Search NASA⌕ Search

SEARCH · Search NASA

Results for “Atmospheric composition”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 199 records · Page 11
All sourcesNASA NTRSDOE OSTI
NASA NTRS2018

Air Quality Satellite Monitoring by TROPOMI on Sentinel-5P

The recently launched Sentinel satellite mission, the Sentinel-5 Precursor (Sentinel-5P), is one of the European Space Agency's (ESA) new mission family – Sentinels. The sole payload on Sentinel-5P is the TROPOspheric Monitoring Instrument (TROPOMI), a nadir-viewing 108⁰ field-of-view push-broom grating hyperspectral spectrometer, covering the wavelengths of ultraviolet-visible (270 nm - 495 nm), near infrared (675 nm - 775 nm), and shortwave infrared (2305 nm - 2385 nm). Sentinel-5P is the first of the Atmospheric Composition Sentinels, and is providing measurements of atmospheric chemistry, aerosols, and clouds at high spatial, temporal, and spectral resolution. The NASA Goddard Earth Sciences Data and Information Services Center (GES DISC) supports over a thousand data collections in the focus areas of Atmospheric Composition, Water & Energy Cycles, and Climate Variability. Sentinel-5P TROPOMI Level-1B (L1B) and Level-2 (L2) products are curated at the GES DISC. Sentinel-5P data are provided by the European Union and the European Space Agency (ESA) through an agreement between ESA and NASA. Through its convenient and enhanced tools/services, such as OPeNDAP and L2 Subsetting, GES DISC offers the air quality remote sensing user community facile solutions for using complex Earth science data and applications. This presentation will demonstrate up-to-date TROPOMI products including EarthView (EV) radiance, solar irradiance, Aerosol Index, Carbon Monoxide, Total column Ozone, Nitrogen Dioxide, and cloud, as well as easy ways to access, visualize and subset TROPOMI data.

TROPOMI↗
NASA NTRS1980

Response of the global climate to changes in atmospheric chemical composition due to fossil fuel burning

Recent modeling of atmospheric chemical processes (Logan et al, 1978; Hameed et al, 1979) suggests that tropospheric ozone and methane might significantly increase in the future as the result of increasing anthropogenic emissions of CO, NO(x), and CH4 due to fossil fuel burning. Since O3 and CH4 are both greenhouse gases, increases in their concentrations could augment global warming due to larger future amounts of atmospheric CO2. To test the possible climatic impact of changes in tropospheric chemical composition, a zonal energy-balance climate model has been combined with a vertically averaged tropospheric chemical model. The latter model includes all relevant chemical reactions which affect species derived from H2O, O2, CH4, and NO(x). The climate model correspondingly incorporates changes in the infrared heating of the surface-troposphere system resulting from chemically induced changes in tropospheric ozone and methane. This coupled climate-chemical model indicates that global climate is sensitive to changes in emissions of CO, NO(x) and CH4, and that future increases in these emissions could augment global warming due to increasing atmospheric CO2.

Hameed, S.↗
NASA NTRS2014

Geostationary Coastal and Air Pollution Events (GEO-CAPE) Sensitivity Analysis Experiment

Geostationary Coastal and Air pollution Events (GEO-CAPE) is a NASA decadal survey mission to be designed to provide surface reflectance at high spectral, spatial, and temporal resolutions from a geostationary orbit necessary for studying regional-scale air quality issues and their impact on global atmospheric composition processes. GEO-CAPE's Atmospheric Science Questions explore the influence of both gases and particles on air quality, atmospheric composition, and climate. The objective of the GEO-CAPE Observing System Simulation Experiment (OSSE) is to analyze the sensitivity of ozone to the global and regional NOx emissions and improve the science impact of GEO-CAPE with respect to the global air quality. The GEO-CAPE OSSE team at Jet propulsion Laboratory has developed a comprehensive OSSE framework that can perform adjoint-sensitivity analysis for a wide range of observation scenarios and measurement qualities. This report discusses the OSSE framework and presents the sensitivity analysis results obtained from the GEO-CAPE OSSE framework for seven observation scenarios and three instrument systems.

