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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 199 records · Page 11

RCT Continuing Training: RCT Job Coverage and CONOPS

RCT Continuing Training covering all of the necessary steps associated with RCT, and how conduct of operations ties in with this process. The terminal objective of this training is: Given the need to perform radiological job coverage, recognize the requirements to maintain radiological work control in accordance with P121, Radiation Protection, RP-PROG-TP-200, Radiation Protection Manual, and P315, Conduct of Operations.

61 RADIATION PROTECTION AND DOSIMETRY↗

Improving the Capabilities and Computational Efficiency of the RTE+RRTMGP Radiation Code (Final Report)

This report details progress on the RTE+RRTMGP radiation codes made during the period of performance. RTE+RRTMGP is a set of codes for computing radiative fluxes in planetary atmospheres. RRTMGP uses a k-distribution to provide an optical description (absorption and possibly Rayleigh optical depth) of the gaseous atmosphere, along with the relevant source functions, on a pre-determined spectral grid given temperatures, pressures, and gas concentration. RTE computes fluxes given spectrally-resolved optical descriptions and source functions. Spectrally-resolved fluxes are summarized (“reduced”) via a user extensible class. The initial release of the code and the design choices are described in Pincus et al. 2019; the codes are available on Github. Although RRTMGP was based on current (at the time) empirical spectroscopic data, RTE and RRTMGP were developed in large part to modernize software practices. The design focused on flexibility broadly interpreted: by separating code from data and allowing data to drive computation; in coupling to the host model (e.g. the coupling of clouds to radiative fluxes is user-controlled); with respect to programming languages (computational tasks are accessed via widely-compatible C interfaces); and with respect to hardware (the codes run on a range of CPU and GPU architectures). The code also puts an emphasis on modularity and clarity. RTE+RRTMGP v1.0 was released in September 20219. This award supported the evolution of the RTE+RRTMGP code base to support greater flexibility, accuracy, and efficiency.

54 ENVIRONMENTAL SCIENCES↗

The response of the Amazon ecosystem to the photosynthetically active radiation fields: integrating impacts of biomass burning aerosol and clouds in the NASA GEOS Earth system model

The Amazon experiences fires every year, and the resulting biomass burning aerosols, together with cloud particles, influence the penetration of sunlight through the atmosphere, increasing the ratio of diffuse to direct photosynthetically active radiation (PAR) reaching the vegetation canopy and thereby potentially increasing ecosystem productivity. In this study, we use the NASA Goddard Earth Observing System (GEOS) model with coupled aerosol, cloud, radiation, and ecosystem modules to investigate the impact of Amazon biomass burning aerosols on ecosystem productivity, as well as the role of the Amazon's clouds in tempering this impact. The study focuses on a 7-year period (2010–2016) during which the Amazon experienced a variety of dynamic environments (e.g., La Niña, normal years, and El Niño). The direct radiative impact of biomass burning aerosols on ecosystem productivity – called here the aerosol diffuse radiation fertilization effect – is found to increase Amazonian gross primary production (GPP) by 2.6 % via a 3.8 % increase in diffuse PAR (DFPAR) despite a 5.4 % decrease in direct PAR (DRPAR) on multiyear average during burning seasons. On a monthly basis, this increase in GPP can be as large as 9.9 % (occurring in August 2010). Consequently, the net primary production (NPP) in the Amazon is increased by 1.5 %, or ~92 Tg C yr -1 – equivalent to ~37 % of the average carbon lost due to Amazon fires over the 7 years considered. Clouds, however, strongly regulate the effectiveness of the aerosol diffuse radiation fertilization effect. The efficiency of this fertilization effect is the highest in cloud-free conditions and linearly decreases with increasing cloud amount until the cloud fraction reaches ~0.8, at which point the aerosol-influenced light changes from being a stimulator to an inhibitor of plant growth. Nevertheless, interannual changes in the overall strength of the aerosol diffuse radiation fertilization effect are primarily controlled by the large interannual changes in biomass burning aerosols rather than by changes in cloudiness during the studied period.

