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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 199 records · Page 11
All sourcesNASA NTRSDOE OSTI
NASA NTRS1984

The effect of physical parameterizations and initial data on the numerical prediction of the President's Day cyclone

Results are presented from a series of forecast experiments which were conducted to assess the importance of large-scale dynamical processes, diabatic heating, and initial data to the prediction of the President's Day cyclone. The synoptic situation and NMC model forecasts for this case are summarized, and the analysis/forecast system and experiments are described. The GLAS Model forecast from the GLAS analysis at 0000 GMT 18 February is found to have correctly predicted intense coastal cyclogenesis and heavy precipitation. A forecast with surface heat and moisture fluxes eliminated failed to predict any cyclogenesis while a similar forecast with only the surface moisture flux excluded showed weak development. Diabatic heating resulting from oceanic fluxes significantly contributed to the generation of low-level cyclonic vorticity and the intensification and slow rate of movement of an upper level ridge over the western Atlantic.

Atlas, R.↗
DOE OSTI2023

Analysis of an Arctic cold air outbreak during autumn and related air mass transformations forced by surface changes and advection in higher altitudes

During marine cold air outbreaks (MCAOs), cold and dry Arctic air masses are transported from the central Arctic southward across the closed sea ice and much warmer open oceans. They experience significant transformations including a rapid heating and moistening, often leading to cloud formation. While intense wintertime MCAOs have been analyzed widely, the air mass transformations during other seasons have been studied sparsely. We address this gap by investigating an MCAO case observed in September 2020. To study the transformation processes, we combine the fifth generation of atmospheric reanalyses of the global climate (ERA5), trajectory calculations, as well as shipborne and airborne measurements. In the central Arctic, observations acquired from aboard the research vessel (RV) Polarstern during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition characterized the initial state of the air mass over closed sea ice. Trajectories indicated the pathway the air mass took from RV Polarstern southward to the Fram Strait. For the first 24 h of the southbound drift, the air masses remained quasi-stationary. Then, still 15 h ahead of the marginal sea ice zone, differential advection across the boundary layer flow introduced humidity and clouds at higher altitudes between 1.5 and 2.5 km. ERA5-derived temperature and humidity tendencies indicated complex vertical interactions. Radiative cloud-top cooling, entrainment, and turbulence were significantly reduced in the lower and enhanced in the upper advected cloud layer. Eventually, the lower cloud deck dissipated. After this confluence of 2 different air masses, observations gathered by Polar 5 in Fram Strait as part of the MOSAiC Airborne observations in the Central Arctic campaign revealed cloudy, moist layers throughout the lowest 3.5 km and an increasing boundary layer height. Comparing the initial with the final state 48 h later, the largest net heating of +8 K was found close to the surface, yet the largest net moistening of +2.5 g kg -1 at an altitude of 1 km, as the initial profile was exceptionally dry here. We conclude that the observed air mass transformations were driven by the surface changes from sea ice to open ocean but additionally strongly impacted by the differential advection of clouds and moisture across the near-surface MCAO flow.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2000

A 3-D Model Analysis of The Impact of Asian Anthropogenic Emissions on the Sulfur Cycle Over the Pacific Ocean

The impact of anthropogenic activities on the SO2 and sulfate aerosol levels over the Pacific region is examined in the Georgia Tech/Goddard Global Ozone Chemistry Aerosol Radiation and Transport (GOCART) model. We focus on the analysis of the data from the NASA Pacific Exploratory Missions (PEM) over the western North Pacific and the tropical Pacific. These missions include PEM-West A in September-October 1991, when the Asian outflow was at the minimum but the upper atmosphere was heavily influenced by the Pinatubo volcanic eruption, and PEM-West B in March-April 1994 when the Asian outflow was at the maximum, and PEM-Tropics A in August-September at a region relatively free of direct anthropogenic influences. Specifically, we will examine the relative importance of anthropogenic, volcanic and biogenic sources to the SO2 and sulfate concentrations over the Pacific, and quantify the processes controlling the distributions of SO2 and sulfate in both the boundary layer and the free troposphere. We will also assess the global impact of SO2 emission in Asia on the sulfate aerosol loading.

