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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 217 records · Page 12

Pathway complexity in fibre assembly: from liquid crystals to hyper-helical gelmorphs

Pathway complexity results in unique materials from the same components according to the assembly conditions. Here a chiral acyl-semicarbazide gelator forms three different gels of contrasting fibre morphology (termed ‘gelmorphs’) as well as lyotropic liquid crystalline droplets depending on the assembly pathway. The gels have morphologies that are either hyperhelical (HH-Gel), tape-fibre (TF-Gel) or thin fibril derived from the liquid crystalline phase (LC-Gels) and exhibit very different rheological properties. The gelator exists as three slowly interconverting conformers in solution. All three gels are comprised of an unsymmetrical, intramolecular hydrogen bonded conformer. The kinetics show that formation of the remarkable HH-Gel is cooperative and is postulated to involve association of the growing fibril with a non-gelling conformer. This single molecule dynamic conformational library shows how very different materials with different morphology and hence very contrasting materials properties can arise from pathway complexity as a result of emergent interactions during the assembly process.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Framework for custom event sample augmentations for ATLAS analysis data

For HEP event processing, data is typically stored in column-wise synchronized containers, such as most prominently ROOT’s TTree, which have been used for several decades to store by now over 1 exabyte. These containers can combine row-wise association capabilities needed by most HEP event processing frameworks (e.g. Athena for ATLAS) with column-wise storage, which typically results in better compression and more efficient support for many analysis use-cases. One disadvantage is that these containers, TTree in the HEP use-case, require to contain the same attributes for each entry/row (representing events), which can make extending the list of attributes very costly in storage, even if those are only required for a small subsample of events. Since the initial design, the ATLAS software framework features powerful navigational infrastructure to allow storing custom data extensions for subsamples of events in separate, but synchronized containers. This allows adding event augmentations to ATLAS standard data products (such as DAOD-PHYS or PHYSLITE) avoiding duplication of those core data products, while limiting their size increase. For this functionality, the framework does not rely on any associations made by the I/O technology (i.e. ROOT), however it supports TTree friends and builds the associated index to allow for analysis outside of the ATLAS framework. A prototype based on the Long-Lived Particle search is implemented and preliminary results with this prototype will be presented. At this point, augmented data are stored within the same file as the core data. Storing them in separate files will be investigated in future, as this could provide more flexibility, e.g. certain sites may only want a subset of several augmentations or augmentations can be archived to tape once their analysis is complete.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Data Placement Optimization for ATLAS in a Multi-Tiered Storage System within a Data Center

Scientific experiments and computations, especially in High Energy Physics, are generating and accumulating data at an unprecedented rate. Effectively managing this vast volume of data while ensuring efficient data analysis poses a significant challenge for data centers, which must integrate various storage technologies. This paper proposes addressing this challenge by designing and developing a precise data popularity prediction model utilizing state-of-theart AI/ML techniques. This model is crafted from the analysis of ATLAS data and access patterns. It enables us to migrate infrequently accessed data to more economical storage media, such as tape drives, while storing frequently accessed data on faster yet costlier storage media like HDD or SSD. This strategic approach ensures data is placed optimally into the appropriate storage classes, thereby maximizing storage capacity while minimizing data access latency for end-users. Furthermore, the paper includes a performance evaluation of the prediction model using various key metrics such as F1 score, accuracy, precision and recall. Finally, we present a prototype use case, leveraging real-world file access data to assess the model’s impact on performance.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Recent Experience with the CMS Data Management System

The CMS[1] experiment manages a large-scale data infrastructure, currently handling over 200 PB of disk and 500 PB of tape storage and transferring more than 1 PB of data per day on average between various WLCG[2] sites. Utilizing Rucio[3] for high-level data management, FTS[4] for data transfers, and a variety of storage and network technologies at the sites, CMS confronts inevitable challenges due to the system’s growing scale and evolving nature. Key challenges include managing transfer and storage failures, optimizing data distribution across different storages based on production and analysis needs, implementing necessary technology upgrades and migrations, and efficiently handling user requests. The data management team has established comprehensive monitoring to supervise this system and has successfully addressed many of these challenges. The team’s efforts aim to ensure data availability and protection, minimize failures and manual interventions, maximize transfer throughput and resource utilization, and provide reliable user support. This paper details the operational experience of CMS with its data management system in recent years, focusing on the encountered challenges, the effective strategies employed to overcome them and the ongoing challenges as we prepare for future demands.

