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At least 217 records · Page 12

Comparison of Shortwave Cloud Radiative Forcing Derived from ARM SGP Surface and GOES-8 Satellite Measurements During ARESE I and ARESE II

One of the objectives of the ARM Enhanced Shortwave Experiment (ARESE) is to investigate the absorption of solar radiation by clouds over the ARM Southern Great Plains central facility. A variety of techniques employing various combinations Of Surface, aircraft, and satellite data have been used to estimate the absorption empirically. During ARESE-I conducted during fall 1995, conflicting results were produced from different analyses of the combined datasets leading to the need for a more controlled experiment. ARESE-II was conducted during spring 2000. Improved calibrations, different sampling strategies, and broadband satellite data were all available to minimize some of the sources of uncertainty in the data. In this paper, cloud absorption or its parametric surrogates (e.g., Cess et al. 1995) are derived from collocated and coincident surface and satellite radiometer data from both ARESE-I and ARESE-II using the latest satellite and surface instrument calibrations.

Rapp, A. D.↗

Modeling radiation forces acting on TOPEX/Poseidon for precision orbit determination

Geodetic satellites such as GEOSAT, SPOT, ERS-1, and TOPEX/Poseidon require accurate orbital computations to support the scientific data they collect. Until recently, gravity field mismodeling was the major source of error in precise orbit definition. However, albedo and infrared re-radiation, and spacecraft thermal imbalances produce in combination no more than a 6-cm radial root-mean-square (RMS) error over a 10-day period. This requires the development of nonconservative force models that take the satellite's complex geometry, attitude, and surface properties into account. For TOPEX/Poseidon, a 'box-wing' satellite form was investigated that models the satellite as a combination of flat plates arranged in a box shape with a connected solar array. The nonconservative forces acting on each of the eight surfaces are computed independently, yielding vector accelerations which are summed to compute the total aggregate effect on the satellite center-of-mass. In order to test the validity of this concept, 'micro-models' based on finite element analysis of TOPEX/Poseidon were used to generate acceleration histories in a wide variety of orbit orientations. These profiles are then compared to the box-wing model. The results of these simulations and their implication on the ability to precisely model the TOPEX/Poseidon orbit are discussed.

Marshall, J. A.↗

Solar Radiation and Cloud Radiative Forcing in the Pacific Warm Pool Estimated Using TOGA COARE Measurements

The energy budget of the tropical western Pacific (TWP) is particularly important because this is one of the most energetic convection regions on the Earth. Nearly half of the solar radiation incident at the top of atmosphere is absorbed at the surface and only about 22% absorbed in the atmosphere. A large portion of the excess heat absorbed at the surface is transferred to the atmosphere through evaporation, which provides energy and water for convection and precipitation. The western equatorial Pacific is characterized by the highest sea surface temperature (SST) and heaviest rainfall in the world ocean. A small variation of SST associated with the eastward shift of the warm pool during El-Nino/Souther Oscillation changes the atmospheric circulation pattern and affects the global climate. In a study of the TWP surface heat and momentum fluxes during the Tropical Ocean and Global Atmosphere Coupled Ocean-Atmosphere Response Experiment (TOGA COARE) Intensive observing period (IOP) from November 1992 to February have found that the solar radiation is the most important component of the surface energy budget, which undergoes significant temporal and spatial variation. The variations are influenced by the two 40-50 days Madden Julian Oscillations (MJOs) which propagated eastward from the Indian Ocean to the Central Pacific during the IOP. The TWP surface solar radiation during the COARE IOP was investigated by a number of studies. In addition, the effects of clouds on the solar heating of the atmosphere in the TWP was studied using energy budget analysis. In this study, we present some results of the TWP surface solar shortwave or SW radiation budget and the effect of clouds on the atmospheric solar heating using the surface radiation measurements and Japan's Geostationary Meteorological Satellite 4 radiance measurements during COARE IOP.

