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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 199 records · Page 11

The Extent of Solar Energetic Particle Irradiation in the Sun’s Protoplanetary Disk

Solar flares emit X-rays and high-energy (MeV to GeV) ions called solar energetic particles (SEPs). Astronomical observations show solar-mass protostellar fluxes are a factor Φ ≈ 3 × 10 2 –3 × 10 3 times higher than the present-day Sun. Constraining Φ in the early solar system is important for modeling ionization in the Sun’s protoplanetary disk, the extent of magnetorotational instability or magnetocentrifugal outflows, or even production of short-lived radionuclides. Recent interpretations of meteoritic data—including cosmogenic Ne in hibonite grains, initial ( 10 Be/ 9 Be) 0 ratios in Ca-rich, Al-rich inclusions (CAIs), or even inferences of live 7 Be in CAIs—suggest values Φ > 10 5 , reaching as high as Φ ≈ 6 × 10 6 , which would make the young Sun extraordinarily active, even for a protostar. We constrain Φ by reexamining these data. We conclude that cosmogenic Ne was produced in hibonite grains as they resided in the disk; 36 Cl was created in Cl-poor grains after the disk dissipated; 10 Be was inherited from the molecular cloud, with almost no (<1%) 10 Be created in the disk; and there is no evidence whatsoever for any live 7 Be in CAIs. We show these data are consistent with a value Φ ≈ 3 × 10 3 for the first >5 Myr of the solar nebula. The early Sun evidently emitted a flux of X-rays and SEPs not atypical for a protostar.

79 ASTRONOMY AND ASTROPHYSICS↗

The CAI Database: 26 Al– 26 Mg Isotope Systematics

We present a publicly available calcium–aluminum-rich inclusion (CAI) database that focuses on the initial 26 Al/ 27 Al 0 ratio in CAIs, designed in a way that researchers in cosmochemistry and astrophysics may find useful. To date, the database contains 497 CAIs from 75 peer-reviewed papers. The CAIs are from all chondrite groups and cover different CAI types, textures, and sizes. The database includes the paper; the host meteorite; the CAI name and type; the 26 Al/ 27 Al 0 , δ 26 Mg$^*_0$, and δ 25 Mg values and their uncertainties; the number of regression points; the maximum 27 Al/ 24 Mg; the mean-squared weighted deviation; the CAI size; and CAI descriptions. We grouped the CAIs in different ways to discuss 26 Al/ 27 Al 0 ratio distributions with implications for the CAI formation timeline. Overall, we agree with previous authors that CAIs have a bimodal 26 Al distribution: CAIs with robust isochrons (n = 151) have a median 26 Al/ 27 Al 0 = 4.8 × 10 −5 (with a 1σ standard error of 0.1), while those with isotopic anomalies (n = 87) have a median 26 Al/ 27 Al 0 = 0.3 × 10 −5 (with a 1σ standard error of 0.2). However, the large standard deviation of both groups (1.3 and 2.3, respectively) indicates that the 26 Al/ 27 Al 0 values scatter significantly within each population. CAI types and groups can have distinct 26 Al/ 27 Al 0 and δ 26 Mg$^*_0$, but the unmelted inclusions (n = 33) have the highest median 26 Al/ 27 Al 0 = 5.1 × 10 −5 and a low median δ 26 Mg$^*_0$ = −0.05‰. We find slightly different 26 Al/ 27 Al 0 distributions between CAI chondrite types, but no differences between petrographic types or sizes. These observations can help us to understand CAI formation in the context of astrophysical models.

Astronomy and AstroPhysics↗

High Optical-to-X-Ray Polarization Ratio Reveals Compton Scattering in BL Lacertae’s Jet

Blazars, supermassive black hole systems with highly relativistic jets aligned with the line of sight, are the most powerful long-lived emitters of electromagnetic emission in the Universe. We report here on a radio-to-gamma-ray multiwavelength campaign on the blazar BL Lacertae with unprecedented polarimetric coverage from radio to X-ray wavelengths. The observations caught an extraordinary event on 2023 November 10–18, when the degree of linear polarization of optical synchrotron radiation reached a record value of 47.5%. In stark contrast, the Imaging X-ray Polarimetry Explorer found that the X-ray (Compton scattering or hadron-induced) emission was polarized at less than 7.4% (3 σ confidence level). We argue here that this observational result rules out a hadronic origin of the high-energy emission and strongly favors a leptonic (Compton scattering) origin, thereby breaking the degeneracy between hadronic and leptonic emission models for BL Lacertae and demonstrating the power of multiwavelength polarimetry to address this question. Furthermore, the multiwavelength flux and polarization variability, featuring an extremely prominent rise and decay of the optical polarization degree, is interpreted for the first time by the relaxation of a magnetic “spring” embedded in the newly injected plasma. This suggests that the plasma jet can maintain a predominant toroidal magnetic field component parsecs away from the central engine.

