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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 199 records · Page 11
All sourcesNASA NTRSDOE OSTI
NASA NTRS2012

Long-Term Changes in Stratospheric Age Spectra in the 21st Century in the Goddard Earth Observing System Chemistry-Climate Model (GEOSCCM)

In this study we investigate the long-term variations in the stratospheric age spectra using simulations of the 21st century with the Goddard Earth Observing System Chemistry- Climate Model (GEOSCCM). Our purposes are to characterize the long-term changes in the age spectra and identify processes that cause the decrease of the mean age in a warming climate. Changes in the age spectra in the 21st century simulations are characterized by decreases in the modal age, the mean age, the spectral width, and the tail decay timescale. Our analyses show that the decrease in the mean age is caused by two processes: the acceleration of the residual circulation that increases the young air masses in the stratosphere, and the weakening of the recirculation that leads to the decrease of tail of the age spectra and the decrease of the old air masses. The weakening of the stratospheric recirculation is also strongly correlated with the increase of the residual circulation. One important result of this study is that the decrease of the tail of the age spectra makes an important contribution to the decrease of the main age. Long-term changes in the stratospheric isentropic mixing are investigated. Mixing increases in the subtropical lower stratosphere, but its impact on the age spectra is outweighed by the increase of the residual circulation. The impacts of the long-term changes in the age spectra on long-lived chemical traces are also investigated. 37 2

Li, Feng↗
NASA NTRS2000

Cloud Condensation Nuclei in Fire-3

The centerpiece of this research was the cloud condensation nuclei (CCN) measurements of the Desert Research Institute (DRI) CCN spectrometers on board the NCAR C-130 aircraft during the Arctic Cloud Experiment (ACE) in May, 1998. These instruments operated successfully throughout all eight 10-hour research flights based in Fairbanks and the two ferry flights between Colorado and Fairbanks. Within a few months of completion of ACE the CCN data was edited and put into the archives. A paper was completed and published on the CCN climatology during the previous two FIRE field projects-FIRE 1 based in San Diego in June and July, 1987 and ASTEX based in the Azores Islands in June, 1992. This showed distinct contrasts in concentrations and spectra between continental and maritime CCN concentrations, which depended on air mass trajectories. Pollution episodes from Europe had distinct influences on particle concentrations at low altitudes especially within the boundary layer. At higher altitudes concentrations were similar in the two air mass regimes. Cloudier atmospheres showed lower concentrations especially below the clouds, which were a result mostly of coalescence scavenging.

Source record↗
DOE OSTI2021

Using ‘heat tagging’ to understand the remote influence of atmospheric diabatic heating through long-range transport

In the circulating atmosphere, diabatic heating influences the potential temperature content of air masses far from where the heating occurs. Budgets that balance local diabatic sources with local heat divergence and storage do not retain information about this remote influence, which requires air-mass tracking. In this study, a process based, passive-tracer diagnostic, called heat tagging, is introduced. Heat tagging locally decomposes the potential temperature into contributions from the distinctive diabatic processes that generate them, wherever they occur. The distribution, variability and transport of atmospheric heat tags are studied in the relatively simple setting of an idealized aquaplanet model. Heat tags from latent heating are generated in the deep tropics and the midlatitude storm track and then transported throughout the troposphere. By contrast dry sensible heat tags are enhanced near the surface, and radiative tags are mainly confined to the stratosphere. As a result, local heat transport, variability of potential temperature and global poleward heat transport are dominated by heat tags related to latent heating, with heat tags from sensible and radiative heating only making contributions in the polar near surface and the stratosphere respectively. Heat tagging thus quantifies how water vapor and latent heating link the structural characteristics of the atmosphere and illustrates the importance of the hydrological cycle in poleward energy transport.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Processes contributing to cloud dissipation and formation events on the North Slope of Alaska

