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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 217 records · Page 12

Differential charge radii: Proton-neutron interaction effects

The analysis of self-consistency and proton-neutron interaction effects in the buildup of differential charge radii were carried out in covariant density functional theoretical calculations without pairing interaction on the example of selected configurations in the Pb isotopes. The proton-neutron interaction of neutron(s) added to the neutron 𝑁 = 126 core and the protons forming the 𝑍 = 82 proton core is responsible for a major contribution to the buildup of differential charge radii. It depends on the products of proton and neutron wave functions and thus on their nodal structure. This interaction leads to a redistribution of single-particle density of occupied proton states which in turn modifies the charge radii. Furthermore, the microscopic origin of this redistribution and its consequences for differential charge radii were investigated for the first time. Self-consistency effects affecting the shape of proton potential, total proton densities and the energies of the single-particle proton states provide only minor contribution to differential charge radii.

190 ≤ A ≤ 219↗

Primary $\gamma$-ray intensities and $\gamma$-strength functions from discrete two-step $\gamma$-ray cascades in radiative proton-capture experiments

Background: Reaction rates of radiative capture reactions can play a crucial role in the nucleosynthesis of heavy nuclei in explosive stellar environments. These reaction rates depend strongly on $\gamma$-ray decay widths in the reaction products, which are, for nonresonant capture reactions at high excitation energies, derived from the $\gamma$-ray strength function and the nuclear level density. Recently, the ratio method was applied to primary $\gamma$ rays observed from ($\textit{d, p}$) reactions and nuclear resonance fluorescence measurements to extract the dipole strength in atomic nuclei and to test the generalized Brink-Axel hypothesis. Purpose: The purpose of this work is to apply the ratio method to primary $\gamma$-ray intensities of the 63,65 Cu($\textit{p},\gamma$) reactions to extract $\gamma$-ray strength information on the nuclei 64,66 Zn. Here, the impact of spin distribution, total $\gamma$-ray decay widths, level densities, and width fluctuations on the application of the ratio method will be discussed. Additionally, by comparing the relative $\gamma$-ray strength at different excitation energies, conclusions on the validity of the generalized Brink-Axel hypothesis can be made. Method: The radiative proton capture reaction measurements have been performed at the HORUS $\gamma$-ray spectrometer of the University of Cologne at one excitation energy for each reaction. Primary $\gamma$-ray intensities have been determined by normalizing secondary $\gamma$-ray transitions in two-step cascades using their absolute branching ratio. The ratio method was applied to the measured primary $\gamma$-ray intensities as well as to previous measurements by Erlandsson et al. at different excitation energies. Results: The relative strength function curve for 64 Zn from our measurement shows no significant deviation from the previous measurement at a different excitation energy. The same is true for 66 Zn where both measurements were at almost the same excitation energy. Absolute $\gamma$-strength function values have been obtained by normalizing the relative curves to quasiparticle random phase approximation calculations because of the absence of experimental data in the respective energy region. Conclusion: The generalized Brink-Axel hypothesis, i.e., the independence of the strength function on the excitation energy, seems to hold in the studied energy region and nuclei. The method to obtain primary $\gamma$-ray intensities from two-step cascade spectra was shown to be a valuable and sensitive tool although its uncertainties are connected to the knowledge of the low-energy level scheme of the investigated nucleus. The scaling in the ratio method should be taken with care, because the relative strength is not a simple sum of $f_{E1}$ and $f_{M1}$ but a somewhat complex linear combination dependent on the excitation energy of the nucleus.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Statistical (n,$$\gamma $$) cross section model comparison for short-lived nuclei

