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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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NASA NTRS1989

The roles of dynamical and chemical processes in determining the stratospheric concentration of ozone in one-dimensional and two-dimensional models

The two-dimensional model of Ko et al. (1985) was used to calculate the stratospheric concentrations of ozone, to determine the principal modes of balance for different stratospheric regions. The results of this analysis show that the local concentration of ozone in different regions of stratosphere is determined by balances between different mechanisms. In the upper stratosphere, the ozone concentration is dominated by photochemical processes, whereas in the mid-lower stratosphere, the bulk of ozone appears to be controlled by an interaction between the transport and the photochemical processes. The results point to the limitations of one-dimensional models, which fail to properly account for the effect of transport in the lower stratosphere.

Ko, Malcolm K. W.↗
NASA NTRS1989

Global stratospheric change: Requirements for a Very-High-Altitude Aircraft for Atmospheric Research

The workshop on Requirements for a Very-High-Altitude Aircraft for Atmospheric Research, sponsored by NASA Ames Research Center, was held July 15 to 16, 1989, at Truckee, CA. The workshop had two purposes: to assess the scientific justification for a new aircraft that will support stratospheric research beyond the altitudes accessible to the NASA ER-2; and to determine the aircraft characteristics (e.g., ceiling altitude, payload accommodations, range, flight duration, operational capabilities) required to perform the stratospheric research referred to in the justification. To accomplish these purposes, the workshop brought together a cross-section of stratospheric scientists with several aircraft design and operations experts. The stratospheric scientists included theoreticians as well as experimenters with experience in remote and in situ measurements from satellites, rockets, balloons, aircraft, and the ground. Discussions of required aircraft characteristics focused on the needs of stratospheric research. It was recognized that an aircraft optimal for stratospheric science would also be useful for other applications, including remote measurements of Earth's surface. A brief description of these other applications was given at the workshop.

Source record↗
NASA NTRS1991

SAM 2 measurements of the polar stratospheric aerosol. Volume 9: October 1982 - April 1983

The Stratospheric Aerosol Measurement (SAM) II sensor aboard Nimbus 7 is providing 1.0 micron extinction measurements of Antarctic and Arctic stratospheric aerosols with a vertical resolution of 1 km. Representative examples and weekly averages including corresponding temperature profiles provided by NOAA for the time and place of each SAM II measurement are presented. Contours of aerosol extinction as a function of altitude and longitude or time are plotted, and aerosol optical depths are calculated for each week. Typical values of aerosol extinction and stratospheric optical depth in the Arctic are unusually large due to the presence of material from the El Chichon volcano eruption in the Spring of 1982. For example, the optical depth peaked at 0.068, more than 50 times background values. Typical values of aerosol extinction and stratospheric optical depth in the Antarctic varied considerably during this period due to the transport and arrival of the material from the El Chichon eruption. For example, the stratospheric optical depth varied from 0.002 in October 1982, to 0.021 in January 1983. Polar stratospheric clouds were observed during the Arctic winter, as expected. A representative sample is provided of the ninth 6-month period of data to be used in atmospheric and climatic studies.

Mcmaster, L. R.↗
NASA NTRS1991

Stratospheric dynamical effects of solar ultraviolet variations - Evidence from zonal mean ozone and temperature data

Cross-spectral analysis of low-latitude average Nimbus 7 stratospheric and mesospheric sounder (SAMS) temperature deviations versus Nimbus 7 solar backscattered ultraviolet (SBUV) solar 205 nm flux measurements in the 1-3 mbar pressure range yields significant coherence at periods near 27 and 13 days. This supports earlier correlative evidence that the ozone response to solar ultraviolet variations is supplemented by a coupled temperature response in the upper stratosphere. Comparisons of improved one-dimensional radiative photochemical model calculations with ozone and temperature response measurements at low latitudes yields agreement only in the case of ozone at levels below 3 mbar. An additional, presumably dynamical, component of the upper stratospheric response is suggested. Cross-spectral analysis of low-latitude average SAMS temperature deviations versus higher-latitude temperature fluctuations of opposite sign in the winter hemisphere also yields significant coherency at periods near 27 and 13 days. Latitudinal temperature oscillations of this type result from interference between stationary and traveling wave components at stratospheric heights. It is therefore hypothesized that solar ultraviolet variations may force or modulate traveling waves with periods near 27 and 13 days in the upper stratosphere. The existence of such waves with higher amplitude near solar maximum than near solar minimum may help to explain observed solar cycle variations of zonally averaged winds and temperature in the upper stratosphere.

