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At least 199 records · Page 11

SILICON CARBIDE THERMOMETRY USING RAMAN SPECTROSCOPY ON IRRADIATED TRISO PARTICLES

Silicon carbide (SiC) passive thermometry has emerged as a promising post-irradiation examination (PIE) technique for estimating irradiation temperature near the end of irradiation. While dilatometry techniques have been traditionally used to analyze prismatic samples after irradiation, Raman spectroscopy has recently been shown to provide comparable results by analyzing Raman-active phonon modes. In this work, Raman spectroscopy has been applied to the SiC layer of cross-sectioned irradiation tristructural isotropic (TRISO) particles from the AGR-5/6/7 experiment to evaluate the feasibility of particle-scale passive thermometry. Two-dimensional Raman mapping was used to measure the position of the SiC longitudinal optical (LO) phonon, which was then converted to an apparent irradiation temperature using a previously established empirical correlation. Particles from AGR-5/6/7 Compacts 2-2-1 and 5-1-3 were selected as their calculated time-averaged, volume-averaged (TAVA) temperatures (828°C and 706°C, respectively) fall within the range of the sensitivity of the experimental approach. The use of SiC thermometry was anticipated to confirm or highlight potential deviations from calculated end-of-life TAVA temperature across compacts. Four particles from Compact 2-2-1 and two particles from Compact 5-1-3 were selected based on 110mAg inventory (either some measurable activity or below the minimum detection limit) which is commonly used as an indicator of in-pile temperature variation of particles within the same compact. Across every particle selected it was determined that the average LO peak position was located around 968 cm-1 to 969 cm-1. Using the previously determined empirical correlation, this corresponds to an irradiation temperature around 950°C to 966°C, which does not align with the reported TAVA temperature values. This discrepancy in apparent irradiation temperatures likely reflects a combination of uncertainties in the calculated particle temperatures and differences in irradiation history between the present specimens and those used to establish the empirical Raman calibration such as neutron flux (damage rate) and SiC microstructure (as fabricated and irradiated).

Vawdrey, Josh [ORNL]↗

Investigation of the Origins of Comets as Revealed through Infrared High-resolution Spectroscopy I. Molecular Abundances

We report and analyze updated molecular abundances in 20 comets obtained by employing modern data reduction procedures and molecular models. Using box and scatter plots, we examine how the different molecular species are distributed among the comet population, while by means of pie charts, we investigate the relative proportions of these molecular species in each comet. We compare these results with the orbital parameters of the selected comets to identify trends related to their dynamical history. With these analyses, we tentatively identify at least three chemical classes based mainly on relative abundances of CO, CH{sub 3}OH, CH{sub 4}, C{sub 2}H{sub 6}, HCN, and NH{sub 3}. The combination of relative abundances and orbital parameters is then compared with recent chemical models of planetary system formation. This approach may help in investigating the origins and evolution of the material in cometary nuclei. Among other aspects, we underline the need to increase our sample size, especially for hypervolatiles (i.e., CH{sub 4} and CO) in Jupiter family comets.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Remote Fiber Based Velocimeter For Interface Strength Measurements

The understanding of the performance of nuclear reactor plate fuels is essential when developing new fuel systems. The condition of pre and post irradiated plate fuels must be characterized effectively and efficiently prior to irradiation and then post irradiation within a high rad environment. The post characterization work must be performed remotely and in an environment hostile to instrumentation. Laser based characterization methods provide the capability to be remote and robust within a hot-cell environment. Laser based characterization can provide high spatial resolution appropriate for scanning and imaging large areas. The INL is currently developing a laser shock system for Post Irradiation Examination (PIE) station for use in the Hot Fuel Examination Facility (HFEF) at the INL. The laser shock system is designed to characterize fuel to cladding and cladding to cladding interface strength. The laser shock-technique induces large amplitude shock waves to mechanically characterize interfaces such as the fuel-clad interface. The shock wave propagates as a compressional wave through the fuel plate to the free (unconfined) backside surface and is reflected back through the test plate as a rarefaction (tensile) wave. This rarefaction wave is the physical mechanism that produces internal delamination failure. The focus or this paper is on the accurate measurement of surface velocity to quantify the amount of energy traveling through the interfaces to the back surface of the fuel plate. The original fiber based velocimeter design was biased by parasitic back reflections. This paper will discuss the discovery of the back-reflection issue and the design changes to resolve the issue. Supporting data will be presented.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

