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At least 217 records · Page 12

NACS 2022 FRIB Investment Strategy

The Facility for Rare Isotope Beams (FRIB) that will begin operations later this year will vastly increase the number of unstable isotopes available for experiments that, together with new theoretical developments will expand our understanding of nuclear structure and nuclear reactions that produce the elements of the periodic table and power the cosmos. The knowledge and understanding gained from FRIB will benefit a variety of applications including stockpile science, nuclear forensics, nonproliferation, nuclear energy, and nuclear medicine. LLNL is actively involved in a variety of basic and applied science activities related to FRIB. These activities are listed below and documented in the following sections: 1. FRIB Decay Station, 2. Isotope Harvesting, 3. Direct Reactions, 4. Surrogate Reactions, 5. Nuclear Structure and Collectivity, 6. Nuclear Fission, and 7. Nuclear Theory.

07 ISOTOPE AND RADIATION SOURCES↗

Modeling Astrophysical Explosions and Nucleosynthesis (Final Technical Report)

The goal of this project was to further our theoretical understanding of the extreme physics and heavy element nucleosynthesis occurring in stellar explosions, in particular supernovae and neutron star mergers. To study these systems, we further developed and applied numerical simulations (radiation hydrodynamical models and nuclear reaction networks) run on high performance computers. The numerical calculations and companion theoretical analysis helped to better define the sites of astrophysical nucleosynthesis, and make predictions of the associated observables (nucleosynthetic yields and electromagnetic signals) that can be used to anticipate and interpret experimental data. This project enhances the scientific value of the nuclear data obtained from current and future experimental facilities (e.g., rare isotope beams) by improving our understanding of the astrophysical context and specific physical conditions under which we expect such reactions to take place in Nature.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Investigation of the Role of the Role of Nuclear Physics in Heavy Element Nucleosynthesis, through the Study of Key Reactions, and the Improvement of Theoretical Reaction Rates (Final Report)

Neutrino-driven winds in core-collapse supernovae have been identified as a possible site for the production of elements heavier than iron. Traditionally, these neutrino-driven winds have been proposed as the site of the main r-process. Recent simulations fail to reproduce the conditions required for the main r-process. while they remain a promising site for producing the lightest elements beyond iron, e.g., Sr, Y, and Zr through the νp process. The efficiency of the νp process depends on the hydrodynamical conditions, the electron fraction (which is related to the neutrino properties), and the nuclear reactions on many short-lived nuclei with limited (if at all) experimental information. The reaction rates on these nuclei are based on theoretical predictions using the Hauser-Feshbach model. Recent sensitivity studies have highlighted the importance of neutron-induced reactions on these nuclei along the νp process path. This work aimed to experimentally constrain reaction rates that are known to play a key role in the neutrino-p process nucleosynthesis. A secondary subsequently-added objective was to start the implementation of techniques that improve the description of nuclear properties in the Hauser-Feshbach model by extending the microscopic nuclear level density description offered via the shell model to high excitation energies without using experiment-based renormalizations. The main objective of this work was the experimental constraint of the 56 Ni(n,p) 56 Co reaction rate via a measurement of the inverse reaction 56 Co(p,n) 56 Ni at the National Superconducting Cyclotron Laboratory (NSCL) and later the Facility for Rare Isotope Beams (FRIB). This reaction is considered the key one for determining the yields possible by the neutrino-p process. A technique for this type of measurement in inverse kinematics at low energies did not exist before this work. The work also had two secondary objectives. First, to contribute to efforts to measure the same reaction in direct kinematics using a radioactive target at Los Alamos National Laboratory (LANL), and second, to advance work to implement shell-model-deduced microscopic level densities in Hauser-Feshbach calculations. The project has resulted in the development of the first technique to perform (p,n) cross-section measurements in relevant-for-astrophysics low energies in inverse kinematics using a magnetic spectrometer or separator, and neutron detectors for neutron tagging. It has also resulted in the precise measurement of the cross-section of the 40 Ar(p,n) 40 K reaction in a proof-of-principle experiment realized by using a beam-line quadrupole of the ReA3 accelerator of NSCL/FRIB. As part of this project the technique was successfully adapted to make use of the superior acceptance of the Separator for Capture Reactions (SECAR) at FRIB. In this project, the required experimental setup simulations and beam optics were developed and tested with the measurement of the 58 Fe(p,n) 58 Cu reaction cross-section. Additionally, this project contributed with simulation work to the development of a technique to measure (n,p) reactions with radioactive targets at LANL, and which resulted in the measurement of the key 56 Ni(n,p) 56 Co reaction cross-section at neutron energies above ≈1 MeV. Last, the project initiated work in the development of shell model based level densities using the moments method.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Fundamental R&D for high-Q0 650 MHz SRF cavities for hadron linacs

