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Introduction to: Atlantic Meridional Overturning Circulation(AMOC)

A striking conclusion of the Intergovernmental Panel on Climate Change 2007 report is the crucial role that the Atlantic Meridional Overturning Circulation (AMOC) may play in anthropogenic climate change. However, these IPCC coupled climate simulations show a broad range of uncertainty in the magnitude and timing of AMOC transport change ranging from none to nearly complete collapse within the 21st century. The potential consequences of large changes in the characteristics of AMOC have motivated the creation in the United States of an interagency program and implementation plan to develop monitoring and prediction capabilities for the AMOC This program parallels the development of substantial monitoring efforts by European, South American and African countries -- notably the UK Rapid and Rapid-Watch programs. The papers contained in this volume are derived from presentations at the First U.S. Atlantic Meridional Overturning Circulation (AMOC) Meeting held 4 - 6 May, 2009 to review the US implementation plan and its coordination with other monitoring activities. The Atlantic Meridional Overturning Circulation consists of multiple components illustrated in an attached figure. Water enters the South Atlantic at upper and intermediate depths through both western and eastern routes (where eddy transport is especially important) and is transported northward across the equator, where it recirculates within the northern subtropical and subpolar gyres. The northern end is defined by the sinking regions of the Nordic Seas and the Labrador Sea where the waters that eventually form the upper and lower branches of North Atlantic Deep Water are conditioned. High surface salinities, the result of high net evaporation in the tropics and subtropics (including the Mediterranean Sea), and presence of regions of the Arctic Ocean that remain ice-free even in winter allow for the rapid cooling and thus densification of surface water. This dense surface water becomes the source of deep water formation in the sinking regions. In addition to transporting mass, the AMOC transports roughly half of the total amount of heat carried northward through the northern subtropics (down the temperature-gradient) by the ocean. In contrast in the Southern Hemisphere AMOC transports heat up-gradient from the cool Circumpolar Current to the warm tropics. Paleoevidence suggests that AMOC heat transport in the two hemispheres has varied over time in ways intimately tied to millennial changes in the Earth's climate. In one example, the abrupt Younger Dryas spell of cold weather over the North Atlantic, which began 13,000 years ago, has generally been linked to a millennial shutdown of the AMOC as a result of massive freshwater discharge from the North American continent. The current AMOC monitoring array consists of a series of instrumented transects located across key passages (see Cunningham et al., 2010 for a recent review). In the Arctic and sub-Arctic, transects cross Fram Strait, Denmark Strait and the Faroe Channel (connecting Greenland, Iceland, and the United Kingdom), as well as the entrance to the Labrador Sea. Further south and extending outwards from the east coast of North America there are a series of monitoring arrays including arrays of the Canadian Atlantic Zone Monitoring Program, deployments of the Rapid Western Atlantic Variability Experiment (WAVE), Line W at 39 N, as well as the Rapid-MOC moored array. The latter spans the entire Atlantic basin along 26.5 N. At tropical latitudes we have the Meridional Overturning Variability Experiment (MOVE) array at 16 N, while in the Southern Hemisphere a corresponding basin-spanning transect is being established at the latitude of Cape of Good Hope, complemented by arrays at Drake Passage.

Hakkinen, Sirpa↗

The Low-Frequency Variability of the Tropical Atlantic Ocean

Upper ocean temperature variability in the tropical Atlantic is examined from the Comprehensive Ocean Atmosphere Data Set (COADS) as well as from an ocean model simulation forced by COADS anomalies appended to a monthly climatology. Our findings are as follows: Only the sea surface temperatures (SST) in the northern tropics are driven by heat fluxes, while the southern tropical variability arises from wind driven ocean circulation changes. The subsurface temperatures in the northern and southern tropics are found to have a strong linkage to buoyancy forcing changes in the northern North Atlantic. Evidence for Kelvin-like boundary wave propagation from the high latitudes is presented from the model simulation. This extratropical influence is associated with wintertime North Atlantic Oscillation (NAO) forcing and manifests itself in the northern and southern tropical temperature anomalies of the same sign at depth of 100-200 meters as result of a Rossby wave propagation away from the eastern boundary in the wake of the boundary wave passage. The most apparent association of the southern tropical sea surface temperature anomalies (STA) arises with the anomalous cross-equatorial winds which can be related to both NAO and the remote influence from the Pacific equatorial region. These teleconnections are seasonal so that the NAO impact on the tropical SST is the largest it mid-winter but in spring and early summer the Pacific remote influence competes with NAO. However, NAO appears to have a more substantial role than the Pacific influence at low frequencies during the last 50 years. The dynamic origin of STA is indirectly confirmed from the SST-heat flux relationship using ocean model experiments which remove either anomalous wind stress forcing or atmospheric forcing anomalies contributing to heat exchange.