As-run physics analysis for the EPRI-3 experiment for cycles 155B and 158B

The purpose of this Engineering Calculations Analysis Report (ECAR) is to document the as-run heat generation rates (W/g), flux/fluence, radio-isotopic source term in Curies and grams, decay heat rate in Watts, and specimen DPA for the post-irradiation shipment and examination of the Electric Power Research Institute (EPRI)-3-1 and EPRI-3-2 experiments. EPRI-3-1 was irradiated during cycle 155B ending April 12, 2014. EPRI-3-2, a modification of EPRI-3-1, was irradiated during cycle 158B ending April 1, 2016. Source term, decay heat rate, and DPA calculations were based on scaled Monte Carlo N-Particle (MCNP) calculated fluxes for the EPRI-3-2 experiment. Although EPRI-3-2 is a modification of EPRI-3-1, no significant changes were made in the placement of experiment specimens. Calculated fluxes were scaled using as-run center lobe source powers of the corresponding irradiation cycles for EPRI-3-1 and EPRI-3-2. ORIGEN2 Version 2.2 was used to determine the decay heat rate and source term for the EPRI-3 experiment. The source term analysis was performed as requested by the project staff. The results of this analysis may be used to demonstrate compliance with shipping requirements in the BEA Research Reactor (BRR) cask following irradiation as well as to provide as-run source term to support Post-Irradiation Examination (PIE).

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

As-Run Physics Analysis for the EPRI-1 Experiment

The purpose of this ECAR is to document the as-run physics analysis for the Electric Power Research Institute (EPRI)-1 experiment located in the Center Flux Trap (CFT). EPRI-1 was irradiated during cycle 157C. The experiment irradiation ended on February 15, 2015. The as-run heat rates, DPA, and flux/fluence results were calculated using the Monte Carlo N-Particle (MCNP) Advanced Test Reactor (ATR) full core model. The heat rates, DPA, and flux are calculated based on an average center lobe power of 21.1 MW. The fluence and DPA is based on the operating time of 5.4 days. ORIGEN2 Version 2.2 was used to calculate the isotopic concentration in grams for the EPRI-1 experiment. The source term analysis was performed as requested by the project staff. The results of this analysis may be used to support Post-Irradiation Examination (PIE)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

AGR-5/6/7 Experiment Monitoring and Simulation Progress

Advanced Gas Reactor (AGR)--5/6/7 is the last of a series of AGR experiments conducted in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL) in support of development and qualification of tri-structural isotropic (TRISO) low-enriched fuel for use in high temperature gas-cooled reactors. The test train contains five separate capsules that are independently controlled and monitored. Each capsule contains multiple 12.51 mm long compacts filled with low-enriched uranium carbide/oxide (UCO) TRISO fuel particles. The objectives of the AGR-5/6/7 experiment are to: 1. Irradiate reference-design fuel particles to support fuel qualification. 2. Establish operating margins for the fuel beyond normal operating conditions. 3. Provide irradiated fuel performance data and irradiated fuel samples for post-irradiation examination (PIE) and safety testing.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

