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At least 199 records · Page 11

High-energy inelastic neutron scattering data taken at the SEQUOIA spectrometer.

INS measurements were performed using the Fine Resolution Chopper Spectrometer SEQUOIA at the Spallation Neutron Source (SNS) at Oak Ridge National Laboratory. A powder sample of SrCoGe2O6 was loaded in an aluminum can for the measurements and a CCR was used to cool the sample down to 6 K. Data were collected using fixed incident neutron energies of 100 and 30 meV.

MATERIALS SCIENCE↗

C 12 ( n , n 1 ′ γ ) partial γ -ray cross section measured using the GENESIS array

Improved neutron inelastic scattering cross sections have repeatedly been identified as a top priority nuclear data need, important for basic science and a range of applications in nuclear energy, stockpile stewardship, and proliferation detection. For the C 12 ( n , n ′ γ ) reaction in particular, recent measurements have unveiled some structural discrepancies, demonstrating incongruities among themselves and in relation to the ENDF/B-VIII.0 nuclear data evaluation. To help resolve these disagreements, a measurement was performed at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory using a broad-spectrum neutron beam and a 99.8% pure natural carbon target. The Gamma Energy Neutron Energy Spectrometer for Inelastic Scattering (GENESIS) was employed to measure energy-differential γ -ray emission spectra as a function of incident neutron energy in the energy range of 5.5 to 16.7 MeV. The C 12 partial γ -ray cross sections were extracted at 63 ∘ , 122 . 5 ∘ , and 150 ∘ with respect to the incoming neutron beam and integrated using angular distribution data available in the literature. The data show agreement with a recent literature measurement and evaluation from 11 to 15 MeV, but indicate a larger cross section for incident neutron energies between 5.5 and 8.5 MeV. The measured relative angular distributions are also reported and were found to agree with evaluation. Published by the American Physical Society 2025

Gordon, J. M. (ORCID:0009000789886897)↗

Science applications of the Mars Observer gamma ray spectrometer

The Mars Observer gamma ray spectrometer will return data related to the elemental composition of Mars. The instrument has both a gamma ray spectrometer and several neutron detectors. The gamma ray spectrometer will return a spectrum nominally every 20 s from Mars permitting a map of the elemental abundances to be made. The gamma rays are emitted from nuclei involved in radioactive decay, from nuclei formed by capture of a thermal neutron, and from nuclei put in an excited state by a fast-neutron interaction. The gamma rays come from an average depth of the order of a few tens of centimeters. The spectrum will show sharp emission lines whose intensity determines the concentration of the element and whose energy identifies the element. The neutron detectors, using the fact that the orbital velocity of the Mars Observer spacecraft is similar to the velocity of thermal neutrons, determine both the thermal and epithermal neutron flux. By combining the results from both techniques it is possible to map the depth dependence of hydrogen in the upper meter as well. These data permit a variety of Martian geoscience problems to be addressed including the crust and mantle composition, weathering processes, volcanism, and the volatile reservoirs and processes.

Boynton, W. V.↗

Forward modeling approach to nuclear reaction cross sections: Applications in neutron inelastic scattering

