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At least 199 records · Page 11

Neutron capture time scale of the s-process, estimated from s-process krypton in a meteorite

A krypton fraction enriched in s-process isotopes was extracted from a mineral fraction of the Murchison C2 chondrite. The (Kr-86)/(Kr-84) ratio is enhanced by 6 standard deviations, showing that significant amounts of Kr-86 were made in the s-process, despite the short, 10.8 yr beta-decay half-life of its precursor, Kr-85. Judging from this sample, the mean neutron capture time in the s-process was on the order of 5-100 yr for nuclei with cross sections of 125 mb.

Matsuda, J.-I.↗

Hafnium isotope variations in oceanic basalts

Hafnium isotope ratios generated by the beta(-) decay of Lu-176 are investigated in volcanic rocks derived from the suboceanic mantle. Hf-176/Hf-177 and Lu/Hf ratios were determined to precisions of 0.01-0.04% and 0.5%, respectively, by routine, low-blank chemistry. The Hf-176/Hf-177 ratio is found to be positively correlated with the Nd-143/Nd-144 ratio and negatively correlated with the Sr-87/Sr-86 and Pb-206/Pb-204 ratios, and to increase southwards along the Iceland-Reykjanes ridge traverse. An approximate bulk earth Hf-176/Hf-177 ratio of 0.28295 is inferred from the bulk earth Nd-143/Nd-144 ratio, which requires a bulk earth Lu/Hf ratio of 0.25, similar to the Juvinas eucrite. Midocean ridge basalts are shown to account for 60% of the range of Hf isotope ratios, and it is suggested that Lu-Hf fractionation is decoupled from Sm-Nd and Rb-Sr fractionation in very trace-element-depleted source regions as a result of partial melting.

Patchett, P. J.↗

Investigations of electron helicity in optically active molecules using polarized beams of electrons and positrons

A positronium-formation experiment with a high sensitivity to a possible relation between the helicity of beta particles emitted in nuclear beta decay and the optical asymmetry of biological molecules is presented. The experiment is based on a mechanism in which the electrons in optically active molecules possess a helicity of less than 0.001, too weak to detect in radiolysis experiments, the sign of which depends on the chirality of the isomer. A helicity-dependent asymmetry is sought in the formation of the triplet ground state of positronium when a low-energy beam of polarized positrons of reversible helicity interacts with an optically active substance coating a channel electron multiplier. Asymmetries between positronium decays observed at positive and negative helicities for the same substance can thus be determined with a sensitivity of 0.0001, which represents a factor of 100 improvement over previous positronium experiments.

Gidley, D. W.↗

The elements just beyond iron - Formation during explosive carbon burning

It is pointed out that the details of the synthesis of the elements just beyond iron are unclear. Thus, a reexamination of the role played by neutron-capture reactions during explosive carbon burning is indicated. A description is given of calculations of explosive carbon-burning nucleosynthesis using a complete neutron capture (n-process) computer code with a network extending from Cr through Zr and including not only (n,gamma), (gamma,n) reactions and beta-decay but also (p,n), (n,p), (p,gamma), and (p,alpha) reactions. Initial conditions indicative of the composition of a massive star following core helium burning were selected, and a comparison is made with conditions similar to those used by Howard et al. (1972). It is found that neutron reactions during explosive carbon burning are an important source for the elements just beyond iron.

Wefel, J. P.↗

Dielectric surface discharges: Effects of combined low-energy and high-energy incident electrons

Dielectric surface discharges affected by the addition of high energy electrons at 5 pA/sq cm to a primary 20 keV, 10 nA/sq cm electron beam with the high energy broad spectrum particles coming from the beta decay of Strontium 90 are studied. Kapton exhibits significantly increased discharge strength, increased waiting time between discharges, and a decreased number of discharges per specimen before discharge cessation. Mylar exhibits similar but less pronounced effects, while Teflon is relatively unaffected. With Kapton and Mylar, the high energy electrons act in some way to delay the instant of discharge ignition so that more charge can be accumulated and hence released during discharge.

