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NASA NTRS2014

Mass Dependency of Isotope Fractionation of Gases Under Thermal Gradient and Its Possible Implications for Planetary Atmosphere Escaping Process

Physical processes that unmix elements/isotopes of gas molecules involve phase changes, diffusion (chemical or thermal), effusion and gravitational settling. Some of those play significant roles for the evolution of chemical and isotopic compositions of gases in planetary bodies which lead to better understanding of surface paleoclimatic conditions, e.g. gas bubbles in Antarctic ice, and planetary evolution, e.g. the solar-wind erosion induced gas escaping from exosphere on terrestrial planets.. A mass dependent relationship is always expected for the kinetic isotope fractionations during these simple physical processes, according to the kinetic theory of gases by Chapman, Enskog and others [3-5]. For O-bearing (O16, -O17, -O18) molecules the alpha O-17/ alpha O-18 is expected at 0.5 to 0.515, and for S-bearing (S32,-S33. -S34, -S36) molecules, the alpha S-33/ αlpha S-34 is expected at 0.5 to 0.508, where alpha is the isotope fractionation factor associated with unmixing processes. Thus, one isotope pair is generally proxied to yield all the information for the physical history of the gases. However, we recently] reported the violation of mass law for isotope fractionation among isotope pairs of multiple isotope system during gas diffusion or convection under thermal gradient (Thermal Gradient Induced Non-Mass Dependent effect, TGI-NMD). The mechanism(s) that is responsible to such striking observation remains unanswered. In our past studies, we investigated polyatomic molecules, O2 and SF6, and we suggested that nuclear spin effect could be responsible to the observed NMD effect in a way of changing diffusion coefficients of certain molecules, owing to the fact of negligible delta S-36 anomaly for SF6.. On the other hand, our results also showed that for both diffusion and convection under thermal gradient, this NMD effect is increased by lower gas pressure, bigger temperature gradient and lower average temperature, which indicate that the nuclear spin effect may not be the significant contributor as the energies involved in the hyperfine effect are much smaller than those with molecular collisions, especially under convective conditions.

Sun, Tao↗

DOE OSTI2021

A CO-to-H{sub 2} Ratio of ≈10{sup -5} toward the Herbig Ae Star HK Ori

Measurements of gas mass in protoplanetary gas disks form the basis for estimating the conditions of planet formation. Among the most important constraints derived from disk diagnostics are the abundances of gas-phase species critical for understanding disk chemistry. Toward this end, we present direct line-of-sight measurements of H{sub 2} and CO, employing UV absorption spectroscopy from Hubble Space Telescope Cosmic Origins Spectrograph to characterize disk composition, molecular excitation temperatures, and spatial distribution in the circumstellar material around the Herbig Ae stars HK Ori and T Ori. We observe strong CO (N(CO) = 10{sup 15.5} cm{sup −2}; T {sub rot}(CO) = 19 K) and H{sub 2} (N(H{sub 2}) = 10{sup 20.34} cm{sup −2}; T {sub rot}(H{sub 2}) = 141 K) absorption toward HK Ori with a CO/H{sub 2} ratio of (≡N(CO)/N(H{sub 2})) = 1.3{sub −0.7}{sup +1.6} × 10{sup −5}. These measurements place direct empirical constraints on the CO-to-H{sub 2} conversion factor in the disk around a Herbig Ae star for the first time, although there is uncertainty concerning the exact viewing geometry of the disk. The spectra of T Ori show CO (N(CO) = 10{sup 14.9} cm{sup −2}; T {sub rot}(CO) = 124 K) absorption. Interestingly, we do not detect any H{sub 2} absorption toward this star (N(H{sub 2}) < 10{sup 15.9} cm{sup −2}). We discuss a potential scenario for the detection of CO without H{sub 2}, which deserves further investigation. The low abundance ratio measured around HK Ori suggests significant depletion of CO in the circumstellar gas, which conforms with the handful of other recent CO abundance measurements in protoplanetary disks.

