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At least 217 records · Page 12

Southern Hemisphere Lidar Measurements of the Aerosol Clouds from Mt. Pinatubo and Mt. Hudson

On 19 Jul., 1991, during tests to determine the ability of the newly-modified CSIRO Ns:YAG lidar to measure signals from the stratosphere before the arrival of dust from the eruption of Mt. Pinatubo, a strongly scattering layer was detected at an altitude of 2 km. That evening, the spectacular sunset and twilight were typical of volcanically disturbed conditions. Lidar measurements at 532 nm were made between 1400 and 1500 EST (0400-0500 UT) on 19 Jul. through broken cloud. Approximately 3800 laser firings were averaged in 256 shot blocks. These and subsequent data have been analyzed to produce profiles of aerosol volume backscatter function and scattering ratio. Clouds again prevented a clear view of the twilights on the next two nights, although there was some evidence for an enhanced glow. The evidence suggested that the aerosol layer had disappeared. An explanation for this disappearance and the earlier than expected arrival of the layer over Melbourne was required. Nimbus 7 TOMS data for 23 Jun. showed that the SO2 from the eruption had extended at least 11000 km to the west and that the southern boundary of the cloud had reached 15 degrees S just 8 days after the climactic eruption. It can be assumed that this cloud also contained dust and sulphuric acid aerosol. It was proposed that a section had then been broken away from the main cloud and carried south by a large scale eddy between the low latitude easterlies and the strong mid-latitude westerlies which finally carried the aerosol cloud over southern Australia. Accompanying 30 mb wind data showed a counter clockwise circulation, responsible for the transport, located in the South Atlantic Ocean.

Young, Stuart A.↗

NASA's Decadal Survey Observing System for Aerosols, Clouds, Convection, and Precipitation (ACCP): The Atmosphere Observing System

The observing system to be described today arose from NASA’s recent Earth Science Decadal Survey. In 2018, NASA funded a 2.5-year study to identify key science requirements and potential architecture solutions to address 2 of the 5 decadal survey recommended designated observables: aerosols and clouds, convection, and precipitation (or ACCP). A set of architectures was recommended to NASA HQ earlier this year, leading to a new mission that we have named the Atmosphere Observing System, or AOS, although that name may eventually change. In this presentation, when I refer to ACCP, I am speaking about the recent 2-year study and when I refer to AOS I am speaking of the new mission currently in its mission concept development phase. I will provide some background on the decadal survey and how it led to the ACCP and AOS goals. I will describe the architecture that was recommended to NASA HQ and summarize current activities as we work toward our mission concept review next spring.

Scott A. Braun↗

Lidar-Polarimeter Retrieval OSSEs using a Nature Run in Support of NASA's Aerosols, Clouds, Convection and Precipitation (ACCP) Study

The 2017 Decadal Survey (DS) highlighted Earth System Science themes, science and application questions, and several high priority objectives that have led to the inclusion of Aerosols (A) and Clouds-Convection-Precipitation (CCP) as Designated Observables (DOs). On June 1, 2018, several NASA centers (GSFC, LaRC, JPL, MSFC, GRC and ARC) submitted a joint Study Plan to the NASA Earth Science Division for the Aerosol (A) and Cloud, Convection, and Precipitation (CCP) Pre-formulation Study (ACCP). The DS and the ACCP team recognized the science merit in combining the A and CCP DOs for both enhancing the ability to address a number of science objectives and also to provide an expanded capability to address additional objectives beyond those addressed by individual DOs. A critical element of the ACCP observing strategy is to make extensive use of new passive and active sensors as well as of the so-called Program-of-Record (PoR), complemented by a fully integrated sub-orbital component. Central to this observing system design is the adoption of a Value Framework in which quantitative assessment of the science benefits of space- and air-borne assets is a key element. Given pre-defined ACCP science objectives and geophysical variables with desired accuracies, ACCP relies on a spectrum of Observing System Simulation Experiments (OSSEs) aimed at addressing pixel level retrieval uncertainties and sampling trade-offs. In this talk we will discuss a subset of Retrieval OSSEs being considered for ACCP, namely, synergistic lidar-polarimeter retrievals based on observation simulations from the GEOS-5 Nature Run (G5NR). Starting with aerosol states from the GEOS-5 Nature Run (G5NR) sampled along specific satellite orbits, we simulate polarized radiances at the desired polarimeter wavelengths with the Vector Linearized Direct Ordinate Radiative Transfer (VLIDORT) model, alongside the lidar signal for the relevant lidars with realistic error characterization. Next, inversions are performed with the Generalized Retrieval of Aerosol and Surface Properties (GRASP) system and the accuracy of the retrieved geophysical variables are assessed. In this presentation we will highlight results for key architectures being considered for ACCP with emphasis on geophysical variables of particular relevance to ACCP’s aerosol science objectives.

