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DOE OSTI2021

Self-Cleaning Cathodes for Endurance to Chromium Poisoning

Chromium (Cr) poisoning remains a significant issue in long-term solid oxide fuel cell (SOFC) operation. While the addition of Cr in the interconnect and balance-of-plant (BOP) materials is effective in improving their resistance to oxidation, it also causes the deposition of resistive phases in the air electrode and thus cell performance loss. Previous work has investigated the mitigation of chromium deposition using getters, Cr diffusion resistant coatings, and more chromium-tolerant air electrode materials. However, these mitigation strategies merely postpone the degradation of performance due to Cr poisoning. Additionally, some strategies require the replacement of components, e.g., use of getters. Here we investigated a new, in-situ Cr poisoning mitigation strategy.

30 DIRECT ENERGY CONVERSION↗

DOE OSTI2017

Land quality, sustainable development and environmental degradation in agricultural districts: A computational approach based on entropy indexes

Land Degradation (LD) in socio-environmental systems negatively impacts sustainable development paths. This study proposes a framework to LD evaluation based on indicators of diversification in the spatial distribution of sensitive land. We hypothesize that conditions for spatial heterogeneity in a composite index of land sensitivity are more frequently associated to areas prone to LD than spatial homogeneity. Spatial heterogeneity is supposed to be associated with degraded areas that act as hotspots for future degradation processes. A diachronic analysis (1960–2010) was performed at the Italian agricultural district scale to identify environmental factors associated with spatial heterogeneity in the degree of land sensitivity to degradation based on the Environmentally Sensitive Area Index (ESAI). In 1960, diversification in the level of land sensitivity measured using two common indexes of entropy (Shannon's diversity and Pielou's evenness) increased significantly with the ESAI, indicating a high level of land sensitivity to degradation. In 2010, surface area classified as “critical” to LD was the highest in districts with diversification in the spatial distribution of ESAI values, confirming the hypothesis formulated above. Entropy indexes, based on observed alignment with the concept of LD, constitute a valuable base to inform mitigation strategies against desertification. - Highlights: • Spatial heterogeneity is supposed to be associated with degraded areas. • Entropy indexes can inform mitigation strategies against desertification. • Assessing spatial diversification in the degree of land sensitivity to degradation. • Mediterranean rural areas have an evident diversity in agricultural systems. • A diachronic analysis carried out at the Italian agricultural district scale.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2015

An Innovative Solution to NASA's NEO Impact Threat Mitigation Grand Challenge and Flight Validation Mission Architecture Development

This paper presents the results of a NASA Innovative Advanced Concept (NIAC) Phase 2 study entitled "An Innovative Solution to NASA's Near-Earth Object (NEO) Impact Threat Mitigation Grand Challenge and Flight Validation Mission Architecture Development." This NIAC Phase 2 study was conducted at the Asteroid Deflection Research Center (ADRC) of Iowa State University in 2012-2014. The study objective was to develop an innovative yet practically implementable mitigation strategy for the most probable impact threat of an asteroid or comet with short warning time (< 5 years). The mitigation strategy described in this paper is intended to optimally reduce the severity and catastrophic damage of the NEO impact event, especially when we don't have sufficient warning times for non-disruptive deflection of a hazardous NEO. This paper provides an executive summary of the NIAC Phase 2 study results. Detailed technical descriptions of the study results are provided in a separate final technical report, which can be downloaded from the ADRC website (www.adrc.iastate.edu).