Upcoming projects requiring high-Q0 ~650 MHz elliptical cavities, such as MSU’s Facility for Rare Isotope Beams’ energy upgrade and Fermilab’s PIP-II, drive a need to better understand RF losses due to magnetic flux. With sample sets from two different Niobium vendors, we explore the efficacy of the fast-cooldown method, and high- temperature annealing in promoting flux expulsion. Additionally, we report the results of vertical tests comparing the effect of electropolishing and furnace baking treatments on the cavity flux sensitivity. We also directly measure the flux pinning force in niobium samples, and correlate it with different heat treatments, and flux expulsion performance.

K.McGee, K.McGee↗

White Paper On Nuclear Structure Reactions and Astrophysics

In preparation for the 2023 NSAC Long Range Plan (LRP), the DNP Town Meeting on Nuclear Structure, Reactions, and Astrophysics was held at Argonne National Laboratory (ANL) on Nov 14-16, 2022. The town meeting brought together 578 members of the low-energy nuclear science community, including 216 in-person attendees and 362 remote participants coming from US national laboratories, a wide range of US universities and other research institutions and universities abroad. Participants met in five topic-oriented and seven cross-cutting and intersecting working groups to discuss progress since the 2015 LRP and identify compelling science opportunities and the resources needed to realize them. These considerations were used during the Town Meeting to determine a set of resolutions outlining the highest priorities for our subfield. The full text of the resolutions endorsed by unanimous consent by the low-energy nuclear science community at the Town Meeting is presented at the end of this executive summary. The reports from all working groups that met during the Town Meeting are included as Secs. 1 to 11 of this Whitepaper. The intellectual challenges for nuclear structure, reactions and astrophysics can be captured in the following questions: What is the nature of the nuclear force that binds protons and neutrons into stable nuclei and rare isotopes, and how do the rich phenomena of nuclear structure and reactions emerge? How do single-nucleon, cluster, and collective degrees of freedom coexist and evolve with increasing proton-neutron imbalance and excitation energies? What are the limits of nuclear existence, and what features arise near and beyond these limits? What are the astrophysical origins of the elements and how did the associated chemical evolution proceed? How do stars evolve, and what nuclear signatures do they leave behind? What is the nature of neutron stars and dense matter? How can the knowledge and technological progress provided by nuclear science best be used to benefit society?

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

A New Era of Discovery: The 2023 Long-Range Plan for Nuclear Science (V.1.2)