Balmain, K. G.↗

Search for effect of longitudinally polarized protons on optically active amino acids

The influence of irradiation by longitudinally polarized protons on the differential decomposition of amino acid is investigated in a test of the Vester Ulbricht hypothesis that L-amino acids were produced in preference to the D isomers on the primitive earth due to the effects of parity violation in beta decay. Samples of DL-leucine were irradiated with protons of both positive and negative longitudinal polarization, then analyzed by gas chromatography. Despite advantages of higher polarization, lower velocity and higher ionization density of protons with respect to electrons, proton irradation is found to lead to no detectable asymmetries in DL-leucine degradation, even at 50% gross degradation.

Lemmon, R. M.↗

A new experiment to investigate the origin of optical activity using a low energy positron beam of controlled helicity

Previous experiments undertaken in search of a correlation between the origin of optical activity in biological molecules and the helicity of beta particles emitted in nuclear beta decay have not provided any useful results. A description is presented of an experiment in which a low energy polarized positron beam of controlled helicity interacts with an optically active material to form positronium in vacuum. Advantages of the current study compared to the previous experiments are mainly related to a much greater sensitivity. Initially, it will be possible to detect a helicity-dependent asymmetry in triplet positronium formation of 1 part in 10,000. Improvements to better than 1 part in 100,000 should be attainable.

Gidley, D. W.↗

Calculation of a mirror asymmetric effect in electron scattering from chiral targets

A dynamical calculation is presented of the helicity induced in an initially unpolarized electron beam after elastic scattering from an optically active medium, a process analogous to the circular polarization induced in unpolarized light following Rayleigh scattering from chiral targets. The calculation is based on the bound helical electron model of a chiral molecule, according to which the major contribution to the helicity is provided by the perturbation of the electron bound state by the spin-orbit interaction of the bound electrons moving in the electric field of the molecular core. The net helicity acquired is found to depend directly on a molecular asymmetry factor and the square of the atomic number of the heaviest atom in an asymmetric environment. For the case of carbon, the induced helicity is on the order of 0.00001, which would account for its lack of observation in a recent experiment. Results may have implications for the origin of optical activity in biological molecules by the differential ionization of D and L isomers by beta-decay electrons.

Rich, A.↗

Dielectric surface discharges - Effects of combined low-energy and high-energy incident electrons

Dielectric surface discharges affected by the addition of high energy electrons at 5 pA/sq cm to a primary 20 keV, 10 nA/sq cm electron beam with the high energy broad spectrum particles coming from the beta decay of Strontium 90 are studied. Kapton exhibits significantly increased discharge strength, increased waiting time between discharges, and a decreased number of discharges per specimen before discharge cessation. Mylar exhibits similar but less pronounced effects, while Teflon is relatively unaffected. With Kapton and Mylar, the high energy electrons act in some way to delay the instant of discharge ignition so that more charge can be accumulated and hence released during discharge. Previously announced in STAR as N82-14222

Balmain, K. G.↗

Segmentation and pulse shape discrimination techniques for rejecting background in germanium detectors

The possibility of rejecting the internal beta-decay background in coaxial germanium detectors by distinguishing between the multi-site energy losses characteristic of photons and the single-site energy losses of electrons in the range 0.2 - 2 MeV is examined. The photon transport was modeled with a Monte Carlo routine. Background rejection by both multiple segmentation and pulse shape discrimination techniques is investigated. The efficiency of a six 1 cm-thick segment coaxial detector operating in coincidence mode alone is compared to that of a two-segment (1 cm and 5 cm) detector employing both front-rear coincidence and PSD in the rear segment to isolate photon events. Both techniques can provide at least 95 percent rejection of single-site events while accepting at least 80 percent of the multi-site events above 500 keV.

