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At least 217 records · Page 12

Advanced Manufactured Strain Sensors for Extreme Environments

Experimentation at irradiation test facilities are essential for reducing the innovation time of developmental fuels, fuel cladding, and structural materials employed in next-generation nuclear reactors. However, due to the harsh conditions generated in such reactors and limited instrumentation space, the evaluation of a material’s mechanical properties is often limited to characterization after the materials have been removed from reactor conditions, or post-irradiation examination. These experiments are costly, time-consuming, and fail to capture the critical time-evolving phenomena that occur during the irradiation experiments. Advanced manufactured digital image correlation patterns and strain sensor devices serve as two promising technologies that can be deployed in the confined and challenging orientations of these irradiation experiments while also providing key insight on salient materials phenomena (i.e., mechanical properties).To guide the development of the printed strain sensors prior to their deployment in critical experiments, the adhesion strength between the substrate and printed film interface is measured via tensile testing and a non-contact laser-induced spallation technique. The establishment of these process control steps helped guide the successful fabrication and testing of direct-write strain sensing devices discussed in this work. The fabrication process controls are necessary for enabling the sustained operation of these strain sensing device through experimentation and minimize the potential for premature failure.

36 - MATERIALS SCIENCE↗

Benchmarking FFTF LOFWOS Test# 13 using SAM code: Baseline model development and uncertainty quantification

The development and deployment of advanced reactors, such as the sodium-cooled fast reactor (SFR), relies on sophisticated modeling tools to ensure the safety of the design under various transients. The predictive capability of these advanced modeling tools requires validation to garner trust in supporting the licensing of the advanced reactors. For this reason, the International Atomic Energy Agency (IAEA) initiated a coordinated research project (CRP) in 2018 for the analysis of the Fast Flux Test Facility (FFTF) Loss of Flow Without Scram (LOFWOS) Test #13.In this study, we present and discuss the benchmarking efforts of the modern system code SAM on the FFTF LOFWOS Test #13. Further, the SAM baseline model was developed according to the benchmark specification, which included a detailed core model with reactivity feedback. Generally, good agreement was observed between the baseline results and benchmark measurements; however, discrepancies persisted, particularly in predicted fuel assembly coolant outlet temperatures. Utilizing the baseline model, uncertainty quantification (UQ) and sensitivity analysis (SA) were conducted with the assistance of various statistical learning and machine learning methods, including kernel density estimation, Gaussian processes, and Sobol indices. Following the baseline model prediction and UQ and SA results, we discuss the reasons for the simulation discrepancies and propose further improvements to the model. This benchmarking effort adheres to the best-estimate plus uncertainty approach and can serve as a valuable example for supporting risk-informed licensing of advanced reactors.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Windowless Optical Cell Flow System

One of the goals for advanced integrated nuclear safeguards is on-line optical analysis of molten salt in molten salt reactors and electrochemical fuel reprocessing facilities. While progress has been made in the development of optical techniques that may be suitable for on-line analysis of molten salts, significant technology gaps exist with regard to integrating these analytical techniques into industrial-scale processes. One key technological hurdle is the short service life of optical window materials, which are subject to clouding and scaling during extended exposure to molten salts. To address this issue, Argonne is developing a gravity flow cell with open-apertures to support on-line optical analysis without the need for salt-wetted windows. The flow cell uses gravity flow and fluid dynamics principles to enable molten salt flow through a pipe that has holes in its wall through which salt does not flow. In FY21, an open-aperture gravity flow cell with windowless optical access to flowing salt was successfully demonstrated. Future work should include the integration of the flow cell into a sampling loop, stakeholder outreach and collaboration, integration of multiple optical analysis techniques, evaluation of the integrated methods, and analyses to determine how the various tools might fit into an integrated safeguards monitoring system of unattended near real time monitoring tools.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

RELAP5-3D Modeling in the OECD-NEA HTTF Benchmark

Prismatic gas-cooled reactors are a technologically mature reactor concept of interest for near- to mid-term deployment. To accelerate the deployment of these reactors, the DOE's Advanced Reactor Technologies Gas-Cooled Reactor campaign is spearheading a thermal hydraulics code validation benchmark based on the High Temperature Test Facility at Oregon State University. This presentation provides an introduction to that benchmark and an overview of some of the RELAP5-3D validation activities stemming from that benchmark.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Analysis of Deformation Mechanisms, Strain Localization, and Fracture in Highly Irradiated Austenitic Steels – Light-Water Reactor Core Materials – via Advanced inSEM Techniques

