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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 181 records · Page 10
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

An Optically Discovered Outburst from XTE J1859+226

Abstract Using the Zwicky Transient Facility, in 2021 February we identified the first known outburst of the black hole X-ray transient XTE J1859+226 since its discovery in 1999. The outburst was visible at X-ray, UV, and optical wavelengths for less than 20 days, substantially shorter than its full outburst of 320 days in 1999, and the observed peak luminosity was 2 orders of magnitude lower. Its peak bolometric luminosity was only 2 × 10 35 erg s −1 , implying an Eddington fraction of about 3 × 10 −4 . The source remained in the hard spectral state throughout the outburst. From optical spectroscopy measurements we estimate an outer disk radius of 10 11 cm. The low observed X-ray luminosity is not sufficient to irradiate the entire disk, but we observe a surprising exponential decline in the X-ray light curve. These observations highlight the potential of optical and infrared synoptic surveys to discover low-luminosity activity from X-ray transients.

Astronomy & Astrophysics↗
DOE OSTI2022

Expediting DECam Multimessenger Counterpart Searches with Convolutional Neural Networks

Searches for counterparts to multimessenger events with optical imagers use difference imaging to detect new transient sources. However, even with existing artifact-detection algorithms, this process simultaneously returns several classes of false positives: false detections from poor-quality image subtractions, false detections from low signal-to-noise images, and detections of preexisting variable sources. Currently, human visual inspection to remove the false positives is a central part of multimessenger follow-up observations, but when next generation gravitational wave and neutrino detectors come online and increase the rate of multimessenger events, the visual inspection process will be prohibitively expensive. We approach this problem with two convolutional neural networks operating on the difference imaging outputs. The first network focuses on removing false detections and demonstrates an accuracy of 92% on our data set. The second network focuses on sorting all real detections by the probability of being a transient source within a host galaxy and distinguishes between various classes of images that previously required additional human inspection. We find the number of images requiring human inspection will decrease by a factor of 1.5 using our approach alone and a factor of 3.6 using our approach in combination with existing algorithms, facilitating rapid multimessenger counterpart identification by the astronomical community.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2025

The ambiguous AT2022rze: changing-look AGN mimicking a supernova in a merging galaxy system

AT2022rze is a luminous, ambiguous transient located south-east of the geometric centre of its host galaxy at redshift $z = 0.08$. The host appears to be formed by a merging galaxy system. The observed characteristics of AT2022rze are reminiscent of active galactic nuclei (AGNs), tidal disruption events, and superluminous supernovae. The transient reached a peak absolute magnitude of $-$20.2 $\pm$ 0.2 mag, showing a sharp rise (t$_{\mathrm{rise,1/e}} = 27.5 \pm 0.6$ d) followed by a slow decline (t$_{\mathrm{dec,1/e}} = 382.9 \pm 0.6$). Its bumpy light curve and narrow Balmer lines indicate the presence of gas (and dust). Its light curve shows rather red colours, indicating that the transient could be affected by significant host extinction. The spectra reveal coronal lines, indicative of high-energy (X-ray/UV) emission. Archival data reveal no prior activity at this location, disfavouring a steady-state AGN, although an optical spectrum obtained prior to the transient is consistent with an AGN classification of the host. Based on this, we conclude that the transient most likely represents a changing-look AGN at the centre of the smallest component of the merging system.

galaxies: active↗
DOE OSTI2022

Light-induced Weyl semiconductor-to-metal transition mediated by Peierls instability

Elemental tellurium is a strongly spin-orbit coupled Peierls-distorted semiconductor whose band structure features topologically protected Weyl nodes. Here, using time-dependent density functional theory calculations, we show that impulsive optical excitation can be used to transiently control the amplitude of the Peierls distortion, realizing a mechanism to switch tellurium between three states: Weyl semiconductor, Weyl metal and non-Weyl metal. Further, we present experimental evidence of this inverse-Peierls distortion using time-resolved optical second harmonic generation measurements. These results provide a pathway to multifunctional ultrafast Weyl devices and introduce Peierls systems as viable hosts of light-induced topological transitions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

