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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 181 records · Page 10
All sourcesNASA NTRSDOE OSTI
NASA NTRS2008

Aerosol and Cloud Interaction Observed From High Spectral Resolution Lidar Data

Recent studies utilizing satellite retrievals have shown a strong correlation between aerosol optical depth (AOD) and cloud cover. However, these retrievals from passive sensors are subject to many limitations, including cloud adjacency (or 3D) effects, possible cloud contamination, uncertainty in the AOD retrieval. Some of these limitations do not exist in High Spectral Resolution Lidar (HSRL) observations; for instance, HSRL observations are not a ected by cloud adjacency effects, are less prone to cloud contamination, and offer accurate aerosol property measurements (backscatter coefficient, extinction coefficient, lidar ratio, backscatter Angstrom exponent,and aerosol optical depth) at a neospatial resolution (less than 100 m) in the vicinity of clouds. Hence, the HSRL provides an important dataset for studying aerosol and cloud interaction. In this study, we statistically analyze aircraft-based HSRL profiles according to their distance from the nearest cloud, assuring that all profile comparisons are subject to the same large-scale meteorological conditions. Our results indicate that AODs from HSRL are about 17% higher in the proximity of clouds (approximately 100 m) than far away from clouds (4.5 km), which is much smaller than the reported cloud 3D effect on AOD retrievals. The backscatter and extinction coefficients also systematically increase in the vicinity of clouds, which can be explained by aerosol swelling in the high relative humidity (RH) environment and/or aerosol growth through in cloud processing (albeit not conclusively). On the other hand, we do not observe a systematic trend in lidar ratio; we hypothesize that this is caused by the opposite effects of aerosol swelling and aerosol in-cloud processing on the lidar ratio. Finally, the observed backscatter Angstrom exponent (BAE) does not show a consistent trend because of the complicated relationship between BAE and RH. We demonstrate that BAE should not be used as a surrogate for Angstrom exponent, especially at high RH.

Su, Wenying↗
NASA NTRS2004

Aerosol Optical Properties Measured Onboard the Ronald H. Brown During ACE Asia as a Function of Aerosol Chemical Composition and Source Region

During the ACE Asia intensive field campaign conducted in the spring of 2001 aerosol properties were measured onboard the R/V Ronald H. Brown to study the effects of the Asian aerosol on atmospheric chemistry and climate in downwind regions. Aerosol properties measured in the marine boundary layer included chemical composition; number size distribution; and light scattering, hemispheric backscattering, and absorption coefficients. In addition, optical depth and vertical profiles of aerosol 180 deg backscatter were measured. Aerosol within the ACE Asia study region was found to be a complex mixture resulting from marine, pollution, volcanic, and dust sources. Presented here as a function of air mass source region are the mass fractions of the dominant aerosol chemical components, the fraction of the scattering measured at the surface due to each component, mass scattering efficiencies of the individual components, aerosol scattering and absorption coefficients, single scattering albedo, Angstrom exponents, optical depth, and vertical profiles of aerosol extinction. All results except aerosol optical depth and the vertical profiles of aerosol extinction are reported at a relative humidity of 55 +/- 5%. An over-determined data set was collected so that measured and calculated aerosol properties could be compared, internal consistency in the data set could be assessed, and sources of uncertainty could be identified. By taking into account non-sphericity of the dust aerosol, calculated and measured aerosol mass and scattering coefficients agreed within overall experimental uncertainties. Differences between measured and calculated aerosol absorption coefficients were not within reasonable uncertainty limits, however, and may indicate the inability of Mie theory and the assumption of internally mixed homogeneous spheres to predict absorption by the ACE Asia aerosol. Mass scattering efficiencies of non-sea salt sulfate aerosol, sea salt, submicron particulate organic matter, and dust found for the ACE Asia aerosol are comparable to values estimated for ACE 1, Aerosols99, and INDOEX. Unique to the ACE Asia aerosol was the large mass fractions of dust, the dominance of dust in controlling the aerosol optical properties, and the interaction of dust with soot aerosol.