NEO Impact Threat Mitigation↗

DOE OSTI2018

General Equilibrium Analysis of the Cobenefits and Trade-Offs of Carbon Mitigation on Local Industrial Water Use and Pollutants Discharge in China

Carbon mitigation strategies have been developed without sufficient consideration of their impacts on the water system. Here, our study evaluates whether carbon mitigation strategies would decrease or increase local industrial water use and water-related pollutants discharge by using a computable general equilibrium (CGE) model coupled with a water withdrawals and pollutants discharge module in Shenzhen, the fourth largest city in China. To fulfill China’s Nationally Determined Contributions (NDC) targets, Shenzhen’s GDP and welfare losses are projected to be 1.6% and 5.6% in 2030, respectively. The carbon abatement cost will increase from 56 USD/t CO2 in 2020 to 274 USD/t CO2 in 2030. The results reveal that carbon mitigation accelerates local industrial structure upgrading by restricting carbon-, energy-, and water-intensive industries, e.g., natural gas mining, nonmetal, agriculture, food production, and textile sectors. Accordingly, carbon mitigation improves energy use efficiency and decreases 55% of primary energy use in 2030. Meanwhile, it reduces 4% of total industrial water use and 2.2–2.4% of two major pollutants discharge, i.e., CODCr and NH3–N. Carbon mitigation can also decrease petroleum (2.2%) and V-ArOH (0.8%) discharge but has negative impacts on most heavy metal(loid)s pollutants discharge (increased by -0.01% to 4.6%). These negative impacts are evaluated to be negligible on the environment. This study highlights the importance of considering the energy–water nexus for better-coordinated energy and water resources management at local and national levels.

Su, Qiong↗

DOE OSTI2019

Piperazine aerosol mitigation for post-combustion carbon capture

Amine loss as aerosol is still a challenge for reliable long-term operations in amine scrubbing units. While attempts have been made to understand, predict, and mitigate amine aerosol growth in the absorber, demonstration of the mitigation of piperazine (PZ) aerosol has not been published. This paper presents results from a comprehensive emission study using 5 m PZ. The focus of this work is not to validate growth mechanisms, but to provide data from which existing hypotheses can be analyzed. PZ aerosol at the water wash outlet was characterized by Fourier Transform Infrared Spectroscopy (FTIR) and an Electrical Low-Pressure Impactor (ELPI + ). Two mitigation strategies were successfully implemented during episodes of PZ aerosol emission. These episodes resulted from the presence of SO 3 in the flue gas due to periods of sub-optimal SO 3 removal upstream of the CO 2 capture facility. Four weeks of aerosol tests were also run with 0–6 ppm of SO 3 generated and injected into the flue gas to evaluate the resilience of the mitigation strategies. The first approach to aerosol emission mitigation was to remove aerosol nuclei present in the flue gas. The second approach was to run the absorber with flue gas containing varying SO 3 at conditions that accelerate aerosol nuclei growth and collection within the packing. SO 3 control via hydrated lime addition upstream of the absorber eliminated aerosol while higher lean solvent temperature in the absorber and a two-stage water wash configuration were tested to accelerate aerosol nuclei growth and collection. Increasing the lean solvent temperature by 11 °C and using a two-stage water wash resulted in 98% reduction of PZ emissions. Absorber performance at the elevated lean solvent temperature was sustained in the existing packing with solvent intercooling. PZ emissions were managed to less than 1 ppm for extended periods during the pilot plant campaign.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NASA NTRS2019

A Discussion of the Need to Sustain Mission Ready TPS and for Continued Development of Innovative Entry System Technologies