54 ENVIRONMENTAL SCIENCES↗

Retrieving microphysical properties of concurrent pristine ice and snow using polarimetric radar observations

Abstract. Ice and mixed-phase clouds play a key role in our climate system because of their strong controls on global precipitation and radiation budget. Their microphysical properties have been characterized commonly by polarimetric radar measurements. However, there remains a lack of robust estimates of microphysical properties of concurrent pristine ice and aggregates because larger snow aggregates often dominate the radar signal and mask contributions of smaller pristine ice crystals. This paper presents a new method that separates the scattering signals of pristine ice embedded in snow aggregates in scanning polarimetric radar observations and retrieves their respective abundances and sizes for the first time. This method, dubbed ENCORE-ice, is built on an iterative stochastic ensemble retrieval framework. It provides the number concentration, ice water content, and effective mean diameter of pristine ice and snow aggregates with uncertainty estimates. Evaluations against synthetic observations show that the overall retrieval biases in the combined total microphysical properties are within 5 % and that the errors with respect to the truth are well within the retrieval uncertainty. The partitioning between pristine ice and snow aggregates also agrees well with the truth. Additional evaluations against in situ cloud probe measurements from a recent campaign for a stratiform cloud system are promising. Our median retrievals have a bias of 98 % in the total ice number concentration and 44 % in the total ice water content. This performance is generally better than the retrieval from empirical relationships. The ability to separate signals of different ice species and to provide their quantitative microphysical properties will open up many research opportunities, such as secondary ice production studies and model evaluations for ice microphysical processes.

54 ENVIRONMENTAL SCIENCES↗

Material Selection and Heat Transfer Model for PTUHS Device

The Path to Ultimate Heat Sink Device (PTUHS) is a passive safety system that utilizes a radiative heat transfer valve to control the rate at which heat is removed from a nuclear reactor pressure vessel (RPV) and dispersed into surrounding soil. The material selection for the PTUHS device is investigated, where the thermophysical properties are either maximized or minimized bases on what section of the PTUHS that material is being used for. Final recommendations of material choice are then presented. The heat transfer model of the PTUHS device is solved in ABAQUS, where a normal operating conditions and SCRAM conditions are solved. These temperature maps and heat flux of the system show the system's ability, where minimal heat is lost during normal operating conditions and system failure in a SCRAM scenario due to temperatures that were reached.

42 - ENGINEERING↗

Effect of natural gamma background radiation on portal monitor radioisotope unmixing

It is well known that national security relies on several layers of protection. One of the most important is the traffic control at borders and ports that exploits Radiation Portal Monitors (RPMs) to detect and deter potential smuggling attempts. Most portal monitors rely on plastic scintillators to detect gamma rays. Despite their poor energy resolution, their cost effectiveness and the possibility of growing them in large sizes make them the gamma-ray detector of choice in RPMs. Unmixing algorithms applied to organic scintillator spectra can be used to reliably identify the bare and unshielded radionuclides that triggered an alarm, even with fewer than 1000 detected counts and in the presence of two or three nuclides at the same time. In this work, we experimentally studied the robustness of a state-of-the-art unmixing algorithm to different radiation background spectra, due to varying atmospheric conditions, in the 16 °C to 28 °C temperature range. In the presence of background, the algorithm is able to identify the nuclides present in unknown radionuclide mixtures of three nuclides, when at least 1000 counts from the sources are detected. With fewer counts available, we found larger differences of approximately 35.9% between estimated nuclide fractions and actual ones. In these low count rate regimes, the uncertainty associated by our algorithm with the identified fractions could be an additional valuable tool to determine whether the identification is reliable or a longer measurement to increase the signal-to-noise ratio is needed. Moreover, the algorithm identification performances are consistent throughout different data sets, with negligible differences in the presence of background types of different intensity and spectral shape.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Real-time machine-learning-driven control system of a deformable mirror for achieving aberration-free X-ray wavefronts

A neural-network machine learning model is developed to control a bimorph adaptive mirror to achieve and preserve aberration-free coherent X-ray wavefronts at synchrotron radiation and free electron laser beamlines. The controller is trained on a mirror actuator response directly measured at a beamline with a real-time single-shot wavefront sensor, which uses a coded mask and wavelet-transform analysis. The system has been successfully tested on a bimorph deformable mirror at the 28-ID IDEA beamline of the Advanced Photon Source at Argonne National Laboratory. It achieved a response time of a few seconds and maintained desired wavefront shapes (e.g., a spherical wavefront) with sub-wavelength accuracy at 20 keV of X-ray energy. This result is significantly better than what can be obtained using a linear model of the mirror’s response. The developed system has not been tailored to a specific mirror and can be applied, in principle, to different kinds of bending mechanisms and actuators.

