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At least 199 records · Page 11

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DOE OSTI2025

Exploring transport-enabled gates with integrated optical addressing to demonstrate high fidelity control of trapped ion qubits in a scalable quantum computer

In recent years, experiments involving micofabricated surface ion traps have grown in complexity, and as this complexity grows, a common design has emerged in the form of quantum charge-coupled device architecture. This architecture, already utilized on multiple systems, supports multiple zones on a device for areas such as memory or computation. The shutting process between these zones is a process often seen to be minimized. An additional component to scalable surface trapped-ion experiments includes some form of integrated photonics, as free space lasers have difficulty scaling to many ions. Here, we discuss recent results in utilizing the shuttling process with integrated photonics to perform a specific type of gate, as well as demonstrating state preparation. Furthermore, we show that these gates can be utilized as a type of optical modulator as the Doppler shift that occurs during shuttling will make the light seen by shuttled ions different than that seen by stationary ions. Furthermore, we show that the shuttling operation can be utilized as an optical modulator, where the Doppler shift changes the frequency from that of a stationary ion.

42 ENGINEERING↗

DOE OSTI2023

3D-Printed Graded Electrode with Ultrahigh MnO 2 Loading for Non-Aqueous Electrochemical Energy Storage

Electrolytic manganese dioxide is one of the promising cathode candidates for electrochemical energy storage devices due to its high redox capacity and ease of synthesis. Yet, high-loading MnO 2 often suffers from sluggish reaction kinetics, especially in non-aqueous electrolytes. The non-uniform deposition of MnO 2 on a porous current collectors also makes it difficult to fully utilize the active materials at high mass loading. Here, a 3D printed graded graphene aerogel (3D GA) that contains sparsely separated exterior ligaments is developed to create large open channels for mass transport as well as densely arranged interior ligaments providing large ion-accessible active surface. The unique structural design homogenizes the thickness of electro deposited MnO 2 even at an ultrahigh mass loading of ≈70 mg cm -2 . The electrode achieves a remarkable volumetric capacity of 29.1 mA h cm -3 in the non-aqueous electrolyte. A Li-ion hybrid capacitor device assembled with a graded 3D GA/MnO2 cathode and graded 3D GA/VO x anode exhibits a wide voltage window of 0–4 V and a superior volumetric energy density of 20.2 W h L -1 . The findings offer guidance on 3D printed electrode design for supporting ultrahigh loading of active materials and developments of high energy density energy storage devices.

electrochemical energy storage↗

DOE OSTI2022

n-Type doping of a solution processed p-type semiconductor using isoelectronic surface dopants for homojunction fabrication

The p-n junction is one of the fundamental requirements for a practical semiconductor-based electronic device. Designing a heterojunction comprising of dissimilar p-type and n-type semiconductors calls for careful energy level considerations, both when selecting the semiconductor materials as well as the metal contacts. A homojunction based on a single semiconductor simplifies this task, as energy levels of the p-type and n-type materials are already fairly similar, allowing for easier selection of contacts. Traditionally, homojunctions rely on doping of a bulk semiconductor to achieve p- and n-type transport through controlled addition of aliovalent dopants via energy-intensive processes such as ion implantation or thermal annealing. Exact control of doping in nanocrystalline semiconductors is significantly more challenging, due to self-purification effects. However, owing to their large surface areas, surface moieties can be utilized to both dope the nanostructures as well as tune their energy levels. Here, we present a facile technique based on an isoelectronic surface dopant in order to achieve p- and n-type materials based on the same semiconductor. We show that thin p-type colloidal Bi 2 Te 3 nanowires can be switched to n-type through surface functionalization, thus increasing the availability of new nanocrystalline solution-processable p-n homojunctions.

