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At least 217 records · Page 12

Final report: Insights from ARM observations into aerosol processing and transport by extratropical cyclones and aerosol effects on cyclone clouds

This project advanced understanding of aerosol–cloud interactions in extratropical cyclones using observations from the Atmospheric Radiation Measurement (ARM) Eastern North Atlantic (ENA) observatory and ACE-ENA field campaigns, along with satellite datasets and numerical modeling. We have quantified the susceptibility of frontal clouds to aerosols, showing that this susceptibility is similar to that in non-frontal clouds despite substantial (factor 2) differences in droplet concentrations between these cloud types, and also significant differences in cloud albedo. A key finding was that Aitken-mode (here, 60-100nm diameter) aerosols play a disproportionately important role in droplet activation in frontal clouds, and concentrations of these particles are frequently strongly biased in climate models. Activation of aerosols depends strongly on updraft speeds, and via collaboration with Argonne National Laboratory we contributed to quantifying these better with the ARM radar wind profiler at the ENA site. Our studies in the North Atlantic have analogs in the Southern Ocean, and to draw these out we examined data from the MARCUS and SOCRATES field campaigns. We identified new particle formation within extratropical cyclones as a potentially important source of cloud condensation nuclei in these pristine marine environments. By combining ARM observations with perturbed parameter ensemble simulations, we demonstrated that surface observations can effectively constrain aerosol–cloud adjustments and reduce uncertainty in simulated cloud liquid water path responses by approximately 15%, yielding stronger constraints on historical aerosol cooling effects. The work further established precipitation processes as a dominant control on aerosol–cloud interactions and Earth system predictability.

Gordon, Hamish [Department of Chemical Engineering↗

Large Eddy Simulation of the Diurnal Cycle of Shallow Convection in the Central Amazon

Climate models often face challenges in accurately simulating the daily precipitation cycle over tropical land areas, particularly in the Amazon. One contributing factor may be the incomplete representation of the diurnal evolution of shallow cumulus (ShCu) clouds. This study aimed to enhance the understanding of the diurnal cycles of ShCu clouds—from formation to maturation and dissipation—over the Central Amazon (CAMZ). Using observational data from the Green Ocean Amazon 2014 (GoAmazon) campaign and large eddy simulation (LES) modeling, we analyzed the diurnal cycles of six selected pure ShCu cases and their composite behavior. Our results revealed a well-defined cycle, with cloud formation occurring between 10 and 11 local time (LT), maturity from 13 to 15 LT, and dissipation by 17–18 LT. The vertical extent of the liquid water mixing ratio and the intensity of the updraft mass flux were closely associated with increases in turbulent kinetic energy (TKE), enhanced buoyancy flux within the cloud layer, and reduced large-scale subsidence. We further analyzed the diurnal cycles of the convective available potential energy (CAPE), the convective inhibition (CIN), the Bowen ratio (BR), and the vertically integrated TKE in the mixed layer (ITKE-ML), exploring their relationships with the cloud base mass flux (Mb) and cloud depth across the six ShCu cases. ITKE-ML and Mb exhibited similar diurnal trends, peaking at approximately 14–15 LT. However, no consistent relationships were found between CAPE (or BR) and Mb. Similarly, comparisons of the cloud depth with CAPE, BR, ITKE-ML, CIN, and Mb revealed no clear relationships. Smaller ShCu clouds were sometimes linked to higher CAPE and lower CIN. It is important to emphasize that these findings are preliminary and based on a limited sample of ShCu cases. Further research involving an expanded dataset and more detailed analyses of the TKE budget and synoptic conditions is necessary. Such efforts would yield a more comprehensive understanding of the factors influencing ShCu clouds’ vertical development.

54 ENVIRONMENTAL SCIENCES↗

Cloud response to co-condensation of water and organic vapors over the boreal forest

