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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 217 records · Page 12
All sourcesNASA NTRSDOE OSTI
NASA NTRS2008

Thermal Expansion Studies of Selected High Temperature Thermoelectric Materials

Radioisotope thermoelectric generators (RTGs) generate electrical power by converting the heat released from the nuclear decay of radioactive isotopes (typically plutonium-238) into electricity using a thermoelectric converter. RTGs have been successfully used to power a number of space missions and have demonstrated their reliability over an extended period of time (tens of years) and are compact, rugged, radiation resistant, scalable, and produce no noise, vibration or torque during operation. System conversion efficiency for state-of-practice RTGs is about 6% and specific power less than or equal to 5.1 W/kg. Higher specific power would result in more on-board power for the same RTG mass, or less RTG mass for the same on-board power. The Jet Propulsion Laboratory has been leading, under the advanced thermoelectric converter (ATEC) project, the development of new high-temperature thermoelectric materials and components for integration into advanced, more efficient RTGs. Thermoelectric materials investigated to date include skutterudites, the Yb14MnSb11 compound, and SiGe alloys. The development of long-lived thermoelectric couples based on some of these materials has been initiated and is assisted by a thermo-mechanical stress analysis to ensure that all stresses under both fabrication and operation conditions will be within yield limits for those materials. Several physical parameters are needed as input to this analysis. Among those parameters, the coefficient of thermal expansion (CTE) is critically important. Thermal expansion coefficient measurements of several thermoelectric materials under consideration for ATEC are described in this paper. The stress response at the interfaces in material stacks subjected to changes in temperature is discussed, drawing on work from the literature and project-specific tools developed here. The degree of CTE mismatch and the associated effect on the formation of stress is highlighted.

silicon germanium↗
NASA NTRS2021

HARM3D+NUC: A New Method for Simulating the Post-merger Phase of Binary Neutron Star Mergers with GRMHD, Tabulated EOS, and Neutrino Leakage

The first binary neutron star merger has already been detected in gravitational waves. The signal was accompanied by an electromagnetic counterpart including a kilonova component powered by the decay of radioactive nuclei, as well as a short γ-ray burst. In order to understand the radioactively powered signal, it is necessary to simulate the outflows and their nucleosynthesis from the post-merger disk. Simulating the disk and predicting the composition of the outflows requires general relativistic magnetohydrodynamical (GRMHD) simulations that include a realistic, finite-temperature equation of state (EOS) and self-consistently calculating the impact of neutrinos. In this work, we detail the implementation of a finite-temperature EOS and the treatment of neutrinos in the GRMHD code HARM3D+NUC, based on HARM3D. We include formal tests of both the finite-temperature EOS and the neutrino-leakage scheme. We further test the code by showing that, given conditions similar to those of published remnant disks following neutron star mergers, it reproduces both recombination of free nucleons to a neutron-rich composition and excitation of a thermal wind.

Ariadna Murguia-Berthier↗
NASA NTRSDate not supplied

Phosphate (U-Th)/He Thermochronology of Apollo 14 Melt Breccia 14311

Our ability to confidently characterize the impact history of the inner solar system is limited by discrepancies in radiometric dates and age interpretations for lunar rocks, impact melts, and recovered meteorites. It is therefore important to explore different thermally sensitive radiometric systems to unravel the timing and extent of the long term impact flux. Low-temperature thermochronology of lunar samples has the potential to provide more complementary geochronological datasets and further test dynamical models related to the evolution of the inner solar system (e.g., [1]). (U-Th)/He dating is based on the production of 4He atoms by radioactive alpha decay of U and Th (and to a lesser extent, Sm) in a crystal and the thermally activated volumetric diffusion of those 4He nuclides. At high temperatures, the crystal is an open system from which 4He can escape; at lower temperatures, 4He may be retained. This retention temperature depends on factors such as crystal structure and volume fraction of radiation damage in the crystal (e.g., [2, 3]), but is significantly lower for phosphate minerals compared to the diffusion of the radiogenic daughter products in other widely used chronometric systems (e.g., ~75°C in terrestrial apatite (U-Th)/He vs. ~500°C in apatite U-Th-Pb vs. ~900°C in zircon U-Th-Pb chronometry). Phosphate (U-Th)/He dating has been used to decipher peak temperatures and cooling rates related to terrestrial impact events (e.g., [4]). Pairing a low-temperature thermochronometer with higher-temperature approaches (i.e., a combined 207Pb-206Pb and (U-Th)/He approach), can therefore resolve multiple impact ages within a given sample or even grain. However, despite its potential, phosphate (U-Th)/He dating has not been reported on any lunar samples. Here we present the first lunar phosphate (U-Th)/He thermochronology on an Apollo 14 impact melt-breccia.