The development of nuclear reaction models for the production of evaluated nuclear data has traditionally been performed by comparing measured cross sections with predictions from reaction model codes whose physical input parameters are adjusted to obtain the best agreement between measured and modeled results. To more directly probe reaction model inputs, this work introduces a forward modeling approach to experimental reaction cross-section determination, where the most important physical input parameters to reaction model calculations are obtained via 𝜒 2 minimization between measured and calculated observables. This was demonstrated using data collected by the Gamma Energy Neutron Energy Spectrometer for Inelastic Scattering (GENESIS) at the 88-inch cyclotron at Lawrence Berkeley National Laboratory, a detection array consisting of organic liquid scintillators and high-purity germanium (HPGe) detectors. Using a broad-spectrum neutron beam and a 99.98%-enriched 56 Fe target, GENESIS was used to perform a simultaneous measurement of 56 Fe 𝛾-ray production cross sections and secondary neutron energy and angle distributions. The results of the forward modeling approach to the determination of energy-differential 𝛾-ray production cross sections for the yrast 4 + → 2 + and 6 + → 4 + transitions, as well as eight other off-yrast transitions, were compared against those obtained using conventional techniques, and the results are in good agreement. In addition to discrete 𝛾-ray yield total scattered neutron energy-angular distributions as a function of incident neutron energy were also obtained using forward modeling and found to agree with evaluated data, with the exception of elastic scattering at small angles. The fitted reaction model parameters obtained through forward modeling were also used to calculate the cross section for the unobserved (𝑛, 2⁢𝑛) reaction; excellent agreement with the current evaluation was obtained, providing a validation of the predictive capabilities of the forward model approach. This work bridges the gap between nuclear data experiment and evaluation by providing a new means for extracting inelastic neutron-scattering cross sections and neutron-induced 𝛾-ray production data while directly probing reaction model physics.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Dataset for First Full Dalitz Plot Measurement in Neutron β-Decay using the Nab Spectrometer and Implications for New Physics

The Nab apparatus at the Fundamental Neutron Physics Beamline at the Spallation Neutron Source was designed to measure key observations in neutron beta decay, test the Standard Model's description of the weak interaction, and search for new physics. This data was collected using the Nab apparatus and are presented in the article "First Full Dalitz Plot Measurement in Neutron β-Decay using the Nab Spectrometer and Implications for New Physics." This data publication includes CSV (comma-separated values) files which are used to generate Figures 3 - 11 in the linked journal article.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Near-Infrared Monitoring of Volatiles in Frozen Lunar Simulants While Drilling

In Situ Resource Utilization (ISRU) focuses on using local resources for mission consumables. The approach can reduce mission cost and risk. Lunar polar volatiles, e.g. water ice, have been detected via remote sensing measurements and represent a potential resource for both humans and propellant. The exact nature of the horizontal and depth distribution of the ice remains to be documented in situ. NASA's Resource Prospector mission (RP) is intended to investigate the polar volatiles using a rover, drill, and the RESOLVE science package. RP component level hardware is undergoing testing in relevant lunar conditions (cryovacuum). In March 2015 a series of drilling tests were undertaken using the Honeybee Robotics RP Drill, Near-Infrared Volatile Spectrometer System (NIRVSS), and sample capture mechanisms (SCM) inside a 'dirty' thermal vacuum chamber at the NASA Glenn Research Center. The goal of these tests was to investigate the ability of NIRVSS to monitor volatiles during drilling activities and assess delivery of soil sample transfer to the SCMs in order to elucidate the concept of operations associated with this regolith sampling method.

Neutron Spectrometer System↗

Inelastic Neutron Scattering Data for Ba₃Zn(Ru₀.₁Sb₁.₉)O₉

This dataset contains inelastic neutron scattering measurements on the magnetically dilute compound Ba₃Zn(Ru₀.₁Sb₁.₉)O₉, collected at the Spallation Neutron Source using the Cold Neutron Chopper Spectrometer (CNCS) and the SEQUOIA Fine-Resolution Fermi Chopper Spectrometer. The sample consists of nominally 5% magnetic Ru⁵⁺ ions (S = 3/2) randomly substituted into a diamagnetic Sb⁵⁺ matrix. Measurements were performed at base temperature (2–5 K) and 300 K using multiple incident energies (1.00, 3.32, 12.0, and 100 meV) to resolve magnetic excitations from isolated monomers and small Ru clusters (dimers, trimers, etc.). The dataset includes raw event-mode files, momentum- and energy-resolved spectra, and supporting metadata for instrument configuration, sample environment, and reduction parameters.

36 MATERIALS SCIENCE↗

Data for NB6 HBRR Science Design ORNL/TM-2025/3807

Data for the report (ORNL/TM-2025/3807) that describes the calculations and the Monte Carlo Ray Tracing simulations performed using the McStas package to determine the coatings and geometry for the NB-6 guide. It provides the information to inform the mechanical design, validation tests and verification that it meets the science requirements.

