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At least 181 records · Page 10

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NASA NTRS2012

Diagnostic modeling of dimethylsulfide production in coastal water west of the Antarctic Peninsula

The rate of gross biological dimethylsulfide (DMS) production at two coastal sites west of the Antarctic Peninsula, off Anvers Island, near Palmer Station, was estimated using a diagnostic approach that combined field measurements from 1 January 2006 through 1 March 2006 and a one-dimensional physical model of ocean mixing. The average DMS production rate in the upper water column (0-60 m) was estimated to be 3.1 +/- 0.6 nM/d at station B (closer to shore) and 2.7 +/- 0.6 nM/d1 at station E (further from shore). The estimated DMS replacement time was on the order of 1 d at both stations. DMS production was greater in the mixed layer than it was below the mixed layer. The average DMS production normalized to chlorophyll was 0.5 +/- nM/d)/(mg cubic m) at station B and 0.7 +/- 0.2 (nM/d)/(mg/cubic m3) at station E. When the diagnosed production rates were normalized to the observed concentrations of total dimethylsulfoniopropionate (DMSPt, the biogenic precursor of DMS), we found a remarkable similarity between our estimates at stations B and E (0.06 +/- 0.02 and 0.04 +/- 0.01 (nM DMS / d1)/(nM DMSP), respectively) and the results obtained in a previous study from a contrasting biogeochemical environment in the North Atlantic subtropical gyre (0.047 =/- 0.006 and 0.087 +/- 0.014 (nM DMS d1)/(nM DMSP) in a cyclonic and anticyclonic eddy, respectively).We propose that gross biological DMS production normalized to DMSPt might be relatively independent of the biogeochemical environment, and place our average estimate at 0.06 +/- 0.01 (nM DMS / d)/(nM DMSPt). The significance of this finding is that it can provide a means to use DMSPt measurements to extrapolate gross biological DMS production, which is extremely difficult to measure experimentally under realistic in situ conditions.

Dimethylsulfide↗

DOE OSTI2024

Approaches for Autonomous Peer to Peer Communication: For Resilient Community Microgrids

The final phase of the Islandable Communications task of the SECURE project consisted of integrating the islandable communications network into a microgrid simulation at NREL. Initially integration was planned for a microgrid implemented as a mix of simulation and physical hardware. As the project evolved, the microgrid became fully simulated. The simulation environment was structured to break out the communication paths that would pass over a communication network in a field demonstration. The Islandable Communication network was integrated into the simulation environment, allowing both a commercial cellular carrier and a Private LTE network to be evaluated. The microgrid simulation showed differences in performance and behavior when operating over the wireless networks (compared to operating over wired Ethernet in the lab). These differences point to further research opportunities to better understand how microgrid communication carried over real-world or impaired networks affects the microgrid system behavior.

24 POWER TRANSMISSION AND DISTRIBUTION↗

DOE OSTI2020

Studies on the Encapsulation of Brine Generated from a Process Using Selective Electrodialysis Reversal