Haekkinen, Sirpa↗

Changing Hydroclimate Dynamics and the 19th to 20th Century Wetting Trend in the English Channel Region of Northwest Europe

Northwestern Europe has experienced a trend of increasingly wet winters over the past 150 years, with few explanations for what may have driven this hydroclimatic change. Here we use the Old World Drought Atlas (OWDA), a tree-ring based reconstruction of the self-calibrating Palmer Drought Severity Index (scPDSI), to examine this wetting trend and place it in a longer hydroclimatic context. We find that scPDSI variability in northwestern Europe is strongly correlated with the leading mode of the OWDA during the last millennium (1000–2012). This leading mode, here named the ‘English Channel’ (EC) mode, has pronounced variability on interannual to centennial timescales and has an expression in scPDSI similar to that of the East Atlantic teleconnection pattern. A shift in the EC mode from a prolonged negative phase to more neutral conditions during the 19th and 20th centuries is associated with the wetting trend over its area of influence in England, Wales, and much of northern continental Europe. The EC mode is the dominant scPDSI mode from approximately 1000–1850, after which its dominance waned in favor of the secondary ‘North–South’ (NS) mode, which has an expression in scPDSI similar to that of the winter North Atlantic Oscillation (NAO). We examine the dynamical nature of both of these modes and how they vary on interannual to centennial timescales. Our results provide insight into the nature of hydroclimate variability in Europe before the widespread availability of instrumental observations.

hydroclimate↗

Can We Better Constrain the Timing of GNAIW/UNADW Variability in the Western Equatorial Atlantic and Its Relationship to Climate Change During the Last Deglaciation?

We have revisited the well-trod VM28-122 core retrieved from the deep Colombian Basin, which includes sediments that reflect modern Upper North Atlantic Deep Water and extends through the last deglaciation into the last glacial period when the site was bathed in Glacial North Atlantic Intermediate Water. Here, we leverage the nearby Cariaco Basin's surface water radiocarbon reconstruction (reservoir age, and ΔR) on the IntCal20 timescale to recast the period of the last deglaciation with a newly constrained age model. Based on the revised age model, we observe that the multimillennial decrease in benthic δ 13 C and B/Ca (which record δ 13 C of dissolved inorganic carbon and Δ[CO 3 –2 ], respectively) began at 18,100 ± 240 (95% CI) calibrated years BP, synchronous with Termination 1, as identified by changes in the Antarctic Ice Sheet composite and by the onset of rapid glacier recession in the Southern Hemisphere (Denton et al., 2010, https://doi.org/10.1126/science.1184119; Denton et al., 2021, https://10.1016/j.quascirev.2020.106771). The beginning of the decrease in benthic δ 18 O is concurrent with the changes in carbon chemistry or at most, a few hundred years later. It is no later than 17,700 ± 300 (95% CI) yrs BP in our record, at the putative start of Heinrich Stadial 1. With sufficient data density (more than 2–3 control points per kyr) and an independent record of past surface water radiocarbon variations, it is possible to achieve late glacial and deglacial chronologies with fidelities similar to those of ice cores. Furthermore, doing so in more oceanographic locations should shed light more broadly on the mechanisms instrumental to abrupt climate change.

