Search NASA⌕ Search

SEARCH · Search NASA

Results for “Rare Isotopes”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 199 records · Page 11
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

China-US Theory Institute for Physics of Exotic Nuclei

The China-US Theory Institute for Physics of Exotic Nuclei (CUSTIPEN) was funded by DOE during May 1, 2013-April 30, 2023. The grant was managed by Texas A&M University-Commerce under the guidance of the CUSTIPEN Governing Board consists of physicists from Michigan State University, Florida State University, and Texas A&M University-Commerce. Its main goal was to support US-based physicists to visit their collaborators in China to work on projects supporting the science goals of DOE's national Facility for Rare Isotope Beams (FRIB) built on the campus of Michigan State University. The project has achieved successfully its scientific goals and mission.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

NUCLEI (SciDAC-4) effort at The University of Tennessee, Knoxville

This Report summarizes the accomplishments of NUCLEI researchers at The University of Tennessee, Knoxville (UTK) and those supported via subcontracts at the University of North Carolina at Chapel Hill (UNC) and Iowa State University (ISU). The SciDAC-4 NUCLEI collaboration had the goal to advance the computation of atomic nuclei and to make reliable predictions including uncertainty estimates for observables of interest. These goals were achieved by developing improved nuclear interactions and currents that are input to the computations, and by advancing the algorithms and techniques used for computing nuclear observables of interest. The computed results advanced our understanding of how nuclei work; they helped to guide and interpret experiments at existing low-energy nuclear physics facilities, the Facility for Rare Isotope Beams, Jefferson Laboratory, and neutrino experiments. In addition, predictions were made that await confrontation with experimental results.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Structure of the high-spin, β-decaying state in the neutron-rich nucleus 146 La

Excited structures in 146 Ce were populated in β decay of the high-spin state in the neutronrich nucleus 146 La. The beam was produced by the Californium Rare Isotope Breeder Upgrade (CARIBU) facility at Argonne National Laboratory, re-accelerated by the ATLAS accelerator and implanted on a moving-tape system in the middle of the GAMMASPHERE array. The decay scheme of the high-spin, β-decaying state in 146 La was revised with respect to previous studies and evaluated nuclear data. The structure of 146 La is discussed in the framework of the deformed Nilsson model and systematics of known quasiparticle structures in the region.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Nuclear Physics of Compact Binaries with GADGET

The research goal of this project was to experimentally constrain the thermonuclear rate of the 15 O(α, Υ) 19 Ne reaction, whose uncertainty has a strong influence on the modeling of astrophysical Type-I X-ray bursts on accreting neutron stars. To this end, Experiment 21072 was run in November 2022 at the Facility for Rare Isotope Beams using the GADGET II detection system. The limited scope and duration of this award included work in the year following the experiment: drafting a technical paper on the time projection chamber of the GADGET II detection system, and analysis of data from Experiment 21072. The award contributed to the education and development of the scientific and technical workforce by partially supporting one postdoctoral Research Associate who did this work.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Physics Design of Proton/Ion SRF Accelerators

Superconducting Radio Frequency (SRF) technology has become foundation of the modern high energy particle accelerators. The technology enables a higher accelerating field with minimal power dissipation and a stronger compact magnetic field. These advancements have broadened the operational horizon of the particle accelerators making a higher duty factor and Continuous Wave (CW) beam operations both feasible and economically viable. The intensity frontier research founded on generation of intense beam of exotic particles including but not limited to neutrinos, muons, kaons and neutrons as well as practical applications involving transmutation of nuclear reactor waste, rare isotopes generation, sub-critical nuclear power generation etc. could be accomplished efficiently only by using superconducting proton/ions particle accelerators. As a result, many newly constructed or under construction high energy accelerator facilities around the world such as Proton Improvement Plan-II (PIP-II) at Fermilab, FRIB at MSU, ESS at Sweden are utilizing SRF accelerators. This talk presents the design philosophy of SRF proton/ion particle accelerator, with a focus on optimizing its performance while addressing physics and operational challenges including the fault scenarios, machine availability and preservation of crucial beam parameters.