47 OTHER INSTRUMENTATION↗

DOE OSTI2021

The Chemical Inventory of the Planet-hosting Disk PDS 70

As host to two accreting planets, PDS 70 provides a unique opportunity to probe the chemical complexity of atmosphere-forming material. We present ALMA Band 6 observations of the PDS 70 disk and report the first chemical inventory of the system. With a spatial resolution of 0."4–0."5 (~50 au), 12 species are detected, including CO isotopologs and formaldehyde, small hydrocarbons, HCN and HCO{sup +} isotopologs, and S-bearing molecules. SO and CH{sub 3}OH are not detected. All lines show a large cavity at the center of the disk, indicative of the deep gap carved by the massive planets. The radial profiles of the line emission are compared to the (sub)millimeter continuum and infrared scattered light intensity profiles. Different molecular transitions peak at different radii, revealing the complex interplay between density, temperature, and chemistry in setting molecular abundances. Column densities and optical depth profiles are derived for all detected molecules, and upper limits obtained for the nondetections. Excitation temperature is obtained for H{sub 2}CO. Deuteration and nitrogen fractionation profiles from the hydrocyanide lines show radially increasing fractionation levels. Comparison of the disk chemical inventory to grids of chemical models from the literature strongly suggests a disk molecular layer hosting a carbon-to-oxygen ratio C/O > 1, thus providing for the first time compelling evidence of planets actively accreting high C/O ratio gas at present time.

74 ATOMIC AND MOLECULAR PHYSICS↗

NASA NTRS1972

Study of the gas contents of rocks: An approach to the evolution of atmospheres on the earth and planets

A high vacuum system was built for extracting volatiles from rocks either by heating or crushing, and preliminary analyses of the volatiles were made for selected terrestrial basalts and granites. The apparatus and experimental procedures are described, and the major problems associated with water measurement and choice of argon to replace neon as the internal standard are discussed. Preliminary analyses of granites and basalts indicate the following: All analyses lie in the H2O-CO2-CO triangle on a C-H-O ternary diagram. The compositions of the volatiles plot in distinct, but overlapping, areas of the C-H-O diagram. Pre-Cambrian granites have a higher volatile content than younger granites. Continental basalts have a higher volatile content than oceanic basalts.

Barker, C.↗

NASA NTRS1995

Urey prize lecture: On the diversity of plausible planetary systems

Models of planet formation and of the orbital stability of planetary systems are used to predict the variety of planetary and satellite systems that may be present within our galaxy. A new approximate global criterion for orbital stability of planetary systems based on an extension of the local resonance overlap criterion is proposed. This criterion implies that at least some of Uranus' small inner moons are significantly less massive than predicted by estimates based on Voyager volumes and densities assumed to equal that of Miranda. Simple calculations (neglecting planetary gravity) suggest that giant planets which acrete substantial amounts of gas while their envelopes are extremely distended ultimately rotate rapidly in the prgrade direction.

Lissauer, J. J.↗

NASA NTRS1999

Implementation of Parallel Computing Technology to Vortex Flow

Mainframe supercomputers such as the Cray C90 was invaluable in obtaining large scale computations using several millions of grid points to resolve salient features of a tip vortex flow over a lifting wing. However, real flight configurations require tracking not only of the flow over several lifting wings but its growth and decay in the near- and intermediate- wake regions, not to mention the interaction of these vortices with each other. Resolving and tracking the evolution and interaction of these vortices shed from complex bodies is computationally intensive. Parallel computing technology is an attractive option in solving these flows. In planetary science vortical flows are also important in studying how planets and protoplanets form when cosmic dust and gases become gravitationally unstable and eventually form planets or protoplanets. The current paradigm for the formation of planetary systems maintains that the planets accreted from the nebula of gas and dust left over from the formation of the Sun. Traditional theory also indicate that such a preplanetary nebula took the form of flattened disk. The coagulation of dust led to the settling of aggregates toward the midplane of the disk, where they grew further into asteroid-like planetesimals. Some of the issues still remaining in this process are the onset of gravitational instability, the role of turbulence in the damping of particles and radial effects. In this study the focus will be with the role of turbulence and the radial effects.

