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At least 217 records · Page 12

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-Resolving Model Simulations

Cloud microphysics are inevitably affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds. Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effects of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates for convective clouds. Recently, two detailed spectral-bin microphysical schemes were implemented into the Goddard Cumulus Ensemble (GCE) model. The formulation for the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e.,pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail]. Each type is described by a special size distribution function containing many categories (i.e. 33 bins). Atmospheric aerosols are also described using number density size-distribution functions.A spectral-bin microphysical model is very expensive from a from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep tropical clouds in the west Pacific warm pool region using identical thermodynamic conditions but with different concentrations of CCN: a low "clean" concentration and a high "dirty" concentration. Besides the initial differences in aerosol concentration, preliminary results indicate that the low CCN concentration case produces rainfall at the surface sooner than the high CCN case but has less cloud water mass aloft. Because the spectral-bin model explicitly calculates and allows for the examination of both the mass and number concentration of species in each size categor, a detailed analysis of the instantaneous size spectrum can be obtained for the two cases. It is shown that since the low CCN case produces fewer droplets, larger sized develop due to the greater condensational and collectional growth, leading to a broader size spectrum in comparison to the high CCN case.

Tao, Wei-Kuo↗

A Nanometer Aerosol Size Analyzer (nASA) for Rapid Measurement of High-Concentration Size Distributions

We have developed a fast-response Nanometer Aerosol Size Analyzer (nASA) that is capable of scanning 30 size channels between 3 and 100 nm in a total time of 3 seconds. The analyzer includes a bipolar charger (P0210), an extended-length Nanometer Differential Mobility Analyzer (Nano-DMA), and an electrometer (TSI 3068). This combination of components provides particle size spectra at a scan rate of 0.1 second per channel free of uncertainties caused by response-time-induced smearing. The nASA thus offers a fast response for aerosol size distribution measurements in high-concentration conditions and also eliminates the need for applying a de-smearing algorithm to resulting data. In addition, because of its thermodynamically stable means of particle detection, the nASA is useful for applications requiring measurements over a broad range of sample pressures and temperatures. Indeed, experimental transfer functions determined for the extended-length Nano-DMA using the Tandem Differential Mobility Analyzer (TDMA) technique indicate the nASA provides good size resolution at pressures as low as 200 Torr. Also, as was demonstrated in tests to characterize the soot emissions from the J85-GE engine of a T38 aircraft, the broad dynamic concentration range of the nASA makes it particularly suitable for studies of combustion or particle formation processes. Further details of the nASA performance as well as results from calibrations, laboratory tests and field applications are presented.

Han, Hee-Siew↗

Profiling Transboundary Aerosols over Taiwan and Assessing Their Radiative Effects

A synergistic process was developed to study the vertical distributions of aerosol optical properties and their effects on solar heating using data retrieved from ground-based radiation measurements and radiative transfer simulations. Continuous MPLNET and AERONET observations were made at a rural site in northern Taiwan from 2005 to 2007. The aerosol vertical extinction profiles retrieved from ground-based lidar measurements were categorized into near-surface, mixed, and two-layer transport types, representing 76% of all cases. Fine-mode (Angstrom exponent, alpha, approx.1.4) and moderate-absorbing aerosols (columnar single-scattering albedo approx.0.93, asymmetry factor approx.0.73 at 440 nm wavelength) dominated in this region. The column-integrated aerosol optical thickness at 500 nm (tau(sub 500nm)) ranges from 0.1 to 0.6 for the near-surface transport type, but can be doubled in the presence of upper-layer aerosol transport. We utilize aerosol radiative efficiency (ARE; the impact on solar radiation per unit change of tau(sub 500nm)) to quantify the radiative effects due to different vertical distributions of aerosols. Our results show that the ARE at the top-of-atmosphere (-23 W/ sq m) is weakly sensitive to aerosol vertical distributions confined in the lower troposphere. On the other hand, values of the ARE at the surface are -44.3, -40.6 and -39.7 W/sq m 38 for near-surface, mixed, and two-layer transport types, respectively. Further analyses show that the impact of aerosols on the vertical profile of solar heating is larger for the near-surface transport type than that of two-layer transport type. The impacts of aerosol on the surface radiation and the solar heating profiles have implications for the stability and convection in the lower troposphere.