Abstract. Clear-sky periods across the high latitudes have profound impacts on the surface energy budget and lower atmospheric stratification; however an understanding of the atmospheric processes leading to low-level cloud dissipation and formation events is limited. A method to identify clear periods at Utqiaġvik (formerly Barrow), Alaska, during a 5-year period (2014–2018) is developed. A suite of remote sensing and in situ measurements from the high-latitude observatory are analyzed; we focus on comparing and contrasting atmospheric properties during low-level (below 2 km) cloud dissipation and formation events to understand the processes controlling clear-sky periods. Vertical profiles of lidar backscatter suggest that aerosol presence across the lower atmosphere is relatively invariant during the periods bookending clear conditions, which suggests that a sparsity of aerosol is not frequently a cause for cloud dissipation on the North Slope of Alaska. Further, meteorological analysis indicates two active processes ongoing that appear to support the formation of low clouds after a clear-sky period: namely, horizontal advection, which was dominant in winter and early spring, and quiescent air mass modification, which was dominant in the summer. During summer, the dominant mode of cloud formation is a low cloud or fog layer developing near the surface. This low cloud formation is driven largely by air mass modification under relatively quiescent synoptic conditions. Near-surface aerosol particles concentrations changed by a factor of 2 around summer formation events. Thermodynamic adjustment and increased aerosol presence under quiescent atmospheric conditions are hypothesized as important mechanisms for fog formation.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1983

Data on total and spectral solar irradiance

This paper presents a brief survey of the data available on solar constant and extraterrestrial solar spectral irradiance. The spectral distribution of solar radiation at ground surface, computed from extraterrestrial solar spectral irradiance for several air mass values and for four levels of atmospheric pollution, is also presented. The total irradiance at ground level is obtained by integration of the area under the spectral irradiance curves. It is significant that, as air mass increases or as turbidity increases, the amount of energy in the infrared relative to the total increases and that the energy in the UV and visible decreases.

Mecherikunnel, A. T.↗
NASA NTRS2012

Current Usage and Future Prospects of Multispectral (RGB) Satellite Imagery in Support of NWS Forecast Offices and National Centers

Current and future satellite sensors provide remotely sensed quantities from a variety of wavelengths ranging from the visible to the passive microwave, from both geostationary and low-Earth orbits. The NASA Short-term Prediction Research and Transition (SPoRT) Center has a long history of providing multispectral imagery from the Moderate Resolution Imaging Spectroradiometer (MODIS) aboard NASA s Terra and Aqua satellites in support of NWS forecast office activities. Products from MODIS have recently been extended to include a broader suite of multispectral imagery similar to those developed by EUMETSAT, based upon the spectral channel s available from the Spinning Enhanced Visible and InfraRed Imager (SEVIRI) aboard METEOSAT-9. This broader suite includes products that discriminate between air mass types associated with synoptic-scale features, assists in the identification of dust, and improves upon paired channel difference detection of fog and low cloud events. Similarly, researchers at NOAA/NESDIS and CIRA have developed air mass discrimination capabilities using channels available from the current GOES Sounders. Other applications of multispectral composites include combinations of high and low frequency, horizontal and vertically polarized passive microwave brightness temperatures to discriminate tropical cyclone structures and other synoptic-scale features. Many of these capabilities have been transitioned for evaluation and operational use at NWS Weather Forecast Offices and National Centers through collaborations with SPoRT and CIRA. Future instruments will continue the availability of these products and also expand upon current capabilities. The Advanced Baseline Imager (ABI) on GOES-R will improve the spectral, spatial, and temporal resolution of our current geostationary capabilities, and the recent launch of the Suomi National Polar-Orbiting Partnership (S-NPP) carries instruments such as the Visible Infrared Imager Radiometer Suite (VIIRS), the Cross-track Infrared Sounder (CrIS), and the Advanced Technology Microwave Sounder (ATMS), which have unrivaled spectral and spatial resolution, as precursors to the JPSS era (i.e., the next generation of polar orbiting satellites). At the same time, new image manipulation and display capabilities are available within AWIPS II, the next generation of the NWS forecaster decision support system. This presentation will present a review of SPoRT, CIRA, and NRL collaborations regarding multispectral satellite imagery and articulate an integrated and collaborative path forward with Raytheon AWIPS II development staff for integrating current and future capabilities that support new satellite instrumentation and the AWIPS II decision support system.

