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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 199 records · Page 11

Current collection in a magnetoplasma

The authors present a survey of a very incomplete subject, current collection in a magnetoplasma. The best-developed and simplest theories for current collection are steady-state collisionless theories, and these must be understood before departures from them can be analyzed usefully. Thus, the authors begin with a review of them. The authors include some recent numerical results which indicate that steady-state collisionless Laplace-limit currents remain substantially below the Parker-Murphy (1967) canonical upper bound out to very large electrode potentials, and approach it as a limit only very slowly if at all. Attempts to correct this theory for space-charge effects lead to potential disturbances which extend to infinite distance along the electrode's magnetic shadow, unless collisional effects are also taken into account. However, even a small amount of relative plasma drift motion, such as that involved in a typical rocket experiment, can change this conclusion fundamentally. It is widely believed that time-averaged current collection may be increased by effects of plasma turbulence, and the authors review the available evidence for and against this contention. Steady-state collisionless particle dynamics predicts the existence of a toroidal region of trapped orbits which surrounds the electrode. Light emissions from this region have been photographed, indicating that collisional ionization may also occur there, and this, and/or scattering by collisions or possibly turbulent fluctuations in this region, may also increase current collection by the electrode. The authors also discuss effects on particle motions near the electrode, associated with breakdown of magnetic insulation in the region of large electric fields near it.

Laframboise, Jim G.↗

The Flux and Energy Spectra of the Protons in the Inner Van Allen Belt

A cylindrical stack of G-5 nuclear emulsions housed in the payload section of a four-stage research rocket was flown into the northern edge of the inner Van Allen belt on September 19, 1960. The experimental design permitted, for the first time, measurements of the particle fluxes and energy spectra as functions of position along the rocket trajectory. Eight points along the trajectory have been selected for analysis. Results are presented herein for three of these points, and they are discussed in the light of various theories on the trapped radiation.

Naugle, John E.↗

Unique optical excitations in topological insulators (Final Technical Report)

The overall objective of this research is to understand how light interacts with topological insulator (TI) films and layered structures. Unlike normal materials, the electrons in TI films are trapped at the top and bottom surfaces of the film. These electrons have unusual properties, including low mass and high velocity. Light shining on these trapped electrons will excite electron density waves, called plasmons, which inherit the unusual properties of the electrons. This project aims to understand how these plasmons interact with each other and how the plasmon properties change as the film dimensions change. By controlling the physical properties of the films, the optical response of the film can also be controlled. In addition to single TI films, the project will also investigate the properties of stacks of TI films layered with normal insulating films. Stacking these materials results in multiple layers of trapped electrons whose plasmons can interact in ever more complex ways. After these interactions are understood, we can begin to engineer complex TI structures to obtain designer optical phenomena in the far-infrared and THz, wavelength ranges of interest for environmental monitoring and chemical sensing. This research directly addresses DOE Grand Challenges, including understanding how properties of matter emerge from complex electronic correlations and learning how to control these properties as well as the mission of the Basic Energy Sciences program to understand and control matter at the electronic/atomic level.

36 MATERIALS SCIENCE↗

Suppressing Polaronic Defect–Photocarrier Interaction in Halide Perovskites by Pre-distorting Its Lattice

In halide perovskites, photocarriers can have strong polaronic interactions with point defects. For iodide-deficient MAPbI 3 , we found that the Fermi level can shift significantly by 0.6–0.7 eV upon light illumination. This energy level shift is accompanied by the formation of deep electron traps. These experimental observations are consistent with the formation of a Pb–Pb dimer when photoexcited electrons are trapped at an iodide vacancy. Interestingly, we found that this polaronic interaction is suppressed when a portion of MA + cations is replaced by smaller Cs + ions. Density functional theory calculations reveal that Cs-doping can reduce the distance between two Pb atoms across an iodide vacancy, even without electron trapping. The predistortion of the lattice induced by cation replacement resembles the Pb–Pb dimer formed by electron trapping at the defect site, which explains the suppression of light-induced effects observed in the experiment. Furthermore, our finding unveils a counterintuitive strategy to enhance the photostability of halide perovskites by preintroducing distortions into its lattice.