A Da Silva↗

SAGE II observations of a previously unreported stratospheric volcanic aerosol cloud in the northern polar summer of 1990

Analysis of aerosol extinction profiles obtained by the spaceborne SAGE II sensor reveals that there was an anomalous increase of aerosol extinction below 18.5 km at latitudes poleward of 50 deg N from July 28 to September 9, 1990. This widespread increase of aerosol extinction in the lower stratosphere was apparently due to a remote high-latitude volcanic eruption that has not been reported to date. The increase in stratospheric optical depth in the northern polar region was about 50% in August and had diminished by October 1990. This eruption caused an increase in stratospheric aerosol mass of about 0.33 x 10(exp 5) tons, assuming the aerosol was composed of sulfuric acid and water.

Yue, Glenn K.↗

Aerosol, Cloud and Trace Gas Observations Derived from Airborne Hyperspectral Radiance and Direct Beam Measurements in Recent Field Campaigns

The AERONET (AErosol RObotic NETwork) ground-based suite of sunphotometers provides measurements of spectral aerosol optical depth (AOD), precipitable water and spectral sky radiance, which can be inverted to retrieve aerosol microphysical properties that are critical to assessments of aerosol-climate interactions. Because of data quality criteria and sampling constraints, there are significant limitations to the temporal and spatial coverage of AERONET data and their representativeness for global aerosol conditions. The 4STAR (Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research) instrument, jointly developed by NASA Ames and PNNL with NASA Goddard collaboration, combines airborne sun tracking and AERONET-like sky scanning with spectroscopic detection. Being an airborne instrument, 4STAR has the potential to fill gaps in the AERONET data set. Dunagan et al. [2013] present results establishing the performance of the instrument, along with calibration, engineering flight test, and preliminary scientific field data. The 4STAR instrument operated successfully in the SEAC4RS [Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys] experiment in Aug./Sep. 2013 aboard the NASA DC-8 and in the DoE [Department of Energy]-sponsored TCAP [Two Column Aerosol Project, July 2012 & Feb. 2013] experiment aboard the DoE G-1 aircraft (Shinozuka et al., 2013), and acquired a wealth of data in support of mission objectives on all SEAC4RS and TCAP research flights. 4STAR provided direct beam measurements of hyperspectral AOD, columnar trace gas retrievals (H2O, O3, NO2; Segal-Rosenheimer et al., 2014), and the first ever airborne hyperspectral sky radiance scans, which can be inverted to yield the same products as AERONET ground-based observations. In addition, 4STAR measured zenith radiances underneath cloud decks for retrievals of cloud optical depth and effective diameter. In this presentation, we provide an overview of the new 4STAR capabilities for airborne field campaigns, with an emphasis on comparisons between 4STAR and AERONET sky radiances, and retrievals of aerosol microphysical properties based on sky radiance measurements, column trace gas amounts from spectral direct beam measurements and cloud property retrievals from zenith mode observations for a few select case studies in the SEAC4RS and TCAP experiments. We summarize the aerosol, trace gas, cloud and airmass characterization studies made possible by the combined 4STAR direct beam, and sky/zenith radiance observations.