Saini, Arun↗
DOE OSTI2025

Development of the detector array for photons, protons, and exotic residues

Accurate neutron capture predictions are needed in fundamental and applied science. Empirical models are constrained largely for stable nuclei, but predictions far from stability are needed. Neutron transfer in (d,p) reactions in inverse kinematics with rare isotope beams offer a means to access key aspects of the capture process. To this end, the detector array for photons, protons, and exotic residues (DAPPER) has been designed, built, tested, and used for measurement at Texas A&M University.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Theoretical Nuclear Physics (Final Report)

This award from the Department of Energy supported the PI, Che-Ming Ko of Texas A&M University, for the period from April 1, 2022 to August 31, 2025 at an amount of $150,000 to carry out the project entitled “Theoretical nuclear physics”. The scientific goal of the project was to develop transport models for heavy ion collisions at various energies and with both stable and rare isotopes and to carry out systematic comparisons of theoretical predictions with experimental data. Results from this project has led to the publication of 14 papers in and the submission of 10 papers to peer-reviewed journals, the publication of 3 papers in and the submission of 1 paper to conference proceedings. Also, the PI has presented 12 invited talks at international conferences and workshops. In the following, a brief summary of these results is given.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

Accelerator Science & Engineering (AS&E) Workforce Roundtable and AS&E Traineeship Principal Investigator Meeting

A one-and-half-day meeting on the Accelerator Science & Engineering (AS&E) Workforce Roundtable and a one-day meeting of Traineeship Principal Investigators took place at Facility for Rare Isotope Beams at Michigan State University on January 21-23, 2025. The meeting identified critical issues in the AS&E workforce and potential solutions, with a focus on DOE’s major accelerator facilities. The Traineeship PIs meeting focused on sharing experience, efficiency, and improvements of the Traineeship Programs conducted in six US universities. Several managers from the DOE High Energy Physics Office participated in the meetings. The discussions resulted in a decision to conduct similar meetings every year.

43 PARTICLE ACCELERATORS↗
DOE OSTI2025

Gas jet targets for direct reaction studies

The study of direct reactions is of broad interest in nuclear physics, providing constraint to models of nuclear structure evolution and data to better understand the creation of the elements. In many cases, however, the data of interest are hindered by backgrounds and poor resolution from contaminants in either the beam, the target, or both. The use of a gas jet can overcome some of these issues through clever engineering, providing a reaction target that is chemically pure and thin enough to significantly reduce the impact on experimental resolution. This Perspective will discuss the effort to design, construct, and operate gas jet targets for direct reaction studies in the rare isotope era.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Direct reactions for astrophysical p-capture rates with ORRUBA and GODDESS

Understanding the nucleosynthesis and energy generation in quiescent and explosive stellar burning requires a detailed understanding of reaction rates on many unstable nuclides. Such reaction rates are often governed by the properties of low-lying, isolated proton resonances. Though direct measurements of resonance strengths are ultimately desired, and are a focus of rare isotope beam facilities worldwide, such tour-de-force experiments must be guided by indirect techniques, in order to know resonance energies, J π assignments, and estimated widths, to inform targeted measurements. Furthermore, some important low-lying resonances may be too weak for direct measurements with radioactive beams, and indirect techniques provide the only practical constraints. Additionally, there has been growing interest in the astrophysical role of isomeric states, which can influence the reaction flow in nucleosynthetic reaction networks, and hence impact the quantitative interpretation of astronomical observables, such as γ-ray signatures, and elemental and isotopic ratios. Properties of single-proton resonances can be obtained by exploiting the selectivity of direct reactions, such as single-nucleon transfer and charge-exchange reactions. Constraining proton-capture rates via direct reactions has been a focus of the astrophysics program at ORNL for over two decades, spurring the development of the ORRUBA and GODDESS detector systems. Herein, a review of recent developments in instrumentation and radioactive beam delivery (including isomeric beam experiments) is presented, along with some specific examples of astrophysically interesting sd-shell nuclides, which have been a target of recent ORRUBA and GODDESS experiments.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

