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NASA NTRS2003

Dissociative Ionization and Product Distributions of Benzene and Pyridine by Electron Impact

We report a theoretical study of the dissociative ionization (DI) and product distributions of benzene (C6H6) and pyridine (C5H5N) from their low-lying ionization channels. Our approach makes use of the fact that electronic motion is much faster than nuclear motion allowing DI to be treated as a two-step process. The first step is the electron-impact ionization resulting in an ion with the same nuclear geometry as the neutral molecule. In the second step, the nuclei relax from the initial geometry and undergo unimolecular dissociation. For the ionization process we use the improved binary-encounter dipole (iBED) model [W.M. Huo, Phys. Rev. A64,042719-I (2001)]. For the unimolecular dissociation, we use multiconfigurational self-consistent field (MCSCF) methods to determine the steepest descent pathways to the possible product channels. More accurate methods are then used to obtain better energetics of the paths which are used to determine unimolecular dissociation probabilities and product distributions. Our analysis of the dissociation products and the thresholds of their productions for benzene are compared with the recent dissociative photoionization meausurements of benzene by Feng et al. [R. Feng, G. Cooper, C.E. Brion, J. Electron Spectrosc. Relat. Phenom. 123,211 (2002)] and the dissociative photoionization measurements of pyridine by Tixier et al. [S. Tixier, G. Cooper, R. Feng, C.E. Brion, J. Electron Spectrosc. Relat. Phenom. 123,185 (2002)] using dipole (e,e+ion) coincidence spectroscopy.

Dateo, Christopher E.↗

NASA NTRS1991

Transport of gyration-dominated space plasmas of thermal origin. I - Generalized transport equations

Grad's 20-moment set of transport equations has been examined in the limit of strong external magnetic fields. This simplified set of equations describes the transport of mass and parallel momentum as well as the transport of parallel and perpendicular energy and heat flow in the magnetic field direction. The effect of collisions was calculated assuming a modified relaxation model. Wave speeds and normal modes of the simplified set of equations were examined for an ion and electron gas. It was found that four of the ten normal modes are electron thermal-heat waves which approximately decouple from the six ion waves in the system. When low-frequency waves are considered (slow-wave approximation), this allows the electron energy and heat flow equations to be solved separately from the ion equations and in a time-independent fashion. When this was done, it was found that, under certain conditions, these equations predict an infinite electron perpendicular temperature, Te-perpendicular, in the collisionless regime. This occurs whenever Te-perpendicular is greater than the parallel temperature, at any point along collisionless and diverging magnetic field lines. When applied appropriately, the significantly simplified set of equations derived here are well suited for application to a large variety of problems in planetary ionospheres and magnetospheres.

Gombosi, Tamas I.↗

NASA NTRS1992

Variable-Compliance Couplings For Heavy Lifting

New coupling devices contain manual or electronically controlled, motorized drives that vary stiffnesses. Short, clamped lengths of cable provide compliance. Using threaded rods, cables stretched, relaxed, or folded to make coupling more or less stiff. In more-advanced device, brackets holding cables moved by stepping motor via gearbox and ball screw. Motor operates under computer control with position feedback. Control computer commands greater stiffness during operations requiring precise positioning, and greater compliance to accommodate manufacturing tolerances. Intended for use in wrist joints of robotic manipulators and other industrial equipment that must lift heavy objects.

Kerley, James↗

NASA NTRS1994

Acceleration of electrons and ions by strong lower-hybrid turbulence in solar flares

One of the outstanding problems in solar flare theory is how to explain the 10-20 keV and greater hard x-ray emissions by a thick target bremsstrahlung model. The model requires the acceleration mechanism to accelerate approximately 10(exp 35) electrons sec(exp -l) with comparable energies, without producing a large return current which persists for long time scales after the beam ceases to exist due to Lenz's law, thereby, producing a self-magnetic field of order a few mega-Gauss. In this paper, we investigate particle acceleration resulting from the relaxation of unstable ion ring distributions, producing strong wave activity at the lower hybrid frequency. It is shown that strong lower hybrid wave turbulence collapses in configuration space producing density cavities containing intense electrostatic lower hybrid wave activity. The collapse of these intense nonlinear wave packets saturate by particle acceleration producing energetic electron and ion tails. There are several mechanisms whereby unstable ion distributions could be formed in the solar atmosphere, including reflection at perpendicular shocks, tearing modes, and loss cone depletion. Numerical simulations of ion ring relaxation processes, obtained using a 2 1/2-D fully electromagnetic, relativistic particle in cell code are discussed. We apply the results to the problem of explaining energetic particle production in solar flares. The results show the simultaneous acceleration of both electrons and ions to very high energies: electrons are accelerated to energies in the range 10-500 keV, while ions are accelerated to energies of the order of MeVs, giving rise to x-ray emission and gamma-ray emission respectively. Our simulations also show wave generation at the electron cyclotron frequency. We suggest that these waves are the solar millisecond radio spikes. The strong turbulence collapse process leads to a highly filamented plasma producing many localized regions for particle acceleration and resulting in approximately 10(exp 17) electron 'beamlets' of width approximately equal to 10 lambda sub De which eliminates the production of large magnetic fields. In this paper, we demonstrate that the model produces an energetic electron spectrum with the right flux to account for the hard x-ray observations.

