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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 217 records · Page 12
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Polarized electron injector for positron production at CEBAF

As a part of the effort to expand the capabilities of CE-BAF 12 GeV (Continuous Electron Beam Accelerator Facility) at Jefferson Lab, the addition of a polarized positron source is considered. This capability would provide acceleration of high duty-cycle polarized posi-trons, with spin >60% polarization, through the same main CEBAF accelerator machine with appropriate mag-net field reversals and linac phasing to the four CEBAF experimental halls. To produce this positron beam, a high average current (3-10 mA) highly polarized electron beam with energy of 100 ? 150 MeV is required at the positron source target. The focus of this paper is the de-sign of that polarized electron beam injector. We will describe the production and delivery of a >3 mA highly polarized electron beam. We will discuss different aspects of the design, the photocathode gun, beam dynamics simulation results, spin manipulation, bunching and accelerating process and final electron beam parameters.

Kazimi, R.↗
DOE OSTI2022

Design and demonstration of an economical SRF structure for Continuous Wave (CW), high-energy, Megawatt-class beams

Due to its very high RF-to-beam efficiency, superconducting radiofrequency (SRF) cavities have become the technology of choice for the construction of large linear accelerators (linacs) for basic science applications (examples, ESS and PIP-II). The technology is also attractive for high volume industrial applications such as electron irradiation processing of wastewater and flue gas. However, SRF’s current reliance on liquid helium for cryogenic cooling introduces infrastructural and safety challenges for use in industrial settings. Cryocooler conduction-cooling is a recently developed novel technique for operating SRF cavities without requiring liquid helium. This project aims for technical design and economic assessment of a medium energy, high average power e-beam linac based on the conduction-cooled SRF technique for high volume irradiation treatment of wastewater. The goals of this project are (1) to design a medium energy (10 MeV), high average power (1 MW) electron beam accelerator around the cryocooler conduction-cooled SRF cavity technology, (2) demonstrate the required accelerating voltage on a prototype cavity, and (3) build a cost-model to evaluate capital and operating expense of the accelerator.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

X-ray free-electron laser wavefront sensing using the fractional Talbot effect

Wavefront sensing at X-ray free-electron lasers is important for quantitatively understanding the fundamental properties of the laser, for aligning X-ray instruments and for conducting scientific experimental analysis. A fractional Talbot wavefront sensor has been developed. This wavefront sensor enables measurements over a wide range of energies, as is common on X-ray instruments, with simplified mechanical requirements and is compatible with the high average power pulses expected in upcoming X-ray free-electron laser upgrades. Single-shot measurements were performed at 500 eV, 1000 eV and 1500 eV at the Linac Coherent Light Source. These measurements were applied to study both mirror alignment and the effects of undulator tapering schemes on source properties. The beamline focal plane position was tracked to an uncertainty of 0.12 mm, and the source location for various undulator tapering schemes to an uncertainty of 1m, demonstrating excellent sensitivity. These findings pave the way to use the fractional Talbot wavefront sensor as a routine, robust and sensitive tool at X-ray free-electron lasers as well as other high-brightness X-ray sources.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

X-ray FEL linear accelerator design via start-to-end global optimization

An X-ray Free Electron Laser (FEL) prefers using an electron beam with low emittance, small energy spread, and a high core current to generate coherent radiation through an undulator. In order to attain such a high brightness beam, the linear accelerator beam dynamics design generally involves separate photoinjector optimization and linac optimization. In this paper, we propose a new beam dynamics design strategy based on global optimization with fast start-to-end simulations from the photocathode to the end of the accelerator. The new start-to-end model significantly reduces the simulation time and makes the global optimization practical. The global optimization method avoids the need to choose a single solution based on bunch length at the injector exit for the linac optimization and helps find the solution with unfavorable bunch length at the injector exit but better phase space distribution that can result in better final electron beam phase space distribution at the entrance of the undulator. Here, using the start-to-end global optimization, we showed in an application example, with a 100 pC beam that good transverse emittance and over kilo-Ampere final core current can be attained using a photoinjector that consists of a VHF gun and boosting RF cavities.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2025