Lee, Meemong↗
DOE OSTI2020

ToF-SIMS Analysis of Chemical Composition of Atmospheric Aerosols in Beijing

Atmospheric aerosols collected from each season in urban Beijing have been studied using time-of-flight secondary ion mass spectrometry (ToF-SIMS). The chemical composition of atmospheric aerosol particles during various atmospheric pollution levels were analyzed and distinguished by principal component analysis (PCA). The differences and sources of the components of the aerosol particles were explored. The results showed that the fine particulate matter from heavily polluted days mainly consists of inorganic salts and organic compounds, such as hydrocarbons, nitrogen- or sulfur-containing hydrocarbons, and their oxides. Samples collected from clean days in the four seasons were also analyzed. Only the samples collected in spring showed a significant difference from the other three seasons. We concluded that the main source of pollution in the Beijing urban area was fossil fuel combustion from motor vehicles.

ToF-SIMS, principal component analysis↗
DOE OSTI2020

Optical Transmission Spectroscopy of the Terrestrial Exoplanet LHS 3844b from 13 Ground-based Transit Observations

Atmospheric studies of spectroscopically accessible terrestrial exoplanets lay the groundwork for comparative planetology between these worlds and the solar system terrestrial planets. LHS 3844b is a highly irradiated terrestrial exoplanet (R = 1.303 ± 0.022R {sub ⊕}) orbiting a mid-M dwarf 15 parsecs away. Work based on near-infrared Spitzer phase curves ruled out atmospheres with surface pressures ≥10 bars on this planet. We present 13 transit observations of LHS 3844b taken with the Magellan Clay telescope and the LDSS3C multi-object spectrograph covering 620–1020 nm. We analyze each of the 13 data sets individually using a Gaussian process regression, and present both white and spectroscopic light curves. In the combined white light curve we achieve an rms precision of 65 ppm when binning to 10 minutes. The mean white light-curve value of (R {sub p}/R {sub s}){sup 2} is 0.4170 ± 0.0046%. To construct the transmission spectrum, we split the white light curves into 20 spectrophotometric bands, each spanning 20 nm, and compute the mean values of (R {sub p}/R {sub s}){sup 2} in each band. We compare the transmission spectrum to two sets of atmospheric models. We disfavor a clear, solar composition atmosphere (μ = 2.34) with surface pressures ≥0.1 bar to 5.2σ confidence. We disfavor a clear, H{sub 2}O steam atmosphere (μ = 18) with surface pressures ≥0.1 bar to low confidence (2.9σ). Our observed transmission spectrum favors a flat line. For solar composition atmospheres with surface pressures ≥1 bar we rule out clouds with cloud-top pressures of 0.1 bar (5.3σ), but we cannot address high-altitude clouds at lower pressures. Our results add further evidence that LHS 3844b is devoid of an atmosphere.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1996

The Galileo probe mass spectrometer: composition of Jupiter's atmosphere

The composition of the jovian atmosphere from 0.5 to 21 bars along the descent trajectory was determined by a quadrupole mass spectrometer on the Galileo probe. The mixing ratio of He (helium) to H2 (hydrogen), 0.156, is close to the solar ratio. The abundances of methane, water, argon, neon, and hydrogen sulfide were measured; krypton and xenon were detected. As measured in the jovian atmosphere, the amount of carbon is 2.9 times the solar abundance relative to H2, the amount of sulfur is greater than the solar abundance, and the amount of oxygen is much less than the solar abundance. The neon abundance compared with that of hydrogen is about an order of magnitude less than the solar abundance. Isotopic ratios of carbon and the noble gases are consistent with solar values. The measured ratio of deuterium to hydrogen (D/H) of (5 +/- 2) x 10(-5) indicates that this ratio is greater in solar-system hydrogen than in local interstellar hydrogen, and the 3He/4He ratio of (1.1 +/- 0.2) x 10(-4) provides a new value for protosolar (solar nebula) helium isotopes. Together, the D/H and 3He/4He ratios are consistent with conversion in the sun of protosolar deuterium to present-day 3He.