Aerosol-Climate↗

Dust Aerosol, Clouds, and the Atmospheric Optical Depth Record over 5 Mars Years of the Mars Exploration Rover Mission

Dust aerosol plays a fundamental role in the behavior and evolution of the Martian atmosphere. The first five Mars years of Mars Exploration Rover data provide an unprecedented record of the dust load at two sites. This record is useful for characterization of the atmosphere at the sites and as ground truth for orbital observations. Atmospheric extinction optical depths have been derived from solar images after calibration and correction for time-varying dust that has accumulated on the camera windows. The record includes local, regional, and globally extensive dust storms. Comparison with contemporaneous thermal infrared data suggests significant variation in the size of the dust aerosols, with a 1 micrometer effective radius during northern summer and a 2 micrometer effective radius at the onset of a dust lifting event. The solar longitude (L (sub s)) 20-136 degrees period is also characterized by the presence of cirriform clouds at the Opportunity site, especially near LS = 50 and 115 degrees. In addition to water ice clouds, a water ice haze may also be present, and carbon dioxide clouds may be present early in the season. Variations in dust opacity are important to the energy balance of each site, and work with seasonal variations in insolation to control dust devil frequency at the Spirit site.

Atmospheric depth↗

Cloud, Aerosol, and Radiative Properties Over the Western North Atlantic Ocean

This study examines the atmospheric properties of weather states (WSs) derived from the International Satellite Cloud Climatology Project (ISCCP) over the Western North Atlantic Ocean. In particular, radiation and aerosol data corresponding to two sites in the study domain, Pennsylvania State University and Bermuda, were examined to characterize the atmospheric properties of the various satellite-derived WSs. At both sites, the fair weather WS was most prevalent, followed by the cirrus WS. Differences in the seasonality of the various WSs were observed at the two sites. Fractional sky cover and effective shortwave cloud transmissivity derived from ground-based radiation measurements were able to capture differences among the satellite-derived WSs. Speciated aerosol optical thicknesses (AOT) from the Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2) were used to investigate potential differences in aerosol properties among the WSs. The clear sky WS exhibited below-average seasonal values of AOT at both sites year-round, as well as relatively high rates of occurrence with low AOT events. In addition, the clear sky WS showed above-average contributions from dust and black carbon to the total AOT year-round. Finally, transitions between various WSs were examined under low, high, and mid-range AOT conditions. The most common pathway was for the WSs to remain in the same state after a 3 hr interval. Some WSs, such as midlatitude storms, deep convection, middle top, and shallow cumulus, were more prevalent as ending states under high AOT conditions. This work motivates examining differences in aerosol properties between WSs in other regions.

54 ENVIRONMENTAL SCIENCES↗

Synthesis of aerosol-cloud interactions over the southeast Atlantic throughout the seasonal cycle (Final Technical Report)

An analysis of the aerosol compositional, physical and optical datasets towards understanding why the single‐scattering‐albedo of smoke is so much lower over the southeast Atlantic than elsewhere, in particular the northern hemisphere. This includes data from the complementary NASA ORACLES aircraft campaign, which sampled closer to the African coast. The first analysis resulting from this prong of research was published earlier this year (Dobracki et al., 2023, ACP) and focused more on the free-tropospheric biomass burning aerosol (BBA). We primarily attributed the low SSA to a high number/mass fraction of black carbon, ranging from 15 to 40% of the total aerosol. We are further able to use other literature, the modified combustion efficiency, and the black carbon and carbon monoxide values to highlight a common source in dry, flame-efficient burning conditions of grasses. Condensation and coagulation of smaller aerosol particles onto the larger black carbon aerosols can also increased the SSA as the aerosol ages from 4 to 5 days. A comparison to data gathered over Ascension Island during the UK CLARIFY aircraft campaign indicates an organic aerosol loss relative to black carbon of about 50%. This is high compared to findings from other campaigns.