Quinn, P. K.↗
NASA NTRS1977

Measured backscatter and attenuation properties, including polarization effects, of various dispersions at 0.9 micron

The optical properties of a wide variety of atmospheric dispersions were studied using a 0.9-micron lidar system which included a GaAs laser stack transmitter emitting a horizontally polarized beam of 4 milliradians vertical divergence and 1.5 milliradians horizontal divergence. A principal means for assessing optical properties was the polarization ratio, that is, the backscattered radiation power perpendicular to the transmitter beam divided by the backscattered radiation power parallel to the beam polarization. The ratio of the backscattered fraction to the attenuation coefficient was also determined. Data on the dispersion properties of black carbon smoke, road dust, fog, fair-weather cumulus clouds, snow and rain were obtained; the adverse effects of sunlight-induced background noise on the readings is also discussed.

Kohl, R. H.↗
NASA NTRS2014

High Spectral Resolution Lidar and MPLNET Micro Pulse Lidar Aerosol Optical Property Retrieval Intercomparison During the 2012 7-SEAS Field Campaign at Singapore

From August 2012 to February 2013 a High Resolution Spectral Lidar (HSRL; 532 nm) was deployed at that National University of Singapore near a NASA Micro Pulse Lidar NETwork (MPLNET; 527 nm) site. A primary objective of the MPLNET lidar project is the production and dissemination of reliable Level 1 measurements and Level 2 retrieval products. This paper characterizes and quantifies error in Level 2 aerosol optical property retrievals conducted through inversion techniques that derive backscattering and extinction coefficients from MPLNET elastic single-wavelength datasets. MPLNET Level 2 retrievals for aerosol optical depth and extinction/backscatter coefficient profiles are compared with corresponding HSRL datasets, for which the instrument collects direct measurements of each using a unique optical configuration that segregates aerosol and cloud backscattered signal from molecular signal. The intercomparison is performed, and error matrices reported, for lower (0-5km) and the upper (>5km) troposphere, respectively, to distinguish uncertainties observed within and above the MPLNET instrument optical overlap regime.

MPL↗
NASA NTRS1990

Summary of results and conclusions based on analysis of volume imaging and high spectral resolution lidar data acquired during FIRE phase 1, part 2

Since the fall of 1986, cirrus clouds were observed with backscatter cross sections ranging from less than 1 x 10(exp -7) to 4.2 x 10(exp -5)m/sr, optical thicknesses ranging from less than .003 to greater than 2.7, and bulk average backscatter phase functions from .02 to .065/sr. Cirrus cloud structures were recorded ranging in vertical extent from 0.1 to 8 km, having horizontal scales from 10's of meters to 266 km, and exhibiting aspect ratios of from 1:5 to 1:100. The altitude relationship between cloud top and bottom boundaries and the optical center of the cloud is influenced by the type of formation observed. Cirrus morphology and generation processes appear to be related to the wind field. The high spectral resolution lidar (HSRL) was adapted to the task of cirrus cloud optical property measurement. The HSRL data reported were collected with the CuCl2 transmitter producing 50 mW of output power, achieving eye safe, direct optical depth and backscatter cross section measurements with 10 minute averaging times.

Grund, Christian J.↗
NASA NTRSDate not supplied

PM 2.5 Concentrations over Major Metropolitan Regions Inferred from Airborne High Spectral Resolution Lidar Measurements Using Machine Learning Regression

We use measurements of near-surface aerosol backscatter, extinction, and depolarization acquired by four NASA Langley Research Center airborne High Spectral Resolution Lidars (HSRLs) to develop a machine learning regression methodology to infer PM2.5 concentrations at the surface and aloft. These airborne HSRL measurements were acquired over major metropolitan regions in the United States and Asia during more than 170 flights since 2010. Hourly surface PM2.5 measurements from the EPA air quality system and similar networks in other countries acquired within 10 km and 15 minutes of these near-surface HSRL measurements are used to train models that compute PM2.5 concentrations from the HSRL measurements. We examine several regression methods and find that exponential Gaussian Process algorithms consistently give the best performance in terms of the lowest root-mean-square (RMS) errors and the highest correlations. Model performance varies significantly depending on various combinations of HSRL aerosol measurements (e.g., aerosol backscatter, extinction, depolarization, backscatter color ratios, lidar ratios, aerosol optical thickness) and retrievals (e.g., mixed layer height, aerosol type) used in the regressions. Models that use near-surface measurements of aerosol backscatter and aerosol intensive properties such as depolarization, backscatter color ratio, and lidar ratio typically give the best performance with RMS errors around 4 mg/m3 and correlation coefficients above 0.9. HSRL measurements were often acquired when the aircraft flew systematic “raster-scan” patterns for several hours over these cities. These flight patterns enabled measurements of the spatial, temporal, and vertical variabilities in the distributions of aerosol backscatter and aerosol intensive properties and allowed us to derive the corresponding variabilities in PM2.5 concentrations. We present examples of such variabilities over urban areas in the United States as well as Asia. We describe also how the distribution of surface PM2.5 varies with aerosol type and use these retrievals to examine model simulations of surface PM2.5 in these metropolitan regions. We also discuss how this methodology may be applied to measurements from satellite lidars such as CALIOP on CALIPSO and ATLID on EarthCARE.

