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At least 217 records · Page 12

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DOE OSTI2025

Covariant Quantum Error-Correcting Codes with Metrological Entanglement Advantage

Here, we show that a subset of the basis for the irreducible representations of a tensor-product SU(2) rotation forms a covariant approximate quantum error-correcting code with transversal U(1) logical gates. Generalizing previous work on “thermodynamic codes” to general local spin and different irreducible representations using only properties of the angular momentum algebra, we obtain bounds on the code inaccuracy under generic noise on any known 𝑑 sites, under independent and identically distributed noise, and under heralded 𝑑-local erasures. We demonstrate that this family of codes protects a probe state with quantum Fisher information surpassing the standard quantum limit when the sensing parameter couples to the generator of the U(1) logical gate.

quantum error correction↗

DOE OSTI2023

On the circularly polarized luminescence of individual triplet sublevels

Here, we discuss the possibility of using circularly polarized luminescence (CPL) as a tool to probe individual triplet spin sublevels that are populated nonadiabatically following photoexcitation. This study is motivated by a mechanism proposed for chirality-induced spin selectivity in which coupled electronic-nuclear dynamics may lead to a non-statistical population of the three triplet sublevels in chiral systems. We find that low-temperature CPL should aid in quantifying the exact spin state/s populated through coupled electronic-nuclear motion in chiral molecules.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NASA NTRS1979

Coupled motion of rigid bodies about their center of mass

Nontrivial analytical solutions for the coupled motion of two rigid bodies about their center of mass are obtained on the assumptions that the rigid bodies are coupled by a massless rigid boom and that no external forces are acting on the system. Both relative rotational and translational motions of the two bodies are considered. General equations of motion are derived by regarding the two bodies as consisting of two distinct systems of particles and by applying the principle of conservation of angular momentum. It is shown that a basic nontrivial solution can be obtained for the translational problem if an assumption is made concerning the relative orientation of one principal axis of inertia of each body and that fundamental nontrivial solutions are readily obtained for the rotational problem if an additional assumption is made with respect to the symmetry of one body. Certain stability criteria are found for some of these motions by defining regions of constraint for the relative translational and rotational elements.

Jezewski, D. J.↗

DOE OSTI2023

Effect of the Coulomb force on fission fragment angular momenta

Nuclear fission produces fragments endowed with typically half a dozen units of angular momentum. After scission has occurred, the fragments are still interacting via the Coulomb force which exerts a torque on deformed fragments, thereby accelerating their rotations. Here, the essential features of this effect can be understood by simple perturbative considerations from which the effect on the fragment spin distributions can be obtained. Complete dynamical calculations of the coupled evolution of the spins validate the perturbative treatment, which ignores the second-order terms, showing that the fragment spins evolve essentially independently in the presence of the Coulomb torques.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2024

Terahertz electric-field-driven dynamical multiferroicity in SrTiO 3

The emergence of collective order in matter is among the most fundamental and intriguing phenomena in physics. In recent years, the dynamical control and creation of novel ordered states of matter not accessible in thermodynamic equilibrium is receiving much attention. The theoretical concept of dynamical multiferroicity has been introduced to describe the emergence of magnetization due to time-dependent electric polarization in non-ferromagnetic materials. In simple terms, the coherent rotating motion of the ions in a crystal induces a magnetic moment along the axis of rotation. Here we provide experimental evidence of room-temperature magnetization in the archetypal paraelectric perovskite SrTiO 3 due to this mechanism. We resonantly drive the infrared-active soft phonon mode with an intense circularly polarized terahertz electric field and detect the time-resolved magneto-optical Kerr effect. A simple model, which includes two coupled nonlinear oscillators whose forces and couplings are derived with ab initio calculations using self-consistent phonon theory at a finite temperature, reproduces qualitatively our experimental observations. A quantitatively correct magnitude was obtained for the effect by also considering the phonon analogue of the reciprocal of the Einstein–de Haas effect, which is also called the Barnett effect, in which the total angular momentum from the phonon order is transferred to the electronic one. Our findings show a new path for the control of magnetism, for example, for ultrafast magnetic switches, by coherently controlling the lattice vibrations with light.