42 ENGINEERING↗

DOE OSTI2019

Approaches to investigate the role of chelation in the corrosivity of biomass-derived oils

The need to provide the U.S. market with a renewable liquid fuel energy source from a non-food feedstock stream has gained considerable traction due to benefits such as improved energy efficiency, reduced environmental impacts, and enhanced national security. Practical achievement of these goals via biomass and bio-waste utilization involves production of liquid intermediates containing corrosive, reactive species like carboxylic acids, ketones, aldehydes, and hydroxyaldehydes. Such mixtures challenge materials of containment, processing, and transport. It is widely recognized that the smaller organic acids, such as acetic and formic, are corrosive and can remove protective surface oxides on alloys used in bio-oil processing infrastructure, and ketones can swell sealing polymers. However, literature shows, and findings herein confirm, larger carboxylic acids and bidentate alcohols are present. This highlights the potential for synergistic, detrimental effects of constituents in bio-oil corrosion, including direct reactivity of small acids compounded with the possibility of mobilization of protective metal oxide layers via chelation by larger acids and oxygenates. The question of whether species beyond small acids can significantly contribute to corrosion requires analytical approaches previously not applied to bio-oil corrosion studies and certainly not previously applied corroboratively. As such, this work introduces a combination of optical, mass spectral, and electrochemical impedance spectroscopies with an incubation approach to study metal mobilization, to facilitate elucidating chelation's role in bio-oil corrosive pathways. To enable systematic study of these oxygenates' material compatibility individually and in combination, a model matrix of bio-oil constituents was also developed based on identification of key components of real bio-oils.

09 BIOMASS FUELS↗

NASA NTRS1975

Development and parametric evaluation of the prototype 2 and 3 flash evaporators

Development of the Prototype 2 and 3 flash evaporator heat sinks which vaporize an expendable fluid to cool a heat transport fluid loop is reported. The units utilize Freon 21 as the heat transport fluid and water as the expendable fluid to meet the projected performance requirements of the space shuttle for both on-orbit and ascent/reentry operations. The evaporant is pulse-sprayed by on-off control onto heat transfer surfaces containing the transport fluid and exhausted to the vacuum environment through fixed area exhaust ducts.

Hixon, C. W.↗

NASA NTRS2010

Analysis of Shroud Options in Support of the Human Exploration of Mars

In support of the Mars Design Reference Architecture (DRA) 5.0, the NASA study team analyzed several shroud options for use on the Ares V launch vehicle.1,2 These shroud options included conventional "large encapsulation" shrouds with outer diameters ranging from 8.4 to 12.9 meters (m) and overall lengths of 22.0 to 54.3 meters, along with a "nosecone-only" shroud option used for Mars transfer vehicle component delivery. Also examined was a "multi-use" aerodynamic encapsulation shroud used for launch, Mars aerocapture, and entry, descent, and landing of the cargo and habitat landers. All conventional shroud options assessed for use on the Mars launch vehicles were the standard biconic design derived from the reference shroud utilized in the Constellation Program s lunar campaign. It is the purpose of this paper to discuss the technical details of each of these shroud options including material properties, structural mass, etc., while also discussing both the volume and mass of the various space transportation and surface system payload elements required to support a "minimum launch" Mars mission strategy, as well as the synergy, potential differences and upgrade paths that may be required between the Lunar and Mars mission shrouds.

Feldman, Stuart↗

DOE OSTI2025

Self-Organization of Plasma-Material Interfaces

The primary goals of the project are a) improve the understanding of transport processes, chemical reactions and plasma-driven self-organization such as stratification and filamentation, formation of anode spots, liquid droplets ejection from cathodes, and plasma electrolysis, b) utilize and share among the project participants computational tools developed by the participants to understand plasma-based surface functionalization and plasma-enabled pattern nucleation in a wide range of scales from nano- to millimeters, and c) use experimental methods and facilities available at the University of Alabama in Huntsville (UAH) and Sandia National Laboratories (SNL) to understand and control plasma processes, reaction pathways and the electric nature of self-organization of the plasma-exposed interface structures.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2023

Source attribution of near-surface ozone trends in the United States during 1995–2019

Emissions of ozone (O 3 ) precursors in the United States have decreased in recent decades, and near-surface O 3 concentrations showed a significant decrease in summer but an increase in winter. In this study, an O 3 source tagging technique is utilized in a chemistry–climate model to investigate the source contributions to O 3 mixing ratios in the US from various emitting sectors and regions of nitrogen oxides (NO x ) and reactive carbon species during 1995–2019. We show that domestic emission reductions from energy and surface transportation are primarily responsible for the decrease in summertime O 3 during 1995–2019. However, in winter, the emission control also weakens the NO x titration process, resulting in considerable increases in O 3 levels from natural sources. Additionally, increases in aviation and shipping emissions and transpacific transport of O 3 from Asia largely contribute to the winter O 3 increase. We also found that changes in large-scale circulation favoring O 3 transport from the upper atmosphere and foreign transport from Asia also explain 15 % of the increase in the US near-surface O 3 levels in winter.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NASA NTRS2013

