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Development of an Activation Analysis Methodology to Support the Disposal of the High Flux Isotope Reactor Metal Pool Waste

During operation and maintenance of the High Flux Isotope Reactor (HFIR), metal waste from reactor components is generated. Due to space limitations in the pool fuel storage, it is necessary to remove the waste and send it to off-site disposal. Most of this waste was in the reactor and is radioactive through neutron activation. Prior to shipping and disposal at a waste disposal facility, the radiological activity of the waste must be determined. Therefore, a conservative methodology to characterize the radiological activity of the waste must be performed. The methodology used was based on being able to determine a conservative overall activity and radionuclide inventory based on radiological survey data and neutron activation products for the materials present.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

International Collaboration Activities in Geologic Disposal Research: FY2021 Progress

This report describes the FY21 status of international collaboration regarding geologic disposal research in the Spent Fuel and Waste Disposition (SFWD) Campaign. Since 2012, in an effort coordinated by Lawrence Berkeley National Laboratory, SFWD has advanced active collaboration with several international geologic disposal programs across the world. Such collaboration has allowed the SFWD Campaign to benefit from a deep knowledge base in regards to alternative repository environments developed over decades and has provided a framework for active peer-to-peer research participation in international groups which conduct, analyze, and model performance-relevant processes. Via international collaboration, the SFWD Campaign also benefits from substantial international investments in research facilities (such as underground research laboratory testing and modeling) and achieves cost savings via joint funding of expensive field experiments. To date, SFWD’s International Disposal R&D Program has established formal collaboration agreements with multiple international initiatives and various international partners, and national lab scientists associated with SFWD have conducted a large number of specific collaborative R&D activities that align well with its R&D priorities.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Performance Assessment for the E-Area Low Level Radioactive Waste Disposal Facility at the Savannah River Site: Chapter 1

This report documents the revised Performance Assessment (PA) analysis for the E-Area Low-Level Waste Facility (ELLWF) at the United States (U.S.) Department of Energy (DOE) Savannah River Site (SRS). A PA analysis is required for DOE-operated facilities that dispose of low-level radioactive waste. PA analyses simulate (1) the release of radionuclides from the disposal site after facility closure, (2) transport of those contaminants through the environment, and (3) exposure/impacts to potential receptors. The purpose of the PA analysis is to demonstrate that the facility is operated in a manner that ensures long-term environmental protection after facility closure, thereby providing for the protection of public health and safety in limiting doses to a hypothetical member of the public (MOP) or an inadvertent human intruder (IHI). DOE Manual (M) 435.1-1, Chg. 3, Radioactive Waste Management (U.S. DOE, 2021b) establishes quantitative post-closure environmental impact limits and requires a facility-specific PA analysis to demonstrate compliance with these limits for DOE low-level waste (LLW) disposed of after September 26, 1988. These limits are defined in terms of human health (e.g., dose limits) with respect to radioactive constituents in the waste.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Performance Assessment for the E-Area Low-Level Radioactive Waste Disposal Facility at the Savannah River Site: Appendix F

As a supplement to Chapter 6, Section 6.1.1.3, Table F-1 through Table F-24 provide tabular results of the sensitivity analysis calculations for waste disposal timing (Sensitivity Case S6) in NR07E (Cases 3 and 4) and NR26E (Cases 1 through 4). The title of each table identifies the DU, sensitivity case, and performance measure. Section F.1.1 (Table F-1 through Table F-8) presents results for NR07E and Section F.1.2 (Table F-9 through Table F-24) presents results for NR26E. In each table, radionuclides are sorted from highest to lowest nominal concentration or dose factor. Nominal values are when waste disposal occurs at the start of operations; timeline values are when waste disposal occurs at the end of operations. The differences (Δ values) in the last column of each table equal the timeline concentration or dose factor minus the nominal concentration or dose factor, where DF and CF are shorthand designations for dose factor and concentration factor, respectively.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Performance Assessment for the Disposal of Low-Level Waste in the 200 East Area Burial Grounds (Annual Summary Report - FY 23)

This annual review provides the projected dose estimates of radionuclide inventories disposed in the 200 East Area Low-Level Waste Burial Grounds (LLBGs) since September 26, 1988. All trenches in these burial grounds except one have remained inactive since 2005. Trench 94 located in 218-E-12B Burial Ground is the only active trench that is dedicated for disposal of U.S. Navy reactor compartments. During this reporting period (fiscal year 2023, from October 1, 2022, through September 30, 2023), no reactor compartments were disposed in Trench 94.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Annual Summary Report (FY 2025) Performance Assessment for the Disposal of Low-Level Waste in the 200 East Area Burial Grounds

This annual review provides the projected dose estimates of radionuclide inventories disposed in the 200 East Area Low Level Burial Grounds (LLBGs) since September 26, 1988. All trenches in these burial grounds except one have remained inactive since July 2004. Trench 94 located in 218-E-12B Burial Ground is the only active trench, which is dedicated for disposal of U.S. Navy reactor compartments. During this reporting period (fiscal year 2025, from October 1, 2024, through September 30, 2025), two reactor compartments were disposed in Trench 94.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Monitoring Plan for the Idaho National Laboratory Remote Handled Low Level Waste Disposal Facility