Roth, J.↗

Instrumental background in balloon-borne gamma-ray spectrometers and techniques for its reduction

Instrumental background in balloon-borne gamma-ray spectrometers is presented. The calculations are based on newly available interaction cross sections and new analytic techniques, and are the most detailed and accurate published to date. Results compare well with measurements made in the 20 keV to 10 MeV energy range by the Goddard Low Energy Gamma-ray Spectrometer (LEGS). The principal components of the continuum background in spectrometers with GE detectors and thick active shields are: (1) elastic neutron scattering of atmospheric neutrons on the Ge nuclei; (2) aperture flux of atmospheric and cosmic gamma rays; (3) beta decays of unstable nuclides produced by nuclear interactions of atmospheric protons and neutrons with Ge nuclei; and (4) shield leakage of atmospheric gamma rays. The improved understanding of these components leads to several recommended techniques for reducing the background.

Gehrels, N.↗

Background events in microchannel plates

Measurements have been made to assess the characteristics and origins of background events in microchannel plates (MCPs). An overall background rate of about 0.4 events/sq cm persec has been achieved consistently for MCPs that have been baked and scrubbed. The temperature and gain of the MCPs are found to have no significant effect on the background rate. Detection of 1.46-MeV gamma rays from the MCP glass confirms the presence of K-40, with a concentration of 0.0007 percent, in MCP glass. It is shown that beta decay from K-40 is sufficient to cause the background rate and spectrum observed. Anticoincidence measurements indicate the the background rate caused by cosmic ray interactions is small (less than 0.016 events/sq cm per sec).

Siegmund, O. H. W.↗

The even-odd systematics in R-process nuclide abundances

The paper reports and discusses solar system N(R) abundances for nuclides A greater than 70, obtained as differences between measured solar system abundances and calculated S-process contributions. The abundance peak at A of about 163 in the rare earth element region reveals properties which are similar to those of the R-process peaks corresponding to magic neutron numbers N = 82 and N = 126. Systematic differences in the N(R) abundances of even-A and odd-A nuclides are restricted to specific mass regions. It is concluded that these differences are most probably related to the properties of nuclear species during beta(-) decay to the stability valley.

Marti, K.↗

The cross section for p + p - d + e(+) + nu(e)

The cross section for the fundamental proton-proton fusion process has been reevaluated, employing more accurate parameters such as the deuteron wave function and the weak-interaction coupling constant (from the neutron beta-decay). Small corrections have been computed, such as the effects of vacuum polarization on barrier penetration and the radiative corrections to the process; these two effects almost cancel. The cross section is larger than that computed in previous work. The effect on the expected flux of neutrinos from B-8 decay is a reduction by a factor of 0.92, narrowing the gap between theory and experiment in the solar neutrino problem.

Gould, Robert J.↗

Isotopically enriched germanium detectors for astrophysical gamma-ray spectroscopy

A study is presented of the instrumental background in astrophysical gamma-ray spectrometers using isotopically enriched germanium detectors. Calculations show that the beta-decay background, which is the largest component between approximately 0.1 and 1.0 MeV in balloonborne and satellite spectrometers, is dominated by the activation of Ge-74. This component can be reduced by an order of magnitude using detectors enriched to more than 80 percent in (Ge-70). The predicted reduction in the total background for current balloonborne instruments is more than a factor of 1.7 between 0.2 and 1.0 MeV. For future satellite instruments, the reduction in this energy range is by more than a factor of 5.

Gehrels, Neil↗

Gallium phosphide energy converters

Gallium phosphide (GaP) energy converters may be successfully deployed to provide new mission capabilities for spacecraft. Betavoltaic power supplies based on the conversion of tritium beta decay to electricity using GaP energy converters can supply long term low-level power with high reliability. High temperature solar cells, also based on GaP, can be used in inward-bound missions greatly reducing the need for thermal dissipation. Results are presented for GaP direct conversion devices powered by Ni-63 and compared to the conversion of light emitted by tritiarated phosphors. Leakage currents as low as 1.2 x 10(exp -17) A/sq cm have been measured and the temperature dependence of the reverse saturation current is found to have ideal behavior. Temperature dependent IV, QE, R(sub sh), and V(sub oc) results are also presented. These data are used to predict the high-temperature solar cell and betacell performance of GaP devices and suggest appropriate applications for the deployment of this technology.

