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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 217 records · Page 12

Harnessing Uncertainty through Functional Data Analysis in Gas Breakthrough Data

Detecting subsurface explosions from radionuclide gas migration through rock fractures is an effective way to identify nuclear activity. Los Alamos National Laboratory (LANL) has developed simulation methods, based on data from the 1962 Hardhat underground nuclear test, to predict gas breakthrough times at the surface. However, these methods rely on an imperfect understanding of the relationship between rock damage and fracture permeability. Our clinic project studies methods for predicting breakthrough curves that characterize total mass produced as a function of time, as well as quantifying the uncertainty associated with these predictions. The model that is currently employed to relate damage to permeability uses an empirically motivated power-law expression, with a range of parameter values that are compatible with the experimental Hardhat data. We develop emulators, built from functional data analysis techniques and trained on simulation data, that rapidly predict the gas breakthrough curve given a damage field and given the parameter values of the power-law equation. Using Bayesian regression, we address the problem of uncertainty quantification in our emulators. Finally, in order to test the robustness of the model, we further validate it on a damage field representing different physical conditions.

58 GEOSCIENCES↗

AGR Program TRISO Fuel Topical Report Dialog

AGR Program Overview and Current Activities Fission Product Transport Data Short-Lived Fission Product Release Fuel Performance Margin Data Oxidation Testing Data

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Construction and Testing of Data Acquisition Components for the Hall A Compton Polarimeter

Nuclear physics experiments require accurate knowledge of the spin polarization of the electron beam delivered to the experimental halls. Hall A is upgrading its Compton polarimeter in support of the lab's 12 GeV beam energy upgrade. This project centered around the data acquisition (DAQ) system for the scattered-photon detection component of the polarimeter. The goal was to test whether the DAQ software and hardware are capable of capturing, recording, and processing electron helicity-dependent scattering rate asymmetry data at high rates, while maintaining appropriate accuracy. We created the necessary circuits, and are able to reliably extract asymmetries of between 0.5{\%} and 11.5{\%} to 0.2{\%}. We did this in a deadtime-free regime at rates between 100 KHz and 350 KHz. We currently are unable to measure the system deadtime after it becomes manifest at about 350 KHz. These tests support the use of a scaled version of this configuration.

Hill, Joshua↗

Deep Inelastic Electron Scattering Off the Helium and Tritium Mirror Nuclei

We discuss a possible measurement of the ratio of nucleon structure functions, F{sub 2}{sup n}/F{sub 2}{sup p}, and the ratio of up to down quark distributions, u/d, at large Bjorken x, by performing deep inelastic electron scattering from the {sup 3}H and {sup 3}He mirror nuclei with the 11 GeV upgraded beam of Jefferson Lab. The measurement is expected to be almost free of nuclear effects, which introduce a significant uncertainty in the extraction of these two ratios from deep inelastic scattering off the proton and deuteron. The results are expected to test perturbative and non-perturbative mechanisms of spin-flavor symmetry breaking in the nucleon, and constrain the structure function parametrizations needed for the interpretation of high energy collider and neutrino oscillations data. The precision of the expected data can also test models of the nuclear EMC effect and provide valuable input for its full explanation.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Data for training and testing radiation detection algorithms in an urban environment

The detection, identification, and localization of illicit nuclear materials in urban environments is of utmost importance for national security. Most often, the process of performing these operations consists of a team of trained individuals equipped with radiation detection devices that have built-in algorithms to alert the user to the presence nuclear material and, if possible, to identify the type of nuclear material present. To encourage the development of new detection, radioisotope identification, and source localization algorithms, a dataset consisting of realistic Monte Carlo-simulated radiation detection data from a 2 in. × 4 in. × 16 in. NaI(Tl) scintillation detector moving through a simulated urban environment based on Knoxville, Tennessee, was developed and made public in the form of a Topcoder competition. The methodology used to create this dataset has been verified using experimental data collected at the Fort Indiantown Gap National Guard facility. Realistic signals from special nuclear material and industrial and medical sources are included in the data for developing and testing algorithms in a dynamic real-world background.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Validating ENDF/B-VIII.1beta3 with LLNL Pulsed-Sphere Experiments and ICSBEP Benchmarks [Slides]