C A Diaz↗
NASA NTRS1974

Experiments on the origin of molecular chirality by parity non-conservation during beta-decay

Experiments are described to test a theory for the origin of optical activity wherein the longitudinally polarized electrons resulting from parity violation during radioactive beta-decay, and their resulting circularly polarized bremsstrahlung, might interact asymmetrically with organic matter to yield optically active products. The historical background to this subject is briefly reviewed. Our experiments involve subjecting a number of racemic and optically active amino acid samples to a beta-radiation source for a period of 1.34 years (total dose: 411 Mrads), then examining them for any asymmetric effects by means of optical rotatory dispersion and analytical gas chromatography.

Bonner, W. A.↗
NASA NTRS1991

Segmented Ge detector rejection of internal beta activity produced by neutron irradiation

Future Ge spectrometers flown in space to observe cosmic gamma-ray sources will incorporate segmented detectors to reduce the background from radioactivity produced by energetic particle reactions. To demonstrate the effectiveness of a segmented Ge detector in rejecting background events due to the beta decay of internal radioactivity, a laboratory experiment has been carried out in which radioactivity was produced in the detector by neutron irradiation. A Cf-252 source of neutrons was used to produce, by neutron capture on Ge-74 (36.5 percent of natural Ge) in the detector itself, Ge-75 (t sub 1/2 = 82.78 min), which decays by beta emission with a maximum electron kinetic energy of 1188 keV. By requiring that an ionizing event deposit energy in two or more of the five segments of the detector, each about 1-cm thick, the beta particles, which have a range of about 1-mm, are rejected, while most external gamma rays incident on the detector are counted. Analysis of this experiment indicates that over 85 percent of the beta events from the decay of Ge-75 are rejected, which is in good agreement with Monte Carlo calculations.

Varnell, L. S.↗
NASA NTRSDate not supplied

Development of Radioluminescent Tritium Polymeric Material for High Visibility Applications

The Development of Radioluminescent Tritium Polymeric Material for High Visibility Applications effort investigates the nature and properties of materials consisting of tritium lights combined with various silicone adhesives. Physical, mechanical, and optical properties will be observed/measured, including their durability in the low earth orbit environment. Tritium or hydrogen-three is a radioactive isotope of hydrogen that emits beta particles as it undergoes a process called beta decay. A beta particle is a high-energy, high-speed electron (or positron) emitted from radioactive decay of an atomic nucleus. Because it is a gas, tritium must be bound to a material or encapsulated in a sealed glass container. The gaseous tritium can then be combined with a phosphor source which when struck with beta particles, fluoresces and emits light. Such a light source is referred to as a gaseous tritium light source (GTLS). A self-powered, radioluminescent tritium material capable of surviving multiple space environments has the potential to fulfill visibility requirements levied on space flight hardware and facilitate additional long term internal and external lighting needs such as for imaging, docking, tracking, and xEMU suits for lunar exploration on the moon.