79 ASTRONOMY AND ASTROPHYSICS↗

Conceptual Spacer Design for the ATR GEN I Target for Pu-238 Production in the Advanced Test Reactor at Idaho National Laboratory

The initial target design used for Pu-238 production at Idaho National Laboratory was designed by Oak Ridge National Laboratory to optimize the production of Pu-238 in the High Flux Isotope Reactor (HFIR) and are referred to as HFIR GEN II targets. To take advantage of the Advanced Test Reactor’s (ATR) taller active core region a redesign of the HFIR GEN II targets was needed. It was proposed to stack two HFIR GEN II targets nose to nose about the core center line; however, this resulted in excessive neutron and photon heating in the pellets located in the center. This peak heating was not desirable so three alternative designs were investigated for the ATR GEN I targets. The python-based code, MCNP to ORIGEN2 in Python (MOPY), was used to calculate the heating rates after 40 days of irradiation to capture the effects of each configuration. The purpose of this paper is to document the details of these conceptual design calculations and comparisons for the ATR GEN I targets.

07 ISOTOPE AND RADIATION SOURCES↗

Process Improvements For Pu-238 Production at Idaho National Laboratory

Idaho National Laboratory (INL) has supported the production of Pu-238 for future NASA deep space missions since 2017. Over this time, INL has worked to improve the qualification process of Pu-238 production targets as well as improve processes related to the shipping, storage, irradiation, and storage of Pu-238 production targets. Qualification of Pu-238 production targets began with flux measurements and scoping analysis to provide fundamental data to confirm the impacts on the operation of the Advanced Test Reactor (ATR), Fig1. Later, initial production targets were irradiated in ATR’s I-7 position, and then the South Flux Trap (SFT). A modified target design was then implemented which would use the full length of the ATR core and increase Pu-238 production. While working to improve and streamline the qualification of the Pu-238 production targets, INL worked to improve multiple operational aspects of the Pu-238 production process. These changes include updating procedures to streamline operations, supporting modification of shipping containers to contain five rather than one production target, reviewing target receipt procedures and changing work flow to provide flexibility in target receipt, and designing and fabricating support equipment for the storage and internal transfer of production targets.

07 ISOTOPE AND RADIATION SOURCES↗

Production of High Specific Activity 155 Tb, 161 Tb and 203 Pb for Research and Clinical Applications: Effective Target Design, Target Material Recycling and Radioisotope Separation (Final Technical Report)

The overall objectives of this project were (1) to develop methods for the production and separation of a diagnostic and therapeutic or “theranostic” pair of radioisotopes, terbium-155 ( 155 Tb) and terbium-161 ( 161 Tb) and (2) to train graduate students and postdoctoral fellows in technologies and methods used in radionuclide production. Radionuclides can be incorporated into drugs called radiopharmaceuticals that target a specific disease (e.g., cancer). The need for theranostic radionuclides is escalating with the clinical translation of radiopharmaceuticals due to their implementation in personalized medicine, which has demonstrated enhanced patient treatments. High purity and high specific activity radionuclides are critical for theranostic agent development, for example to maintain diagnostic image quality, to minimize radiation dose to the patient, and to increase uptake in the targeted tissue (e.g., tumor), especially in the case of receptor- and antigen-targeted agents. The 155 Tb (diagnostic) and 161 Tb (therapeutic) radioisotopes that were generated through this project are a theranostic pair with demonstrated potential for the development and translation into individualized, targeted, and dosimetry-driven radiotherapies. However, the development of such radiotherapies has been hindered by the lack of a routine and reliable supply of these isotopes in the United States. Methods for the production, separation, and supply of 155 Tb and 161 Tb were investigated and developed in this project. Further, the strong emphasis throughout the project on the training of graduate students and postdoctoral fellows has helped to ensure and enhance the nuclear science workforce through the training of the next generation of highly qualified scientists in nuclear and radiochemistry. This grant also continued a collaboration between scientists at the University of Washington (UW), the University of Missouri (MU) and Brookhaven National Laboratory (BNL). All three institutions were involved in the project, but to different degrees on the various tasks through which the overall objectives were met.