Demonstration of closed shell breeding of cesium ions with an electron beam ion source

An electron beam ion source serves as a charge breeder for the Californium Rare Isotope Breeder Upgrade (CARIBU) at the Argonne Tandem Linac Accelerator System (ATLAS). The source accepts radioactive beams of 1+ or 2+ ions and raises their charge state for post-acceleration by ATLAS. The efficiency of this process impacts the length of each experiment and, hence, the type and number of experiments that can be run in each program cycle. Recent efforts to improve the charge breeding efficiency for the 80 < A < 160 species typical of CARIBU have focused on utilizing the closed shell breeding technique. Here, with this technique, the electron beam energy is manipulated to take advantage of the large gap in ionization energies at shell closures and selectively populate a single charge state. Charge breeding studies with stable cesium ions have demonstrated an absolute efficiency of 72% for Cs 27+ and a total efficiency of 93%. The Cs 27+ efficiency result represents a factor of 3 improvement over the previous best charge breeding result of 23% for Cs 27+ .

Vondrasek, R. [Argonne National Laboratory (ANL), ↗
DOE OSTI2025

Extending JuTrack’s capabilities to the FRIB accelerator to enhance online modeling

JuTrack is a Julia-based accelerator modeling and tracking package that utilizes compiler-level automatic differentiation (AD) to enable fast and accurate derivative calculations. While JuTrack provides a solid foundation for beam dynamics simulations, its capabilities must be extended to support the Facility for Rare Isotopes (FRIB) linac. This includes modeling heavy-ion linac accelerator components such as the liquid-lithium charge stripper, which facilitates efficient acceleration by remove electrons from heavy isotopes, and incorporating multi-charge state acceleration tracking, which allows for charge-dependent beam dynamics. These extensions address challenges such as the beam matching and optimization of multi charge state through various accelerating structures and beam-material interaction modeling while maintaining the auto differentiation capability. This work focuses on adapting JuTrack to incorporate these elements, enhancing its online modeling abilities. We present modifications to JuTrack’s framework and demonstrate their performance in FRIB simulations.

Accelerator Physics↗
DOE OSTI2022

Manufacturing the Harmonic Kicker Cavity Prototype for the Electron-Ion Collider

High-bunch-frequency beam-separation schemes, such as the injection scheme proposed for the Rapid Cycling Synchrotron at the Electron-Ion Collider, demand rise and fall times an order of magnitude below what can realistically be accomplished with a stripline kicker. Nanosecond-time-scale kick waveforms can instead be obtained by Fourier synthesis in a harmonically resonant quarter-wave radio-frequency cavity which is optimized for high shunt impedance. Originally developed for the Jefferson Lab Electron-Ion Collider (JLEIC) Circulator Cooler Ring, a hypothetical 11-pass ring driven by an energy-recovery linac at Jefferson Lab, our high-power prototype of such a harmonic kicker cavity, which operates at five modes at the same time, will demonstrate the viability of this concept with a beam test at Jefferson Lab. As the geometry of the cavity, tight mechanical tolerances, and number of ports complicate the design and manufacturing process, special care must be given to the order of the manufacturing steps. We present our experiences with the manufacturability of the present design, lessons learned, and first RF test results from the prototype.

Overstreet, S. A.↗
DOE OSTI2022

Manufacturing the Harmonic Kicker Cavity Prototype for the Electron-Ion Collider

High-bunch-frequency beam-separation schemes, such as the injection scheme proposed for the Rapid Cycling Synchrotron at the Electron-Ion Collider, demand rise and fall times an order of magnitude below what can realistically be accomplished with a stripline kicker. Nanosecond-time-scale kick waveforms can instead be obtained by Fourier synthesis in a harmonically resonant quarter-wave radio-frequency cavity which is optimized for high shunt impedance. Originally developed for the Jefferson Lab Electron-Ion Collider (JLEIC) Circulator Cooler Ring, a hypothetical 11-pass ring driven by an energy-recovery linac at Jefferson Lab, our high-power prototype of such a harmonic kicker cavity, which operates at five modes at the same time, will demonstrate the viability of this concept with a beam test at Jefferson Lab. As the geometry of the cavity, tight mechanical tolerances, and number of ports complicate the design and manufacturing process, special care must be given to the order of the manufacturing steps. We present our experiences with the manufacturability of the present design, lessons learned, and first RF test results from the prototype.

