol Radiation Transport (GOCART) and Global Modeling Initiative (GMI) model simulations. The so-derived seasonally and spatially varying f(sub m) is then implemented into a method of estimating tau(sub a) and direct radiative forcing from the MODIS measurements. It is found that the use of a constant value for fm as in previous studies would have overestimated Ta by about 20% over global ocean, with the overestimation up to 45% in some regions and seasons. The 7-year (2001-2007) global ocean average tau(sub a) is 0.035, with yearly average ranging from 0.031 to 0.039. Future improvement in measurements is needed to better separate anthropogenic aerosol from natural ones and to narrow down the wide range of aerosol direct radiative forcing.

Yu, Hongbin↗

Assessing Uncertainties in Gridded Emissions: A Case Study for Fossil Fuel Carbon Dioxide (FFCO2) Emission Data

Fossil fuel carbon dioxide (CO2) emissions (FFCO2) are the largest input to the global carbon cycle on a decadal time scale. Because total emissions are assumed to be reasonably well constrained by fuel statistics, FFCO2 often serves as a reference in order to deduce carbon uptake by poorly understood terrestrial and ocean sinks. Conventional atmospheric CO2 flux inversions solve for spatially explicit regional sources and sinks and estimate land and ocean fluxes by subtracting FFCO2. Thus, errors in FFCO2 can propagate into the final inferred flux estimates. Gridded emissions are often based on disaggregation of emissions estimated at national or regional level. Although national and regional total FFCO2 are well known, gridded emission fields are subject to additional uncertainties due to the emission disaggregation. Assessing such uncertainties is often challenging because of the lack of physical measurements for evaluation. We first review difficulties in assessing uncertainties associated with gridded FFCO2 emission data and present several approaches for evaluation of such uncertainties at multiple scales. Given known limitations, inter-emission data differences are often used as a proxy for the uncertainty. The popular approach allows us to characterize differences in emissions, but does not allow us to fully quantify emission disaggregation biases. Our work aims to vicariously evaluate FFCO2 emission data using atmospheric models and measurements. We show a global simulation experiment where uncertainty estimates are propagated as an atmospheric tracer (uncertainty tracer) alongside CO2 in NASA's GEOS model and discuss implications of FFCO2 uncertainties in the context of flux inversions. We also demonstrate the use of high resolution urban CO2 simulations as a tool for objectively evaluating FFCO2 data over intense emission regions. Though this study focuses on FFCO2 emission data, the outcome of this study could also help improve the knowledge of similar gridded emissions data for non-CO2 compounds with similar emission characteristics.

FFCO↗