lidar↗
NASA NTRS2013

CALIOP and AERONET Aerosol Optical Depth Comparisons: One Size Fits None

We compare the aerosol optical depths (AOD) retrieved from backscatter measurements of the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) aboard the Cloud Aerosol Lidar Infrared Pathfinder Satellite Observations (CALIPSO) satellite with coincident Aerosol Robotic Network (AERONET) measurements. Overpass coincidence criteria of +/- 2 h and within a 40 km radius are satisfied at least once at 149 globally distributed AERONET sites from 2006 to 2010. Most data pairs (>80%) use AERONET measurements acquired +/- 30 min of the overpass. We examine the differences in AOD estimates between CALIOP and AERONET for various aerosol, environmental, and geographic conditions. Results show CALIOP AOD are lower than AERONET AOD especially at low optical depths as measured by AERONET (500 nm AOD<0.1). Furthermore, the median relative AOD difference between the two measurements is 25% of the AERONET AOD for AOD>0.1. Differences in AOD between CALIOP and AERONET are possibly due to cloud contamination, scene inhomogeneity, instrument view angle differences, CALIOP retrieval errors, and detection limits. Comparison of daytime to nighttime number of 5 km 60m (60m in the vertical) features detected by CALIOP show that there are 20% more aerosol features at night. We find that CALIPSO and AERONET do not agree on the cloudiness of scenes. Of the scenes that meet the above coincidence criteria, CALIPSO finds clouds in more than 45% of the coincident atmospheric columns AERONET classifies as clear.

Omar, A. H.↗
NASA NTRS1975

Optical design of the SBUV/TOMS experiment on Nimbus G

The paper examines the tradeoffs performed in optimizing the optical design of the solar backscatter ultraviolet/total ozone mapping spectrometer (SBUV/TOMS) experiment on Nimbus G to stringent performance requirements within the limitations of the spacecraft interface. The SBUV portion of the experiment incorporates a double monochromator optimized for better than 1.0 A spectral resolution over the wavelength range 1600-4000 A. The TOMS portion of the experiment is a stepped line scanning system with a 105-deg total field of view. Special techniques are used to reduce the polarization sensitivity of the instrument to less than 5% for 100% linearly polarized incident radiation and to keep the spectral stray light to less than 0.000001 of the incident solar spectrum. Optical material selection is imperative in order to minimize the effects of fluorescence and phosphorescence arising from the bombardment of particulate radiation in space.

Henderson, B. D.↗
NASA NTRSDate not supplied

Exploring Environmental and Aerosol Impacts on Maritime Tropical Convection using Airborne Radiometer, Radar, Lidar, and Dropsondes