Global Mobile Satellite Service Interference Analysis for the AeroMACS

The AeroMACS (Aeronautical Mobile Airport Communications System), which is based on the IEEE 802.16-2009 mobile wireless standard, is envisioned as the wireless network which will cover all areas of airport surfaces for next generation air transportation. It is expected to be implemented in the 5091-5150 MHz frequency band which is also occupied by mobile satellite service uplinks. Thus the AeroMACS must be designed to avoid interference with this incumbent service. Simulations using Visualyse software were performed utilizing a global database of 6207 airports. Variations in base station and subscriber antenna distribution and gain pattern were examined. Based on these simulations, recommendations for global airport base station and subscriber antenna power transmission limitations are provided.

Wilson, Jeffrey D.↗

NASA NTRS2013

Global Mobile Satellite Service Interference Analysis for the AeroMACS

Wilson, Jeffrey D.↗

NASA NTRS2015

Human Exploration of Phobos

This study developed, analyzed, and compared mission architectures for human exploration of Mars' Moons within the context of an Evolvable Mars Campaign. METHODS: All trades assumed conjunction class missions to Phobos (approximately 500 days in Mars system) as it was considered the driving case for the transportation architecture. All architectures assumed that the Mars Transit Habitat would remain in a High Mars Orbit with crewmembers transferring between HMO and Phobos in a small crew taxi vehicle. A reference science / exploration program was developed including performance of a standard set of tasks at 55 locations on the Phobos surface. Detailed EVA timelines were developed using realistic flight rules to accomplish the reference science tasks using exploration systems ranging from jetpacks to multi-person pressurized excursion vehicles combined with Phobos surface and orbital (L1, L4/L5, 20km Distant Retrograde Orbit) habitat options. Detailed models of propellant mass, crew time, science productivity, radiation exposure, systems and consumables masses, and other figures of merit were integrated to enable quantitative comparison of different architectural options. Options for pre-staging assets using solar electric propulsion (SEP) vs. delivering all systems with the crew were also evaluated. Seven discrete mission architectures were evaluated. RESULTS: The driving consideration for habitat location (Phobos surface vs. orbital) was radiation exposure, with an estimated reduction in cumulative mission radiation exposure of up to 34% (vs. Mars orbital mission) when the habitat is located on the Phobos surface, compared with only 3-6% reduction for a habitat in a 20km DRO. The exploration utility of lightweight unpressurized excursion vehicles was limited by the need to remain within 20 minutes of Solar Particle Event radiation protection combined with complex GN&C systems required by the non-intuitive and highly-variable gravitational environment. Two-person pressurized excursion vehicles as well as mobile surface habitats offer significant exploration capability and operational benefits compared with unpressurized EVA mobility systems at the cost of increased system and propellant mass. Mechanical surface translation modes (i.e. hopping) were modeled and offer potentially significant propellant savings and the possibility of extended exploration operations between crewed missions. Options for extending the utilization of the crew taxi vehicle were examined, including use as an exploration asset for Phobos surface exploration (when combined with an alternate mobility system) and as an EVA platform, both on Phobos and for contingency EVA on the Mars Transit Habitat. CONCLUSIONS: Human exploration of Phobos offers a scientifically meaningful first step towards human Mars surface missions that develops and validates transportation, habitation, and exploration systems and operations in advance of the Mars landing systems.

Abercromby, Andrew F. J.↗

NASA NTRS1997

In Situ Resource Utilization (ISRU II) Technical Interchange Meeting

This volume contains extended abstracts that have been accepted for presentation at the In Situ Resource Utilization (ISRU II) Technical Interchange Meeting, November 18-19, 1997, at the Lunar and Planetary Institute, Houston, Texas. Included are topics which include: Extraterrestrial resources, in situ propellant production, sampling of planetary surfaces, oxygen production, water vapor extraction from the Martian atmosphere, gas generation, cryogenic refrigeration, and propellant transport and storage.