Chin, Mian↗
DOE OSTI2020

Impacts of Ice-Shelf Melting on Water-Mass Transformation in the Southern Ocean from E3SM Simulations

Abstract The Southern Ocean overturning circulation is driven by winds, heat fluxes, and freshwater sources. Among these sources of freshwater, Antarctic sea ice formation and melting play the dominant role. Even though ice-shelf melt is relatively small in magnitude, it is located close to regions of convection, where it may influence dense water formation. Here, we explore the impacts of ice-shelf melting on Southern Ocean water-mass transformation (WMT) using simulations from the Energy Exascale Earth System Model (E3SM) both with and without the explicit representation of melt fluxes from beneath Antarctic ice shelves. We find that ice-shelf melting enhances transformation of Upper Circumpolar Deep Water, converting it to lower density values. While the overall differences in Southern Ocean WMT between the two simulations are moderate, freshwater fluxes produced by ice-shelf melting have a further, indirect impact on the Southern Ocean overturning circulation through their interaction with sea ice formation and melting, which also cause considerable upwelling. We further find that surface freshening and cooling by ice-shelf melting cause increased Antarctic sea ice production and stronger density stratification near the Antarctic coast. In addition, ice-shelf melting causes decreasing air temperature, which may be directly related to sea ice expansion. The increased stratification reduces vertical heat transport from the deeper ocean. Although the addition of ice-shelf melting processes leads to no significant changes in Southern Ocean WMT, the simulations and analysis conducted here point to a relationship between increased Antarctic ice-shelf melting and the increased role of sea ice in Southern Ocean overturning.

Jeong, Hyein↗
NASA NTRS1995

Radiative flux opens new window on climate research

For several decades, global satellite observations have been made of the rate at which electromagnetic energy (radiative flux) is emerging from the top of the atmosphere of our planet in the spectral range of about 0.2-50.0 microns. At the same time, models have been developed to infer the radiative flux at the surface from the values observed by the satellites at the upper boundary. The balance of incoming and outgoing radiative flux (radiation budget) at both boundaries, determines the net gain or loss of the radiative energy within an atmospheric column. Climate researchers can use the radiative flux as a tool to validate climate models, separate the radiative impact of clouds from surface and atmosphere contributions, and to understand the global hydrological cycle. When applied to physical processes occurring at the surface, information on the radiative flux has the potential to substantially advance our understanding of the transport of heat, moisture, and momentum across the surface/atmosphere interface. Geophysicists of many disciplines stand to benefit from efforts to improve the use of this latter untapped resource. Oceanographers can improve the representation of the selective absorption of radiation in the oceans; biologists and ecologists can improve their models for carbon dioxide exchange and biological heating in oceans; agronomists can model more realistically biomass and crop yields; and environmentalists can obtain better assessment of natural resources of radiation.

Pinker, R. T.↗
DOE OSTI2019

What Drives Upper-Ocean Temperature Variability in Coupled Climate Models and Observations?

Abstract A key question in climate modeling is to what extent sea surface temperature and upper-ocean heat content are driven passively by air–sea heat fluxes, as opposed to forcing by ocean dynamics. This paper investigates the question using a climate model at different resolutions, and observations, for monthly variability. At the grid scale in a high-resolution climate model with resolved mesoscale ocean eddies, ocean dynamics (i.e., ocean heat flux convergence) dominates upper 50 m heat content variability over most of the globe. For deeper depths of integration to 400 m, the heat content variability at the grid scale is almost totally controlled by ocean heat flux convergence. However, a strong dependence on spatial scale is found—for the upper 50 m of ocean, after smoothing the data to around 7°, air–sea heat fluxes, augmented by Ekman heat transports, dominate. For deeper depths of integration to 400 m, the transition scale becomes larger and is above 10° in western boundary currents. Comparison of climate model results with observations show that the small-scale influence of ocean intrinsic variability is well captured by the high-resolution model but is missing from a comparable model with parameterized ocean-eddy effects. In the deep tropics, ocean dynamics dominates in all cases and all scales. In the subtropical gyres at large scales, air–sea heat fluxes play the biggest role. In the midlatitudes, at large scales >10°, atmosphere-driven air–sea heat fluxes and Ekman heat transport variability are the dominant processes except in the western boundary currents for the 400 m heat content.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2017

