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At least 181 records · Page 10
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Detector Calibration to Quantify Random Summing in HPGe Spectroscopy

While calibrating a High Purity Germanium (HPGe) Radiation Detector for Xenon-133 (133Xe) the process of random summing occurs which leads to excess counts in the 160.6keV peak from random summing of the 81keV photons at the 162keV energy. Multiple samples of 133Xe with varying levels of radioactivity were assayed to determine a relationship between the occurrence of random summing and the net area of the 160.6keV peak. When the calculated efficiencies in the 160.6keV peak were compared to the theoretical efficiency obtained from a multi-energy calibration at 160.6keV, the amount of random summing could be estimated as excess observed efficiency and correlated to the sample activity. While a trend is apparent in the data, the mechanisms that contribute to the trend are still being studied so the data can be accurately correlated.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2026

Detector Characterization for SuperCDMS Commissioning

Super Cryogenic Dark Matter Search (SuperCDMS) SNOLAB is a next generation direct detection experiment search ing for low mass dark matter using cryogenic germanium and silicon detectors operated at millikelvin temperatures. As the experiment begins its first commissioning data taking, establishing that the detectors respond to energy deposits in a stable, predictable way is a prerequisite for any future physics analysis. This work presents a study of detector stability for four SuperCDMS SNOLAB detectors, det 7 and det 15 (germanium), and det 11 and det 14 (silicon), using two data sets taken during early commissioning: dedicated Barium-133 calibration runs, which provide a known gamma ray energy reference at 356 keV, and low background runs, which record whatever background radiation the detectors see with no external source present. The Ba-133 data do not show a distinct, well localized line at the expected energy, and the low background data show a baseline that drifts and oscillates over time rather than remaining flat. This baseline instability appears consistently across multiple channels rather than being confined to one, suggesting a shared, detector wide cause rather than a single faulty channel. Together, these observations point to the detectors’ cryogenic support system as the likely source of the instability, since small temperature fluctuations introduced during normal operation of the cooling system could plausibly couple into the exquisitely temperature sensitive detectors. These results inform the ongoing commissioning effort by narrowing down where instability in the current data is originating from.

O'Hanlon, Viktoria M. [Skidmore Coll.; Fermilab]↗
DOE OSTI2026

Detector Characterization for SuperCDMS Commissioning

Super Cryogenic Dark Matter Search (SuperCDMS) SNOLAB is a next generation direct detection experiment search ing for low mass dark matter using cryogenic germanium and silicon detectors operated at millikelvin temperatures. As the experiment begins its first commissioning data taking, establishing that the detectors respond to energy deposits in a stable, predictable way is a prerequisite for any future physics analysis. This work presents a study of detector stability for four SuperCDMS SNOLAB detectors, det 7 and det 15 (germanium), and det 11 and det 14 (silicon), using two data sets taken during early commissioning: dedicated Barium-133 calibration runs, which provide a known gamma ray energy reference at 356 keV, and low background runs, which record whatever background radiation the detectors see with no external source present. The Ba-133 data do not show a distinct, well localized line at the expected energy, and the low background data show a baseline that drifts and oscillates over time rather than remaining flat. This baseline instability appears consistently across multiple channels rather than being confined to one, suggesting a shared, detector wide cause rather than a single faulty channel. Together, these observations point to the detectors’ cryogenic support system as the likely source of the instability, since small temperature fluctuations introduced during normal operation of the cooling system could plausibly couple into the exquisitely temperature sensitive detectors. These results inform the ongoing commissioning effort by narrowing down where instability in the current data is originating from.

O'Hanlon, Viktoria M. [Skidmore Coll.; Fermilab]↗
DOE OSTI2023

Reduction in radioactivity-induced backgrounds using a novel active veto detector for rare event search experiments

The results of a newly developed annular cryogenic phonon-mediated active veto detector are discussed which shows a significant reduction of radioactivity-induced backgrounds in rare event search experiments. The veto detector is made up of germanium weighing ∼500 g with an outer diameter of 76 mm and an inner diameter of 28 mm. The detector can host a 25 mm diameter germanium inner target detector of mass ∼10 g. A GEANT4 simulation with the active veto and inner target detector shows a gamma background reduction of 50 - 80% which is further improved (> 90%) with 4pi veto coverage. Experimental measurements with the detector assembly agree well with the simulation.