David Kaplan↗

NASA NTRS2017

Robust Exploration and Commercial Missions to the Moon Using LANTR Propulsion and Lunar Liquid Oxygen Derived from FeO-Rich Pyroclastic Deposits

Studies conducted by NASA and its contractors (early 1980s early 1990s) indicated a substantial benefit from using lunar-derived propellants specifically lunar-derived LO2 (LLO2) or LUNOX in a lunar space transportation system (LTS). With a LTS using LO2/LH2 chemical rockets, approx. 6 kilograms (kg) of mass in low Earth orbit (LEO) is required to place 1 kg of payload on the lunar surface (LS). Of this 6 kg, approx. 70% (4.2 kg) is propellant and 6/7th of this mass (3.6 kg) is oxygen assuming an O/H MR 6:1. Since the cost of placing a kilogram of mass on the LS is approx. 6X the cost of delivering it to LEO, the ability to produce and utilize LUNOX or lunar-derived LO2 and hydrogen (LLH2) from lunar polar ice (LPI) deposits can provide significant mission leverage. Providing LUNOX for use in fuel cells, life support systems and LO2/LH2 chemical rockets used on lunar landing vehicles (LLVs), can allow high value cargo (people, manufacturing and scientific equipment, etc.) to be transported to LEO, then to the Moon instead of bulk LO2 propellant. Oxygen is abundant in the lunar regolith (approx. 43% by mass) and can be extracted using a variety of techniques, such as hydrogen reduction of ilmenite (FeOTiO2) or FeO-rich volcanic glass (orange soil) discovered during the Apollo 17 mission to Taurus-Littrow. While considerable interest has been expressed about mining and processing LPI for rocket propellant, ground truth must first be established to quantify the physical state of the ice (e.g., its vertical thickness and areal extent, levels of soil contamination, etc.) and the deep, extremely cold (approx. 26-100 K) permanently shadowed craters where the ice resides.

Nuclear Thermal Propulsion↗

NASA NTRSDate not supplied

NASA Plans for In Situ Resource Utilization (ISRU) Development, Demonstration, and Implementation

The United States (US) National Aeronautics and Space Administration’s (NASA) Artemis Moon to Mars program has four major goals: (1) Returning Americans to the Moon: 1st Woman & 1st Person of Color, (2) Learning to live and work on the Moon, (3) Translating lessons learned so that the United States has capabilities and operational experience for a mission to Mars, and (4) Inspires the next generation of explorers, researchers, scientists, and engineers worldwide. Overarching all of this, the NASA Artemis program also continues to follow Space Policy Directive One (SPD-1) which directs the US to lead an innovative and sustainable exploration program with commercial and international partners. A major objective to achieve the Artemis program goals and SPD-1 is to understand and characterize the resources that exist at these destinations, and to learn how to utilize these resources for sustained human exploration and the commercialization of space. This ability, commonly known as In Situ Resource Utilization (ISRU), involves any hardware or operation that harnesses and utilizes local resources to create products and services for robotic and human explo-ration. The NASA ISRU program is focused on the production of mission consumables and com-modities to enable sustained human exploration, such as rocket propellants, life support consuma-bles, fuel cell reactants, feedstock for manufacturing and construction, and nutrients for food and plant growth. In particular, propellants make up a significant fraction of the mass launched from Earth, are critical to mission success, and can reduce the cost for reusable transportation. Important for enabling long term surface stays, greater independence from Earth, and growing lunar infra-structure are the abilities to perform construction and manufacturing from in situ-derived metals and materials to create and expand on the infrastructure and reduce the logistical resupply needed for sustained surface and space operations. To achieve these ISRU capabilities, NASA, in partner-ship with industry, academia, and international partners has initiated a multi-faceted program which involves (i) Determining Customer Needs (Type and Quantity of Commodities), (ii) supporting ground Development of Hardware and Systems until Ready for Lunar Flight, (iii) utilize Commer-cial Lunar Payload Services (CLPS) flights to fly resource assessment missions with the Science Mission Directorate (SMD), and public-private partnership (PPP) ISRU demonstrations of critical technologies and processes, and (iv) performing commercial-led end-to-end ‘Pilot’ Plant production of commodities and demonstration of usage at a scale and duration that minimizes or eliminates risk for full implementation of ISRU-derived commodities in mission critical applications. This paper will discuss the technologies, mission studies, and accomplishments achieved to date for the ISRU multi-faceted program, and plans for continued ground development and flight missions to reduce the risk of full ISRU implementation.

