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At least 199 records · Page 11
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NASA NTRS1994

An analysis of aircraft exhaust plumes form accidental encounters

An analysis of data obtained during the second Airborne Arctic Stratospheric Expedition (AASE-II) was made with emphasis on aircraft exhaust plumes accidentally encountered during the mission. Twenty spikes were found with peak NO(y) increments greater than or equal to 1 ppbv. The examination of CO and CO2 indicated that there was only one NO(y) spike having clearly corresponding spikes of both CO and CO2 and another four with unambigious CO2 spikes. No significant increases were found for CH4 and N2O for these 5 spikes. The ratio of the excess CO2 and NO(y) compares well with the ratio of published subsonic aircraft emission indices. The study of the selected spikes from the DC-8 and another two spikes observed during other missions shows that the odd nitrogen other than NO(x) accounts for a very small percentage of the NO(y) increase associated with the observed spikes.

Zheng, J.↗
NASA NTRS1994

Meridional distributions of NO(X), NO(Y), and other species in the lower statosphere and upper troposphere during AASE 2

The meridional distribution of NO(x) in the lower stratosphere and upper troposphere is inferred form 10 flights of the NASA DC-8 in the northern winter of 1992 along with like distributions of NO(y), NO(x)/NO(y), CO, and C2Cl4. In the lowest few km of the stratosphere there is little vertical gradient in NO(x) over the range of latitiudes measured (40 deg-90 deg N). There is a substantial latitudinal gradient, with 50 pptv above the pole and 120 pptv near 40 deg N. In the uppermost few km of the troposphere, background values range from 30 pptv over the pole to 90 pptv near 40 deg N. On two occasions higher values, up to 140 pptv in the mean, were seen 2-3 km below the tropopause in association with frontal systems. The meridional distributions of CO and C2Cl4 show the same feature, suggesting that the source of the elevated NO(x) is near the earth's system.

Weinheimer, A. J.↗
NASA NTRS1994

Chemical change in the arctic vortex during AASE 2

We measured column abundances of HF, HCl, O3, HNO3, and H2O on the NASA DC-8 during the AASE II campaign, using thermal emission spectroscopy. We made multiple traversals of the Arctic vortex and surroundings. Using HF as a tracer, we remove the effects of subsidence from the measured column abundances; perturbations in the resulting column abundances are attributed to chemical processing. We find that by January 1992 the stratospheric column in the vortex had been chemically depleted by about (55+/-10)% in HCl and (35+/-10)% in O3, and enhanced by about (15+/-10)% in HNO3 and (0+/-10)% in H2O.

Traub, Wesley A.↗
NASA NTRS1994

Latitude variations of stratospheric trace gases

We present vertical column abundances of H2O, N2O, HNO3, NO2, O3, HF, HCl, and ClNO3, determined from solar absorption spectra measured by the JPL MkIV interferometer from the NASA DC-8 aircraft. These observations, taken in 1987 and 1992, covered latitudes ranging from 85 deg S to 85 deg N. Although most gases display latitude symmetry, large asymmetries in H2O, HNO3, and O3 are apparent, which can be ascribed to processes enhanced by the colder Antarctic winter temperatures.

Toon, G. C.↗
NASA NTRS1994

Fine-scale, poleward transport of tropical air during AASE 2

The poleward transport of tropical air in the lower stratosphere during the winter period of the second Airborne Arctic Stratospheric Expedition (AASE 2) (December 1991-March 1992) is examined using contour advection calcutions. These calculations show that filaments of tropical air extend into mid-latitudes, and are wrapped around the equatorward edge of the polar jet. Simultaneously filaments are drawn from the polar vortex and are intermingled with the filaments of tropical air. The tropical filaments are consistent with measurements of chemical tracers taken aboard the ER-2 and DC-8 aircraft which show localized regions, in mid-latitudes, of air with the characteristics of tropical air.