Hood, L. L.↗
NASA NTRS1991

The potential for ozone depletion in the Arctic polar stratosphere

The nature of the Arctic polar stratosphere is observed to be similar in many respects to that of the Antarctic polar stratosphere, where an ozone hole has been identified. Most of the available chlorine (CHl and ClONO2) was converted by reactions on polar stratospheric clouds to reactive ClO and Cl2O2 thoroughout the Arctic polar vortex before midwinter. Reactive nitrogen was converted to HNO3, and some, with spatial inhomogeneity, fell out of the stratosphere. These chemical changes ensured characteristic ozone losses of 10 to 15 percent at altitudes inside the polar vortex where polar stratospheric clouds had occurred. These local losses can translate into 5 to 8 percent losses in the vertical column abundance of ozone. As the amount of stratospheric chlorine inevitably increases by 50 percent over the next two decades, ozone losses recognizable as an ozone hole may well appear.

Brune, W. H.↗
NASA NTRS1991

Soot in the stratosphere - The impact of current and HSCT aircraft emissions

The emission of soot from existing and proposed aircraft and the contribution of this soot to concentrations observed in the troposphere and stratosphere are discussed. The implications of these emissions for issues in stratospheric physics and chemistry are examined. It is argued that, since soot concentrations in the stratosphere exceed those measured in the cleanest regions of the troposphere, it is possible that current aircraft emissions are the dominant source of stratospheric soot. A simple emission/dispersion model is presented that yields an estimate of aircraft contributions which is in agreement with the observations. The soot concentration is found to be too low to cause any detectable direct optical effects. It is estimated that emissions from the proposed fleet of high-speed civil transport stratospheric aircraft will lead to an increase in concentration of soot in the stratosphere by a factor of two or three.

Hansen, A. D. A.↗
NASA NTRS1990

In situ ozone measurements for the airborne arctic stratospheric experiment

The research provided in-situ ozone measurements onboard the NASA Ames DC-8 research aircraft during the 1989 Airborne Arctic Stratospheric Experiment. The Ames DC-8 and ER-2 aircraft performed extensive sampling of the Arctic stratosphere and troposphere in a program designed to study those factors important in ozone depletion in the Arctic during times when the polar vortex and meteorology are conducive to the formation of polar stratospheric clouds and/or an Arctic ozone hole. The DC-8 ozone instrument complement included in-situ measurements for H2O, NO, NO2, NO(y) gas, NO(y) particulate, as well as remote sensors for measuring the vertical distribution and column density of ozone above the aircraft altitude. The in-situ data (ozone, water vapor, and nitrogen species) at the aircraft altitude provide a definition of tropospheric conditions in the vicinity of the polar vortex and polar stratospheric clouds. Defining tropospheric conditions will assist in the understanding of the chemistry of both stratosphere and troposphere and the extent to which polar stratospheric clouds affect the chemistry of transported air.

Gregory, Gerald L.↗
NASA NTRS1992

Lidar Observations of Stratospheric Aerosol Layer After the Mt. Pinatubo Volcanic Eruption

The volcano Mt. Pinatubo located on the Luzon Island, Philippines, had explosively erupted on June 15, 1991. The volcanic eruptions such as volcanic ash, SO2 and H2O reached into the stratosphere over 30 km altitude by the NOAA-11 satellite observation and this is considered one of the biggest volcanic eruptions in this century. A grandiose volcanic eruption influences the atmosphere seriously and causes many climatic effects globally. There had been many impacts on radiation, atmospheric temperature and stratospheric ozone after some past volcanic eruptions. The main cause of volcanic influence depends on stratospheric aerosol, that stay long enough to change climate and other meteorological conditions. Therefore it is very important to watch stratospheric aerosol layers carefully and continuously. Standing on this respect, we do not only continue stratospheric aerosol observation at Tsukuba but also have urgently developed another lidar observational point at Naha in Okinawa Island. This observational station could be thought valuable since there is no lidar observational station in this latitudinal zone and it is much nearer to Mt. Pinatubo. Especially, there is advantage to link up these two stations on studying the transportation mechanism in the stratosphere. In this paper, we present the results of lidar observations at Tsukuba and Naha by lidar systems with Nd:YAG laser.