Chaudhuri, Mouli↗
DOE OSTI2022

Low-threshold sapphire detector for rare event searches

Low mass nuclear recoil dark matter and coherent-elastic-neutrino-nucleus-scattering (CE$v$NS) searches confront similar challenges in choosing ultra-low threshold and large-mass detectors. Here, we report experimental results from a 100 g single-crystal sapphire detector design with a diameter of 76 mm and thickness of 4 mm instrumented with transition edge sensors (TES). Sapphire is a crystal of aluminum oxide (Al 2 O) and has been found to be a good candidate for light mass dark matter search experiments due to its lower atomic mass compared to other detector materials such as germanium and silicon. This new phonon-assisted sapphire detector was characterized to yield a baseline recoil energy resolution of 28.4 ± 0.4 eV. The detector is designed to be sensitive to low-energy rare interactions with an intention to investigate the low-mass region of dark matter phase-space and search for CE$v$NS at the reactor site.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Identify and Assess Technical Challenges in Safeguards Measurements of Spent Advanced Reactor Fuels

Advanced reactor (AR) designs use various nuclear fuel types that can be significantly different than conventional light-water reactor (LWR) fuels, including differences in sizes, compositions, and chemical forms (e.g., oxide, carbide, metal). Nearly all the proposed AR fuels use high-assay low-enriched uranium (HALEU), which will have higher enrichments (5–20 wt% 235 U) than LWR fuels (currently limited to <5 wt% 235 U). In advance of the wide use of these new fuel types around the world, international safeguards organizations such as the International Atomic Energy Agency (IAEA]) are working with some of the AR vendors to formulate safeguards approaches for these AR fuel cycles. As part of the overall safeguards approach, it is important to identify the potential technical challenges in performing safeguards verification measurements of these AR fuels (both fresh and spent fuels) in advance of the widespread adoption of these new fuel types, because new safeguards technologies can take several years to develop, test, and approve for use. This report documents work performed in fiscal year 2024 based on modeling and simulation to assess the performance of the existing safeguards measurement technologies for irradiated or spent AR fuel elements or items. This work is a continuation of the work performed in fiscal year 2023 that focused on fresh AR fuels. Spent AR fuels have a distinct difference from their LWR counterparts: unlike the spent LWR fuels typically stored in a water-filled pool, some spent AR fuels—such as tristructural-isotropic (TRISO)-based fuels—will most likely be stored in air-filled hot cells. Because most safeguards measurements on spent fuel performed to date have been conducted under water, the air-filled hot cell environment could present unique challenges to safeguards measurements. Fork detector (FDET) and Cerenkov viewing device (CVD) systems have been the two primary instruments used by the IAEA for several decades to measure spent LWR fuel assemblies stored in pools for safeguards verification purposes. Because the lower refractive index of air causes Cerenkov light to be of lower intensity in air than in water, existing CVDs are likely unable to perform safeguards verification measurements for spent fuel stored in an air-filled hot cell, as is the case for the TRISO-based spent fuel elements (e.g., pebbles, graphite fuel blocks). Unlike FDET measurements, CVD measurements do not require fuel be moved, so they are a simpler and faster to take than FDET measurements. The inability to perform CVD measurements on the TRISO-based AR fuel types presents a major technical challenge in the effort to use existing technology to perform safeguards measurements on spent AR fuels. This study was mainly conducted through the modeling and simulation of an FDET or an FDET-like system on five spent AR fuel types, including one metallic fuel type and four TRISO-based fuel types in both pebble and graphite block forms in their respective storage configurations and environments. Because the various AR fuel types have significantly different dimensions, FDET systems must be adapted to accommodate them. Partial defect tests were also simulated in this study to assess the FDET’s ability to detect potential fuel diversions. The FDET measures the fuel’s total passive neutron and gamma emissions. The simulated FDET results from spent AR fuel items are compared against results from a typical spent pressurized water reactor (PWR) assembly. High-purity germanium (HPGe) gamma detector measurements were also simulated for the spent AR fuel types and the PWR assembly because the signature photopeaks have been used in LWR safeguards verifications, although HPGe is usually not used to detect diversions because of the fuel’s self-attenuation effects on those photopeaks. The results indicate that these detectors have significant challenges in performing safeguards measurements of the spent AR fuel items, including incompatibilities between AR fuel items and existing FDETs, lower neutron count rates, lower sensitivities to fuel diversions in certain AR fuel items, and significantly higher interference from a neighboring fuel item when the measurement is performed in air. These results suggest that an alternative technology or significant and timely technology development is needed to perform adequate safeguards measurements of some of these AR fuel items.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2020