Adapting DESGW Single Epoch Image Differencing to the LSST Software Stack

As gravitational wave detections become an ever-increasing part of cosmological research, the Gravitational Waves Group of the Dark Energy Survey (DESGW) seeks to match and interpret optical observations for these short-lived, transient events.[1]To provide timely analysis for each follow up, DESGW has developed a custom Single Epoch Differencing Pipeline for processing optical data obtained from the Dark Energy Camera (DECam).[2]While effective, the pipeline is a custom design and thus requires extra maintenance and specialized knowledge to operate and modify at a time when new projects are taking precedence.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

SOAR/Goodman Spectroscopic Assessment of Candidate Counterparts of the LIGO/Virgo Event GW190814*

On 2019 August 14 at 21:10:39 UTC, the LIGO/Virgo Collaboration (LVC) detected a possible neutron star–black hole merger (NSBH), the first ever identified. An extensive search for an optical counterpart of this event, designated GW190814, was undertaken using the Dark Energy Camera on the 4 m Victor M. Blanco Telescope at the Cerro Tololo Inter-American Observatory. Target of Opportunity interrupts were issued on eight separate nights to observe 11 candidates using the 4.1 m Southern Astrophysical Research (SOAR) telescope’s Goodman High Throughput Spectrograph in order to assess whether any of these transients was likely to be an optical counterpart of the possible NSBH merger. Here, we describe the process of observing with SOAR, the analysis of our spectra, our spectroscopic typing methodology, and our resultant conclusion that none of the candidates corresponded to the gravitational wave merger event but were all instead other transients. Finally, we describe the lessons learned from this effort. Application of these lessons will be critical for a successful community spectroscopic follow-up program for LVC observing run 4 (O4) and beyond.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Excitonic Dynamics in Janus MoSSe and WSSe Monolayers

We report here details of steady-state and time-resolved spectroscopy of excitonic dynamics for Janus transition metal dichalcogenide monolayers, including MoSSe and WSSe, which were synthesized by low-energy implantation of Se into transition metal disulfides. Absorbance and photoluminescence spectroscopic measurements determined the room-temperature exciton resonances for MoSSe and WSSe monolayers. Transient absorption measurements revealed that the excitons in Janus structures form faster than those in pristine transition metal dichalcogenides by about 30% due to their enhanced electron–phonon interaction by the built-in dipole moment. Here, by combining steady-state photoluminescence quantum yield and time-resolved transient absorption measurements, we find that the exciton radiative recombination lifetime in Janus structures is significantly longer than in their pristine samples, supporting the predicted spatial separation of the electron and hole wave functions due to the built-in dipole moment. These results provide fundamental insight in the optical properties of Janus transition metal dichalcogenides.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Ultrafast dynamics of CN radical reactions with chloroform solvent under vibrational strong coupling

Polariton chemistry may provide a new means to control molecular reactivity, permitting remote, reversible modification of reaction energetics, kinetics, and product yields. A considerable body of experimental and theoretical work has already demonstrated that strong coupling between a molecular vibrational mode and the confined electromagnetic field of an optical cavity can alter chemical reactivity without external illumination. However, the mechanisms underlying cavity-altered chemistry remain unclear in large part because the experimental systems examined previously are too complex for detailed analysis of their reaction dynamics. Here, we experimentally investigate photolysis-induced reactions of cyanide radicals with strongly-coupled chloroform (CHCl 3 ) solvent molecules and examine the intracavity rates of photofragment recombination, solvent complexation, and hydrogen abstraction. Here we use a microfluidic optical cavity fitted with dichroic mirrors to facilitate vibrational strong coupling (VSC) of the C–H stretching mode of CHCl 3 while simultaneously permitting optical access at visible wavelengths. Ultrafast transient absorption experiments performed with cavities tuned on- and off-resonance reveal that VSC of the CHCl 3 C–H stretching transition does not significantly modify any measured rate constants, including those associated with the hydrogen abstraction reaction. This work represents, to the best of our knowledge, the first experimental study of an elementary bimolecular reaction under VSC. We discuss how the conspicuous absence of cavity-altered effects in this system may provide insights into the mechanisms of modified ground state reactivity under VSC and help bridge the divide between experimental results and theoretical predictions in vibrational polariton chemistry.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2026