Nuclear science is the investigation of how protons and neutrons are formed from elementary particles and how the forces between those particles produce both nuclei and the vast variety of nuclear phenomena that occur in the universe. It has evolved into a broad field that addresses profound scientific questions: Where does the mass of visible matter come from? How do stars ignite, live, and die? How do nuclei illuminate the search for new laws of nature? This science points the way to using nuclei to build new technologies that benefit society. The 2015 Nobel Prize in physics was shared by nuclear physicists Art McDonald and Takaaki Kajita for the discovery of neutrino oscillations, which confirmed that neutrinos have mass. Our progress on big questions like this one since 2015 has been remarkable owing to new experimental tools, theoretical breakthroughs, powerful computational techniques, and the talented people who make these innovations possible. Focusing on these new tools, the Facility for Rare Isotope Beams (FRIB) at Michigan State University is already producing exciting results on decays of never-before-produced isotopes a year after it was completed on time and on budget. The energy upgrade of the Continuous Electron Beam Accelerator Facility (CEBAF) at the Thomas Jefferson National Accelerator Facility (Jefferson Lab) was also completed on schedule and on budget—new data from this facility are revealing the spectrum, structure, and dynamics of protons, neutrons, nuclei, and mesons. On the theory front, we can now calculate the distribution of quarks inside the proton from first principles. The implementation of artificial intelligence (AI) and machine learning (ML) techniques has led to improved data analysis and increased efficiency in running experiments and theoretical calculations. The impact of nuclear science goes beyond expanding the frontiers of knowledge about matter in the universe. We simultaneously develop a STEM work force that advances the security, technology, health, and wealth of our nation. Some connections are obvious. Expert scientists trained to work with radioactive nuclei are in demand in nuclear security arenas and are highly sought after by various government agencies and private industries. Graduate students and postdoctoral fellows (postdocs) obtain extensive computational, modeling, and data science skills that are similarly in high demand. Less obvious but equally important is the connection between these trained scientists and success in other professions, including medicine, energy, and entrepreneurial pursuits. The workforce that enables discovery in nuclear science also makes breakthroughs in technologies with tremendous impact on the nation’s economic advancement.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

China-US Theory Institute for Physics of Exotic Nuclei

The China-US Theory Institute for Physics of Exotic Nuclei (CUSTIPEN) was funded by DOE during May 1, 2013-April 30, 2023. The grant was managed by Texas A&M University-Commerce under the guidance of the CUSTIPEN Governing Board consists of physicists from Michigan State University, Florida State University, and Texas A&M University-Commerce. Its main goal was to support US-based physicists to visit their collaborators in China to work on projects supporting the science goals of DOE's national Facility for Rare Isotope Beams (FRIB) built on the campus of Michigan State University. The project has achieved successfully its scientific goals and mission.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

NUCLEI (SciDAC-4) effort at The University of Tennessee, Knoxville

This Report summarizes the accomplishments of NUCLEI researchers at The University of Tennessee, Knoxville (UTK) and those supported via subcontracts at the University of North Carolina at Chapel Hill (UNC) and Iowa State University (ISU). The SciDAC-4 NUCLEI collaboration had the goal to advance the computation of atomic nuclei and to make reliable predictions including uncertainty estimates for observables of interest. These goals were achieved by developing improved nuclear interactions and currents that are input to the computations, and by advancing the algorithms and techniques used for computing nuclear observables of interest. The computed results advanced our understanding of how nuclei work; they helped to guide and interpret experiments at existing low-energy nuclear physics facilities, the Facility for Rare Isotope Beams, Jefferson Laboratory, and neutrino experiments. In addition, predictions were made that await confrontation with experimental results.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Structure of the high-spin, β-decaying state in the neutron-rich nucleus 146 La

Excited structures in 146 Ce were populated in β decay of the high-spin state in the neutronrich nucleus 146 La. The beam was produced by the Californium Rare Isotope Breeder Upgrade (CARIBU) facility at Argonne National Laboratory, re-accelerated by the ATLAS accelerator and implanted on a moving-tape system in the middle of the GAMMASPHERE array. The decay scheme of the high-spin, β-decaying state in 146 La was revised with respect to previous studies and evaluated nuclear data. The structure of 146 La is discussed in the framework of the deformed Nilsson model and systematics of known quasiparticle structures in the region.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Nuclear Physics of Compact Binaries with GADGET

