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At least 217 records · Page 12

Effect of particle size in composite materials on radiative properties

A numerical model for the radiative properties of a composite material composed of ceramic oxide fibers and particles was developed and used to determine the effect of the size parameters of the two components. Results include the computed phase functions for the zirconia and silica composite materials, showing the location and strength of the strong forward-scattering peak. The phase function and the optical properties of the composite are strongly influenced by the particle size parameter through the fiber or particle diameter and the wavelength, the material, and the mixture fraction.

Lee, Siu-Chun↗

Photographic method measures particle size and velocity in fluid stream

Method employing a nonframing motion picture camera, a continuous front light source, and a strobe light determines the size and velocity of small particles in nonturbulent fluid streams. This method is used in the study of the motion of solid and liquid particles in research and industrial fluid flow systems.

Dickerson, R. A.↗

A fiber-optic probe for particle sizing in concentrated suspensions

A fiber-optic probe employing two monomode optical fibers, one for transmitting a Gaussian laser beam to the scattering volume and the second, positioned at some backscatter angle, for receiving the scattered light is described. Performance and suitability of the system for a process control environment is assessed by studying a suspension of polystyrene latex particles over a wide range of sizes and concentrations. The results show that the probe is ideal for a process control environment in industrial and laboratory applications. Particle size is recovered, without any additional corrections for multiple light scattering, in concentrations containing up to 10 percent solids of 39-nm polystyrene latex spheres.

Dhadwal, Harbans S.↗

Production of large-particle-size monodisperse latexes

The research program achieved two objectives: (1) it has refined and extended the experimental techniques for preparing monodisperse latexes in quantity on the ground up to a particle diameter of 10 microns; and (2) it has demonstrated that a microgravity environment can be used to grow monodisperse latexes to larger sizes, where the limitations in size have yet to be defined. The experimental development of the monodisperse latex reactor (MLR) and the seeded emulsion polymerizations carried out in the laboratory prototype of the flight hardware, as a function of the operational parameters is discussed. The emphasis is directed towards the measurement, interpretation, and modeling of the kinetics of seeded emulsion polymerization and successive seeded emulsion polymerization. The recipe development of seeded emulsion polymerization as a function of particle size is discussed. The equilibrium swelling of latex particles with monomers was investigated both theoretically and experimentally. Extensive studies are reported on both the type and concentration of initiators, surfactants, and inhibitors, which eventually led to the development of the flight recipes. The experimental results of the flight experiments are discussed, as well as the experimental development of inhibition of seeded emulsion polymerization in terms of time of inhibition and the effect of inhibitors on the kinetics of polymerization.

Vanderhoff, J. W.↗

Laser Doppler spectrometer method of particle sizing

A spectrometer for the detection of airborne particulate pollution in the submicron size range is described. In this device, airborne particles are accelerated through a supersonic nozzle, with different sizes achieving different velocities in the gas flow. Information about the velocities of the accelerated particles is obtained with a laser-heterodyne optical system through the Doppler shift of light scattered from the particles. Detection is accomplished by means of a photomultiplier. Nozzle design and signal processing techniques are also discussed.

Weber, F. N.↗

Particle sizes of the Uranus delta ring's inner diffuse companion through comparison of RSS and PPS Voyager occultation data

In January, 1976, Voyager 2's photopolarimeter and UV spectrometer observed Delta Sagitarii and Beta Persei during their occultation by the Uranian delta ring. An inner diffuse companion of this ring was detected and found to have an average width of 12 km. By comparing the widths and equivalent depths of the two sets of data, it is established that the particles making the greatest contribution to the integrated opacities of the companion are of greater-than-several-cm sizes. The particles appear to be located away from the photopolarimetry edges, where there may be particles smaller than those observed elsewhere.

Hui, John↗

Pinatubo and pre-Pinatubo optical-depth spectra: Mauna Loa measurements, comparisons, inferred particle size distributions, radiative effects, and relationship to lidar data