Dacles-Mariani, Jennifer↗

NASA NTRS2004

Analysis of Organic Compounds in Mars Analog Samples

The detailed characterization of organic compounds that might be preserved in rocks, ices, or sedimentary layers on Mars would be a significant step toward resolving the question of the habitability and potential for life on that planet. The fact that the Viking gas chromatograph mass spectrometer (GCMS) did not detect organic compounds should not discourage further investigations since (a) an oxidizing environment in the near surface fines analyzed by Viking is likely to have destroyed many reduced carbon species; (b) there are classes of refractory or partially oxidized species such as carboxylic acids that would not have been detected by the Viking GCMS; and (c) the Viking landing sites are not representative of Mars overall. These factors motivate the development of advanced in situ analytical protocols to carry out a comprehensive survey of organic compounds in martian regolith, ices, and rocks. We combine pyrolysis GCMS for analysis of volatile species, chemical derivatization for transformation of less volatile organics, and laser desorption mass spectrometry (LDMS) for analysis of elements and more refractory, higher-mass organics. To evaluate this approach and enable a comparison with other measurement techniques we analyze organics in Mars simulant samples.

Mahaffy, P. R.↗

NASA NTRS2004

Development of the Terrestrial Planet Finder Coronagraph membrane V-grooves

The Terrestrial Planet Finder mission will study all aaspecs of planets outside our solar system: from their formation and development in disks of dust and gas around newly forming stars to the presence of those planets orbiting the nearest stars; from the numbers at various sizes and places to their suitability as an abode for life.

vibration↗

NASA NTRS2012

Transiting Exoplanet Survey Satellite (TESS)

The Transiting Exoplanet Survey Satellite (TESS) will discover thousands of exoplanets in orbit around the brightest stars in the sky. In a two-year survey, TESS will monitor more than 500,000 stars for temporary drops in brightness caused by planetary transits. This first-ever spaceborne all-sky transit survey will identify planets ranging from Earth-sized to gas giants, around a wide range of stellar types and orbital distances. No ground-based survey can achieve this feat. A large fraction of TESS target stars will be 30-100 times brighter than those observed by Kepler satellite, and therefore TESS . planets will be far easier to characterize with follow-up observations. TESS will make it possible to study the masses, sizes, densities, orbits, and atmospheres of a large cohort of small planets, including a sample of rocky worlds in the habitable zones of their host stars. TESS will provide prime targets for observation with the James Webb Space Telescope (JWST), as well as other large ground-based and space-based telescopes of the future. TESS data will be released with minimal delay (no proprietary period), inviting immediate community-wide efforts to study the new planets. The TESS legacy will be a catalog of the very nearest and brightest main-sequence stars hosting transiting exoplanets, thus providing future observers with the most favorable targets for detailed investigations.

Ricker, G. R.↗

DOE OSTI2025

Gas and dust dynamics in γ Cephei-type disks

Context. Giant planets are observed orbiting the primary stars of close binary systems. Such planets may have formed in compact circumprimary disks, which once surrounded these stars, under conditions much different than those encountered around single stars. Aims. In order to quantify the effects of the strong gravitational perturbations exerted on circumprimary disk material, the three-dimensional (3D) dynamics of gas and dust in orbit around the primary star of a compact and eccentric binary system was modeled by applying the stellar and orbital parameters of γ Cephei, a well-known system that can be representative of a class of close binaries. Methods. Circumprimary gas was approximated as an Eulerian viscous and compressible fluid and modeled by means of 3D hydrodynamical simulations, assuming locally isothermal conditions in the medium around the primary star. Dust grains were modeled as Lagrangean particles, subjected to gravity and aerodynamic drag forces. Models that include a giant planet were also considered. Results. Models indicate that spiral density waves excited around pericenter passage propagate toward the inner boundary of the disk, through at least a few pressure scale-heights from the mid-plane, inducing radial and vertical mixing in the gas. However, perturbations imparted to gas, both in terms of eccentricity and precession, are far weaker than previously estimated by two-dimensional (2D) simulations. Models predict small eccentricities, ≲0.03, and slow retrograde precession. The addition of a giant planet does not change the low eccentricity state of the disk. The parameters applied to the disk would lead to the formation of a massive planet, many times the mass of Jupiter, in agreement with some observations. Micron to mm-size dust grains are well coupled to the gas, resulting in similar dynamics and statistically similar distributions of orbital elements. The planet only affects the dust distributions locally. In agreement with outcomes of recent 2D models, the lifetime of an isolated circumprimary disk would be brief, ~10 5 years, because of its compact nature, requiring a long-term external supply of mass to allow for the in situ formation of a giant planet.