AGR 5/6/7 Data Qualification Report for ATR Cycles 162B through 168A

This report provides the qualification status of experimental data for the Advanced Gas Reactor (AGR) 5/6/7 fuel irradiation. AGR-5/6/7 was conducted in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL) in support of development and qualification of tri-structural isotropic (TRISO) low-enriched fuel for use in high temperature gas-cooled reactors. The objectives of the AGR-5/6/7 experiments are to: (i) irradiate reference-design fuel particles to support fuel qualification, (ii) establish operating margins for the fuel beyond normal operating conditions, and (iii) provide irradiated-fuel performance data and irradiated-fuel samples for post-irradiation examination (PIE) and safety testing. The test train contains five separate capsules that were independently controlled and monitored. Each capsule contains multiple 12.51-mm-long compacts filled with low enriched uranium carbide/oxide (UCO) TRISO fuel particles. The primary objective of the AGR-5/6 test (Capsules 1, 2, 4, and 5) is to verify successful performance of the reference-design fuel under normal operating conditions. The AGR-7 test (Capsule 3) was designed to explore fuel performance at higher temperatures to demonstrate the capability of the fuel to withstand conditions beyond normal operating conditions in support of plant design and licensing. AGR 5/6/7 will also provide irradiated-fuel performance data on fission-gas release from failed particles during irradiation. The AGR-5/6/7 capsules were irradiated in the ATR northeast flux trap location. The experiment began on February 16, 2018 and ended on July 22, 2020, spanning nine ATR cycles over two and a half years. Thus, the AGR-5/6/7 fuel compacts were irradiated for a total of 360.9 effective full power days. The AGR 5/6/7 experiment was able to remain in the reactor core during all three Powered Axial Locator Mechanism (PALM) cycles (163A, 165A, and 167A) without overheating its fuel compacts. This report includes irradiation monitoring data from nine ATR Cycles: 162B, 163A, 164A, 164B, 165A, 166A, 166B, 167A, and 168A, as stored in the Nuclear Data Management and Analysis System (NDMAS). During irradiation, data records consisted of instantaneous measurements recorded every minute and provided by text files automatically every 2 hours. The AGR 5/6/7 data streams addressed in this report include thermocouple (TC) temperatures, sweep gas data (flow rates [capsule inlet, outlet, and downstream at detector], pressure, and moisture content), and Fission Product Monitoring System (FPMS) data (release rates and release to birth rate ratios [R/Bs]) for each of the five capsules. A total of 94,989,908 TC temperature and sweep gas data records were received and processed by NDMAS for AGR 5/6/7 irradiation. Of these records, 41,593,387 (or 43.7% of the total) met data collection and accuracy requirements and are labeled as Qualified. A total of 57,746,693 TC temperature readings were captured from 54 installed TCs. Among them, 10,034,676 TC temperature records (only 17.4%) were Qualified and 47,701,371 TC temperatures (or 82.6%) are Failed due to 48 TC failures (63.5%) and due to missing values (19.1%). To assess performance of the operational TCs, analysis of daily correlations between TCs found no evidence of virtual junction failure for any TCs. Analyses on control charts of TC temperature differences revealed trending in TC readings for TC2, 4, 5, and 13 in Capsule 3, but there is no conclusive indication of TC drift failure that caused those trends. Therefore, TC control charts are not used to disqualify TC data, but only for users’ consideration. For sweep gas flow rates, a total of 31,519,747 gas flow records (84.4%) are Qualified for use for AGR-5/6/7 experiment; 5,723,468 gas flow records (15.4%) are Failed due mostly to missing values; and 74,641 high sweep gas flow rates (0.2 %) are Trend. A large number of Failed missing TC temperature and gas flow values were caused by an error in the data output script that outputted a ‘NULL’ value when values were unchanged. This problem was fixed during the outage of Cycle 166B, which led to a substantially decreased number of missing values during the last three cycles. Nonetheless, a large amount of non-missing data remained because of the high data acquisition frequency (1-minute) and still provided sufficient data to effectively monitor the experiment as designed. For FPMS data, NDMAS received and processed fission product release and R/B data for nine ATR cycles, when ATR core reached full power during AGR 5/6/7 irradiation. These data consist of 110,388 release rate records and 110,388 R/B records for the twelve radionuclides (Kr 85m, Kr 87, Kr 88, Kr 89, Kr 90, Xe 131m, Xe 133, Xe 135, Xe 135m, Xe 137, Xe 138, and Xe 139) for each of the five capsules. Equivalent numbers of uncertainty records associated the release rates and R/B values were provided. To date, qualification status of the FPMS data stored in the NDMAS dat

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Fatigue Test Result for High Burnup Pressurized Water Reactor Rods

The High Burnup Spent Fuel Data Project, sponsored by DOE-NE, is focused on understanding the effects of long-term storage and transportation on high burnup (HBU) (>45 gigawatt days per metric ton uranium) light water reactor fuel. The experiment includes 32 HBU spent nuclear fuel (SNF) assemblies that will be stored in a typical Independent Spent Fuel Storage Installation (ISFSI) and 25 sister rods - nine SNF rods that were removed from the fuel assemblies prior to insertion to the ISFSI and 16 SNF rods removed from similar HBU assemblies. The sister rods provide a baseline of the condition of the HBU rods prior to loading, drying, and long-term dry storage. Destructive examinations of the sister rods are focused on understanding overall SNF rod strength and durability. Both composite fuel and empty cladding will be tested to derive material properties. While the data generated can be used for multiple purposes, a primary goal of the sister rod PIE data and associated measured mechanical properties is to support existing fuel storage licensing and relicensing activities by addressing identified knowledge gaps, and enhance the technical basis for post-storage transportation, handling, and consolidation activities. Fatigue tests of HBU M5-clad, ZIRLO-clad, Zircaloy-4, and low tin Zircaloy-4 segments have been completed using ORNL’s Cyclic Integral Reversible Fatigue Tester (CIRFT). This is the first time ZIRLO-clad rods have been tested. Some of the segments were heat-treated to understand the effects of thermal transients such as those encountered during dry storage vacuum drying on the fatigue lifetime. This paper presents results of the fatigue tests obtained to date and discusses planned future tests.

