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DOE OSTI2024

CROCUS High-Frequency Measurements of CO₂, H₂O, Wind, and Temperature at University of Illinois Chicago

As of April 9, 2026: this dataset is currently being versioned to include data up to March 31, 2026. Once the versioning process is complete, new data files will be available for access. The dataset metadata will also be updated to reflect the data availability of the new data being versioned. Raw atmospheric measurements collected at the University of Illinois Chicago (UIC) as part of the Community Research on Climate and Urban Science (CROCUS) project. The data includes high-frequency measurements of carbon dioxide (CO₂) concentration, water vapor (H₂O) concentration, wind speed (U, V, W components), temperature, and atmospheric pressure. These raw data are recorded by the LI-7500DS Open Path CO₂/H₂O Analyzer and a sonic anemometer at a 10 Hz acquisition frequency, providing the necessary inputs for calculating fluxes of CO₂, H₂O, heat, and momentum. In addition to gas concentration measurements, the dataset includes diagnostic information from the instruments, including absorptance, sample and reference signals, and diagnostic values. The data were collected to study urban atmospheric conditions and contribute to flux calculations for urban climate research. These measurements form the basis for calculating 30-minute average fluxes of key atmospheric variables using the eddy covariance method. This dataset provides critical raw input data for researchers interested in atmospheric fluxes, urban air quality, and the interaction between the urban environment and atmospheric processes. The data is part of the U.S. Department of Energy’s Biological and Environmental Research (BER) program, under the CROCUS Urban Integrated Field Laboratory (UIFL) project.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2025

Modeling Protocol for Evaluation of Air Emissions for the Idaho National Laboratory Site-wide Permit to Construct and Facility Emission Cap (PTC/FEC)

This document outlines the methods to be used for calculating non-radiological air quality impacts from proposed emissions at the Idaho National Laboratory (INL) Site in support of applying for a renewal to a Permit to Construct with a Facility Emissions Cap (PTC/FEC). The INL Site is seeking to maintain a state enforceable limit on emissions to maintain synthetic minor status in accordance with Idaho Administrative Procedures Act (IDAPA) 58.01.01.175-181 and IDAPA 58.01.01.200-228.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2025

New Particle Formation and Growth in the Houston Atmosphere During TRACER (Final Report)

From 2020-2025, researchers from UC Irvine, UC Riverside, and Colorado State University collaborated on a Department of Energy-funded project to understand how airborne particles form and grow in urban atmospheres, conducting an intensive field campaign in Houston, Texas during summer 2022. Using advanced instruments to measure gas-phase chemicals, particle composition, and a specialized chamber to study particle growth, the team discovered that sulfur-containing compounds from industrial and power plant emissions are the dominant driver of new particle formation in Houston, with particles typically forming locally in the city and growing as air moves away in the urban plume. The research revealed an important methodological insight: measurements from fixed ground stations can be misleading when interpreting how particles actually evolve as air masses move, which has significant implications for how scientists worldwide interpret atmospheric observations. These findings improve understanding of urban air quality and help reduce uncertainties in climate models, since these particles play critical roles in cloud formation and Earth's radiation balance, while also providing detailed information about ultrafine particle composition relevant to public health. The project trained three doctoral students, developed enhanced computer models for urban particle formation, and made all data publicly available through the DOE Atmospheric Radiation Measurement data archive for use by the broader scientific community.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Development of Advanced Smart Ventilation Controls for Residential Applications

This study examined the use of zoned ventilation systems using a coupled CONTAM/EnergyPlus model for new California dwellings. Several smart control strategies were developed with a target of halving ventilation-related energy use, largely through reducing dwelling ventilation rates based on zone occupancy. The controls were evaluated based on the annual energy consumption relative to continuously operating non-zoned, code-compliant mechanical ventilation systems. The systems were also evaluated from an indoor air quality perspective using the equivalency approach, where the annual personal concentration of a contaminant for a control strategy is compared to the personal concentration that would have occurred using a continuously operating, non-zoned system. Individual occupant personal concentrations were calculated for the following contaminants of concern: moisture, CO2, particles, and a generic contaminant. Zonal controls that saved energy by reducing outside airflow achieved typical reductions in ventilation-related energy of 10% to 30%, compared to the 7% savings from the unzoned control. However, this was at the expense of increased personal concentrations for some contaminants in most cases. In addition, care is required in the design and evaluation of zonal controls, because control strategies may reduce exposure to some contaminants, while increasing exposure to others.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