Spicer, D. S.↗

NASA NTRS1987

A theory for the Langmuir waves in the electron foreshock

A comprehensive theory for the Langmuir waves in the earth's foreshock involving saturation of the kinetic version of the beam instability by quasi-linear relaxation is proposed in this paper. Reactive and kinetic beam instabilities are shown to be the two limiting versions of a single instability whose analytically and numerically derived descriptions are shown to form a consistent picture. It is pointed out that the reactive instability gives rise only to narrow-band growth while the kinetic instability gives rise to wide-band growth. Arguments for describing the Langmuir wave growth in terms of the kinetic instability are given, and four suppression mechanisms for the kinetic instability are discussed. It is suggested that quasi-linear relaxation limits the Langmuir growth and gives rise to distributions qualitatively similar to the observed distribution functions, and arguments in favor of this hypothesis are presented.

Cairns, Iver H.↗

NASA NTRS1981

On a theory of temporal fluctuations in the electrostatic potential structures associated with auroral arcs

A possible mechanism is presented for the generation of large-amplitude temporal fluctuations in the structure of the electron energization region associated with auroral arcs. The mechanism is based on the observation that the auroral arc system resembles a laboratory circuit consisting of the series connection of battery, resistance and a forward biased diode containing collisionless plasma in which large-amplitude relaxation oscillations are sometimes observed to be superimposed on the steady-state current. It is shown that in both the laboratory and auroral systems, in which a localized auroral arc dynamo, the ionosphere and the electron energization region are involved, the oscillations are controlled by the times for ions and electrons to traverse the acceleration region, which also characterize the low- and high-frequency structure of the fluctuating waveform. It is demonstrated that a plausible one-dimensional double-layer model of the auroral arc acceleration region exhibits the dynamic negative resistance necessary for the generation of oscillations by the present mechanism. Finally, consideration is given to two kinds of auroral phenomena which might be associated with the mechanism: the 10-Hz quasi-periodic flickering aurora and 10-Hz modulations in the intensity of electrostatic hydrogen cyclotron waves.

Silevitch, M. B.↗

NASA NTRS1991

Comptonization of gamma rays by cold electrons

An analytic method is developed for calculating the emergent spectrum of gamma-rays and X-rays scattered in a homogeneous medium with low-temperature electrons. The Klein-Nishina corrections of the scattering cross section and absorption processes are taken in account. The wavelength relaxation and the spatial diffusion problems are solved separately, and the emergent spectrum is calculated by convolving the evolution function of the spectrum in an infinite medium with the photon luminosity resulting from the spatial diffusion in a finite sphere. The analytic results are compared with that of Monte Carlo calculations and it is concluded that the analytic result is quite accurate.

Xu, Yueming↗

NASA NTRS2008

A KPC-Scale X-Ray Jet in the BL Lac Source S5 2007+777

X-ray jets in AGN are commonly observed in FRII and FRI radiogalaxies, but rarely in BL Lacs, most probably due to their orientation close to the line of sight and the ensuing foreshortening effects. Only three BL Lacs are known so far to contain a kpc-scale X-ray jet. In this paper, we present the evidence for the existence of a fourth extended X-ray jet in the classical radio-selected source S5 2007+777, which for its hybrid FRI/II radio morphology has been classified as a HYMOR (HYbrid MOrphology Radio source). Our Chandra ACISS observations of this source revealed an X-ray counterpart to the 19"-long radio jet. Interestingly, the X-ray properties of the kpc-scale jet in S5 2007+777 are very similar to those observed in FRII jets. First, the X-ray morphology closely mirrors the radio one, with the X-rays being concentrated in the discrete radio knots. Second, the X-ray continuum of the jet/brightest knot is described by a very hard power law, with photon index gamma(sub x) approximately 1. Third, the optical upper limit from archival HST data implies a concave radio-to-X-ray SED. If the X-ray emission is attributed to IC/CMB with equipartition, strong beaming (delta= 13) is required, implying a very large scale (Mpc) jet. The beaming requirement can be somewhat relaxed assuming a magnetic field lower than equipartition. Alternatively, synchrotron emission from a second population of very high-energy electrons is viable. Comparison to other HYMOR jets detected with Chandra is discussed, as well as general implications for the origin of the FRI/II division.