The field deployment phase of NASA’s Cloud, Aerosol and Monsoon Processes Philippines Experiment (CAMP2Ex) took place around the Philippines during August–October 2019, with the primary goal of jointly investigating aerosols and tropical meteorology at the micro-β to meso-β scales. A suite of instruments was deployed on NASA’s P-3B Orion aircraft to accomplish this mission, including: the Advanced Microwave Precipitation Radiometer (AMPR), Airborne Precipitation and cloud Radar 3rd Generation (APR-3), High Spectral Resolution Lidar 2 (HSRL2), and Advanced Vertical Atmospheric Profiling System (AVAPS) dropsondes. To examine potential aerosol influences on maritime tropical convection, P-3 flight segments throughout CAMP2Ex were binned into similar environmental groups using “low,” “medium,” and “high” values of nine AVAPS-derived parameters with known physical connections to convective frequency and/or intensity. Aerosol concentrations in each flight segment were evaluated using three HSRL2 variables at 355 and 532 nm: aerosol backscatter, aerosol extinction, and aerosol optical thickness. A set of radiometer- and radar-derived variables directly related to convective frequency and/or intensity was used to characterize convection, which included: AMPR-derived integrated cloud liquid water; polarization-corrected temperatures at 10.7, 19.35, 37.1, and 85.5 GHz; peak equivalent radar reflectivity factor (ZH); peak height of 30-dBZ ZH; and the number of radar data columns with composite ZH > 30 dBZ. The ZH analyses were performed using both Ku- and Ka-band APR-3 data. For each flight segment, correlation coefficients were calculated between each convective parameter and aerosol concentrations within the “low,” “medium,” and “high” groups for each environmental variable. The environmental stratification thresholds were then varied in a series of sensitivity tests. Several noteworthy correlations were observed between the convective and aerosol parameters within the environmental groups, especially when stratifying the environments based on their 850–500-hPa temperature lapse rate, 700–500-hPa temperature lapse rate, and K-Index. The convective parameters were often correlated most strongly with 355-nm extinction, 532-nm extinction, and 532-nm backscatter, while the presence of precipitation-sized liquid and ice hydrometeors contributed to some unexpected negative correlations. In general, as environmental conditions became more favorable for convection, a stronger correlation was observed between the convective parameters and aerosol concentrations. However, a “Goldilocks” zone of medium aerosol concentration was correlated most strongly with the convective parameters in many cases. These results stress the importance of considering environmental and aerosol conditions together when evaluating their impacts on convection. This presentation will provide a detailed discussion of these results and their implications, a summary of the limitations associated with such an analysis, and suggestions for future work.

Corey G. Amiot↗
NASA NTRSDate not supplied

CALIPSO’s New ODCOD Product Compared to Langley’s HSRL and HSRL-2

CALIPSO’s Version 4.51 Level 2 data release introduces an all-new group of science data sets containing estimates of total column two-way transmittances and effective optical depths derived from CALIOP ocean surface backscatter measurements and MERRA-2 reanalysis wind speed data. This new data product is known as the Ocean Derived Column Optical Depth product (ODCOD). These estimates use CALIOP’s ocean surface lidar return to estimate the total column optical depth overhead. This new retrieval will be provided for the entire mission, day and night, at 532nm, and are reported at single shot, 1km, and 5km resolutions for all profiles in which a valid lidar ocean surface return is detected. This poster will present a collection of HSRL and HSRL-2 CALIPSO under flights and compare the HSRL measured aerosol optical depth with the estimated total column optical depth of ODCOD. The ODCOD algorithm uses CALIOP’s ocean surface lidar return to estimate the effective total column optical depth overhead; i.e., the single scattering optical depth reduced by the contributions of multiple scattering to the ocean surface signal. Because the retrieval generates a single estimate for the entire column based solely on the surface backscatter, there is currently no way to correct for multiple scattering effects from different kinds of features within the column. This new retrieval will be provided for the entire mission, day and night, at 532nm, and is reported at single shot, 1km, and 5km resolutions for all profiles in which a valid lidar ocean surface return is detected. This poster presents a collection of HSRL and HSRL-2 CALIPSO under-flight case studies that compare the HSRL measured aerosol optical depth with the estimated total column optical depth derived by ODCOD.