This topical report summarizes the laboratory testing, geochemical modeling, and mineralogical testing conducted to examine the efficacy of wastewater encapsulation for the brine generated from the Saltworks Flex electrodialysis reversal technology. Within the laboratory testing, the short- and long-term physical properties of seven separate mix designs were examined along with the leaching of each mix design. Additionally, geochemical thermodynamic modeling was used along with mineralogical analyses to help gain a fundamental understanding of the chemistry involved in the encapsulation process. Encapsulation is a process that results in the immobilization of constituents of interest by creating an engineered material that contains the waste within its matrix, both physically and chemically, in such a manner that the receiving environment is protected from adverse effects. Within the context of this study, encapsulation mix designs involved mixing the Saltworks brine with fly ash and various additives, principally lime (calcium oxide) and cement, to form a paste that eventually sets and hardens into a monolith upon placement in a landfill. Moisture conditioning fly ash with wastewater sources for on-site landfill disposal is a process that is in use at some sites and has been presented as a viable option to dispose of liquid wastes. However, because chemical reactions that can lead to sequestration of constituents of interest are not optimized, leaching can occur. Therefore, in this study, mixes were created to mimic moisture conditioning, as well as engineered pastes of varying mix designs. The study found that engineered encapsulation mixes provide significant resistance to leaching compared to moisture conditioning alone. The best performing encapsulation mix used lime as the additive, which proved superior to the use of cement. After 90 days of curing, this encapsulated mix was 5.5 times stronger than the moisture conditioned mix. Additionally, this mix exhibited an approximate 2.5 order of magnitude drop in hydraulic conductivity compared to the moisture conditioned mix. When comparing leaching, nearly all the chloride was found to evolve from the moisture conditioned mix, whereas only 6.7% of the chlorine contained in the best performing encapsulated mix leached out. Mineralogical analysis via X-ray diffraction (XRD) showed a significant concentration of the chloride sequestering mineral, Friedel’s salt, in the best performing encapsulation mix, whereas none was observed in the moisture conditioned mix, pointing to it being the primary chemical mechanism for chloride retention, along with the physical impermeability of the material. With respect to the modeling study, the model was successful in predicting the presence of most mineral phases observed in the XRD analysis.

01 COAL, LIGNITE, AND PEAT↗

DOE OSTI2026

Review of Particle Physics

The Review summarizes much of particle physics and cosmology. Using data from previous editions, plus 3,200 new measurements from 903 papers, we list, evaluate, and average measured properties of gauge bosons and the recently discovered Higgs boson, leptons, quarks, mesons, and baryons. We summarize searches for hypothetical particles such as supersymmetric particles, heavy bosons, axions, dark photons, etc. Particle properties and search limits are listed in Summary Tables. We give numerous tables, figures, formulae, and reviews of topics such as Higgs Boson Physics, Supersymmetry, Grand Unified Theories, Neutrino Mixing, Dark Energy, Dark Matter, Cosmology, Particle Detectors, Colliders, Probability and Statistics. Most of the 118 reviews are updated, including many that are heavily revised.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2021

Use of kaolinite clays in development of a low carbon MgO-clay binder system

Magnesium oxide based cements may provide a promising alternative to the conventional Portland cement in many applications. This study investigates the feasibility of using calcined kaolinitic clay to produce an MgO binder. The MgO-based binder were prepared using a low kaolinite content clay and metakaolin and were compared with a silica fume system. Implications of the addition of magnesium carbonate in the binder were also investigated. Isothermal calorimetry, X-ray diffraction (XRD), thermogravimetric analysis (TGA) and Fourier transform infrared spectroscopy (FTIR) were used to study the hydration characteristics of the binder system whereas compressive strength and porosity were measured to determine mechanical and durability attributes. The economic and environmental aspects of the binder system is also discussed. Hydrotalcite like phases were clearly produced on hydration in the clay mixes containing carbonate additions. The compressive strength of clay mixes was at par or better compared to systems containing silica fume, and the clay systems had significantly lower porosity levels. The presence of magnesium carbonate further enhanced the physical properties of the clay mixes.

36 MATERIALS SCIENCE↗

NASA NTRS1971

Zero-gravity transient thermal mixing simulation

The experimental program described is an outgrowth of independent investigations into alternate redesign concepts for the Apollo SM cryogenic oxygen storage system. The experiments were continued, after the redesign was established, to provide physical insight into transient thermal mixing in zero-gravity and to aid in the characterization of the system performance in flight. Zero-gravity heat transfer and fluid mixing were simulated experimentally through an analogy between unsteady heat conduction and species diffusion. To further support numerical analyses of the cryogenic oxygen storage system, the experimental investigation was extended to include a cubical tank geometry, representative of existing numerical models. In general, the transient flow patterns in the cubical tank are far more complex than those of the spherical tank and the extent of fluid mixing is significantly greater but less repeatable.