Wang, Sheng-Hsiang↗

The Role of Aerosols on Precipitation Processes

Cloud physics is inevitably affected by the smoke particle (CCN, cloud condensation nuclei) size distribution below the clouds. Therefore, the size distributions parameterized as spectral bin microphysics are needed to explicitly study the effects of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates for convective clouds. Recently, a detailed spectral--bin microphysical scheme was implemented into the Goddard Cumulus Ensemble (GCE) model. The formulation for the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e., pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail]. Each type is described by a special size distribution function containing many categories (i.e., 33 bins). Atmospheric aerosols are also described using number density size-distribution functions.

Tao, Wei-Kuo↗

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-Resolving Model Simulations

Cloud microphysics is inevitably affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds. Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effects of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates for convective clouds. Recently, two detailed spectral-bin microphysical schemes were implemented into the Goddard Cumulus Ensembel (GCE) model. The formulation for the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e. pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail]. Each type is described by a special size distribution function containing many categories (i.e. 33 bins). Atmospheric aerosols are also described using number density size distribution functions. A spectral-bin microphysical model is very expensive from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep tropical clouds in the west Pacific warm pool region and in the mid-latitude continent with different concentrations of CCN: a low "c1ean"concentration and a high "dirty" concentration. In addition, differences and similarities between bulk microphysics and spectral-bin microphysical schemes will be examined and discussed.

Tao, Wei-Kuo↗

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-Resolving Model Simulations

Cloud microphysics are inevitably affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds. Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effects of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates for convective clouds. Recently, two detailed spectral-bin microphysical schemes were implemented into the Goddard Cumulus Ensemble (GCE) model. The formulation for the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles (i.e., pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail). Each type is described by a special size distribution function containing many categories (i.e. 33 bins). Atmospheric aerosols are also described using number density size-distribution functions. A spectral-bin microphysical model is very expensive from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep cloud systems in the west Pacific warm pool region, in the sub-tropics (Florida) and in the mid-latitude using identical thermodynamic conditions but with different concentrations of CCN: a low 'clean' concentration and a high 'dirty' concentration.

Tao, Wei-Kuo↗

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-resolving Model Simulations

Cloud microphysics is inevitably affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds. Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effects of atmospheric aerosol concentration on cloud development, r d a U production, and rainfall rates for convective clouds. Recently, two detailed spectral-bin microphysical schemes were implemented into the Goddard Cumulus Ensembe1 (GCE) model. The formulation for the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e. pristine ice crystals (columnar and platelike), snow (dendrites and aggregates), graupel and frozen drops/hail]. Each type is described by a special size distribution function containing many categories (i.e. 33 bins). Atmospheric aerosols are also described using number density size-distribution functions. A spectral-bin microphysical model is very expensive from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep tropical clouds in the west Pacific warm pool region and in the mid-latitude continent with different concentrations of CCN: a low "c1ean"concentration and a high "dirty" concentration. In addition, differences and similarities between bulk microphysics and spectral-bin microphysical schemes will be examined and discussed.

Tao, Wei-Kuo↗

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-Resolving Model Simulations

Cloud microphysics are inevitable affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds, Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effect of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates for convective clouds. Recently, a detailed spectral-bin microphysical scheme was implemented into the the Goddard Cumulus Ensemble (GCE) model. The formulation for the explicit spectral-bim microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e., pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail]. Each type is described by a special size distribution function containing many categories (i.e., 33 bins). Atmospheric aerosols are also described using number density size-distribution functions.