36 MATERIALS SCIENCE↗

DOE OSTI2022

Single-ion properties of the transverse-field Ising model material CoNb 2 O 6

We report CoNb 2 O 6 is one of the few materials that is known to approximate the one-dimensional transverse-field Ising model (1D-TFIM) near its quantum critical point. It has been inferred that Co 2+ acts as a pseudospin 1/2 with anisotropic exchange interactions that are largely Ising-like, enabling the realization of the TFIM. However, the behavior of CoNb 2 O 6 is known to diverge from the ideal TFIM under transverse magnetic fields that are far from the quantum critical point, requiring the consideration of additional anisotropic, bond-dependent (Kitaev-like) terms in the microscopic pseudospin-1/2 Hamiltonian. These terms are expected to be controlled in part by single-ion physics, namely the wave function for the pseudospin-1/2 angular momentum doublet. Here, we present the results of both inelastic neutron scattering measurements and electron paramagnetic resonance spectroscopy on CoNb 2 O 6 , which elucidate the single-ion physics of Co 2+ in CoNb 2 O 6 for the first time. We find that the system is well-described by an intermediate spin-orbit coupled Hamiltonian, and the ground state is a well-isolated Kramers doublet with an anisotropic g tensor. We provide the approximate wave functions for this doublet, which we expect will be useful in theoretical investigations of the anisotropic exchange interactions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

NASA NTRS1989

Toward higher order tests of the gravitational interaction

Analyses and interpretations of experiments which test post-Newtonian gravity are usually done under the assumption that gravity is a metric field phenomenon - a manifestation of space-time geometry. This, however, is unnecessary and one can start at a more primitive level - that there simply exists a phenomenological, gravitational, many-body equation of motion which must be determined by a package of observations. In fact, over the last couple decades, a diverse collection of solar system interbody tracking observations, supplemented by data from the binary pulsar system PSR 1913 + 16, has completely mapped out the first post-Newtonian order. After the fact, using empirically determined equations of motion, along with some observed properties of nongravitational clocks and rulers and conservation laws for energy, momentum and angular momentum, a post-Newtonian Lagrangian can be constructed, a geometrical space-time metric field conceptual interpretation can be developed, Lorentz invariance of the equations of motion can be shown, and the equations of motion are found to agree with the predictions of Einstein's gravitational theory, General Relativity, within experimental accuracy.

Nordtvedt, Ken↗

NASA NTRS1985

Jet production in super-Eddington accretion disks

A two-dimensional, radiation-coupled, Newtonian hydrodynamic simulation is reported for a super-Eddington, mass accretion rate, M = 4 M(E) disk accretion flow onto a 3-solar mass pseudoblack hole. Near the disk midplane, convection cells effectively block the accretion flow, even though viscous heating maximizes there. Accretion predominantly occurs in a supersonic inflow which follows streamlines of approximately constant angular momentum. The optically thick inflow traps radiation so that 80 percent of the luminosity is absorbed by the black hole; the emergent power is sub-Eddington. An axial jet self consistently forms just outside a conical photosphere which bounds the accretion zone; radiation pressure accelerates the jet to about 10 to the 10th cm/s. The jet's mass efflux is only 0.4 percent of the total mass accretion rate.

Eggum, G. E.↗

NASA NTRS1995

High-frequency variations in Earth rotation and the planetary momentum budget

The major focus of the subject contract was on helping to resolve one of the more notable discrepancies still existing in the axial momentum budget of the solid Earth-atmosphere system, namely the disappearance of coherence between length-of-day (l.o.d.) and atmospheric angular momentum (AAM) at periods shorter than about a fortnight. Recognizing the importance of identifying the source of the high-frequency momentum budget anomaly, the scientific community organized two special measurement campaigns (SEARCH '92 and CONT '94) to obtain the best possible determinations of l.o.d. and AAM. An additional goal was to analyze newly developed estimates of the torques that transfer momentum between the atmosphere and its underlying surface to determine whether the ocean might be a reservoir of momentum on short time scales. Discrepancies between AAM and l.o.d. at sub-fortnightly periods have been attributed to either measurement errors in these quantities or the need to incorporate oceanic angular momentum into the planetary budget. Results from the SEARCH '92 and CONT '94 campaigns suggest that when special attention is paid to the quality of the measurements, better agreement between l.o.d. and AAM at high frequencies can be obtained. The mechanism most responsible for the high-frequency changes observed in AAM during these campaigns involves a direct coupling to the solid Earth, i.e, the mountain torque, thereby obviating a significant oceanic role.