54 ENVIRONMENTAL SCIENCES↗

Observations of Aerosol, Cloud, Turbulence, and Radiation Properties at the Top of the Marine Boundary Layer over the Eastern North Atlantic Ocean: The ACORES Campaign

We report on the Azores Stratocumulus Measurements of Radiation, Turbulence and Aerosols (ACORES) campaign, which took place around Graciosa and Pico Islands/Azores in July 2017. The main objective was to investigate the vertical distribution of aerosol particles, stratocumulus microphysical and radiative properties, and turbulence parameters in the eastern North Atlantic. The vertical exchange of mass, momentum, and energy between the free troposphere (FT) and the cloudy marine boundary layer (MBL) was explored over a range of scales from submeters to kilometers. To cover these spatial scales with appropriate measurements, helicopter-borne observations with unprecedented high resolution were realized using the Airborne Cloud Turbulence Observation System (ACTOS) and Spectral Modular Airborne Radiation Measurement System–Helicopter-Borne Observations (SMART-HELIOS) instrumental payloads. Here, the helicopter-borne observations were combined with ground-based aerosol measurements collected at two continuously running field stations on Pico Mountain (2,225 m above sea level, in the FT), and at the Atmospheric Radiation Measurement (ARM) station on Graciosa (at sea level). First findings from the ACORES observations we are discussing in the paper are as follows: (i) we have observed a high variability of the turbulent cloud-top structure on horizontal scales below 100 m with local temperature gradients of up to 4 K over less than 1 m vertical distance, (ii) we have collected strictly collocated radiation measurements supporting the relevance of small-scale processes by revealing significant inhomogeneities in cloud-top brightness temperature to scales well below 100 m, and (iii) we have concluded that aerosol properties are completely different in the MBL and FT with often-complex stratification and frequently observed burst-like new particle formation.

54 ENVIRONMENTAL SCIENCES↗

Cloud Aerosol LIDAR Infrared Pathfinder Satellite Observations (CALIPSO) - Data Management - Data Products Catalog V4.94

The CALIPSO V2.00 Lidar Level 2 Polar Stratospheric Cloud data product is an updated version of an already order-able dat set. The changes were signed off by the CALIPSO Configuration Control Board, versioned, and the code uploaded to a code repository. There is no ITAR/SBU data or code associated with this product. Data will be publicly order-able at the NASA LaRC Atmospheric Sciences Data Center (ASDC). All documentation and web sites will be made public once the data product is released. The data is in HDF4 format and will be generated for majority of the mission (June 2006 - March 2021). The attached Data Products Catalog (v4.94) describes this new product in section 2.14, pp 115- 119.

Mark Vaughan↗

Direct numerical simulation of turbulent dispersion of evaporative aerosol clouds produced by an intense expiratory event

Airborne particles are a major route for transmission of COVID-19 and many other infectious diseases. When a person talks, sings, coughs, or sneezes, nasal and throat secretions are spewed into the air. After a short initial fragmentation stage, the expelled material is mostly composed of spherical particles of different sizes. While the dynamics of the largest droplets are dominated by gravitational effects, the smaller aerosol particles, mostly transported by means of hydrodynamic drag, form clouds that can remain afloat for long times. In subsaturated air environments, the dependence of pathogen-laden particle dispersion on their size is complicated due to evaporation of the aqueous fraction. Particle dynamics can significantly change when ambient conditions favor rapid evaporation rates that result in a transition from buoyancyto-drag dominated dispersion regimes. To investigate the effect of particle size and evaporation on pathogen-laden cloud evolution, a direct numerical simulation of a mild cough was coupled with an evaporative Lagrangian particle advection model. The results suggest that while the dispersion of cough particles in the tails of the size distribution are unlikely to be disrupted by evaporative effects, preferential aerosol diameters (30-40 μm) may exhibit significant increases in the residence time and horizontal range under typical ambient conditions. Using estimations of the viral concentration in the spewed fluid and the number of ejected particles in a typical respiratory event, we obtained a map of viral load per volume of air at the end of the cough and the number of virus copies per inhalation in the emitter vicinity.