The present report describes the establishing of an advanced experimental approach – high-resolution digital image correlation or µDIC – for testing miniature irradiated specimens in the ORNL’s Low Activation Materials Development and Analysis (LAMDA) facility. As expected, the µDIC approach will allow for studying strain localization inside grains, for instance, during dislocation channel-grain boundary interaction processes. This information is of high importance for understanding degradation processes in irradiated austenitic steels – in-core materials of Light Water Reactors. The Level 4 report provides a brief introduction, lists materials designated for µDIC testing and delivered in LAMDA this FY, discusses methodical concerns and preliminary observations.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Design Readiness And Maturity Assessment (DRAMA) Tool for Advanced Reactors

Abstract – This research is developing a formal, repeatable method to assess the readiness and maturity of an advanced nuclear reactor design for licensing and deployment. This design readiness and maturity assessment (DRAMA) tool will be capable of determining the readiness of the design and of all parties needed to bring a particular advanced reactor design to fruition. Beneficiaries and stakeholders include the design team, research organizations (required to collect needed data and develop design tools), standards organizations, research facilities to support gathering of needed data, supply chain and construction organizations, and everyone responsible for legal and regulatory infrastructure (including defining import-export requirements). Recent experience has shown that even the most experienced engineering and construction organizations, with decades of experience in the nuclear power business, have had significant challenges in bringing designs to completion, licensing the designs, and constructing new plants. For new entries into the field, simply understanding the unique environmental and regulatory requirements have been daunting. A significant part of the challenge is that new entries into the market do not know what they don't know. This tool will provide design teams a better understanding of their readiness to proceed to licensing (and other steps in the process), while at the same time providing a valuable metric for other interested organizations, such as funding agencies, national regulators, and international markets. The DRAMA tool will provide an assessment of the likelihood of successfully completing licensing and deployment and will also create the capability to assess the ability of regulatory infrastructure and the supply chain to support the deployment of any design or class of designs. It will also help prioritize research and policy efforts to improve the likelihood of deployment of the next generation of advanced reactors.

Arndt, Steven↗

Advancement of LANSCE accelerator facility as a 1-MW Fusion Prototypic Neutron Source

The Fusion Prototypic Neutron Source (FPNS) is considered to be a testbed for scientific understanding of material degradation in future nuclear fusion reactors (Zinkle and Moeslang, 2013; Summary Report on the FPNS Workshop, 2018; Pitcher et al., 2019). The primary mission of FPNS is to provide a damage rate in iron samples of 8-11 dpa/calendar year with He/dpa ratio of 10 appm in irradiation volume of 50 cm 3 or larger with irradiation temperature 300–1000 °C and flux gradient less than 20%/cm in the plane of the sample. The Los Alamos Neutron Science Center (LANSCE) is an attractive candidate for the FPNS project. The Accelerator Facility was designed and operated for an extended period as a 0.8-MW Meson Factory. The existing setup of the LANSCE accelerator complex can nearly fulfill requirements of the fusion neutron source station. The primary function of the upgraded accelerator systems is the safe and reliable delivery of a 1.25-mA continuous proton beam current at 800-MeV beam energy from the switchyard to the target assembly to create 1 MW power of proton beam interacting with a solid tungsten target. The present study describes existing accelerator setup and further development required to meet the needs of FPNS project.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

ACCELERATING MICROREACTOR DEVELOPMENT AND DEPLOYMENT THROUGH JOINT PUBLIC TEST BEDS AND PRIVATE ADVANCED REACTOR DEVELOPMENT

The United States Department of Energy (DOE) has funded the National Reactor Innovation Center (NRIC) to accelerate the development and commercialization of small modular reactors and other advanced reactor technologies. As part of this effort NIRC is building two strategic assets at the Idaho National Laboratory (INL) to facilitate public-private partnerships for the development and testing of advanced nuclear microreactors and Small Modular Reactors (SMR). One will provide a safe, secure, and affordable location for High-Assay Low Enriched Uranium (HALEU) fueled reactors and a second for Highly Enriched Uranium (HEU) fueled reactors. Together these testbeds fill a nuclear testing infrastructure gap. The availability of such comprehensive testing facilities at the national labs eliminates the significant financial and operational burdens associated with each developer building and licensing their own test facilities. Consequently, this approach will not only accelerate technological innovation and reduce time-to-market for advanced nuclear solutions but it also underscores the DOE's commitment to fostering an ecosystem where nuclear energy will thrive as a clean, reliable, and efficient source of power. The Demonstration of Microreactor Experiments (DOME) and Laboratory for Operations and Testing in the United States (LOTUS) have planned availability in 2026, and 2027 respectively.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Droplet Entrainment in Steam Supply System of Water-Cooled Small Modular Reactors: Experiment and Modeling Approaches