Rosen, Richard D.↗

DOE OSTI2024

Controlling the orbital Hall effect in gapped bilayer graphene in the terahertz regime

We study the orbital Hall effect (OHE) in the AC regime using bilayer graphene (BLG) as a prototypical material platform. While the unbiased BLG has gapless electronic spectra, applying a perpendicular electric field creates an energy band gap that can be continuously tuned from zero to high values. By exploiting this flexibility, we demonstrate the ability to control the behavior of AC orbital Hall conductivity. Particularly, we demonstrate that the orbital Hall conductivity at the neutrality point changes its signal at a critical frequency, the value of which is proportional to the perpendicular electric field. For BLG with narrow band gaps, the active frequency region for the AC OHE may extend to a few terahertz, which is experimentally accessible with current technologies. We also consider the introduction of a perpendicular magnetic field in the weak-coupling regime using first-order perturbation theory to illustrate how the breaking of time-reversal symmetry enables the emergence of the AC charge Hall effect in the charge-doped situation and modifies the AC orbital Hall conductivity. Our calculations suggest that BLG with narrow band gaps is a practical candidate for investigating time-dependent orbital angular momentum transport. Published by the American Physical Society 2024

36 MATERIALS SCIENCE↗

DOE OSTI2024

Controlling the orbital Hall effect in gapped bilayer graphene in the terahertz regime

36 MATERIALS SCIENCE↗

DOE OSTI2020

Preparation of high orbital angular momentum Rydberg states by optical-millimeter-wave STIRAP

Rydberg states of molecules are intrinsically challenging to study due to the presence of fast non-radiative decay pathways, such as predissociation. However, selectively exciting Rydberg states with values of the orbital angular momentum (ℓ) ℓ ≳ 3 is a productive strategy to minimize this rapid decay and to populate molecular Rydberg states with lifetimes that approach those of atoms. Here, in this proof-of-principle demonstration, we transfer population to an nf Rydberg state of the calcium atom by stimulated Raman adiabatic passage, in which an optical and a millimeter-wave field couple the initial and final states via an intermediate nd Rydberg state. Numerical simulations reproduce the observed time and frequency dependences of the population transfer and suggest the utility of this scheme to populate high-ℓ Rydberg states of molecules.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2022

Unimolecular dissociation dynamics of electronically excited HCO(Ã 2 A"): rotational control of nonadiabatic decay

The photoinduced unimolecular decay of the electronically excited HCO(Ã 2 A") is investigated in a combined experimental–theoretical study. The molecule is excited to the (1, n 2 , 0) combination bands, which decay via Renner–Teller coupling to the ground electronic state. The rovibrational state distribution of the CO fragment was measured via the high-n Rydberg H-atom time-of-flight method and calculated using a wave packet method on an accurate set of potential energy surfaces. It is shown that the non-adiabatic decay rate is strongly modulated by the HCO rotational angular momentum, which leaves unique signatures in the product state distribution. Finally, the experimentally observed bimodal rotational distribution of the dominant CO(v = 0) fragment is likely due to decay of different vibronic states populated by the excitation and modulated by the excited state lifetime, which is in turn controlled by the parent rotational quantum number.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2026

Ultrafast local demagnetization in 𝑑 6 systems via driven Jahn-Teller distortions

Ultrafast control of spin orientations without relying on highly nonequilibrium electron distributions offers a new pathway for femtosecond spintronics. It is shown that excitation of specific vibronic modes can drive a substantial demagnetization of a local moment relative to the magnetization axis, while preserving its total spin quantum number. Using a fully quantum many-body treatment of a local 𝑆=2 (𝑑 6 ) many-body spin coupled to a driven Jahn-Teller mode with quantum dissipation, we find that the projected spin can be strongly reduced via a Jahn-Teller-induced 𝑥⁢𝑦↑→𝑦⁢𝑧/𝑧⁢𝑥↓ transition, which occurs without additional Coulomb exchange cost. The excited state subsequently relaxes back to its original electronic configuration with a rotated spin direction, enabling spin reorientation without generating a large net angular momentum in the electronic subsystem.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2022