DOE OSTI2020

Ultra-Low SWaP CO 2 Sensing for Demand Control Ventilation (Final Report)

In this project PARC and Energy ETC aimed to develop an ultra-low cost, size, weight, and power (SWaP) printed CO 2 sensor system for occupancy detection to enable Demand Control Ventilation (DCV) on a per-room basis. The CO 2 sensor technology is based on the temperature variation when CO 2 reversibly physisorbs to a highly conductive and high surface area sorbent surface, and is compatible with integration with PARC innovations in printed sensors and flexible electronics, for which PARC is a globally leading research center. The printed CO 2 sensor itself is designed to be compatible with PARC’s “peel-and-stick” platform of ultra-low power, low-cost, distributed sensors, and to facilitate real-time DCV based on overall indoor air quality (IAQ). Previously, PARC has developed flexible hybrid electronics (FHE) compatible materials to measure humidity, temperature, light, strain, and gases such as carbon monoxide, methane, ammonia, and hydrogen sulfide. Through this project, PARC developed FHE-compatible materials to measure CO 2 . Thus, with one <$15 FHE “peel-and-stick” based sensor node, a building management system (BMS) will be able to capture a complete picture of the indoor environment. This includes IAQ, light, temperature, and other comfort factors that impact building operations. Combined with optimized DCV, this low-cost sensor capability can be a key enabler of annual primary energy savings of ~ 0.3-0.4 Quad in commercial buildings while ensuring healthy IAQ. Energy ETC is a leader in supplier-agnostic BMS deployments and will design the commissioning and deployment procedures to maximize system interoperability.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

DOE OSTI2024

Characterizing Overwater High Ozone Events in the Houston–Galveston–Brazoria Region during the 2021 GO3 and TRACER-AQ Campaigns

Photochemical modeling outputs showing high ozone concentrations over the Gulf of Mexico and Galveston Bay during ozone episodes in the Houston–Galveston–Brazoria (HGB) region have not been previously verified using in situ observations. Such data were collected systematically, for the first time, from July to October 2021 from three boats deployed for the Galveston Offshore Ozone Observations (GO3) and Tracking Aerosol Convection Interactions Experiment—Air Quality (TRACER-AQ) field campaigns. A pontoon boat and a commercial vessel operated in Galveston Bay, while another commercial vessel operated in the Gulf of Mexico offshore of Galveston. All three boats had continuously operating sampling systems that included ozone analyzers and weather stations, and the two boats operating in Galveston Bay had a ceilometer. The sampling systems operated autonomously on the two commercial boats as they traveled their daily routes. Thirty-seven ozonesondes were launched over water on forecast high ozone days in Galveston Bay and the Gulf of Mexico. During the campaigns, multiple periods of ozone exceeding 100 ppbv were observed over water in Galveston Bay and the Gulf of Mexico. These events included previously identified conditions for high ozone events in the HGB region, such as the bay/sea-breeze recirculation and postfrontal environments, as well as a localized coastal high ozone event after the passing of a tropical system (Hurricane Nicholas) that was not well forecast.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2020

Understanding the Applicability of Gas/Particle Partitioning Theory to SOA using Novel Chemically-Speciated Partitioning Measurements (Final Report)