Droplet entrainment in steam-flow is a prominent phenomenon that needs adequate safety and risk analysis of postulated transient and accident scenarios—including experimental investigation and representative modeling and simulation (M&S)—for small modular reactor (SMR) system design and demonstration. This study identifies knowledge gaps by evaluating experimental and computational fluid dynamics modeling approaches to support early-stage reactor system design, testing, and model evaluation. Previous studies reported in the literature for steam-flow entrainment primarily focused on gigawatt capacity pressurized water reactor (PWR) systems. However, entrainment phenomena are even more prominent for PWR-type SMRs due to their more compact integrated designs, which need further research and development. To fill the research gaps, this study provides insight by specifying the phenomena of interest by leveraging the lessons learned from past research, adopting advanced M&S techniques and advanced instrumentation and control. The findings and recommendations are applicable for evaluating steam-flow entrainment models and for designing integral effect test and separate effect test facilities for gaining reactor design approvals.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Perspective on “code qualifying” new graphite grades for use in advanced nuclear reactors*

The American Society of Mechanical Engineers (ASME) publishes the Boiler and Pressure Vessel (BPV) Code, which include guidance for the safe development, construction, and operation of boilers and pressure vessels. ASME BPV Code Section III “Rules for Construction of Nuclear Facility Components” Division 5 focuses on “High Temperature Reactors”. Subsection HH, subpart A lists the different materials properties that are to be measured and how those properties change due to different environmental conditions (oxidation and irradiation damage) for a graphite to be accepted for use in a high temperature reactor core (i.e., “Code Qualified”). Currently there are no nuclear graphite grades that are “Code Qualified” (i.e., a reactor designer can select a graphite grade and build their reactor without any additional testing), which is due in part to development of new graphite grades in the last 20 years and the lack of comprehensive programs needed to produce the data for the code cases. This perspective is going to discuss the requirements, as called out in the ASME BPV Code, that are necessary to “code qualify” a nuclear graphite grade but will primarily focus on the practical and technical challenges associated with irradiation-induced property changes and how to address these to assist with getting graphite ready for use in advanced nuclear reactors. These same technical challenges can be expected to arise for other materials being developed for advanced reactor concepts.

advanced nuclear reactors↗

Benchmark Modeling and Simulation of the FFTF LOFWOS Test #13 Using SAM

The Fast Flux Test Facility (FFTF) was a 400 MW thermal powered, oxide-fueled, liquid sodium cooled test reactor, built to assist development and testing of advanced fuels and materials for fast breeder reactors. In July 1986, a series of unprotected Loss of Flow Without Scram (LOFWOS) transients were performed in FFTF as part of the Passive Safety Testing (PST) program. The LOFWOS Test #13, which was initiated at 50% power and 100% flow with the pump pony motors left off, has been chosen as a benchmark case by IAEA to support collaborative efforts within international partnerships on the validation of simulation tools and models in the area of sodium fast reactor passive safety in an IAEA Coordinated Research Project (CRP), launched in October 2018. The System Analysis Module (SAM) is an advanced and modern system analysis tool under development at Argonne National Laboratory for advanced non-LWR safety analysis. It utilizes the object-oriented application framework MOOSE to leverage the modern software environment and advanced numerical methods. The capabilities of SAM are being extended to enable the transient modeling, analysis, and design of various advanced nuclear reactor systems. To participate the IAEA CRP and enhance the SAM validation base for advanced reactor transient safety analysis, benchmark simulations of the FFTF LOFWOS Test #13 are performed using the SAM code. In this first phase of the validation effort, the thermal-hydraulic behavior of the reactor system is the focus and the reactor kinetics is not considered in the SAM FFTF model. Instead, the results of Argonne’s neutronics calculations are directly used, including the power shape of the active core region and the power history during the transient. The simulation results of FFTF at steady state agreed well with the measured data from the test. During the transient, reasonably good agreement were also obtained. Future work to improve the model will focus on introducing the reactivity predictions into the model, as well as better understanding or resolving the current discrepancies with the measured data.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Volume 9: Critical Facility with Add-On Ion Beam