Montgomery, Rose↗

AGR-5/6/7 Experiment Monitoring and Simulation Progress

Advanced Gas Reactor (AGR)--5/6/7 is the last of a series of AGR experiments conducted in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL) in support of development and qualification of tri-structural isotropic (TRISO) low-enriched fuel for use in high temperature gas-cooled reactors. The test train contains five separate capsules that are independently controlled and monitored. Each capsule contains multiple 12.51 mm long compacts filled with low-enriched uranium carbide/oxide (UCO) TRISO fuel particles. The objectives of the AGR-5/6/7 experiment are to: 1. Irradiate reference-design fuel particles to support fuel qualification. 2. Establish operating margins for the fuel beyond normal operating conditions. 3. Provide irradiated fuel performance data and irradiated fuel samples for post-irradiation examination (PIE) and safety testing.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

PLN-6268 Yttrium Hydride Post Irradiation Examination Plan

The overarching goal of the Department of Energy Office of Nuclear Energy (DOE-NE) microreactor program is to develop technologies for the deployment of civilian microreactors by stakeholders1. Microreactors are expressed as advanced transportable nuclear reactors operating at low power (<20MWth) but high temperatures (>600°C), as well as plug-and-play and inherently safe designs. One prerequisite of a microreactor is the compactness, so that a truck can transport the reactor under safe conditions with the current road infrastructure1,2. The compactness of these reactors likely can be attainable by use of solid components for the essentials of the nuclear core, such as fuel, core heat removal components, reflectors, and moderators. Among these essentials, where fuel enrichment must remain < 20% to meet High Assay Low Enrichment Uranium criteria (HALEU), the largest contribution to the compactness is offered by use of solid moderators which benefit from light atomic weight elements, such as hydrogen, carbon, and beryllium2. Among these, hydrogen-bearing materials, such as metal hydrides, are superior to other options from the lowest critical mass standpoint. Noting that, factors other than critical mass should be considered for a specific reactor design. Yttrium- or zirconium-based metal hydrides have been down-selected due to their neutronic performance. In addition to the neutronic perspective, maintaining hydrogen within the metal hydride is important at the high operating temperatures proposed by advanced reactors. Yttrium hydride (YHx) is, therefore, a proposed moderator material that offers better hydrogen retention at higher operating temperatures than zirconium hydrides due to higher retention and thermal stability of hydrogen in the metal3. The irradiated materials properties of metal hydrides, in this case YHx, must be assessed for the qualification of these moderators. Material testing and inspection processes must illustrate that the effects of dimensional and property changes on thermophysical and mechanical properties do not cause any significant changes on the microreactor safety, and the moderating power is maintained within design limits. Thus, the effect of irradiation on the thermophysical and mechanical properties must be determined. This post-irradiation examination (PIE) plan specifically aims to determine these properties for YHx following Advanced Test Reactor (ATR) irradiation.

99 GENERAL AND MISCELLANEOUS↗

ECAR-1943 AGC-1 INDIVIDUAL SPECIMEN FLUENCE, TEMPERATURE, AND LOAD CALCULATION AND TABULATION

This ECAR calculates the fluence and temperature of the AGC-1 specimens as they change elevation through the course of the experiment. The specimen elevation varies as the specimen stack shrinks due to irradiation and load induced creep. The compressed specimen stacks (S-1 thru S-6) have a graphite pushrod that applies a gas cylinder load. The top of the pushrod position is measured and recorded in the NGNP Data Management and Analysis System (NDMAS). The bottom of each of these compressed stacks is supported by the lower specimen holder which also shrinks as a result of irradiation and load. The specimen holder post-irradiation length was recorded during post-irradiation examination (PIE). Assuming the specimen holder shrinkage is linear with respect to the fluence received, the position of the top of the specimen holder can be calculated with respect to reactor integrated power. Assuming that individual specimen shrinkage is proportional to the fluence received, and that the shrinkage behavior is similar in all the specimens, the individual specimen position can be calculated.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Initial Observations from AGR 5/6/7 Capsule 1