Nagai, Tomohiro↗
NASA NTRS1992

Lidar Measurements of Stratospheric Ozone, Temperature and Aerosol During 1992 UARS Correlative Measurement Campaign

Measurements of stratospheric ozone, temperature, and aerosols were made by the NASA/GSFC mobile stratospheric lidar during the UARS (Upper Atmospheric Research Satellite) Correlative Measurement Campaign at the JPL-Table Mountain Facility in Feb. and Mar. 1992. Due to the presence of substantial amounts of residual volcanic aerosol from the eruption of Mt. Pinatubo, the GSFC lidar system was modified for an accurate measurement of ozone concentration in the stratosphere. While designed primarily for the measurement of stratospheric ozone, this lidar system was also used to measure middle atmosphere temperature and density from 30 to 65 km and stratospheric aerosol from 15 to 35 km. In the following sections, we will briefly describe and present some typical measurements made during this campaign. Stratospheric ozone, temperature, and aerosols profiles derived from data taken between 15 Feb. and 20 Mar., 1992 will be presented at the conference.

Mcgee, Thomas J.↗
NASA NTRS1992

Black carbon (soot) aerosol in the lower stratosphere and upper troposphere

As determined by impactor samplers flown on ER-2 and DC-8 aircraft, black carbon aerosol (BCA) mass loadings in the stratosphere average 0.6 nanograms per standard cubic meter, or 0.01 percent of the total aerosol. Upper tropospheric BCA increases to 0.3 percent. Low stratospheric concentration is commensurate with present commercial air traffic fuel consumption, given the following assumptions: the BCA emissions are 0.1 grams per kilogram of fuel consumed, 10 percent of route mileage is above the tropopause, and average BCA stratospheric residence time is about one year. Taking BCA into account, the stratospheric single scatter albedo is about 0.99. Using parameters for planned supersonic commercial aircraft, whose emissions will be predominantly in the stratosphere, it is shown that such traffic will double stratospheric BCA concentration. This would reduce the aerosol single scattering albedo by one percent, and double the BCA surface area that is available for heterogeneous chemistry.

Pueschel, R. F.↗
NASA NTRS1993

Overview of the Stratospheric Aerosol and Gas Experiment II water vapor observations - Method, validation, and data characteristics

Results are presented of water vapor observations in the troposphere and stratosphere performed by the Stratospheric Aerosol and Gas Experiment II solar occultation instrument, and the analysis procedure, the instrument errors, and data characteristics are discussed. The results are compared with correlative in situ measurements and other satellite data. The features of the data set collected between 1985 and 1989 include an increase in middle- and upper-tropospheric water vapor during northern hemisphere summer and autumn; minimum water vapor values of 2.5-3 ppmv in the tropical lower stratosphere; slowly increasing water vapor values with altitude in the stratosphere, reaching 5-6 ppmv or greater near the stratopause; extratropical values with minimum profile amounts occurring above the conventionally defined tropopause; and higher extratropical than tropical water vapor values throughout the stratosphere except in locations of possible polar stratospheric clouds.

Rind, D.↗
NASA NTRS1993

Observational evidence of preferred flow regimes in the Northern Hemisphere winter stratosphere

Ten years of stratospheric geopotential height data are analyzed in an attempt to determine whether there are preferred flow regimes in the Northern Hemisphere winter stratosphere. The data are taken from Stratospheric Sounding Units on board NOAA satellites. The probability density estimate of the amplitude of the wavenumber 1 10-mb height is found to be bimodal. The density distribution is composed of a dominant large-amplitude mode and a less frequent low-amplitude mode. When the wavenumber 1 10-mb height data are projected onto the phase plane defined by the 10-mb zonal-mean winds and wavenumber 1 100-mb heights, three preferred regimes are evident. The small-amplitude mode separates into a strong zonal wind-weak wave regime and a weak zonal wind-weak wave regime. The large-amplitude mode is an intermediate zonal wind-strong wave regime. Transitions between the large-amplitude regime and the weak zonal wind-weak wave regime are found to be associated with major stratospheric warmings. The clustering of the stratospheric data into the preferred flow regimes is interpreted in light of the bifurcation properties of the Holton and Mass model. The interannual variability of the Northern Hemisphere winter stratosphere is interpreted in terms of the relative frequency of the observed preferred regimes.