The main objective of this research grant project was to investigate the physical-chemical processes and properties of particles and partitioning gases that influence gas/particle (G/P) partitioning and timescales for equilibration, to directly determine the conditions under which equilibrium G/P partitioning theory can be applied to secondary organic aerosol (SOA). SOA constitutes a major component of submicron particles in the atmosphere, which have important implications for air quality, human and ecosystem health, radiation balance, and climate; however SOA formation, evolution and losses are not well understood. Use of novel on-line measurements of chemically-speciated partitioning measurements of both gas-phase and particle-phase components was a central component to advancing these scientific goals. The key approach was to conduct environmental chamber studies with systems of increasing complexity to determine G/P partitioning rates and equilibrium states for chemically-speciated SOA components. The project builds on our previous work on gas-wall partitioning that must be understood in order to study G/P partitioning in chambers, and to help extrapolate the results to be atmospherically relevant. The goal was to employ measurements and modeling to systematically determine when G/P partitioning theory accurately describes the distribution of oxidized organic compounds in the gas and aerosol phases, and when and why it does not (e.g., aerosol phase-state kinetic limitations, non-ideal mixing, phase separation, oligomer formation,), for chemical and physical conditions typically found throughout the continental boundary layer.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2023

Implementing and Improving CBMZ-MAM3 Chemistry and Aerosol Modules in the Regional Climate Model WRF-CAM5: An Evaluation over the Western US and Eastern North Pacific

The representation of aerosols in climate-chemistry models is important for air quality and climate change research, but it can require significant computational resources. The objective of this study was to improve the representation of aerosols in climate–chemistry models, specifically in the carbon bond mechanism, version Z (CBMZ), and modal aerosol modules with three lognormal modes (MAM3) in the WRF-CAM5 model. The study aimed to enhance the model’s chemistry capabilities by incorporating biomass burning emissions, establishing a conversion mechanism between volatile organic compounds (VOCs) and secondary organic carbons (SOCs), and evaluating its performance against observational benchmarks. The results of the study demonstrated the effectiveness of the enhanced chemistry capabilities in the WRF-CAM5 model. Six simulations were conducted over the western U.S. and northeastern Pacific region, comparing the model’s performance with observational benchmarks such as reanalysis, ground-based, and satellite data. The findings revealed a significant reduction in root-mean-square errors (RMSE) for surface concentrations of black carbon (BC) and organic carbon (OC). Specifically, the model exhibited a 31% reduction in RMSE for BC concentrations and a 58% reduction in RMSE for OC concentrations. These outcomes underscored the importance of accurate aerosol representation in climate-chemistry models and emphasized the potential for improving simulation accuracy and reducing errors through the incorporation of enhanced chemistry modules in such models.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Effective Kitchen Ventilation for Healthy Zero Net Energy Homes with Natural Gas

Past studies indicate that kitchen ventilation that minimally complies with California’s Residential Building Code is inadequate at controlling combustion pollutants from natural gas burners and particulate matter produced during cooking. Effectiveness is further limited by misperceptions that kitchen ventilation is infrequently needed. This project developed the technical basis for updating kitchen ventilation requirements to protect health in new California homes, especially in smaller homes common among low-income renters. Tasks included (1) a field study of ventilation equipment performance and indoor air quality in 23 low-income apartments at four sites; (2) analysis of range hood use related to cooking time and household parameters using data from 54 houses and 17 low-income apartments; (3)a measurement-based study to quantify performance of over-the-range microwave ovens with integrated exhaust fans;and (4) pollutant exposure simulations to inform capture efficiency standards.The field study found operational deficiencies with mechanical ventilation systems in a substantial fraction of low-income apartments that affected performance, resulting in higher exposures to pollutants generated indoors. Using gas cooking burners produced high short-term and weekly time-averaged nitrogen dioxide in apartments.Range hoods were used more frequently with cooking in houses (36percent) than apartments (28percent); use increased with overall cooking frequency in a home and with duration of cooktop but not oven events; actual use was correlated to, but lower than,self-reported use;and use was more frequent in houses when cooking generated any fine particulate matter (PM2.5)or when high PM2.5resulted from cooking in apartments. Performance of over-the-range microwaves with integrated exhaust fans was similar to that of range hoods of comparable price. Simulation analysis found that performance standards need to be updated to ensure that kitchen exhaust ventilation adequately protects for substantial cooking in new California residences.