Waugh, D. W.↗
NASA NTRS1993

Observations of upper atmospheric optical flashes recorded from an aircraft

Short-duration upper atmospheric optical flashes were recorded on the night of 8 July, 1993 (9 July UT) from the NASA DC-8 Airborne Laboratory flying over the American Midwest. All-sky video images from an intensified silicon intensified target (ISIT) camera revealed 19 upper atmospheric flashes occurring over a period of approximately 100 min. The flashes were similar in appearance to previously reported ground and shuttle-based video observations. Detailed analysis of 12 of the events yielded these parameters: (1) duration less than or equal to 17 ms; (2) brightness 10-50 kR, roughly that of bright aurorae; (3) terminal heights 30-100 km, with a mean of approximately 60 km; (4) horizontal extent 10-50 km; (5) emission volumes greater than 1000 cu km. The relative frequency of the optical flashes was (6) 1:200-1:400 compared to negative cloud-to-ground discharges and 1:20-1:40 compared to positive cloud-to-ground discharges.

Sentman, D. D.↗
NASA NTRS1994

Aerosol Abundances and Optical Characteristics in the Pacific Basin Free Troposphere

During NASA's Global Backscatter Experiment (GLOBE) mission flights in November 1989 and May 1990, a DC-8 research aircraft probed the Pacific Basin free troposphere for about 90 flight hours in each month between +72 and -62 degrees latitude, +130 and -120 degrees longitude, and up to 39,000 feet pressure altitudes. Aerosols were sampled continuously in situ by optical particle counters to measure concentration and particle size, and during 48 10-min intervals during each mission by wire impactors for concentration, size, composition, phase and shape analyses. The optical particle counters cover a particle diameter range between 0.3 and 20 microns; wire impactors extend the range down to 0.03 microns. Results of particle number, size, shape, together with the assumption of a refractive index corresponding to (NH4)2SO4 to account for the prevalence of aerosol sulfur, were utilized in a Mie algorithm to calculate aerosol extinction and backscatter for a range of wavelengths (0.385 less than lambda less than 10.64 microns). Computations for 22 randomly selected size distributions yield coefficients of extinction E(0.525) = (2.03 +/- 1.20) x 10(exp -4) km(exp -1) and backscatter beta(0.525) = (6.45 +/- 3.49) x 10(exp -6) km(exp -1) sr(exp -1) in the visible, and E(10.64) = (8.13 +/- 6.47) x 10(exp -6) km(exp -1) and beta(10.64) = (9.98 +/- 10.69) x 10(exp -8) km(exp -1) sr(exp -1) in the infrared, respectively. Large particles (D greater than 0.3 microns) contribute two-thirds to the total extinction in the visible (lambda = 0.525 microns), and almost 100% in the infrared (lambda = 10.64 microns). These results have been used to define an IR optical aerosol climatology of the Pacific Basin free troposphere, from which it follows that the infrared backscatter coefficient at lambda = 9.25 microns wavelength fluctuates between 5.0 x 10(exp -10) and 2.0 x 10(exp -7) km(exp -1) sr(exp -1) with a modal value 2.0 x 10(exp -8) km(exp -1) sr(exp -1).

Pueschel, R. F.↗
NASA NTRS1993

Observations of Upper Atmospheric Optical Flashes Recorded From an Aircraft

Short-duration upper atmospheric optical flashes were recorded on the night of 8 July, 1993 (9 July UT) from the NASA DC-8 Airborne Laboratory flying over the American Midwest. All-sky video images from an intensified silicon intensified target (ISIT) camera revealed 19 upper atmospheric flashes occurring over a period of approximately 100 min. The flashes were similar in appearance to previously reported ground and shuttle-based video observations. Detailed analysis of 12 of the events yielded these parameters: (1) duration less than or = 17 ms; (2) brightness 10-50 kR, roughly that of bright aurorae; (3) terminal heights 30-100 km, with a mean of approximately 60 km; (4) horizontal extent 10-50 km; and (5) emission volume greater than 1000 km(sup 3). The relative frequency of the optical flashes was (6) 1:200-1:400 compared to negative cloud-to-ground discharges and 1:20-1:40 compared to positive cloud-to-ground discharges.