Hot-Carrier Photoluminescence in Low-Temperature CsSnI3 Nanocrystals

In the halide perovskites, the B-site metal lone-pairs electrons are strongly suspected to underpin many of the interesting properties of the inorganic halide perovskites. Recently, a stable low-temperature monoclinic polar phase was predicted for CsSnI3, opening the possibility of direct investigation of both these lone pair electrons and a ferroelectric distorted structure. To date there are no other reports of such a structure in CsSnI3, and a known low-temperature monoclinic structure in CsSnBr3 remains unexplored. We have found optical evidence of a transformation occurring around 240 K in CsSnI3 nanocrystals, with several changes in optical behavior below this transition point, including novel high-energy photoluminescene and new states in the transient absorption spectrum. We have successfully characterized the optical properties of this low-temperature phase and found evidence for a polar, monoclinic structure. Discovery of a stable monoclinic polar structure in the halide perovskites opens many new potential directions for further research and electronics applications.

14 SOLAR ENERGY↗
DOE OSTI2020

Light-Induced Renormalization of the Dirac Quasiparticles in the Nodal-Line Semimetal ZrSiSe

In nodal-line semimetals, linearly dispersing states form Dirac loops in the reciprocal space with a high degree of electron-hole symmetry and a reduced density of states near the Fermi level. The result is reduced electronic screening and enhanced correlations between Dirac quasiparticles. In this study we investigate the electronic structure of ZrSiSe, by combining time- and angle-resolved photoelectron spectroscopy with ab initio density functional theory (DFT) complemented by an extended Hubbard model ( DFT + U + V ) and by time-dependent DFT + U + V . We show that electronic correlations are reduced on an ultrashort timescale by optical excitation of high-energy electrons-hole pairs, which transiently screen the Coulomb interaction. Our findings demonstrate an all-optical method for engineering the band structure of a quantum material.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2025

The Dynamical Role of Optical Phonons and Sublattice Screening in a Solid-State Ion Conductor

Solid-state electrolytes (SSEs) require ionic conductivities that are competitive with liquid electrolytes to realize applications in all-solid-state batteries. Although candidate SSEs have been discovered, the underlying mechanisms enabling superionic conduction (>1 mS cm –1 ) remain elusive. In particular, the role of ultrafast lattice dynamics in mediating ion migration, which involves couplings between ions, phonons, and electrons, is rarely explored experimentally at their corresponding time scales. To investigate the complex contributions of coupled lattice dynamics on ion migration, we modulate the charge density occupations within the crystal framework and then measure the time-resolved change in impedance on picosecond time scales for a candidate SSE, Li 0.5 La 0.5 TiO 3 (LLTO). Upon perturbation, we observe enhanced ion migration at ultrafast time scales. The respective transients match the time scales of optical and acoustic phonon vibrations, suggesting their involvement in ion migration. We further computationally evaluate the effect of a charge transfer from the O 2p to the Ti 3d band on the electronic and physical structure of LLTO. We hypothesize that the charge-transfer excitation distorts the TiO 6 polyhedra by altering the local charge density occupancy of the hopping site at the migration pathway saddle point, thereby causing a reduction in the migration barrier for the Li + hop. We rule out the contribution of photogenerated electron carriers and laser heating. Overall, our investigation introduces a new spectroscopic tool to probe fundamental ion hopping mechanisms transiently at ultrafast time scales, which has previously only been achieved in a time-averaged manner or solely via computational methods.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

In-Cell Deployment and First Use of Digital Image Correlation for In-Situ Strain Analysis of Irradiated Nuclear Fuel Rods During LOCA Transient