Lands, J. F., Jr.↗

DOE OSTI2022

Origins of magnetic memory and strong exchange bias bordering magnetic compensation in mixed-lanthanide systems

Here, the unexpected physical phenomena resulting from the seemingly inconsequential substitutions of chemically similar lanthanide elements in the Pr 1-x Gd x ScGe system are exploited to further the understanding of rare-earth magnetism and inform materials design. By directly probing magnetic moments of crystallographically indistinguishable Pr and Gd we solve the puzzles of how an unusual magnetic memory and strong exchange bias emerge at specific, easily predictable chemistries. Both effects are rooted in a robust antiparallel arrangement of large 4f magnetic moments of light and heavy lanthanides. This enables precise control of nearly zero net magnetization either opposed to, or aligned with, the external magnetic field that persists over a wide range of temperatures and fields. Further, spontaneous perturbations in the random distribution of lanthanide ions makes strong exchange bias possible in bulk single-phase compounds bordering magnetic compensation, consequently expanding the materials base beyond artificial magnetic multilayers and broadening the range of potential applications of the phenomenon.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

NASA NTRS1976

Magnetohydrodynamic and gasdynamic aspects of solar-wind flow around terrestrial planets: A critical review

Problems in space physics are discussed whose models, in simplified form, reduce to a supersonic flow scheme with a detached shock wave, namely: (1) solar wind interaction with an intrinsic planetary magnetic field; (2) solar wind interaction with the ionized component of the atmosphere of a comet; and (3) solar wind interaction with the ionosphere of a planet which does not possess its own magnetic field. The numerical study of the above problems is performed with the use of magnetogasdynamic equations for an ideal single fluid model. From the physical veiwpoint, the problems are solved in terms of as simple phenomena as possible; the principal objective is to make recently developed methods of numerical analysis of mixed flows applicable to space physics problems.

Spreiter, J. R.↗

NASA NTRS1989

Idealized model for stratocumulus cloud layer thickness

Equilibrium solutions are constructed using an idealized model for mixed and partially mixed boundary layers to show the dependence of the equilibrium cloud layer thickness on different physical processes. The condition when a mixed layer becomes cloud-free is reduced to a comparison between three pressure scales, associated with the surface wind and divergence, the radiative cooling and the subsaturation of the entrained air. The evaporation of layer cloud by cloud-top mixing is also formulated in terms of simple pressure scales.

Betts, Alan K.↗

NASA NTRS1999

Physical Parameters of Hot Horizontal-Branch Stars in NGC 6752: Deep Mixing and Radiative Levitation

Atmospheric parameters (T(sub eff), log g and log n(sub He)/n(sub H-dot)) are derived for 42 hot horizontal branch (HB) stars in the globular cluster NGC 6752. For 19 stars Mg II and Fe II lines are detected indicating an iron enrichment by a factor 50 on average with respect to the cluster abundance whereas the magnesium abundances are consistent with the cluster metallicity. This finding adds to the growing evidence that radiative levitation plays a significant role in determining the physical parameters of blue HB stars. Indeed, we find that iron enrichment can explain part, but not all, of the problem of anomalously low gravities along the blue HB. Thus the physical parameters of horizontal branch stars hotter than about 11,500 K in NGC 6752, as derived in this paper, are best explained by a combination of helium mixing and radiative levitation effects.

Moehler, S.↗

NASA NTRS1984

Assessment of technologies for classification of mixed pixels

A new method of directly classifying mixed pixels is described. This method and four frequently used indirect mixed pixel classification techniques are evaluated on Landsat MSS data from the U.S. Corn Belt using an automatic corn and soybean labeling technique. The results indicate that while more sophisticated, physically-based techniques for classsifying mixed pixels may yield a higher Percent Correct Classification (PCC) for those pixels, the net effect on a crop area proportion estimation procedure may be negative.