Direct reactions with the AT-TPC

Direct reactions are crucial tools for accessing properties of the atomic nucleus. Fundamental and exotic phenomena such as collective modes, pairing, weakbinding effects and evolution of single-particles energies can be investigated in peripheral collisions between a heavy nucleus and a light target. The necessity of using inverse kinematics to reveal how these structural properties change with isospin imbalance renders direct reactions a challenging technique when using the missing mass method. In this scenario, Active Target Time Projection Chambers (AT-TPC) have demonstrated an outstanding performance in enabling these types of reactions even under conditions of very low beam intensities. The AT-TPC of the Facility for Rare Isotope Beams (FRIB) is a next generation multipurpose Active Target. When operated inside a solenoidal magnet, direct reactions benefit from the measurement of the magnetic rigidity that enables particle identification and the determination of the excitation energy with high resolution without the need of auxiliary detectors. Additionally, the AT-TPC can be coupled to a magnetic spectrometer improving even further its spectroscopic investigation capability. In this contribution, we discuss inelastic scattering and transfer reaction data obtained via the AT-TPC and compare them to theory. In particular, we present the results for the 14 C(p,p′) and 12 Be (p,d) 11 Be reactions. For 14 C, we compare the experimental excitation energy of the first 1 – excited state with coupled-cluster calculationsbased on nuclear interactions from chiral effective field theory and with available shell-model predictions. For 12 Be, we determine the theoretical spectroscopic factors of the 12 Be (p,d) 11 Be transfer reaction in the shell modeland compare them to the experimental excitation spectrum from a qualitative standpoint.

active target↗
DOE OSTI2022

Radiation hardened beam instrumentations for multi-Mega-Watt beam facilities

The radiation hardened beam instrumentations workshop was held on February 3rd and 4th, 2022 to identify the technological challenges on the beam instrumentation for multi-Mega-Watt (MW) beam facilities. We invited a speaker from a high energy neutrino beam facility (CERN, Fermilab and J-PARC), a collider detector group (CERN and Fermilab), a neutron spallation source facility (ESS, J-PARC and SNS), and a rare-isotope beam facility (FRIB). Although, the operational beam parameter for each institution is unique due to their different physics goals, we realize that there is a common issue on the beam instrumentation. Therefore, it will be tackled by a collaborative R&D effort among facilities. We summarize an output from the workshop in the paper, and propose a possible R&D for the future radiation hardened beam instrumentations with a global effort.

43 PARTICLE ACCELERATORS↗
DOE OSTI2021

Heating events in the nascent solar system recorded by rare earth element isotopic fractionation in refractory inclusions

Equilibrium condensation of solar gas is often invoked to explain the abundance of refractory elements in planets and meteorites. This is partly motivated, by the observation that the depletions in both the least and most refractory rare earth elements (REEs) in meteoritic group II calcium-aluminum–rich inclusions (CAIs) can be reproduced by thermodynamic models of solar nebula condensation. We measured the isotopic compositions of Ce, Nd, Sm, Eu, Gd, Dy, Er, and Yb in eight CAIs to test this scenario. Contrary to expectation for equilibrium condensation, we find light isotope enrichment for the most refractory REEs and more subdued isotopic variations for the least refractory REEs. This suggests that group II CAIs formed by a two-stage process involving fast evaporation of preexisting materials, followed by near-equilibrium recondensation. The calculated time scales are consistent with heating in events akin to FU Orionis– or EX Lupi–type outbursts of eruptive pre–main-sequence stars.

58 GEOSCIENCES↗
DOE OSTI2025

Constraining the Synthesis of the Lightest 𝑝 Nucleus 74 Se

We provide the first experimental cross section of the 73 As(p, γ) 74 Se reaction to constrain one of the main destruction mechanisms of the p nucleus 74 Se in explosive stellar environments. The measurement was done using a radioactive 73 As beam at incident energies of 3.1 and 3.7 MeV/nucleon. Along with the total cross section measurement, statistical properties of the 74 Se compound nucleus were extracted, constraining the reaction cross section across the entire Gamow window of the γ process. The impact of the experimentally constrained reaction rate on 74 Se production in Type II supernovae is investigated through Monte Carlo one-zone network simulations. The results indicate that the overproduction of 74 Se by Type II supernova models cannot be resolved by nuclear physics and point towards the description of the astrophysical conditions of the γ process.

59 ≤ A ≤ 89↗
DOE OSTI2022

Column separation of tetravalent cerium fission products from trivalent rare earth radio-isotopes

Rapid and efficient isolation of individual rare earth element (REE) radioisotopes from complex mixtures is necessary to support the fields of nuclear forensics, medical isotope production and nuclear physics measurements. The separations must be robust and generate sufficiently high purity samples for subsequent radiological analysis. Current methodologies utilize a laborious two step Ce(IV)-iodate precipitation followed by Ce(IV)-nitrate di-(2-ethylhexyl)phosphoric acid/n-heptane extraction. This work reports an alternative method to isolate Ce fission product isotopes equilibrated with milligrams of cold carrier, from the remaining REE’s using a Ce(IV)/LN-resin (Eichrom Technologies) based separation. Optimization of Ce(IV) loading, REE(III) elution volume and subsequent Ce(III) stripping step utilized 166m Ho tracer. Mixed fission product experiments provided a further test of this LN-resin method, with analysis of purified 141/144 Ce, 147 Nd and 91 Y. Overall, while decontamination factors were lower for the LN-resin method, (vs. the combined precipitation/extraction) the simplicity of the technique and the satisfactory fission product analysis results point to the efficacy of this method.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2026