Öztürk, Hasan [CERN]↗

Automated tabletop exfoliation and identification of monolayer graphene flakes

Over the past two decades, graphene has been intensively studied because of its remarkable mechanical, optical, and electronic properties. Initial studies were enabled by manual “Scotch Tape” exfoliation; nearly two decades later, this method is still widely used to obtain chemically pristine flakes of graphene and other 2D van der Waals materials. Unfortunately, the yield of large, pristine flakes with uniform thickness is inconsistent. Thus, significant time and effort are required to exfoliate and locate flakes suitable for fabricating multilayer van der Waals heterostructures. Here, we describe a relatively affordable tabletop device (the “eXfoliator”) that can reproducibly control key parameters and largely automate the exfoliation process. In a typical exfoliation run, the eXfoliator produces 3 or more large (≥ 400 μm 2 ) high-quality graphene monolayer flakes, allowing new users to produce such flakes at a rate comparable to manual exfoliation by an experienced user. Furthermore, we use an automated mapping system and a computer vision algorithm to locate candidate flakes. Our results provide a starting point for future research efforts to identify more precisely which parameters matter for the success of exfoliation and to optimize them.

47 OTHER INSTRUMENTATION↗

Determining the complex second-order optical susceptibility in macroscale van der Waals heterobilayers

In this work, we report on the experimental characterization of the second-order susceptibility in MoSe 2 /WS 2 heterobilayers, including their hidden complex phases. To this end, we developed a heterodyne-detection scheme for second-harmonic generation and applied it to macroscale heterobilayer samples prepared using the gold-tape exfoliation method. The heterodyne scheme enabled us to distinguish the relative orientation of the crystal domains, and furthermore, it allowed us to characterize the complex phases of the susceptibility relative to a reference quartz sample. By comparing the results from the monolayer regions and the heterobilayer region over several hundred microns of the sample area, we determined that the contribution of interlayer effects to second-harmonic generation is within the experimental uncertainty arising from the sample inhomogeneity. The results here provide fundamental quantitative information necessary for the precise design of nanophotonic systems based on stacking engineering.

2D materials↗

Transmission of Images on High-Temperature Nuclear-Grade Metallic Pipe with Ultrasonic Elastic Waves

Transmission of information using elastic ultrasonic waves on existing metallic pipes provides an alternative communication option for a nuclear facility. The advantages of this approach consist of transmitting information through barriers, such as the containment building wall, with minimal modification of the existing hardware. Because bit rates on the order of kilobits per second are achievable, relatively large volumes of data, such as images, can be transmitted. A viable candidate for an ultrasonic communication channel is a stainless steel pipe of the chemical volume control system (CVCS) that penetrates through the reactor containment building wall through a sealed tunnel. To study ultrasonic communication under simulated nuclear facility conditions of high temperature, a test article was developed by installing heating tapes, temperature controllers, and thermal insulation on a laboratory CVCS-like stainless steel pipe. High temperature and radiation-resilient lithium niobate ultrasonic transducers were utilized for information transmission on the heated pipe. The amplitude shift keying (ASK) digital communication protocol was developed and implemented in a GNU Radio software-defined radio environment. A root-raised-cosine filter was introduced to suppress ultrasonic transducer ringing and thus reduce inter-symbol interference. This resulted in the enhancement of the data transmission bit rate compared to information encoding with square pulses. Demonstrations of communication at high temperature included transmission of a 90-KB image at the bit rate of 10 Kbps with a bit error rate of 10 -3 across a 6-ft-long straight pipe heated up to 230 degrees C. Additional preliminary studies were conducted to evaluate ultrasonic communication system resilience to environmental degradation and damage.

42 ENGINEERING↗

Droplet and Particle Methods to Investigate Turbulent Particle Laden Jets

The SARS-CoV-2 pandemic has heightened the interest in particle-laden turbulent jets generated by breathing, talking, coughing and sneezing, and how these can contribute to disease transmission. We present quantitative measurement methods for such flows, while exploring and offering improvements for common shortcomings. We generate jets consisting of either liquid droplets or solid particles in an isothermal, quiescent and electrically isopotential experimental chamber that was constructed to control the effects of ambient forcing on jet behavior. For liquid droplets, we find promise in surface deposition analysis based on fluorescent tracer use. For particles, we explore the performance of commercially available adhesive sampling strips and develop conductive grounded carbon tape based sampling strips. We explore ways in which the smallest of thermal gradients or electrostatic charge issues can affect particle dispersion, and suggest practical methods to address these issues. The developed methods are applied to study the simultaneous deposition of (Formula presented.) 25, 50 and 200 μm solid particles from a particle laden turbulent jet with a mean velocity of 33.2 m/s. The deposition location as a function of particle size was compared to results from a simple numerical RANS model, and illustrates ways in which imprecise initial or boundary conditions can lead to a notable deviation from experimental results. The differences in deposition pattern seen in experimental and numerical results despite a carefully controlled environment and characterized particle ejection indicate the need for a more stringent numerical model validation, especially when studying fate and transport of mid-range (neither purely aerosol or ballistic) sized particles.