03 NATURAL GAS↗

DOE OSTI2025

A formaldehyde and nitrogen dioxide toxics monitor for environmental justice

DOE’s Integrated Field Laboratories (IFLs) require a vast array of measurements to measure urban air quality. Nitrogen dioxide (NO2) and formaldehyde (HCHO) are ubiquitous pollutants with numerous sources, most notably vehicle exhaust. High-spatial density measurements are critical to understanding how certain neighborhoods are more adversely impacted by pollutants. This report describes the results of a Phase I SBIR project to develop and demonstrate a rapid, affordable, low-power monitor to provide high spatial resolution mobile measurements of formaldehyde and nitrogen dioxide at street-level, where people live and walk. The spatial density will be achieved via rapid measurements on a mobile platform. This sensor will quantify spatial disparities in cities of the toxics, HCHO and NO2, as well as carbon monoxide and carbon dioxide for better source identification. These species are detected in the mid infrared by laser absorption spectroscopy, and fiberoptics are used. Tasks accomplished include identification and testing of the appropriate spectroscopic regions; coupling of laser light into a fiberoptic system; development of software to control miniature electronics to scan and control two lasers simultaneously; coupling of the mid infrared fiber into a multipass cell for enhanced pathlength and sensitivity; characterization of sources of instrument noise; and design work for a Phase II prototype.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2025

CROCUS Dual Polarization Ceilometer Data at Northeastern Illinois University Rooftop

This dataset is from the Department of Energy Office of Science funded project, CROCUS Urban Integrated Field Laboratory (https://crocus-urban.org/). The dual-polarization ceilometer (Vaisala CL61) is an autonomous lidar system operating at 910 nm wavelength, providing valuable measurements for understanding atmospheric boundary layer evolution, air quality, and cloud-aerosol interactions. The CL61 measures the backscattered signal intensity alternating between parallel- and cross-polarization signals. The unique depolarization measurement capability improves discrimination between different particle types, such as liquid droplets, ice crystals, and aerosols. The depolarization is highly dependent on the scatterer shape and orientation (spherical vs non-spherical particles), with the linear depolarization ratio providing a measure of dominant backscatter signal component from atmospheric particles at various heights, essentially allowing discrimination between liquid and solid particles. With its efficient optical system, CL61’s improved signal-to-noise ratio compared to traditional ceilometers allows studying detailed vertical profiles of aerosols and clouds up to 15 km height.Datasets are stored in a netCDF data format, and we we encourage users to make use of the associated toolkits available from Unidata (https://www.unidata.ucar.edu/software/netcdf/), Project Pythia (https://foundations.projectpythia.org/core/data-formats/netcdf-cf.html), and our “Instrument Cookbooks” (https://crocus-urban.github.io/instrument-cookbooks) for more information on how to process the metadata-rich datasets.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2022

Impact of acute temperature and air pollution exposures on adult lung function: A panel study of asthmatics

Background Individuals with respiratory conditions, such as asthma, are particularly susceptible to adverse health effects associated with higher levels of ambient air pollution and temperature. This study evaluates whether hourly levels of fine particulate matter (PM 2.5 ) and dry bulb globe temperature (DBGT) are associated with the lung function of adult participants with asthma. Methods and findings Global positioning system (GPS) location, respiratory function (measured as forced expiratory volume at 1 second (FEV 1 )), and self-reports of asthma medication usage and symptoms were collected as part of the Exposure, Location, and Lung Function (ELF) study. Hourly ambient PM 2.5 and DBGT exposures were estimated by integrating air quality and temperature public records with time-activity patterns using GPS coordinates for each participant (n = 35). The relationships between acute PM 2.5 , DBGT, rescue bronchodilator use, and lung function collected in one week periods and over two seasons (summer/winter) were analyzed by multivariate regression, using different exposure time frames. In separate models, increasing levels in PM 2.5 , but not DBGT, were associated with rescue bronchodilator use. Conversely DBGT, but not PM 2.5 , had a significant association with FEV 1 . When DBGT and PM 2.5 exposures were placed in the same model, the strongest association between cumulative PM 2.5 exposures and the use of rescue bronchodilator was identified at the 0–24 hours (OR = 1.030; 95% CI = 1.012–1.049; p-value = 0.001) and 0–48 hours (OR = 1.030; 95% CI = 1.013–1.057; p-value = 0.001) prior to lung function measure. Conversely, DBGT exposure at 0 hours (β = 3.257; SE = 0.879; p-value>0.001) and 0–6 hours (β = 2.885; SE = 0.903; p-value = 0.001) hours before a reading were associated with FEV 1 . No significant interactions between DBGT and PM 2.5 were observed for rescue bronchodilator use or FEV 1 . Conclusions Short-term increases in PM 2.5 were associated with increased rescue bronchodilator use, while DBGT was associated with higher lung function (i.e. FEV 1 ). Further studies are needed to continue to elucidate the mechanisms of acute exposure to PM 2.5 and DBGT on lung function in asthmatics.

