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Intensity measurements on molecular oxygen Herzberg I system emitting in afterglow of microwave discharge, noting dependence of transition moment on internuclear distance
Electron energy loss in afterglow plasmas, plasma transport and stability and electromagnetic wave propagation through magnetoplasmas
Recombination in helium plasma afterglows, discussing unexplained sudden electron temperature increase at cryogenic temperatures
NonMaxwellian electron velocity distribution in active discharge and afterglow of N plasma determined by microwave radiation temperature measurements
Electron beam fluorescence probe and afterglow investigation for hypersonic He flow visualization, observing qualitative structure
Photoelectric intensity measurements on emission bands of oxygen Herzberg I system excited in argon-oxygen afterglow
Measuring rate constants for reactions of various gas phases with water by flowing afterglow technique
The reaction sequence leading from O2(+) to H3O(+)-H2O was examined in He, Ar, N2 and O2 carrier gases in a flowing afterglow system. The rate constants for the reactions were measured and the kinetic analysis for their determination is presented. For M = N2, two new steps involving the formation and reaction of O2(+)-N2 were proposed and examined. The rate constants are discussed and compared with other experimental values.
Study of the space and time resolved structure of a helium plasma produced with a repetitive CO2 laser during the first 15 microsec of the afterglow period. The spectra of several neutral and ionized helium lines are used in the determination of the density and temperature profiles of the luminous fireball. It is found that the plasma is comprised of a dense hot core, which emits primarily ionic lines, and a well-defined tenuous outer shell, which is primarily the source of neutral emission lines. This ?two-component' plasma structure develops at about 0.4 microsec after breakdown, at about the time when the luminous fireball dissipates its expansion energy and comes to a virtual standstill.
A flowing afterglow has been used to produce metastable He(2 super 3 S). It is shown that when He(2 super 3 S) interacts with a diatomic or triatomic molecule, its electronic excitation energy can be transferred to electronic and vibrational excitation of the molecule. To examine this mechanism, the rates for the production of electronically excited molecules, observed spectroscopically between 190 and 750 nm in the reaction of He(2 super 3 S) with CO2, have been measured. Results are tabulated.
Recombination coefficients of electrons with HCO(+) ions were determined with a microwave afterglow/mass spectrometer apparatus. Afterglow measurements of electron density decays in neon-hydrogen-carbon monoxide mixtures are correlated with the decay of mass-identified ion currents to the wall of the microwave cavity. At the appropriate partial pressures of hydrogen and carbon monoxide in the mixture, the ion HCO(+) dominates the ion composition and its wall current approximately tracks the electron density decay curve. From recombination controlled electron density decay curves, the values alpha (HCO(+)) = (3.3 + or - 0.5) and (2.0 + or - 0.3) 0.0000001 cu cm/sec are obtained at 205 and 300 K, respectively. The implications of these results for models of polyatomic molecule formation in dense interstellar clouds are briefly discussed.
The fourth positive system of CO has been excited in a static afterglow experiment by the dissociative recombination of CO2(+) ions. From combined absolute optical and microwave measurements the specific recombination coefficient for exciting the CO system was found to be (2 plus 1 or minus 0.5) x 10 to the minus 8th cu cm/sec. This value represents approximately 5% of the total recombination coefficient (4.0 plus or minus 0.5) x 10 to the minus 7th cu cm/sec measured in this experiment, implying that CO2(+) dissociative recombination will contribute significantly to the excitation of the CO fourth positive system in the Martian airglow. Corroborative electron heating experiments showed that the magnitude of the specific recombination coefficient decreased as the electron temperature was increased. Evidence was also found for the presence of vibrationally excited ions in the CO2(+) plasma, a result which indicates that analogous laboratory studies on the dissociative recombination of O2(+), N2(+), and NO(+) ions may have also involved vibrationally hot plasmas.
Experimental and theoretical aspects of the mobility and diffusion of ions in gases are studied in detail. Some of the subjects discussed include ion-ion interaction, boundary condition and ion and electron behavior. Also discussed in separate chapters are the problems of the diffusion coefficients and the afterglow techniques. Finally, a special chapter studies the kinetic theory of diffusion and mobility, stressing the low-, medium- and high-field theory.
The antenna studies were performed in a large magnetized plasma source, a schematic drawing of which is shown. The plasma diagnostics consist of a 70 GHz (4 mm) microwave interferometer for density measurements and of various Langmuir probes for spatially resolved measurements of t sub e, n sub e and the shape of the electron distribution function. All diagnostic data are time-resolved by sample-and-hold techniques so as to yield information about the plasma build-up, the steady-state discharge, and the plasma decay in the afterglow. Whistler waves are excited and detected with various antennas which are inserted into the center of the plasma column through one axial and two orthogonal radial ports. The antennas were tested for their proper dipole response and then calibrated in a known field geometry in air. For the electric dipole, a parallel plate capacitor field was used; the magnetic loop is calibrated in the near-zone field of a long linear conductor of known radio frequency current distribution. Results are presented and discussed.
From the Ogo 6 horizon-scanning-photometer data a useful upper limit can be set to the radiance of nightglow in the O-NO afterglow continuum above 105 km. The upper limit is a factor of about 5 less than the product of observed NO densities and Jacchia (1971) O model densities.
Report contains evaluations of flammability and physical properties of twenty-four upholstery and furnishing materials, such as those used in commercial aircraft. Data presented include degradation upon heating, limited oxygen indices, smoke generation, flammability afterglow, and char length.
Experiments performed in a pulsed afterglow plasma column with specified parameters revealed a filamentation instability of a large-amplitude whistler wave launched from antennas which produce a diverging energy flow in the linear regime. The difficult problem of diagnosing local density perturbations in a magnetized plasma in the presence of large-amplitude RF signals and nonuniform anisotropic electron distributions is discussed. Since Langmuir probes are too unreliable under these conditions, a microwave probe is developed based on the principle of the cavity shift method. The temporal and spatial evolution of the duct formation and wave propagation are shown. The role of the observed electron heating in the filamentation process is examined. The observed self-focusing process appears to be the result of the reinforcing interaction between the wave-induced density depression and the density-induced wave refraction. Interesting applications are noted.
The first direct nuclear pumped laser using the He-2-(n,p) H-3 reaction is reported. Lasing took place on the 1.79 microns Ar I transition in a mixture of He-3-Ar at approximately 600 Torr total pressure. It was found that the electrically pulsed afterglow He-Ar laser had the same concentration profile as the nuclear pumped laser. As a result, nuclear lasing was also achieved in He-3-Xe (2.027 micron) and He-3-Kr (2.52 micron). Scaling of laser output with both thermal flux and total pressure as well as minority concentration has been completed. A peak output (He-3-Ar) of 3.7 watts has been achieved at a total pressure of 4 atm. Direct nuclear pumping of He-3-Ne has also been achieved. Nuclear pumping of a He-3-NF3 mixture was attempted, lasing in FI at approximately 7000 A, without success, although the potential lasing transitions appeared in spontaneous emission. Both NF3 and 238UF6 appear to quench spontaneous emission when they constitute more than 1% of the gas mixture.