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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 217 records · Page 12
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Non-Equilibrium in a Dust-Forming Low-Temperature Plasma: A CARS Study

Dust-forming low-temperature plasmas are versatile systems for the production of nanoparticles with tunable functionalities. While attractive from a materials processing point of view, these systems are inherently complex, with several plasma-induced phenomena determining the properties of the produced materials. Here, we characterize a carbon nanoparticle-forming plasma using coherent anti-Stokes Raman spectroscopy (CARS), with the primary goal of measuring gas temperature. While gas temperature is typically assumed to be at or slightly above room temperature in these reactors, we measure gas temperatures exceeding 1000 K under typical process conditions. We find a correlation between the gas temperature and the nanoparticle yield, suggesting that the particle nucleation and growth process releases energy within the reaction volume, leading to significant gas heating. In addition, we find that the relaxation of vibrationally excited species at the particle surfaces is a major contributor to their heating. In conclusion, these results underscore the complexity of these systems and the need for their more in-depth characterization using advanced techniques such as CARS.

Basic Plasma Phenomena and Gas Discharges↗
DOE OSTI2025

Initiation of dusting corrosion in high-temperature alloys under CO exposure

Carbon monoxide is commonly encountered in energy systems, yet its reactivity with structural alloys—critical heat-resistant components in these systems—has been largely overlooked compared to the well-documented effects of oxidizing gases. In contrast, we demonstrate the high-temperature reaction of CO with NiAl using in-situ low-energy electron microscopy and X-ray photoemission electron microscopy. Our results show that CO dissociates into atomic oxygen and carbon, resulting in two concurrent reactions: selective oxidation of aluminum to form Al 2 O 3 and the initiation of dusting corrosion through carbon dissolution into the alloy and subsequent carbon deposition on the surface. These reactions produce spatially distinct surface products, preventing the formation of a continuous protective Al oxide layer. These results reveal a preference for the dissociative pathway of CO over the classic Boudouard disproportionation reaction that forms CO 2 . These insights not only advance our understanding of CO-induced alloy degradation but also highlight the practical implications for managing alloy stability and optimizing catalysis in carbon-rich environments, such as those in petrochemical processing and hydrocarbon combustion.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Search for meteoritic GEMS II: Comparison of inclusions in amorphous silicates from the Paris chondrite and from anhydrous chondritic interplanetary dust particles

Amorphous silicates containing abundant nano-inclusions have been reported in the Paris CM chondrite (Leroux et al., 2015). They have chemical and morphological similarities to glass with embedded metal and sulfides (GEMS) found in interplanetary dust particles (IDPs) and micrometeorites believed to originate from comets. We used scanning transmission electron microscopy (STEM) with energy-dispersive X-ray spectroscopy (EDS) and nanodiffraction to study the chemistry and mineralogy of these inclusions in order to understand the origin of the GEMS-like material in Paris and its possible relationships to other materials found in primitive chondritic materials including IDP GEMS. EDS and diffraction analyses indicate compositional and mineralogical differences between the nanophase inclusions in cometary GEMS and Paris GEMS-like material. Metal inclusions are notably absent within Paris amorphous silicate. Ni-rich sulfides, including pentlandite, are common in even the least altered matrix material of Paris, while they are absent in GEMS-bearing IDPs and Ultracarbonaceous Antarctic Micrometeorites (UCAMMs). From examination of the inclusions, we cannot yet confirm or refute the possibility that GEMS-like material in Paris is related to cometary GEMS. The distinct compositions and mineralogy of the Paris material may be due to aqueous alteration of cometary GEMS precursors, but they may also denote an independent origin for meteoritic GEMS-like assemblages.

58 GEOSCIENCES↗
DOE OSTI2022

How the Great Plains Dust Bowl drought spread heat extremes around the Northern Hemisphere

Abstract Extraordinary heat extremes occurred in the 1930s in areas of the Northern Hemisphere far from the record setting heat over the US associated with the Great Plains Dust Bowl drought. A climate model sensitivity experiment is used to identify a new mechanism involving a warm season circumglobal atmospheric teleconnection pattern that spread heat extremes over far-flung areas of the Northern Hemisphere arising from the intense heating over the desiccated Great Plains themselves. It has only been in the twenty-first century that human populations in these regions of the Northern Hemisphere have experienced heat extremes comparable to the 1930s. This demonstrates that humans influenced Northern Hemisphere temperature and heat extremes through disastrous and unprecedented regional land use practices over the Great Plains, and points to the possibility that future intense regional droughts could affect heat extremes on hemispheric scales.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Spin–orbit torques in structures with asymmetric dusting layers