79 ASTRONOMY AND ASTROPHYSICS↗

NASA NTRS1989

Origin and evolution of planetary and satellite atmospheres

The present volume on the origin and evolution of planet and satellite atmospheres discusses the chemistry of interstellar gas and grains, planetary accretion, cometary composition, the inventories of asteroid volatiles, key similarities and differences among the terrestrial planets' atmospheric compositions, and planets' atmospheric escape and water loss. Also discussed are planetary atmosphere-planetary interior evolutionary coupling, the atmospheric composition of the outer planets, the structure and composition of giant planet interiors, the tenuous atmosphere of Io, the sources of the atmospheres of the outer solar system's satellites, the present state and chemical evolution of the Titan, Triton, and Pluto atmospheres, and the thermal structure and heat balance of the outer planets.

Atreya, S. K.↗

NASA NTRS1992

Giant planets: Clues on current and past organic chemistry in the outer solar system

The giant planets of the outer solar system - Jupiter, Saturn, Uranus, and Neptune - were formed in the same flattened disk of gas and dust, the solar nebula, as the terrestrial planets were. Yet, the giant planets differ in some very fundamental ways from the terrestrial planets. Despite enormous differences, the giant planets are relevant to exobiology in general and the origin of life on the Earth in particular. The giant planets are described as they are today. Their basic properties and the chemistry occurring in their atmospheres is discussed. Theories of their origin are explored and aspects of these theories that may have relevance to exobiology and the origin of life on Earth are stressed.

Pollack, James B.↗

NASA NTRS1990

An assessment of the conditions for critical velocity ionization at the weakly magnetized planets

It has been proposed that critical velocity ionization (CVI) may occur in the magnetosheaths of weakly magnetized planets where the solar wind flows through the planets' upper atmospheres. One can examine this possibility for Venus and Mars by using magnetosheath flow and exosphere models to determine whether the criteria for CVI are met. These criteria include Brenning's empirical condition on the cross-field flow velocity (it must not exceed the local magnetosonic velocity) and the 'Townsend condition' requiring that the integrated probability of impact ionization by a hot electron be greater than 1 along a streamline past the planet. Application of the Spreiter-Stahara gas dynamic flow model and the Nagy and coworkers' models for the exospheres lead to the conclusion that the conditions can be met in a limited region near Venus. However, evidence for CVI has not been identified in in-situ data. Since key details of the planet-solar wind interaction can be explained in terms of photoionization alone, other signatures of the process must be sought in the observations if the presence of CVI is to be positively inferred.

Luhmann, J. G.↗

NASA NTRS1981

Effect of a finite ionization rate on the radiative heating of outer planet atmospheric entry probes

The influence of finite rate ionization in the inviscid gas just behind the stagnation shock wave on the radiation heating of probes entering the hydrogen helium atmospere of the major planets was investigated. At the present time, there is disagreement as to whether the radiative flux increases or decreases relative to its equilibrium value when finite rate ionization is considered. Leibowitz and Kuo content that the finite rate ionization in the hydrogen gas just behind the shock wave reduces the radiative flux to the probe, whereas Tiwari and Szema predict that it increases the radiative flux. The radiation modeling used in the calculations of both pairs of these investigators was reviewed. It is concluded that finite rate ionization in the inviscid region of the shock layer should reduce the cold wall radiative heating below the values predicted by equilibrium chemistry assumptions.

Nelson, H. F.↗

DOE OSTI2021

TOI-532b: The Habitable-zone Planet Finder confirms a Large Super Neptune in the Neptune Desert orbiting a metal-rich M-dwarf host

We confirm the planetary nature of TOI-532b, using a combination of precise near-infrared radial velocities with the Habitable-zone Planet Finder, Transiting Exoplanet Survey Satellite (TESS) light curves, ground-based photometric follow up, and high-contrast imaging. TOI-532 is a faint (J ~ 11.5) metal-rich M dwarf with T{sub eff} = 3957 ± 69 K and [Fe/H] = 0.38 ± 0.04; it hosts a transiting gaseous planet with a period of ~2.3 days. Joint fitting of the radial velocities with the TESS and ground-based transits reveal a planet with radius of 5.82 ± 0.19 R {sub ⊕}, and a mass of 61.5{sub -9.3}{sup +9.7} M {sub ⊕}. TOI-532b is the largest and most massive super Neptune detected around an M dwarf with both mass and radius measurements, and it bridges the gap between the Neptune-sized planets and the heavier Jovian planets known to orbit M dwarfs. It also follows the previously noted trend between gas giants and host-star metallicity for M-dwarf planets. In addition, it is situated at the edge of the Neptune desert in the Radius–Insolation plane, helping place constraints on the mechanisms responsible for sculpting this region of planetary parameter space.

