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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 217 records · Page 12
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Measurements of displacement cross sections of metals for 120-GeV proton beam irradiation

The number of displacements per atom (dpa) is widely used as an indicator of irradiation damage of materials in proton accelerator facilities. Experiments have been carried out to validate the dpa of metallic materials for protons with energies below 3 GeV. However, measurements of the displacement cross-sections for high-energy protons above 3 GeV have not been carried out and the calculations have not been validated. To validate the displacement cross section of metals in high-energy region, electrical resistivity changes in wires of aluminum, copper and tungsten at 8 K were measured using protons with energies of 120-GeV. The results show that the Norgett-Robinson-Torrens dpa model of the Particle and Heavy Ion Transport Calculation Code overestimates the experimental data. On the other hand, the calculated results using the athermal recombination corrected dpa model were in agreement with the measured displacement cross sections. In the proton energy region above 1 GeV, the displacement cross section is almost constant, which is due to the fact that the damage energy of the material under 1 GeV proton irradiation is almost the same as under 120 GeV proton irradiation. Damage recovery of defects accumulated in the sample was also measured using isochronal annealing: At 80 K, approximately 60 % and 80 % of the damage remains for copper and tungsten, respectively. These results are the same as those obtained from other experiments on proton and neutron irradiation.

43 PARTICLE ACCELERATORS↗
DOE OSTI2025

Symmetrization of Strong Hydrogen Bond under High Pressure in Bihydroxide-Ion-Containing NaCu 2 (SO 4 ) 2 ·H 3 O 2 Revealed by Experimental Charge Density, Single-Crystal Electron Diffraction, and Neutron Diffraction Studies

In minerals and inorganic compounds, strong hydrogen bonding can lead to the formation of complex ionic species such as the H 3 O 2 – bihydroxide anion and Zundel cation H 5 O 2 + . We studied [NaCu 2 (SO 4 ) 2 ·H 3 O 2 ] natrochalcite, which contains bihydroxide anions and undergoes hydrogen bond symmetrization at the lowest pressure reported so far among inorganic compounds. Hydrogen bond symmetrization leads to changes in the bulk modulus, seismic wave velocities, and proton mobility and plays a primary role in high-temperature superconductivity, but its characteristics are not well understood due to a lack of systematic studies and limitations of experimental methods sensitive to this subtle change. In this work, we applied experimental charge density analysis based on in situ single-crystal X-ray diffraction data, along with the single-crystal neutron and electron diffraction experiments, to probe the behavior of hydrogen atoms during the hydrogen bond symmetrization process under high-pressure conditions. On the way to the symmetrical H-bonding, natrochalcite undergoes a series of complex redistributions of electron density, which we trace with multipole refinement and detailed analysis of changes in the Laplacian of electron density values. Additionally, we deconvoluted the equation of state (volume of the unit cell vs pressure relation) into the atomic equation of states describing dependencies of atomic charges or volumes vs pressure.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2026

Inferring performance metrics for laser direct drive experiments on OMEGA

Quantifying performance improvements on the OMEGA laser facility requires robust inference of established no-alpha performance metrics, which requires, at minimum, a model to infer the shocked fuel mass and pressure of the confined fusion plasma. In this work, we describe the methodology used to infer performance metrics on OMEGA and present the current state-of-the art model used to infer these metrics from OMEGA experiments. In particular, since neutron images of cryogenic implosions are not available on OMEGA at present, we present how x-ray sizes are determined on OMEGA using a Gaussian Process regression model and how the neutron production region's size is inferred from them. As a result, we end by benchmarking the model using synthetic data and 1-D LILAC simulations and test its experimental self-consistency across available x-ray diagnostic channels.