NASA Discipline Number 52-10↗
DOE OSTI2021

Phase Modeling of the TRAPPIST-1 Planetary Atmospheres

Transiting compact multiplanet systems provide many unique opportunities to characterize the planets, including studies of size distributions, mean densities, orbital dynamics, and atmospheric compositions. The relatively short orbital periods in these systems ensure that events requiring specific orbital locations of the planets (such as primary transit and secondary eclipse points) occur with high frequency. The orbital motion and associated phase variations of the planets provide a means to constrain the atmospheric compositions through measurement of their albedos. Here we describe the expected phase variations of the TRAPPIST-1 system and times of superior conjunction when the summation of phase effects produce maximum amplitudes. We also describe the infrared flux emitted by the TRAPPIST-1 planets and the influence on the overall phase amplitudes. We further present the results from using the global circulation model ROCKE-3D to model the atmospheres of TRAPPIST-1e and TRAPPIST-1f assuming modern Earth and Archean atmospheric compositions. These simulations are used to calculate predicted phase curves for both reflected light and thermal emission components. We discuss the detectability of these signatures and the future prospects for similar studies of phase variations for relatively faint M stars.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

Atmosphere Effects in Laser Powder Bed Fusion: A Review

The use of components fabricated by laser powder bed fusion (LPBF) requires the development of processing parameters that can produce high-quality material. Manipulating the most commonly identified critical build parameters (e.g., laser power, laser scan speed, and layer thickness) on LPBF equipment can generate acceptable parts for established materials and moderately intricate part geometries. The need to fabricate increasingly complex parts from unique materials drives the limited research into LPBF process control using underutilized parameters, such as atmosphere composition and pressure. As presented in this review, manipulating atmosphere composition and pressure in laser beam welding has been shown to expand processing windows and produce higher-quality welds. The similarities between laser beam welding and laser-based AM processes suggest that this atmosphere control research could be effectively adapted for LPBF, an area that has not been widely explored. Tailoring this research for LPBF has significant potential to reveal novel processing regimes. This review presents the current state of the art in atmosphere research for laser beam welding and LPBF, with a focus on studies exploring cover gas composition and pressure, and concludes with an outlook on future LPBF atmosphere control systems.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Impact of vegetation physiology and phenology on watershed hydrology in a semiarid watershed in the Pacific Northwest in a changing climate

Concurrent with changes in climate conditions, increases in atmospheric composition and transport can affect land surface processes by regulating physiological and phenological responses of plants, and consequently perturb water, carbon, and nitrogen (N) dynamics at multiple scales. Howerver, the relationships bwtween plants physiological and phenological and land surface processes in a changing climate are less well known due to the limitation of representing palnts properties in traditional hydrological models. In this study, we use the Community Land Model version 5 (CLM5) to investigate how projected changes in large scale atmospheric conditions can affect hydrologic and biogeochemical dynamics in the Upper Columbia-Priest Rapids (UCPR) watershed, a typical semi-arid watershed located in the north-western United States dominated by croplands. Six numerical experiments considering climate change, CO2 concentration, and N deposition consistent with the Representative Concentration Pathways (RCPs) 4.5 and 8.5 are performed at 1-km resolution over the period of 2015-2099. Our results show that, compared with historical results (1985-2014), the elevated CO2 directly increases plants N uptake rates that provide additional leaf N to enhance photosynthesis by the end of 21st century (2070-2099). The higher GPP leads to changes in stomatal resistance and increased leaf area index (LAI) that affect evaporatranspiration (ET) and its components. As a result of stomatal responses to a higher CO2 concentration, ET over corn fields declines by 24.6 mm yr-1 under RCP4.5, and by 64.0 mm yr-1 under RCP8.5, respectively by the end of the century from its historical mean of 428 mm yr-1. Meanwhile, ET over soybean fields increases by 27.7 mm yr-1 under RCP4.5 and 9.98 mm yr-1 under RCP8.5 from its historical mean of 507 mm yr-1 as a result of CO2 fertilization as soybeans are able to uptake more N to increase LAI significantly. Furtherfore, the changes in physiological and phenological in corn and soybean can strongly modulate water budget terms over the watershed in response to expected changes in greenhouse gas concentrations and atmospheric composition. Additionally, increases in CO2 concentration and N deposition are beneficial for improving water use efficiency of corn and soybean, therefore lead to less water consumption per unit gram of carbon produced from these crops. Our study elucidates the need to jointly consider effects of surface climate and atmospheric composition and transport in understanding and predicting watershed hydrologic and biogeochemical responses, especially for an agricultural watershed.