Sambruna, Rita M.↗

NASA NTRS1976

An interpretation of Jupiter's decametric radiation and the terrestrial kilometric radiation as direct amplified gyroemission

Direct amplified gyroemission due to an anisotropic distribution of suprathermal electrons is proposed as the most plausible emission mechanism for Jupiter's decametric radiation (DAM) and the terrestrial auroral kilometric radiation (AKR). It is suggested that the required electron distribution could be produced by electrons, initially with small pitch angles, precipitating from the magnetosphere. A quasi-linear treatment of the proposed mechanism is outlined, including satisfaction of the Doppler condition, calculation of the growth rate, conditions for quasi-linear relaxation, and generation of the anisotropy. The mechanism is applied to the Jovian DAM, emphasizing the growth rate, the power radiated, and the elliptical polarization of the radiation. It is found that the theory can account for the gross features of the DAM, provided the number density in the precipitating electron streams exceeds 20 per cu cm. Application of the theory to the AKR shows that the requirements concerning the properties of the precipitating electrons appear to be satisfied by the observed properties of those inverted V events which correlate with the emission of AKR.

Melrose, D. B.↗

NASA NTRS2002

Dissociative Ionization of Benzene by Electron Impact

We report a theoretical study of the dissociative ionization (DI) of benzene from the low-lying ionization channels. Our approach makes use of the fact that electron motion is much faster than nuclear motion and DI is treated as a two-step process. The first step is electron-impact ionization resulting in an ion with the same nuclear geometry as the neutral molecule. In the second step the nuclei relax from the initial geometry and undergo unimolecular dissociation. For the ionization process we use the improved binary-encounter dipole (iBED) model. For the unimolecular dissociation step, we study the steepest descent reaction path to the minimum of the ion potential energy surface. The path is used to analyze the probability of unimolecular dissociation and to determine the product distributions. Our analysis of the dissociation products and the thresholds of the productions are compared with the result dissociative photoionization measurements of Feng et al. The partial oscillator strengths from Feng et al. are then used in the iBED cross section calculations.

Huo, Winifred↗

NASA NTRS1972

Resonance quasi-projection operators - Calculation of the super 2 S autoionization state of He/-/.

Development of a method to remedy the defects of the projection-operator technique for calculating electron resonances in scattering from many-electron targets. It is recommended that the projection operator Q be replaced by a quasi-projection operator which yields a discrete spectrum which can be made to be in essentially a unique correspondence with resonance energies. By relaxing the idempotency requirement, it is found possible to define two forms of this quasi-projection operator. The simpler of the two forms is tested on e-H and e-H(+) systems; the two lowest resonant energies differ by less than 0.01 eV from rigorous QHQ results. For many-electron targets it is further argued that replacement of the exact target eigenfunction by reasonable approximations in constructing the quasi-projection operator will affect neither the discreteness of the above-mentioned discrete spectrum nor the proximity of its eigenvalues to the resonant energies.

Temkin, A.↗

NASA NTRS1980

Bulk submillimeter-wave mixers: Strain and superlattices

Strained germanium crystals, doped with gallium, were used as heterodyne mixers at THz frequencies, with infrared bandwidths approaching a GHz. The mixer performance (conversion loss and mixer noise) was analyzed in terms of nonlinearities associated with acceptor levels and with relaxation rates of free holes. Comparison was made with similar mixers employing low lying donor levels in high purity GaAs and with hot electron InSb mixers.

Litvak, M. M.↗

NASA NTRS1984

Thermal detectors as X-ray spectrometers

Sensitive thermal detectors should be useful for measuring very small energy pulses, such as those produced by the absorption of X-ray photons. The measurement uncertainty can be very small, making the technique promising for high resolution nondispersive X-ray spectroscopy. The limits to the energy resolution of such thermal detectors are derived and used to find the resolution to be expected for a detector suitable for X-ray spectroscopy in the 100 eV to 10,000 eV range. If there is no noise in the thermalization of the X-ray, resolution better than 1 eV full width at half maximum is possible for detectors operating at 0.1 K. Energy loss in the conversion of the photon energy to heat is a potential problem. The loss mechanisms may include emission of photons or electrons, or the trapping of energy in long lived metastable states. Fluctuations in the phonon spectrum could also limit the resolution if phonon relaxation times are very long. Conceptual solutions are given for each of these possible problems.