Gopalaswamy, V. [Laboratory for Laser Energetics, ↗
DOE OSTI2025

PMT calibration for the JSNS^2-II far detector with an embedded LED system

The JSNS^2-II (the second phase of JSNS^2, J-PARC Sterile Neutrino Search at J-PARC Spallation Neutron Source) is an experiment aimed at searching for sterile neutrinos. Here, this experiment has entered its second phase, employing two liquid scintillator detectors located at near and far positions from the neutrino source. Recently, the far detector of the experiment has been completed and is currently in the calibration phase. The following properties of all functioning Photo-Multiplier-Tubes (PMTs) to detect the neutrino events in the far detector have been calibrated: PMT gain, its dependence of supplied High Voltage (HV), Peak-to-Valley (PV), and signal timing. This paper presents a detailed description of the calibration process utilizing the LED system. The LED system of the far detector uses two Ultra-Violet (UV) LEDs, which are effective in calibrating all of the PMTs at once. The UV light is converted into the visible light wavelengths inside liquid scintillator via the wavelength shifters, providing pseudo-isotropic light. To achieve a good energy resolution for physics events, a relative gain adjustment of up to 10% is required for all functioning PMTs. This will be achieved using the HV curves measured and the results of the LED calibration. The Peak-to-Valley (PV) ratio values, which distinguish the single photo-electron signal from the pedestal, are similar to those from the production company. Additionally, the precision of the PMT signal timing is measured to be 2.1 ns. This meets the event reconstruction requirement of 10 ns.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

First JSNS 2 measurement of the electron neutrino flux using the 12 C⁡(𝜈 𝑒 ,𝑒 − )⁢ 12 N g.s. reaction

JSNS2 (J-PARC Sterile Neutrino Search at J-PARC Spallation Neutron Source) is an experiment searching for sterile neutrinos through the observation of ν¯μ→ν¯e appearance oscillations, using neutrinos produced by muon decay-at-rest. A key aspect of the experiment involves accurately understanding the neutrino flux and the quantities of pions and muons, which are progenitors of (anti)neutrinos, given that their production rates have yet to be measured. We present the first electron-neutrino flux measurement using C12(νe,e−)12Ng.s. reaction in JSNS2, yielding a flux of (6.7±1.6(stat)±1.7(syst))×10−9 cm−2 proton−1 at the JSNS2 detector location, located at 24 meters distance from the mercury target. This flux measurement is consistent with predictions from simulations based on hadron models.

Particle decays↗
DOE OSTI2024

Electronic and magnetic structures of a mixed triple perovskite: Ba 3 NiRuIrO 9

In search of spin-orbit coupling driven nonmagnetic J = 0 ground state and excitonic magnetism, various pentavalent iridates have been studied in recent years. However, a finite moment was observed in most of the cases due to solid state effects. Here, in this work, we investigate the electronic and magnetic structure of 6H hexagonal compound Ba 3 NiRuIrO 9 , where Ir 5+ is present along with magnetic Ni 2+ and Ru 5+ ions. Magnetic susceptibility measurements and neutron powder diffraction (NPD) experiments demonstrate the appearance of short-range magnetic ordering below 170 K and a long-range antiferromagnetic ordering below 80 K. The refinement of the NPD pattern further shows that the Ru and Ir moments interact antiferromagnetically within the dimer and interact ferromagnetically with the Ni sublattice. These experimental findings have been complemented by first-principles density functional theory calculations incorporating spin-orbit coupling effects and electronic correlations for the transitional metal d states. The computed magnetocrystalline anisotropy is also found to be significant and the crystallographic c axis comes out to be the easy axis of magnetization, consistent with the spin alignment direction found from NPD. This study shows that the mixed ruthenate iridate triple perovskite series is a promising family to study the interplay among spin-orbit coupling, electron correlation, and electron filling as a variety of Ba 3 M RuIrO 9 with M as a transition metal ion, rare-earth ion, and alkali metal ions can be synthesized.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2025

Preliminary Results on Bayesian Inverse UQ for OECD/NEA WPNCS Subgroup 14 Benchmark Exercise for Error Recovery and Experimental Coverage

The Organization for Economic Cooperation and Development (OECD) Working Party on Nucelar Criticality Safety (WPNCS) has proposed a benchmark exercise representative of neutronic behavior in criticality experiments. Here, the goal is to develop confidence in data assimilation techniques used to adjust nuclear data. Participants are given synthetic experimental models with associated measured data and asked to estimate the model parameters given the model and measurements as well as provide predictions for separate application models. In this work, we performed data assimilation using Bayesian inverse Uncertainty Quantification (UQ) with machine learning surrogate models to produce posterior parameter distributions for the requested parameters and posterior predictive distributions for the requested responses. Several experimental models are shown to insufficiently inform the posterior parameter distributions for the applications involved. However, given sufficient experimental data, posterior parameter estimates yielded reduced uncertainty in the response predictions of interest while covering the experimental data.