Flight proven entry system and TPS technologies are critical for the successful execution of in-situ science missions at Venus. Emerging new technologies point to new possibilities and offer innovative approaches to delivering small satellites for orbital science. Venus entry can be very demanding and there are only a few flight proven TPS, some developed by Industry and others by NASA, capable of meeting the mission needs. NASA developed TPS has predominately been transferred to Industry and it is assumed industry will maintain the fabrication capability. However, lack of mission needs may result in obsolence of TSP fabrication capability if there is no money and no motivation. Even within NASA, its' expertise could be diverted to higher priority objectives and thereby the readiness for particular material systems can be impacted or lost. Atrophy of capabilities can come about in other ways as well such as changes to raw materials. Even small manufacturing process changes can demand requalification and TRL may be degraded. Carbon-Phenolic is a text book example. After a long period of absence of US Venus missions, VEXG and the Science community is making the case for future missions. It is insufficient to assume the TSP technologies will be there in 5 or 10 years without active and continual planning and assessment. After Galileo, Carbon-Phenolic materials and fabrication skills were allowed to atrophy. Then when missions needed it, in early 2000, it was no longer possible to make the heritage Carbon-Phenolic. What do we need to do? The first step is to advocate for the establishment of TPS readiness assess-ment. The assessment will involve understanding threats and opportunities, and the development of risk mitigation strategies. VEXAG needs to advocate for such an active monitoring of the needed capabilities, assessment of emerging risks and development of risk mitigation strategies with implementation plans. Such an approach reduces the threat of material obsolence and helps maintain the availability of entry system and TPS technology capabilities, both old and new. Venus probes, landers, balloons and other variable altitude missions, and skimmer missions such as "Cu-pid's Arrow" as well as aerocapture missions to deliver small spacecraft require qualified entry systems and ablative TPS. VEXAG advocated for HEEET in 2013/2014 and the community is well versed with the need to sustain it. But, other TPS that need to be sustained may not be apparent to VEXAG community. The following figure summarizes the ablative TPS capabilities vs Venus mission needs for both primary heatshield and backshell.

Venkatapathy, Ethiraj↗

NASA NTRS2008

Assessment of Medical Risks and Optimization of their Management using Integrated Medical Model

The Integrated Medical Model (IMM) Project is a software-based technique that will identify and quantify the medical needs and health risks of exploration crew members during space flight and evaluate the effectiveness of potential mitigation strategies. The IMM Project employs an evidence-based approach that will quantify probability and consequences of defined in-flight medical risks, mitigation strategies, and tactics to optimize crew member health. Using stochastic techniques, the IMM will ultimately inform decision makers at both programmatic and institutional levels and will enable objective assessment of crew health and optimization of mission success using data from relevant cohort populations and from the astronaut population. The objectives of the project include: 1) identification and documentation of conditions that may occur during exploration missions (Baseline Medical Conditions List [BMCL), 2) assessment of the likelihood of conditions in the BMCL occurring during exploration missions (incidence rate), 3) determination of the risk associated with these conditions and quantify in terms of end states (Loss of Crew, Loss of Mission, Evacuation), 4) optimization of in-flight hardware mass, volume, power, bandwidth and cost for a given level of risk or uncertainty, and .. validation of the methodologies used.

Fitts, Mary A.↗

DOE OSTI2016

Calcium-based multi-element chemistry for grid-scale electrochemical energy storage

Calcium is an attractive material for the negative electrode in a rechargeable battery due to its low electronegativity (high cell voltage), double valence, earth abundance and low cost; however, the use of calcium has historically eluded researchers due to its high melting temperature, high reactivity and unfavorably high solubility in molten salts. Here we demonstrate a long-cycle-life calcium-metal-based rechargeable battery for grid-scale energy storage. By deploying a multi-cation binary electrolyte in concert with an alloyed negative electrode, calcium solubility in the electrolyte is suppressed and operating temperature is reduced. These chemical mitigation strategies also engage another element in energy storage reactions resulting in a multi-element battery. These initial results demonstrate how the synergistic effects of deploying multiple chemical mitigation strategies coupled with the relaxation of the requirement of a single itinerant ion can unlock calcium-based chemistries and produce a battery with enhanced performance.

25 ENERGY STORAGE↗

NASA NTRSDate not supplied

NASA's Integrated Dust Strategy

An Overview of Dust Mitigation Investments and overall NASA's Dust Mitigation Strategy.