47 OTHER INSTRUMENTATION↗

Development of the Probing In-Situ with Neutron and Gamma Rays (PING) Instrument for Planetary Science Applications

The Probing In situ with Neutrons and Gamma rays (PING) instrument is a promising planetary science application of the active neutron-gamma ray technology that has been used successfully in oil field well logging and mineral exploration on Earth for decades. Similar techniques can be very powerful for non-invasive in situ measurements of the subsurface elemental composition on other planets. The objective of our active neutron-gamma ray technology program at NASA Goddard Space Flight Center (NASA/GSFC) is to bring instruments using this technology to the point where they can be flown on a variety of surface lander or rover missions to the Moon, Mars, Venus, asteroids, comets and the satellites of the outer planets. PING combines a 14 MeV deuterium-tritium pulsed neutron generator with a gamma ray spectrometer and two neutron detectors to produce a landed instrument that can determine the elemental composition of a planet down to 30 - 50 cm below the planet's surface. The penetrating nature of.5 - 10 MeV gamma rays and 14 MeV neutrons allows such sub-surface composition measurements to be made without the need to drill into or otherwise disturb the planetary surface, thus greatly simplifying the lander design. We are currently testing a PING prototype at a unique outdoor neutron instrumentation test facility at NASA/GSFC that provides two large (1.8 m x 1.8 m x.9 m) granite and basalt test formations placed outdoors in an empty field. Since an independent trace elemental analysis has been performed on both the Columbia River basalt and Concord Gray granite materials, these samples present two known standards with which to compare PING's experimentally measured elemental composition results. We will present experimental results from PING measurements of both the granite and basalt test formations and show how and why the optimum PING instrument operating parameters differ for studying the two materials.

Parsons, A.↗

Neutral Pion Electroproduction and development of a Neutral Particle Spectrometer

Protons and neutrons, i.e. nucleons, are the basic building blocks of the matter in the visible universe. The strong force binds the nucleons to form nuclei. The electromagnetic force forms the atoms by binding the electrons with the nuclei. The electromagnetic interaction is well understood by Quantum Electrodynamics (QED), which shows the most precise predictability amongst all the theories in physics. In QED, charges interact with each other by exchanging photons. The Quantum Chromodynamics (QCD) describes the strong interaction. Its degrees of freedom are quarks and gluons, the fundamental constituents of the nucleons. The quarks interact with each other by exchanging gluons. However, unlike QED, the gluons interact amongst themselves. This feature of self bindings of the gluons confines the quarks and gluons in the nucleons/hadrons, never to be seen as free. In order to study some of the features of QCD, such as confinement or the structure of the nucleon, one usually needs to rely on experiments. Electromagnetic probes, governed by the well-understood QED, are excellent tools to probe the nucleon. In general, different scales, e.g. electron beam energies, probe different regions of the nucleon. At low energy, of the order of a few GeV, the electron probes the nucleon in the valence quark region. As its energy increases, the electron probes the sea quark and gluon regions. The study of the nucleon structure in all these regions is needed to fully understand QCD. Form factors and parton distribution functions measured from elastic scattering and deep inelastic scattering of leptons off nucleons have provided a partial view of the internal structure of the nucleon. In the mid-1990s, Generalized Parton Distributions (GPDs) were developed. These new objects are a generalization of the form factors and parton distribution functions, but contain richer information on the nucleon internal structure. GPDs are accessible experimentally by deep exclusive reactions. Deeply virtual Compton scattering (DVCS) and deeply virtual meson production (DVMP) are some examples. The first dedicated DVCS/DVMP experiment took place in 2004 in Hall A at The Thomas Jefferson National Accelerator Facility, i.e. Jefferson Lab, in Virginia, U.S.A. A new DVCS/DVMP experiment, after the beam energy upgrade of Jefferson Lab, was carried out in Hall A in a wider kinematic range. Its data were taken from 2014 to 2016. In Hall C at Jefferson Lab, the next DVCS/DVMP experiment will take place. The Hall C experiment will further exploit the kinematic range with higher precision. A Neutral Particle Spectrometer (NPS) is in development to measure DVCS/DVMP events under high background conditions. Jefferson Lab will provide the highest precision data in the valence quark region for various exclusive reactions. The Electron-Ion Collider (EIC) is a future experimental facility currently planned to start operations around 2030 in the U.S.A. Its high energy and high luminosity will probe the sea quark and gluon regions providing answers to the outstanding questions of QCD, in particular in the region where matter is dominated by gluons. First of all, this document describes the data analysis and results of the Hall A neutral pion electroproduction off the proton, from the data taken in 2014-2016. Later, some of the developments towards the construction of the electromagnetic calorimeter of the NPS for the upcoming DVCS/DVMP experiment in Hall C are presented. Finally, one of the candidate materials for the EIC calorimeter, a glass scintillator, will be briefly introduced. I have participated to all these projects, in collaboration with many colleagues. I present in this thesis my contributions to each of these projects. My contributions to the neutral pion data analysis were focused on background subtractions on the calorimeter, acceptance calculations, and the estimation of the systematic uncertainty associated to the event selection cuts. Some necessary information on calibrations of the detectors and data analysis methods are also described. In the NPS project, I performed background dose calculations and energy and position resolution studies of the calorimeter, all using Monte Carlo simulations, with realistic geometries of the experimental apparatus. Characterization of the crystals of the calorimeter was also done. Additionally, I measured the radiation hardness of some glass scintillator in its early stage of development. In order to have a future reference when the glass calorimeter prototype will be tested, I simulated the energy resolution of the prototype.