The research goal of this project was to experimentally constrain the thermonuclear rate of the 15 O(α, Υ) 19 Ne reaction, whose uncertainty has a strong influence on the modeling of astrophysical Type-I X-ray bursts on accreting neutron stars. To this end, Experiment 21072 was run in November 2022 at the Facility for Rare Isotope Beams using the GADGET II detection system. The limited scope and duration of this award included work in the year following the experiment: drafting a technical paper on the time projection chamber of the GADGET II detection system, and analysis of data from Experiment 21072. The award contributed to the education and development of the scientific and technical workforce by partially supporting one postdoctoral Research Associate who did this work.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Physics Design of Proton/Ion SRF Accelerators

Superconducting Radio Frequency (SRF) technology has become foundation of the modern high energy particle accelerators. The technology enables a higher accelerating field with minimal power dissipation and a stronger compact magnetic field. These advancements have broadened the operational horizon of the particle accelerators making a higher duty factor and Continuous Wave (CW) beam operations both feasible and economically viable. The intensity frontier research founded on generation of intense beam of exotic particles including but not limited to neutrinos, muons, kaons and neutrons as well as practical applications involving transmutation of nuclear reactor waste, rare isotopes generation, sub-critical nuclear power generation etc. could be accomplished efficiently only by using superconducting proton/ions particle accelerators. As a result, many newly constructed or under construction high energy accelerator facilities around the world such as Proton Improvement Plan-II (PIP-II) at Fermilab, FRIB at MSU, ESS at Sweden are utilizing SRF accelerators. This talk presents the design philosophy of SRF proton/ion particle accelerator, with a focus on optimizing its performance while addressing physics and operational challenges including the fault scenarios, machine availability and preservation of crucial beam parameters.

Saini, Arun↗

Development of the detector array for photons, protons, and exotic residues

Accurate neutron capture predictions are needed in fundamental and applied science. Empirical models are constrained largely for stable nuclei, but predictions far from stability are needed. Neutron transfer in (d,p) reactions in inverse kinematics with rare isotope beams offer a means to access key aspects of the capture process. To this end, the detector array for photons, protons, and exotic residues (DAPPER) has been designed, built, tested, and used for measurement at Texas A&M University.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Theoretical Nuclear Physics (Final Report)

This award from the Department of Energy supported the PI, Che-Ming Ko of Texas A&M University, for the period from April 1, 2022 to August 31, 2025 at an amount of $150,000 to carry out the project entitled “Theoretical nuclear physics”. The scientific goal of the project was to develop transport models for heavy ion collisions at various energies and with both stable and rare isotopes and to carry out systematic comparisons of theoretical predictions with experimental data. Results from this project has led to the publication of 14 papers in and the submission of 10 papers to peer-reviewed journals, the publication of 3 papers in and the submission of 1 paper to conference proceedings. Also, the PI has presented 12 invited talks at international conferences and workshops. In the following, a brief summary of these results is given.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Accelerator Science & Engineering (AS&E) Workforce Roundtable and AS&E Traineeship Principal Investigator Meeting

A one-and-half-day meeting on the Accelerator Science & Engineering (AS&E) Workforce Roundtable and a one-day meeting of Traineeship Principal Investigators took place at Facility for Rare Isotope Beams at Michigan State University on January 21-23, 2025. The meeting identified critical issues in the AS&E workforce and potential solutions, with a focus on DOE’s major accelerator facilities. The Traineeship PIs meeting focused on sharing experience, efficiency, and improvements of the Traineeship Programs conducted in six US universities. Several managers from the DOE High Energy Physics Office participated in the meetings. The discussions resulted in a decision to conduct similar meetings every year.

43 PARTICLE ACCELERATORS↗

Gas jet targets for direct reaction studies

The study of direct reactions is of broad interest in nuclear physics, providing constraint to models of nuclear structure evolution and data to better understand the creation of the elements. In many cases, however, the data of interest are hindered by backgrounds and poor resolution from contaminants in either the beam, the target, or both. The use of a gas jet can overcome some of these issues through clever engineering, providing a reaction target that is chemically pure and thin enough to significantly reduce the impact on experimental resolution. This Perspective will discuss the effort to design, construct, and operate gas jet targets for direct reaction studies in the rare isotope era.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Direct reactions for astrophysical p-capture rates with ORRUBA and GODDESS