R. Ryan↗
NASA NTRS2010

Statistics of Cloud Optical Properties from Airborne Lidar Measurements

Cloud optical properties, such as extinction-to-backscatter ratio and depolarization ratio, have a significant impact on the accuracy of cloud extinction retrievals from lidar systems because parameterizations of these variables are often used in non-ideal conditions to determine cloud type and optical depth. Statistics and trends of these optical parameters were analyzed for four years, 2003-2007, of Cloud Physics Lidar data during five projects of varying geographic locations. Extinction-to-backscatter ratio (at 532 nm) was derived by calculating the transmission loss through the cloud layer, while depolarization ratio was computed using the parallel and perpendicular polarized 1064 nm channels. The majority of the cloud layers yielded an S-ratio between 10 and 40 sr with the S-ratio frequency distribution centered at 25 sr for ice clouds, 21 sr for mixed phase clouds, and 11 sr for water clouds. On average for ice clouds, S ratio slightly decreased with decreasing temperature, while depolarization ratio increased significantly as temperatures decreased. Trends for water and mixed phase clouds were also observed. Ultimately, these observed trends in optical properties as a function of temperature and geographic location will improve current parameterizations of extinction-to-backscatter ratio, which consequently increases accuracy in cloud optical depth and radiative forcing estimates.

Yorks, John E.↗
NASA NTRS2004

Subtropical Cirrus Properties Derived from GSFC Scanning Raman Lidar Measurements during CAMEX 3

The NASA/GSFC Scanning Raman Lidar (SRL) was stationed on Andros Island, Bahamas for the third Convection and Moisture Experiment (CAMEX 3) held in August - September, 1998 and acquired an extensive set of water vapor and cirrus cloud measurements (Whiteman et al., 2001). The cirrus data studied here have been segmented by generating mechanism. Distinct differences in the optical properties of the clouds are found when the cirrus are hurricane-induced versus thunderstom-induced. Relationships of cirrus cloud optical depth, mean cloud temperature, and layer mean extinction-to-backscatter ratio (S) are presented and compared with mid-latitude and tropical results. Hurricane-induced cirrus clouds are found to generally possess lower values of S than thunderstorm induced clouds. Comparison of these measurements of S are made with other studies revealing at times large differences in the measurements. Given that S is a required parameter for spacebased retrievals of cloud optical depth using backscatter lidar, these large diffaences in S measurements present difficulties for space-based retrievals of cirrus cloud extinction and optical depth.

Whiteman, D. N.↗
DOE OSTI2023

Implementation and experimental validation of nonlocal damage in a large-strain elasto-viscoplastic FFT-based framework for predicting ductile fracture in 3D polycrystalline materials

Ductile materials, such as metal alloys, can undergo substantial deformation before failure. Additionally, these materials are usually of polycrystalline composition and exhibit strongly anisotropic behavior at small length scales. Previously developed fast Fourier transform (FFT)-based models can model ductile fracture of isotropic materials or the elastic–plastic behavior of anisotropic polycrystalline materials; however, there remains a need to couple both capabilities. This work extends a large-strain FFT-based crystal plasticity model to simulate ductile fracture of polycrystalline materials. In this work, a triaxiality-based continuum damage mechanics (CDM) formulation is incorporated into a large-strain elasto-viscoplastic FFT (LS-EVPFFT) framework. The CDM formulation is augmented with an integral-based nonlocal regularization approach that correctly handles gas-phase material necessary to model unconstrained surfaces. To validate the damage-enabled LS-EVPFFT framework, mesoscale copper tensile coupons were machined using microwire electrical discharge machining and experimentally characterized using electron backscatter diffraction. In-situ optical digital image correlation was performed during uniaxial testing to provide a side-by-side comparison of the experimental and computational strain fields and stress–strain responses. The damage-enabled LS-EVPFFT framework can simulate the complete macroscopic stress–strain response of ductile polycrystals to failure. The model reproduces necking behavior that qualitatively agrees with experimental observations. By leveraging the relatively low computational cost of the damage-enabled LS-EVPFFT framework, the framework presented here allows the ductile fracture response of 3D polycrystalline materials to be tractably predicted.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Spall and subsequent recompaction of copper under shock loading

Research was undertaken to study spall and subsequent recompaction of oxygen-free high-thermal-conductivity copper using a single-stage large-bore light gas gun capable of planar impacts. Gun experiments were conducted that produced an initial spall in the target with a subsequent recompaction of the spall damage/layer by the use of layered impactors. Symmetric spall experiments at similar conditions were also conducted as a control to the recompaction experiments. Photonic Doppler velocimetry was used to obtain the velocity history of the target’s back surface; these velocity histories were analyzed, and the results were compared to numerical simulations. After recovery of selected samples, the microstructure was analyzed using optical imaging microscopy and electron backscatter diffraction. Recompaction waves were clearly observed in the time-resolved data obtained at the back surface of the targets. Two different series of experiments were performed to understand the effect of damage morphology on the stress required for spall recompaction. In the initial series, the peak pressure of the first shock was systematically increased to alter the amount of damage in the material. While in the second series, the peak pressure of the second shock was increased, keeping the magnitude of the first shock relatively constant to understand the effect of peak stress on the recompaction process. Findings clearly show that recompaction results in a perturbed band of the microstructure at the location of the expected spall plane in all cases except where the peak stress of the second shock is lower than the critical value.