The fourth and final irradiation experiment in the Advanced Reactor Technologies (ART) Advanced Gas Reactor (AGR) fuel development and qualification program is designated as AGR-5/6/7. Data collected from the fabrication, irradiation, and post-irradiation examination (PIE) of this tristructural isotropic (TRISO) fuel are intended to serve as the primary data set for the qualification of this fuel for use in high-temperature gas-cooled reactors (INL 2021, Collin 2018b). However, data collected from the three preceding irradiations (i.e., AGR-1, AGR-2, and AGR-3/4) may also be used to supplement data collected from AGR-5/6/7. All components of the AGR-5/6/7 fuel (i.e., UCO kernels, TRISO coatings, and fuel compacts) were produced on an engineering scale at BWXT (Lynchburg, Virginia USA) according to the fuel specification (Marshall 2017). This fuel was irradiated in the northeast flux trap (NEFT) at the Advanced Test Reactor (ATR) at Idaho national Laboratory (INL) from February 16, 2018 to July 22, 2020 (Pham et al. 2021). Measurements in the fission product monitoring system (FPMS) indicated unexpected and significant numbers of failures of TRISO particles in Capsule 1 near the end of the sixth irradiation cycle (ATR Cycle 166A). In the fourth cycle (ATR Cycle 164B) and beyond, the sweep gas flow became very low (presumably from degradation of the capsule gas outlet line via an unidentified mechanism), and the program deliberately isolated Capsule 1 from gas flow periodically. In later cycles, attempts to reestablish any kind of flow in Capsule 1 were unsuccessful. With little or no flow through Capsule 1, FPMS measurements and enumerations of failed particles in Capsule 1 were difficult or impossible as was the ability to control the helium/neon gas mixture used for temperature control. Gas flows and fission gas activity in the effluent gas from the other AGR-5/6/7 capsules were also impacted by the Capsule 1 gas flow issues and the large increase in fission gas released from the Capsule 1.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Development of Accelerated Steady-state Test Capsule Experiments to Replicate EBR-II Fuel Behavior Using BISON Fuel Performance Analysis

Here in this work, BISON fuel performance calculations were performed to predict the fuel behavior of accelerated burnup U-Pu-Zr fuel, with temperature operation conditions of the fuel and the cladding mirroring conditions within EBR-II fuel pins. The temperature operating conditions within the FAST accelerated burnup rods were aimed at replicating EBR-II X447/X447A fuel surface and inner cladding surface temperatures. Due to the FAST capsule design, these temperatures can be replicated with fission rate densities being significantly increased. fuel performance modeling has not been assessed for novel experiments such as accelerated burnup utilizing the FAST capsule within ATR. This is an important step in understanding accelerated irradiation methods as many performance models are empirical models conforming to the results of PIE but do not always include physical models that would represent the changes in irradiation tests.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

AGR-2 Compact 6-4-1 Post-Irradiation Examination Results

The Advanced Gas Reactor (AGR) Fuel Development and Qualification Program was established to perform research and development on tristructural isotropic (TRISO)-coated particle fuel to support deployment of a high-temperature gas-cooled reactor (HTGR). The work continues as part of the Advanced Reactor Technologies (ART) TRISO Fuel Program. The overarching goal of the program is to provide a baseline fuel qualification data set to support licensing and operation of an HTGR. To achieve these goals, the program includes the elements of fuel fabrication, irradiation, post-irradiation examination (PIE) and safety/heating testing, fuel performance modeling, and fission product transport (INL 2017). Several fuel irradiation experiments have been performed at the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL), and additional irradiations are planned. These experiments are intended to provide data on fuel performance under irradiation, support fuel fabrication process development, qualify fuel for operating and accident conditions, provide irradiated fuel for accident testing, and support development of fuel performance and fission product transport models.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Accelerating Nuclear Fuels and Materials Qualification-Learning from MeV Summer School 2022