Abstract Neutron-capture cross sections of neutron-rich nuclei are calculated using a Hauser–Feshbach model when direct experimental cross sections cannot be obtained. A number of codes to perform these calculations exist, and each makes different assumptions about the underlying nuclear physics. We investigated the systematic uncertainty associated with the choice of Hauser-Feshbach code used to calculate the neutron-capture cross section of a short-lived nucleus. The neutron-capture cross section for $$^{73}\hbox {Zn}$$ 73 Zn (n, $$\gamma $$ γ ) $$^{74}\hbox {Zn}$$ 74 Zn was calculated using three Hauser-Feshbach statistical model codes: TALYS, CoH, and EMPIRE. The calculation was first performed without any changes to the default settings in each code. Then an experimentally obtained nuclear level density (NLD) and $$\gamma $$ γ -ray strength function ( $$\gamma \hbox {SF}$$ γ SF ) were included. Finally, the nuclear structure information was made consistent across the codes. The neutron-capture cross sections obtained from the three codes are in good agreement after including the experimentally obtained NLD and $$\gamma \hbox {SF}$$ γ SF , accounting for differences in the underlying nuclear reaction models, and enforcing consistent approximations for unknown nuclear data. It is possible to use consistent inputs and nuclear physics to reduce the differences in the calculated neutron-capture cross section from different Hauser-Feshbach codes. However, ensuring the treatment of the input of experimental data and other nuclear physics are similar across multiple codes requires a careful investigation. For this reason, more complete documentation of the inputs and physics chosen is important.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Global optimization of harmonic oscillator basis in covariant density functional theory

The present investigation focuses on the improvement of the accuracy of the description of binding energies within moderately sized fermionic basis. Using the solutions corresponding to infinite fermionic basis it was shown that in the case of meson exchange (ME) covariant energy density functionals (CEDFs) the global accuracy of the description of binding energies in the finite $N_F$ = 16 - 20 bases can be drastically (by a factor ranging from ~3 up to ~9 dependent on the functional and $N_F$) improved by a global optimization of oscillator frequency of the basis. This is a consequence of the unique feature of the ME functionals in which with increasing fermionic basis size fermionic and mesonic energies approach the exact (infinite basis) solution from above and below, respectively. As a consequence, an optimal oscillator frequency $\hbar\omega_0$ of the basis can be defined which provides an accurate reproduction of exact total binding energies by the ones calculated in truncated basis. This leads to a very high accuracy of the calculations in moderately sized $N_F=20$ basis when mass dependent oscillator frequency is used: global rms differences $\delta B_{rms}$ between the binding energies calculated in infinite and truncated bases are only 0.025 MeV and 0.031 MeV for the NL5(Z) and DD-MEZ functionals, respectively. Optimized values of the oscillator frequency $\hbar\omega_0$ are provided for three major classes of CEDFs, i.e. for density dependent meson exchange functionals, nonlinear meson exchange ones and point coupling functionals.

Binding energy & masses↗

Accessing the Single-Particle Structure of the Pygmy Dipole Resonance in 208 Pb

New experimental data on the neutron single-particle character of the Pygmy Dipole Resonance (PDR) in Pb 208 are presented. They were obtained from ( d , p ) and resonant proton scattering experiments performed at the Q3D spectrograph of the Maier-Leibnitz Laboratory in Garching, Germany. The new data are compared to the large suite of complementary, experimental data available for Pb 208 and establish ( d , p ) as an additional, valuable, experimental probe to study the PDR and its collectivity. Furthermore, besides the single-particle character of the states, different features of the strength distributions are discussed and compared to large-scale shell model (LSSM) and energy-density functional plus quasiparticle-phonon model theoretical approaches to elucidate the microscopic structure of the PDR in Pb 208 .

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Lightweight Radiator for in Space Nuclear Electric Propulsion

Nuclear electric propulsion (NEP) is a promising option for high‐speed in‐space travel due to the high energy density of nuclear fission power sources and efficient electric thrusters. Advanced power conversion technologies may require high operating temperatures and would benefit from lightweight radiator materials. Radiator performance dictates power output for nuclear electric propulsion systems. Game‐changing propulsion systems are often enabled by novel designs using advanced materials. Pitch‐based carbon fiber materials have the potential to offer significant improvements in operating temperature, thermal conductivity, and mass. These properties combine to allow advances in operational efficiency and high temperature feasibility. An effort at the NASA Marshall Space Flight Center to show that woven high thermal conductivity carbon fiber mats can be used to replace standard metal and composite radiator fins to dissipate waste heat from NEP systems is ongoing. The goals of this effort are to demonstrate a proof of concept, to show that a significant improvement of specific power (power/mass) can be achieved, and to develop a thermal model with predictive capabilities making use of constrained input parameter space. A description of this effort is presented.