Lauren Fisher↗
NASA NTRS1980

Actinide cosmic ray chronometers - Relative abundances and the cosmic ray lifetime

Measurements of ultraheavy cosmic rays will provide radioactive chronometers, including the actinides, which are expected to be present in the source. These primary chronometers differ from the Be-10 secondary chronometer in total inelastic cross-section and decay half-life. A propagation code, which includes nuclear fragmentation, radioactive decay, and ionization energy-loss of cosmic rays is being used to investigate the variations in the fluxes and mean ages which would be expected for various models of cosmic ray propagation. Some preliminary results in the actinide region are presented here which indicate that measurements of the relative abundances of the actinides in the cosmic rays will be very useful for understanding source abundances but less useful for studying propagation effects.

Margolis, S. H.↗
NASA NTRS1990

Segmented Ge detectors and mechanical coolers for future gamma-ray astronomy instruments

The effectiveness of a segmented Ge detector in rejecting background events due to the beta decay of internal radioactivity is demonstrated by a laboratory experiment in which radioactivity was produced in the detector by neutron irradiation. A Cf-252 source of neutrons was used to produce, by neutron capture on Ge-74 in the detector itself, Ge-75, which decays by beta emission with a maximum energy of 1188 keV. Simultaneous spectra are taken of the activity in the detector under two conditions: a free spectrum in which all events in the detector are accumulated, and a gated spectrum in which events are accumulated only if they deposit energy in two or more segments. A comparison of the spectra shows that over 85 percent of the beta events are rejected, which is in good agreement with predictions.

Varnell, Larry S.↗
DOE OSTI2024

SCALE Analyses of Scenarios in the Molten Salt Reactor Fuel Cycle

In support of the US Nuclear Regulatory Commission non-light-water reactor fuel cycle demonstration project, the capabilities of SCALE 6.3.1 for radionuclide characterization, criticality, and shielding were demonstrated through several scenarios in a molten salt reactor (MSR) nuclear fuel cycle. Three scenarios were selected for this study, with the molten salt breeder reactor (MSBR) serving as the reference design. The original thorium-based fuel salt used in MSBR was replaced with a 235 U-enriched fuel salt to better reflect anticipated future MSR concepts. The first scenario focused on the fuel salt preparation stage. Criticality analyses, using SCALE/CSAS-Shift and SCALE/SAMPLER, examined potential critical configurations in the fresh fuel salt container based on variables such as 235 U enrichment, UF 4 molar fraction, temperature, and container geometry. The second scenario explored the release of fission products during reactor operation in which the tritium buildup in the primary fuel salt was quantified through depletion calculations using SCALE/TRITON with continuous fuel makeup and fractional fission product removal. This scenario also assessed radioactivity levels in the off-gas system (OGS), quantifying radiotoxic nuclides that could be released into the environment. SCALE/SAMPLER was employed to perform uncertainty quantification to identify key operating parameters influencing the buildup of radiotoxic nuclides in the OGS. Additionally, radiation dose rates were calculated using SCALE/MAVRIC to estimate the maximum exposure levels within the reactor cell complex during operation. The final scenario evaluated the decay heat and radioactivity of the primary fuel salt collected in the drain tank, as well as the radiation dose rate outside the building from the presence of the drain tank. Overall, the application of SCALE’s various capabilities for radionuclide inventory generation, criticality analysis, and shielding in MSR fuel cycles was successfully demonstrated across these scenarios.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2026

Shakeup and shakeoff spectra in the electron capture decay of atomic 7 Be

The most stringent laboratory-based experimental limits on the existence of submegaelectronvolt sterile neutrinos are currently set by decay spectroscopy of radioactive 7 Be embedded into superconducting sensors. The systematic uncertainties are dominated by the modeling of the electron shakeup and shakeoff spectra that are not based on state-of-the-art atomic theory and do not include electron correlations or relativistic effects. We have used the multiconfiguration Dirac-Fock formalism to obtain correlated wave functions ab initio and compute all single and double shake processes in the electron capture decay of atomic 7 Be . The simulations can explain some but not all of the observed spectral features, likely because the wave functions are modified by the Ta sensor material that the 7 Be is embedded into. The new models also show that the 𝐿/𝐾 electron capture ratio of 7 Be in Ta has previously been slightly underestimated revising the previous value of 0.070(7) to a new value of 0.0756(20).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