Zhu, Bowen↗
NASA NTRS2003

New Particle Formation in Anthropogenic Plumes Advecting from Asia Observed During TRACE-P

The characteristics and sources of what are believed to be newly formed 3 to 4 nm particles in anthropogenic plumes advecting from Asian are reported. Airborne measurements were made from March to April 2001 as part of the NASA TRACE-P experiment at latitudes ranging from North of the Philippines to Northern Japan (20 to 45 deg. N). In the more polluted plumes, high concentrations of 3 to 4 nm diameter particles (less than 100/qu cm) were observed both within and along the upper outer edges of plumes that were identified by enhanced carbon monoxide and fine particulate sulfate concentrations. The results from two research flights are investigated in detail. Three to four-nm particle concentrations are generally correlated with gas phase sulfuric acid and found in regions of low surface areas relative to the immediate surroundings or where there are steep transitions to lower surface areas. Sulfuric acid and surface area concentrations in the most polluted plume reached 6 x l0(exp 7) and 750 micro sq m/qu cm, respectively, in regions of particle formation. In contrast to these anthropogenic plumes, few 3 to 4 nm particles were observed in the clean background and few were detected within a volcanic plume where the studies highest H2SO4 concentrations (less than lO(exp 8)/qu cm) were recorded. Enhanced SO2 concentrations in the range of approximately 2 to 7 ppb, in conjunction with other unidentified, possibly coemitted species, appear to be the driving factor for nucleation. (0345, 4801); 0322 Atmospheric Composition and Structure: Constituent sources and sinks; 0345 Atmospheric Composition and Structure: Pollution-urban and regional (0305); 4801 Oceanography: Biological and Chemical: Aerosols (0305).

Weber, R. J.↗
NASA NTRSDate not supplied

Evaluation of the GEOS-Chem UCX Stratosphere in the GEOS Composition Forecast System

The NASA GEOS Composition Forecast (GEOS-CF) system provides 3-dimensional atmospheric composition analyses and forecasts to the public in near-real time at the high spatial resolution of 25 km. While the main focus of this new product is on tropospheric air quality information, the GEOS-Chem chemistry model (v12) used in this system includes the UCX stratospheric chemistry mechanism. Here, we describe the GEOS-CF system and provide comparisons against remote-sensed observations for stratospheric composition, including measurements of HCl, ClO, NO2, and O3. The GEOS-CF nudges the stratospheric ozone towards the GEOS Forward Processing (GEOS FP) assimilated ozone product; as a result the stratospheric ozone analysis in theGEOS-CF agrees well with observations. Additionally, with the inclusion of the GEOS-Chem UCX stratospheric chemistry mechanism in GEOS-CF, 5-day forecasts, especially during the abnormal 2020 NH polar spring, capture the chemical and dynamical changes missed by the GEOS FP system, which tends towards climatology. The GEOS-CF is a new tool for the research community providing near-real time 3-dimensional gridded information on atmospheric composition throughout the troposphere and stratosphere.

Stratosphere↗
NASA NTRS2012

Standardization of the Definitions of Vertical Resolution and Uncertainty in the NDACC-archived Ozone and Temperature Lidar Measurements

The international Network for the Detection of Atmospheric Composition Change (NDACC) is a global network of high-quality, remote-sensing research stations for observing and understanding the physical and chemical state of the Earth atmosphere. As part of NDACC, over 20 ground-based lidar instruments are dedicated to the long-term monitoring of atmospheric composition and to the validation of space-borne measurements of the atmosphere from environmental satellites such as Aura and ENVISAT. One caveat of large networks such as NDACC is the difficulty to archive measurement and analysis information consistently from one research group (or instrument) to another [1][2][3]. Yet the need for consistent definitions has strengthened as datasets of various origin (e.g., satellite and ground-based) are increasingly used for intercomparisons, validation, and ingested together in global assimilation systems.In the framework of the 2010 Call for Proposals by the International Space Science Institute (ISSI) located in Bern, Switzerland, a Team of lidar experts was created to address existing issues in three critical aspects of the NDACC lidar ozone and temperature data retrievals: signal filtering and the vertical filtering of the retrieved profiles, the quantification and propagation of the uncertainties, and the consistent definition and reporting of filtering and uncertainties in the NDACC- archived products. Additional experts from the satellite and global data standards communities complement the team to help address issues specific to the latter aspect.

Detection of Atmospheric Composition Change (NDACC↗