Craven, Paul↗

New transitions and levels for 163 Tb obtained from β-decay studies

Transitions in 163 Tb following β decay of 163 Gd were obtained as part of investigations of γ rays emitted following 163 Euβ decay to 163 Gd. In this work, detailed analysis of the low-energy structure of 163 Tb has been carried out with these data to expand previous β-decay studies and reactions studies of levels in 163 Tb. Data were collected at the LeRIBSS station of the Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory with an array of four Clover HPGe detectors for γ rays and two plastic scintillators for β detection. The γ rays were identified as belonging to 163 Gd and 163 Tb via mass selection and γ-γ-β, γ-γ, or γ-x-ray coincidence. In total, 38 new γ-ray transitions were observed in 163 Tb from 15 newly identified levels and 12 previously identified levels. Potential energy surface calculations were performed which support a rigid prolate deformation. Previously identified unplaced transitions in 163 Tb have been placed within the level scheme of 163 Tb and additional states and transitions have been identified.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Mapping of fragmented νf 5/2 →πf 7/2 transitions in the 73 Co→ 73 Ni decay

Excited states in 73 , 75 Ni were investigated through the β decay of 73 , 75 Co in an experiment performed at the National Superconducting Cyclotron Laboratory (NSCL) at Michigan State University (MSU). The experimental results extended the level scheme of Ni 73 to 3.2-MeV excitation energy and provided the experimental information on excited states in Ni 75 . The β -delayed neutron branching ratio for Co 73 was obtained. Furthermore, the experimental results are discussed in comparison with shell-model calculations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Structure of 30 Mg explored via in-beam γ-ray spectroscopy

In the island of inversion, ground states of neutron-rich sd-shell nuclei exhibit strong admixtures of intruder configurations from the fp shell. The nucleus 30 Mg, located at the boundary of the island of inversion, serves as a cornerstone to track the structural evolution as one approaches this region. Spin-parity assignments for excited states in 30 Mg, especially negative-parity levels, have yet to be established. In the present work, the nuclear structure of 30Mg was investigated by in-beam gamma-ray spectroscopy mainly focusing on firm spin-parity determinations. High-intensity rare-isotope beams of 31 Mg, 32 Mg, 34 Si, and 35 P bombarded a Be target to induce nucleon removal reactions populating states in 30 Mg. Gamma rays were detected by the state-of-the-art gamma-ray tracking array GRETINA. For the direct one-neutron removal reaction, final-state exclusive cross sections and parallel momentum distributions were deduced. Multi-nucleon removal reactions from different projectiles were exploited to gain complementary information. With the aid of the parallel momentum distributions, an updated level scheme with revised spin-parity assignments was constructed. Spectroscopic factors associated with each state were also deduced. Results were confronted with large-scale shell-model calculations using two different effective interactions, showing excellent agreement with the present level scheme. Furthermore, a marked difference in the spectroscopic factors indicates that the full delineation of the transition into the island of inversion remains a challenge for theoretical models.