07 ISOTOPE AND RADIATION SOURCES↗

DoD Symposium Presentation

TRISO fuel, or TRi-structural ISOtropic, is a ceramic based nuclear fuel capable of operating at high temperatures (up to 1600°C). The fuel, consisting of uranium oxycarbide (UCO) fuel kernels, is coated with three layers of carbon and ceramic (dense silicon carbide) materials to capture and contain radioactive fission products. BWXT, located in Lynchburg, VA, has perfected the manufacturing techniques to produce this fuel and is currently the only US company licensed to produce this irradiation-tested fuel. BWXT is currently producing fuel in support of a demonstration reactor scheduled for startup on the INL site in 2025. The first fuel delivery, estimated at 200 kilograms High Assay Low Enriched Uranium, is targeted for the end of CY2024.

07 ISOTOPE AND RADIATION SOURCES↗

Benchmark results with a new evaluation of 155 Gd and 157 Gd

Evaluations of gadolinium isotopes 155 Gd and 157 Gd in the resolved resonance region were performed with the code SAMMY. The main objective for revising the resonance evaluations of these isotopes was to address issues related to critical benchmark results.

07 ISOTOPE AND RADIATION SOURCES↗

Performance Evaluation of Different Parallel Programming Models in SCALE-Shift Sequences for Criticality and Shielding Applications [Abstract]

The SCALE code system has been widely used for nuclear criticality safety, reactor physics, radiation shielding, source term generation, and inventory analyses by researchers, industry, and regulatory bodies. Although limited support for shared- and distributed-memory parallel processing was introduced via C++ threading, OpenMP, and MPI, a hybrid parallel programming model with both distributed- and shared-memory parallelism has not been fully supported in the SCALE code system.

Nuclear Criticality Safety Program (NCSP)↗

Simulating Alpha Particles Incident on MKID Chips for Quantum Sensitivity Analysis

Superconducting quantum devices, such as microwave kinetic inductance detectors (MKIDs), are highly sensitive instruments used in quantum computing and advanced sensing technologies. However, their extreme sensitivity also makes them vulnerable to background noise from natural sources like radiation. One significant contributor to this noise is alpha particles emitted by 210Po, a radon decay daughter that accumulates on surfaces near the detector. This project investigates how alpha particles emitted from 210Po interact with MKID chips. These particles can deposit energy on the detector surface, disrupting its operation and generating false signals. Understanding the energy and behavior of these particles is crucial for improving the design and reliability of quantum devices. To explore this, we first modeled the decay chain starting from 210Pb to 210Po using differential equations. This allowed us to predict how the activity of alpha-emitting isotopes changes over time, reaching a steady state after about two years. Next, we simulated alpha particle interactions with the MKID chip using the Geant4 software toolkit. We built a detailed computer model of the detector housing, including the copper lid where alpha particles originate, the silicon chip, and a thin aluminum sensor layer. Alpha particles were emitted isotropically from just beneath the copper lid’s surface, mimicking natural decay conditions. The simulation tracked how these particles deposit energy on the chip, generating electron-hole pairs and phonons. The results provide insight into the behavior of the resultant electron-hole pairs and phonons, giving us a clear understanding of the energy deposition distribution on the chip. This work supports efforts to mitigate background noise in superconducting sensors, advancing their use in quantum computing and sensitive physics experiments.

Hall, Matthew [Fermilab; UCLA]↗

High Spatial Resolution Mapping of Retained Fission Gas

Fission gas isotopic analysis provides quantitative high precision determination of irradiated nuclear fuel burnup, offers diagnostic value, and informs fuel performance models. A measurement capability has been developed at Idaho National Laboratory (INL) for the release of retained fission gas using a focused laser and static noble gas mass spectrometry (MS) analysis. This high resolution (10s microns spot size) capability was demonstrated using Xe implanted metal foils.

07 - ISOTOPES AND RADIATION SOURCES↗

FGMS-poster

Idaho National Laboratory (INL) performs post irradiation examination (PIE) of tri-structural isotropic (TRISO)-coated particle fuel to help qualify it for high temperature gas cooled reactors. TRISO fuel compacts are re-irradiated in the Neutron Radiography Reactor (NRAD) to generate the short lived fission products needed for fission product release testing. The Fuel Accident Condition Simulator (FACS) furnace and newly added Screen Neutron Irradiated Fuel for Failure (SNIFF) furnace heat the compacts in helium to temperatures of up to 2,000°C, prompting fission product release—predominantly gaseous xenon and krypton isotopes and condensable products such as cesium—from failed particles. These released isotopes are transported to a fission gas monitoring system (FGMS 1 or FGMS 3), where they accumulate in cryogenic cold traps and are quantified using high-purity germanium (HPGe) detectors. The addition of SNIFF and FGMS 3 increases throughput by enabling simultaneous testing of multiple compacts. Furthermore, automated INL developed software provides continuous, near-real time monitoring of fission product inventories and manages the liquid nitrogen cooling of the traps. These system enhancements improve the efficiency, data quality, and testing capacity of TRISO fuel performance evaluations.