A Future Mars Environment for Science and Exploration

Today, Mars is arid and cold with a very thin atmosphere that has significant frozen and underground water resources. The thin atmosphere prevents liquid water from residing permanently on its surface and makes it difficult to land missions since it is not thick enough to completely facilitate a soft landing. In its past, under the influence of a significant greenhouse effect, Mars must have had a significant water ocean covering perhaps 30% of the northern hemisphere. Mars lost its protective magnetosphere and therefore much of its atmosphere around 3 Ga ago, due to the solar wind. The atmospheric loss into the solar wind is somewhat balanced by the outgassing of the Mars interior and crust that contributes to the existing atmosphere leading to a global-mean surface atmosphere of ~6 mbar pressure currently. By using our extensive simulation tools and physics capabilities in Space Weather and Mars global climate modeling, we have started to explore the effects on Mars of placing an artificial magnetic dipole field at the Mars L1 Lagrange point putting Mars in a magnetotail. This situation then eliminates many of the solar-wind erosion processes that occur with the planet's ionosphere and upper atmosphere allowing the Martian atmosphere to grow in pressure and bulk temperature over time. Under thicker atmospheres, the global circulation patterns and seasonal changes are much different than at present. An enhanced atmosphere would: allow larger landed mass of equipment to the surface, shield against some cosmic and solar particle radiation, extend the ability for extraction, and provide "open air" greenhouses to exist for plant production, just to name a few. These new conditions on Mars would allow human explorers and researchers to study the planet in much greater detail and enable a truly profound new understanding of the habitability of this planet.

Space Weather and Mars global climate modeling↗
NASA NTRS1987

Evidence for variations in magma production along oceanic spreading centers - A critical appraisal

Recent geologic, geophysical, and geochemical studies of the oceanic lithosphere near fracture zones have resulted in the proposal that the 'magma budget,' defined as the amount of magma delivered to magma chambers or conduits beneath a spreading center for a given amount of spreading, decreases as fracture zones are approached. Seismic reflection and refraction studies indicate that the crust becomes anomalously thin near fracture zones, but reference must be made to the boundary between residual upper mantle peridotites and overlying cumulate rocks in order to assess potential variations in the magma budget. The position of this interface, however, generally is not constrained by geophysical studies. Geochemical variations in basaltic glasses collected near fracture zones are consistent with a decrease in partial melting as fracture zones are approached, but they could also be produced by variations in open-system magmatic processes with no change in the extent of partial melting. Although a decrease in the magma budget as fracture zones are approached is consistent with these data, so are alternative models that incorporate a constant magma budget.

Karson, J. A.↗
NASA NTRS2003

Elevated Ozone in the Troposphere over the Atlantic and Pacific Oceans in the Northern Hemisphere

Tropospheric column ozone (TCO) is derived from differential measurements of total column ozone from Nimus-7 and Earth Probe TOMS, and stratospheric column ozone from the Microwave Limb Sounder instrument on the Upper Atmospheric Research Satellite. It is shown that TCO during summer months over the Atlantic and Pacific Oceans at northern mid-latitudes is about the same (50-60 Dobson Units) as over the continents of North America, Europe and Asia, where surface emissions of nitrogen oxides from industrial sources, biomass and biofuel burning and biogenic emissions are significantly larger. This nearly uniform zonal variation in TCO is modulated by surface topography of the Rocky and Himalayan mountains and Tibetan Plateau where TCO is reduced by 20-30 Dobson Units. The zonal characteristics of TCO derived from satellite measurements are well simulated by a global chemical transport model called MOZART-2 (Model of Ozone and Related Chemical Tracers, version 2). The model results are analyzed to delineate the relative importance of various processes contributing to observed zonal characteristics of TCO, and they are shown that the surface emission of NOx contributes about 50% of the TCO at northern mid-latitudes, especially over the continents of North America, Europe and Asia. The result of TCO derived from TOMS and the analysis from MOZART-2 indicate that TCO is a very useful tool to study tropospheric O3 pollution resulting from surface emissions of pollutants.

Chandra, S.↗
NASA NTRS2017

Causes of Interannual Variability over the Southern Hemispheric Tropospheric Ozone Maximum

We examine the relative contribution of processes controlling the interannual variability (IAV) of tropospheric ozone over four sub-regions of the southern hemispheric tropospheric ozone maximum (SHTOM) over a 20-year period. Our study is based on hindcast simulations from the National Aeronautics and Space Administration Global Modeling Initiative chemistry transport model (NASA GMI-CTM) of tropospheric and stratospheric chemistry, driven by assimilated Modern Era Retrospective Analysis for Research and Applications (MERRA) meteorological fields. Our analysis shows that over SHTOM region, the IAV of the stratospheric contribution is the most important factor driving the IAV of upper tropospheric ozone (270 hectopascals), where ozone has a strong radiative effect. Over the South Atlantic region, the contribution from surface emissions to the IAV of ozone exceeds that from stratospheric input at and below 430 hectopascals. Over the South Indian Ocean, the IAV of stratospheric ozone makes the largest contribution to the IAV of ozone with little or no influence from surface emissions at 270 and 430 hectopascals in austral winter. Over the tropical South Atlantic region, the contribution from IAV of stratospheric input dominates in austral winter at 270 hectopascals and drops to less than half but is still significant at 430 hectopascals. Emission contributions are not significant at these two levels. The IAV of lightning over this region also contributes to the IAV of ozone in September and December. Over the tropical southeastern Pacific, the contribution of the IAV of stratospheric input is significant at 270 and 430 hectopascals in austral winter, and emissions have little influence.