42 ENGINEERING↗

Quench detection using Hall sensors in high-temperature superconducting CORC ® -based cable-in-conduit-conductors for fusion applications

Advanced magnet systems for fusion applications would greatly benefit from the use of high-temperature superconductors (HTS). These materials allow fusion magnets to operate at higher magnetic fields, allowing for more compact fusion machines, and allow for operation at elevated temperatures, enabling demountable coils that provide access for maintenance of the fusion reactor. Quench detection remains a major challenge in the protection of HTS magnets that are vulnerable to localized conductor burnout due to their low quench propagation velocities. One of the methods explored is the use of Hall sensors that are incorporated in or near the magnet terminations that can detect local field variations that occur as a result of current redistribution within the conductor to bypass a hotspot within the magnet winding. This method is potentially well suited for Cable in Conduit Conductors, such as those made from Conductor on Round Core (CORC) cables, in which sub-cables containing HTS tapes are connected to the terminations at a low resistance. Here, to demonstrate the technique, a CORC ® triplet consisting of three sub-cables, rated for 4 kA operation at 77 K, was manufactured and Hall sensors were used to measure local field variations next to the terminations due to current redistribution between the cables. The Hall response was compared to voltages that developed over the cables and terminations as a local hotspot was applied to different cables in the triplet. It was found that the Hall sensors were faster and more sensitive than voltage contact measurements and were able to reliably detect current redistribution of only a few amperes caused by a hotspot, well before the triplet exceeded its critical current. The method also allowed the detection of heater-induced hotspots during high ramp rates of 2 kA s<:sup>–1 relevant for fusion applications. Hall sensors have a distinct benefit of being less sensitive to inductive pickup of AC interference compared to voltage contact measurements that make quench detection through voltage measurements in magnets especially challenging. The method can also be used for diagnostic measurements of current redistribution caused by other sources such as inhomogeneous current injection from faulty joints, or localized conductor damage. The Hall sensors are likely capable of detecting the onset of a quench that may occur a far distance away from the sensor location, presenting a breakthrough in HTS quench detection that potentially removes one of the remaining barriers to reliable operation of large HTS magnet systems.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Development and performance of a 2.9 Tesla dipole magnet using high-temperature superconducting CORC® wires

Although the high-temperature superconducting (HTS) REBa 2 Cu 3 O x (REBCO, RE-rare earth elements) material has a strong potential to enable dipole magnetic fields above 20 T in future circular particle colliders, the magnet and conductor technology needs to be developed. As part of an ongoing development to address this need, here we report on our CORC® canted cosθ magnet called C2 with a target dipole field of 3 T in a 65 mm aperture. The magnet was wound with 70 m of 3.8 mm diameter CORC® wire on machined metal mandrels. The wire had 30 commercial REBCO tapes from SuperPower Inc. each 2 mm wide with a 30 µm thick substrate. The magnet generated a peak dipole field of 2.91 T at 6.290 kA, 4.2 K. The magnet could be consistently driven into the flux-flow regime with reproducible voltage rise at an engineering current density between 400-550 A mm -2 , allowing reliable quench detection and magnet protection. The C2 magnet represents another successful step towards the development of high-field accelerator magnet and CORC® conductor technologies. The test results highlighted two development needs: continue improving the performance and flexibility of CORC® wires and develop the capability to identify locations of first onset of flux-flow voltage.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

SMART conductor on round core (CORC ® ) wire via integrated optical fibers

Superconducting cables based on high temperature superconductors (HTS) are necessary for applications requiring large currents and low inductance, such as compact fusion reactors. In this paper, we report the proof-of-concept of a SMART Conductor on Round Core (CORC ® ) wire realized via integration of optical fibers into the copper core. A SMART CORC ® wire with integrated optical fibers was manufactured and its capabilities have been experimentally demonstrated. Results show that by interrogating the optical fibers via Rayleigh backscattering, a Spectral Shift signal as a function of time and position along the cable can be used to detect and locate hot-spots that are developed within the wire or its terminations. It has been found that highly localized current injection into the terminations could initiate hot-spots within the cable at locations where current redistribution between tapes occur. This effect is virtually eliminated when adequate current connections are used that inject current evenly along the cable terminations. Normal zone propagation velocities have been calculated as a function of time using Spectral Shift data for a heater-induced quench as well as a quench induced by overcurrent. In both cases the normal zone propagation velocity was about 6 cm s -1 , but in the heater-induced experiment it was preceded by 500 ms of slower propagation at 2.5 cm s -1 .