Sentman, D. D.↗
NASA NTRS1993

Post-Pinatubo Optical Depth Spectra VS. Latitude and Vortex Structure: Airborne Tracking Sunphotometer Measurements in AASE 2

In January and March 1992, DC-8-measured stratospheric particle optical depth spectra, (tau)(sub p)(lambda), peaked broadly at midvisible or longer wavelengths. At mid-to-high northern latitudes outside the vortex, tau(sub p)(526 microns) above about 11 km was as large as 0.22 in both January and March, reflecting continued Pinatubo volcanic influence. In both months, in-vortex tau(sub p) above 11 km was smaller than outside-vortex values by a factor of two or more, and in January a strong anticorrelation was observed between tau(sub p)(lambda) and HF column content (an indicator of vortex penetration). In late January at 18-20S, near the edge of the southern subtropical jet, tau(sub p)(526 microns) above 12 km was only about 0.07- 0.09, with a flatter spectral shape than northern mid-to high-latitude measurements in both January and March. Occasional high-latitude vertical profiles indicate 6-1 km slab optical depths, delta(tau)(sub p)(526 micron), of 0.05 to 0.1, which should be added to the above-11-km values to yield values above 6 km.

Russell, P. B.↗
NASA NTRS1993

Airborne Arctic Stratospheric Expedition 2: Air Parcel Trajectories

An overview of Airborne Arctic Stratospheric Expedition 2 is given. Effects of Pinatubo aerosol on stratospheric ozone at mid-latitudes, in situ measurements of ClO and ClO/HCl ratio, balloon-borne measurements of ClO, NO, and O3 in a volcanic cloud, and new observations of the NO(y)/N2O correlation in the lower stratosphere are discussed. Among other topics addressed are the following: in situ tracer correlations of methane, nitrous oxide, and ozone as observed aboard the DC-8, in situ measurements of changes in stratospheric aerosol and the N2O-aerosol relationship inside and outside of the polar vortex, measurements of halogenated organic compounds near the tropical tropopause, and airborne brightness measurements of the polar winter troposphere.

Source record↗
NASA NTRS1993

Airborne Arctic Stratospheric Expedition 2: An Overview

The sudden onset of ozone depletion in the antarctic vortex set a precedent for both the time scale and the severity of global change. The Airborne Antarctic Ozone Experiment (AAOE), staged from Punta Arenas, Chile, in 1987, established that CFCs, halons, and methyl bromide, the dominant sources of chlorine and bromine radicals in the stratosphere, control the rate of ozone destruction over the Antarctic; that the vortex is depleted in reactive nitrogen and water vapor; and that diabatic cooling during the antarctic winter leads to subsidence within the vortex core, importing air from higher altitudes and lower latitudes. This last conclusion is based on observed dramatic distortion in the tracer fields, most notably N2O. In 1989, the first Airborne Arctic Stratospheric Expedition (AASE-I), staged from Stavanger, Norway, and using the same aircraft employed for AAOE (the NASA ER-2 and the NASA DC-8), discovered that while NO(x) and to some degree NO(y) were perturbed within the arctic vortex, there was little evidence for desiccation. Under these (in contrast to the antarctic) marginally perturbed conditions, however, Cl0 was found to be dramatically enhanced such that a large fraction of the available (inorganic) chlorine resided in the form of Cl0 and its dimer ClOOCl. This leaves two abiding issues for the northern hemisphere and the mission of the second Airborne Arctic Stratospheric Expedition (AASE-II): (1) Will significant ozone erosion occur within the arctic vortex in the next ten years as chlorine loading in the stratosphere exceeds four parts per billion by volume? and (2) Which mechanisms are responsible for the observed ozone erosion poleward of 30 deg N in the winter/spring northern hemisphere reported in satellite observations?