The Ames airborne tracking sunphotometer was operated at the National Oceanic and Atmospheric Administration (NOAA) Mauna Loa Observatory (MLO) in 1991 and 1992 along with the NOAA Climate Monitoring and Diagnostics Laboratory (CMDL) automated tracking sunphotometer and lidar. June 1991 measurements provided calibrations, optical-depth spectra, and intercomparisons under relatively clean conditions; later measurements provided spectra and comparisons for the Pinatubo cloud plus calibration checks. June 1991 results are similar to previous MLO springtime measurements, with midvisible particle optical depth at the near-background level of 0.012 +/- 0.006 and no significant wavelength dependence in the measured range (lambda = 0.38 to 1.06 micrometers). The arrival of the Pinatubo cloud in July 1991 increased midvisible particle optical depth by more than an order of magnitude and changed the spectral shape of to an approximate power law with an exponent of about -1.4. By clearly September 1991, the spectrum was broadly peaked near 0.5 micrometers, and by July 1992, it was peaked near 0.8 micrometers. Our optical-depth spectra include corrections for diffuse light. NOAA- and Ames Research Center (ARC)-measured spectra are in good agreement. Columnar size distributions inverted from the spectra show that the initial (July 1991) post-Pinatubo cloud was relatively rich in small particles (r less than 0.25 micrometers), which were progressively depleted in the August-September 1991 and July 1992 periods. Conversely, both of the later periods had more of the optically efficient medium-sized particles (0.25 less than r less than 1 micrometers) than did the fresh July 1991 cloud. These changes are consistent with particle growth by condensation and coagulation. Photometer-inferred column backscatter values agree with those measured by the CMDL lidar on nearby nights. Combining lidar-measured backscatter profiles with photometer-derived backscatter-to-area ratios gives peak particle areas that could cause rapid heterogeneous loss of ozone, given sufficiently low particle acidity and suitable solar zenith angles (achieved at mid- to high latitudes). Top-of-troposphere radiative forcings for the September 1991 and July 1992 optical depths and size distributions over MLO are about -5 and -3 W/sq m, respectively (hence comparable in magnitude but opposite in sign to the radiative forcing caused by the increase in manmade greenhouse gases since the industrial revolution). Heating rates in the Pinatubo layer over MLO are 0.55 +/- 0.13 and 0.41 +/- 0.14 K/d for September 1991 and July 1992, respectively.

Russell, P. B.↗

Pinatubo and Pre-Pinatubo Optical-Depth Spectra: Mauna Loa Measurements, Comparisons, Inferred Particle Size Distributions, Radiative Effects, and Relationship to Lidar Data

The Ames airborne tracking sunphotometer was operated at the National Oceanic and Atmospheric Administration (NOAA) Mauna Loa Observatory (MLO) in 1991 and 1992 along with the NOAA Climate Monitoring and Diagnostics Laboratory (CMDL) automated tracking sunphotometer and lidar. June 1991 measurements provided calibrations, optical-depth spectra, and intercomparisons under relatively clean conditions; later measurements provided spectra and comparisons for the Pinatubo cloud plus calibration checks. June 1991 results are similar to previous MLO springtime measurements, with midvisible particle optical depth tau(sub p)(lambda = 0.526 microns) at the near-background level of 0.012 +/- 0.006 and no significant wavelength dependence in the measured range (lambda = 0.38 to 1.06 microns). The arrival of the Pinatubo cloud in July 1991 increased midvisible particle optical depth by more than an order of magnitude and changed the spectral shape of tau(sub p)(lambda) to an approximate power law with an exponent of about -1.4. By early September 1991, the spectrum was broadly peaked near 0.5 microns, and by July 1992, it was peaked near 0.8 microns. Our optical-depth spectra include corrections for diffuse light which increase postvolcanic midvisible tau(sub p) values by 1 to 3% (i.e., 0.0015 to 0.0023). NOAA- and Ames Research Center (ARC)-measured spectra are in good agreement. Columnar size distributions inverted from the spectra show that the initial (July 1991) post-Pinatubo cloud was relatively rich in small particles (r less than 0.25 microns), which were progressively depleted in the August-September 1991 and July 1992 periods. Conversely, both of the later periods had more of the optically efficient medium-sized particles (0.25 less than r less than 1 micron) than did the fresh July 1991 cloud. These changes are consistent with particle growth by condensation and coagulation. The effective, or area-weighted, radius increased from 0.22 +/- 0.06 micron in July 1991 to 0.56 +/- 0.12 micron in August-September 1991 and to 0.86 +/- 0.29 micron in July 1992. Corresponding column mass values were 4.8 +/- 0.7, 9.1 +/- 2.7, and 5.5 +/- 2 micro g/sq cm, and corresponding column surface areas were 4.4 +/- 0.5, 2.9 +/- 0.2, and 1.1 +/- 0.1 sq micron/sq cm,. Photometer-inferred column backscatter values agree with those measured by the CMDL lidar on nearby nights. Combining lidar-measured backscatter profiles with photometer-derived backscatter-to-area ratios gives peak particle areas that could cause rapid heterogeneous loss of ozone, given sufficiently low particle acidity and suitable solar zenith angles (achieved at mid- to high latitudes). Top-of-troposphere radiative forcings for the September 1991 and July 1992 optical depths and size distributions over MLO are about -5 and -3 W 1/sq m, respectively (hence comparable in magnitude but opposite in sign to the radiative forcing caused by the increase in manmade greenhouse gases since the industrial revolution). Heating rates in Pinatubo layer over MLO are 0.55 +/- 0.13 and 0.41 +/- 0.14 K/d for September 1991 and July 1992, respectively.