20 ≤ A ≤ 38↗

Covariant density functional theory input for r-process simulations in actinides and superheavy nuclei: The ground state and fission properties

A systematic investigation of the ground-state and fission properties of even-even actinides and superheavy nuclei with Z = 90–120 from the two-proton up to two-neutron drip lines with proper assessment of systematic theoretical uncertainties has been performed for the first time in the framework of covariant density functional theory (CDFT). Furthermore, these results provide a necessary theoretical input for the r-process modeling in heavy nuclei and, in particular, for the study of fission cycling. Four state-of-the-art globally tested covariant energy density functionals (CEDFs), namely, DD-PC1, DD-ME2, NL3*, and PC-PK1, representing the major classes of the CDFT models are employed in the present paper. Ground-state deformations, binding energies, two-neutron separation energies, α-decay Q α values and half-lives, and the heights of fission barriers have been calculated for all these nuclei. Theoretical uncertainties in these physical observables and their evolution as a function of proton and neutron numbers have been quantified and their major sources have been identified. Spherical shell closures at Z = 120, N = 184, and N = 258 and the structure of the single-particle (especially, high-j) states in their vicinities as well as nuclear matter properties of employed CEDFs are two major factors contributing to theoretical uncertainties. However, different physical observables are affected in a different way by these two factors. For example, theoretical uncertainties in calculated ground-state deformations are affected mostly by the former factor, while theoretical uncertainties in fission barriers depend on both of these factors.

190 ≤ A ≤ 219↗

Complete set of bound negative-parity states in the neutron-rich nucleus 18 N

High-resolution γ -ray spectroscopy of N 18 is performed with the Advanced GAmma Tracking Array, following deep-inelastic processes induced by an O 18 beam on a Ta 181 target. Six states are newly identified, which together with the three known excitations exhaust all negative-parity excited states expected in N 18 below the neutron threshold. Spin and parities are proposed for all located states on the basis of decay branchings and comparison with large-scale shell-model calculations performed in the p-sd space, with the YSOX interaction. Of particular interest is the location of the 0 1 - and 1 2 - excitations, which provide strong constrains for cross-shell p-sd matrix elements based on realistic interactions and help to simultaneously reproduce the ground and first-excited states in N 16 and N 18 , for the first time. Overall, understanding the N 18 structure may also have significant impact on neutron-capture cross-section calculations in r-process modeling including light neutron-rich nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Deciphering Nb 98 β decay with the Modular Total Absorption Spectrometer at ORNL

An assessment done under the auspices of the Organization for Economic Co-operation and Developement Nuclear Energy Agency (OECD-NEA) in 2007 suggested that the β decays of many abundantly produced fission products in nuclear reactors may be incomplete. In this assessment, the fission product 98 Nb was assigned the highest priority for study by total absorption spectroscopy due to its large cumulative fission branching fraction and because the β-decay data from several experiments are discrepant. To obtain the complete β-decay feeding pattern of 98 Nb and determine the impact on the average γ energy per 98 Nb β decay and v¯e emission calculations. The complete 98 Nb β-decay feeding pattern includes ground-state to ground-state β feeding and direct β feeding to the 0 + first-excited state (both have no associated γ rays), and the ground-state to excited-state β transitions followed by γ transitions to the ground state of the daughter nucleus, 98 Mo. The complete β-decay intensities of 98 Nb were measured with the Modular Total Absorption Spectrometer at Oak Ridge National Laboratory (ORNL). Here, the 98 Nb was produced by the β decay of mass 98 fission fragments at ORNL's On-Line Test Facility (OLTF) using proton-induced fission of 238 U. We find that changes to the current ENSDF assessment of 98 Nb β-decay intensity are required. We report improved uncertainties for the β-decay feeding values and report new β feedings to high-energy levels in 98 Mo. A more complete 98 Nb β-feeding pattern with improved accuracy and precision is offered. The impacts of the measured changes to the 98 Nb β-feeding pattern on both reactor decay heat calculations and predicted detection rates of reactor v¯e are presented. The Modular Total Absorption Spectrometer measurements of 98 Nb demonstrate the importance of reexamining and remeasuring complex β-decaying fission products with total absorption spectroscopy, including nuclei very near β stability.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Reinvestigation of the level structures of the N=49 isotones 89 Zr and 91 Mo