Anderson, James G.↗
NASA NTRS1993

AASE-2 Observations of Trace Carbon Species Distributions in the Mid to Upper Troposphere

We report tropospheric (altitudes greater than 5 km) observations of CO2, CO, CH4, and light hydrocarbons (C2-C4) over the latitude range from 90 deg N to 23 deg S recorded onboard the NASA DC-8 aircraft during the winter 1992 Second Airborne Arctic Stratospheric Expedition (AASE-II). Mixing ratios for these species exhibited significant north-south gradients with maximum values in subpolar and arctic regions and minima over the southern tropics. At latitudes greater than 40 deg N, the mixing ratios of most species increased significantly over the course of the 3-month measurement period. Also at high northern latitudes, the variations of all relatively long-lived reactive carbon species were linearly correlated with fluctuations of CO2 with CO, CH4, C2H6, C2H2, C3H8, and n-C4H10 exhibiting average enhancement ratios in terms of ppbv(X)/ppmv(CO2) of 13.8, 8.4, 0.21, 0.075, 0.085, and 0.037, respectively.

Anderson, B. E.↗
NASA NTRS1993

Post-Pinatubo Optical Depth Spectra vs Latitude and Vortex Structure: Airborne Tracking Sunphotometer Measurements in AASE 2

In January and March 1992, DC-8-measured stratospheric particle optical depth spectra, tau(sub p)(lambda), peaked broadly at midvisible or longer wavelengths. At mid-to-high northern latitudes outside the vortex, tau(sub p)(526 nm) nm) above about 11 km was as large as 0.22 in both January and March, reflecting continued Pinatubo volcanic influence. In both months, in-vortex tau(sub p)(lambda) above 11 km was smaller than outside-vortex values by a factor of two or more, and in January a strong anticorrelation was observed between tau(sub p)(lambda) and HF column content (an indicator of vortex penetration). In late January at 18-20S, near the edge of the southern subtropical jet, tau(sub p)(526 nm) above 12 km was only about 0.07-0.09, with a flatter spectral shape than northern mid- to high-latitude measurements in both January and March. Occasional high-latitude vertical profiles indicate 6-11-km slab optical depths, Delta tau(sub p)(526 nm), of 0.05 to 0.1, which should be added to the above-11-km values to yield values above 6 km.

Russell, P. B.↗
NASA NTRS1993

Airborne Brightness Temperature Measurements of the Polar Winter Troposphere as Part of the Airborne Arctic Stratosphere Experiment 2 and the Effect of Brightness Temperature Variations on the Diabatic Heating in the Lower Stratosphere

In this paper we report radiometric measurements of tropospheric brightness temperatures obtained during the AASE 2 experiment. These measurements represent the first attempt to characterize effective radiative temperatures as seen from above the troposphere during the Arctic winter. The reported measurements include brightness temperatures at 6.7 and 10.5 micrometers as seen from the NASA DC-8 aircraft flying at about 11 km altitude. We also present radiative transfer calculations to estimate the effect of tropospheric brightness temperature on the lower stratospheric heating rates. Because of the recent massive eruption of the Pinatubo volcano, we also discuss the effects of a volcanic aerosol layer. It is concluded that small particles like the volcanic aerosol or PSCs type 1 do not affect stratospheric heating rates by much; on the other hand, larger particles, PSCs types 2 and 3, may have significant effects on heating rates and consequently on dynamics of the lower stratosphere. The dynamical effects of local stratospheric temperature variations are briefly discussed.