58 GEOSCIENCES↗

Impacts, processes and projections of the quasi-biennial oscillation

In the tropical stratosphere, deep layers of eastward and westward winds encircle the globe and descend regularly from the upper stratosphere to the tropical tropopause. With a complete cycle typically lasting almost 2.5 years, this quasi-biennial oscillation (QBO) is arguably the most predictable mode of atmospheric variability that is not linked to the changing seasons. Here, the QBO affects climate phenomena outside the tropical stratosphere, including ozone transport, the North Atlantic Oscillation and the Madden–Julian Oscillation, and its high predictability could enable better forecasts of these phenomena if models can accurately represent the coupling processes. Climate and forecasting models are increasingly able to simulate stratospheric oscillations resembling the QBO, but exhibit common systematic errors such as weak amplitude in the lowermost tropical stratosphere. Uncertainties about the waves that force the oscillation, particularly the momentum fluxes from small-scale gravity waves excited by deep convection, make its simulation challenging. Improved representation of the processes governing the QBO is expected to lead to better forecasts of the oscillation and its impacts, increased understanding of unusual events such as the two QBO disruptions observed since 2016, and more reliable future projections of QBO behaviour under climate change.

54 ENVIRONMENTAL SCIENCES↗

Subtropical Gyre Variability as Seen from Satellites

A satellite multi-sensor approach is used to analyse the biological response of open ocean regions of the subtropical gyres to changes in physical forcing. Thirteen years (1998-2010) of SeaWiFS chlorophyll a (Chl-a), combined with concurrent satellite records of sea-surface temperature (SST) and sea level height, were analysed to investigate the seasonal and interannual variability of Chl-a concentration within these immense so-called ocean deserts. The seasonal variability of Chl-a within the gyres is driven mostly by the warming/cooling of surface waters. Summer warming promotes shallower mixed layers and lower Chl-a due to a reduction of vertical mixing and consequently a decrease in nutrient supply. The opposite happens during the winter cooling period. Therefore, long-term trends in SST have the potential to cause an impact on the interannual variability of Chl-a. Our analyses show that, during the 13 whole years of SeaWiFS data record, the North Pacific, Indian Ocean, and North Atlantic gyres experienced a decrease in Chl-a of 9%, 12%, and 11%, respectively, with corresponding SST increases of 0.27 C, 0.42 C, and 0.32 C. The South Pacific and South Atlantic gyres also showed warming trends but with weak positive trends in Chl-a that are not statistically significant. We hypothesize that the warming of surface waters in these two gyres are counterbalanced by other interacting physical and biological driving mechanisms, as indicated in previous studies.

Signorini, Sergio R.↗

Revisiting the Relationship between Atlantic Dust and Tropical Cyclone Activity using Aerosol Optical Depth Reanalyses: 2003-2018

Previous studies have noted a relationship between African dust and Atlantic tropical cyclone (TC) activity. However, due to the limitations of past dust analyses, the strength of this relationship remains uncertain. The emergence of aerosol reanalyses, including the Navy Aerosol Analysis and Prediction System (NAAPS) aerosol optical depth (AOD) reanalysis, NASA Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2), and ECMWF Copernicus Atmosphere Monitoring Service reanalysis (CAMSRA), enables an investigation of the relationship between African dust and TC activity over the tropical Atlantic and Caribbean in a consistent temporal and spatial manner for 2003–2018. Although June–July–August (JJA) 550 nm dust AOD (DAOD) from all three reanalysis products correlates significantly over the tropical Atlantic and Caribbean, the difference in DAOD magnitude between products can be as large as 60 % over the Caribbean and 20 % over the tropical North Atlantic. Based on the three individual reanalyses, we have created an aerosol multi-reanalysis consensus (MRC). The MRC presents overall better root mean square error over the tropical Atlantic and Caribbean compared to individual reanalyses when verified with ground-based AErosol RObotic NETwork (AERONET) AOD measurements. Each of the three individual reanalyses and the MRC have significant negative correlations between JJA Caribbean DAOD and seasonal Atlantic accumulated cyclone energy (ACE), while the correlation between JJA tropical North Atlantic DAOD and seasonal ACE is weaker. Possible reasons for this regional difference are provided. A composite analysis of 3 high-JJA-Caribbean-DAOD years versus 3 low-JJA-Caribbean-DAOD years reveals large differences in overall Atlantic TC activity. We also show that JJA Caribbean DAOD is significantly correlated with large-scale fields associated with variability in interannual Atlantic TC activity including zonal wind shear, mid-level moisture, and sea surface temperature (SST), as well as the El Niño–Southern Oscillation (ENSO) and the Atlantic Meridional Mode (AMM), implying confounding effects of these factors on the dust–TC relationship. We find that seasonal Atlantic DAOD and the AMM, the leading mode of coupled Atlantic variability, are inversely related and intertwined in the dust–TC relationship. Overall, DAOD in both the tropical Atlantic and Caribbean is negatively correlated with Atlantic hurricane frequency and intensity, with stronger correlations in the Caribbean than farther east in the tropical North Atlantic.