Michael R. Johansen↗

DOE OSTI2018

Perchlorate contamination in Chile: Legacy, challenges, and potential solutions

Highlights: • Perchlorate occurs naturally at high concentrations in Chile, for millions of years. • Perchlorate contaminates soils, sediments, drinking water and food products. • Trade of contaminated food products and fertilizers may affect countries worldwide. • Atacama Desert can be used as a natural laboratory for bioprospecting new bacteria. • Chile should evaluate population risks and mitigation strategies for perchlorate. This paper reviews the unique situation of perchlorate contamination in Chile, including its sources, presence in environmental media and in the human population, and possible steps to mitigate its health impacts. Perchlorate is a ubiquitous water contaminant that inhibits thyroid function. Standards for drinking water range from 2 to 18 µg L{sup −1} in United States and Europe. A major natural source of perchlorate contamination is Chile saltpeter, found in the Atacama Desert. High concentrations of perchlorate have presumably existed in this region, in soils, sediments, surface waters and groundwaters, for millions of years. As a result of this presence, and the use of Chile saltpeter as a nitrogen fertilizer, perchlorate in Chile has been found at concentrations as high as 1480 µg L{sup −1} in drinking water, 140 µg/kg{sup −1} in fruits, and 30 µg L{sup −1} in wine. Health studies in Chile have shown concentrations of 100 µg L{sup −1} in breast milk and 20 µg L{sup −1} in neonatal serum. It is important to acknowledge perchlorate as a potential health concern in Chile, and assess mitigation strategies. A more thorough survey of perchlorate in Chilean soils, sediments, surface waters, groundwaters, and food products can help better assess the risks and potentially develop standards. Also, perchlorate treatment technologies should be more closely assessed for relevance to Chile. The Atacama Desert is a unique biogeochemical environment, with millions of years of perchlorate exposure, which can be mined for novel perchlorate-reducing microorganisms, potentially leading to new biological treatment processes for perchlorate-containing waters, brines, and fertilizers.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2005

Remote Sensing Characterization of the Urban Landscape for Improvement of Air Quality Modeling

The urban landscape is inherently complex and this complexity is not adequately captured in air quality models, particularly the Community Multiscale Air Quality (CMAQ) model that is used to assess whether urban areas are in attainment of EPA air quality standards, primarily for ground level ozone. This inadequacy of the CMAQ model to sufficiently respond to the heterogeneous nature of the urban landscape can impact how well the model predicts ozone pollutant levels over metropolitan areas and ultimately, whether cities exceed EPA ozone air quality standards. We are exploring the utility of high-resolution remote sensing data and urban growth projections as improved inputs to the meteorology component of the CMAQ model focusing on the Atlanta, Georgia metropolitan area as a case study. These growth projections include "business as usual" and "smart growth" scenarios out to 2030. The growth projections illustrate the effects of employing urban heat island mitigation strategies, such as increasing tree canopy and albedo across the Atlanta metro area, in moderating ground-level ozone and air temperature, compared to "business as usual" simulations in which heat island mitigation strategies are not applied. The National Land Cover Dataset at 30m resolution is being used as the land use/land cover input and aggregated to the 4km scale for the MM5 mesoscale meteorological model and the (CMAQ) modeling schemes. Use of these data has been found to better characterize low densityhburban development as compared with USGS 1 km land use/land cover data that have traditionally been used in modeling. Air quality prediction for fiture scenarios to 2030 is being facilitated by land use projections using a spatial growth model. Land use projections were developed using the 2030 Regional Transportation Plan developed by the Atlanta Regional Commission, the regional planning agency for the area. This allows the state Environmental Protection agency to evaluate how these transportation plans will affect fbture air quality.

Quattrochi, Dale A.↗

DOE OSTI2020

2-D moving mesh modeling of lithium dryout in open surface liquid metal flow applications

Liquid lithium displays increasing promise as a replacement for solid plasma facing components (PFCs) in fusion device applications. The Liquid Metal Infused Trench (LiMIT) system, developed at the University of Illinois (UIUC), has demonstrated how thermoelectric magnetohydrodynamics (TEMHD) can be harnessed to drive liquid lithium flow in an open surface PFC. However, in the highest heat flux applications, large local acceleration is created via TEMHD, and the sudden increase in velocity can cause the liquid level to expose the underlying solid, eliminating the protective benefits of the lithium. In order to study potential mitigation strategies, a 2-D COMSOL Multiphysics model was developed using the moving mesh module to capture free surface flow. The model depicts the development of the dryout phenomenon for 2 test cases – slow (1 cm/s) and medium (10 cm/s) flow in 5 mm deep trenches – including the liquid level reduction under the high heat flux and the pileup of slower flow both upstream and downstream of the heat stripe. The effectiveness of trench shaping dryout mitigation strategies is examined. For the slow flow case, it is shown that a 1.8 mm ledge placed under the heat stripe will stop dryout, and for the medium flow case, a 2.7 mm ledge is required to mitigate the effect. This model can be used to identify strategies for increasing the viable heat load for open surface liquid lithium PFCs.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2022