Applications of HPGe-detected high energy gamma rays toward quantifying neutron emission rates and 234 U enrichment in UF 6 cylinders

This study presents a 234 U enrichment meter that uses high energy gamma and neutron count rate as measured by a portable, high-purity germanium gamma ray detector. Twenty-one 30B cylinders containing UF 6 of varying origin were analyzed with an HPGe detector for high-energy gamma ray and neutron counts. Excellent correlations (R 2 0.95) between various regions of 3.0 MeV gamma rays, neutron count rate, and uranium enrichment were found. These neutron and high-energy gamma data are used to create calibration-dependent enrichment meters for 234 U. The 234 U enrichment calculated from the neutron count rate and 4 – 6 MeV gamma count rate is more accurate than methods that rely on the 120.9 keV peak which is strongly attenuated inside commercial sized UF 6 cylinders. These neutron and high-energy gamma enrichment calculators can also be used to determine a 235 U enrichment, assuming mass-based enrichment from natural uranium, but the results are not as accurate as the traditional 185.7 keV peak enrichment meter.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

β decay of neutron-rich 76 Cu and the structure of 76 Zn

In this work, the β decay of 76 Cu to the levels of 76 Zn was studied at the Holifield Radioactive Ion Beam Facility (HRIBF) at Oak Ridge National Lab (ORNL). A purified 76 Cu beam was developed and data were recorded for the decay of the A=76 decay chain using four high-purity germanium (HPGe) clover detectors at the Low-energy Radioactive Ion Beam Spectroscopy Station (LeRIBSS). In this measurement, data on γ-ray emission following β decay, including βγ and γγ coincidences, were collected and γγ spectra were analyzed to identify the statistically significant coincidences. From this analysis, we propose a level scheme for 76 Zn which contains a total of 59 energy levels up to 6.0 MeV containing 105 γ rays. We have identified an additional 53 γ rays associated with this decay which could not be place in the decay scheme due to insufficient coincidence information or no energy match to identified levels. No γ rays from states in 75 Zn fed in the delayed-neutron branch were observed even though other γ rays in the A=75 decay chain were observed. Spin and parity assignments are proposed for some levels based on comparison to systematics and shell model calculations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Specification of EBR-II Gamma Scan Data from the Precision Gamma Scanner

The gamma scan data stored in the FIPD was originally measured using the Precision Gamma Scanner (PGS) at the Hot Fuel Examination Facility (HFEF) at Idaho National Laboratory (INL). This system was originally manufactured in 1971 (when the facilities, now at INL, were operated by Argonne National Laboratory) and was upgraded on several occasions. It consists of a germanium gamma ray detector (the exact nature of which changed over time as technology improved), a variable-slit collimator that blocks the view of gamma emissions from all but the selected area of the target, and a computer-controlled system for translating a sample past the slit and logging the data.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2025

Multi-channel, multi-template event reconstruction for SuperCDMS data using machine learning