Chou, Ming-Dah↗

Strategy to use the Terra Aerosol Information to Derive the Global Aerosol Radiative Forcing of Climate

Terra will derive the aerosol optical thickness and properties. The aerosol properties can be used to distinguish between natural and human-made aerosol. In the polar orbit Terra will measure aerosol only once a day, around 10:30 am. How will we use this information to study the global radiative impacts of aerosol on climate? We shall present a strategy to address this problem. It includes the following steps: - From the Terra aerosol optical thickness and size distribution model we derive the effect of aerosol on reflection of solar radiation at the top of the atmosphere. In a sensitivity study we show that the effect of aerosol on solar fluxes can be derived 10 times more accurately from the MODIS data than derivation of the optical thickness itself. Applications to data over several regions will be given. - Using 1/2 million AERONET global data of aerosol spectral optical thickness we show that the aerosol optical thickness and properties during the Terra 10:30 pass are equivalent to the daily average. Due to the aerosol lifetime of several days measurements at this time of the day are enough to assess the daily impact of aerosol on radiation. - Aerosol impact on the top of the atmosphere is only part of the climate question. The INDOEX experiment showed that addressing the impact of aerosol on climate, requires also measurements of the aerosol forcing at the surface. This can be done by a combination of measurements of MODIS and AERONET data.

Kaufman, Yoram J.↗

Direct and semi-direct radiative forcing of biomass-burning aerosols over the southeast Atlantic (SEA) and its sensitivity to absorbing properties: a regional climate modeling study

Simulations are performed for the period 2000-2015 by two different regional climate models, ALADIN and RegCM, to quantify the direct and semi-direct radiative effects of biomass-burning aerosols (BBAs) in the southeast Atlantic (SEA) region. Different simulations have been performed using strongly absorbing BBAs in accordance with recent in situ observations over the SEA. For the July-August-September (JAS) season, the single scattering albedo (SSA) and total aerosol optical depth (AOD) simulated by the ALADIN and RegCM models are consistent with the MACv2 climatology and MERRA-2 and CAMS-RA reanalyses near the biomass-burning emission sources. However, the above-cloud AOD is slightly underestimated compared to satellite (MODIS and POLDER) data during the transport over the SEA. The direct radiative effect exerted at the continental and oceanic surfaces by BBAs is significant in both models and the radiative effects at the top of the atmosphere indicate a remarkable regional contrast over SEA (in all-sky conditions), with a cooling (warming) north (south) of 10°S, which is in agreement with the recent MACv2 climatology. In addition, the two models indicate that BBAs are responsible for an important shortwave radiative heating of ~0.5-1K per day over SEA during JAS with maxima between 2 and 4 km a.m.s.l. (above mean sea level). At these altitudes, BBAs increase air temperature by ~0.2-0.5 K, with the highest values being co-located with low stratocumulus clouds. Vertical changes in air temperature limit the subsidence of air mass over SEA, creating a cyclonic anomaly. The opposite effect is simulated over the continent due to the increase in lower troposphere stability. The BBA semi-direct effect on the lower troposphere circulation is found to be consistent between the two models. Changes in the cloud fraction are moderate in response to the presence of smoke, and the models differ over the Gulf of Guinea. Finally, the results indicate an important sensitivity of the direct and semi-direct effects to the absorbing properties of BBAs. Over the stratocumulus (Sc) region, DRE varies from +0.94 W m -2 (scattering BBAs) to +3.93 W m -2 (most absorbing BBAs).