Shake-up and shake-off spectra in the electron capture decay of atomic $^7$Be

The most stringent laboratory-based experimental limits on the existence of sub-MeV sterile neutrinos are currently set by decay spectroscopy of radioactive $^7$Be embedded into superconducting sensors. The systematic uncertainties are dominated by the modeling of the electron shake-up and shake-off spectra that are not based on state-of-the-art atomic theory and do not include electron correlations or relativistic effects. We have used the multiconfiguration Dirac-Fock formalism to obtain correlated wavefunctions ab initio and compute all single and double shake processes in the electron capture decay of atomic $^7$Be. The simulations can explain some but not all of the observed spectral features, likely because the wave functions are modified by the Ta sensor material that the $^7$Be is embedded into. The new models also show that the L/K electron capture ratio of $^7$Be in Ta has previously been slightly underestimated revising the previous value of 0.070(7) to a new value of 0.0756(20).

Atomic Physics (physics.atom-ph)↗
NASA NTRS2008

Simulating the Gradually Deteriorating Performance of an RTG

Degra (now in version 3) is a computer program that simulates the performance of a radioisotope thermoelectric generator (RTG) over its lifetime. Degra is provided with a graphical user interface that is used to edit input parameters that describe the initial state of the RTG and the time-varying loads and environment to which it will be exposed. Performance is computed by modeling the flows of heat from the radioactive source and through the thermocouples, also allowing for losses, to determine the temperature drop across the thermocouples. This temperature drop is used to determine the open-circuit voltage, electrical resistance, and thermal conductance of the thermocouples. Output power can then be computed by relating the open-circuit voltage and the electrical resistance of the thermocouples to a specified time-varying load voltage. Degra accounts for the gradual deterioration of performance attributable primarily to decay of the radioactive source and secondarily to gradual deterioration of the thermoelectric material. To provide guidance to an RTG designer, given a minimum of input, Degra computes the dimensions, masses, and thermal conductances of important internal structures as well as the overall external dimensions and total mass.

Wood, Eric G.↗
NASA NTRS1993

Al-26-Mg-26 ages of iron meteorites

An exposure age for an iron meteorite can be calculated from measurements of a radioactive nuclide and a stable nuclide that are produced by similar sets of nuclear reactions, provided that the stable nuclide is present with low initial abundance. The standard methods rely on either K-40 (t(sub 1/2) = 1.26 Gy), K-39, and K-41 or on a shorter-lived radionuclide and a stable, noble gas isotope. Widely used pairs of this type include Cl-36/Ar-36 and Al-26/Ne-21. Other pairs that may serve the purpose for iron meteorites contain many stable isotopes besides those of K and the noble gases that are produced partly by cosmic rays. We consider here the calculation of exposure ages, t(sub 26), from measurements of Al-26 (t(sub 1/2) = 0.7 My) and (stable) Mg-26. Ages based on Al-26/Mg-26 ratios, like those based on Cl-36/Ar-36 ratios, are 'buffered' against changes in relative production rates due to shielding because decay of the radioactive nuclide accounts for a good part of the inventory of the stable nuclide.