In situ resource utilization↗

NASA NTRS2012

Modular Flooring System

The modular flooring system (MFS) was developed to provide a portable, modular, durable carpeting solution for NASA fs Robotics Alliance Project fs (RAP) outreach efforts. It was also designed to improve and replace a modular flooring system that was too heavy for safe use and transportation. The MFS was developed for use as the flooring for various robotics competitions that RAP utilizes to meet its mission goals. One of these competitions, the FIRST Robotics Competition (FRC), currently uses two massive rolls of broadloom carpet for the foundation of the arena in which the robots are contained during the competition. The area of the arena is approximately 30 by 72 ft (approximately 9 by 22 m). This carpet is very cumbersome and requires large-capacity vehicles, and handling equipment and personnel to transport and deploy. The broadloom carpet sustains severe abuse from the robots during a regular three-day competition, and as a result, the carpet is not used again for competition. Similarly, broadloom carpets used for trade shows at convention centers around the world are typically discarded after only one use. This innovation provides a green solution to this wasteful practice. Each of the flooring modules in the previous system weighed 44 lb (.20 kg). The improvements in the overall design of the system reduce the weight of each module by approximately 22 lb (.10 kg) (50 %), and utilize an improved "module-to-module" connection method that is superior to the previous system. The MFS comprises 4-by-4-ft (.1.2-by- 1.2-m) carpet module assemblies that utilize commercially available carpet tiles that are bonded to a lightweight substrate. The substrate surface opposite from the carpeted surface has a module-to-module connecting interface that allows for the modules to be connected, one to the other, as the modules are constructed. This connection is hidden underneath the modules, creating a smooth, co-planar flooring surface. The modules are stacked and strapped onto durable, commercially available drywall carts for storage and/or transportation. This method of storage and transportation makes it very convenient and safe when handling large quantities of modules.

Thate, Robert↗

DOE OSTI2025

Sulfonated Diels–Alder Poly(Phenylene)s in Membrane Electrode Assemblies for Fuel Cells

The transition to environmentally sustainable materials in fuel cells requires alternatives to persistent polyfluoroalkyl substances (PFAS) like Nafion. This study investigates the performance-limiting factors of membrane electrode assemblies (MEAs) utilizing sulfonated Diels–Alder poly(phenylene)s (sDAPPs) as PFAS-free polymer electrolytes. Among the configurations evaluated, the greatest performance loss occurred when sDAPP is used as the cathode binder, primarily due to phenyl group adsorption on catalyst surfaces, which reduces oxygen reduction reaction activity and impedes oxygen transport. Additional performance degradation arises from membrane-electrode interfacial incompatibility and insufficient ionomer hydrophobicity. By addressing ionomer adsorption and improving interfacial contact, an sDAPP-based cathode achieved a current density of 1.57 A cm −2 at 0.6 V under fully humidified H 2 /air conditions at 80 °C and 150 kPa abs . These results offer key insights for advancing high-performance, PFAS-free fuel cell technologies.

08 HYDROGEN↗

NASA NTRS1971

Field evaporation ion source with possible application to electrostatic propulsion

Field evaporation of solid metal electrodes has been proposed as an ion source for an electrostatic propulsion device. The chief advantage over existing ion sources is the prospect of 100 percent fuel utilization efficiency. This advantage arises as a result of the elimination of the need for a gaseous precursor state for propellant ionization. The attainment of required high surface field strengths is achieved through field-induced extrusion of the electrode geometry at elevated temperatures. Contributions of both surface and bulk transport mechanisms are taken into account.

Weizer, V. G.↗

NASA NTRS1979

Solar energy collection system

A fixed, linear, ground-based primary reflector having an extended curved sawtooth-contoured surface covered with a metalized polymeric reflecting material, reflects solar energy to a movably supported collector that is kept at the concentrated line focus reflector primary. The primary reflector may be constructed by a process utilizing well known freeway paving machinery. The solar energy absorber is preferably a fluid transporting pipe. Efficient utilization leading to high temperatures from the reflected solar energy is obtained by cylindrical shaped secondary reflectors that direct off-angle energy to the absorber pipe. A seriatim arrangement of cylindrical secondary reflector stages and spot-forming reflector stages produces a high temperature solar energy collection system of greater efficiency.

Miller, C. G.↗