LPS experiments are not benchmarks but can provide valuable input. 22/1/24 LPS experiments are not benchmarks but can provide valuable input. LPS (run by Denise) help validate nuclear data up to 15 MeV. They test scattering and fission data. They have incomplete uncertainties from 2-8%. I take note when: (1) I see C/E differences above the peak and before late times => 20%. (2) Simulated results between libraries change by => 20% without a good explanation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Preliminary Scaling Analysis of Reactivity Initiated Accidents

The life cycle for new fuel development requires extensive modeling and testing of the fuel concept from benchtop scale experiments to full scale assemblies in prototypical conditions. As a result, the timeline to develop new fuel types can extend up to 20 years and hinders the ability to develop a diverse assortment of fuel types. The licensing of recent reactor designs such as Westinghouse's AP-600/1000 designs utilized a scaling methodology to perform nuclear safety code validation on experimental test data from scaled down thermal hydraulic facilities. The advantage of using a scaling methodology was a significant cost decrease in the testing program because it avoided needing to build full scale prototypes and focused on improving safety code's ability to predict test data. This study investigates how to apply a scaling hierarchy for fuel performance during a Reactivity Initiated Accident that could be implemented with scaling methods such as Hierarchical Two Tiered Scaling (H2TS), Fractional Scaling Analysis (FSA), and Dynamical System Scaling (DSS) .

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Expanding Benchmarks for Nuclear Data Validation [Slides]

The presentation discusses benchmarking in comparison to experimental truth, the integral experiments that were performed, and that benchmarks are evaluated experiments. It also discusses validation testing, and that the ultimate goal of the validation end product is to improve evaluated nuclear data for applications It does state that validation highlights errors in the Nuclear Data Pipeline that affect applications, for example: Missing Cd Capture Gammas in ENDF/B-VII.1. It acknowledges that additional types of experiments are needed to test data used in applications, and that validation experiments do not have to be complicated and expensive. The presentation also discusses different types of measurements including activation foil and fission chamber measurements, reactor kinetics measurements, and subcritical measurements. The presentation concludes with an experiment summary and states that all applications need validation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Continuous-Energy Data Checks

The purpose of this report is to provide an overview of all Quality Assurance tests that have to be performed on a nuclear data set to be transformed into an ACE formatted nuclear data file. The ACE file is capable of containing different types of data such as continuous energy neutron data, thermal scattering data, etc. Within this report, we will limit ourselves to continuous energy neutron data.

99 GENERAL AND MISCELLANEOUS↗

Nevada National Security Site Underground Radionuclide Inventory, 1951-1992: Accounting for Radionuclide Decay through September 30, 2012