Dust particles↗

Remote Sensing of Particulate Organic Carbon Pools in the High-Latitude Oceans

The general goal of this project was to characterize spatial distributions at basin scales and variability on monthly to interannual timescales of particulate organic carbon (POC) in the high-latitude oceans. The primary objectives were: (1) To collect in situ data in the north polar waters of the Atlantic and in the Southern Ocean, necessary for the derivation of POC ocean color algorithms for these regions. (2) To derive regional POC algorithms and refine existing regional chlorophyll (Chl) algorithms, to develop understanding of processes that control bio-optical relationships underlying ocean color algorithms for POC and Chl, and to explain bio-optical differentiation between the examined polar regions and within the regions. (3) To determine basin-scale spatial patterns and temporal variability on monthly to interannual scales in satellite-derived estimates of POC and Chl pools in the investigated regions for the period of time covered by SeaWiFS and MODIS missions.

Stramski, Dariusz↗

Relative frequency and diurnal variation of high cold clouds in the tropical Atlantic and Pacific

The percentage of cold clouds less than or equal to 240 K was tabulated from Nimbus-5 data in 2 deg latitude-longitude squares over tropical oceans in the North Atlantic and Pacific for day (1130 LST) and night (2330 LST). The maximum percentage and amplitude of the diurnal variation are in the eastern Atlantic and Pacific. Day percentages are higher than at night in the entire 6-10 deg N belt of the Atlantic. Weaker night maxima are to the north and south of this belt. In the Pacific, the distribution of day and night predominance is more variable.

Wexler, R.↗

Observations of the Global Characteristics and Regional Radiative Effects of Marine Cloud Liquid Water

The large-scale spatial distribution and temporal variability of cloud liquid water path (LWP) over the world's oceans and the relationship of cloud LWP to temperature and the radiation budget are investigated using recent satellite measurements from the Special Sensor Microwave/Imager (SSM/I), the Earth Radiation Budget Experiment (ERBE), and the International Satellite Cloud Climatology Project (ISCCP). Observations of cloud liquid water on a 2.5 deg x 2.5 deg and are used over a 53-month period beginning July 1987 and ending in December 1991. The highest values of cloud liquid water (greater than 0.13 kg/sq m) occur largely along principal routes of northern midlatitude storms and in areas dominated by tropical convection. The zonally averaged structure is distinctly trimodal, where maxima appear in the midlatitudes and near the equator. The average marine cloud LWP over the globe is estimated to be about 0.113 kg/sq m. Its highest seasonal variability is typically between 15% and 25% of the annual mean but in certain locations can exceed 30%. Comparisons of cloud LWP to temperature for low clouds during JJA and DJF of 1990 show significant positive correlations at colder temperatures and negative correlations at warmer temperatures. The correlations also exhibit strong seasonal and regional variation. Coincident and collocated observations of cloud LWP from the SSM/I and albedo measurements from the Earth Radiation Budget Satellite (ERBS) and the NOAA-10 satellite are compared for low clouds in the North Pacific and North Atlantic. The observed albedo-LWP relationships correspond reasonably well with theory, where the average cloud effective radius (r(sub e)) is 11.1 microns and the standard deviation is 5.2 microns. The large variability in the inferred values of r(sub e) suggests that other factors may be important in the albedo-LWP relationships. In terms of the effect of the LWP on the net cloud forcing, the authors find that a 0.05 kg/sq m increase in LWP (for LWP less than 0.2 kg/sq m) results in a -25 W/sq m change in the net cloud forcing at a solar zenith angle of 75 deg.