The Three-dimensional Collapse of a Rapidly Rotating 16 M ⊙ Star

I report on the three-dimensional (3D) hydrodynamic evolution of a rapidly rotating 16 M ⊙ star to iron core collapse. For the first time, I follow the 3D evolution of the angular momentum (AM) distribution in the iron core and convective shell burning regions for the final 10 minutes up to and including gravitational instability and core collapse. In 3D, convective regions show efficient AM transport that leads to an AM profile that differs in shape and magnitude from MESA within a few shell convective turnover timescales. For different progenitor models, such as those with tightly coupled Si/O convective shells, efficient AM transport in 3D simulations could lead to a significantly different AM distribution in the stellar interior affecting estimates of the natal neutron star or black hole spin. The results suggest that 3D AM transport in convective and rotating shell burning regions are critical components in models of massive stars and could qualitatively alter the explosion outcome and inferred compact remnant properties.

79 ASTRONOMY AND ASTROPHYSICS↗

NASA NTRS1978

Graphical evaluation of relativistic matrix elements

A graphical representation of angular momentum was used to evaluate relativistic matrix elements between antisymmetrized states of many particle configurations having any number of open shells. The antisymmetrized matrix element was expanded as a sum of semisymmetrized matrix elements. The diagram representing a semisymmetrized matrix element was composed of four diagram blocks; the bra block, the ket block, the spectator block, and the interaction block. The first three blocks indicate the couplings of the two interacting configurations while the last depends on the interaction and is the replaceable component. Interaction blocks for relativistic operators and commonly used potentials were summarized in ready to use forms. A simple step by step procedure was prescribed generally for calculating antisymmetrized matrix elements of one and two particle operators.

Huang, K. N.↗

NASA NTRS2018

Imaging X-Ray Polarimetry Explorer Mission Attitude Determination and Control Concept

The goal of the Imaging X-Ray Polarimetry Explorer (IXPE) Mission is to expand understanding of high-energy astrophysical processes and sources, in support of NASA's first science objective in Astrophysics: "Discover how the universe works." X-ray polarimetry is the focus of the IXPE science mission. Polarimetry uniquely probes physical anisotropies-ordered magnetic fields, aspheric matter distributions, or general relativistic coupling to black-hole spin-that are not otherwise measurable. The IXPE Observatory consists of Spacecraft and Payload modules. The Payload includes three polarization sensitive, X-ray detector units (DU), each paired with its corresponding grazing incidence mirror module assemblies (MMA). A deployable boom provides the correct separation (focal length) between the DUs and MMAs. These Payload elements are supported by the IXPE Spacecraft. A star tracker is mounted directly with the deployed Payload to minimize alignment errors between the star tracker line of sight (LoS) and Payload LoS. Stringent pointing requirements coupled with a flexible structure and a non-collocated attitude sensor-actuator configuration requires a thorough analysis of control-structure interactions. A non-minimum phase notch filter supports robust control loop stability margins. This paper summarizes the IXPE mission science objectives and Observatory concepts, and then it describes IXPE attitude determination and control implementation. IXPE LoS pointing accuracy, control loop stability, and angular momentum management are discussed.

Attitude Determination and Contro↗

DOE OSTI2022

Spiers Memorial Lecture: Theory of unimolecular reactions

One hundred years ago, at an earlier Faraday Discussion meeting, Lindemann presented a mechanism that provides the foundation for contemplating the pressure dependence of unimolecular reactions. Since that time, our ability to model and predict the kinetics of such reactions has grown in leaps and bounds through the synergy of ever more sophisticated experimental studies with increasingly high level theoretical analyses. Herein, this review begins with a brief historical overview of the progress from the Lindemann mechanism to the master equation, which now provides the cornerstone for most theoretical analyses. The current status of ab initio transition state theory based implementations of the master equation is then reviewed, beginning with a discussion of the energy resolved chemical conversion rates, followed by a review of the pressure dependence of the thermal kinetics. The latter discussion focusses on the collisional energy and angular momentum transfer rates as well as the complexities of non-thermal effects and of multiple-well multiple-channel reactions. The synergy with recent state-of-the-art experiments is used to motivate these discussions. Attempts to automate the calculations are also briefly reviewed. Throughout the discussion, we provide our perspective on current understanding and continuing challenges and opportunities. One key challenge relates to the coupling of sequences of reactions, which frequently leads to deviations from the classic presumption of thermal reactants.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