This report is an update of report LA-13859-MS (Bowen et al., 2001). In that original report, the underground radionuclide inventory at the Nevada National Security Site (NNSS) was decay corrected to September 23, 1992, the date of the last underground nuclear test at the NNSS. In this report, the inventory is updated to account for the decay of radionuclides over two additional decades (1992-2012) and revised tritium, fission product and actinide inventory figures and tables are presented. The maximum contaminant levels for radionuclides were also updated to Safe Drinking Water Act Maximum Contaminant Levels (MCLs) (CFR, 2013). Also, a number of minor errata found in the original publication were corrected. An inventory of radionuclides produced by 828 underground nuclear tests conducted at the NNSS by the Lawrence Livermore National Laboratory, the Los Alamos National Laboratory, and the Department of the Defense from 1951 to 1992 includes tritium, fission products, actinides, and activation products. The inventory presented in this report provides an estimate of radioactivity remaining underground at the NNSS after nuclear testing. The original test inventory is decayed to September 30, 2012, and predictions of inventory decay over the subsequent 1000 years are presented. For the purposes of summary and publication, the Los Alamos National Laboratory and Lawrence Livermore National Laboratory authors of this report subdivided the inventory into five areas corresponding to the principal geographic test centers at the NNSS. The five areas roughly correspond to Underground Test Area “Corrective Action Units” (CAUs) for remediation of groundwater. In addition, the inventory is further subdivided for the Yucca Flat region by tests where the working point depth is more than 328 feet (100 meters) above the water table and tests that were detonated below that level. Water levels used were those from the U. S. Department of Energy, Nevada Operations Office (1997), now called the Nevada Field Office. Curie activities and atoms are reported as of September 30, 2012. This inventory is strictly a compilation of the residual radiologic inventory remaining from the underground nuclear tests conducted by Lawrence Livermore National Laboratory, Los Alamos National Laboratory and the Department of the Defense from 1951 to 1992 and does not include radioactivity from other types of nuclear testing (e.g., atmospheric, reactors, rocket engines). A companion classified report (Miller et al., 2002) contains test-specific data for each test performed at the NNSS. This work has been sponsored by the U. S. Department of Energy, National Nuclear Security Administration Nevada Field Office.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Towards Reliable Cross Sections for National Security Applications

Stockpile stewardship requires the description of weapons performance without resorting to underground nuclear testing. In the earlier tests, selected isotopes were used as detectors, and recovered after irradiation. Aspects of nuclear device performance were inferred by comparing the measured isotopic ratios to those predicted from simulations. The reaction flows that produce the final isotopic distributions proceed through regions of the nuclear chart that include unstable nuclei. Presently, improved nuclear data input is required to reanalyze prior tests and to certify the stockpile's reliability and safety. Many important cross sections are unknown, as is shown in the example of the Yttrium reaction network (Figure 1). The relevant reactions include (n,2n), (n,n'), (n,gamma), (n,p) and other charged-particle emitting reactions. The cross sections have to be calculated or inferred from indirect measurements. In both cases, reliable optical models that are valid a few nucleons away from stability are needed. The UNEDF Nuclear Reaction activities address this need by combining nuclear-structure input from UNEDF structure calculations with modern reaction theory and large-scale computational capabilities to develop microscopic nucleon-nucleus optical potentials that can be extrapolated to unstable nuclei. In addition, the reaction calculation tools and optical models developed in this context are proving valuable for planning and interpreting indirect (surrogate) measurements of the required cross sections.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Nuclear characterization of a general-purpose instrumentation and materials testing location in TREAT

The Transient Reactor Test facility (TREAT) was constructed in the late 1950s, provided thousands of transient irradiations before being placed in standby in 1994, and resumed operations in 2017 in order to reclaim its crucial role in nuclear-heated safety research. The latter half of TREAT’s historic operation was best known for integral-scale testing of fuel specimens under postulated reactor plant accident conditions, while TREAT’s earlier history included extensive simpler phenomena identification tests that elucidated fundamental behaviors and paved the way for these integral-scale tests. Advances in modern computational capabilities and a resurgence of interest in novel reactor technology have created an opportunity for emphasizing modernized science-based and separate effects test capabilities once again at TREAT. An innovative approach to this type of testing has been developed to leverage minor radioactivity built-in during brief TREAT irradiations in low activation hardware to facilitate handling for materials and instrumentation testing. This capability, termed the Minimal Activation Retrievable Capsule Holder (MARCH) irradiation vehicle system, will be used for inaugural fueled experiments in TREAT’s modern era as well as novel approaches to study materials undergoing neutron irradiation and instrumentation development and qualifications. This paper describes a comprehensive nuclear characterization, obtained via computational modeling, of the test position in the MARCH system. Though directly applicable to the MARCH system, the results also provide general quantification of the nuclear performance of the reactor and potential test materials, crucial for evaluating potential experiment design and response in TREAT. The neutron and photon flux environment was calculated via MCNP with ENDF/B-VII.1 nuclear data. Wire heating rate and DPA calculations were also performed and evaluated using historic TREAT test data. Furthermore, these calculations were performed to provide steady-state baseline reference values typical in both half- and full-slotted TREAT core configurations, enabling design scoping analysis prior to development of more specific design testing needs and transient testing experimentation.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Assessing the viability of a new subsize tensile specimen geometry for evaluation of structural nuclear and additively manufactured materials