07 - ISOTOPES AND RADIATION SOURCES↗

Improvements to In-Canal Assay of High Specific Activity 60Co at the ATR

Improvements to the quality of measurements in the assaying of High Specific Activity (HSA) cobalt 60 produced at the Advanced Test Reactor at the Idaho National Laboratory are presented. Such assays are conducted regularly between cycles at the ATR, and due to the radiological safety concerns, they are performed within the ATR canal. A standard ion chamber detector was placed in a collimated assay tube within the canal. Another tube, parallel to the detector, was used to position various cobalt 60 standards and targets. The collimated port between these tubes allows for the targets to be pulled across via a winch system. Previous measurements were performed at discrete 1.5-inch steps using a hand-cranked winch system. Charge was collected and integrated for 10 seconds at each discrete step during a scan. Two substantial improvements to the assay include an electronically controlled, motor-driven winch system and a software controlled continuous charge collection. Combined, these changes improved the quality of measurements as well as streamline the assay process. Further examination of these charge profiles indicated a reasonable amount of photon scattering, or shine, before a line-of-sight is established. This created inaccuracies in the reported activity of the cobalt targets. A series of MCNP-6.3 calculations were performed in an effort to quantify and correct for this shine effect. The results of the calculations and how they were employed to a create shine correction factor for the in-canal cobalt assay at the ATR are presented. The overall bias showed an overestimation of the HSA cobalt 60 activity by around 7-8%.

07 - ISOTOPES AND RADIATION SOURCES↗

Shear-Wave Radiation Patterns from Explosive and Earthquake Sources in Scattering, Heterogeneous Media

Distinguishing whether a seismic event is an earthquake or an explosion is a core problem in explosion monitoring. For simplistic models, earthquakes produce a predictable S-wavefield based on their radiation pattern, while an explosion produces no S-wavefield. However, observations from nuclear tests show that explosions can produce significant S-wave energy on both horizontal components. We perform numerical experiments using SPECFEM to constrain when an S-wavefield generated from an explosion might differ from one produced by an earthquake. We generate the S-wavefield for our explosions by placing the source location within a small region consisting of large velocity heterogeneities. For the 2D cases investigated here, a crucial condition is that the size of the region of heterogeneities must be much smaller (approximately 1/12th) than the minimum wavelength of the wavefield for our simulation setups. We investigate both isotropic heterogeneities and anisotropic heterogeneities. Initial results demonstrate that the heterogeneous region lowers the P/S amplitude ratios of an explosion. The presence of strong anisotropic heterogeneities near the source can also produce an S-wavefield with similar amplitudes to the P-wavefield. Lastly, we show that S-wave polarization angles vary as a function of azimuth and distance for explosive sources in the presence of small-scale heterogeneities.

58 GEOSCIENCES↗

Radiation monitoring devices and associated methods

Radiation monitoring devices and associated methods are described. According to one aspect, a radiation monitoring device includes a housing configured to pass radiation emitted from a radiological source located in proximity to the radiation monitoring device, a radiation detector configured to receive the radiation emitted from the radiological source and to generate information regarding the radiation, and communications circuitry configured to communicate the information regarding the radiation in a plurality of communications at a plurality of different moments in time externally of the radiation monitoring device.

Burghard, Brion J.↗

Understanding Radiotropism in Filamentous Fungi

Melanized species of filamentous fungi isolated from high radiation environments have been reported to exhibit radiotropism, defined as the directed growth toward a source of ionizing radiation. Inconsistencies in the experimental approaches and results have impeded our understanding of the key factors involved in radiotropism. In the present study, we assessed radiotropism in four isolates of fungi: Aspergillus niger, A. calidoustus JC-1043, Paecilomyces variotii SNL-1, and P. variotii IMV-00236. Of these fungi, only P. variotii IMV-00236 had been previously reported to exhibit radiotropic behavior. Plates of each fungus were placed in equivalent proximity to a 137 Cs source, with a primary gamma emission of 662 keV, and differences in the rate and direction of mycelia growth were measured over a seven-day period. Significant differences were not observed in the rate or direction of growth of the different fungi based on exposure to gamma radiation, which suggested a lack of measurable radiotropism in these experiments. Additional studies varying parameters such gamma emission rates and energies, as well as other types of ionizing radiation (e.g., alpha and beta particles, neutrons) are necessary to gain further insights to the factors critical to the expression of radiotropic behavior in filamentous fungi.

59 BASIC BIOLOGICAL SCIENCES↗