Valero, Francisoco P. J.↗
NASA NTRS1992

Black Carbon (Soot) Aerosol in the Lower Stratosphere and Upper Troposphere

We have used two approaches to measure BCA in the stratosphere. The first method consists of collecting aerosols by impaction on quartz rods, upon which are mounted strips of polystyrene filter material. Each 25 mm by 0.5 mm filter strip is alternately masked and exposed in 5 mm long sections. After sampling, the optical density of the exposed sections is measured and compared with the optical density of the masked (unexposed) sections. The filter strip is a Lambertian collector, the scattering property of which is not affected by the deposition of liquid sulfuric acid droplets which dominate the stratospheric aerosol. Hence, all attenuation greater in the exposed than in the non-exposed sections is due to absorption by BCA or rare opaque materials such as meteoritic iron. In a second approach we expose carbon-coated gold or palladium wires to air outside the aircraft boundary layer [Farlow et al., 1979; Pueschel et al., 1989]. With a field emission scanning electron microscope we are able to characterize BCA particles in addition to the dominant sulfuric acid droplets. Typically, soot is comprised of 20 nm diameter spheres linked together as branching chains or loosely packed aggregates (Figure 1a). The microscope has a lateral image resolution of 1.5 nm and can clearly resolve individual spheres making up BCA aggregates. Their morphology is uniquely different from that of the liquid sulfuric acid-water aerosol (Figure 1b). We approximate the size of each BCA particle by that of a sphere of equivalent volume and fit a lognormal size distribution to both the BCA and H2SO4/H2O aerosols. Both sampler types have been mounted on NASA's ER-2 high-altitude research aircraft (altitude ceiling of 70,000 feet), and on NASA's DC-8 (40,000 feet ceiling) aircraft to sample aerosols from a significant portion of the atmosphere.

Pueschel, R. F.↗
NASA NTRS1994

Cloud-Aerosol Interactions in Tropical Storms

During the Coupled Ocean-Atmosphere Response Experiment (COARE) of the Tropical Ocean and the Global Atmosphere (TOGA) program we measured cloud and aerosol particles aboard the NASA DC-8 over the warm pool of the western Pacific. Instruments on the aircraft included a condensation nuclei counter, optical particle counters, two-dimensional shadow probes and an ice crystal replicator. The size range covered by these instruments was from =0.01 micron to 6.4 mm diameter; particle shapes were determined for particles of sizes D greater than 1 micron.

Puesschel, R. F.↗
NASA NTRS1994

Direct Monitoring of Trace Atmospheric Species via Ion Trap Mass Spectrometry

There is an ever-increasing emphasis on the part of government agencies, academia, and industry on enhancing our understanding of atmospheric processes and assessing the impact of human activities on these processes. While issues such as the ozone hole and rising levels of greenhouse gases have received major attention. relatively little is known about the types, concentrations, sources, and sinks of hydrocarbons in the troposphere and stratosphere. Such information would be of tremendous utility in assessing the roles of various anthropogenic and biogenic processes on global carbon cycles. An ion trap mass spectrometer has been developed for monitoring trace levels of hydrocarbons in the atmosphere on NASA's DC-8 "flying laboratory". This aircraft is used to provide measurements in support of a number of "Mission to Planet Earth" activities and tropospheric chemistry experiments. In past missions, specific compounds have been monitored via highly specialized instrumentation, fast GO, or collection of whole air samples for subsequent ground-based analysis. The ion trap has several features. including small size. excellent sensitivity, and broad applicability, which make it highly atttrat:ive for atmospheric monitoring. The design of this instrument, its air sampling interface. and the various complications associated with aircraft-deployment will be described. Data showing the sensitivity of the instrument for detecting hydrocarbons at mixing ratios below one part-per-billion, and the use of MS/MS for direct, on-line, real-time monitoring will be presented.

Palmer, P. T.↗
NASA NTRS1994

ARMAR Observations during TOGA/COARE

The NASA/JPL Airborne Rain Mapping Radar (ARMAR) was deployed for rainfall observations during TOGA/COARE on the NASA DC-8 aircraft. A total of approx. 30 hours of rain profiling measurements were collected over the Western Pacific Ocean during January and February 1993.

radar bright bands rain attenuation study Airborne↗