SuperCDMS SNOLAB uses kilogram-scale germanium and silicon detectors to search for dark matter. Each detector has Transition Edge Sensors (TESs) patterned on the top and bottom faces of a large crystal substrate, with the TESs electrically grouped into six phonon readout channels per face. Noise correlations are expected among a detector's readout channels, in part because the channels and their readout electronics are located in close proximity to one another. Moreover, owing to the large size of the detectors, energy deposits can produce vastly different phonon propagation patterns depending on their location in the substrate, resulting in a strong position dependence in the readout-channel pulse shapes. Both of these effects can degrade the energy resolution and consequently diminish the dark matter search sensitivity of the experiment if not accounted for properly. We present a new algorithm for pulse reconstruction, mathematically formulated to take into account correlated noise and pulse shape variations. This new algorithm fits N readout channels with a superposition of M pulse templates simultaneously - hence termed the N$\times$M filter. We describe a method to derive the pulse templates using principal component analysis (PCA) and to extract energy and position information using a gradient boosted decision tree (GBDT). We show that these new N$\times$M and GBDT analysis tools can reduce the impact from correlated noise sources while improving the reconstructed energy resolution for simulated mono-energetic events by more than a factor of three and for the 71Ge K-shell electron-capture peak recoils measured in a previous version of SuperCDMS called CDMSlite to $<$ 50 eV from the previously published value of $\sim$100 eV. These results lay the groundwork for position reconstruction in SuperCDMS with the N$\times$M outputs.

Albakry, M. F. [British Columbia U.; TRIUMF]↗
DOE OSTI2024

Investigating Influential Parameters for High-Purity Germanium Crystal Growth

This paper focuses on the research and development of high-purity germanium (HPGe) crystals for detector fabrication, specifically targeting applications in rare-event physics searches. The primary objective was to produce large-scale germanium crystals weighing >1 kg with a controlled diameter of ∼10 cm and an impurity range of approximately 1010/cm 3. Ensuring structural integrity and excellent crystalline quality requires a thorough assessment of dislocation density, a critical aspect of the crystal development process. Dislocation density measurements play a crucial role in maximizing the sensitivity of HPGe detectors, and our findings confirmed that the dislocation density fell within acceptable ranges for detector fabrication. Additionally, this paper examines the segregation coefficient of various contaminants during the crystal development process. Comprehensive analysis of impurity segregation is essential for reducing contaminant quantities in the crystal lattice and customizing purification processes. This, in turn, minimizes undesired background noise, enhancing signal-to-noise ratios for rare-event physics searches and overall detector performance. The investigation included the segregation coefficients of three major acceptors and one donor in crystals grown at the University of South Dakota, providing valuable insights for optimizing crystal purity and detector efficiency.

Bhattarai, Sanjay↗
DOE OSTI2024

Phonon-mediated quantum efficiency measurement in semiconductors

Accurate quantum efficiency measurement not only provides crucial information for the photovoltaic cell industry but also supports experiments aimed at directly detecting dark matter and elastic neutrino interactions. The dark matter direct searches paradigm has recently expanded to include particles with masses below 1,MeV/c2, where the expected signal in an electron–recoil interaction is approximately in the eV range, just above the energy gap for silicon and germanium. A robust calibration method for ionization signals in this lower energy region is essential. This paper presents a method for measuring quantum efficiency and yield (q/E) in semiconductors using phonon-mediated calorimetry. The Neganov–Trofimov–Luke phonon amplification method in low-temperature semiconductor crystals has been employed to indirectly measure ionization down to single-electron accuracy. Specifically, at zero bias, the phonon readout directly quantifies the total energy deposited within the detector, independent of the ionization yield. This eliminates a significant source of systematic uncertainty in quantum efficiency estimates associated with total energy uncertainty. The paper includes results from an updated ionization efficiency measurement in a germanium detector.