Magnetic character of the low-energy enhancement in 70 Zn

The transition of an atomic nucleus from an excited state to a state of lower energy is typically accompanied by the emission of photons. The likelihood of photon emission is a function of the photon energy and of properties of the initial and final nuclear states and is known as the photon (or γ-ray) strength function (γSF). Of the features present in the γSF, an enhancement in the low-energy region has been observed in some nuclei, but the electromagnetic nature of this enhancement remains an open question. This low-energy enhancement in the γSF significantly impacts our understanding of how elements are created in stars and the structure of the nucleus. Here we present the results from an experiment on the γSF of 70 Zn that show that the enhancement in the γSF of this nucleus is of magnetic nature. This observation helps address a long-open question about γSFs in atomic nuclei and directly impacts our predictive capabilities in nuclear science.

Physics - Nuclear physics and radiation physics↗
DOE OSTI2025

Universal Effective Charges in the 𝑠⁢𝑑 and 𝑓⁡𝑝 Shells

The 247-keV state in 54 Sc, populated in the 𝛽 decay of 54 Ca, is reported here as a nanosecond isomer with a half-life of 26.0(22) ns. The state is interpreted as the 1 + member of the 𝜋⁢𝑓 7/2 ⊗ 𝜈⁢𝑓 5/2 spin-coupled multiplet, which decays to the 3 + ,𝜋⁢𝑓 7/2 ⊗ 𝜈⁢𝑝 1/2 ground state. The new half-life corresponds to a pure 𝐸⁢2 transition with a strength of 1.93(16) W.u., providing the most precise, unambiguous 𝐵⁡(𝐸⁢2) value in the neutron-rich 𝑓⁡𝑝 region to date for a nucleus with valence protons above 𝑍 = 20. Notably, it is roughly 4 times larger than the 𝐵⁡(𝐸⁢2;1/2 − → 5/2 − ) value in 55 Ca. The results, as compared to semiempirical and ab initio shell-model calculations, indicate (1) a weak 𝑁 = 34 subshell gap relative to 𝑁 = 32, (2) a large 𝐸⁢2 enhancement in Sc as compared to Ca due to 1⁢𝑝 − 1⁢ℎ proton excitations across 𝑍 = 28, and (3) empirical effective proton and neutron charges 𝑒 𝜋 = 1.30⁢(8)⁢𝑒 and 𝑒 𝜈 = 0.452⁢(7)⁢𝑒, respectively, that are in contrast to reports of 𝑒 𝜋 ≈1.1–1.15⁢𝑒 and 𝑒 𝜈 ≈ 0.6–0.8⁢𝑒 for 𝑓⁡𝑝-shell nuclei near 𝑁 = 𝑍. Here, we demonstrate that these reports are erroneous and that, in fact, a universal set of effective charges can be used across the 𝑠⁢𝑑 and 𝑓⁡𝑝 shells.

Beta decay↗
DOE OSTI2026

Total absorption spectroscopy of two isomers in 70 Cu influencing nucleosynthesis signatures

Isomers have long been known to be important for astrophysical nucleosynthesis processes, yet they are often neglected in network calculations due to computational limitations or lack of data. "Astromers" are astrophysically metastable nuclear states that can greatly impact nucleosynthesis pathways. In this work we show that astromers further impact the time-dependent electromagnetic signal during heavy element nucleosynthesis. In an experiment performed at the National Superconducting Cyclotron Laboratory, three 𝛽-decaying states of 70 Cu (6 − ground state, and two isomeric states: 3 − and 1 + ) were produced. 𝛽-feeding values were extracted from experimental spectra and compared to shell-model and QRPA+PVC calculations. Here, average 𝛾-ray energies from the 𝛽-decay events were incorporated into simulations of heavy element nucleosynthesis and were found to exhibit different energy release profiles over time, which may impact, in aggregate, time-dependent observable signals.

59 ≤ A ≤ 89↗