Overstreet, S. A.↗
DOE OSTI2026

Beam Performance of the Positron Transport Line for CEBAF Positron Upgrade

The Low Energy Recirculator Facility (LERF) at Jefferson Lab, formerly operated for the Free-Electron Laser program, has been proposed as the injector complex for the planned 12 GeV CEBAF positron upgrade (Ce+BAF), with an additional pathway to support a potential 22 GeV CEBAF electron upgrade. In this configuration, LERF would generate and pre-accelerate positrons to 123 MeV, matching the present injection energy into the North Linac. Due to the relatively large emittance expected from the positron source, a comprehensive acceptance study has been performed from LERF through the CEBAF recirculating linacs and beam transport lines to the experimental halls. The objective is to establish the positron phase-space acceptance and provide design feedback to the positron production and capture systems. Furthermore, given CEBAF’s capability to deliver highly polarized beams, spin-tracking simulations have been carried out including magnet imperfections, alignment errors, and synchrotron-radiation–induced energy spread. Particular attention is given to the evolution of the spin tune and the corresponding depolarization mechanisms along the beam delivery path, especially for providing longitudinal polarization at the experimental halls. These results inform injector design choices and assess the overall feasibility of delivering high-polarization positron beams in CEBAF.

Ogur, S. [Thomas Jefferson National Accelerator Fa↗
DOE OSTI2020

Probing the Electronic Structure of Warm Dense Nickel via Resonant Inelastic X-Ray Scattering

The development of bright free-electron lasers (FEL) has revolutionized our ability to create and study matter in the high-energy-density (HED) regime. Current diagnostic techniques have been successful in yielding information on fundamental thermodynamic plasma properties, but provide only limited or indirect information on the detailed quantum structure of these systems, and on how it is affected by ionization dynamics. In this work we show how the valence electronic structure of solid-density nickel, heated to temperatures of around 10 of eV on femtosecond timescales, can be probed by single-shot resonant inelastic x-ray scattering (RIXS) at the Linac Coherent Light Source FEL. The RIXS spectrum provides a wealth of information on the HED system that goes well beyond what can be extracted from x-ray absorption or emission spectroscopy alone, and is particularly well suited to time-resolved studies of electronic-structure dynamics.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Summary Report on Ion Irradiation Study of Ceramic Coating on Suppressing FCCI

Advanced cladding is critical for advanced nuclear reactors with an enhanced performance in radiation tolerance and neutron transparency. Using advanced cladding will ensure the adequate thermal conductivity and mechanical stability of the cladding base material, corrosion resistance, high-temperature coolant compatibility of the cladding surface, and chemical stability in the cladding inner wall against fuel cladding chemical interaction (FCCI). An innovative cladding with a three-layer structure (i.e., a modified surface, a clad base material, and a modified inner wall) promises to meet all these requirements. Initial research and development (R&D) regarding this innovative cladding seek to demonstrate the effectiveness of a thin ceramic coating in suppressing FCCI under ion irradiation to high dose. This United States (U.S.) Department of Energy (DOE)–Office of Nuclear Energy (NE) project report summarizes the results of recent ion irradiation studies of diffusion-couple samples with details of an ion irradiation experiment, the characterization of the interface microstructure of cerium (Ce)/titanium nitride (TiN)/oxide-dispersion strengthened (ODS), Ce/TiN/iron (Fe), Ce/ODS, and Ce/Fe samples irradiated with 80 million electron-volts (MeV) of xenon (Xe) ions to 100 displacements per atom (dpa) at 500?C using the Argonne Tandem Linac Accelerator System (ATLAS) facility at Argonne National Laboratory (ANL). The results of the ODS-substrate sample are encouraging and demonstrate the effectiveness of a thin ceramic coating on FCCI mitigation under irradiation. The results from an Fe-substrate sample revealed a complex microstructure, and the root cause is discussed.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Electronic Population Transfer via Impulsive Stimulated X-Ray Raman Scattering with Attosecond Soft-X-Ray Pulses