Current-induced spin–orbit torques (SOTs) in heavy metal/ferromagnet heterostructures have emerged as an efficient method for magnetization switching with applications in nonvolatile magnetic memory and logic devices. However, experimental realization of SOT switching of perpendicular magnetization requires an additional inversion symmetry breaking, calling for modifications of the conventional SOT heterostructures. In this work, we study SOTs and deterministic switching of perpendicular magnetization by inserting different asymmetric dusting layers at the heavy metal/ferromagnet interface. Similar to the previous works with lateral structural asymmetry, we study the emergence of current-induced perpendicular effective magnetic fields (H z eff ). By examining three different material combinations of heavy metal/dusting layers (W/IrMn, Pt/IrMn, and W/Ta), we shed light on the origins of H z eff ; we show that H z eff is generically created in all the studied asymmetric structures, has a close correlation with the interfacial magnetic anisotropy, and is independent of the signs of spin Hall angles of the materials. Furthermore, we show that the induction of H z eff enables field-free deterministic SOT switching of perpendicular magnetization. Our results can be used in designing SOT heterostructures for practical applications in nonvolatile technologies.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Mitigating dust particle contamination in an afterglow plasma by controlled lifting with a DC electric field

Abstract Particle contamination due to plasma processing motivates the design of a method of electrically lifting particles in a time interval after a plasma’s power is turned off. Small solid dust particles have electric charges that are not frozen until a late stage of the plasma afterglow. Beyond that time, before they fall to a surface below and cause defects, particles can be lifted in a controlled manner by applying an appropriate direct-current (DC) electric field, as we demonstrate experimentally. A few milliseconds after an argon plasma’s capacitively coupled radio-frequency power is switched off, a vertical DC electric field is applied. Thereafter, video imaging shows that the falling of the particles is slowed or stopped altogether, depending on the magnitude of the upward electric force.

Physics↗
DOE OSTI2023

Synchronization of dust acoustic waves in a forced Korteweg–de Vries–Burgers model

The synchronization of dust acoustic waves to an external periodic source is studied in the framework of a driven Korteweg–de Vries–Burgers equation that takes into account the appropriate nonlinear and dispersive nature of low-frequency waves in a dusty plasma medium. For a spatiotemporally varying source term, the system is shown to demonstrate harmonic (1:1) and superharmonic (1:2) synchronized states. Here, the existence domains of these states are delineated in the form of Arnold tongue diagrams in the parametric space of the forcing amplitude and forcing frequency and their resemblance to some past experimental results is discussed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Doppler Boosted Dust Emission and Cosmic Infrared Background–Galaxy Cross-Correlations: A New Probe of Cosmology and Astrophysics

We identify a new cosmological signal, the Doppler-boosted Cosmic Infrared Background (DB-CIB), arising from the peculiar motion of the galaxies whose thermal dust emission source the cosmic infrared background (CIB). This new observable is an independent probe of the cosmic velocity field, highly analogous to the well-known kinematic Sunyaev-Zel'dovich (KSZ) effect. Interestingly, DB-CIB does not suffer from the "KSZ optical depth degeneracy", making it immune from the complex astrophysics of galaxy formation. We forecast that the DB CIB effect is detectable in the cross-correlation of CCAT-Prime and DESI-like experiments. Here,we show that it also acts as a new CMB foreground which can bias future KSZ cross-correlations, if not properly accounted for.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Uranium Dust Cloud Combustion: Burning Characteristics and Absorption Spectroscopy Measurements

This study characterized uranium metal dust cloud combustion using absorption spectroscopy, imaging, and broadband emission measurements. Other metals were similarly combusted to establish correlations between results from this study and those found in the literature. It was determined that the burn temperature of uranium was limited to the volatilization temperature of uranium dioxide. Combustion behavior was similar to that of other refractory metals in terms of burn time and the observation of exploding particle behavior.