Molthan, Andrew L.↗
NASA NTRS1996

Chemical Characteristics of Continental Outflow Over the Tropical South Atlantic Ocean from Brazil and Africa

The chemical characteristics of air parcels over the tropical South Atlantic during September - October 1992 are summarized by analysis of aged marine and continental outflow classifications. Positive correlations between CO and CH3CL and minimal enhancements of C2CL40, and various ChloroFluoroCarbon (CFC) species in air parcels recently advected over the South Atlantic basin strongly suggest an impact on tropospheric chemistry from biomass burning on adjacent continental areas of Brazil and Africa. Comparison of the composition of aged Pacific air with aged marine air over the South Atlantic basin from 0.3 to 12.5 km altitude indicates potential accumulation of long-lived species during the local dry season. This may amount to enhancements of up to two-fold for C2H6, 30% for CO, and 10% for CH3Cl. Nitric oxide and NO(x) were significantly enhanced (up to approx. 1 part per billion by volume (ppbv)) above 10 km altitude and poorly correlated with CO and CH3Cl. In addition, median mixing ratios of NO and NO(x) were essentially identical in aged marine and continental outflow air masses. It appears that in addition to biomass burning, lightning or recycled reactive nitrogen may be an important source of NO(x) to the upper troposphere. Methane exhibited a monotonic increase with altitude from approx. 1690 to 1720 ppbv in both aged marine and continental outflow air masses. The largest mixing ratios in the upper troposphere were often anticorrelated with CO, CH3Cl, and CO2, suggesting CH, contributions from natural sources. We also argue, based on CH4/CO ratios and relationships with various hydrocarbon and CFC species, that inputs from biomass burning and the northern hemisphere are unlikely to be the dominant sources of CO, CH4 and C2H6 in aged marine air. Emissions from urban areas would seem to be necessary to account for the distribution of at least CH4 and C2H6. Over the African and South American continents an efficient mechanism of convective vertical transport coupled with large-scale circulations conveys biomass burning, urban, and natural emissions to the upper troposphere over the South Atlantic basin. Slow subsidence over the eastern South Atlantic basin may play an important role in establishing and maintaining the rather uniform vertical distribution of long-lived species over this region. The common occurrence of values greater than 1 for the ratio CH3OOH/H2O2 in the upper troposphere suggests that precipitation scavenging effectively removed highly water soluble gases (H2O2, HNO3, HCOOH, and CH3COOH) and aerosols during vertical convective transport over the continents. However, horizontal injection of biomass burning products over the South Atlantic, particularly water soluble species and aerosol particles, was frequent below 6 km altitude.

Talbot, R. W.↗
NASA NTRS1976

Sensitivity of solar-cell performance to atmospheric variables. 1: Single cell

The short circuit current of a typical silicon solar cell under direct solar radiation was measured for a range of turbidity, water vapor content, and air mass to determine the relation of the solar cell calibration value (current-to-intensity ratio) to those atmospheric variables. A previously developed regression equation was modified to describe the relation between calibration value, turbidity, water vapor content, and air mass. Based on the value of the constants obtained by a least squares fit of the data to the equation, it was found that turbidity lowers the value, while increase in water vapor increases the calibration value. Cell calibration values exhibited a change of about 6% over the range of atmospheric conditions experienced.

Klucher, T. M.↗
NASA NTRS1980

Spectral distribution of solar radiation

Available quantitative data on solar total and spectral irradiance are examined in the context of utilization of solar irradiance for terrestrial applications of solar energy. The extraterrestrial solar total and spectral irradiance values are also reviewed. Computed values of solar spectral irradiance at ground level for different air mass values and various levels of atmospheric pollution or turbidity are presented. Wavelengths are given for computation of solar, absorptance, transmittance and reflectance by the 100 selected-ordinate method and by the 50 selected-ordinate method for air mass 1.5 and 2 solar spectral irradiance for the four levels of atmospheric pollution.

Mecherikunnel, A. T.↗
NASA NTRS1996

A Comparison of Aircraft and Ground-Based Measurements at Mauna Loa Observatory, Hawaii, During GTE PEM-West and MLOPEX 2

During October 19-20, 1991, one flight of the NASA Global Tropospheric Experiment (GTE) Pacific Exploratory Mission (PEM-West A) mission was conducted near Hawaii as an intercomparison with ground-based measurements of the Mauna Loa Observatory Photochemistry Experiment (MLOPEX 2) and the NOAA Climate Modeling and Diagnostics Laboratory (CMDL). Ozone, reactive nitrogen species, peroxides, hydrocarbons, and halogenated hydrocarbons were measured by investigators aboard the DC-8 aircraft and at the ground site. Lidar cross sections of ozone revealed a complex air mass structure near the island of Hawaii which was evidenced by large variation in some trace gas mixing ratios. This variation limited the time and spatial scales for direct measurement intercomparisons. Where differences occurred between measurements in the same air masses, the intercomparison suggested that biases for some trace gases was due to different calibration scales or, in some cases, instrumental or sampling biases. Relatively large uncertainties were associated with those trace gases present in the low parts per trillion by volume range. Trace gas correlations were used to expand the scope of the intercomparison to identify consistent trends between the different data sets.