Here, excited states of 89 Zr and 91 Mo have been investigated using the fusion reaction 6 Li+ 89 Y at beam energy of 34 MeV. Based on new experimental data, about 16 (13) new transitions have been added to the level scheme of 89 Zr ( 91 Mo). The level structures are investigated in the framework of the spherical-basis shell model using the effective interactions JUN45 and GWBXG. Reasonable agreement is obtained between the experimental results and the calculations. The calculated results indicate the newly proposed states are characterized by proton excitations from the 1f 5/2 , 2p 3/2 , 2p 1/2 orbits to the high-j 1g 9/2 orbit. The systematic features of low lying states in the N = 49 isotones are discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Microscopic constraints for the equation of state and structure of neutron stars: A Bayesian model mixing framework

Bayesian model mixing (BMM) is a statistical technique that can combine constraints from different regions of an input space in a principled way. Here we extend our BMM framework for the equation of state (EOS) of strongly interacting matter from symmetric nuclear matter to asymmetric matter, specifically focusing on zero-temperature, charge-neutral, 𝛽-equilibrated matter. We use Gaussian processes (GPs) to infer constraints on the neutron-star matter EOS at intermediate densities from two different microscopic theories: chiral effective-field theory (𝜒⁢EFT) at baryon densities around nuclear saturation, 𝑛 𝐵 ∼ 𝑛 0 , and perturbative QCD at asymptotically high baryon densities, 𝑛 𝐵 ⩾ 20⁢𝑛 0 . The uncertainties of the 𝜒⁢EFT and pQCD EOSs are obtained using the BUQEYE truncation error model. We demonstrate the flexibility of our framework through the use of two categories of GP kernels: conventional stationary kernels and a nonstationary changepoint kernel. We use the latter to explore potential constraints on the dense matter EOS by including exogenous data representing theory predictions and heavy-ion collision measurements at densities ⩾ 2⁢𝑛 0 . We also use our EOSs to obtain neutron-star mass-radius relations and their uncertainties. Finally, our framework, whose implementation will be available through a GitHub repository, provides a prior distribution for the EOS that can be used in large-scale neutron-star inference frameworks.

Bayesian methods↗

Assessing the impact of uniform rotation on the structure of neutron stars

Driven by recent laboratory experiments and astronomical observations, significant advances have deepened our understanding of neutron-star physics. NICER's Pulse Profile Modeling has refined our knowledge of neutron star masses and radii, while gravitational-wave detections have revealed key insights into the structure of neutron stars. Particularly relevant is the extraction of the tidal deformability by the LIGO-Virgo collaboration and the most recent determination of stellar radii by NICER, both suggesting a relatively soft equation of state (EOS) at intermediate densities. Additionally, measurements from the PREX collaboration and from pulsar timing suggest instead that the EOS is stiff in the vicinity of saturation density and at the highest densities accessible to date. But how stiff can the EOS be at these very high densities? Recent events featuring compact objects near the “lower mass gap” have raised questions about the existence of very massive neutron stars. Motivated by this finding and in light of new refinements to theoretical models, we explore the possibility that these massive objects may indeed be rapidly rotating neutron stars. Here, we explore how rotation affects both the maximum neutron star mass and their associated radii, and discuss the implications they may have on the equation of state.

Equations of state of nuclear matter↗

Lightweight Damage Tolerant Radiators for In-Space Nuclear Electric Power and Propulsion

Nuclear electric propulsion (NEP) is a promising option for high-speed in-space travel due to the high energy density of nuclear power sources and efficient electric thrusters. Advanced power conversion technologies for converting thermal energy from the reactor to electrical energy at high operating temperatures would benefit from lightweight, high temperature radiator materials. Radiator performance dictates power output for nuclear electric propulsion systems. Pitch-based carbon fiber materials have the potential to offer significant improvements in operating temperature and mass. An effort at the NASA Marshall Space Flight Center to show that woven high thermal conductivity carbon fiber mats can be used to replace standard metal and composite radiator fins to dissipate waste heat from NEP systems is ongoing. The goals of this effort are to demonstrate a proof of concept, to show that a significant improvement of specific power (power/mass) can be achieved, and to develop a thermal model with predictive capabilities. A description of this effort is presented.

Craven, Paul↗