14 SOLAR ENERGY↗

Spatial coherence of room-temperature monolayer WSe 2 exciton-polaritons in a trap

The emergence of spatial and temporal coherence of light emitted from solid-state systems is a fundamental phenomenon intrinsically aligned with the control of light-matter coupling. It is canonical for laser oscillation, emerges in the superradiance of collective emitters, and has been investigated in bosonic condensates of thermalized light, as well as exciton-polaritons. Our room temperature experiments show the strong light-matter coupling between microcavity photons and excitons in atomically thin WSe 2 . We evidence the density-dependent expansion of spatial and temporal coherence of the emitted light from the spatially confined system ground-state, which is accompanied by a threshold-like response of the emitted light intensity. Additionally, valley-physics is manifested in the presence of an external magnetic field, which allows us to manipulate K and K’ polaritons via the valley-Zeeman-effect. Our findings validate the potential of atomically thin crystals as versatile components of coherent light-sources, and in valleytronic applications at room temperature.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Photophysical properties of zero-dimensional perovskites studied by PBE0 and GW+BSE methods

Due to the exceptional photophysical properties and great potential applications in solid state lighting, zero-dimensional halide perovskites with broadband emitting have recently attracted much attention. In this work, to reveal the origin of the broadband absorption and emission spectra of 0D (C 4 N 2 H 14 Br) 4 SnBr x I 6-x (x = 3), the ground state and exciton dynamics properties have been studied by hybrid PBE0 functional and the GW+BSE method. Different self-trapped excitons (STEs) are obtained, and their emission energies by PBE0 are consistent well with experimental data. By considering the vibrational broadening of emission, our calculated full width at half maximum of emission accords well with the experiment. The absorption of free exciton and STEs is also calculated by considering the quasiparticle and excitonic effect. Our results show that these light-induced trapped states can be observed by experiments, as confirmed in other similar systems by the femtosecond transient absorption spectra.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Recent developments and proposed schemes for trapped ion frequency standards

Ion traps are exciting candidates as future precision frequency sources. Recent developments demonstrate that mercury ion frequency standards are capable of a stability performance comparable to commercial cesium standards. There is, however, considerable room for improvement with regard to the signal to noise problem. The 40 GHz microwave frequency implies that a careful design should be implemented to ensure the elimination of the unwanted side bands in the microwave pump signal. A long life, high performance light source to be used in a trapped mercury ion microwave standard must be developed and the long term performance of a trapped mercury ion microwave standard must be investigated. While newly proposed two photon pumping schemes in conjuction with mercury ions promise exciting developments for both microwave and optical frequency standards, other ions that may be potential candidates should be evaluated for their usefulness.

Maleki, L.↗

Optical Levitation of Micro-Scale Particles in Air

Success has been achieved using a radiation pressure gradient to levitate microscale particles in air for as long as four hours. This work is performed as a precursor to the development of a vacuum based optical tweezers interrogation tool for nanotechnology research. It was decided to first proceed with solving the problem of achieving optical levitation of a micro-scale particle in air before trying the same in a vacuum environment. This successful optical levitation in air confirms the work of Ashkin and Dziedzic. Levitation of 10 and 13.8 microns diameter polystyrene spheres was achieved, as well as the levitation of 10 and 100 microns diameter glass spheres. Particles were raised and lowered. A modicum of success was achieved translating particles horizontally. Trapping of multiple particles in one laser beam has been photographed. Also, it has been observed that particles, that may be conglomerates or irregular in shape, can also be trapped by a focused laser beam. Levitated glass beads were photographed using laser light scattered from the beads. The fact that there is evidence of optical traps in air containing irregular and conglomerate particles provides hope that future tool particles need not be perfect spheres.

Wrbanek, Susan Y.↗

Neural Network for Image-to-Image Control of Optical Tweezers

A method is discussed for using neural networks to control optical tweezers. Neural-net outputs are combined with scaling and tiling to generate 480 by 480-pixel control patterns for a spatial light modulator (SLM). The SLM can be combined in various ways with a microscope to create movable tweezers traps with controllable profiles. The neural nets are intended to respond to scattered light from carbon and silicon carbide nanotube sensors. The nanotube sensors are to be held by the traps for manipulation and calibration. Scaling and tiling allow the 100 by 100-pixel maximum resolution of the neural-net software to be applied in stages to exploit the full 480 by 480-pixel resolution of the SLM. One of these stages is intended to create sensitive null detectors for detecting variations in the scattered light from the nanotube sensors.

Decker, Arthur J.↗

Trapping and actively transporting single particles of arbitrary properties in low-pressure rf plasmas with and without a magnetic field

We report the experimental realization of optical trapping and controlled manipulations of single particles of arbitrary properties, e.g., nano- to micrometer in size, transparent spheres to strongly light absorbing nonspherical particles, in low-pressure rf plasmas. First, we show optical trapping and transport of single particles in an unmagnetized rf plasma. Then, we show similar observations in a weakly magnetized rf plasma. This is the first demonstration of actively transporting (pushing and pulling) light-absorbing, nonspherical single particles in plasmas. The result suggests that optically trapped, actively controlled, single plasma dust particles (not limited to those externally sampled spheres) could be an in situ micro-probe for dusty plasma and magnetized dusty plasma diagnostics.