Physics↗
DOE OSTI2024

First demonstration of 30 eVee ionization energy resolution with RICOCHET germanium cryogenic bolometers

The future RICOCHET experiment aims to search for new physics in the electroweak sector by measuring the Coherent Elastic Neutrino-Nucleus Scattering process from reactor antineutrinos with high precision down to the sub-100 eV nuclear recoil energy range. While the RICOCHET collaboration is currently building the experimental setup at the reactor site, it is also finalizing the cryogenic detector arrays that will be integrated into the cryostat at the Institut Laue Langevin in early 2024. In this paper, we report on recent progress from the Ge cryogenic detector technology, called the CryoCube. More specifically, we present the first demonstration of a 30 eVee (electron equivalent) baseline ionization resolution (RMS) achieved with an early design of the detector assembly and its dedicated High Electron Mobility Transistor (HEMT) based front-end electronics with a total input capacitance of about 40 pF. This represents an order of magnitude improvement over the best ionization resolutions obtained on similar phonon-and-ionization germanium cryogenic detectors from the EDELWEISS and SuperCDMS dark matter experiments, and a factor of three improvement compared to the first fully-cryogenic HEMT-based preamplifier coupled to a CDMS-II germanium detector with a total input capacitance of 250 pF. Additionally, we discuss the implications of these results in the context of the future RICOCHET experiment and its expected background mitigation performance.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Investigation of ASIC-based signal readout electronics for LEGEND-1000

LEGEND, the Large Enriched Germanium Experiment for Neutrinoless ββ Decay, is a ton-scale experimental program to search for neutrinoless double beta (0νββ) decay in the isotope 76 Ge with an unprecedented sensitivity. Building on the success of the low-background 76 Ge-based GERDA and Majorana Demonstrator experiments, the LEGEND collaboration is targeting a signal discovery sensitivity beyond 10 28 yr on the decay half-life with approximately 10 t∙yr of exposure. Signal readout electronics in close proximity to the detectors plays a major role in maximizing the experiment's discovery sensitivity by reducing electronic noise and improving pulse shape analysis capabilities for the rejection of backgrounds. However, the proximity also poses unique challenges for the radiopurity of the electronics. Application-specific integrated circuit (ASIC) technology allows the implementation of the entire charge sensitive amplifier (CSA) into a single low-mass chip while improving the electronic noise and reducing the power consumption. In this work, we investigated the properties and electronic performance of a commercially available ASIC CSA, the XGLab CUBE preamplifier, together with a p-type point contact high-purity germanium detector. We show that low noise levels and excellent energy resolutions can be obtained with this readout. Moreover, we demonstrate the viability of pulse shape discrimination techniques for reducing background events.

47 OTHER INSTRUMENTATION↗
DOE OSTI2025

Improved field assessments of chemicals and explosives using high-resolution gamma-ray spectroscopy with a tagged neutron interrogation system

A fi eld-portable tagged neutron interrogation system is being developed for detection of explosives and chemical warfare agents by prompt gamma-ray neutron activation analysis. The system combines an associated particle imaging deuterium-tritium neutron generator with a high-purity germanium gamma-ray detector. Fine spatial resolution neutron and alpha detectors enable precise mapping of characteristic gamma-ray emission distributions onto high-clarity neutron radiographic images. A narrow coincidence gate associated with each tagged neutron ensures a large signal-to-background ratio, thus signifi cantly improving sensitivity to the chemical compositions of the items being assessed. Recent experimental results recorded from test objects involving mock explosives and other chemicals are presented.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗
DOE OSTI2025

Improved field assessments of chemicals and explosives using high-resolution gamma-ray spectroscopy with a tagged neutron interrogation system

A fi eld-portable tagged neutron interrogation system is being developed for detection of explosives and chemical warfare agents by prompt gamma-ray neutron activation analysis. The system combines an associated particle imaging deuterium-tritium neutron generator with a high-purity germanium gamma-ray detector. Fine spatial resolution neutron and alpha detectors enable precise mapping of characteristic gamma-ray emission distributions onto high-clarity neutron radiographic images. A narrow coincidence gate associated with each tagged neutron ensures a large signal-to-background ratio, thus signifi cantly improving sensitivity to the chemical compositions of the items being assessed. Recent experimental results recorded from test objects involving mock explosives and other chemicals are presented.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