Understanding the nucleosynthesis and energy generation in quiescent and explosive stellar burning requires a detailed understanding of reaction rates on many unstable nuclides. Such reaction rates are often governed by the properties of low-lying, isolated proton resonances. Though direct measurements of resonance strengths are ultimately desired, and are a focus of rare isotope beam facilities worldwide, such tour-de-force experiments must be guided by indirect techniques, in order to know resonance energies, J π assignments, and estimated widths, to inform targeted measurements. Furthermore, some important low-lying resonances may be too weak for direct measurements with radioactive beams, and indirect techniques provide the only practical constraints. Additionally, there has been growing interest in the astrophysical role of isomeric states, which can influence the reaction flow in nucleosynthetic reaction networks, and hence impact the quantitative interpretation of astronomical observables, such as γ-ray signatures, and elemental and isotopic ratios. Properties of single-proton resonances can be obtained by exploiting the selectivity of direct reactions, such as single-nucleon transfer and charge-exchange reactions. Constraining proton-capture rates via direct reactions has been a focus of the astrophysics program at ORNL for over two decades, spurring the development of the ORRUBA and GODDESS detector systems. Herein, a review of recent developments in instrumentation and radioactive beam delivery (including isomeric beam experiments) is presented, along with some specific examples of astrophysically interesting sd-shell nuclides, which have been a target of recent ORRUBA and GODDESS experiments.

79 ASTRONOMY AND ASTROPHYSICS↗

Direct reactions with the AT-TPC

Direct reactions are crucial tools for accessing properties of the atomic nucleus. Fundamental and exotic phenomena such as collective modes, pairing, weakbinding effects and evolution of single-particles energies can be investigated in peripheral collisions between a heavy nucleus and a light target. The necessity of using inverse kinematics to reveal how these structural properties change with isospin imbalance renders direct reactions a challenging technique when using the missing mass method. In this scenario, Active Target Time Projection Chambers (AT-TPC) have demonstrated an outstanding performance in enabling these types of reactions even under conditions of very low beam intensities. The AT-TPC of the Facility for Rare Isotope Beams (FRIB) is a next generation multipurpose Active Target. When operated inside a solenoidal magnet, direct reactions benefit from the measurement of the magnetic rigidity that enables particle identification and the determination of the excitation energy with high resolution without the need of auxiliary detectors. Additionally, the AT-TPC can be coupled to a magnetic spectrometer improving even further its spectroscopic investigation capability. In this contribution, we discuss inelastic scattering and transfer reaction data obtained via the AT-TPC and compare them to theory. In particular, we present the results for the 14 C(p,p′) and 12 Be (p,d) 11 Be reactions. For 14 C, we compare the experimental excitation energy of the first 1 – excited state with coupled-cluster calculationsbased on nuclear interactions from chiral effective field theory and with available shell-model predictions. For 12 Be, we determine the theoretical spectroscopic factors of the 12 Be (p,d) 11 Be transfer reaction in the shell modeland compare them to the experimental excitation spectrum from a qualitative standpoint.

active target↗

DIAL with heterodyne detection including speckle noise: Aircraft/shuttle measurements of O3, H2O, and NH3 with pulsed tunable CO2lasers

A parametric analysis of DIAL sensitivity with heterodyne detection is presented and comparisons with direct detection are discussed. Examples are given for monitoring vertical distributions of O3, H2O, and NH3 using a ground-, aircraft-, or shuttle-based pulsed tunable CO2 laser DIAL system. Results indicate that maximum sensitivity at minimum laser energy per measurement requires multiple pulse operation with the energy per pulse selected so that the measured photon rate is approximately equal to the detector IF bandwidth. Measurement sensitivities can be maximized and interference effects minimized by fine adjustment of measurement frequencies using the tunability of high pressure lasers. The use of rare isotope lasers minimizes loss due to CO2 atmospheric absorption.

Brockman, P.↗