Greenwald, Thomas J.↗

Are 100 Ensemble Members Enough to Capture the Remote Atmospheric Response to +2°C Arctic Sea Ice Loss?

This study presents results from the Polar Amplification Multimodel Intercomparison Project (PAMIP) single-year time-slice experiments that aim to isolate the atmospheric response to Arctic sea ice loss at global warming levels of +2°C. Using two general circulation models (GCMs), the ensemble size is increased up to 300 ensemble members, beyond the recommended 100 members. After partitioning the response in groups of 100 ensemble members, the reproducibility of the results is evaluated, with a focus on the response of the midlatitude jet streams in the North Atlantic and North Pacific. Both atmosphere-only and coupled ocean–atmosphere PAMIP experiments are analyzed. Substantial differences in the midlatitude response are found among the different experiment subsets, suggesting that 100-member ensembles are still significantly influenced by internal variability, which can mislead conclusions. Despite an overall stronger response, the coupled ocean–atmosphere runs exhibit greater spread due to additional ENSO-related internal variability when the ocean is interactive. The lack of consistency in the response is true for anomalies that are statistically significant according to Student’s t and false discovery rate tests. This is problematic for the multimodel assessment of the response, as some of the spread may be attributed to different model sensitivities whereas it is due to internal variability. Here, we propose a method to overcome this consistency issue that allows for more robust conclusions when only 100 ensemble members are used.

58 GEOSCIENCES↗

Constraining the Varied Response of Northern Hemisphere Winter Circulation Waviness to Climate Change

Abstract While a large latitudinal displacement of the westerly jet brings about disproportionate socioeconomic impacts over Northern Hemisphere midlatitude continents, it is not well understood as to whether the winter circulation will become wavier or less in response to climate change. Here, using observations and large ensembles of climate models, we show that changes in atmospheric waviness can be estimated from the optimal structures of the westerly jet for wavier circulation, which are obtained from an advection‐diffusion model. Thus, the changes in westerly jet structure in climate models under climate change provide a physical constraint on changes in atmospheric waviness, indicating that the North Atlantic wave activity will experience a robust decline in a warmer climate, while future North Pacific wave activity is obscured by model uncertainty rather than internal variability. These findings highlight the changes to jet stream structure as a constraint for regional circulation waviness in a changing climate.

54 ENVIRONMENTAL SCIENCES↗

Evaluating Entrainment–Mixing Characteristics through Direct Comparisons of Drop Size Distributions Using In Situ Observations from ACE-ENA

Abstract Constraining the impacts of entrainment and associated mixing (i.e., entrainment–mixing) on cloud properties continues to be difficult, partly due to observational uncertainties as well as a lacking consensus of which methodologies for diagnosing entrainment–mixing are most appropriate. This study introduces a novel method to evaluate the presence and degree of inhomogeneous and homogeneous mixing using ∼100 h of in situ observations from a research aircraft over the northeastern Atlantic. Specifically, drop size distributions are compared between regions containing negligible and significant entrainment for select flight legs, making a direct characterization of the degree of homogeneous and inhomogeneous mixing possible. A measure of drop concentration variance is used as a proxy variable to diagnose entrainment–mixing. Results correspond well with entrainment–mixing metrics, showing lower Damköhler numbers where drop size distributions shift toward smaller drop sizes (i.e., inhomogeneous mixing) and greater transition length scales where drop size distributions do not (i.e., homogeneous mixing). Inhomogeneous mixing occurs in most samples from Aerosol and Cloud Experiment in the Eastern North Atlantic (ACE-ENA) (regardless of homogeneous mixing frequencies increasing with increasing spatial resolution from ∼100 to ∼10 m) and is associated with decreased drop size relative dispersion and both greater aerosol and drop concentrations compared with homogeneous mixing. Precipitating clouds have a greater frequency of homogeneous mixing compared with nonprecipitating clouds. The proposed methodology is similarly applied to in situ observations of southeast Pacific stratocumulus, shallow convective clouds over central Oklahoma and low-level clouds over the Southern Ocean. All four locations are primarily dominated by inhomogeneous mixing with minimal variability among each region.