Global Modeling Initiative chemistry transport mod↗
NASA NTRS2006

A Lagrangian trajectory view on transport and mixing processes between the eye, eyewall, and environment using a high resolution simulation of Hurricane Bonnie (1998)

The transport and mixing characteristics of a large sample of air parcels within a mature and vertically sheared hurricane vortex is examined. Data from a high-resolution (2 km grid spacing) numerical simulation of "real-case" Hurricane Bonnie (1998) is used to calculate Lagrangian trajectories of air parcels in various subdomains of the hurricane (namely, the eye, eyewall, and near-environment) to study the degree of interaction (transport and mixing) between these subdomains. It is found that 1) there is transport and mixing from the low-level eye to the eyewall that carries high- Be air which can enhance the efficiency of the hurricane heat engine; 2) a portion of the low-level inflow of the hurricane bypasses the eyewall to enter the eye, that both replaces the mass of the low-level eye and lingers for a sufficient time (order 1 hour) to acquire enhanced entropy characteristics through interaction with the ocean beneath the eye; 3) air in the mid- to upper-level eye is exchanged with the eyewall such that more than half the air of the eye is exchanged in five hours in this case of a sheared hurricane; and 4) that one-fifth of the mass in the eyewall at a height of 5 km has an origin in the mid- to upper-level environment where thet(sub e) is much less than in the eyewall, which ventilates the ensemble average eyewall theta(sub e) by about 1 K. Implications of these findings to the problem of hurricane intensity forecasting are discussed.

Cram, Thomas A.↗
DOE OSTI2021

An Improved Representation of Aerosol Wet Removal by Deep Convection and Impacts on Simulated Aerosol Vertical Profiles

Here, we introduce a physics-based aerosol wet removal scheme with unified treatments of aerosol transport and removal by convective clouds into the Community Atmosphere Model version 6. Since several important physical processes are still neglected or poorly represented in this new physics-based scheme, we develop secondary improvements to the parameterizations of aerosol activation, resuspension, and cloud-borne aerosol detrainment in this new scheme. Changes in the aerosol wet removal scheme cause tropospheric aerosol concentrations to decrease to different extents: compared to the control run, the physics-based scheme significantly decreases aerosol burdens by up to 60% over the southern Pacific Ocean, whereas the secondary improvements mitigate the decreasing tendency. The burden changes also depend on aerosol chemical components: the sulfate mass decrease is compensated by secondary production, black carbon (BC) is effectively removed via increasing the hygroscopicity of particulate organic matter from 0 to 0.2, and dust shows the most spatially heterogeneous changes. Simulated aerosol profiles are evaluated against aircraft-based observations over the Pacific and Atlantic Oceans. The secondary-improved scheme reduces the overestimations of upper tropospheric BC and sea salt concentrations by a factor of 10 and 1,000, respectively, and reproduces the dependence of BC mass decrease rates on cloud types. Consideration of convective cloud-borne aerosol detrainment plays the most important role in enhancing the aerosol wet removal and decreasing the positive biases of tropospheric BC and sea salt concentrations. We also summarize unresolved issues related to convective cloud genesis and microphysics, cloud-borne aerosol evolution, and BC and dust emissions.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1993

The meteorological environment of the tropospheric ozone maximum over the tropical South Atlantic Ocean