Digital image correlation (DIC) is a noncontact, optical method increasingly used across industries and research environments for acquiring multidimensional strain data. At Oak Ridge National Laboratory’s (ORNL’s) Severe Accident Test Station (SATS), DIC has been extensively applied to study the thermomechanical response of nuclear fuel claddings, yielding fundamental insights into material behavior. However, these efforts have focused exclusively on unirradiated materials and relied on the SATS out-of-cell infrastructure. Efforts over the past two years have been made to extend these capabilities to ORNL’s Irradiated Fuels Examination Laboratory SATS system within the hot-cells to enable testing of irradiated fuel cladding materials. Integrating DIC into the hot-cell SATS infrastructure presents unique challenges, including enabling remote operation of optical equipment and adapting auxiliary hot-cell systems for DIC implementation. This report discusses design, stand-up testing, and application of DIC to an irradiated nuclear fuel cladding segment. A DIC testing rig was successfully built and validated out-of-cell through extensive surrogate tests and calibrations. The rig and specialized DIC furnace were installed in the hot-cell, and a DIC test was successfully conducted. Results from that test correspond to expectations for Zr-based alloys and showed similar uncertainties compared to out-of-cell tests.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2021

Combined Optical and Radio-Frequency Perspectives on a Hybrid Cloud-To-Ground Lightning Flash Observed by the FORTE Satellite

In this work, we use the coincident optical and radio-frequency (RF) measurements taken by the Fast On-orbit Recording of Transient Events (FORTE) satellite to shed light on common optical signatures recorded by NASA and NOAA lightning imagers during Cloud-to-Ground (CG) lightning. We build flash cluster data for FORTE using the same techniques as the NASA/NOAA instruments to document the optical/RF evolution of an oceanic hybrid -CG flash. The flash began with strong Very High Frequency (VHF)-band emission from a Narrow Bipolar Event (NBE) that initiated a period of normal bilevel intracloud (IC) activity in two vertical layers (8 and 12 km) that lasted for 490 ms. VHF waveforms show step leader activity ahead of the return stroke. All impulsive VHF sources after the stroke come from the lower (8 km) layer. K-changes are noted following the return stroke, but no subsequent strokes are detected. The optical flash began 136 ms after the NBE RF pulse. Twenty-two of the 33 optical groups were dim and occurred during the in-cloud phase of the flash. This activity included both isolated pulses and sustained periods of illumination over tens of milliseconds. Initial cloud pulses accounted for 23% of the total optical radiance from the flash. Illumination during the return stroke contributed 58% of the total radiance, and the K-changes and cloud pulses after the stroke supplied the remaining 19%. These results highlight the benefit of having RF alongside optical lightning measurements for clarifying signatures in the optical data and providing information on their physical origins.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

The Illumination of Thunderclouds by Lightning: 1. The Extent and Altitude of Optical Lightning Sources

Abstract Optical space‐based lightning sensors including NOAA's Geostationary Lightning Mapper (GLM) detect lightning though its transient illumination of the surrounding clouds. What space‐based optical lightning sensors measure is influenced by the physical attributes of the light source, the location of the source within the cloud scene, and the spatial variations in cloud composition. We focus on the lightning channels that serve as optical sources for GLM groups and flashes in this first part of our thundercloud illumination study. We match Lightning Mapping Array (LMA) sources with GLM groups and flashes during two thunderstorms to examine channel segments that are active during optical emission. We find that in each storm, the LMA sources matched with GLM groups are small (median: 3 km) compared to GLM pixels (nominal: 8 km), and preferentially come from high altitudes in the cloud (>8–10 km). The detection advantage for high‐altitude sources permits GLM to resolve faint optical pulses near the cloud top that might be missed from lower altitudes. However, the most energetic groups can be detected from all altitudes, and the largest groups largely originate at low altitudes. The relationship between group energy and illuminated area depends on flash development within the cloud medium, and flash development into different cloud regions can be identified by tracking GLM metrics of cloud illumination over time.

58 GEOSCIENCES↗
DOE OSTI2023

Short Communication: Observation of Initial Burst Release of Fission Gas from High-Burnup UO 2 Nuclear Fuel During Thermal Transient

A system was developed and tested to provide a deeper understanding of the fission gas release kinetics from nuclear fuel during thermal transients. Pressure, temperature, spectral data, and optical images were simultaneously collected during resistive sample heating, and all released gases were collected in liquid nitrogen-cooled charcoal traps. Standup testing was performed with a high-burnup nuclear fuel segment from rod section with an average local burnup of 77 GWd/tU. During heating, the segment released approximately 6 ± 2% of generated fission gas inventory after ramp heating to 460°C. Here, heating ceased when the sample ejected from the holder, as observed by constant imaging.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2021