This monitoring plan for Idaho National Laboratory’s Remote-Handled Low Level Waste Disposal Facility was developed to meet the requirements for monitoring low-level waste disposal facilities according to the U.S. Department of Energy (DOE) Order 435.1, “Radioactive Waste Management,” and the guidance provided in the associated technical standard “Disposal Authorization Statement and Tank Closure Documentation” (DOE-STD-5002-2017). The purpose of this monitoring plan is to document a monitoring strategy that includes (1) compliance monitoring activities to demonstrate compliance with regulatory standards/limits and (2) performance monitoring to build confidence the facility is performing as demonstrated in the facility performance assessment (PA) (DOE-ID 2018a), composite analysis (CA) (DOE ID 2012), and CA addendum (DOE-ID 2018b). The de minimus impact to the aquifer predicted by the PA suggests that aquifer compliance monitoring should be augmented with performance monitoring of the drainage course materials and sedimentary interbeds in the vadose zone beneath the facility to provide a more effective means of identifying performance deviations. The monitoring approach delineated in this document was informed by the systems evaluation of natural and engineered facility features presented in the PA, an assessment of aquifer baseline conditions (INL 2017d), the dose analysis conducted in support of the PA and CA, and monitoring data collected during the first four years of facility operations (baseline monitoring phase) (INL 2023b). This plan provides monitoring locations, sampling frequencies, and sampling methods; recommendations for data evaluation; and a description of the monitoring plan implementation. Collected data will be used to demonstrate facility compliance and to identify conditions that are not consistent with the key assumptions made by the PA and CA.

12 - MGMT OF RADIOACTIVE AND NON-RADIOACTIVE WASTE↗

Perspective Chapter: Safe Disposal and Storage of Nuclear Waste

The use of nuclear energy inevitably generates nuclear waste as the byproduct of fission reactions. Depending on the initial composition of the fuel that goes into the reactor and the subsequent burn-up level, the chemistry of the resulting nuclear waste can vary substantially. This waste typically exhibits a broad spectrum of radioactivity and half-lives, making effective management one of the most critical challenges for global nuclear energy. This chapter provides a comprehensive overview of the origin and classification of nuclear waste and various strategies for its safe immobilization and disposal. The short- and long-term storage of waste with varying radioactivity is addressed. The significant technical and political complexities involving primarily long-term disposal are also discussed. To ensure the safe and permanent disposal of hazardous waste with extremely long half-lives, future efforts should focus on both technical innovation and public engagement.

36 MATERIALS SCIENCE↗

Monitoring the dispersion of ocean waste disposal plumes from ERTS-1 and Skylab

The author has identified the following significant results. About forty miles off the Delaware coast is located the disposal site for waste discharged from a plant processing titanium dioxide. The discharge is a greenish-brown; 15-20% acid liquid which consists primarily of iron chlorides and sulfates. The barge which transports this waste has a 1,000,000 gallon capacity and makes approximately three trips to the disposal site per week. ERTS-1 MSS digital tapes are being used to study the dispersion patterns and drift velocities of the iron-acid plume. Careful examination of ERTS-1 imagery disclosed a fishhook-shaped plume about 40 miles east of Cape Henlopen caused by a barge disposing acid wastes. The plume shows up more strongly in the green band than in the red band. Since some acids have a strong green component during dumping and turn slowly more brownish-reddish with age, the ratio of radiance signatures between the green and red bands may give an indication of how long before the satellite overpass the acid was dumped. Enlarged enhancements of the acid waste plumes, prepared from the ERTS-1 MSS digital tapes aided considerably in studies of the dispersion of the waste plume. Currently acid dumps are being coordinated with ERTS-1 overpasses.

Klemas, V.↗

Summary of the study of disposal of nuclear waste into space

NASA, at the request of the AEC, is conducting a preliminary study to determine the feasibility of disposing of nuclear waste material into space. The study has indicated that the Space Shuttle together with expendable and nonexpendable orbital stages such as the Space Tug or Centaur can safety dispose of waste material by ejecting it from the solar system. The safety problems associated with all phases of launching and operation (normal, emergency and accident) of such a system are being examined. From the preliminary study it appears that solutions can be found that should make the risks acceptable when compared to the benefits to be obtained from the disposal of the nuclear waste.

Rom, F. E.↗

Space disposal of nuclear wastes. Volume 1: Socio-political aspects

The history and interpretation of radioactive waste management in the U.S., criteria for choosing from various options for waste disposal, and the impact of nuclear power growth from 1975 to 2000 are discussed. Preconditions for the existence of high level wastes in a form suitable for space disposal are explored. The role of the NASA space shuttle program in the space disposal of nuclear wastes, and the impact on program management, resources and regulation are examined.