Completion of the originally planned critical facility has been considered as part of the High Flux Isotope Reactor (HFIR) Sustaining and Enhancing Neutron Science Initiative at Oak Ridge National Laboratory (ORNL). A working group of ORNL staff members was formed to develop the idea and to recommend one or more configurations to best support future HFIR operations and scientific capacities. HFIR was designed with a critical pool in the reactor bay that was projected to be outfitted as a critical facility. The primary purpose of the planned critical facility was to measure the subcritical worth of fresh fuel elements to support startup requirements. However, the Y-12 National Security Complex already housed a critical facility that was used for this purpose. This report presents the working group’s efforts, including determination of the proposed critical facility’s high-impact benefits. A generic low-power critical facility would be employed for reactor physics measurements, code and data validation, reactor operator and staff training, and education. This facility would be instrumental in supporting current HFIR operations, conversion of HFIR to low-enriched uranium, existing light water reactor operations, and advanced reactor development and deployment.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Of Ashes and Atoms

This feature length DVD documentary, reviews the history of the Plum Brook Nuclear Reactor from the initial settlers of the area, through its use as a munitions facility during the second World War to the development of the nuclear facility and its use as one of the first nuclear test reactors built in the United States, and the only one built by NASA. It concludes with the beginning of the decommissioning of the facility. There is a brief review of the reactor design, and its workings. Through discussions with the NASA engineers and operators of the facility, the film reviews the work done to advance the knowledge of the effects of radiation, the properties of radiated materials, and the work to advance the state of the art in nuclear propulsion. The film shows footage of public tours, and shows actual footage of the facility in operation, and after its shutdown in 1973. The DVD was narrated by Kate Mulgrew, who leads the viewer through the history of the facility to its eventual ongoing decommissioning, and return to the state of pastoral uses.

Source record↗

Perovskite-Derived Cs 2 SnCl 6 –Silica Composites as Advanced Waste Forms for Chloride Salt Wastes

Advanced materials and processes are required to separate halides and fission products from complex salt waste streams associated with the chemical reprocessing of used nuclear fuels and molten salt reactor technologies for immobilization into chemically durable waste forms. Here, in this work, we explore an innovative concept using metal-halide perovskites as advanced host phases to incorporate Cs and Cl with very high waste loadings. Wet chemistry-synthesized Cs 2 SnCl 6 powders from CsCl salt solutions are successfully encapsulated into a silica matrix to form a composite using low-temperature spark plasma sintering with tunable Cs and Cl loadings up to 31 wt.% and 26 wt.%, respectively. Chemical durability testing of the composite waste forms by semi-dynamic leaching experiments demonstrates that incongruent leaching mechanism dominated. The metal-halide perovskite-silica composite waste forms display exceptional chemical durability with the long-term release rates of Cs and Cl comparable to or outperforming the state-of-the-art waste form materials but with significantly higher waste loadings. The scalable synthesis of the metal-halide perovskite from wet-chemistry processes opens up new opportunities in designing perovskite-glass composite waste forms for salt wastes with very high waste loadings and exceptional chemical durability for the sustainable development of advanced fuel cycles and next-generation reactor technologies.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Irradiation performance of a U-7Mo in Al-Si matrix dispersion full-size fuel plate assembly

The Korea Atomic Energy Research Institute (KAERI) is leading the Ki-Jang Research Reactor (KJRR) project with the intent to develop a new reactor for medical isotope production and other nuclear research purposes. The KJRR core is designed to use high density fuel system where uranium alloyed with 7 wt% molybdenum (U-7Mo) particles are dispersed in a matrix of aluminum alloyed with 5 wt% silicon (Al-5Si) and clad in aluminum alloy 6061 (Al-6061) to form fuel plates. KAERI developed a fabrication facility to construct KJRR fuel assemblies and partnered with the Idaho National Laboratory (INL) to irradiate a full-size fuel assembly, with 21 total fuel plates, in the Advanced Test Reactor (ATR). Irradiation testing and subsequent Post Irradiation Exam (PIE) campaigns were performed successfully over a multi-year project. Monte Carlo neutronic calculations, coupling with a depletion code, were performed based on ATR’s as-run power history which showed that the highest power plate (plate 20) reached 83.1 % end-of-life (EOL) local burnup based on initial 235 U content. Additionally, finite element thermal modeling was performed based as-run power history which showed a beginning-of-life (BOL) peak local heat flux of 184 W/cm 2 . No anomalous fuel performance was observed during the irradiation and target test conditions were achieved. PIE showed favorable performance of the fuel assembly regarding all important phenomena. This paper describes the KJRR fuel assembly irradiation conditions and PIE data to support the conclusion that it performed well, without evidence of unexpected or problematic fuel performance, within an irradiation test designed to bound the KJRR design environment.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