Physics↗

Rapid assessment of REBCO CC angular critical current density J c (B, T = 4.2 K, θ) using torque magnetometry up to at least 30 tesla

Abstract Detailed design of REBa 2 Cu 3 O 7 − x (REBCO)-based magnets ideally relies on knowledge of the full angular and wide temperature range characterization of the critical current I c of the REBCO coated conductors (CC) at high magnetic fields. In practice, however, obtaining I c ( B , T , θ ) data by the commonly used electrical transport technique is expensive, tedious, and difficult, due to high critical current values that exceed 2000 A for B | | a b -plane ( θ = 90 deg). The conductors are often damaged during angular transport measurements at angles approaching the ab -plane. Therefore, so far, REBCO magnets have been designed without full I c ( B , T , θ ) data sets. Here, we present J c ( B , T , θ ) results for more than twenty samples of CC all made to the same advanced pinning specification produced by SuperPower Inc. For this, we employed torque magnetometry, benchmarking the results to transport I c measurements mostly made away from ab -plane, finding good agreement with scaling factors ≈1–1.3. What is striking is the huge variety of properties exhibited by the samples, even for CC made recently. Given the huge attention now being paid to the effects of screening currents and to the torques generated by offsets between the tape plane and the local magnetic field vector, our data set suggests some caution in detailed design of such magnets without having data of the type presented here.

Physics↗

Quench protection for high-temperature superconductor cables using active control of current distribution

Superconducting magnets of future fusion reactors are expected to rely on composite high-temperature superconductor (HTS) cable conductors. In presently used HTS cables, current sharing between components is limited due to poorly defined contact resistances between superconducting tapes or by design. The interplay between contact and termination resistances is the defining factor for power dissipation in these cables and ultimately defines their safe operational margins. However, the current distribution between components along the composite conductor and inside its terminations is a priori unknown, and presently, no means are available to actively tune current flow distribution in real-time to improve margins of quench protection. Also, the lack of ability to electrically probe individual components makes it impossible to identify conductor damage locations within the cable. In this work, we address both problems by introducing active current control of current distribution between components using cryogenically operated metal-oxide-semiconductor-field-effect transistors (MOSFETs). We demonstrate through simulation and experiments how real-time current controls can help to drastically reduce heat dissipation in a developing hot spot in a two-conductor model system and help identify critical current degradation of individual cable components. Finally, prospects of other potential uses of MOSFET devices for improved voltage detection, AC loss-driven active quench protection, and remnant magnetization reduction in HTS magnets are also discussed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Simulations of the fault current limiting operation of a long-length REBCO CORC ® superconducting cable cooled by helium gas

Conductor-on-round-core (CORC®) cables composed of rare-earth-barium-copper-oxide high-temperature superconducting (HTS) tapes are of great interest for power transmission applications due to their many advantages such as high power density, light weight, and low loss. Closed circulation loops of cryogenic helium gas can be used to cool HTS cables down to low temperatures to significantly improve their current-carrying capacity. Coupled circuit-electromagnetic-thermal finite element simulations implemented in the COMSOL Multiphysics package were developed, validated, and then used for simulating the fault current limiting (FCL) performance and the cooling processes of an 8-layer CORC® cable cooled with a flow of cryogenic helium gas. In the simulations, the temperature dependence of the electrical and thermal properties of all component materials is implemented for improved accuracy. To overcome computational challenges caused by the considerable difference in geometrical scales (i.e. few-µm-thick HTS layers versus 10 m-long HTS cable), the model is divided into two separate simulations. The first simulation is performed on the transverse cross-section of the cable to calculate the electric field, heating power and temperature rise in each component of a CORC® cable during FCL operation. The heating power calculated in the first simulation is transferred to the second model to simulate the cooling of a 10 m-long cable after the fault is cleared. The effect of the helium gas flow rate on the cooling process is also investigated to develop strategic approaches for optimizing cooling systems for HTS cables with FCL capability. The simulations indicated that a 40 ms fault with a voltage drop of 20 V m −1 along the cable can result in a temperature increase from 60 K to about 165 K inside the cable, and it takes about 500 s to cool the cable back to nearly 60 K with a flow of cold helium gas at a rate of 5 g s −1 .