Atlas, E.↗
NASA NTRS1978

Solar spectral irradiance at ground level

Available quantitative data on solar total and spectral irradiance is examined in the context of utilization of solar irradiance for terrestrial applications of solar energy. A brief review is given on the extraterrestrial solar total and spectral irradiance values. Computed values of solar spectral irradiance at ground level for different air mass values and various levels of atmospheric pollution or turbidity are also presented. Wavelengths are given for computation of solar absorptance, transmittance and reflectance by the 100-selected-ordinate method and by the 50-selected-ordinate method from air mass two solar spectral irradiance for the four degrees of atmospheric pollution. Total solar spectral irradiance measured with a prism monochromator is examined to evaluate the direct solar spectral irradiance for a surface normal to the sun's rays and to compare the computed spectrum with the experimentally observed one.

Mecherikunnel, A. T.↗
NASA NTRS1994

Three-dimensional model interpretation of NO(x) measurements from the lower stratosphere

A three-dimensional off-line chemistry transport model, driven by European Center for Medium-Range Forecasts winds and temperatures, is used to interpret measurements of NO and NO2 taken from the DC-8 during the second Airborne Arctic Stratospheric Expedition. The model was run in three configurations: gas phase chemistry alone, inclusion of the N2O5 aerosol reaction, and inclusion of both N2O5 and ClONO2 aerosol reactions. The run including the N2O5 aerosol reaction alone usually agreed best with measured NO(x)/NO(y) ratios in midlatitude air masses. The NO(x)/NO(y) ratios of the run with both aerosol reactions were always too low, while the gas phase ratios were usually too high, especially during March. All three simulations generated extremely low NO2/NO(y) ratios in air parcels that had spent several days or more in the polar night. Measured NO2/NO(y) ratios in these types of air masses were sometimes equally low but could also be considerably higher. Observed NO/NO2 ratios differed strongly from known theory.

Folkins, Ian↗
NASA NTRS2016

How We Can Constrain Aerosol Type Globally

In addition to aerosol number concentration, aerosol size and composition are essential attributes needed to adequately represent aerosol-cloud interactions (ACI) in models. As the nature of ACI varies enormously with environmental conditions, global-scale constraints on particle properties are indicated. And although advanced satellite remote-sensing instruments can provide categorical aerosol-type classification globally, detailed particle microphysical properties are unobtainable from space with currently available or planned technologies. For the foreseeable future, only in situ measurements can constrain particle properties at the level-of-detail required for ACI, as well as to reduce uncertainties in regional-to-global-scale direct aerosol radiative forcing (DARF). The limitation of in situ measurements for this application is sampling. However, there is a simplifying factor: for a given aerosol source, in a given season, particle microphysical properties tend to be repeatable, even if the amount varies from day-to-day and year-to-year, because the physical nature of the particles is determined primarily by the regional environment. So, if the PDFs of particle properties from major aerosol sources can be adequately characterized, they can be used to add the missing microphysical detail the better sampled satellite aerosol-type maps. This calls for Systematic Aircraft Measurements to Characterize Aerosol Air Masses (SAM-CAAM). We are defining a relatively modest and readily deployable, operational aircraft payload capable of measuring key aerosol absorption, scattering, and chemical properties in situ, and a program for characterizing statistically these properties for the major aerosol air mass types, at a level-of-detail unobtainable from space. It is aimed at: (1) enhancing satellite aerosol-type retrieval products with better aerosol climatology assumptions, and (2) improving the translation between satellite-retrieved aerosol optical properties and species-specific aerosol mass and size that are tracked in aerosol transport and climate models used to assess aerosol forcing and its anthropogenic components. This presentation will summarize where we stand on the development of the SAM-CAAM concept.