This presentation focused on the general overview of the lecture content that related to nuclear fuels and material qualification. The content of this presentation is taken from the lecture notes of MeV Summer School 2022. The sources are cited as per lecture notes. The focus of this presentation is to review the learning from the Modeling, Experiment, and Validation (MeV) Summer School (July 18-29, 2022) for early career researchers and scientists. This year's school was hosted by Oak Ridge National Laboratory (ORNL) and was focused on Accelerating nuclear fuels, and materials qualification by combining high through-put materials irradiation and testing, advanced PIE, and Multiphysics modeling.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Comparison of Fission Product Release Predictions using PARFUME and BISON with Results from the AGR-3/4 Irradiation Experiment

The PARFUME (PARticle Fuel ModEl) fuel performance modeling code and the BISON nuclear fuel performance application built on the Multiphysics Object-Oriented Simulation Environment (MOOSE) finite element library were used to predict the fission product release from tristructural isotropic (TRISO) coated fuel particles and compacts during the third and fourth irradiation experiment of the Advanced Gas Reactor (AGR-3/4) Fuel Development and Qualification Program. The fuel performance modeling codes PARFUME and BISON modeled the AGR-3/4 irradiation experiment using the fuel compact time-averaged volume averaged (TAVA) daily temperatures for a total irradiation duration of 369.1 effective full power days (EFPD) to predict the release fraction of the fission product silver (Ag-110m) from a representative TRISO-coated fuel particle from AGR-3/4 compacts. Post-irradiation examination (PIE) measurements provided data on the release of these fission products in the compacts outside of the silicon carbide (SIC) layer. The PARFUME and BISON results were then compared to the silver release measured from compact gamma scanning. The results showed good agreement between PARFUME and BISON but both codes under-predicted the silver release fraction for all the compacts. In addition, BISON was used to model and predict the fission product concentration radial profile outside of the compacts in capsules’ inner and outer rings. These rings were either comprised of matrix and/or structural graphite. To obtain the concentration profiles of silver, cesium, and strontium, a sorption isotherm model was developed in BISON to capture the effects of fission product transport across the gaps between the concentric rings. The general shape of the concentration radial profiles as calculated by BISON were similar in the inner ring (IR) but varied in the outer ring (OR) depending on the fission product of interest or capsule temperature. Using this methodology and model, BISON now has the capability to aid in developing new fission product diffusion coefficients for matrix or structural graphite materials.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

BISON As-run AGR-3/4 Irradiation Test Predictions

BISON, a nuclear fuel performance application built using the Multiphysics Object-Oriented Simulation Environment (MOOSE) finite element library, was used to model the Advanced Gas Reactor (AGR)-3/4 irradiation test using as-run physics and thermal hydraulics data. The AGR-3/4 test consists of the combined third and fourth planned irradiations of the AGR Fuel Development and Qualification Program. The AGR-3/4 test train consists of twelve separate and independently controlled and monitored capsules. Each capsule contains four compacts filled with both uranium oxycarbide (UCO) unaltered “driver” fuel particles and UCO designed-to-fail (DTF) fuel particles. The DTF fraction was specified to be 1×10-2. This report documents the calculations performed to predict the failure probability of tristructural isotropic (TRISO) coated driver fuel particles during the AGR-3/4 experiment on a single compact. This report will demonstrate the capabilities of BISON to model the complex AGR-3/4 irradiation test and identify further development needed to capture the fuel particle failure probability and source term on every compact for further comparison from post-irradiation examination (PIE) data. The calculations include the modeling of the AGR-3/4 irradiation that occurred from December 2011 to April 2014 in the Advanced Test Reactor (ATR) over a total of 10 ATR cycles including seven normal cycles, one low power cycle, one unplanned outage cycle, and one Power Axial Locator Mechanism (PALM) cycle.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Fuel Performance Modeling Plan to Support the Advance Gas Reactor Program

This report documents the current status of the fuel performance modeling initiative to support the Advanced Gas Reactor (AGR) program in the development of tristructural isotropic (TRISO) coated fuel particles. A brief summary of the modeling codes that have been developed to support TRISO modeling is included along with a summary of the behavior of fuel particles during irradiation and the modeling used to capture these effects. In addition, this report identifies further modeling and material property needs that have been identified for further development based on experience from previously performed AGR experiments. In general, the remaining activities to support fuel performance modeling for the AGR program include continued AGR experiment support for AGR-3/4 and AGR-5/6/7 as well as modeling improvements identified throughout the course of the program. These modeling improvements can be summarized as the following: Fission product transport Thermomechanical particle behavior Additional modeling needs may be identified during the processing the data collected during the AGR post-irradiation examination (PIE) campaign and may lead to further modeling improvements that are not included in this report.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