Atmospheric flow patterns are examined over the South Atlantic Ocean where a maximum of tropospheric ozone has been observed just west of southern Africa. We investigate the flow climatology during October and perform a case study for six days during October 1989. Horizontal and vertical motions are examined and used to prepare 3D backward trajectories from the region of greatest ozone. An initially zonally symmetric distribution of ozone is treated as a passive tracer and advected by 3D flows forecast by the global model. Results from the passive tracer simulation indicate that 3D advection alone can produce a maximum of tropospheric ozone in the observed location. In addition, the trajectories suggest that by-products of biomass burning could be transported to the area of maximum ozone. Low-level flow from commonly observed regions of burning in Africa streams westward to the area of interest. Over Brazil, if the burning by-products are carried into the upper troposphere by convective process, they then could be transported eastward to the ozone feature in approximately five days. There is considerable subsidence over the tropical southern Atlantic, such that stratospheric influences also are a factor in producing the ozone maximum. Both planetary-scale and transient synoptic-scale circulation features play major roles in the various transport processes that influence the region. In summary, the observed tropospheric ozone maximum appears to be caused by a complex set of horizontal and vertical advections, transport from regions of biomass burning, and stratospheric influences.

Krishnamurti, T. N.↗
NASA NTRS2012

The Distribution of Snow Black Carbon observed in the Arctic and Compared to the GISS-PUCCINI Model

In this study, we evaluate the ability of the latest NASA GISS composition-climate model, GISS-E2- PUCCINI, to simulate the spatial distribution of snow BC (sBC) in the Arctic relative to present-day observations. Radiative forcing due to BC deposition onto Arctic snow and sea ice is also estimated. Two sets of model simulations are analyzed, where meteorology is linearly relaxed towards National Centers for Environmental Prediction (NCEP) and towards NASA Modern Era Reanalysis for Research and Applications (MERRA) reanalyses. Results indicate that the modeled concentrations of sBC are comparable with presentday observations in and around the Arctic Ocean, except for apparent underestimation at a few sites in the Russian Arctic. That said, the model has some biases in its simulated spatial distribution of BC deposition to the Arctic. The simulations from the two model runs are roughly equal, indicating that discrepancies between model and observations come from other sources. Underestimation of biomass burning emissions in Northern Eurasia may be the main cause of the low biases in the Russian Arctic. Comparisons of modeled aerosol BC (aBC) with long-term surface observations at Barrow, Alert, Zeppelin and Nord stations show significant underestimation in winter and spring concentrations in the Arctic (most significant in Alaska), although the simulated seasonality of aBC has been greatly improved relative to earlier model versions. This is consistent with simulated biases in vertical profiles of aBC, with underestimation in the lower and middle troposphere but overestimation in the upper troposphere and lower stratosphere, suggesting that the wet removal processes in the current model may be too weak or that vertical transport is too rapid, although the simulated BC lifetime seems reasonable. The combination of observations and modeling provides a comprehensive distribution of sBC over the Arctic. On the basis of this distribution, we estimate the decrease in snow and sea ice albedo and the resulting radiative forcing. We suggest that the albedo reduction due to BC deposition presents significant space-time variations, with highest mean reductions of 1.25% in the Russian Arctic, which are much larger than those in other Arctic regions (0.39% to 0.64 %). The averaged value over the Arctic north of 66degN is 0.4-0.6% during spring, leading to regional surface radiative forcings of 0.7, 1.1 and 1.0Wm(exp−2) in spring 2007, 2008 and 2009, respectively.

Dou, T.↗
NASA NTRS2018

Effects of Greenhouse Gas Increase and Stratospheric Ozone Depletion on Stratospheric Mean Age of Air in 1960-2010

The relative impacts of greenhouse gas (GHG) increase and stratospheric ozone depletion on stratospheric mean age of air in the 1960-2010 period are quantified using the Goddard Earth Observing System Chemistry-Climate Model. The experiment compares controlled simulations using a coupled atmosphere-ocean version of the Goddard Earth Observing System Chemistry-Climate Model, in which either GHGs or ozone depleting substances, or both factors evolve over time. The model results show that GHGs and ozone-depleting substances have about equal contributions to the simulated mean age decrease, but GHG increases account for about two thirds of the enhanced strength of the lower stratospheric residual circulation. It is also found that both the acceleration of the diabatic circulation and the decrease of the mean age difference between downwelling and upwelling regions are mainly caused by GHG forcing. The results show that ozone depletion causes an increase in the mean age of air in the Antarctic summer lower stratosphere through two processes: (1) a seasonal delay in the Antarctic polar vortex breakup that inhibits young midlatitude air from mixing with the older air inside the vortex, and (2) enhanced Antarctic downwelling that brings older air from middle and upper stratosphere into the lower stratosphere.

stratospheric ozone depletion↗
NASA NTRSDate not supplied

Influence of sediment resuspension on deep-ocean Pa-231 and Th-230 cycling: A PROGRESS REPORT