Ko, Ho-San↗

The inertial confinement fusion experimental platform and diagnostics for studies of nuclear reactions relevant to nuclear astrophysics

High energy density plasmas generated in laser-driven inertial confinement fusion implosions provide unparalleled laboratory conditions for studying stellar-relevant nuclear reactions: plasma environment; hot and dense; uniquely high achievable neutron flux. These experiments have the potential to address long-standing questions about plasma effects on nuclear reactions hitherto experimentally inaccessible, including nuclear rates with thermally distributed reactants, plasma screening, and reactions involving nuclei in excited states. The National Ignition Facility (NIF) and OMEGA lasers are two primary facilities for executing experiments of this type. Existing and future nuclear diagnostics, along with supporting diagnostics to characterize the platform, enable exploitation of these plasmas for such nuclear astrophysics-relevant experiments. Here, this review describes the nuclear diagnostic capabilities currently available for these types of experiments at the NIF and OMEGA, including neutron time-of-flight spectrometers, charged-particle detectors, gamma detectors and radiochemistry diagnostics, and briefly summarizes other available diagnostic capabilities used for platform characterization. Enabling tools not yet available are also identified, including a rapid radioactive sample retrieval system, a low-energy neutron spectrometer and a high-efficiency gamma spectrometer.

National Ignition Facility↗

A super-resolution technique to analyze single-crystal inelastic neutron scattering measurements using direct-geometry chopper spectrometers

Direct-geometry time-of-flight chopper neutron spectroscopy is instrumental in studying dynamics in liquid, powder, and single crystal systems. We report here that real-space techniques in optical imagery can be adapted to obtain reciprocal-space super resolution dispersion for phonon or magnetic excitations from single-crystal neutron spectroscopy measurements. The procedure to reconstruct super-resolution energy dispersion of excitations relies on an accurate determination of the momentum and energy-dependent point spread function and a dispersion correction technique inspired by an image disparity calculation technique commonly used in stereo imaging. Here by, applying these methods to spinwave dispersion data from a virtual neutron experiment demonstrates ~5-fold improvement over nominal energy resolution.