54 ENVIRONMENTAL SCIENCES↗

Direct and Semi-Direct Radiative Forcing of Biomass-Burning Aerosols Over the Southeast Atlantic (SEA) And Its Sensitivity to Absorbing Properties: A Regional Climate Modeling Study

Simulations are performed for the period 2000–2015 by two different regional climate models, ALADIN and RegCM, to quantify the direct and semi-direct radiative effects of biomass-burning aerosols (BBAs) in the southeast Atlantic (SEA) region. Different simulations have been performed using strongly absorbing BBAs in accordance with recent in situ observations over the SEA. For the July–August–September (JAS) season, the single scattering albedo (SSA) and total aerosol optical depth (AOD) simulated by the ALADIN and RegCM models are consistent with the MACv2 climatology and MERRA-2 and CAMS-RA reanalyses near the biomass-burning emission sources. However, the above-cloud AOD is slightly underestimated compared to satellite (MODIS and POLDER) data during the transport over the SEA. The direct radiative effect exerted at the continental and oceanic surfaces by BBAs is significant in both models and the radiative effects at the top of the atmosphere indicate a remarkable regional contrast over SEA (in all-sky conditions), with a cooling (warming) north (south) of 10 ∘S, which is in agreement with the recent MACv2 climatology. In addition, the two models indicate that BBAs are responsible for an important shortwave radiative heating of ∼0.5–1 K per day over SEA during JAS with maxima between 2 and 4 km a.m.s.l. (above mean sea level). At these altitudes, BBAs increase air temperature by ∼0.2–0.5 K, with the highest values being co-located with low stratocumulus clouds. Vertical changes in air temperature limit the subsidence of air mass over SEA, creating a cyclonic anomaly. The opposite effect is simulated over the continent due to the increase in lower troposphere stability. The BBA semi-direct effect on the lower troposphere circulation is found to be consistent between the two models. Changes in the cloud fraction are moderate in response to the presence of smoke, and the models differ over the Gulf of Guinea. Finally, the results indicate an important sensitivity of the direct and semi-direct effects to the absorbing properties of BBAs. Over the stratocumulus (Sc) region, DRE varies from +0.94 W m−2 (scattering BBAs) to +3.93 W m−2 (most absorbing BBAs).

Marc Mallet↗

Radiatively forced dispersion of the Mt. Pinatubo volcanic cloud and induced temperature perturbations in the stratosphere during the first few months following the eruption

A combined 3-dimensional circulation model and aerosol microphysical/transport model is used to simulate the dispersion of the Mt. Pinatubo volcanic cloud in the stratosphere for the first few months following the eruption. Radiative heating of the cloud due to upwelling infrared radiation from the troposphere is shown to be an important factor affecting the transport. Without cloud heating, cloud material stays mostly north of the equator, whereas with cloud heating, the cloud is transported southward across the equator within the first two weeks following the eruption. Generally the simulations agree with Total Ozone Mapping Spectrometer (TOMS), Advanced Very High Resolution Radiometer (AVHRR), and Stratospheric Aerosol and Gas Experiment (SAGE) satellite observations showing the latitude distribution of cloud material to be between about 20 deg S and 30 deg N within the first few months. Temperature perturbations in the stratosphere induced by the aerosol heating are generally 1-4 K, in the range of those observed.

Young, Richard E.↗

Cloud Radiative Forcing at the ARM Climate Research Facility: Technique, Validation, and Comparison to Satellite-derived Diagnostic Quantities - Part 1