Russell, P. B.↗

Particle sizes and composition of Mars atmospheric dust based upon Viking and Mariner 9 observations

Mars atmospheric dust can play an important role in the thermal structure of the Mars atmosphere during periods of high dust loading. However, the radiative properties of Mars atmospheric dust remain uncertain due to uncertain definitions of the dust composition and size distribution. The analysis by Toon et al., of Mariner 9 IRIS spectra during the 1971-1972 global dust storm indicated a reasonable match between the modeled 9-micron absorption of montmorillinite and the observed 9-micron absorption. Toon et al. also determined that an effective (cross-section weighted) mean radius of 2.5 microns (R(sub mode) = 0.4 microns) provided a consistent fit of montmorillinite to the IRIS dust spectra at 9 microns. Pollack et al. analyzed Viking lander observations of atmospheric extinction and scattering at visible-near IR wavelengths (0.5-1.0 microns), and obtained consistency with the Toon et al. dust size distribution when the effects of nonspherical particle shapes were included. An additional, minor (1 percent) component of visible-ultraviolet absorbing material was required to model the derived visible (0.86) and ultraviolet (0.4-0.6) single-scattering albedos of the dust, since montmorillinite does not absorb sufficiently in this wavelength region. A combined analysis of the Viking IRTM and Mariner 9 observations was conducted to reassess the model of Mars atmospheric ultraviolet-to-infrared measurements of dust absorption and scattering. The optical constants for palagonite are incorporated in a doubling-adding radiative transfer model of the Mars atmosphere to simulate Mariner 9 IRIS spectra as well as the Viking IRTM IR band observations. Visible and ultraviolet single-scattering albedos based on the Hansen and Travis Mie scattering code were also derived. A tentative conclusion is that smaller dust particles (R(sub mode) = 0.15 microns, cross-section weighted mean R = 1.2 microns) composed of palagonite provide a much improved fit to the Mariner 9 IRIS spectra; agreement with the observed ratio of visible-to-infrared extinction opacities; and ultraviolet and visible single-scattering albedos comparable to their observed values.

Clancy, R. T.↗

Scattering and Absorption Properties of Polydisperse Wavelength-sized Particles Covered with Much Smaller Grains

Using the results of direct, numerically exact computer solutions of the Maxwell equations, we analyze scattering and absorption characteristics of polydisperse compound particles in the form of wavelength-sized spheres covered with a large number of much smaller spherical grains.The results pertain to the complex refractive indices1.55 + i0.0003,1.55 + i0.3, and 3 + i0.1. We show that the optical effects of dusting wavelength-sized hosts by microscopic grains can vary depending on the number and size of the grains as well as on the complex refractive index. Our computations also demonstrate the high efficiency of the new superposition T-matrix code developed for use on distributed memory computer clusters.

Dlugach, Jana M.↗

Interaction of Wheat Bran Particle Size and Stimbiotic Supplementation on Growth Performance and Gut Health Parameters in Broilers

A 42-day study was conducted with 720-day-old Cobb male broiler chicks allocated to treatments in a 3 × 2 factorial, with the factors as wheat bran (WB) inclusion (no WB, 50 g/kg coarse WB, or 50 g/kg fine WB) and stimbiotic (STB) supplementation in corn-based diets. The inclusion of WB (p < 0.05) or STB supplementation (p < 0.05) increased the FCR and feed intake in the day 0–10 phase. During the day 0–28 phase, coarse-WB inclusion increased (p < 0.05) the FCR, compared to fine WB or diets without WB. In the day 0–42 phase, WB marginally decreased weight gain in diets without STB supplementation, but the STB-supplemented diet, weight gain was greater (p < 0.05) the diet with fine WB compared with diets with coarse WB. Fine-WB inclusion increased the ileal nitrogen and energy digestibility determined at day 18 compared to coarse WB or diets without WB. Supplementation with STB (p < 0.05) or fine WB (p < 0.05) inclusion increased the villi height compared to diets without STB supplementation or coarse WB, or the diet without WB. Coarse or fine WB decreased (p < 0.05) cecal branched-chain fatty acids compared to diets without WB. In conclusion, stimbiotic supplementation to fine WB improved the performance and nutrient digestibility of broilers compared to coarse WB with no effects on the caeca total SCFA concentration.