47 OTHER INSTRUMENTATION↗

Polarization and phase control of electron injection and acceleration in the plasma by a self-steepening laser pulse

Abstract We describe an interplay between two injection mechanism of background electrons into an evolving plasma bubble behind an intense laser pulse: one due to the overall bubble expansion, and another due to its periodic undulation. The two mechanisms occur simultaneously when an intense laser pulse propagating inside a plasma forms a shock-like steepened front. Periodic undulations of the plasma bubble along the laser propagation path can either inhibit or conspire with electron injection due to bubble expansion. We show that carrier-envelope-phase (CEP) controlled plasma bubble undulation induced by the self-steepening laser pulse produces a unique electron injector—expanding phase-controlled undulating bubble (EPUB). The longitudinal structure of the electron bunch injected by the EPUB can be controlled by laser polarization and power, resulting in high-charge (multiple nano-Coulombs) high-current (tens of kilo-amperes) electron beams with ultra-short (femtosecond-scale) temporal structure. Generation of high-energy betatron radiation with polarization- and CEP-controlled energy spectrum and angular distribution is analyzed as a promising application of EPUB-produced beams.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Radiation Mapping UAV [Poster]

The NuMI (Neutrinos at the Main Injector) target system delivers a high-energy flux of muon-neutrinos towards a detector more than 800 km away with the goal of better understanding the origin of the universe and its evolution. The target system becomes radioactive because it is irradiated by a sub-Mega-Watt power proton beam. Radiological hazard is one of critical issues for a radiological worker which limits the iractivities near the target system; however, they often need to quantify the radiation level of the target system manually. Thus, the objective of this project is to reduce their exposure to radiation while improving the accuracy of the measurements. A quadcopter UAV fitted with a radiation dosimeter is ideal to traverse the irradiated environment as it can be deployed in any space and requires minimal hardware integration to the test room. Due to the lack of indoor GPS signal, this UAV utilizes a series of ultrasonic beacons that release several varied-frequency pulses simultaneously in order to localize the drone. The flight controller returns a 3D coordinate tied to the radiation data to understand precisely where radiation spikes are being emitted from the horn. The flight controller stores log data that can be processed into an easily interpretable map of radiation intensities. The radiation map serves as one of the primary references for planning the transportation of the NuMI horn.

43 PARTICLE ACCELERATORS↗

Fast-current-heating devices to study in situ phase formation in metallic glasses by using high-energy synchrotron radiation

Details of fast-resistive-heating setups, controlled heating ranging from ~10 1 K s –1 to ~10 3 K s –1 , to study in situ phase transformations (on heating and on cooling) in metallic glasses by high-energy synchrotron x-ray diffraction are discussed here. Both setups were designed and custom built at the Leibniz Institute for Solid State and Materials Research Dresden (IFW Dresden) and have been implemented at the P02.1 Powder Diffraction and Total Scattering Beamline and the P21.1 Swedish Materials Science Beamline at PETRA III storage ring, DESY, Hamburg. The devices are interchangeable at both beamlines. Joule heating is triggered automatically and is timed with the incident beam and detector. The crystallization process can be controlled via a feedback circuit by monitoring the change in the time-dependent resistivity and temperature of glasses. Different ambient atmospheres, such as vacuum and inert gases (He and Ar), can be used to control oxidation and cooling. The main focus of these devices is on understanding the crystallization mechanism and kinetics in metallic glasses, which are brittle and for which fast heating gives defined glass–crystal composites with enhanced plasticity. As an example, phase-transformation sequence(s) in a prototyped Cu–Zr-based metallic glass is described on heating, and a crystalline phase beneficial to the plasticity is identified.

47 OTHER INSTRUMENTATION↗

Impact of gas injection location and divertor surface material on ITER fusion power operation phase divertor performance assessed with SOLPS-ITER *