36 MATERIALS SCIENCE↗

NASA NTRS2006

Difficulties in Laboratory Studies and Astronomical Observations of Organic Molecules: Hydroxyacetone and Lactic Acid

For the past 35 years, radio astronomy has revealed a rich organic chemistry in the interstellar gas, which is exceptionally complex towards active star-forming regions. New solar systems condense out of this gas and may influence the evolution of life on newly formed planets. Much of the biologically important functionality is present among the some 130 gas-phase molecules found to date, including alcohols, aldehydes, ketones, acids, amines, amides and even the simplest sugar - glycolaldehyde. Still, many unidentified interstellar radio signals remain, and their identification relies on further laboratory study. The molecules hydroxyacetone and lactic acid are relatively small organic molecules, but possess rather complex rotational spectra owing to their high asymmetry. Hydroxyacetone is particularly problematic because it possess a very low barrier to internal rotation, and exhibits strong coupling of the free-rotor states with the overall rotation of the molecule. As in the case of acetamide, a full decomposition method was employed to order the resultant eigenstates onto normal asymmetric top eigenvectors.

Apponi, A. J.↗

DOE OSTI2021

A Gaussian Process Regression Reveals No Evidence for Planets Orbiting Kapteyn’s Star

Radial–velocity (RV) planet searches are often polluted by signals caused by gas motion at the star’s surface. Stellar activity can mimic or mask changes in the RVs caused by orbiting planets, resulting in false positives or missed detections. Here we use Gaussian process regression to disentangle the contradictory reports of planets versus rotation artifacts from Kapteyn’s star. To model rotation, we use joint quasiperiodic kernels for the RV and Hα signals, requiring that their periods and correlation timescales be the same. We find that the rotation period of Kapteyn’s star is 125 days, while the characteristic active-region lifetime is 694 days. Adding a planet to the RV model produces a best-fit orbital period of 100 yr, or 10 times the observing time baseline, indicating that the observed RVs are best explained by star rotation only. We also find no significant periodic signals in residual RV data sets constructed by subtracting off realizations of the best-fit rotation model and conclude that both previously reported “planets” are artifacts of the star’s rotation and activity. Our results highlight the pitfalls of using sinusoids to model quasiperiodic rotation signals.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

NASA NTRS2001

Orbits of Saturn's Inner Moons and Other Observations Connected within the 1995-1996 Saturnian Ring Plane Crossing

We reduced and analyzed radio images of Saturn taken in 1990-1995 at 0.35, 2.0, 3.6 and 6.1 cm wavelength. The latitudinal brightness distribution varies substantially over time. Detailed modeling of these data shows that NH4SH condenses at the thermochemical equilibrium temperature of 235.5 K only at Northern mid-latitudes. Over most of the planet, condensation does not occur until the gas cools to 190 +/- 5 K. Supersaturation may also cause the dark equatorial region seen in 1995 at 6.1 cm. Observations of the rings show that the West (dusk) ansa is brighter than the East (dawn) ansa by factors up to 2. The magnitude of the asymmetry increases with increasing wavelength and with decreasing distance to the planet. This East-West asymmetry may be due to multiple scattering in gravitational wakes. We improved the Monte Carlo scattering code used to model the microwave emission from Saturn's rings at multiple wavelengths. The basic code outlined in Dunn, Molnar, and Fix describes the rings as a uniform, infinite layer of ice spheres with a finite vertical extent. The particle sizes follow a power law distribution and scatter light according to a linear combination of Mie and isotropic phase functions. These parameters may be adjusted to reflect the physical properties in the scattering properties of the ring particles. This is used to construct a model which can be directly compared to Very Large Array data. The code has been extended by including anisotropic particle distributions, primarily in the form of the wake structures that are likely to exist in the enhancements. The vertical extent of the wakes equals that of the ring layer. Between the wakes are regions of diminished density so that the optical depth integrated over many wakes matches that of the Voyager occultation experiments. This allows us to model the brightness temperature as a function of azimuth and look for asymmetric scattering behavior in the rings. By changing the width and relative density of the wakes, we can alter the nature of the gross scattering properties of the rings to match what is seen in our data.

Lissauer, Jack J.↗