Physics↗

Evaluation of the characteristics of a field emission cathode for use in a Mercury ion trap frequency standard

The performance is reported of a field emission array characterized for the purpose of replacing the filament in a trapped ion frequency standard. This dark electron emitter eliminates the need for the interference filter currently used in the trapped ion standard. While reducing the filament's unwanted light, this filter causes a significant reduction in the signal. The magnetic field associated with the filament is also eliminated, thus potentially improving the present stability of the trapped ion standard. The operation of the filament in the present system is described, as well as the associated concerns. The cathode considered for the filament's replacement is then described along with the experimental system. Experimental results, observations, and conclusions are presented.

Christman, J. M.↗

Study of perovskite CsPbBr 3 detector polarization and its mitigation with ultrahigh x-ray flux

High-flux capable semiconductor x-ray detectors are essential in various applications, but the detrimental effects of detector polarization limit their use in many cases. Here, for this work, we studied the polarization of perovskite CsPbBr 3 semiconductor detectors using ultrahigh flux synchrotron x rays (10 6 –10 12 photons s –1 mm –2 at 58.61 keV). The CsPbBr 3 detectors did not show immediate polarization prominently until a flux higher than 10 10 photons s –1 mm –2 . Using the pump-and-probe technique, we visualized the spatial and temporal effects of polarization. The polarized region, represented by reduced photocurrent, extended beyond the area under direct irradiation, and the reduced photocurrent persisted after potential de-polarization treatments. We found that stronger applied electric fields and fewer carrier traps can mitigate polarization, represented by less photocurrent deficit. By examining the detectors’ current response under controlled ambient light, low, and high-flux x rays, we studied the trap filling and release behavior of CsPbBr 3 . We discovered that the polarization is caused by partial detector damage due to deep defects generated by ultrahigh flux x-ray irradiation. Our work provides insight into CsPbBr 3 polarization under extremely intense x-ray radiation and shows that reducing crystal defects and increasing detector bias voltage are effective solutions.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Optical Tweezers and Optical Trapping Improved for Future Automated Micromanipulation and Characterization

Optical trap arrays are being developed at the NASA Glenn Research Center for holding, manipulating, and optically interrogating arrays of nanotube sensors. The trap arrays, for example, might be used to arrange arrays of chemical sensors for insertion onto a chip in liquid, air, and vacuum environments. Neural-network-controlled spatial light modulators (SLMs) are to generate and control the trap positions and trap profiles in three dimensions.

Wrbanek, Susan Y.↗

Detecting Cracks on Inner Surfaces

Microscopic cracks or flaws in surface of a workpiece are often detected with fluorescent dye. Dye is spread over surface to be inspected and then washed off. When piece is viewed under ultraviolet light, a glow is seen from dye trapped in any flaws. Intensity of fluorescence gives a rough indication of depth of defect. Fluorescent inspection procedure is fast, inexpensive and simple to perform.

Sax, A.↗

Effect of short wavelength illumination on the characteristic bulk diffusion length in ribbon silicon solar cells

The influence of short wavelength light on the characteristic bulk minority carrier diffusion length of the ribbon silicon photovoltaic cell has been investigated. We have measured the intensity and wavelength dependence of the diffusion length in an EFG ribbon cell, and compared it with a standard Czochralski grown silicon cell. While the various short wavelength illuminations have shown no influence on the diffusion length in the CZ cell, the diffusion lengths in the ribbon cell exhibit a strong dependence on the volume generation rate as well as on the wavelength of the superimposed lights. We have concluded that the trap-filling phenomenon at various depths in the bulk neutral region of the cell is consistent with the experimental observation.

Ho, C. T.↗

Photometric and spectroscopic observations of SN 1990E in NGC 1035 - Observational constraints for models of type II supernovae

We present 126 photometric and 30 spectral observations of SN 1990E spanning from 12 days before B maximum to 600 days past discovery. These observations show that SN 1990E was of type II-P, displaying hydrogen in its spectrum, and the characteristic plateau in its light curve. SN 1990E is one of the few SNe II which has been well observed before maximum light, and we present evidence that this SN was discovered very soon after its explosion. In the earliest spectra we identify, for the first time, several N II lines. We present a new technique for measuring extinction to SNe II based on the evolution of absorption lines, and use this method to estimate the extinction to SN 1990E, A(V) = 1.5 +/- 0.3 mag. From our photometric data we have constructed a bolometric light curve for SN 1990E and show that, even at the earliest times, the bolometric luminosity was failing rapidly. We use the late-time bolometric light curve to show that SN 1990E trapped a majority of the gamma rays produced by the radioactive decay of Co-56, and estimate that SN 1990E ejected an amount of Ni-56 virtually identical to that of SN 1987A.

Schmidt, Brian P.↗