Abstract The ITER divertor design and performance assessment, primarily based on the SOLPS-4.3 burning plasma database (Pitts R. et al 2019 Nucl. Mater. Energy 20 100696), assumes the use of beryllium (Be) as the divertor surface material and the injection of gas from the main chamber top. However, the current ITER baseline favors gas injection from the more toroidally symmetric sub-divertor region. This paper evaluates the implications of these assumptions for divertor performance in the ITER fusion power operation phase. The impact of the divertor surface material and the gas injection location on the main ions mirrors the hydrogen only low power phase scenario shown in Park J.-S. et al (2020 Nucl. Fusion 61 016021). However, during burning plasma operation, extrinsic impurity seeding will be required. In the case of neon (Ne), studied here, impurity retention is influenced by both the divertor surface material and the fueling location. Neon leakage increases due to more energetic reflection from tungsten than beryllium, but equivalent divertor performance can be achieved by adjusting the neon seeding rate. While the impurity seeding location does not affect the distributions of impurity or radiation, the fueling location does. Top fueling provides local ionization sources mainly in the mid-SOL under detached conditions, enhancing divergences of the flux there (source-driven flow), bringing stagnation points close to the fueling location, and equilibrating flows towards both targets. In contrast, the global flow pattern (in the absence of fluid drifts) in the case of sub-divertor fueling is biased towards the inner target. Impurity flows, driven by force balance, largely mirror those of the main ion flow, including the stagnation point. The case with top fueling enhances Ne retention and corresponding radiation in the outer divertor, effectively reducing the total and peak target heat fluxes by 20%–40%, compared to the case with divertor fueling. Meanwhile, the case with outer target fueling also achieves similar reductions by enhancing plasma-neutral interactions. These results suggest the possibility that the selection of the fueling location and throughput can be used as an actuator to control impurity divertor retention and divertor radiation asymmetry.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Effects of radiative heat loss on extinction limits of counterflow premixed ammonia-air flames

The effect of radiative heat loss on counterflow premixed ammonia-air flames has been investigated as a function of equivalence ratio and system pressure. Non-adiabatic counterflow premixed flame simulations incorporating detailed chemistry, transport, and radiative heat transfer in the optically thin limit have been employed to elucidate important underlying physics and extinction characteristics. Similar to methane-air flame systems, non-adiabatic counterflow premixed computations show that the combined effects of positive flame stretch, sub-unity Lewis number, and radiative heat loss lead to the extension of the lean flammability limit for ammonia-air flames, revealing a C-shaped curve near the lean flammability limit that exhibits both radiation-induced and stretch-induced extinction states. Here, the computations compare favorably with the experimentally determined extinction stretch rate values for the stretch-induced extinction states over a wide range of equivalence ratios at different pressures up to 5 atm. A novel feature sensitivity analysis has also been developed to highlight important sensitive reactions for the stretch- and radiation-induced extinction states. Furthermore, the controlling chemistry at the dual-extinction states and at varying pressures are compared and discussed.

10 SYNTHETIC FUELS↗

Non-Equilibrium Actinide Radiation Chemistry and the Nuclear Fuel Cycle

Actinides are inherently unstable elements that frequently coexist with other radioisotopes, generating intense ionizing radiation fields that drive the formation of non equilibrium oxidation states. These transient species exert a profound mechanistic influence on the radiation response of actinide containing systems due to their unique redox chemistry. Despite their importance, they remain poorly understood, yet such insight is essential for advancing actinide science and accurately predicting radiation driven behavior. Actinide separations—critical for nuclear energy technologies, strategic deterrence, space exploration, and nuclear medicine—depend on precise control of actinide oxidation states to recover targeted elements from complex matrices such as used nuclear fuel. However, during these processes, actinides, their coordination complexes, and the separation media are all exposed to intense, multicomponent (alpha, beta, gamma, etc.) radiation fields that can alter process efficiency, selectivity, and chemical stability. Understanding, controlling, and mitigating radiation induced reactions is therefore key to innovating and optimizing next generation separation technologies. This seminar will provide an overview of the nuclear fuel cycle and non equilibrium actinide radiation chemistry in the context of recovering actinides from used nuclear fuel, with a particular emphasis on direct dissolution–based reprocessing strategies. We will explore time resolved electron pulse radiolysis and alpha and gamma dose accumulation studies, integrated with multiscale computational modeling, to elucidate the molecular level roles of radiation driven, non equilibrium actinide species in process performance and in the radiolytic stability of organic ligands used for actinide recovery. These insights offer new pathways for designing advanced separation methods and next generation solvent systems, with broad implications for the future of the nuclear fuel cycle.