Bayesian Inference↗
DOE OSTI2026

Resonance Self-Shielding: Why it is so Important

This paper is one of a series that I am writing to document my 58 years of experience with ENDF and Neutron Transport calculations, beginning when I worked at the National Nuclear Data Center (NNDC), Brookhaven National Laboratory (BNL), from 1967 to 1972. During those years I was the head of the computer unit of NNDC, assigned to develop computer codes to pre-process, view and test ENDF/B data. Since then, I have continued to support the ENDF effort without any official position or monetary compensation, because I realized how important accurate nuclear data is for use in use in our Engineering applications. It is so important to realize that regardless of how accurate or even perfect our application codes may be to transport particles, without accurate nuclear data we are in a “Garbage In = Garbage Out” situation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Characterizing the AFP Spin Flipper for the Nab Experiment

The Nab experiment at the Spallation Neutron Source (SNS) at Oak Ridge National Laboratory (ORNL) aims to yield a precise measurement of the electron-neutrino correlation parameter, a , to $\frac{Δa}{a}$ = 1 × 10 −3 from the beta-decay of the free neutron. To achieve Nab’s precision goal, polarization of the neutron beam must be near-zero. A polarizer/analyzer combination, neutron monitors, and an Adiabatic Fast Passage (AFP) spin flipper will be used to determine a beam polarization effectively less than 2 × 10 −5 . Here, I will discuss the initial characterization efforts of the Nab spin flipper as well as plans for further testing.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

HighNESS conceptual design report: Volume II. The NNBAR experiment.

A key aim of the HighNESS project for the European Spallation Source is to enable cutting-edge particle physics experiments. This volume presents a conceptual design report for the NNBAR experiment. NNBAR would exploit a new cold lower moderator to make the first search in over thirty years for free neutrons converting to anti-neutrons. The observation of such a baryon-number-violating signature would be of fundamental significance and tackle open questions in modern physics, including the origin of the matter-antimatter asymmetry. This report shows the design of the beamline, supermirror focusing system, magnetic and radiation shielding, and anti-neutron detector necessary for the experiment. A range of simulation programs are employed to quantify the performance of the experiment and show how background can be suppressed. For a search with full background suppression, a sensitivity improvement of three orders of magnitude is expected, as compared with the previous search. Civil engineering studies for the NNBAR beamline are also shown, as is a costing model for the experiment.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

THE STRUCTURE FUNCTION OF THE FREE NEUTRON AT HIGH X-BJORKEN

Understanding the internal structure of nucleons is one of the primary goal of nuclear physicists. As protons and neutrons are only the bound state solution of the QCD lagrangian (at least inside atomic nuclei), studying protons and neutrons helps uncover nuclear struc ture. Due to its easy availability, many studies on protons have been done on a wide range of kinematics. However, free neutron targets are not readily achievable. So, any information on neutrons has to be extracted from neutron-rich nuclei, and some nuclear models have to be used to subtract the contributions from other nucleons to extract the information on neutrons. So, the Barely Off-shell Nucleon Structure (BONuS12) experiment at Jefferson Lab was conducted to overcome these challenges by using spectator tagging. The experiment effectively created a quasi-free neutron target by scattering electrons off a deuterium target and detecting low-momentum, backward-moving protons using a custom-built Radial Time Projection Chamber (RTPC). Selecting the low momentum and backward-moving spectators would enable us to minimize the model-dependent effects due to final state interactions and target fragmentation. The RTPC was a 40 cm-long cylindrical detector that works on the principle of gaseous ionization. It had three layers of Gas Electron Multipliers (GEMs) for charge amplification and a surrounding readout pad. The scattered electrons were measured using the CLAS12 detector, and data were collected using a 10.4 GeV electron beam dur ing Spring and Summer 2020. Using spectator tagging, we extracted the structure function ratio Fn 2 of the quasi-free neutron in the deep inelastic scattering at high x, upto x ~ 0.8. The result was extracted in the region with the invariant mass W > 1.8 GeV/c2, and Q2 in the range 1.3 to 11 GeV2. This dissertation presents the methodology, event selection criteria and refinements, estimation and subtraction of backgrounds, and complete analysis of extraction of Fn 2/Fp 2 in a model-independent way. Also, systematic uncertainties in our final analysis will be discussed in detail.