Abstract. Accounting for the condensation of organic vapors along with water vapor (co-condensation) has been shown in adiabatic cloud parcel model (CPM) simulations to enhance the number of aerosol particles that activate to form cloud droplets. The boreal forest is an important source of biogenic organic vapors, but the role of these vapors in co-condensation has not been systematically investigated. In this work, the environmental conditions under which strong co-condensation-driven cloud droplet number enhancements would be expected over the boreal biome are identified. Recent measurement technology, specifically the Filter Inlet for Gases and AEROsols (FIGAERO) coupled to an iodide-adduct chemical ionization mass spectrometer (I-CIMS), is utilized to construct volatility distributions of the boreal atmospheric organics. Then, a suite of CPM simulations initialized with a comprehensive set of concurrent aerosol observations collected in the boreal forest of Finland during spring 2014 is performed. The degree to which co-condensation impacts droplet formation in the model is shown to be dependent on the initialization of temperature, relative humidity, updraft velocity, aerosol size distribution, organic vapor concentration, and the volatility distribution. The predicted median enhancements in cloud droplet number concentration (CDNC) due to accounting for the co-condensation of water and organics fall on average between 16 % and 22 %. This corresponds to activating particles 10–16 nm smaller in dry diameter that would otherwise remain as interstitial aerosol. The highest CDNC enhancements (ΔCDNC) are predicted in the presence of a nascent ultrafine aerosol mode with a geometric mean diameter of ∼ 40 nm and no clear Hoppel minimum, indicative of pristine environments with a source of ultrafine particles (e.g., via new particle formation processes). Such aerosol size distributions are observed 30 %–40 % of the time in the studied boreal forest environment in spring and fall when new particle formation frequency is the highest. To evaluate the frequencies with which such distributions are experienced by an Earth system model over the whole boreal biome, 5 years of UK Earth System Model (UKESM1) simulations are further used. The frequencies are substantially lower than those observed at the boreal forest measurement site (< 6 % of the time), and the positive values, peaking in spring, are modeled only over Fennoscandia and the western parts of Siberia. Overall, the similarities in the size distributions between observed and modeled (UKESM1) are limited, which would limit the ability of this model, or any model with a similar aerosol representation, to project the climate relevance of co-condensation over the boreal forest. For the critical aerosol size distribution regime, ΔCDNC is shown to be sensitive to the concentrations of semi-volatile and some intermediate-volatility organic compounds (SVOCs and IVOCs), especially when the overall particle surface area is low. The magnitudes of ΔCDNC remain less affected by the more volatile vapors such as formic acid and extremely low- and low-volatility organic compounds (ELVOCs and LVOCs). The reasons for this are that most volatile organic vapors condense inefficiently due to their high volatility below the cloud base, and the concentrations of LVOCs and ELVOCs are too low to gain significant concentrations of soluble mass to reduce the critical supersaturations enough for droplet activation to occur. A reduction in the critical supersaturation caused by organic condensation emerges as the main driver of the modeled ΔCDNC. The results highlight the potential significance of co-condensation in pristine boreal environments close to sources of fresh ultrafine particles. For accurate predictions of co-condensation effects on CDNC, also in larger-scale models, an accurate representation of the aerosol size distribution is critical. Further studies targeted at finding observational evidence and constraints for co-condensation in the field are encouraged.

54 ENVIRONMENTAL SCIENCES↗

High sensitivity of simulated fog properties to parameterized aerosol activation in case studies from ParisFog

Aerosols influence fog properties such as visibility and lifetime by affecting fog droplet number concentrations (N d ). Numerical weather prediction (NWP) models often represent aerosol–fog interactions using highly simplified approaches. Incorporating prognostic size-resolved aerosol microphysics from climate models could allow them to simulate N d and aerosol–fog interactions without incurring excessive computational expense. However, microphysics code designed for coarse spatial resolution may struggle with sub-kilometer-scale grid spacings. Here, we test the ability of the UK Met Office Unified Model to simulate aerosol and fog properties during case studies from the ParisFog field campaign in 2011. We examine the sensitivity of fog properties to variations in N d caused by modifications to simulated aerosol activation. Our model, with a 500 m horizontal resolution and interactive aerosol and cloud microphysics, significantly underpredicts N d , although it only slightly underestimates the cloud condensation nuclei concentration. With an updated version of the Abdul-Razzak and Ghan (2000) activation scheme, we produce N d that are more consistent with those predicted by a cloud parcel model under fog-like conditions. We activate droplets only by adiabatic cooling. We incorporate more realistic hygroscopicities for sulfate and organic aerosols and explore the sensitivity of simulated N d to unresolved updrafts. We find that both N d and simulated fog liquid water content are very sensitive to the updated activation scheme but remain less affected by the update to hygroscopicities. Our improvements offer insights into the physical processes regulating N d in stable conditions, potentially laying foundations for improved operational fog forecasts that incorporate interactive aerosol simulations or aerosol climatologies.