37 - INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL C↗

Multiscale Modeling of Plutonium Radiation Chemistry in Nitric Acid Solutions. 1. Cobalt-60 Gamma Irradiation of Pu(IV)

We report careful manipulation of the plutonium oxidation states is essential in the study and utilization of its rich redox chemistry. To achieve this level of control, a comprehensive mechanistic understanding of radiation-induced plutonium redox chemistry is critical due to the unavoidable exposure of plutonium to ionizing radiation fields, both inherent and from in-process applications. To this end, we have developed an experimentally evaluated multiscale computer model for the prediction of gamma radiation-induced Pu(IV) redox chemistry in concentrated nitric acid solutions (1.0, 3.0, and 6.0 M). Under these acidic, aqueous solution conditions, cobalt-60 gamma irradiation afforded marginal net conversion of Pu(IV) to Pu(VI), the extent of which was dependent on the concentration of HNO 3 and absorbed gamma dose. Multiscale calculations, which are in excellent agreement with experimental data, indicate that this observation is due to a combination of inherent plutonium disproportionation reactions and several radiation-induced processes, including redox cycling between Pu(IV) and Pu(III), as achieved by the reduction of Pu(IV) by nitrous acid and hydrogen peroxide, the oxidation of Pu(III) by nitrate and hydroxyl radicals, and the sequential oxidation of Pu(IV) to Pu(V) and Pu(VI) by the remaining available yield of nitrate radicals.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Data on erosion and hydrogen fuel retention in Beryllium plasma-facing materials

ITER will use beryllium as a plasma-facing material in the main chamber, covering a total surface area of about 620 m 2 . Given the importance of beryllium erosion and co-deposition for tritium retention in ITER, significant efforts have been made to understand the behaviour of beryllium under fusion-relevant conditions with high particle and heat loads. This paper provides a comprehensive report on the state of knowledge of beryllium behaviour under fusion-relevant conditions: the erosion mechanisms and their consequences, beryllium migration in JET, fuel retention and dust generation. The paper reviews basic laboratory studies, advanced computer simulations and experience from laboratory plasma experiments in linear simulators of plasma–wall interactions and in controlled fusion devices using beryllium plasma-facing components. A critical assessment of analytical methods and simulation codes used in beryllium studies is given. The overall objective is to review the existing set of data with a broad literature survey and to identify gaps and research needs to broaden the database for ITER.

Erosion–deposition↗

Surface Brightening in Eastern and Central China Since the Implementation of the Clean Air Action in 2013: Causes and Implications

Surface brightening has been observed in China since 2005. However, it remains unclear whether the brightening has accelerated recently in response to the strictest ever air pollution control policies since 2013. By combining intensive surface and satellite observations, we find an unprecedented rapid increasing trend in surface solar radiation (SSR) of 0.70–1.16 W m-2 yr-1 over the eastern and central China for 2014–2019. Using a novel method to identify the relative contributions of aerosol and cloud radiative effects to the SSR trends, we find that the strongly declining aerosol radiative effect due to the strict air pollution controls is the main cause of the upward SSR trends; cloud variations should not be the main reason. Distinction exists in seasonal trends of SSR, with decreasing trends in winter and increasing trends in other seasons. Air pollution controls play an important role in regulating SSR, which has valuable implications for photovoltaic power generation.

Shi, Hongrong↗

Nonlinear Thomson scattering with ponderomotive control

In nonlinear Thomson scattering, a relativistic electron re-radiates the photons of a laser pulse, converting optical light to x rays or beyond. While this extreme frequency conversion offers a promising source for probing high-energy-density materials and driving uncharted regimes of nonlinear quantum electrodynamics, conventional nonlinear Thomson scattering has inherent tradeoffs in its scaling with laser intensity. Here we discover that the ponderomotive control afforded by spatiotemporal pulse shaping enables novel regimes of nonlinear Thomson scattering that substantially enhance the scaling of the radiated power, emission angle, and frequency with laser intensity. By appropriately setting the velocity of the intensity peak, a spatiotemporally shaped pulse can increase the power radiated by orders of magnitude. Here, the enhanced scaling with laser intensity allows for operation at significantly lower electron energies or intensities.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Sustained edge-localized-modes suppression and radiative divertor with an impurity-driven instability in tokamak plasmas

We report simultaneous control of the large edge localized modes (ELMs) and divertor heat fluxes in a metal wall environment is a critical issue for steady-state operation of a tokamak fusion reactors. Here we report a sustained ELM suppression scenario achieved in the EAST tokamak compatible with radiative divertor using different seeding impurity species over a wide range of conditions. A low-n mode appears, as manifested by the oscillations of a radiation front near the X-point. This mode appears to drive strong particle transport and tungsten exhaust, which is essential to the maintenance of the ELM-stable state. We have developed a model to explain the mode excitation, by coupling the impurity radiative condensation instability to drift waves, which could explain some characteristics of the low-n mode well. The low-n mode may offer a new ELM-stable scenario compatible with radiative divertor for future fusion reactors.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