The use of subsize specimens in nuclear materials testing has been a subject of ongoing interest due to radiation safety concerns and resource conservation needs. It is also of interest in additive manufacturing (AM), also known as 3D-printing, as subsize specimens can more accurately represent the behavior of the small, intricate geometries often produced using AM. A novel, extremely small geometry, called the Subsize Teeny (SST) was recently developed and is of interest for implementation. Given its extraordinarily small size and the complexities associated with subsize specimen testing, adequate vetting of this geometry is necessary to ensure data quality. Here, a variety of unirradiated nuclear structural materials were tested in the SST geometry and compared against the well-established SSJ3 geometry. In addition, two case studies implementing the SST as a screening geometry for AM materials were also conducted. The question of SST viability was found to be highly nuanced and will often be dependent on the context or application in question. It was determined, however, that the SST is a largely invalid geometry for exceptionally coarse-grained materials or in cases where the physical defect volume equals or exceeds 0.1 % or where the specimen machining parameters result in significant surface alterations. On the other hand, it was determined that the SST may be employed with confidence if the test material is nearly or totally free of physical defects, isotropic, demonstrates homogeneous plastic deformation, and possesses a fine-grained, nearly or totally homogeneous microstructure with at least twelve slip systems.

Additive manufacturing↗

Phase II testing of Xenon International on Mount Schauinsland, Germany

Station RN33 on Mount Schauinsland near Freiburg, Germany, is part of the International Monitoring System monitoring radioxenon in air ( 131m Xe, 133 Xe, 133m Xe, and 135 Xe) for verification of the Comprehensive Nuclear Test Ban Treaty. Here, we present data from phase II testing of a new system, Xenon International at RN33, July 14th, 2021 to Jan 22nd, 2022, together with SPALAX data from the same time period. Radioxenon could be detected in 473 of 719 samples, among them many multiple isotope detections. Activity concentrations of spiked and selected environmental samples were verified by laboratory reanalysis. Finally, the sensitivity of Xenon International for radioxenons is up to one order of magnitude better for the metastable isotopes than that of the SPALAX, with a shorter sampling duration of 6 h.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Development and Testing of Neutron Cross Section Covariance Data for SCALE 6.2

Neutron cross-section covariance data are essential for many sensitivity/uncertainty and uncertainty quantification assessments performed both within the TSUNAMI suite and more broadly throughout the SCALE code system. The release of ENDF/B-VII.1 included a more complete set of neutron cross-section covariance data: these data form the basis for a new cross-section covariance library to be released in SCALE 6.2. A range of testing is conducted to investigate the properties of these covariance data and ensure that the data are reasonable. These tests include examination of the uncertainty in critical experiment benchmark model k eff values due to nuclear data uncertainties, as well as similarity assessments of irradiated pressurized water reactor (PWR) and boiling water reactor (BWR) fuel with suites of critical experiments. The contents of the new covariance library, the testing performed, and the behavior of the new covariance data are described in this paper. The neutron cross-section covariances can be combined with a sensitivity data file generated using the TSUNAMI suite of codes within SCALE to determine the uncertainty in system k eff caused by nuclear data uncertainties. The Verified, Archived Library of Inputs and Data (VALID) maintained at Oak Ridge National Laboratory (ORNL) contains over 400 critical experiment benchmark models, and sensitivity data are generated for each of these models. The nuclear data uncertainty in k eff is generated for each experiment, and the resulting uncertainties are tabulated and compared to the differences in measured and calculated results. The magnitude of the uncertainty for categories of nuclides (such as actinides, fission products, and structural materials) is calculated for irradiated PWR and BWR fuel to quantify the effect of covariance library changes between the SCALE 6.1 and 6.2 libraries. One of the primary applications of sensitivity/uncertainty methods within SCALE is the assessment of similarities between benchmark experiments and safety applications. This is described by a c k value for each experiment with each application. Several studies have analyzed typical c k values for a range of critical experiments compared with hypothetical irradiated fuel applications. The c k value is sensitive to the cross-section covariance data because the contribution of each nuclide is influenced by its uncertainty; large uncertainties indicate more likely bias sources and are thus given more weight. Changes in c k values resulting from different covariance data can be used to examine and assess underlying data changes. These comparisons are performed for PWR and BWR fuel in storage and transportation systems.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