Tao, Wei-Kuo↗

The Design & Development of the Ocean Color Instrument Precision Superduplex Hybrid Bearing Cartridge

A high precision, high-resolution Ocean Color Imaging (OCI) instrument is under development for the Plankton, Aerosol, Cloud, ocean Ecosystem (PACE) mission which requires a pair of medium speed mechanisms to scan the ocean surface continuously. The design of the rotating telescope (RT) mechanism operating at 360 RPM and the half-angle mirror (HAM) mechanism synchronized at 180 RPM was concern for maintaining pointing precision over the required life and continuous operations. An effort was undertaken with the manufacturer to design and analyze a special bearing configuration to minimize axial and radial runout, minimize torque, and maintain nominal contact stresses and stiffness over the operating temperature range and to maximize life. The bearing design, development effort, analysis and testing will be discussed as will the technical challenges that this specific design imposed upon the mechanism engineers. Bearing performance, runout as achieved and verified during encoder installation and operating torque will be described.

mechanism↗

Silicon production in an aerosol reactor

An aerosol reactor system was developed in which large particles of silicon can be grown by silane pyrolysis. To grow particles to sizes larger than one micron, vapor deposition must be used to grow a relatively small number of seed particles. Suppression of nucleation is achieved by limiting the rate of gas phase chemical reactions such that the condensible products of the gas phase chemical reactions diffuse to the surface of the seed particles as rapidly as they are produced. This prevents high degrees of supersaturation and runaway nucleation during the growth process. Particles on the order of 10 microns were grown repeatedly with the present aersol reactor. The nucleation controlled aerosol reactor is, therefore, a suitable system for the production of powders that can readily be separated from the gas by aerodynamic means.

Wu, J. J.↗

Uncertainty in Aerosol–Cloud Radiative Forcing Is Driven By Clean Conditions

Atmospheric aerosols and their impact on cloud properties remain the largest uncertainty in the human forcing of the climate system. By increasing the concentration of cloud droplets (Nd), aerosols reduce droplet size and increase the reflectivity of clouds (a negative radiative forcing). Central to this climate impact is the susceptibility of cloud droplet number to aerosol (β), the diversity of which explains much of the variation in the radiative forcing from aerosol–cloud interactions (RFaci) in global climate models. This has made measuring β a key target for developing observational constraints of the aerosol forcing.

Edward Gryspeerdt↗

Lessons Learned From Evaluation and Mitigation of Space Charging Threat Due to Use of Isolated (Hybrid) Bearings on the Pace Ocean Color Instrument

A high precision, high resolution Ocean Color Instrument (OCI) was developed for the Plankton, Aerosol, Cloud ocean Ecosystem (PACE) mission which required the use of electrically isolated Hybrid Bearings (silicon nitride balls). While desirable for technical performance of the instrument, this application caused portions of the instrument to become electrically isolated and come under threat of space charging effects from charged particles and the resultant differential charging. An evaluation of the environment, susceptibility of the components, such as bearings and electronics, and mitigation strategies were performed. As part of that process, simulations of the charging environment, analysis of internal mechanism charging and prediction of most likely discharge paths, testing of the bearings for susceptibility as well as resulting damage were performed and analyzed. Additionally, a novel method to deal with charging was developed. Considerations for dealing with electrically isolated mechanisms, results of the above-mentioned efforts as well as lessons learned are presented.

space charging↗

Use of Combined A-Train Observations to Validate GEOS Model Simulated Dust Distributions During NAMMA

During August 2006, the NASA African Multidisciplinary Analyses Mission (NAMMA) field experiment was conducted to characterize the structure of African Easterly Waves and their evolution into tropical storms. Mineral dust aerosols affect tropical storm development, although their exact role remains to be understood. To better understand the role of dust on tropical cyclogenesis, we have implemented a dust source, transport, and optical model in the NASA Goddard Earth Observing System (GEOS) atmospheric general circulation model and data assimilation system. Our dust source scheme is more physically based scheme than previous incarnations of the model, and we introduce improved dust optical and microphysical processes through inclusion of a detailed microphysical scheme. Here we use A-Train observations from MODIS, OMI, and CALIPSO with NAMMA DC-8 flight data to evaluate the simulated dust distributions and microphysical properties. Our goal is to synthesize the multi-spectral observations from the A-Train sensors to arrive at a consistent set of optical properties for the dust aerosols suitable for direct forcing calculations.