DARF↗
DOE OSTI2025

Characteristics and effects of aerosols during blowing snow events in the central Arctic

Sea salt aerosol (SSaer) significantly impacts aerosol-radiation and aerosol-cloud interactions, and sublimated blowing snow is hypothesized to be an important SSaer source in polar regions. Understanding blowing snow and other wind-sourced aerosols’ climate relevant properties is needed, especially during winter when Arctic amplification is greatest. However, most of our understanding of blowing snow SSaer comes from modeling studies, and direct observations are sparse. Additionally, SSaer can originate from multiple sources, making it difficult to disentangle emission processes. Here, we present comprehensive observations of wind-sourced aerosol during blowing snow events from the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition in the central Arctic. High wind speed strongly enhances total aerosol number, submicron sodium chloride mass, cloud condensation nuclei concentrations, and scattering coefficients. Generally, the relative response of aerosol properties to wind speed enhancement is strongest in fall when Arctic aerosol concentrations are lowest. Blowing snow events showed similar aerosol and environmental properties across events, apart from occasions with high snow age (>6 days since last snowfall). Coarse-mode number concentrations (>1 μm) are better explained by variability in wind speed averaged over 12-h air mass back trajectories arriving at the MOSAiC site compared to local, instantaneous wind speed, suggesting the importance of regional transport and consideration of air mass history for wind-driven aerosol production. These MOSAiC observations provide new insights into wind-driven aerosol in the central Arctic and may help validate modeling studies and improve model parameterizations particularly for aerosol direct and indirect radiative forcing.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2003

Environmental Snapshots for Satellite Multi-Angle Aerosol Retrieval Validation During the ACE-Asia Field Campaign

On five occasions spanning the ACE-Asia field experiment in spring 2001, the multi-angle imaging MISR instrument, flying aboard the NASA Earth Observing System s Terra satellite, took quarter-kilometer data over a 400-km-wide swath, coincident with high-quality observations by multiple instruments on two or more participating surface and airborne platforms. The cases capture a range of clean, polluted, and dusty aerosol conditions. They represent some of the best opportunities during ACE- Asia for comparative studies among intensive and extensive aerosol observations in their environmental context. We inter-compare related measurements and discuss the implications of apparent discrepancies for each case, at a level of detail appropriate to the analysis of satellite observations. With a three-stage optical modeling process, we synthesize data from multiple sources into layer-by-layer snapshots that summarize what we know about the state of the atmosphere and surface at key locations during each event, to be used for satellite vicarious calibration and aerosol retrieval validation. Aerosols within a few kilometers of the surface were composed primarily of pollution and Asian dust mixtures, as expected. Accumulation and coarse-mode particle size distributions varied little among the events studied, but column aerosol optical depth changed by more than a factor of four, and the near-surface proportion of dust ranged from about 25% to 50%. The amount of absorbing material in the sub-micron fraction was highest when near-surface winds crossed Beijing and the Korean Peninsula, and was considerably lower for all other cases. Ambiguities remain in segregating size distributions by composition; having simultaneous single scattering albedo measurements at more than a single wavelength would significantly reduce the resulting optical model uncertainties, as would integral constraints from surface and atmospheric radiative flux observations. The consistency of component particle micro-physical properties among the five events, even in this relatively complex aerosol environment, suggests that global, satellite-derived maps of aerosol-air-mass-type extent, combined with targeted in situ measurements, can provide a detailed global picture of aerosol behavior. Further joint satellite and in situ analysis is needed to assess the spatial variability of both intensive and extensive aerosol properties within aerosol air masses in two spatial dimensions.

Kahn, Ralph↗
NASA NTRS2000

LIDAR Measurements During Aerosols99

The Aerosols99 cruise took place during the period from January 14, to February 8 1999 on the R/V Ron Brown. The cruise track was almost a straight line from Norfolk, Va. to Cape Town, South Africa and afforded the opportunity to sample several different aerosol regimes over the North and South Atlantic. A Micro Pulse LIDAR system was used continually during this cruise to profile the aerosol vertical structure. Inversions of this data illustrated a varying vertical structure depending on the dominant air mass. In clean maritime aerosols in the Northern and Southern Hemispheres the aerosols were capped at 1 km. When a Dust event from Africa was encountered the aerosol extinction increased its maximum height to above 2 km. During a period in which the air mass was dominated by biomass burning from Southern Africa, the aerosol layer extended to 4 km. Comparisons of the aerosol optical depth derived from LIDAR inversion and surface sunphotometers showed an agreement within +/- 0.05 RMS Similar comparisons between the extinction measured with a nephelometer and particle soot absorption photometer (at 19 m altitude) and the lowest LIDAR measurement (75 m) showed good agreement (+/- 0.014/km . The LIDAR underestimated surface extinction during periods when an elevated aerosol layer was present over a relatively clean surface layer, but otherwise gave accurate results.