Free electron lasers provide a source of X-ray pulses short enough and intense enough to drive nonlinearities in molecular systems. Impulsive interactions driven by these X-ray pulses provide a way to create and probe valence electron motions with high temporal and spatial resolution. Observing these electronic motions is crucial to understand the role of electronic coherence in chemical processes. A simple nonlinear technique for probing electronic motion, impulsive stimulated X-ray Raman scattering (ISXRS), involves a single impulsive interaction to produce a coherent superposition of electronic states. In this work, we demonstrate electronic population transfer via ISXRS using broad bandwidth (5.5 eV full width at half maximum) attosecond X-ray pulses produced by the Linac Coherent Light Source (LCLS). The impulsive excitation is resonantly enhanced by the oxygen 1s &rarr; 2π* resonance of nitric oxide (NO), and excited state neutral molecules are probed with a time-delayed UV laser pulse.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2025

Influence of substitution pattern on the dynamics of internal conversion and intersystem crossing in thiopyridone isomers

We report a combined experimental and theoretical investigation of the ultrafast internal conversion (IC) and intersystem crossing (ISC) dynamics of two thiopyridone (TP) isomers in solution. Our study used ultrafast transient X-ray absorption spectroscopy (XAS) at the sulfur K-edge, in conjunction with electronic excited state surface hopping molecular dynamics and simulations of the excited state XAS, to investigate the impact of the functional group substitution pattern and solvent on the dynamics of IC and ISC. The combination of the localized X-ray probe and the simulation results enables, in part, the differentiation between ππ* and nπ* character excited states, as well as singlet and triplet states. Access to nπ* character excitations has particular value since they often prove challenging to assess with optical spectroscopy. For 2-TP, the photoexcited S 2 (ππ*) state rapidly undergoes IC to the S 1 (nπ*) state below the instrument response time, followed by ISC to the T 1 (ππ*) state on a timescale of 600 fs in acetonitrile. For 4-TP, the timescale of S 2 to S 1 IC increases to 330 fs and the timescale of ISC increases to more than 10 ps. The differences between isomers are rationalized by considering the key role of the, nπ* intermediates in mediating the intersystem crossing of these systems. Varying the substitution pattern of the molecule can stabilize or destabilize these intermediates leading to the increase in ISC rate in the ortho isomer as compared to the para isomer, while changing the solvent from acetonitrile to water had minimal effect on the electronic excited state relaxation mechanism.

Garratt, Douglas [SLAC National Accelerator Labora↗
DOE OSTI2022

PERLE - ERL Test Facility at Orsay

PERLE (Powerful ERL for Experiments)[1] is a novel Energy Recovery Linac (ERL) test facility, designed to validate choices for a 50 GeV ERL foreseen in the design of the Large Hadron Electron Collider (LHeC) and the Future Circular Collider (FCC-eh), and to host dedicated nuclear and particle physics experiments. Its main thrust is to probe high current, continuous wave (CW), multi-pass operation with superconducting cavities at 802 MHz. With very high transient beam power (10 MW), PERLE offers an opportunity for controllable study of every beam dynamic effect of interest in the next generation of ERL design and becomes a ‘stepping stone’ between present state-of-art 1 MW ERLs and future 100 MW scale applications.