Nowottnick, E.↗

Asian Summer Monsoon Anomalies Induced by Aerosol Direct Forcing: The Role of the Tibetan Plateau

In this paper we present results of a numerical study using the NASA finite-volume GCM to elucidate a plausible mechanism for aerosol impact on the Asian summer monsoon involving interaction with physical processes over the Tibetan Plateau (TP). During the premonsoon season of March April, dusts from the deserts of western China, Afghanistan/Pakistan, and the Middle East are transported into and stacked up against the northern and southern slopes of the TP. The absorption of solar radiation by dust heats up the elevated surface air over the slopes. On the southern slopes, the atmospheric heating is reinforced by black carbon from local emission. The heated air rises via dry convection, creating a positive temperature anomaly in the mid-to-upper troposphere over the TP relative to the region to the south. In May through early June in a manner akin to an elevated heat pump , the rising hot air forced by the increasing heating in the upper troposphere, draws in warm and moist air over the Indian subcontinent, setting the stage for the onset of the South Asia summer monsoon. Our results suggest that increased dust loading coupled with black carbon emission from local sources in northern India during late spring may lead to an advance of the rainy periods and subsequently an intensification of the Indian summer monsoon. The enhanced rainfall over India is associated with the development of an aerosol-induced large-scale sea level pressure anomaly pattern, which causes the East Asia (Mei-yu) rain belt to shift northwestward, suppressing rainfall over East Asia and the adjacent oceanic regions.

Lau, K. M.↗

A lidar equipped with photon counter for measuring stratospheric aerosols

A large lidar system was developed at the Anhui Institute of Optics and Fine Mechanics. It is composed of a high power frequency doubled Nd:YAG laser (120 mJ at 532 nm, 1 mrad), a 651 mm diameter receiving telescope, and a 64 channel photon counter. The lidar observations are controlled by an IBM PC/AT computer. One of the projects is to use the lidar system to make regular observations of stratospheric aerosols. Profiles of scattering ratio have been obtained since November 1989. Meanwhile, an Xe-Cl laser (308 nm wavelength) was assembled to allow the lidar to make measurements of vertical ozone distributions.

Zhou, Jun↗

Evaluation of the Impacts of Biomass Burning Aerosols on the NASA GEOS Sub-Seasonal Climate Forecasts