Clouds↗

Aircraft NO(x) had no Unique Fingerprint on Sonex; Lightning Dominated Fresh NO(x) Sources

Key questions to which SONEX was directed were the following: Can aircraft corridors be detected? Is there a unique tracer for aircraft NO(x)? Can a "background" NO(x) (or NO(y) be defined? What fraction of NO(x) measured during SONEX was from aircraft? How representative was SONEX of the North Atlantic in 1997 and how typical of other years? We attempt to answer these questions through species-species correlations, probability distribution functions (PDFs), and meteorological history. There is not a unique aircraft tracer, largely due to the high variability of air mass origins and tracer ratios, which render "average" quantities meaningless. The greatest NO and NO(y) signals were associated with lightning and convective NO sources. Well-defined background CO, NO(y) and NO(y)/ozone ratio appear in subsets of two cross-track flights with subtropical origins and five flights with predominantly mid-latitude air. Forty percent of the observations on these 7 flights showed NO(y)/ozone to be above background, evidently due to unreacted NO(x). This NO(x) is a combination of aircraft, lightning and surface pollution injected by convection. The strongly subtropical signatures in SONEX observations, confirmed by pv (potential vorticity) values along flight tracks, argues for most of the unreacted NO(x) originating from lightning. Potential vorticity statistics along SONEX flight tracks in 1992-1998, and for the North Atlantic as a whole, show the SONEX meteorological environment to be representative of the North Atlantic flight corridor in the October-November period.

Thompson, A.↗

Formaldehyde Distribution over North America: Implications for Satellite Retrievals of Formaldehyde Columns and Isoprene Emission

Formaldehyde (HCHO) columns measured from space provide constraints on emissions of volatile organic compounds (VOCs). Quantitative interpretation requires characterization of errors in HCHO column retrievals and relating these columns to VOC emissions. Retrieval error is mainly in the air mass factor (AMF) which relates fitted backscattered radiances to vertical columns and requires external information on HCHO, aerosols, and clouds. Here we use aircraft data collected over North America and the Atlantic to determine the local relationships between HCHO columns and VOC emissions, calculate AMFs for HCHO retrievals, assess the errors in deriving AMFs with a chemical transport model (GEOS-Chem), and draw conclusions regarding space-based mapping of VOC emissions. We show that isoprene drives observed HCHO column variability over North America; HCHO column data from space can thus be used effectively as a proxy for isoprene emission. From observed HCHO and isoprene profiles we find an HCHO molar yield from isoprene oxidation of 1.6 +/- 0.5, consistent with current chemical mechanisms. Clouds are the primary error source in the AMF calculation; errors in the HCHO vertical profile and aerosols have comparatively little effect. The mean bias and 1Q uncertainty in the GEOS-Chem AMF calculation increase from <1% and 15% for clear skies to 17% and 24% for half-cloudy scenes. With fitting errors, this gives an overall 1 Q error in HCHO satellite measurements of 25-31%. Retrieval errors, combined with uncertainties in the HCHO yield from isoprene oxidation, result in a 40% (1sigma) error in inferring isoprene emissions from HCHO satellite measurements.

Millet, Dylan B.↗

A numerical framework for simulating the atmospheric variability of supermicron marine biogenic ice nucleating particles

Abstract. We present a framework for estimating concentrations of episodically elevated high-temperature marine ice nucleating particles (INPs) in the sea surface microlayer and their subsequent emission into the atmospheric boundary layer. These episodic INPs have been observed in multiple ship-based and coastal field campaigns, but the processes controlling their ocean concentrations and transfer to the atmosphere are not yet fully understood. We use a combination of empirical constraints and simulation outputs from an Earth system model to explore different hypotheses for explaining the variability of INP concentrations, and the occurrence of episodic INPs, in the marine atmosphere. In our calculations, we examine the following two proposed oceanic sources of high-temperature INPs: heterotrophic bacteria and marine biopolymer aggregates (MBPAs). Furthermore, we assume that the emission of these INPs is determined by the production of supermicron sea spray aerosol formed from jet drops, with an entrainment probability that is described by Poisson statistics. The concentration of jet drops is derived from the number concentration of supermicron sea spray aerosol calculated from model runs. We then derive the resulting number concentrations of marine high-temperature INPs (at 253 K) in the atmospheric boundary layer and compare their variability to atmospheric observations of INP variability. Specifically, we compare against concentrations of episodically occurring high-temperature INPs observed during field campaigns in the Southern Ocean, the Equatorial Pacific, and the North Atlantic. In this case study, we evaluate our framework at 253 K because reliable observational data at this temperature are available across three different ocean regions, but suitable data are sparse at higher temperatures. We find that heterotrophic bacteria and MBPAs acting as INPs provide only a partial explanation for the observed high INP concentrations. We note, however, that there are still substantial knowledge gaps, particularly concerning the identity of the oceanic INPs contributing most frequently to episodic high-temperature INPs, their specific ice nucleation activity, and the enrichment of their concentrations during the sea–air transfer process. Therefore, targeted measurements investigating the composition of these marine INPs and drivers for their emissions are needed, ideally in combination with modeling studies focused on the potential cloud impacts of these high-temperature INPs.