It has been hypothesized that continuous ground-based remote sensing measurements from active and passive remote sensors combined with regular soundings of the atmospheric thermodynamic structure can be combined to describe the effects of clouds on the clear sky radiation fluxes. We critically test that hypothesis in this paper and a companion paper (Part II). Using data collected at the Southern Great Plains (SGP) Atmospheric Radiation Measurement (ARM) site sponsored by the U.S. Department of Energy, we explore an analysis methodology that results in the characterization of the physical state of the atmospheric profile at time resolutions of five minutes and vertical resolutions of 90 m. The description includes thermodynamics and water vapor profile information derived by merging radiosonde soundings with ground-based data, and continues through specification of the cloud layer occurrence and microphysical and radiative properties derived from retrieval algorithms and parameterizations. The description of the atmospheric physical state includes a calculation of the infrared and clear and cloudy sky solar flux profiles. Validation of the methodology is provided by comparing the calculated fluxes with top of atmosphere (TOA) and surface flux measurements and by comparing the total column optical depths to independently derived estimates. We find over a 1-year period of comparison in overcast uniform skies, that the calculations are strongly correlated to measurements with biases in the flux quantities at the surface and TOA of less than 10% and median fractional errors ranging from 20% to as low as 2%. In the optical depth comparison for uniform overcast skies during the year 2000 where the optical depth varies over 3 orders of magnitude we find a mean positive bias of 46% with a median bias of less than 10% and a 0.89 correlation coefficient. The slope of the linear regression line for the optical depth comparison is 0.86 with a normal deviation of 20% about this line. In addition to a case study where we examine the cloud radiative effects at the TOA, surface and atmosphere by a middle latitude synoptic-scale cyclone, we examine the cloud top pressure and optical depth retrievals of ISCCP and LBTM over a period of 1 year. Using overcast period from the year 2000, we find that the satellite algorithms tend to bias cloud tops into the middle troposphere and underestimate optical depth in high optical depth events (greater than 100) by as much as a factor of 2.

Mace, Gerald G.↗

Radiative Forcing of the Lower Stratosphere over the Arctic by Light Absorbing Particles

Light absorbing particles (LAP), such as soot and dust, change the thermodynamic structure of the atmosphere and contribute to regional and global climate change. The lower stratosphere (LS) is particularly sensitive to the presence of LAP since the lifetime of particles in the LS may extend from months to years, in contrast to tropospheric lifetimes of at most a few days. The source of particles in the LS may be aircraft, meteorites or emissions from tropospheric sources. There has been a lack, however, of accurate, quantitative measurements made with sufficiently sensitive instruments. This limits our understanding of the origin and lifetime of aerosols in this region of the atmosphere. Here we present recent measurements in the Arctic UT/LS with a new, highly sensitive instrument that has detected black carbon (BC) mass concentrations of 20-1000 ng m(exp -3) that are 10-1000 times larger than those reported in previous studies and are at least 30 times larger than predicted masses based on fuel consumption by commercial aircraft that fly in these regions. Scattering and absorption of solar and terrestrial radiation by the particles in a layer from 8- 12 Km leads to a negative net forcing of -0.5 W sq m at the top of the atmosphere and 9C of heating in this layer during the average aerosol lifetime at these altitudes. The new measurements suggest that the influence of aircraft emissions have been underestimated or that aircraft may not be the only significant source of light absorbing particles in the UT/LS. The presence of these aerosols can cause local changes in the thermal structure of the lower stratosphere and a subsequent modification of stratosphere/tropopause exchange of gases and particles.

Baumgardner, D.↗

Analysis of the Diurnal Cycle of Precipitation and its Relation to Cloud Radiative Forcing using TRMM Products

By incorporating the Tropical Rain Measuring Mission (TRMM) satellite orbital information into the geodesic version of the Colorado State University General Circulation Model (CSU GCM), we are able to fly a satellite in the GCM, and sample the simulated atmosphere in the same way as the TRMM sensors sample the real atmosphere. The TRMM sampling statistics of precipitation and radiative fluxes at annual, intraseasonal, monthly-mean and composited diurnal time scales are evaluated by comparing the satellite-sampled against fully-sampled simulated atmospheres. This information provides a valuable guidance for efficient usage of TRMM data and future satellite mission planning.

Randall, David A.↗

Atmospheric Composition and Radiative Forcing Effects due to UN International Ship Emissions Regulations (ACRUISE) Field Campaign Report

Aerosols, or atmospheric particulates, are long known to be able to seed clouds and modify their characteristics (e.g., cloud brightness, coverage, lifetime). However, the impact of aerosols on clouds is highly complex and non-linear. As a result, aerosol-cloud interaction remains the largest uncertainty in our understanding of the Earth’s radiative balance and in any future climate projections. Aerosols are also a principal component of air pollution and are known to adversely affect respiratory and cardiovascular health.