Emission sources of trace gases and aerosol particles in the South American (SA)and African (Af) continents have a strong seasonal and space variability associated with the extensive vegetation fires activities. In both continents, during the austral winter, the fires affect mainly tropical forest and savannah-type biomes and are mostly associated with deforestation and agricultural/pasture land management. Smoke aerosol particles, on average, contribute to at least 90% of the total aerosol optical depth (AOD) in the visible spectrum in the case of the South America regional smoke. Smoke aerosols also act as cloud condensation nuclei affecting cloud microphysics properties and therefore, changing the radiation budget, hydrological cycle and global circulation patterns over disturbed areas (Kaufman, 1995; Rosenfeld, 1999; Andreae,et al., 2004; Koren et al., 2004, Zhang, 2008; Ott et al., 2010; Randles et al., 2013). This study aims to evaluate and quantify the impact of including a comprehensive emission field of biomass burning aerosol on the performance of a seasonal climate forecast system, not only regarding the AOD itself but mainly on the meteorological state variable (e.g., precipitation and temperature). To address the questions put above, we designed two numerical experiments: 1- named"AERO_CTL" which applies the Quick Fire Emissions Dataset (QFED) emissions estimated with intra-diurnal variation (hereafter, BBE), and 2- named "AERO_CLM" where the sourcee mission is based on a climatology of the QFED emissions, with only monthly variation(hereafter, BBCLIM). Hindcast simulations were produced using the Goddard Earth ObservingSystem global circulation model, version 5, sub-seasonal to seasonal (GEOS5-S2S) system with a nominal spatial resolution of 56km (Rienecker et al., 2008). In both experiments, the aerosol feedbacks from cloud developments and radiation interactions were accounted. The two experiments consisted of 4 members each and ran from June to November spanning over the years 2000 to 2015. Model performance was evaluated by calculating statistical metrics on the mean area of SA and Af. Our results demonstrated that the skill model in predicting AOD is significantly improve when BBE source emission is applied over SA, but not over the Afcontinent. Over SA, the correlation between the AERO_CTL model configuration and MERRA-2 is 0.93 (R2= 0.86, RMS=0.02, BIAS=0.01), while the AERO_CLM model presents a value of0.81 (R2= 0.65, RMS=0.04, BIAS=0.06). However, the AERO_CTL experiment better represents the inter-annual variability of the AOS in both regions. The gain of the skill in predicting the AOD by the AERO_CTL experiment is also seen in some meteorological variables. We observed an increase in the model skill in predicting the 2-meter temperature and precipitation of up to 0.3 for the AERO_CTL experiment in comparison to the AERO_CLM. AERO_CLM. According to the analyzed hindcast, we inferred that representing the BBE more realistically implies in a significant gain of skills in the seasonal climate forecasting over SA and Af continents.

Aerosol↗

Clouds, aerosols, and photochemistry in the Jovian atmosphere

An assessment is made of the development status of concepts for cloud and aerosol compositions, vertical and horizontal distributions, and microphysical properties, in the Jovian upper troposphere and stratosphere. Attention is given to several key photochemical species' relationships to aerosol formation as well as their transport process implications, treating photochemistry in the context of comparative planetology and noting differences and similarities among the outer planet atmospheres; since this approach emphasizes observational data, a variegated assortment of ground-based and spacecraft observations is assembled. Current views on the tropospheric distribution of clouds are challenged, and a rationale is presented for alternative accounts.

West, R. A.↗

Development and Testing of the New Surface LER Climatology for OMI UV Aerosol Retrievals

Ozone Monitoring Instrument (OMI) onboard Aura satellite retrieved aerosols properties using UV part of solar spectrum. The OMI near UV aerosol algorithm (OMAERUV) is a global inversion scheme which retrieves aerosol properties both over ocean and land. The current version of the algorithm makes use of TOMS derived Lambertian Equivalent Reflectance (LER) climatology. A new monthly climatology of surface LER at 354 and 388 nm have been developed. This will replace TOMS LER (380 nm and 354nm) climatology in OMI near UV aerosol retrieval algorithm. The main objectives of this study is to produce high resolution (quarter degree) surface LER sets as compared to existing one degree TOMS surface LERs, to product instrument and wavelength consistent surface climatology. Nine years of OMI observations have been used to derive monthly climatology of surface LER. MODIS derived aerosol optical depth (AOD) have been used to make aerosol corrections on OMI wavelengths. MODIS derived BRDF adjusted reflectance product has been also used to capture seasonal changes in the surface characteristics. Finally spatial and temporal averaging techniques have been used to fill the gaps around the globes, especially in the regions with consistent cloud cover such as Amazon. After implementation of new surface data in the research version of algorithm, comparisons of AOD and single scattering albedo (SSA) have been performed over global AERONET sites for year 2007. Preliminary results shows improvements in AOD retrievals globally but more significance improvement were observed over desert and bright locations. We will present methodology of deriving surface data sets and will discuss the observed changes in retrieved aerosol properties with respect to reference AERONET measurements.

Aerosol↗