Pokhrel, Madhusudhan [Old Dominion Univ., Norfolk,↗
DOE OSTI2025

Probing the shear-induced microstructure of a smectite clay aqueous suspensions using rheo-USANS and rheo-SIPLI measurements

Hypothesis: The static microstructure of aqueous sodium-montmorillonite (Na-Mt) suspensions at low ionic strengths (where Particle Size/Debye Length ≈1) exhibits both the particle–particle ordering as well as aggregation with repulsive ordered domains having characteristic optical birefringence and attractive aggregated entities larger than 20 µm resulting in ever-increasing yield stresses also known as physical aging-rejuvenation behavior. We hypothesize that the attractive particle–particle aggregation is the underlying cause behind the physical aging-rejuvenation behavior observed in Na-Mt suspensions with no contribution from structural dynamics driven by repulsive particle–particle ordering or jamming. Experiments: We investigate the shear-induced microstructure of aqueous Na-Mt suspensions in the sol and gel state using rheo-ultra-small angle neutron scattering (rheo-USANS) experiments at shear rates of 1, 50, 500, and 2000 s −1 . We also perform rheo-shear-induced polarization light imaging (rheo-SIPLI) experiments to relate ordering with shearing and aging. Findings: Shearing the suspensions at low to moderate shear rates induces particle–particle aggregation and shearing at high shear rates induces the breakage of particle–particle aggregation in the sol and gel states, suggesting the microstructural aggregation in the sol and gel state is shear sensitive and a full rejuvenation or breakage of particle–particle aggregation is only achieved at a minimum critical shear rate. The rheo-SIPLI experiments reveal that the sol and gel state exhibited strong Maltese cross patterns at a shear rate of 1000 s −1 , indicating particle–particle ordering. Post shearing, the gel exhibited temporal evolution of storage modulus without any noticeable influence on the appearance of the Maltese cross pattern indicating physical aging and particle ordering are distinct length scale phenomena in Na-Mt suspensions and the physical aging-rejuvenation behaviour is a feature of particle–particle aggregation as opposed to ordering.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2026

Measurement of the 75 As ⁢(𝑛, 2⁢𝑛) cross section at 14.1 MeV at the National Ignition Facility

Here, a new measurement of the 75 As (𝑛, 2⁢𝑛) measurement was performed using the 14.1 MeV neutron pulse produced by fusion experiments at the National Ignition Facility (NIF). The target material consisted of GaAs foils encapsulated in aluminum irradiation containers, along with Au monitor foils, and positioned in the NIF chamber during high neutron yield shots. After irradiation, the GaAs and Au foils were counted with high purity germanium detectors to assess the production of (𝑛, 2⁢𝑛) activation products to determine the flux and the cross section of interest. The measured cross section was 966 ± 71 mb at 14.1 ± 0.37 MeV. This work provides a proof of concept for a platform for performing “ride-along” cross section measurements at NIF to contribute to existing nuclear data as well as measure new cross sections in the future.

and nuclear chemistry↗
DOE OSTI2025

Anomalous neutron nuclear-magnetic interference spectroscopy

The electron–phonon interaction plays a critical role in materials’ electrical, thermal, optical, and superconducting properties. However, measuring the phonon mode-resolved electron–phonon interaction has been challenging. Here we propose neutron-scattering-based Anomalous Neutron nUclear-Magnetic Interference Spectroscopy (ANUBIS), where the co-existence of neutron nuclear scattering and magnetic scattering leads to anomalous dynamical structure factor under the presence of the electron–phonon interaction. Such anomalous structure factor is linear in electron–phonon coupling constant at the phonon wavevector, and is directly proportional to the momentum and energy-resolved dielectric function. The experimental configuration can be achieved using existing polarized inelastic neutron scattering setup, and an order-of-magnitude estimate shows the viability to observe the anomalous scattering signal is around to 10 –4 to 10 –3 relative to phonon scattering, which is examined through the preliminary experiments and achievable at emerging neutron facilities. As a result, our proposal offers an alternative neutron-based metrology to probe the crucial electronic properties.