Voss, Kenneth J.↗
NASA NTRS2013

Evaluation of Aerosol Mixing State Classes in the GISS Modele-matrix Climate Model Using Single-particle Mass Spectrometry Measurements

Aerosol particles in the atmosphere are composed of multiple chemical species. The aerosol mixing state, which describes how chemical species are mixed at the single-particle level, provides critical information on microphysical characteristics that determine the interaction of aerosols with the climate system. The evaluation of mixing state has become the next challenge. This study uses aerosol time-of-flight mass spectrometry (ATOFMS) data and compares the results to those of the Goddard Institute for Space Studies modelE-MATRIX (Multiconfiguration Aerosol TRacker of mIXing state) model, a global climate model that includes a detailed aerosol microphysical scheme. We use data from field campaigns that examine a variety of air mass regimens (urban, rural, and maritime). At all locations, polluted areas in California (Riverside, La Jolla, and Long Beach), a remote location in the Sierra Nevada Mountains (Sugar Pine) and observations from Jeju (South Korea), the majority of aerosol species are internally mixed. Coarse aerosol particles, those above 1 micron, are typically aged, such as coated dust or reacted sea-salt particles. Particles below 1 micron contain large fractions of organic material, internally-mixed with sulfate and black carbon, and few external mixtures. We conclude that observations taken over multiple weeks characterize typical air mass types at a given location well; however, due to the instrumentation, we could not evaluate mass budgets. These results represent the first detailed comparison of single-particle mixing states in a global climate model with real-time single-particle mass spectrometry data, an important step in improving the representation of mixing state in global climate models.

climate models↗
NASA NTRS2001

Measurements of Aerosol Vertical Profiles and Optical Properties during INDOEX 1999 Using Micro-Pulse Lidars

Micro-pulse lidar systems (MPL) were used to measure aerosol properties during the Indian Ocean Experiment (INDOEX) 1999 field phase. Measurements were made from two platforms: the NOAA ship RN Ronald H. Brown, and the Kaashidhoo Climate Observatory (KCO) in the Maldives. Sunphotometers were used to provide aerosol optical depths (AOD) needed to calibrate the MPL. This study focuses on the height distribution and optical properties (at 523 nm) of aerosols observed during the campaign. The height of the highest aerosols (top height) was calculated and found to be below 4 km for most of the cruise. The marine boundary layer (MBL) top was calculated and found to be less than 1 km. MPL results were combined with air mass trajectories, radiosonde profiles of temperature and humidity, and aerosol concentration and optical measurements. Humidity varied from approximately 80% near the surface to 50% near the top height during the entire cruise. The average value and standard deviation of aerosol optical parameters were determined for characteristic air mass regimes. Marine aerosols in the absence of any continental influence were found to have an AOD of 0.05 +/- 0.03, an extinction-to-backscatter ratio (S-ratio) of 33 +/- 6 sr, and peak extinction values around 0.05/km (near the MBL top). The marine results are shown to be in agreement with previously measured and expected values. Polluted marine areas over the Indian Ocean, influenced by continental aerosols, had AOD values in excess of 0.2, S-ratios well above 40 sr, and peak extinction values approximately 0.20/km (near the MBL top). The polluted marine results are shown to be similar to previously published values for continental aerosols. Comparisons between MPL derived extinction near the ship (75 m) and extinction calculated at ship-level using scattering measured by a nephelometer and absorption using a PSAP were conducted. The comparisons indicated that the MPL algorithm (using a constant S-ratio throughout the lower troposphere) calculates extinction near the surface in agreement with the ship-level measurements only when the MBL aerosols are well mixed with aerosols above. Finally, a review of the MPL extinction profiles showed that the model of aerosol vertical extinction developed during an earlier INDOEX field campaign (at the Maldives) did not correctly describe the true vertical distribution over the greater Indian Ocean region. Using the average extinction profile and AOD obtained during marine conditions, a new model of aerosol vertical extinction was determined for marine atmospheres over the Indian Ocean. A new model of aerosol vertical extinction for polluted marine atmospheres was also developed using the average extinction profile and AOD obtained during marine conditions influenced by continental aerosols.

Welton, Ellsworth J.↗