42 ENGINEERING↗
DOE OSTI2020

Final Fugitive Dust Control NOV Causal Report

On June 30, 2020, a Notice of Violation (NOV) was issued by the City of Albuquerque (COA) Environmental Health Department, Air Quality Program. The NOV identified two violations of New Mexico Administrative Code (NMAC) 20.11.20, Fugitive Dust Control, stemming from an August 30, 2019 inspection of the construction site at Sandia/New Mexico (SNL/NM) Building 812. After the August 30 inspection, a Post-Instruction Notification (PIN) was issued to the SNL Construction Facilities Manager. The PIN was acknowledged by Department 4722 and sent to the COA on September 13, 2020 via email. The PIN "Comply by" date was September 13, 2019 was transmitted by National Nuclear Security Administration/ Sandia Field Office (NNSA/SFO) to COA offices on November 12, 2019. The PIN response was 48 business days past due for various reasons which were explored during the causal analysis.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Fire, dust, air and water: Improving aerosol biogeochemistry interactions in ACME. Final report

Aerosol-biogeochemistry interactions will have important consequences for human health, ecosystem services, and climate feedbacks over the next several decades. In this proposal we seek to link how human activities on land, including direct industrial emissions and landscape fires, impact the atmosphere and the biogeochemistry of the ocean and land. Our overall goal was to complement existing work at DOE labs to improve the capability and performance of the E3SM model in short-term, high-resolution projections of climate. Projections of ocean uptake of anthropogenic carbon are highly dependent on the details of the ocean physical and biogeochemistry parameterizations. Potentially equally important are the estimates of increases in iron and soluble nitrogen deposition in aerosols to the open ocean, but there are substantial uncertainties in these feedbacks. The E3SM land model simulates natural and anthropogenic fires, but improvement is needed to more accurately simulate fire responses to climate variability as well as fire contributions to terrestrial climate feedbacks. This proposal addressed four of the six priorities within the ACME/E3SM call by improving the representation of fire, industrial combustion sources, and desert dust and adding iron and soluble iron to the atmospheric chemistry (1). Our work focused on improving ocean biogeochemistry and the response of the oceans to anthropogenic atmospheric iron and nitrogen (3). We also improved the representation of land disturbance on fires and fire mediated carbon cycle feedbacks in the land model (4). Finally we had planned to couple the land, atmosphere and ocean biogeochemical systems (6) and explore how this coupling changes the feedbacks in the climate system. Our work under this proposal was separated into the following 5 tasks: i) improve representation of fire dynamics in both boreal and tropical ecosystems, ii) improve estimates of industrial emissions of iron and phosphorus, iii) improve representation of atmospheric iron, phosphorus and nitrogen transport, chemistry and deposition, iv) improve representation of iron, phosphorus and nitrogen deposition impacts on ocean biogeochemistry, and v) couple emissions into atmosphere, to deposition onto land and ocean biogeochemistry. For all 5 tasks, we conducted offline experiments of the historical period to enable comparison with available aerosol and land surface observations. We had planned to conduct fully coupled simulations, however, these will be conducted as part of the coupling in version 3 and 4 of the E3SM model, and thus have not been completed.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

A glimpse of stars the size of dust particles

The Nuclear Imaging System (NIS) is an important diagnostic tool used to study nuclear fusion implosions at a research facility in California. There a capsule the size of a flea is compressed until it reaches the size of a speck of dust. As the capsule collapses on itself and ignites under extreme temperature and pressure, NIS detects particles emitted from that process at a scale that would correspond to watching a 32-inch TV screen from 100 miles away. My work involves taking snapshots of one of the most minuscule, fleeting and amazing experiments on Earth in order to ensure the safety and reliability of the US nuclear stockpile and get closer to developing a new form of clean energy.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Synthesis of Si-Fe Chondrule-like Dust Analogues in RF Discharge Plasmas

Chondrules are tiny particles that occur in stony meteorites and are considered as the building blocks of early asteroids and planets. It is believed that they were formed by the fast heating of the dust in the solar nebula. To date, there is no lab-scale experimental study of the formation of chondrules from the initial gas phase precursors following fast heating and crystallisation. The motivation of this work is a pre-trial study of the formation of chnodrule-like particles. The formation of meteorites in the space environment is associated with the aggregation of small particles or molecular clouds under the influence of shock waves or high-energy gas discharges in the solar nebula. In this work, the properties of product formation at the nanoscale-level were investigated using different feedstock materials which are the dominant elements in the meteorite. The structural and morphological properties of the synthesised Si-Fe nanomaterials were analysed by scanning/transmission electron microscopy (SEM/TEM), and chemical composition was analysed by X-ray energy-dispersive spectroscopy (EDS). The identification of crystalline phases was carried out by X-ray diffraction (XRD), whereas the presence of an Fe-Si system in the synthesised particles was demonstrated by Mössbauer spectroscopy. The obtained materials were exposed to the relatively high-energy pulsed plasma beam on the substrate with the aim to emulate the possible fast heating and melting of the formed nanoparticles. The formation steps of growing synthetic (engineered) chondro-like particles and nanostructures in laboratory conditions is discussed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Gas and Cosmic-Ray Properties in the MBM 53, 54, and 55 Molecular Clouds and the Pegasus Loops Revealed by H i Line Profiles, Dust, and Gamma-Ray Data