Laporte, T.↗

Earth reencounter probabilities for aborted space disposal of hazardous nuclear waste

A quantitative assessment is made of the long-term risk of earth reencounter and reentry associated with aborted disposal of hazardous material in the space environment. Numerical results are presented for 10 candidate disposal options covering a broad spectrum of disposal destinations and deployment propulsion systems. Based on representative models of system failure, the probability that a single payload will return and collide with earth within a period of 250,000 years is found to lie in the range .0002-.006. Proportionately smaller risk attaches to shorter time intervals. Risk-critical factors related to trajectory geometry and system reliability are identified as possible mechanisms of hazard reduction.

Friedlander, A. L.↗

Space augmentation of military high-level waste disposal

Space disposal of selected components of military high-level waste (HLW) is considered. This disposal option offers the promise of eliminating the long-lived radionuclides in military HLW from the earth. A space mission which meets the dual requirements of long-term orbital stability and a maximum of one space shuttle launch per week over a period of 20-40 years, is a heliocentric orbit about halfway between the orbits of earth and Venus. Space disposal of high-level radioactive waste is characterized by long-term predictability and short-term uncertainties which must be reduced to acceptably low levels. For example, failure of either the Orbit Transfer Vehicle after leaving low earth orbit, or the storable propellant stage failure at perihelion would leave the nuclear waste package in an unplanned and potentially unstable orbit. Since potential earth reencounter and subsequent burn-up in the earth's atmosphere is unacceptable, a deep space rendezvous, docking, and retrieval capability must be developed.

English, T.↗

SPS salvage and disposal alternatives

A wide range of salvage options exist for the satellite power system (SPS) satellite, ranging from use in and beyond geosynchronous orbit to use in low Earth orbit to return and use on Earth. The satellite might be used intact to provide for various purposes, it might be cannibalized, or it might be melted down to supply materials for space- or ground-based products. The use of SPS beyond its nominal lifetime provides value that can be deducted from the SPS capital investment cost. It is shown that the present value of the salvage value of the SPS satellites, referenced to the system initial operation data, is likely to be on the order of five to ten percent of its on-orbit capital cost. (Given a 30 year satellite lifetime and a four percent discount rate, the theoretical maximum salvage value is 30.8 percent of the initial capital cost). The SPS demonstration satellite is available some 30 years earlier than the first full-scale SPS satellite and has a likely salvage value on the order of 80 percent of its on site capital cost. In the event that it becomes desirable to dispose of either the demonstration or full-scale SPS satellite, a number of disposal options appear to exist for which intact disposal costs are less than one percent of capital costs.

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Satellite power system salvage and disposal alternatives

A wide range of salvage options for the SPS satellite, ranging from use in and beyond geosynchronous orbit to use in low Earth orbit in return and use on Earth are presented. The satellite can be used intact to provide power for various purposes, it can be cannibalized or it can be melted down to supply materials for space or ground based products. The use of SPS beyond its nominal lifetime provides value that can be deducted from the SPS capital investment cost. The present value of the salvage value of the SPS satellites, referenced to the system initial operation data, is on the order of five to ten percent of its on-orbit capital cost. (Given a 30 year satellite lifetime and a four percent discount rate, the theoretical maximum salvage value is 30.8 percent of the capital cost.) The SPS demonstration satellite is available some 30 years earlier than the first full scale SPS satellite and has a salvage value on the order of 80 percent of its on-orbit capital cost. In the event that it becomes desirable to dispose of either the demonstration of full scale SPS satellite, a number of disposal options is presented for which intact disposal costs are less than one percent of capital costs.

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U.S. program assessing nuclear waste disposal in space - A status report

Various concepts for the space disposal of nuclear waste are discussed, with attention given to the destinations now being considered (high earth orbit, lunar orbit, lunar surface, solar orbit, solar system escape, sun). Waste mixes are considered in the context of the 'Purex' (Plutonium and Uranium extraction) process and the potential forms for nuclear waste disposal (ORNL cermet, Boro-silicate glass, Metal matrix, Hot-pressed supercalcine) are described. Preliminary estimates of the energy required and the cost surcharge needed to support the space disposal of nuclear waste are presented (8 metric tons/year, requiring three Shuttle launches). When Purex is employed, the generated electrical energy needed to support the Shuttle launches is shown to be less than 1%, and the projected surcharge to electrical users is shown to be slightly more than two mills/kW-hour.

Rice, E. E.↗

Analysis of space systems for the space disposal of nuclear waste follow-on study. Volume 1: Executive summary

The impact on space systems of three alternative waste mixes was evaluated as part of an effort to investigate the disposal of certain high-level nuclear wastes in space as a complement to mined geologic repositories. A brief overview of the study background, objectives, scope, approach and guidelines, and limitations is presented. The effects of variations in waste mixes on space system concepts were studied in order to provide data for determining relative total system risk benefits resulting from space disposal of the alternative waste mixes. Overall objectives of the NASA-DOE sustaining-level study program are to investigate space disposal concepts which can provide information to support future nuclear waste terminal storage programmatic decisions and to maintain a low level of research activity in this area to provide a baseline for future development should a decision be made to increase the emphasis on this option.

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