Metzler, M. D.↗

DOE OSTI2021

Neural network-based order parameter for phase transitions and its applications in high-entropy alloys

Phase transition is one of the most important phenomena in nature and plays a central role in materials design. All phase transitions are characterized by suitable order parameters, including the order–disorder phase transition. However, finding a representative order parameter for complex systems is non-trivial, such as for high-entropy alloys. Given the strength of dimensionality reduction of a variational autoencoder (VAE), we introduce a VAE-based order parameter. Here, we propose that the Manhattan distance in the VAE latent space can serve as a generic order parameter for order–disorder phase transitions. The physical properties of our order parameter are quantitatively interpreted and demonstrated by multiple refractory high-entropy alloys. Using this order parameter, a generally applicable alloy design concept is proposed by mimicking the natural mixing process of elements. Our physically interpretable VAE-based order parameter provides a computational technique for understanding chemical ordering in alloys, which can facilitate the development of rational alloy design strategies.

36 MATERIALS SCIENCE↗

NASA NTRS1992

Direct numerical simulations of a reacting turbulent mixing layer by a pseudospectral-spectral element method

An account is given of the implementation of the spectral-element technique for simulating a chemically reacting, spatially developing turbulent mixing layer. Attention is given to experimental and numerical studies that have investigated the development, evolution, and mixing characteristics of shear flows. A mathematical formulation is presented of the physical configuration of the spatially developing reacting mixing layer, in conjunction with a detailed representation of the spectral-element method's application to the numerical simulation of mixing layers. Results from 2D and 3D calculations of chemically reacting mixing layers are given.

Mcmurtry, Patrick A.↗

DOE OSTI2023

NOvA in 10 Minutes

NOvA is a long-baseline oscillation neutrino experiment composed by two functional identical detectors, a 300 ton Near Detector and 14kton Far Detector separated by 809 km and placed in an off-axis neutrino beam created at Fermilab, this configuration provides NOvA with a rich neutrino physics program to measure neutrino mixing parameters, determine the neutrino mass hierarchy and CP violation in the leptonic sector. In this talk an overview and results from the NOvA experiment are presented

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS1976

Autoignition - A liquid propellant explosive potential limiting phenomena

It has been thought that the unplanned mixing of the propellants of liquid launch vehicles could result in massive explosion and destruction. This paper presents results of NASA's attempt to develop a precise analytical theory and predictive model for liquid propellant explosives. Prediction model experiments involving a 'seven-chart' approach showing the relationship between yield function, mixing function, time dependence, chemical and physical reactant properties and quantity effects were used to establish a theory that autoignition takes place when propellants mix in a certain 'critical mass' or greater. An analytical confirmation of the theory has been carried out, with particular reference to possible autoignition in LOX/LH2 and LOX/RP-1 and Saturn V: it was confirmed that autoignition occurs and prevents the mixing of more than the 'critical mass' and therefore limits the explosive yield to several thousand pounds, which will disperse the remaining propellant and prohibit detonation of the total quantities otherwise suspected.

Boggs, W. H.↗

DOE OSTI2026

Characterizing the impact of water uptake on light absorption by aerosol particles

Absorbing aerosols (AA) have an important impact on the global radiation budget. The composition and properties of AA can vary substantially throughout the atmosphere, depending on the particle source and the influence of chemical aging. Uncertainties associated with the radiative effects of AA remain substantial. A key contributor to this uncertainty is understanding the extent to which water uptake alters absorption by AA particles and how this depends on particle composition. We have used new and existing experimental tools to systematically characterize the relationship(s) between AA chemical and physical characteristics, relative humidity, and mixing of AA with other aerosol components through a combination of laboratory and field measurements. We have developed fundamental understanding through laboratory experiments that will enable interpretation of field observations at DOE ARM sites and facilitate process-based improvements in the simulation of absorption by carbonaceous aerosols in climate models. In the laboratory experiments we have considered a variety of different AA types, including fullerene soot (a surrogate for refractory black carbon, or BC) and nigrosine (a surrogate for partially soluble brown carbon, or BrC). By examining a range of AA types we will develop insight into how the chemical and physical properties of AA particles (e.g. whether they are refractory or soluble) impact the influence of water uptake on absorption. These AA particles will also be mixed—both internally and externally—with compounds having a wide range of hygroscopic properties to establish how the impact of water uptake on absorption will vary with photochemical processing. These laboratory observations have been compared with commonly used theoretical models, enabling development of empirical models that will facilitate improved representation of absorption by AA particles in regional and global climate models. Overall, our study has contributed to the mission of the Atmospheric System Research program by quantifying how interactions between aerosols and radiation depend on relative humidity. Through this, our work will improve understanding and model representation of aerosol processes as they affect the Earth’s radiation budget.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Mixed Tin-Titanium Oxides by Atomic Layer Deposition on Planar Substrates: Physical and Electronic Structure