Tradeoffs among indoor air quality, financial costs, and CO 2 emissions for HVAC operation strategies to mitigate indoor virus in U.S. office buildings

Adapting building operation during the COVID-19 pandemic to improve indoor air quality (IAQ) while ensuring sustainable solutions in terms of costs and CO 2 emissions is challenging and limited in literature. Our previous study investigated different HVAC operation strategies, including increased filtration using MERV 10, MERV 13, or HEPA filters, as well as supplying 100% outdoor air into buildings for a system initially sized for MERV 10 filtration. This paper significantly extends that research by systematically analyzing the potential financial and environmental impact for different locations in the U.S. The previous medium office building system model is improved to account for operation in different climates. New evaluation metrics are created to consider the comprehensive impact of improving IAQ on costs and CO 2 emissions, using dynamic emission factors for electricity generation depending on the location. HVAC operation strategies are studied in five different locations across the United States, with distinct climates and electricity sources. In four of the five locations, MERV 13 filtration offers the best improvement in IAQ per increase in costs and emissions relative to MERV 10. The exception is the mildest climate of San Diego, where use of 100% outdoor air provides the best IAQ with a limited increase in costs and emissions. Finally, a system not sized for HEPA filtration can lead to increased costs and emissions without much improvement in IAQ.

29 ENERGY PLANNING, POLICY, AND ECONOMY↗

DOE OSTI2019

Understanding, Predicting, and Mitigating Catastrophic Shorts for Improved OLED Lighting Panel Reliability (Final Report)

Catastrophic OLED lighting panel failure due to electrical shorting was a significant reliability challenge facing the industry. The goal of this program was to develop a basic scientific understanding of how incipient shorts in an OLED originate and grow to a catastrophic level, and to develop mitigation strategies that enable the industry to reach the DOE target of 0.01% failure rate. We accomplished this goal, identifying the origin of shorts, understanding how the evolve over time, and ultimately identifying a mitigation strategy that was implemented by our industry partner and demonstrated to completely eliminate catastrophic shorts in production OLED panels. We identified two general classes of panel defect, termed bright spots and hot spots, that respectively originate from indium-tin-oxide agglomerations and microscale organic semiconductor dust particles on the substrate. The former are largely benign whereas the latter can lead to local shunts that grow over time and cause catastrophic failure. We understand the growth process as a self-reinforcing cycle, where shunt-induced heating volatilizes the surrounding organic semiconductor, which in turn expands the shunt and leads to even more heating. Based on these results, we identified several practical strategies to arrest the growth of early-stage shorts or prevent them entirely. These results will reduce the cost and improve the reliability of OLED lighting.

36 MATERIALS SCIENCE↗

DOE OSTI2017

Greening the Grid: Pathways to Integrate 175 Gigawatts of Renewable Energy into India's Electric Grid, Vol. II - Regional Study