Moseley, S. H.↗

NASA NTRS1984

Thermal detectors as X-ray spectrometers

Moseley, S. H.↗

NASA NTRS2005

Energetic Metastable Oxygen and Nitrogen Atoms in the Terrestrial Atmosphere

This report summarizes our research performed under NASA Grant NAG5-11857. The three-year grant have been supported by the Geospace Sciences SR&T program. We have investigated the energetic metastable oxygen and nitrogen atoms in the terrestrial stratosphere, mesosphere and thermosphere. Hot atoms in the atmosphere are produced by solar radiation, the solar wind and various ionic reactions. Nascent hot atoms arise in ground and excited electronic states, and their translational energies are larger by two - three orders of magnitude than the thermal energies of the ambient gas. The relaxation kinetics of hot atoms determines the rate of atmospheric heating, the intensities of aeronomic reactions, and the rate of atom escape from the planet. Modeling of the non-Maxwellian energy distributions of metastable oxygen and nitrogen atoms have been focused on the determination of their impact on the energetics and chemistry of the terrestrial atmosphere between 25 and 250 km . At this altitudes, we have calculated the energy distribution functions of metastable O and N atoms and computed non-equilibrium rates of important aeronomic reactions, such as destruction of the water molecules by O(1D) atoms and production of highly excited nitric oxide molecules. In the upper atmosphere, the metastable O(lD) and N(2D) play important role in formation of the upward atomic fluxes. We have computed the upward fluxes of the metastable and ground state oxygen atoms in the upper atmosphere above 250 km. The accurate distributions of the metastable atoms have been evaluated for the day and night-time conditions.

Kharchenko, Vasili↗

NASA NTRS1999

The Radio Plasma Imager Investigation on the IMAGE Spacecraft

Radio plasma imaging uses total reflection of electromagnetic waves from plasmas whose plasma frequencies equal the radio sounding frequency and whose electron density gradients are parallel to the wave normals. The Radio Plasma Imager (RPI) has two orthogonal 500-m long dipole antennas in the spin plane for near omni-directional transmission. The third antenna is a 20-m dipole. Echoes from the magnetopause, plasmasphere and cusp will be received with three orthogonal antennas, allowing the determination of their angle-of-arrival. Thus it will be possible to create image fragments of the reflecting density structures. The instrument can execute a large variety of programmable measuring programs operating at frequencies between 3 kHz and 3 MHz. Tuning of the transmit antennas provides optimum power transfer from the 10 W transmitter to the antennas. The instrument can operate in three active sounding modes: (1) remote sounding to probe magnetospheric boundaries, (2) local (relaxation) sounding to probe the local plasma, and (3) whistler stimulation sounding. In addition, there is a passive mode to record natural emissions, and to determine the local electron density and temperature by using a thermal noise spectroscopy technique.

Reinisch, Bodo W.↗

NASA NTRS1974

The spin-temperature theory of dynamic nuclear polarization and nuclear spin-lattice relaxation

A detailed derivation of the equations governing dynamic nuclear polarization (DNP) and nuclear spin lattice relaxation by use of the spin temperature theory has been carried to second order in a perturbation expansion of the density matrix. Nuclear spin diffusion in the rapid diffusion limit and the effects of the coupling of the electron dipole-dipole reservoir (EDDR) with the nuclear spins are incorporated. The complete expression for the dynamic nuclear polarization has been derived and then examined in detail for the limit of well resolved solid effect transitions. Exactly at the solid effect transition peaks, the conventional solid-effect DNP results are obtained, but with EDDR effects on the nuclear relaxation and DNP leakage factor included. Explicit EDDR contributions to DNP are discussed, and a new DNP effect is predicted.

Byvik, C. E.↗

NASA NTRS1980

A laboratory study on the dissociative recombination of vibrationally excited O2/+/ions

The dissociative recombination of vibrationally excited O2(+) ions is studied in light of the possible importance of this reaction in upper atmospheric chemistry. A plasma spectroscopy experiment was performed in a microwave cavity filled by an argon-oxygen mixture, with O(1S) production monitored by measurements of the 5577-A afterglow, the O2(+) density and the electron concentration. Plasma and optical data reveal the predominant afterglow ions to be Ar2(+) and O2(+), with an effective O(1S) dissociative recombination coefficient of 2.1 x 10 to the -8th cu cm/sec, corresponding to a quantum yield of 10%. Experiments with an argon-krypton-oxygen mixture reveal that vibrationally excited O2(+) ions are the chief source of the O(1S) atoms, with a specific recombination coefficient for the dissociation of O2(+)(2 pi g) into O(1S) and O(1D) of 4.2 x 10 to the -9th cu cm/sec. A comparison of the laboratory results with Atmospheric Explorer data on the 5577-A airglow implies that O2(+) ions in the sunlit ionosphere are vibrationally excited to the same degree as in the laboratory, with the vibrational relaxation of these ions much slower than dissociative recombination. Results also predict a dawn-twilight asymmetry in the effective O(1S) yield due to the normal variation of electron content.

Zipf, E. C.↗