Pierce, R. B.↗
NASA NTRS1994

Laboratory studies of chemical and photochemical processes relevant to stratospheric ozone

The purpose of this project is to reduce the uncertainty in several key gas-phase kinetic processes which impact our understanding of stratospheric ozone. The main emphasis of this work is on measuring rate coefficients and product channels for reactions of HO(sub x) and NO(sub x) species in the temperature range 200 K to 240 K relevant to the lower stratosphere. Other areas of study have included infrared spectroscopic studies of the HO2 radical, measurements of OH radical reactions with alternative fluorocarbons, and determination of the vapor pressures of nitric acid hydrates under stratospheric conditions. The results of these studies will improve models of stratospheric ozone chemistry and predictions of perturbations due to human influences. In this annual report, we focus on our recent accomplishments in the quantitative spectroscopy of the HO2 radical. This report details the measurements of the broadening coefficients for the v(sub 2) vibrational band. Further measurements of the vapor pressures of nitric acid hydrates relevant to the polar stratospheric cloud formation indicate the importance of metastable crystalline phases of H2SO4, HNO3, and H2O. Large particles produced from these metastable phases may provide a removal mechanism for HNO3 in the polar stratosphere.

Zahniser, Mark S.↗
NASA NTRS1994

Use of radon and cosmogenic radionuclides as indicators of exchange between troposphere and stratosphere

This research grant covered participation in the operational phase of NASA's Stratosphere-Troposphere Exchange Project (STEP), a multi-agency airborne science program conducted aboard NASA U-2 and ER-2 high altitude research aircraft. The primary goals of STEP were to investigate the mechanisms of irreversible movement of mass, trace gases, and aerosols from the troposphere into the stratosphere, and to explain the observed dryness of the stratosphere. Three flight experiments were conducted to address these questions: two extratropical experiments, in 1984 and 1986, and a tropical experiment, in 1987. The cosmogenic radionuclides Be-7 and P-32, produced in the stratosphere by cosmic rays, and Rn-222 (radon), emitted from continental soils, were well-suited as tracers of intra-stratospheric air mass movements, and to follow episodes of troposphere to stratosphere exchange. Measurements of Be-7 and P-32 were made in all three STEP experiments. Measurements of radon were made in the tropical experiment only. The equipment worked well, and produced a valuable data set in support of the STEP objectives, as indicated by the 'quick-look' results outlined.

Kritz, Mark A.↗
NASA NTRS1994

Observations of lower-stratospheric ClONO2, HNO3, and aerosol by the UARS CLAES experiment between January 1992 and April 1993

This paper discusses simultaneous measurements of stratospheric ClONO2, HNO3, temperature, and aerosol extinction coefficient by the Cryogenic Limb Array Etalon Spectrometer (CLAES) on the NASA Upper Atmosphere Research Satellite (UARS), obtained over the period 9 January 1992 through 23 April 1993. The discussion concentrates on the stratosphere region near 21 km of particular interest to heterogeneously driven ozone depletion. For periods between 12 June and 1 September 1992 at latitudes poleward of about 60 deg S, when temperatures were below type I polar stratospheric cloud (PSC) formation thresholds throughout the lower stratosphere, CLAES observed high levels of PSCs coincident with highly depleted fields of both HNO3 and ClONO2. By 17 September, the incidence of PSCs had greatly diminished in the lower stratosphere, but both CLONO2 and HNO3 remained highly depleted. These observations are consistent with the removal of gaseous HNO3 through the formation of nitric acid trihydrate (NAT) particles and the removal of ClONO2 through heterogeneous reactions on the particle surfaces. They also suggest substantial denitrification of the lower Antarctic vortex through sedimentation of PSC particles. In the Northern Hemisphere winter of 1992/93 far fewer PSCs were observed in the Arctic lower-stratosphere vortex, which had shorter periods and more localized regions of cold temperatures. Both HNO3 and ClONO2 maintained much higher levels inside the Arctic vortex than seen in the Antarctic throughout the winter/spring period. Following 28 February 1993 when Arctic vortex temperatures rose above 195 K, ClONO2 was observed in large quantities (greater than 2.1 ppbv near 21 km) inside the vortex. The persistence of relatively high levels of HNO3 inside the Arctic spring vortex compared with the low levels seen in the Antarctic spring vortex suggest a much lower level of denitrification in the Arctic.