60 APPLIED LIFE SCIENCES↗

Ozone within the El Chichon aerosol cloud inferred from solar backscatter ultraviolet continuous-scan measurements

Large amounts of SO2 injected into the stratosphere by the El Chichon volcanic eruption greatly enhanced the sulfuric acid aerosol loading. According to laboratory studies, the increase in aerosol surface area would lead to a loss of ozone. Radiation measurements from the solar backscatter ultraviolet spectroradiometer are used to probe the absorbing and scattering properties of the stratosphere after the eruption. The backscattered radiation is enhanced for wavelengths greater than 290 nm, with a peak at about 302 nm. The enhancements associated with aerosol backscattering and ozone change can be separated. A decrease in column ozone of 8 to 30 Dobson units was deduced within the aerosol layer at an altitude between 20 and 30 km following the month of the eruption.

Wen, Guoyong↗

The NASA Aerosols, Clouds, Convection, and Precipitation (ACCP) Observing System

NASA’s new Earth System Observatory (ESO) will provide key information related to understanding climate change processes, mitigating natural hazards, fighting forest fires, and improving real-time agricultural processes. The ACCP observing system will address two of the five major focus areas: aerosols, which determine air quality and affect the global energy balance, a key source of uncertainty in predicting climate change; and clouds, convection, and precipitation, whose processes are also a large source of uncertainty in future projections of climate change as well as predictions of severe weather. ACCP, currently in the concept investigation phase, is made up of two projects, one in an inclined orbit and the other in a polar orbit, with both projects addressing synergistic A and CCP science. Suborbital science is also a significant element of ACCP. This talk will describe the science objectives of ACCP and their relationship to the 2017 NASA Earth Science Decadal Survey as well as summarize the orbital architecture and major science activities during the concept investigation phase.

Scott Braun↗

Monitoring the 2022 Hunga Tonga-Hunga Ha'apai Aerosol Cloud Using Space-Based Observations

- We will analyze the volcanic plume progression, spread and properties using space-based observations - OMPS LP, SAGE III/ISS, CALIPSO, TROPOMI - OMPS LP and SAGE III/ISS are limb instruments that measure the aerosol vertical profiles globally, while CALIPSO is a LIDAR that measures the backscatter and depolarization ratio of the aerosol profiles. -TROPOMI is a UV instrument that measures SO2 and absorbing aerosol total column - Volcanic plume in the upper stratosphere - The main plume in middle stratosphere - Volcanic aerosol transport to SH/NH - Volcanic aerosol optical properties

Atmospheric Science↗

Remote Sensing of Cloud, Aerosol, and Water Vapor Properties from MODIS

MODIS is an earth-viewing cross-track scanning spectroradiometer launched on the Terra satellite in December 1999. MODIS scans a swath width sufficient to provide nearly complete global coverage every two days from a polar orbiting, sun-synchronous, platform at an altitude of 705 kilometers, and provides images in 36 spectral bands between 0.415 and 14.235 micrometers with spatial resolutions of 250 meters (2 bands), 500 meters (5 bands) and 1000 meters (29 bands). These bands have been carefully selected to enable advanced studies of land, ocean, and atmospheric processes. In this presentation we review the comprehensive set of remote sensing algorithms that have been developed for the remote sensing of atmospheric properties using MODIS data, placing primary emphasis on the principal atmospheric applications of (i) developing a cloud mask for distinguishing clear sky from clouds, (ii) retrieving global cloud radiative and microphysical properties, including cloud top pressure and temperature, effective emissivity, cloud optical thickness, thermodynamic phase, and effective radius, (iii) monitoring tropospheric aerosol optical thickness over the land and ocean and aerosol size distribution over the ocean, (iv) determining atmospheric profiles of moisture and temperature, and (v) estimating column water amount. The physical principles behind the determination of each of these atmospheric products will be described, together with an example of their application using MODIS observations. All products are archived into two categories: pixel-level retrievals (referred to as Level-2 products) and global gridded products at a latitude and longitude resolution of 1 degree (Level-3 products). An overview of the MODIS atmosphere algorithms and products, status, validation activities, and early level-2 and -3 results will be presented.

King, Michael D.↗