Holes in Optical Lightning Flashes: Identifying Poorly Transmissive Clouds in Lightning Imager Data

Space-based optical lightning sensors including the lightning imaging sensor (LIS) and geostationary lightning mapper (GLM) are pixelated imagers that detect lightning as transient increases in cloud top illumination. Detection requires optical emissions to escape the cloud top to space with sufficient energy to trigger a pixel on the imaging array. Through scattering and absorption, certain clouds are able to block most light from reaching the instrument, causing a reduction in detection efficiency (DE) and possibly location accuracy (LA). Radiant lightning emissions that illuminate large cloud top areas are used to examine scenarios where clouds block light from reaching orbit. In some cases, these anomalies in the spatial radiance distribution from the lightning pulse lead to “holes” in the optical lightning flash where certain pixels fail to trigger. Such holes are identified algorithmically in the Tropical Rainfall Measuring Mission satellite LIS record and the microphysical properties of the coincident storm region are queried. We find that holes primarily occur in tall (IR T b < 235 K) convection (87%) and overhanging anvil clouds (10%). The remaining 3% of holes occur in moderate-to-weak convection or in clear air breaks between stormclouds. We further demonstrate how an algorithm that assesses the spatial radiance patterns from energetic lightning pulses might be used to construct an optical transmission gridded stoplight product for GLM that could help operators identify clouds with a potentially reduced DE and LA.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Dual-pace transient heat conduction in vertically aligned carbon nanotube arrays induced by structure separation

Vertically aligned arrays of carbon nanotubes (CNTs) are attractive for a wide range of macroscopic applications which can exploit the remarkable properties of individual nanotubes. In this work, an abnormal behavior of CNT bundles in heat conduction is discovered under the transient electro-thermal characterization. The measured voltage change over the sample shows a dual-pace thermal response (DTR), which could not be fitted using a single thermal diffusivity heat transfer model. Instead, two thermal diffusivities are determined from the DTR phenomenon. Three rounds of cryogenic experiments are conducted to investigate the physics behind DTR phenomenon. It starts to emerge when the temperature is reduced to a certain level. After two rounds of cryogenic experiments, the DTR phenomenon becomes permanent from 295 K to 10 K. The nano-scale structure separation induced by the increased thermal strain leads to macroscale structure separation, which results in two parallel heat conduction paths responsible for the DTR phenomenon. By building a new parallel heat transfer model taking both the transient and steady-state electrical and thermal response into consideration, the area ratio of separated CNTs is determined. Furthermore, this result uncovers the existence of coiled morphology and nano-structure evolution of CNTs under cryogenic state and its effect on thermal and electrical transport, especially on their transient behaviors. Knowledge of the thermal transport in these CNTs arrays is important considering the fact that transient thermal response strongly affects their mechanical, optical, and electrical behaviors.

42 ENGINEERING↗
DOE OSTI2024

Deep drilling in the time domain with DECam – II: characterizing the light curves of candidates in the extragalactic fields

ABSTRACT In this second paper on the DECam deep-drilling field (DDF) program, we release 2020 optical $gri$-band light curves for transients and variables in the extragalactic COSMOS and ELAIS fields based on time series observations with a 3-d cadence from semester 2021A through 2023A. In order to demonstrate the wide variety of time domain events detected by the program and encourage others to use the data set, we characterize the sample by presenting a brief analysis of the light-curve parameters such as time span, amplitude, and peak brightness. We also present preliminary light-curve categorizations, and identify potential stellar variables, active galactic nuclei, tidal disruption events, supernovae (SNe) (such as Type Ia, Type IIP, superluminous, and gravitationally lensed SNe), and fast transients. Where relevant, the number of identified transients is compared to the predictions of the original proposal. We also discuss the challenges of analyzing DDF data in the context of the upcoming Vera C. Rubin Observatory and its Legacy Survey of Space and Time, which will include DDFs. Images from the Dark Energy Camera DDF program are available without proprietary period and the light curves presented in this work are publicly available for analysis.

Graham, Melissa L. (ORCID:0000000291543136)↗