Roche, A. E.↗
NASA NTRS1994

On the motion of air through the stratospheric polar vortex

Trajectory calculations using horizontal winds from the U.K. Meteorological Office data assimilation system and vertical velocities from a radiation calculation are used to simulate the three-dimensional motion of air through the stratospheric polar vortex for Northern Hemisphere (NH) and Southern Hemisphere (SH) winters since the launch of the Upper Atmosphere Research Satellite (UARS). Throughout the winter, air from the upper stratosphere moves poleward and descends into the middle stratosphere. In the SH lower to middle stratosphere, strongest descent occurs near the edge of the polar vortex, with that edge defined by mixing characteristics. The NH shows a similar pattern in late winter, but in early winter strongest descent is near the center of the vortex, except when wave activity is particularly strong. Strong barriers to latitudinal mixing exist above about 420 K throughout the winter. Below this, the polar night jet is weak in early winter, so air descending below that level mixes between polar and middle latitudes. In late winter, parcels descend less and the polar night jet moves downward, so there is less latitudinal mixing. The degree of mixing in the lower stratosphere thus depends strongly on the position and evolution of the polar night jet and on the amount of descent experienced by the air parcels; these characteristics show considerable interannual variability in both hemispheres. The computed trajectories provide a three-dimensional picture of air motion during the final warming. Large tongues of air are drawn off the vortex and stretched into increasingly long and narrow tongues extending into low latitudes. This vortex erosion process proceeds more rapidly in the NH than in he SH. In the lower stratosphere, the majority of air parcels remain confined within a lingering region of strong potential vorticity gradients into December in the SH and April in the NH, well after the vortex breaks up in the midstratosphere.

Manney, G. L.↗
NASA NTRS1995

Post-entry and volcanic contaminant abundances of zinc, copper, selenium, germanium and gallium in stratospheric micrometeorites

Some fraction of Zn, Cu, Se, Ga and Ge in chondritic interplanetary dust particles (IDPs) collected in the lower stratosphere between 1981 May and 1984 June has a volcanic origin. I present a method to evaluate the extent of this unavoidable type of stratospheric contamination for individual particles. The mass-normalized abundances for Cu and Ge as a function of mass-normalized stratospheric residence time show their time-integrated stratospheric aerosol abundances. The Zn, Se and Ga abundances show a subdivision into two groups that span approximately two-year periods following the eruptions of the Mount St. Helens (1980 May) and El Chichon (1982 April) volcanoes. Elemental abundances in particles collected at the end of each two-year period indicate low, but not necessarily ambient, volcanic stratospheric abundances. Using this time-integrated baseline, I calculate the straospheric contaminant fractions in nine IDPs and show that Zn, SE and Ga abundances in chondritic IDPs derive in part from stratospheric aerosol contaminants. Post-entry elemental abundances (i.e., the amount that survived atmospheric entry heating of the IDP) show enrichments relative to the CI abundances but in a smaller number of particles than previously suggested.

Rietmeijer, Frans J. M.↗
NASA NTRS1994

A model for studying the composition and chemical effects of stratospheric aerosols

We developed polynomial expressions for the temperature dependence of the mean binary and water activity coefficients for H2SO4 and HNO3 solutions. These activities were used in an equilibrium model to predict the composition of stratospheric aerosols under a wide range of environmental conditions. For typical concentrations of H2O, H2SO4, HNO3, HCl, HBr, HF, and HOCl in the lower stratosphere, the aerosol composition is estimated as a function of the local temperature and the ambient relative humidity. For temperatures below 200 K, our results indicate that (1) HNO3 contributes a significant mass fraction to stratospheric aerosols, and (2) HCl solubility is considerably affected by HNO3 dissolution into sulfate aerosols. We also show that, in volcanically disturbed periods, changes in stratospheric aerosol composition can significantly alter the microphysics that leads to the formation of polar stratospheric clouds. The effects caused by HNO3 dissolution on the physical and chemical properties of stratospheric aerosols are discussed.

Tabazadeh, Azadeh↗