Electron-phonon interactions↗
DOE OSTI2025

Cosmic-ray cooling in active galactic nuclei as a new probe of inelastic dark matter

We present a novel way to probe inelastic dark matter using cosmic-ray (CR) cooling in active galactic nuclei (AGNs). Dark matter (DM) in the vicinity of supermassive black holes may scatter off CRs, resulting in the rapid cooling of CRs for sufficiently large cross sections. This in turn can alter the high-energy neutrino and gamma-ray fluxes detected from these sources. We show that AGN cooling bounds obtained through the multimessenger data of NGC 1068 and TXS 0506 + 056 allows us to reach unprecedently large mass splittings for inelastic DM (≳ TeV), orders of magnitude larger than those probed by direct detection experiments and DM capture in neutron stars. Furthermore, we demonstrate that cooling bounds from AGNs can probe thermal light DM with small mass splittings. This provides novel and complementary constraints in parts of a parameter space accessible solely by colliders and beam-dump experiments.

astronomical black holes↗
DOE OSTI2025

Review of Neutron Yield from (α, n) Reactions: Data, Methods, and Prospects

Understanding the radiogenic neutron production rate through the (α, n) reaction is crucial in many areas of physics, including dark matter searches, neutrino studies, and nuclear astrophysics. In addition to its relevance for fundamental research, the (α, n) reaction also plays a significant role in nuclear energy technologies, for example by contributing to neutron production in subcritical systems using UO2, as well as in applications such as medical physics. This review examines the current state of (α, n) yield calculations and neutron spectra, describes the computational tools used for their estimation, and discusses the available cross-section data. We discuss the uncertainties affecting (α, n) yield estimations and propose a strategy to enhance their accuracy. Furthermore, this paper discusses and emphasizes the need for new measurements of (α, n) cross-sections for a variety of relevant materials. Such measurements are essential for improving neutron flux predictions, which are crucial for reducing uncertainties in sensitivity estimates for next-generation physics experiments operating in the keV—MeV range.

(α, n)reactions↗
DOE OSTI2026

Benchmark of the Chlorine Worth Study Experiments in Support of Chlorine Nuclear Data Validation for Nuclear Criticality Safety

The Chlorine Worth Study (CWS) was a critical experiment to address an urgent need for thermal chlorine nuclear data validation in plutonium systems. This urgent need is tied directly to plutonium recycle and recovery operations in the plutonium facility at Los Alamos National Laboratory, where exceptionally conservative criticality safety limits are used because no credit is taken for the neutron capture by chlorine. The experiment used weapons-grade plutonium metal plates clad in stainless steel, known as the PANN (plutonium aluminum no nickel) ZPPR (zero power physics reactor) plates. The plutonium was reflected and moderated by high-density polyethylene and included combinations of polyvinyl chloride (PVC) and chlorinated polyvinyl chloride (CPVC) as absorbers. The experiment and benchmark included three configurations mimicking 30 g 239 Pu/L plutonium, 300 g 239 Pu/L plutonium, and 600 g 239 Pu/L plutonium in an aqueous chloride solution. Uncertainties in the benchmark included five broad categories: (1) criticality measurement, (2) mass and density, (3) dimensions, (4) material compositions, and (5) positioning. The largest contribution to the overall uncertainties for all three cases came from the material compositions, in particular the PVC and CPVC absorber compositions. A detailed model was created to be a near match (that is within expectations of transport code users) and a simplified model was created to minimize offset dimensions and expedite modeling for code validation. Sample calculations were completed in MCNP6.3 with ENDF/B-VIII.0 and ENDF/B-VII.1 nuclear data. For the detailed and simplified models, the average difference between the computed and experimental k eff was 951 pcm. CWS will serve as the key validation experiment for nuclear criticality safety in support of aqueous chloride operations. The sensitivity to the chlorine capture cross section is orders of magnitude greater than other existing benchmarks. The current limits, as defined by nuclear criticality safety, are 520 g Pu per batch, i.e. the minimum critical mass of the Pu solution infinitely reflected by water [Criticality Handbook: Volume II, (1969)]. This extremely conservative critical mass limit does not credit any neutron capture by chlorine (in particular neutron capture by 35 Cl) and greatly impedes the throughput required for current and future operations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