54 ENVIRONMENTAL SCIENCES↗

Atmospheric Radiation Measurement (ARM) airborne field campaign data products between 2013 and 2018

Airborne measurements are pivotal for providing detailed, spatiotemporally resolved information about atmospheric parameters and aerosol and cloud properties, thereby enhancing our understanding of dynamic atmospheric processes. For 30 years, the US Department of Energy (DOE) Office of Science supported an instrumented Gulfstream 1 (G-1) aircraft for atmospheric field campaigns. Data from the final decade of G-1 operations were archived by the Atmospheric Radiation Measurement (ARM) Data Center and made publicly available at no cost to all registered users. To ensure a consistent data format and to improve the accessibility of the ARM airborne data, an integrated dataset was recently developed covering the final 6 years of G-1 operations (2013 to 2018, https://doi.org/10.5439/1999133; Mei and Gaustad, 2024). The integrated dataset includes data collected from 236 flights (766.4 h), which covered the Arctic, the US Southern Great Plains (SGP), the US West Coast, the eastern North Atlantic (ENA), the Amazon Basin in Brazil, and the Sierras de Córdoba range in Argentina. These comprehensive data streams provide much-needed insight into spatiotemporal variability in the thermodynamic quantities and aerosol and cloud properties for addressing essential science questions in Earth system process studies. This paper describes the DOE ARM merged G-1 datasets, including information on the acquisition, data collection challenges and future potentials, and quality control processes. It further illustrates the usage of this merged dataset to evaluate the Energy Exascale Earth System Model (E3SM) with the Earth System Model Aerosol–Cloud Diagnostics (ESMAC Diags) package.

54 ENVIRONMENTAL SCIENCES↗

Volcanic Imprints in Last-Millennium Land Summer Temperatures in the Circum-North Atlantic Area

Summer cooling is one of the most direct consequences of explosive volcanic eruptions that can affect ecosystems and human societies. Recent studies revealed a multiyear cooling impact on hemispheric and global summer temperatures after tropical eruptions, yet the volcanic responses appear to vary on regional scales. Here, in this work, we revisit volcano-induced summer cooling in eastern Canada and northern and central Europe by applying superposed epoch analysis on CMIP6-PMIP4 simulations and millennial temperature reconstructions based on tree-ring density. We then examine potential causes modulating region-specific volcanic impact. While confirming that, on average, tropical eruptions over the last millennium have induced a longer cooling (>4 yr) than eruptions from extratropical Northern Hemisphere in all three North Atlantic regions, we show that the peak magnitude of cooling is stronger in eastern Canada. We also find that the detected volcanic temperature anomalies can be strongly affected by the selection and number of volcanic events and nonvolcanic signals embedded in the climate time series. This study highlights the risks of using highly noisy proxy records to investigate volcanic impacts, especially in regions with strong unforced climate variability. The CMIP6-PMIP4 simulations generally agree with the three reconstructions on the average response to tropical eruptions, but their performance is poorer regarding the production of significant cooling after extratropical eruptions. Our results further suggest that the particular sensitivity to tropical eruptions in eastern Canada is likely related to increased sea ice surrounding Quebec–Labrador associated with the positive Arctic Oscillation and North Atlantic Oscillation formed during the first posteruption winter.

54 ENVIRONMENTAL SCIENCES↗