Ghosh, Pratapaditya [Carnegie Mellon University, P↗

Adiabatic and radiative cooling are both important causes of aerosol activation in simulated fog events in Europe

Aerosol–fog interactions affect the visibility in, and life cycle of, fog and are difficult to represent in weather and climate models. Here we explore processes that impact the simulation of fog droplet number concentrations (N d ) at sub-kilometer scale horizontal grid resolutions in the UK Met Office Unified Model. We modify the parameterization of aerosol activation to include droplet activation by radiative cooling in addition to adiabatic cooling and determine the relative importance of the two cooling mechanisms. We further test the sensitivity of simulated N d to: (a) interception of droplets by trees and buildings, (b) overestimation of updrafts in temperature inversions (which leads to artificially high N d values), and (c) potential mechanisms for droplet deactivation due to downward fluctuations in supersaturation. We evaluate our model against observations from the ParisFog and LANFEX field campaigns, building on evaluation described in the companion paper. Including radiative cooling in the activation mechanism improves how accurately we represent the liquid water path and the vertical structure of the fog in our LANFEX case study. However, with radiative cooling, the N d are overestimated for most of the ParisFog cases and for the LANFEX case. The time-averaged overestimate exceeds a factor of three (the normalized mean bias factor exceeds 2.0) in 4 out of 11 ParisFog cases. Our sensitivity studies demonstrate how these overestimates can be mitigated. Assuming the overestimate affects both radiative and adiabatic cooling, we find that although radiative cooling is more often the dominant source, both cooling sources can sometimes dominate activation.

Ghosh, Pratapaditya [Carnegie Mellon University, P↗

Identifying synoptic controls on boundary layer thermodynamic and cloud properties in a regional forecast model

Although most of our understanding of boundary layer cloudiness is based on idealized, subtropical, barotropic marine environments, boundary layer clouds exist across a range of conditions. In this study, we use the Naval Research Laboratory's Coupled Ocean/Atmosphere Mesoscale Prediction System (COAMPS) and an automated cold-front-relative analysis framework to explore the boundary layer structure associated with low clouds across a transect through the cold front of a midlatitude synoptic cyclone. The model credibly captures boundary layer structure in line with conceptual models of midlatitude cyclones and ground-based observations at Graciosa Island in the Azores. The warm sector is conditionally unstable, with clouds that are too shallow and with too little liquid water, compared to cloud property retrievals from satellite and surface-based instruments. The cold-frontal region exhibits convection associated with weak stability and ascent. Northwest of the cold front, the boundary layer is well mixed, deeper, and capped by a strong inversion maintained by large-scale subsidence. Simulated clouds in frontal and post-frontal regions are mostly too thick, with too much liquid water and too little cloud base drizzle. The post-frontal clouds are associated with grid-scale updrafts, which appear to be the model's attempt to represent mesoscale organization of cellular convection typically observed in the cold sector of midlatitude cyclones. The deep, well-mixed post-frontal boundary layers and cloudiness are maintained by strong surface fluxes, as in cold air outbreaks. Our analysis framework serves as a unique approach to model verification, and our results offer insights into differences in boundary layer cloud behavior between subtropical and synoptic cold-sector regimes.

Eissner, Jordan M. [Univ. of Kansas, Lawrence, KS ↗

Aerosol impacts on isolated deep convection: findings from TRACER

This study focuses on quantifying the conditional relationship between aerosol and convective precipitation properties of isolated deep convective clouds (DCCs) in the Houston–Galveston region, after adjusting for confounding effects. We leverage comprehensive ground-based observations from the TRacking Aerosol Convection interactions ExpeRiment (TRACER) to estimate aerosol effects on convective echo top height (ETH), intensity, and area separately. Our results show that greater aerosol number concentrations generally have a limited impact on these convective properties, showing relationships consistent with the possibility of both invigoration and suppression effects. Under certain conditions, where ultrafine particles are abundant, aerosols exhibit a positive effect on ETH, increasing it by about 1 km. However, it is inevitable to consider measurement uncertainties and the limitations of temporal and spatial resolution in the data, as these factors can further contribute to uncertainties in our estimates. In DCCs associated with sea breezes, the estimated aerosol effects on DCCs are found to be more pronounced. However, this heightened effect could be attributed to the exclusion of key confounders such as boundary layer updrafts in the analysis.