Ternary atomic layer deposition of Sn-doped TiO x (Sn:TiO x ) and Ti-doped SnO x (Ti:SnO x ) was performed using tetrakisdimethylamidotitanium (IV) and tin(IV) with water at 150 °C on (1 0 0) Si and quartz substrates. The physical structure of the films was investigated using scanning electron, atomic force, and Kelvin probe force microscopies as well as spectroscopic ellipsometry, Raman spectroscopy, and X-ray diffraction. All as-deposited films are amorphous and possessed flat and conformal topographies with low surface roughness (<1 nm). Annealed Sn:TiO x and Ti:SnO x crystallize into the tetragonal anatase TiO 2 and cassiterite SnO 2 structures, respectively, without large variations to the film topography. The chemical composition of the as-deposited and annealed films was investigated through X-ray photoelectron spectroscopy. While dopants are homogenously mixed, the ternary ALD to form Sn:TiO x and Ti:SnO x surprisingly does not follow the rule of mixtures, despite similarities in both the growth rates of binary SnO x and TiO x and the precursors used. This finding is also supported by spectroscopic ellipsometry. Here, we postulate the deviation from the rule of mixtures is due to non-ideal surface chemistry of the binary ALD of SnO x . The optical bandgap of all films was quantified by the Tauc analysis and the valence band position was investigated by valence band X-ray photoelectron spectroscopy. Intra-bandgap states above the valence band maximum were observed for as-deposited Ti:SnO x and Sn:TiO x and ascribed to 5 s states from Sn 2+ ions. The presence of these intra-bandgap states induces enhanced visible absorption and bathochromic shifts to the apparent bandgap for all as-deposited films. Annealing the films removes the intra-bandgap states and increases the optical bandgap. Simplified band diagrams created using the data available demonstrated that the conduction and valence band positions did not vary between the positions of pure TiO 2 or SnO 2 with monotonic increases to the dopant incorporation.

36 MATERIALS SCIENCE↗

DOE OSTI2025

Review of Particle Physics - Scalar Mesons below 1 GeV

The summarizes much of particle physics and cosmology. Using data from previous editions, plus 2,717 new measurements from 869 papers, we list, evaluate, and average measured properties of gauge bosons and the recently discovered Higgs boson, leptons, quarks, mesons, and baryons. We summarize searches for hypothetical particles such as supersymmetric particles, heavy bosons, axions, dark photons, etc. Particle properties and search limits are listed in Summary Tables. We give numerous tables, figures, formulae, and reviews of topics such as Higgs Boson Physics, Supersymmetry, Grand Unified Theories, Neutrino Mixing, Dark Energy, Dark Matter, Cosmology, Particle Detectors, Colliders, Probability and Statistics. Most of the 120 reviews are updated, including many that are heavily revised. The is divided into two volumes. Volume 1 includes the Summary Tables and 97 review articles. Volume 2 consists of the Particle Listings and contains also 23 reviews that address specific aspects of the data presented in the Listings. The complete (both volumes) is published online on the website of the Particle Data Group () and in a journal. Volume 1 is available in print as the . A with the Summary Tables and essential tables, figures, and equations from selected review articles is available in print, as a web version optimized for use on phones, and as an Android app. The 2024 edition of the Review of Particle Physics should be cited as: S. Navas et al. (Particle Data Group), Phys. Rev. D 110, 030001 (2024)© 20242024

Navas, S. [Universidad de Granada]↗