In studying the interstellar medium (ISM) and Galactic cosmic rays (CRs), uncertainty of the interstellar gas density has always been an issue. To overcome this difficulty, we used a component decomposition of the 21 cm H i emission line and used the resulting gas maps in an analysis of γ-ray data obtained by the Fermi Large Area Telescope (LAT) for the MBM 53, 54, and 55 molecular clouds and the Pegasus loop. We decomposed the ISM gas into intermediate-velocity clouds, narrow-line and optically thick H i, broad-line and optically thin H i, CO-bright H 2 , and CO-dark H 2 using detailed correlations with the H i line profiles from the HI4PI survey, the Planck dust-emission model, and the Fermi-LAT γ-ray data. We found the fractions of the optical depth correction to the H i column density and CO-dark H 2 to be nearly equal. We fitted the CR spectra directly measured at/near the Earth and the measured γ-ray emissivity spectrum simultaneously. We obtained a spectral break in the interstellar proton spectrum at ~7 GeV, and found that the γ-ray emissivity normalization agrees with the AMS-02 proton spectrum within 10%, relaxing the tension with the CR spectra previously claimed.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2026

JWST Observations of Starbursts: Dust Processing in the M82 Superwind

We present JWST MIRI and NIRCam imaging of the inner ∼5 kpc of the M82 superwind at ~ $0''_{.}05 - 0''_{.}375$(∼0.9–6.5 pc) resolution. Targeted filters probe emission from polycyclic aromatic hydrocarbons (PAHs; F335M, F360M, F770W, F1130W) and continuum (F250M, F360M) The images reveal a network of cool wind filaments traced by PAHs. PAH surface brightness declines with the inverse square of distance to the midplane, suggesting that the incident radiation field from the starburst drives the observed PAH intensity out to ±2.5 kpc. The 3.3/11.3 and 3.3/7.7 μm band ratios show uniformity with distance from the starburst, though comparisons with mid-IR dust emission models indicate a modest shift toward larger PAHs. Outside the disk, 11.3/7.7 μm increases moderately, reflecting that PAHs become more neutral with distance from the starburst as they are exposed to a declining radiation field and ionization parameter. Overall, PAHs in the wind are consistent with standard-to-large sizes and standard-to-high ionization states. Including Spitzer and Herschel data, PAH abundance (q PAH ) is set at ∼1% in the starburst and remains unchanging out to ±5 kpc off the disk. This flat q PAH profile suggests that PAHs are shielded from the hot wind, perhaps residing in the surface layers of cool clouds, with possible replenishment from cloud interiors and enrichment of the halo from previous bursts. In this picture, clouds are not dense enough to promote PAH growth, and they likely undergo radiative cooling and mixing with the hot phase to survive the gauntlet for at least ∼20 Myr.

Cronin, Serena A. [University of Maryland, College↗
DOE OSTI2020

Recovery of Cs-137 from Electric Arc Furnace Dust - 20562

The present work proposes the Cs-137 recovery from Electric Arc Furnace Dusts (EAFD) by leaching, in order to reduce the volume of radioactive waste to be managed. Leaching tests were performed on different samples of EAFD contaminated with Cs-137. Two leaching methodologies were tested: dynamic and static using as medium distilled water and in some cases NaOH. The results indicate the possibility of recovering Cs-137 from EAFD using the dynamic method; however, the recovery efficiencies of Cs-137 depend on EAFD's chemical composition. The leachates of Cs-137 were quantitatively adsorbed on exchange resins, showing its great potential to isolate or contain the Cs-137 recovery from EAFD. This study shows the feasible to apply the dynamic leaching methodology to recover Cs-137 from EAFD and the use of ion exchange resins for the isolation of removed Cs-137. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