The naturally-occurring particle-reactive radionuclides protactinium-231 (231Pa) and thorium-230 (230Th) are used as tracers of a variety of oceanic processes, both at present and in the past. Most notably, the sediment 231Pa/230Th ratio has been used to infer changes in the Atlantic Meridional Overturning Circulation over the last (de)glaciation. However, recent measurements along the U.S. GEOTRACES North Atlantic transect (GA03) revealed two features which are at odds with current understanding about 231Pa and 230Th behaviour in the ocean: (i) a sharp decrease in dissolved 231Pa and 230Th activities with depth below 2000-4000 m and (ii) very large particulate 231Pa and 230Th activities near the bottom, at a number of stations between the New England continental shelf and Bermuda. Concomitant measurements of particulate matter concentration and potential temperature showed that both features are associated with the benthic nepheloid layer (BNL) and the bottom mixed layer (BML) that are present at these stations. Here we develop and apply a simplified model of the exchange of particles, 231Pa, and 230Th between the BNL and the upper sediment, to explore the extent to which the radionuclide anomalies observed near the bottom at a number of GA03 stations can be explained by local sediment resuspension. We find that the model can broadly reproduce the observed anomalies at two stations where samples for radionuclide analyses were collected near the seafloor. Sensitivity tests with the model show that the 231Pa/230Th ratio of particles in the BML and the sediment varies by a factor of 3 as the sediment resuspension rate fluctuates within a range consistent with observational estimates. The modelled variability is comparable to the spatial variability of 231Pa/230Th of suspended particles in the modern North Atlantic and to the variability of Atlantic sediment 231Pa/230Th records across the last (de)glacial period. Two factors are found to contribute to the modelled sensitivity of the sediment 231Pa/230Th to sediment resuspension rate: the vertical turbulent mixing in the BML and the differential scavenging intensity of Pa and Th due to variation in particle concentration. Overall, our study indicates that the exchange of material between the BNL and the upper sediment can affect the particulate 231Pa/230Th ratio in the bottom water and the sediment, which may complicate the use of sediment 231Pa/230Th as a palaeoceanographic tracer.

particle-reactive radionuclides↗
NASA NTRS2007

Os-186 and Os-187 Enrichments and High-He-3/He-4 sources in the Earth's Mantle: Evidence from Icelandic Picrites

Picrites from the neovolcanic zones in Iceland display a range in Os-187/Os-188O from 0.1297 to 0.1381 ((gamma)Os = 0.0 to 6.5) and uniform Os-186/Os-188 of 0.1198375+/-32 (2 (sigma)). The value for Os-186/Os-188 is within uncertainty of the present-day value for the primitive upper mantle of 0.1198398+/-16. These Os isotope systematics are best explained by ancient recycled crust or melt enrichment in the mantle source region. If so, then the coupled enrichments displayed in Os-186/Os-188 and Os-187/Os-188 from lavas of other plume systems must result from an independent process, the most viable candidate at present remains core-mantle interaction. While some plumes with high He-3/He-4, such as Hawaii, appear to have been subjected to detectable addition of Os (and possibly He) from the outer core, others such as Iceland do not. A positive correlation between Os-187/Os-188 and He-3/He-4 from 9.6 to 19 RA in Iceland picrites is best modeled as mixtures of 500 Ma or older ancient recycled crust mixed with primitive mantle, creating a hybrid source region that subsequently mixes with the convecting MORB mantle during ascent and melting. This multistage mechanism to explain these isotope systematics is consistent with ancient recycled crust juxtaposed with more primitive, relatively He-rich mantle, in convective isolation from the upper mantle, most likely in the lowermost mantle. This is inconsistent with models that propose random mixing between heterogeneities in the convecting upper mantle as a mechanism to explain the observed isotopic variation in oceanic lavas or models that produce a high He-3/He-4 signature in melt depleted and strongly outgassed, He-poor mantle. Instead these systematics require a deep mantle source to explain the 3He/4He signature in Iceland lavas. The He-3/He-4 of lavas derived from the Iceland plume changed over time, from a maximum of 50 RA at 60 Ma, to approximately 25-27 RA at present. The changes are coupled with distinct compositional gaps between the different aged lavas when H-3/He-4 is plotted versus various geochemical parameters such as Nd-143/Nd-144 and La/Sm. These relationships can be interpreted as an increase in the proportion of ancient recycled crust in the upwelling plume over this time period.

Brandon, Alan D.↗