54 ENVIRONMENTAL SCIENCES↗

Aerosol-deep convection interaction based on joint cell-thermal tracking in Large Eddy Simulations during the TRACER campaign

In cumulus clouds, aerosol concentrations control cloud droplet concentrations, modifying cloud radiative properties, precipitation processes, and cloud electrification. However, mechanisms of aerosol-deep convection interactions are not well understood due to complex cloud dynamics and microphysics. We investigate the interaction of aerosols with isolated deep convection using Large Eddy Simulations of two cases during the TRacking Aerosol Convection interactions ExpeRiment (TRACER) near Houston, Texas, using a joint cell-thermal tracking algorithm. Cumulus thermals are droplet generators, since supersaturation and droplet nucleation coincide with thermal centers, where the strongest updrafts occur. Primary ice crystal formation does not take place inside thermals, but at layers where previous thermals detrained moisture. As subsequent thermals containing supercooled droplets penetrate these layers, hail and graupel form at or near these thermals. Higher aerosol concentrations result in higher droplet concentrations that suppress drizzle, delay warm rain processes, and transport more moisture aloft. This increases snow and ice amount, as well as graupel and hail, leading to more lightning. Polluted thermals initiate at slightly higher altitudes, and are slightly larger and faster, suggesting a weak invigoration. We also find more thermals per cell, but fewer isolated cells, since convection is more aggregated and intense, especially near the end of the 24 h simulation. Non-linear mesoscale feedback likely triggered by temperature and moisture responses to aerosol-thermal interactions causes the aggregation. Time-lagged aerosol-reinitialization experiments show that the mesoscale response is the predominant forcing for the invigoration. These changes happen within one day, on a smaller scale than previously suggested.

54 ENVIRONMENTAL SCIENCES↗

An analysis of the Venus measurements

Plots of the Mariner 5 and Venera 4, 5, and 6 pressure vs temperature show that the Venera profiles are essentially congruent with the Mariner 5 day and night profiles, but are displaced 28 percent higher in pressure. Data suggest a variability in the atmospheric water vapor content in the region from 30 to 50 km. The Venera 7 measurements are interpreted as evidence for updrafts, down-drafts, horizontal wind layers, and nonaqueous precipitation. The previously observed band of retrograde winds which circle the equator with an average speed of 110 m/s is found to extend downward to the one atmosphere level at the equatorial morning terminator. The possibility of a low altitude equator-to-pole circulation with warm gas rising at the poles is inferred. Venera 7 temperature data used with radar topography and microwaves interferometer measurements suggest that the variation of surface temperature with altitude in a band about the equator is less than 5 K/km. The available data are used to calculate a model of the structure of the Venus atmosphere for the first 75 km above the equatorial region.

Ainsworth, J. E.↗

Controlled generation of large volumes of atmospheric clouds in a ground-based environmental chamber

Atmospheric clouds were generated in a 23,000 cubic meter environmental chamber as the first step in a two part study on the effects of contaminants on cloud formation. The generation procedure was modeled on the terrestrial generation mechanism so that naturally occurring microphysics mechanisms were operative in the cloud generation process. Temperature, altitude, liquid water content, and convective updraft velocity could be selected independently over the range of terrestrially realizable clouds. To provide cloud stability, a cotton muslin cylinder 29.3 meters in diameter and 24.2 meters high was erected within the chamber and continuously wetted with water at precisely the same temperature as the cloud. The improved instrumentation which permitted fast, precise, and continual measurements of cloud temperature and liquid water content is described.

Hettel, H. J.↗

Venus wind and temperature structure - The Venera 8 data

Our analysis of the Venera 8 measurements yields equatorial morning terminator horizontal and vertical winds that are similar in a number of respects to the winds we obtained from our analysis of the Venera 7 measurements. The lower boundary of the horizontal retrograde '4-day' wind is defined by a 50-60% decrease in wind speed in the vicinity of 44 km, and there exists a retrograde wind 'plateau' of 15- to 40-m/s winds extending from 40 km down to the vicinity of 18 km, where the winds decrease rapidly to the order of 0.1 m/s near the surface. Updrafts of 2-5 m/s exist in the vicinity of 20-30 km and are apparently associated with a slightly superadiabatic lapse rate.

Ainsworth, J. E.↗

Equivalent blackbody temperature of the top of a severe storm

An RB-57F high-altitude aircraft equipped with Wilde RC-8 cameras and an infrared spectrometer was used in the investigations. A storm was overflown over Graham, Texas, on April 29, 1970. In the experiment, the average radiometric temperature was determined to be very near the environmental temperature near the cloud tops. However, hot and cold regions in and near the updrafts and downdrafts were found to be significantly out of equilibrium. It is recommended that caution should be exercised in determining cloud top altitude from equivalent blackbody temperature.