24 POWER TRANSMISSION AND DISTRIBUTION↗

Structure of beta-decaying states in the deformed, neutron-rich nucleus 104 Nb

Excited structures in 104 Mo were populated by β decays of the ground and isomeric states in the neutron-rich nucleus 104 Nb. The beams were produced by the CARIBU facility at Argonne National Laboratory, re-accelerated by the ATLAS accelerator and implanted on a moving-tape system in the middle of the GAMMASPHERE array. Separate decay schemes for the two β-decaying states in 104 Nb were constructed for the first time. The structure of the isomers are discussed in the framework of the deformed Nilsson model and systematics of known quasiparticle structures in neighboring nuclei.

Nilsson model↗

Design and calibration of an optically segmented single volume scatter camera for neutron imaging

The Optically Segmented Single Volume Scatter Camera (OS-SVSC) aims to image neutron sources for non-proliferation applications using the kinematic reconstruction of elastic double-scatter events. Our prototype system consists of 64 EJ-204 organic plastic scintillator bars, each measuring 5mm &#x00d7; 5mm &#x00d7; 200mm and individually wrapped in Teflon tape. The scintillator array is optically coupled to two silicon photomultiplier ArrayJ-60035 64P-PCB arrays, each comprised of 64 individual 6x6mm J-Series sensors arranged in an 8 &#x00d7; 8 array. We report on the design details, including component selections, mechanical design and assembly, and the electronics system. The described design leveraged existing off-the-shelf solutions to support the rapid development of a phase 1 prototype. Several valuable lessons were learned from component and system testing, including those related to the detector's mechanical structure and electrical crosstalk that we conclude originates in the commercial photodetector arrays and the associated custom breakout cards. We detail our calibration efforts, beginning with calibrations for the electronics, based on the IRS3D application-specific integrated circuits, and their associated timing resolutions, ranging from 3090ps. With electronics calibrations applied, energy and position calibrations were performed for a set of edge bars using 22 Na and 90 Sr, respectively, reporting an average resolution of 12.07±0.03mm for energy depositions between 900keVee and 1000keVee. We further demonstrate a position calibration method for the internal bars of the matrix using cosmic-ray muons as an alternative to emission sources that cannot easily access these bars, with an average measured resolution of 14.86+-0.29mm for depositions between 900keVee and 1000keVee. The coincident time resolution reported between pairs of bars measured up to 400ps from muon acquisitions. Energy and position calibration values measured with muons are consistent with those obtained using particle emission sources.

47 OTHER INSTRUMENTATION↗

New precise half-life measurement for the superallowed β+ emitter Ar34

We have measured the half-life of 34 Ar, the parent of a superallowed 0 + → 0 + β transition, to be 0.84646(35) s. With a precision of 0.04%, this result is an essential ingredient needed to complete a third pair of mirror superallowed transitions, 34 Ar → 34 Cl and 34 Cl → 34 S, the ratio of whose ft values would provide the most sensitive test yet of the isospin-symmetry-breaking corrections used to obtain V ud . In a sequence repeated thousands of times, we implanted a very pure 34 Ar beam into tape for 0.7 s, and then rapidly transported the collected source to a shielded 4π proportional gas counter, which detected the decay positrons from the combined decays of 34 Ar and its daughter 34 Cl. The data were analyzed as a linked parent-daughter pair. Our new result replaces one we published 13 years ago.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Levels in 125 Cd populated by the β decay of 125 m Ag and 125 Ag

Here, the β decay of 125 m, 125 Ag into levels in 125 Cd was investigated at the Holifield Radioactive Ion Beam Facility (HRIBF). Uranium-238 targets were bombarded with 50-MeV protons with an intensity of 15 μ A, and the induced fission products were mass separated and deposited on a moving tape in the center of the VANDLE array consisting of γ detectors and plastic scintillators. A partial decay scheme has been assigned for both β decay of the (9/2 + ) ground state of 125 Ag and its low-lying (1/2 - ) isomer, with the energy of the low-lying (11/2 - ) isomeric state in 125 Cd assigned as 188.5 keV. In addition, β -delayed neutron emission probabilities were also determined to be 1.2(2)% for the (9/2 + ) 125 Ag ground state and 4.6(10)% for the (1/2 - ) isomer, which are substantially lower than the previously reported value.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