54 ENVIRONMENTAL SCIENCES↗

Radiative Forcing of the Stratosphere by SO(sub 2) Gas, Silicate Ash, and H(sub 2)SO(sub 4) Aerosols Shortly after the 1982 Eruptions of El Chichon

The 1982 eruptions of El Chichon Volcano injected large quantities of sulfur dioxide gas and silicate ash into the stratosphere. Several studies have shown that the long-lived sulfuric acid aerosols derived from these volcanic effluents produced measurable changes in the radiative heating rates and the global circulation. The radiative and dynamical perturbations associated with the short-lived, but more strongly absorbing sulfur dioxide and ash clouds have received much less attention. We therefore used an atmospheric radiative transfer model and observations collected by satellites, aircraft, and ground based observers to estimate the amplitudes of the stratospheric radiative heating rate perturbations produced by each of these components during the first few weeks after the El Chichon eruption. One week after the April 4, 1982 eruption, net radiative heating rate perturbations exceeding 20 Kelvin per day were found at altitudes near 26 km.

El Chichon↗

Improving Aerosol Radiative Forcing and Climate in E3SM: Impacts of New Cloud Microphysics and Improved Wet Removal Treatments

Abstract Numerous Earth system models exhibit excessive aerosol effective forcing at the top of the atmosphere (TOA), including the Department of Energy's Energy Exascale Earth System Model (E3SM). Here, in the context of the E3SM version 3 effort, the predicted particle property (P3) stratiform cloud microphysics scheme and an enhanced deep convection parameterization suite (ZM_plus) are implemented into E3SM. The ZM_plus includes a convective cloud microphysics scheme, a multi‐scale coherent structure parameterization for mesoscale convective systems, and a revised cloud base mass flux formulation considering impacts of the large‐scale environment. The P3 scheme improved cloud and radiation particularly over the Northern Hemisphere and the frequency of heavy precipitation over the tropics, and the ZM_plus improved clouds in the tropics. P3 decreases aerosol effective forcing by 0.15 W m −2 , while the ZM_plus increases it by 0.27 W m −2 , resulting from excessive direct (0.31 W m −2 ) and indirect forcing (−1.79 W m −2 ). The excessive aerosol forcings are due to aerosol overestimation associated with insufficient aerosol wet removal. By improving the physical treatments in the aerosol wet removal, we effectively mitigate anthropogenic aerosol overestimation and thus attenuate direct (0.09 W m −2 ) and indirect aerosol forcing (−1.52 W m −2 ). Adjustment to primary organic matter hygroscopicity reduces direct and indirect forcing to more reasonable values: −0.13 W m −2 and −1.31 W m −2 , respectively. On climatology, improved aerosol treatments mitigate overestimation of aerosol optical depth.

54 ENVIRONMENTAL SCIENCES↗

The Influence of Aerosols on the Shortwave Cloud Radiative Forcing from North Pacific Oceanic Clouds: Results from the Cloud Indirect Forcing Experiment (CIFEX)

Aerosols over the Northeastern Pacific Ocean enhance the cloud drop number concentration and reduce the drop size for marine stratocumulus and cumulus clouds. These microphysical effects result in brighter clouds, as evidenced by a combination of aircraft and satellite observations. In-situ measurements from the Cloud Indirect Forcing Experiment (CIFEX) indicate that the mean cloud drop number concentration in low clouds over the polluted marine boundary layer is greater by 53/cu cm compared to clean clouds, and the mean cloud drop effective radius is smaller by 4 microns. We link these in-situ measurements of cloud modification by aerosols, for the first time, with collocated satellite broadband radiative flux observations from the Clouds and the Earth's Radiant Energy System (CERES) to show that these microphysical effects of aerosols enhance the top-of-atmosphere cooling by -9.9+/-4.3 W/sq m for overcast conditions.