Pitts, D. E.↗

Tornadoes and other atmospheric vortices

The growth of random vortices in an atmosphere with buoyant instability and vertical wind shear is studied along with the velocities in a single gravity-driven vortex; a frictionless adiabatic model which is supported by laboratory experiments is first considered. The effects of axial drag, heat transfer, and precipitation-induced downdrafts are then calculated. Heat transfer and axial drag tend to have stabilizing effects; they reduce the downdrafts of updrafts due to buoyancy. It is found that downdrafts or tornadic magnitude might occur in negatively-buoyant columns. The radial-inflow velocity required to maintain a given maximum tangential velocity in a tornado is determined by using a turbulent vortex model. Conditions under which radial-inflow velocities become sufficiently large to produce tangential velocities of tornadic magnitude are determined. The radial velocities in the outer regions, as well as the tangential velocities in the inner regions may be large enough to cause damage. The surface boundary layer, which is a region where large radial inflows can occur, is studied, and the thickness of the radial-inflow friction layer is estimated. A tornado model which involves a rotating parent cloud, as well as buoyancy and precipitation effects, is discussed.

Deissler, R. G.↗

Detection of severe storms by satellites

Ideas are presented for severe storm identification based on satellite data. The tops of huge thunderstorms in satellite pictures often appear as vast areas of extensive cirrus cloud; they consist of clusters of anvil clouds, each generated by vigorous thunderstorm circulation. The overshooting tops observed in satellite pictures are located where the subanvil updrafts are the strongest. Learjet experiment results show that an overshooting top varies either quickly or slowly, depending on the characteristics of individual clouds. When an overshooting top collapses, a small segment of the anvil cirrus jumps upward in the wake of the overshooting top. Also discussed is the monitoring of vertical motions from satellites and tornado-producing thunderstorms from geostationary altitude. A very high-resolution imagery of both infrared and visual spectral bands makes it possible to infer vertical motions beneath the anvil top. A combination of cloud velocity and anvil expansion rate will permit, in the future, determining the location of severe storms within the vast areas of anvil clouds.

Fujita, T. T.↗

Cloud-top parameters - A hail indicator

Airborne photographic observations of four hail-producing storms are discussed. With the exception of one storm producing a tornadic event, the overshooting tops were nearly steady-state. The tops were consistently high and wide, reaching maximum heights within about 5 minutes of the initiation of hail. Measured updraft velocities in the turrets composing the overshooting top were 25 m/sec. The dimensions of the overshooting tops were sufficiently large to permit satellite observation.

Pearl, E. W.↗

Clear air convective behavior revealed by radar chaff

A simple experiment is described in which chaff was injected into the updraft region of individual clear-air convective cells in order to clarify characteristics of such convective elements. The chaff was dispensed automatically by a small radio-controlled drone aircraft and also by hand from the ground. It is found that clear-air convective cells are roughly spherical in form, that rapid mixing occurs within a cell, and that little mixing occurs between adjacent cells. Some suggestions are offered for future work in the tracing of air motions arising from the ground.

Rowland, J. R.↗

A theoretical analysis of airplane longitudinal stability and control as affected by wind shear

The longitudinal equations of motion with wind shear terms were used to analyze the stability and motions of a jet transport. A positive wind shear gives a decreasing head wind or changes a head wind into a tail wind. A negative wind shear gives a decreasing tail wind or changes a tail wind into a head wind. It was found that wind shear had very little effect on the short period mode and that negative wind shear, although it affected the phugoid, did not cause stability problems. On the other hand, it was found that positive wind shear can cause the phugoid to become aperiodic and unstable. In this case, a stability boundary for the phugoid was found that is valid for most aircraft at all flight speeds. Calculations of aircraft motions confirmed the results of the stability analysis. It was found that a flight path control automatic pilot and an airspeed control system provide good control in all types of wind shear. Appendixes give equations of motion that include the effects of downdrafts and updrafts and extend the longitudinal equations of motion for shear to six degrees of freedom.

Sherman, W. L.↗

An analysis of maximum vertical gusts recorded at NASA's 150-meter ground winds tower facility at Kennedy Space Center, Florida

A statistical summary is presented of vertical wind speed data recorded at NASA's 150-Meter Ground Winds Tower Facility on Merritt Island, Kennedy Space Center, Florida. One year of continuous around-the-clock vertical wind speed measurements processed by the Automatic Data Acquisition System (ADAS) is classified as a function of tower level (10, 18, 60, and 150 meters) and period of reference day, month, season: winter (October through March) and summer (April through September), and annual. Intensity, frequency, time of occurrence, prevailing conditions, etc., of the daily maximum vertical gusts (i.e., updraft and downdraft) are determined. The results are compared with the vertical gusts associated with the daily maximum horizontal gust. The intent of this summarization of vertical wind speed data is to provide a general description of wind flow in the lower 150 meters of the atmosphere for the identification of hazards involved in wind shear encounters relative to ascent and descent of the Space Shuttle and conventional aircraft.

Alexander, M. B.↗