SMR safety through HTTF modeling and benchmark efforts for code validation for gas-cooled reactor applications

Accurate modeling and simulation tools for thermal-hydraulics calculations are a key element needed to design and license new advanced reactors including Small Modular Reactors (SMR) and Microreactors. Uncertainties in modeling and simulation can have significant safety and economic implications. The High Temperature Test Facility (HTTF) at Oregon State University (OSU) is a scaled integral effects experiment designed to investigate transient behavior in high-temperature gas-cooled prismatic-block nuclear reactors. High-quality measurement data is available from the HTTF that is suitable for a thermal-hydraulics code validation benchmark for gas-cooled reactor simulations. Here, this paper summarizes individual HTTF modeling efforts to date for tool validation at Idaho National Laboratory (INL), Argonne National Laboratory (ANL), Oregon State University (OSU) and Canadian Nuclear Laboratories (CNL) using system thermal-hydraulics codes, Computational Fluid Dynamics (CFD) codes and system-CFD code couplings. Also, the paper introduces the ongoing OECD Nuclear Energy Agency (NEA) High Temperature Gas Reactor Thermal-Hydraulics (HTGR T/H) benchmark that allows for better comparisons of results between different international modeling teams. The benchmark provides well defined computational problems that include code-to-code comparisons and comparisons to measured data. These problems provide an avenue for quantifying accuracy and identifying sources of uncertainty in thermal-hydraulics calculations, including in measured thermophysical properties, as part of validation for gas-cooled reactor simulation tools.

21 - SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLAN↗

Calculation of Critical Heat Flux Using an Inverse Heat Transfer Method to Support TREAT Experiment Analysis

Heat transfer between cladding and coolant during transient scenarios remains a critical area of uncertainty in understanding nuclear reactor safety. To advance the understanding of transient and accident scenarios involving critical heat flux (CHF), an in-pile experiment for the Transient Reactor Test (TREAT) facility at Idaho National Laboratory was developed. The experiment named CHF-Static Environment Rodlet Transient Test Apparatus (CHF-SERTTA), consists of a hollow borated stainless steel heater rod submerged in a static water pool which is heated via the (n, a) reaction in boron-10. This paper presents a novel inverse heat transfer method to determine CHF by using the optimization and uncertainty software DAKOTA to calibrate a RELAP5-3D model of CHF-SERTTA to temperature measurements obtained from a thermocouple welded to the surface of the rod.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Combined TREAT-LOC & SATS Integral LOCA Experiment Plan

The Transient Reactor Test Facility (TREAT) loss-of-coolant (LOC) and highburnup (HBu) experiment series, along with the Severe Accident Test Station (SATS) HBu experiment series, are integral LOC accident (LOCA) experiments planned under the Department of Energy (DOE) Advanced Fuels Campaign (AFC) program, which aims to support burnup extension needs by addressing identified R&D priorities in order to achieve an improved understanding of fuel fragmentation, relocation, and dispersal (FFRD) of HBu fuel during LOCA events. Priorities have been identified by the Electric Power Research Institute (EPRI)’s Collaborative Research on Advanced Fuel Technologies (CRAFT) Fuel Performance and Testing Technical Experts Group (FPTTEG). The data produced under this plan will be used to further validate and confirm existing models and inform future R&D and model development. The experimental program was specifically developed to address data gaps and opportunities identified via detailed review of the existing public knowledge base on LOCA FFRD, as well as reviewing specific experimental development activities regarding prototypic LOCA conditions for light-water reactor (LWR) systems. The test program relies on a unique combination of in- and out-of-pile experimental approaches to provide a clear tieback to the existing integral and semi-integral LOCA experiment database, using state-of-the-art facilities. More importantly, the program will systematically investigate the impacts of prototypic HBu fuel/cladding thermomechanical behaviors under postulated LWR LOCA conditions not yet fully investigated. These conditions correspond with prototypic decay-energy heatup (DEH) and stored-energy heatup (SEH) conditions. First, TREAT’s unique capability will enable the first evaluation of the impact of SEH conditions on HBu fuels. The test program will emphasize the development of an improved mechanistic understanding of key phenomena through independent experimental systems, development of a database to support fuel performance modeling tools, world-leading advanced materials characterization, and the most advanced approach to in situ diagnostics ever deployed to evaluate FFRD. The results will represent a significant leap forward in evaluating prototypic conditions and novel data to support modeling development and validation, as well as to inform the technical basis for LOCA-induced FFRD.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