Wilcox, Eric M.↗

Influence of Aerosols on the Shortwave Cloud Radiative Forcing from North Pacific Oceanic Clouds: Results from the Cloud Indirect Forcing Experiment (CIFEX)

Aerosols over the Northeastern Pacific Ocean enhance the cloud drop number concentration and reduce the drop size for marine stratocumulus and cumulus clouds. These microphysical effects result in brighter clouds, as evidenced by a combination of aircraft and satellite observations. In-situ measurements from the Cloud Indirect Forcing Experiment (CIFEX) indicate that the mean cloud drop number concentration in low clouds over the polluted marine boundary layer is greater by 53 cm(sup -3) compared to clean clouds, and the mean cloud drop effective radius is smaller by 4 micrometers. We link these in-situ measurements of cloud modification by aerosols, for the first time, with collocated satellite broadband radiative flux observations from the Clouds and the Earth s Radiant Energy System to show that these microphysical effects of aerosols enhance the top-of-atmosphere cooling by -.9.9 plus or minus 4.3 W m(sup -2) for overcast conditions.

Wilcox, Eric M.↗

Aerosol Radiative Forcing in Asian Continental Outflow

Aerosols in elevated layers were sampled with FSSP-probes and wire impactors over the Pacific ocean aboard the NASA DC-8 aircraft. Analyses of particle size and morphology identifies two distinctly different aerosol types for cases when the mid-visible extinctions exceed 0.2/km. Smaller sizes (effective radii of 0.2 um) and moderate absorption (mid-visible single scattering albedo of.935) are typical for urban-industrial pollution. Larger sizes (effective radii of 0.7 um) and weak absorption (mid-visible single scattering albedo of 0.985) identify dust. This aerosol classification is in agreement with its origin as determined by airmass back trajectory analysis. Based on lidar vertical profiling, aerosol dominated by dust and urban-industrial pollution above 3km were assigned mid-visible optical depths of 0.50 and 0.27, respectively. Radiative transfer simulations, considering a 50% cloud-cover below the aerosol layers, suggest (on a daily tP C)C> basis) small reductions (-4W/m2) to the energy budget at the top of the atmosphere for both aerosol types. For c' 0 dust, more backscattering of sunlight (weaker solar absorption) is compensated by a stronger greenhouse effect due to larger sizes. Forced reductions to the energy budget at the surface are 12W/m2 for both aerosol types. In contrast, impacts on heating rates within the aerosol layers are quite different: While urban-industrial aerosol warms the layer (at +0.6K/day as solar heating dominates), dust cools (at -0.5K/day as infrared cooling dominates). Sensitivity tests show the dependence of the aerosol climatic impact on the optical depth, particle size, absorptivity, and altitude of the layers, as well as clouds and surface properties. Climatic cooling can be eliminated (1) for the urban-industrial aerosol if absorption is increased to yield a mid-visible single scattering albedo of 0.89, or if the ocean is replaced by a land surface; (2) for the dust aerosol if the effective radius is increased from 0.7 to 1.2 um. The removal of low-level clouds doubles the cooling at the top of the atmosphere to about -8W/m2.

Pueschel, R.↗

Remote Sensing of Aerosol and Aerosol Radiative Forcing of Climate from EOS Terra MODIS Instrument

The recent launch of EOS-Terra into polar orbit has begun to revolutionize remote sensing of aerosol and their effect on climate. Terra has five instruments, two of them,Moderate Resolution Imaging Spectroradiometer (MODIS) and Multiangle Imaging Spectro-Radiometer (MISR) are designed to monitor global aerosol in two different complementary ways. Here we shall discuss the use of the multispectral measurements of MODIS to derive: (1) the global distribution of aerosol load (and optical thickness) over ocean and land; (2) to measure the impact of aerosol on reflection of sunlight to space; and (3) to measure the ability of aerosol to absorb solar radiation. These measurements have direct applications on the understanding of the effect of aerosol on climate, the ability to predict climate change, and on the monitoring of dust episodes and man-made pollution. Principles of remote sensing of aerosol from MODIS will be discussed and first examples of measurements from MODIS will be provided.

Kaufman, Yoram↗