The higher-spatial-resolution model of 'Greening the Grid: Pathways to Integrate 175 Gigawatts of Renewable Energy into India's Electric Grid, Vol. II - Regional Study' (the Regional Study), which better represents the impact of congestion on least-cost scheduling and dispatch, provides a deeper understanding of the relationship among renewable energy (RE) location, transmission, and system flexibility with regard to RE integration, compared to 'Greening the Grid: Pathways to Integrate 175 Gigawatts of Renewable Energy into India's Electric Grid, Vol. I - National Study.' The Regional Study validates the relative value of mitigation strategies demonstrated in the National Study - namely, coordinated operations among states reduce production costs, and reducing coal minimum generation levels reduces RE curtailment. Significantly, the Regional Study also highlights a potential barrier to realizing the value of these mitigation strategies: when locations of RE development are planned independently of state-level transmission, intrastate congestion can result in undesirable levels of RE curtailment. Therefore a key objective of this study is to illustrate to state-level power system planners and operators, in particular, how a higher-resolution model, inclusive of intrastate granularity, can be used as a planning tool for two primary purposes: -To better anticipate, understand, and mitigate system constraints that could affect RE integration; and - To provide a modeling framework that can be used as part of future transmission studies and planning efforts. The Regional Study is not intended to predict precisely how RE will affect state-level operations. There is considerable uncertainty regarding the locations of the RE development, as well as how contract terms can affect access to the inherent physical flexibility of the system. But the scenarios analyzed identify the types of issues that can arise under various RE and transmission expansion pathways. The model developed for this study provides a rigorous framework for future work and can be updated with the characteristics of new capacity as more information on the future power system is known.

24 POWER TRANSMISSION AND DISTRIBUTION↗

DOE OSTI2017

Greening the Grid: Integrating 175 Gigawatts of Renewable Energy into India's Electric Grid - A Detailed Look at the Western Region

24 POWER TRANSMISSION AND DISTRIBUTION↗

DOE OSTI2017

Greening the Grid: Integrating 175 Gigawatts of Renewable Energy into India's Electric Grid - A Detailed Look at the Southern Region

The higher-spatial-resolution model of 'Greening the Grid: Pathways to Integrate 175 Gigawatts of Renewable Energy into India's Electric Grid, Vol. II - Regional Study' (the Regional Study), which better represents the impact of congestion on least-cost scheduling and dispatch, provides a deeper understanding of the relationship among renewable energy (RE) location, transmission, and system flexibility with regard to RE integration, compared to 'Greening the Grid: Pathways to Integrate 175 Gigawatts of Renewable Energy into India's Electric Grid, Vol. I - National Study.' The Regional Study validates the relative value of mitigation strategies demonstrated in the National Study - namely, coordinated operations among states reduce production costs, and reducing coal minimum generation levels reduces RE curtailment. Significantly, the Regional Study also highlights a potential barrier to realizing the value of these mitigation strategies: when locations of RE development are planned independently of state-level transmission, intrastate congestion can result in undesirable levels of RE curtailment. Therefore a key objective of this study is to illustrate to state-level power system planners and operators, in particular, how a higher-resolution model, inclusive of intrastate granularity, can be used as a planning tool for two primary purposes: to better anticipate, understand, and mitigate system constraints that could affect RE integration; and to provide a modeling framework that can be used as part of future transmission studies and planning efforts. The Regional Study is not intended to predict precisely how RE will affect state-level operations. There is considerable uncertainty regarding the locations of the RE development, as well as how contract terms can affect access to the inherent physical flexibility of the system. But the scenarios analyzed identify the types of issues that can arise under various RE and transmission expansion pathways. The model developed for this study provides a rigorous framework for future work and can be updated with the characteristics of new capacity as more information on the future power system is known.

24 POWER TRANSMISSION AND DISTRIBUTION↗

NASA NTRS2011

The Analysis of Rush Orders Risk in Supply Chain: A Simulation Approach

Satisfying customers by delivering demands at agreed time, with competitive prices, and in satisfactory quality level are crucial requirements for supply chain survival. Incidence of risks in supply chain often causes sudden disruptions in the processes and consequently leads to customers losing their trust in a company's competence. Rush orders are considered to be one of the main types of supply chain risks due to their negative impact on the overall performance, Using integrated definition modeling approaches (i.e. IDEF0 & IDEF3) and simulation modeling technique, a comprehensive integrated model has been developed to assess rush order risks and examine two risk mitigation strategies. Detailed functions sequence and objects flow were conceptually modeled to reflect on macro and micro levels of the studied supply chain. Discrete event simulation models were then developed to assess and investigate the mitigation strategies of rush order risks, the objective of this is to minimize order cycle time and cost.

Mahfouz, Amr↗