End-to-End Demonstrator of the Safe Affordable Fission Engine (SAFE) 30: Power Conversion and Ion Engine Operation

The Safe Affordable Fission Engine (SAFE) test series addresses Phase 1 Space Fission Systems issues in particular non-nuclear testing and system integration issues leading to the testing and non-nuclear demonstration of a 400-kW fully integrated flight unit. The first part of the SAFE 30 test series demonstrated operation of the simulated nuclear core and heat pipe system. Experimental data acquired in a number of different test scenarios will validate existing computational models, demonstrated system flexibility (fast start-ups, multiple start-ups/shut downs), simulate predictable failure modes and operating environments. The objective of the second part is to demonstrate an integrated propulsion system consisting of a core, conversion system and a thruster where the system converts thermal heat into jet power. This end-to-end system demonstration sets a precedent for ground testing of nuclear electric propulsion systems. The paper describes the SAFE 30 end-to-end system demonstration and its subsystems.

Hrbud, Ivana↗

An End-To-End Test of A Simulated Nuclear Electric Propulsion System

The Safe Affordable Fission Engine (SAFE) test series addresses Phase I Space Fission Systems issues in it particular non-nuclear testing and system integration issues leading to the testing and non-nuclear demonstration of a 400-kW fully integrated flight unit. The first part of the SAFE 30 test series demonstrated operation of the simulated nuclear core and heat pipe system. Experimental data acquired in a number of different test scenarios will validate existing computational models, demonstrated system flexibility (fast start-ups, multiple start-ups/shut downs), simulate predictable failure modes and operating environments. The objective of the second part is to demonstrate an integrated propulsion system consisting of a core, conversion system and a thruster where the system converts thermal heat into jet power. This end-to-end system demonstration sets a precedent for ground testing of nuclear electric propulsion systems. The paper describes the SAFE 30 end-to-end system demonstration and its subsystems.

VanDyke, Melissa↗

When the dust settles: stable xenon isotope constraints on the formation of nuclear fallout

Nuclear weapons represent one of the most immediate threats of mass destruction. In the event that a procured or developed nuclear weapon is detonated in a populated metropolitan area, timely and accurate nuclear forensic analysis and fallout modeling would be needed to support attribution efforts and hazard assessments. In this work, we demonstrate that fissiogenic xenon isotopes retained in radioactive fallout generated by a nuclear explosion provide unique constraints on (1) the timescale of fallout formation, (2) chemical fractionation that occurs when fission products and nuclear fuel are incorporated into fallout, and (3) the speciation of fission products in the fireball. Our data suggest that, in near surface nuclear tests, the presence of a significant quantity of metal in a device assembly, combined with a short time allowed for mixing with the ambient atmosphere (seconds), may prevent complete oxidation of fission products prior to their incorporation into fallout. Xenon isotopes thus provide a window into the chemical composition of the fireball in the seconds that follow a nuclear explosion, thereby improving our understanding of the physical and thermo-chemical conditions under which fallout forms.

63 RADIATION, THERMAL, AND OTHER ENVIRON. POLLUTAN↗