60 APPLIED LIFE SCIENCES↗

Assessment of Holographic Microscopy for Quantifying Marine Particle Size and Concentration

Holographic microscopy has emerged as a tool for in situ imaging of microscopic organisms and other particles in the marine environment: appealing because of relatively larger sampling volumes and simpler optical configurations compared to similar imaging systems. However, its quantitative capabilities have remained uncertain, in part because hologram reconstruction and image recognition have required manual operation. Here we assess the quantitative skill of our automated hologram processing pipeline, the CCV Pipeline, to evaluate the size and concentration measurements of environmental and cultured assemblages of marine plankton particles, and microspheres. Over one-million particles, ranging from 10-200 microns equivalent spherical diameter (ESD), imaged by the 4-Deep HoloSea digital inline holographic microscope (DIHM) are analyzed. These measurements were collected in parallel with FlowCam, Imaging FlowCytobot, and manual microscope identification. Once corrections for particle location and nonuniform illumination were developed and applied, the DIHM showed an underestimate in ESD of about 3-10%, but successfully reproduced the size-spectral-slope from environmental samples, and the size distribution of monocultures and microspheres. DIHM concentrations (order 1-1000 particles~ml-1) showed linear agreement (r^2=0.73) with the other instruments, but individual comparisons at times had large uncertainty.

holograpy↗

Assessment of holographic microscopy for quantifying marine particle size and concentration

Holographic microscopy has emerged as a tool for in situ imaging of microscopic organisms and other particles in the marine environment: appealing because of the relatively larger sampling volume and simpler optical configuration compared to other imaging systems. However, its quantitative capabilities have so far remained uncertain, in part because hologram reconstruction and image recognition have required manual operation. Here, we assess the quantitative skill of our automated hologram processing pipeline (CCV Pipeline), to evaluate the size and concentration measurements of environmental and cultured assemblages of marine plankton particles, and microspheres. Over 1 million particles, ranging from 10 to 200 μm in equivalent spherical diameter, imaged by the 4‐Deep HoloSea digital inline holographic microscope (DIHM) are analyzed. These measurements were collected in parallel with a FlowCam (FC), Imaging FlowCytobot (IFCB), and manual microscope identification. Once corrections for particle location and nonuniform illumination were developed and applied, the DIHM showed an underestimate in ESD of about 3% to 10%, but successfully reproduced the size spectral slope from environmental samples, and the size distribution of cultures (Dunaliella tertiolecta, Heterosigma akashiwo, and Prorocentrum micans) and microspheres. DIHM concentrations (order 1 to 1000 particles ml(exp −1)) showed a linear agreement (r(exp 2) = 0.73) with the other instruments, but individual comparisons at times had large uncertainty. Overall, we found the DIHM and the CCV Pipeline required extensive manual correction, but once corrected, provided concentration and size estimates comparable to the other imaging systems assessed in this study. Holographic cameras are mechanically simple, autonomous, can operate at very high pressures, and provide a larger sampling volume than comparable lens‐based tools. Thus, we anticipate that these characterization efforts will be rewarded with novel discovery in new oceanic environments.

Noah L. Walcutt↗

Vertical Variation of Ice Particle Size in Convective Cloud Tops

A novel technique is used to estimate derivatives of ice effective radius with respect to height near convective cloud tops (dr(sub e)/dz) from airborne shortwave reflectance measurements and lidar. Values of dr(sub e)/dz are about −6 micrometer/km for cloud tops below the homogeneous freezing level, increasing to near 0 micrometer/km above the estimated level of neutral buoyancy. Retrieved dr(sub e)/dz compares well with previously documented remote sensing and in situ estimates. Effective radii decrease with increasing cloud top height, while cloud top extinction increases. This is consistent with weaker size sorting in high, dense cloud tops above the level of neutral buoyancy where fewer large particles are present and with stronger size sorting in lower cloud tops that are less dense. The results also confirm that cloud top trends of effective radius can generally be used as surrogates for trends with height within convective cloud tops. These results provide valuable observational targets for model evaluation.

cloud height indicators↗