Sims, P. E.↗

Lunar and Planetary Surface Dynamics and Early History

This document, submitted as part of this proposal renewal represents the Final Report required by NASA for Grant NAGS-9442. It should be emphasized that, while this work statement in the original proposal outlined anticipated directions of our research, the specific activities we carried out during this period differed slightly from those proposed, capitalizing on new unexpected results and new advances in analytical capability. The thrust of all the work we completed were completely within the stated research goals of the proposal and significantly advanced our knowledge of planetary processes and our understanding of the early solar system. The following summary outlines our achievements in the different areas of research. These include: A) Early solar system processes and time scales using I-Xe chronometry; B) The Active Capture of Volatiles: A new mechanism for the capture of heavy noble gases, possible implications for phase Q and planetary heavy noble gases; C) Separation of Xe-L from Xe-H: Physically selective experiments; D) Abundances of Presolar grains; E) Studies of Neon and Helium from single interstellar SiC and graphite grains; F) Pre-compaction exposure of meteoritic grains and chondrules; G) Geochemically Measured Half-Lives: Double beta-decay of Te and Ba isotopes; H) Noble gases in stratospheric interplanetary dust particles; I) New Analytical Instrument.

Source record↗

Saturn Neutron Exosphere as Source for Inner and Innermost Radiation Belts

Energetic proton and electron measurements by the ongoing Cassini orbiter mission are expanding our knowledge of the highest energy components of the Saturn magnetosphere in the inner radiation belt region after the initial discoveries of these belts by the Pioneer 11 and Voyager 2 missions. Saturn has a neutron exosphere that extends throughout the magnetosphere from the cosmic ray albedo neutron source at the planetary main rings and atmosphere. The neutrons emitted from these sources at energies respectively above 4 and 8 eV escape the Saturn system, while those at lower energies are gravitationally bound. The neutrons undergo beta decay in average times of about 1000 seconds to provide distributed sources of protons and electrons throughout Saturn's magnetosphere with highest injection rates close to the Saturn and ring sources. The competing radiation belt source for energetic electrons is rapid inward diffusion and acceleration of electrons from the middle magnetosphere and beyond. Minimal losses during diffusive transport across the moon orbits, e.g. of Mimas and Enceladus, and local time asymmetries in electron intensity, suggest that drift resonance effects preferentially boost the diffusion rates of electrons from both sources. Energy dependences of longitudinal gradient-curvature drift speeds relative to the icy moons are likely responsible for hemispheric differences (e.g., Mimas, Tethys) in composition and thermal properties as at least partly produced by radiolytic processes. A continuing mystery is the similar radial profiles of lower energy (<10 MeV) protons in the inner belt region. Either the source of these lower energy protons is also neutron decay, but perhaps alternatively from atmospheric albedo, or else all protons from diverse distributed sources are similarly affected by losses at the moon' orbits, e.g. because the proton diffusion rates are extremely low. Enceladus cryovolcanism, and radiolytic processing elsewhere on the icy moon and ring surfaces, are additional sources of protons via ionization and charge exchange from breakup of water molecules. But one must then account somehow for local acceleration to the observed keV-MeV energies, since moon sweeping and E-ring absorption would remove protons diffusing inward from the middle magnetosphere. Although the main rings block further inward diffusion from the inner radiation belts, the exospheric neutron-decay source, combined with much slower diffusion of protons relative to electrons, may produce an innermost radiation belt in the gap between the upper atmosphere and the D-ring. This innermost belt will first be explored in-situ during the final proximal orbits of the Cassini mission.

Cooper, John↗