Herzog, G. F.↗
DOE OSTI2025

A machine learning framework for accurate and robust analysis of radiation detector pulses

The microscopic properties of atomic nuclei are used to study various scientific questions. They are essential for understanding the fundamental forces of nature and the chemical evolution of the universe. Detecting decay radiation from radioactive nuclei makes it possible to probe these fundamental nuclear properties. Detector waveform traces may contain additional information about the radiation. Generally, advanced signal processing techniques are needed to extract this additional information, often involving fitting the waveform with model response functions using non-linear least-squares optimization with second-order gradient methods. While this is a powerful technique, it is also computationally expensive, leading to slow processing time, which scales with the volume of data. To address this problem, we have developed a machine learning (ML) approach that infers the characteristics of traces from a model detector response function. In particular, we are interested in classifying whether a single recorded trace consists of one or two pulse constituents and estimating the pulse parameters. Furthermore, our proposed ML method can precisely extract the pulses’ parameters, such as energy and timing information, and accurately classify the pulse multiplicity of a trace. Unlike non-learning-based approaches, our ML approach uses neural networks that are significantly faster at inference, as they do not require any optimization during this stage.

Curve fitting↗
NASA NTRS1973

The relative abundance of the isotopes of Li, Be and B and the age of cosmic rays

Using a balloon borne double dE/dx total energy telescope, we have determined the isotopic composition of cosmic ray Li, Be and B nuclei in the energy range 100-250 MeV/nuc. The measured mass resolution for these nuclei is about 0.3 AMU. The observed isotopic composition is in agreement with that predicted on the basis of interstellar fragmentation with the exception of a deficiency of Be-10. If the low abundance of Be-10 is attributed to the decay of this radioactive isotope, we obtain a mean cosmic ray lifetime of 3.4 (plus 3.4 or minus 1.3) m.y.

Webber, W. R.↗
NASA NTRS1975

Time-dependent 2.2 MeV and 0.5 MeV lines from solar flares

The time dependences of the 2.2 MeV and 0.51 MeV gamma ray lines from solar flares are calculated and the results are compared with observations of the 1972, August 4 and 7 flares. Time lag between the nuclear reactions and the formation of these two lines are caused, respectively, by capture of the neutrons, and by deceleration of the positrons and decay of the radioactive nuclei. Results show that the calculation is consistent with the observed rise of the 2.2 MeV line on August 4, and it does not require different time dependences for the accelerated protons and electrons in the flare region. The above lags can explain the delayed gamma ray emission observed on August 7. Positrons of energies greater than about 10 MeV could be detected in interplanetary space following large solar flares.

Wang, H. T.↗
NASA NTRS1975

Time-dependent 2.2-MeV and 0.5-MeV lines from solar flares

The time dependences of the 2.2- and 0.51-MeV gamma-ray lines from solar flares are calculated, and the results are compared with observations of the 1972 August 4 and 7 flares. The time lag between the nuclear reactions and the formation of these two lines is caused by capture of the neutrons and subsequent deceleration of the positrons and decay of the radioactive nuclei. Our main results are that the calculation is consistent with the observed rise of the 2.2-MeV line on August 4, and it does not require different time dependences for the accelerated protons and high-energy electrons in the flare region. The above lags can explain the delayed gamma-ray emission observed on August 7. Positrons of energies greater than about 10 MeV could be detected in interplanetary space following large solar flares.

Wang, H. T.↗
NASA NTRS1979

Predictions of induced background radiations at gamma/X-ray experiment envelopes in NASA spacecraft

This work seeks to predict secondary radiation levels induced in spacecraft structures by space protons. The radiations analyzed are secondary neutrons from spallation and evaporation reactions and gamma and beta rays from the decay of induced radioactivity, as sources of interfering background to spaceborne measurements of galactic and planetary gamma rays below 10 MeV. The spacecraft considered are the Multi-Mission Spacecraft (MMS) and the Space Shuttle, modeled as spherical shells. The proton environment is that of the South Atlantic Anomaly, as well as cosmic ray protons. The induced radioactivity is analyzed in terms of its interference with various gamma-ray lines of astrophysical interest, as well as its contribution to several spectral regions of the gamma-ray continuum. The buildup of the line and continuum radioactivity background is predicted for a period of nearly 9 months in orbit (approximately 4100 orbits). In addition, background contributions from cosmic ray electron bremsstrahlung and earth gamma-ray albedo are estimated.

Fischbein, W. L.↗