Bogacz, S. Alex↗
DOE OSTI2021

Deep learning reconstruction of attosecond X-ray pulses from an angularly streaked 2D photoelectron momentum distribution

The Linac Coherent Light Source (LCLS) at SLAC National Accelerator Laboratory produces intense X-ray pulses using a beam of accelerated electrons. The X-ray laser enhanced attosecond pulse generation (XLEAP) project at SLAC has enabled LCLS to produce much shorter X-ray pulses than previously possible, with durations of a few hundred attoseconds. To measure the time-profile of these extremely short pulses a velocity map imaging spectrometer (VMI) was developed. The pulse duration is measured with using an angular streaking method.

Franz, Paris↗
DOE OSTI2025

Experimental investigation of longitudinal scraping of H- bunches via photo-detachment

Longitudinal emittance growth is a significant challenge in RF linacs, especially for poorly bunched beams. This stems from particles occupying outer synchrotron oscillation orbits in the LBET, causing unwanted bunch-bunch interactions and degraded beam quality. To address this, we proposed using temporally spaced laser pulses to selectively photo-detach electrons from the longitudinal head and tail regions of H- ion bunches. This approach aims to reduce particle density in extreme orbits, enhancing beam uniformity and limiting emittance growth. Our experiments employed Fermilab's 'LaserNotcher' system at the font end of the linac, delivering 1.6 MW peak power with sub-nanosecond precision. By neutralizing the first and last half-nanosecond of several H- bunches, we measured their propagation injection into the booster. Measurements of pulse width, average height, and temporal spacing over booster cycles were compared between the scraped and unscraped bunches. Statistical analysis evaluated the results’ significance, highlighting the feasibility of laser-based scraping for future linac designs to achieve higher beam energies with improved emittance control.

Landon, Parker [Boston U.]↗
DOE OSTI2025

Experimental investigation of longitudinal scraping of $H-$ bunches via photo-detachment

Longitudinal emittance growth is a significant challenge in RF linacs, especially for poorly bunched beams. This stems from particles occupying outer synchrotron oscillation orbits in the LBET, causing unwanted bunch-bunch interactions and degraded beam quality. To address this, we proposed using temporally spaced laser pulses to selectively photo-detach electrons from the longitudinal head and tail regions of H- ion bunches. This approach aims to reduce particle density in extreme orbits, enhancing beam uniformity and limiting emittance growth. Our experiments employed Fermilab's 'LaserNotcher' system at the font end of the linac, delivering 1.6 MW peak power with sub-nanosecond precision. By neutralizing the first and last half-nanosecond of several H- bunches, we measured their propagation injection into the booster. Measurements of pulse width, average height, and temporal spacing over booster cycles were compared between the scraped and unscraped bunches. Statistical analysis evaluated the results’ significance, highlighting the feasibility of laser-based scraping for future linac designs to achieve higher beam energies with improved emittance control.

Landon, P. [Boston U.; Fermilab]↗
DOE OSTI2025

Real-time data processing for serial crystallography experiments

We report the use of streaming data interfaces to perform fully online data processing for serial crystallography experiments, without storing intermediate data on disk. The system produces Bragg reflection intensity measurements suitable for scaling and merging, with a latency of less than 1 s per frame. Our system uses the CrystFEL software in combination with the ASAP::O data framework. In a series of user experiments at PETRA III, frames from a 16 megapixel Dectris EIGER2 X detector were searched for peaks, indexed and integrated at the maximum full-frame readout speed of 133 frames per second. The computational resources required depend on various factors, most significantly the fraction of non-blank frames ('hits'). The average single-thread processing time per frame was 242 ms for blank frames and 455 ms for hits, meaning that a single 96-core computing node was sufficient to keep up with the data, with ample headroom for unexpected throughput reductions. Further significant improvements are expected, for example by binning pixel intensities together to reduce the pixel count. We discuss the implications of real-time data processing on the `data deluge' problem from recent and future photon-science experiments, in particular on calibration requirements, computing access patterns and the need for the preservation of raw data.

47 OTHER INSTRUMENTATION↗