47 OTHER INSTRUMENTATION↗

Accelerator measurement of NaI response to medium energy neutrons and application to a satellite-borne spectrometer

We report on the response of a prototype detector to medium energy neutrons. The neutrons were produced by n-p scattering of a neutron beam on a hydrogen target. The measurements provide unique data on the efficiency and response of large NaI scintillators to neutrons in the energy range 36-709 MeV. We apply the results to the high-energy mode of the Gamma-Ray Spectrometer (GRS) on the Solar Maximum Mission satellite by estimating its efficiency for neutron detection. This estimate is compared to earlier Monte Carlo calculations of the GRS efficiency.

Dunphy, P. P.↗

Thermal scattering law for ice based on neutron time-of-flight experiments carried out at the SEQUOIA spectrometer at the Oak Ridge National Laboratory

Precise estimation of neutron thermalization in moderators relies on high-fidelity thermal scattering cross-section data governed by the thermal scattering law (TSL). The Institut de Radioprotection et de Sûreté Nucléaire (IRSN) has been working on the development of improved TSL for light water ice. Many polymorphic phases of light water ice exist depending on the thermodynamic conditions. The most common type of ice at standard pressure and temperature below water freezing point (273.15 K) is ice-Ih. It is essential to have high-resolution experimental double differential data for developing and/or validating TSL for moderator materials.Existing experimental double-differential scattering data for ice-Ih are extremely sparse and of limited quality. New high-quality double-differential measurements for ice-Ih over multiple temperatures and incident neutron energies would directly support the validation and improvement of ice-Ih TSL models for criticality safety applications.Series of time-of-flight (TOF) inelastic neutron scattering experiments on ice-Ih at temperatures starting at 271 K and down to 6 K, have been carried out at the SEQUOIA spectrometer at the Spallation Neutron Source (SNS) at the Oak Ridge National Laboratory (ORNL), United States. The experiments have been performed for incident neutron energies, Ei= 11, 55, 160, 250, and 600 meV, to explore different excitation energies in the vibrational phonon spectrum. This paper presents the thermodynamic conditions and the details of the TOF measurements on ice-Ih and the derived phonon spectrum from the experimentally measured double differential data. A study of the variation of the phonon spectrum of ice-Ih as a function of temperature is highlighted, and a preliminary TSL evaluation is developed based on the experimental phonon spectrum.

Jaiswal, V↗

Oak Ridge National Laboratory Neutron Spin Echo Beamline on NB-2

Neutron Spin Echo (NSE) spectroscopy uniquely measures the Q-dependence of slow relaxation dynamics, and having such a machine at HFIR will advance polarized neutron spectroscopy and promote the study of biophysical and energy materials using neutrons. The 2018 Instrument Advisory Board (IAB) advises Neutron Sciences Directorate, ORNL to upgrade the cold neutron delivery system at HFIR, addressing geometrical challenges in neutron transfer from the bright cold source. This is being optimized now: the entrance to the guide system is moving closer to the source, and more guides are being added. However, there are still significant challenges to making the cold flux at the sample world-class. With the proposed guide system, NB-2 can deliver more than 10 6 polarized neutrons per cm 2 /sec below 8Å, and probably 10Å with further optimization. With no potential for running user experiments with neutrons longer than 15Å, the utility of such a machine for biological studies is limited. However, there is a large demand for this class of spectrometer in materials science, chemical engineering, and nanotechnology. Workshops held over the past decade and the three-source vision have highlighted the community's need for a low-angle, high-energy resolution spectrometer at HFIR. A detailed design study of this spectrometer is needed, focusing on optimizing the neutron delivery system for SANS-type studies. This neutron spectrometer would complement studies already performed on both SNSNSE and BASIS by overlapping and extend the dynamic range accessible, while acknowledging the proposed machine, EXPANSE, at the Second Target Station. Two technologies currently exist for such a spectrometer: traditional DC solenoids like those on BL-15 at SNS and IN15 at the ILL, and RF-flipper-based machines similar to RESEDA at FRMII. Either instrument would satisfy the scientific justification. However, there are strong business and scientific cases to utilize the thermal flux, the resonant expertise developed at ORNL, and the potential to utilize an entangled beam of neutrons to probe quantum matter by adopting the neutron resonant spin-echo configuration.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