, recompaction↗
NASA NTRS1978

Correlation of laser velocimeter measurements over a wing with results of two prediction techniques

The flow field at the center line of an unswept wing with an aspect ratio of eight was determined using a two dimensional viscous flow prediction technique for the flow field calculation, and a three dimensional potential flow panel method to evaluate the degree of two dimensionality achieved at the wing center line. The analysis was made to provide an acceptable reference for comparison with velocity measurements obtained from a fringe type laser velocimeter optics systems operating in the backscatter mode in the Langley V/STOL tunnel. Good agreement between laser velocimeter measurements and theoretical results indicate that both methods provide a true representation of the velocity field about the wing at angles of attack of 0.6 and 4.75 deg.

Hoad, D. R.↗
NASA NTRS2014

A-Train Aerosol Observations Preliminary Comparisons with AeroCom Models and Pathways to Observationally Based All-Sky Estimates

We have developed a technique for combining CALIOP aerosol backscatter, MODIS spectral AOD (aerosol optical depth), and OMI AAOD (absorption aerosol optical depth) retrievals for the purpose of estimating full spectral sets of aerosol radiative properties, and ultimately for calculating the 3-D distribution of direct aerosol radiative forcing. We present results using one year of data collected in 2007 and show comparisons of the aerosol radiative property estimates to collocated AERONET retrievals. Use of the recently released MODIS Collection 6 data for aerosol optical depths derived with the dark target and deep blue algorithms has extended the coverage of the multi-sensor estimates towards higher latitudes. We compare the spatio-temporal distribution of our multi-sensor aerosol retrievals and calculations of seasonal clear-sky aerosol radiative forcing based on the aerosol retrievals to values derived from four models that participated in the latest AeroCom model intercomparison initiative. We find significant inter-model differences, in particular for the aerosol single scattering albedo, which can be evaluated using the multi-sensor A-Train retrievals. We discuss the major challenges that exist in extending our clear-sky results to all-sky conditions. On the basis of comparisons to suborbital measurements, we present some of the limitations of the MODIS and CALIOP retrievals in the presence of adjacent or underlying clouds. Strategies for meeting these challenges are discussed.

Aerosol↗
NASA NTRS2014

Direct Aerosol Radiative Forcing Based on Combined A-Train Observations: Towards All-sky Estimates and Attribution to Aerosol Type

We describe a technique for combining CALIOP aerosol backscatter, MODIS spectral AOD (aerosol optical depth), and OMI AAOD (absorption aerosol optical depth) measurements for the purpose of estimating full spectral sets of aerosol radiative properties, and ultimately for calculating the 3-D distribution of direct aerosol radiative forcing. We present results using one year of data collected in 2007 and show comparisons of the aerosol radiative property estimates to collocated AERONET retrievals. Initial calculations of seasonal clear-sky aerosol radiative forcing based on our multi-sensor aerosol retrievals compare well with over-ocean and top of the atmosphere IPCC-2007 model-based results, and with more recent assessments in the "Climate Change Science Program Report: Atmospheric Aerosol Properties and Climate Impacts" (2009). We discuss some of the challenges that exist in extending our clear-sky results to all-sky conditions. On the basis of comparisons to suborbital measurements, we present some of the limitations of the MODIS and CALIOP retrievals in the presence of adjacent or underlying clouds. Strategies for meeting these challenges are discussed. We also discuss a methodology for using the multi-sensor aerosol retrievals for aerosol type classification based on advanced clustering techniques. The combination of research results permits conclusions regarding the attribution of aerosol radiative forcing to aerosol type.

AOD↗