60 APPLIED LIFE SCIENCES↗

DOE OSTI2024

Aircraft Measurements from a U.S. Western Wildfire Demonstrating Day and Night Differences in the Chemical Composition and Optical Properties of Biomass Burning Aerosols and Their Atmospheric Evolution

The composition and transformations of biomass burning aerosols (BBA) have been measured onboard the NOAA Twin Otter research aircraft during the Fire Influence on Regional to Global Environments and Air Quality field study. Here, we analyze real-time aerosol mass spectrometry measurements across three flights during the afternoon, late afternoon, and night of August 28, 2019, for one midsized wildfire. Analysis of several metrics showed that the aerosol composition and optical properties varied depending on the burning conditions at the fire zone and the time of day the BBA was emitted, with substantial variations in the available sunlight. The total aerosol mass loadings were dominated by organic components with a much smaller contribution from inorganic species. A gradual buildup of organic material was observed during the afternoon as the plume aged, indicating the condensation of photochemically formed low-volatility oxidized organic compounds. Highly hygroscopic ammonium nitrate was the main inorganic component, suggesting potential water content in BBA particles and the likelihood of their aqueous-phase reactivity. Depletions of particle-phase NO 3 – and Cl – relative to carbon monoxide were observed in the late afternoon and nighttime plumes, respectively, aligning with known gas-particle partitioning thermodynamics and the heterogeneous chemistry of dissolved nitrate and chloride. The wavelength-dependent light absorption by aerosol species was higher for the plume sampled at night and showed no significant changes with plume age, despite observed trends in composition and mass downwind. These differences in particle composition and optical properties demonstrate that the processes involved in BBA aging are not uniform for the same wildfire over the course of the day and depend highly on when the BBA was emitted, as well as the burning phase at the emissions source.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2025

A Year-Round Energy-Efficient Fresh Air Handling System with Two-Stage Heat Pumps and Lake Water Pre-Treatment

Supplying fresh air is important for indoor air quality, but the energy consumption to treat fresh air is significant. The main problems in existing fresh air system include: supplying single-temperature water to treat fresh air and not applying natural energy sufficiently restrict the efficiency improvement of cooling and heat sources; unused air handling devices under most operating conditions throughout the year increase the fan energy consumption. Thus, this study proposes an efficient fresh air system that uses lake water to pre-treat fresh air and two-stage heat pumps for further treatment, and the unused air handling devices in the system are bypassed. A fresh air system in northern China is selected as a case to show the annual energy performance of the proposed system, and a comparative analysis is conducted between the proposed system and a traditional system. The results show that the annual energy-savings of the proposed system compared to the traditional system come from fans, and compressors, which are 56.5%, and 31.1%, respectively, with an entire system energy saving of 32.2%. The proposed system can achieve an annual system coefficient of performance (COP) of 5.5. This study provides potential for further improving the energy efficiency in fresh air treatment.

Liang, Chenjiyu↗

DOE OSTI2021

Research and Development of a Ventilation-Integrated Comfort System

From an indoor air quality perspective, the best residential ventilation strategies include filtering outdoor air and distributing that air to all occupied parts of a home. From an energy standpoint, it is desirable that energy be transferred from the exhaust air to the incoming outdoor air to limit heating and cooling impacts. Heat or energy recovery ventilators (HRVs or ERVs) can provide these functions, but researchers have seen many poor installations related to design, installation, and operation and maintenance. More robust ventilation systems may involve an ERV with a dedicated duct distribution system and controls. Such a duct system can be costly to install, and many builders reduce these costs by connecting an ERV to a central heating and cooling duct system. Although this can sometimes be done effectively, researchers have seen consistent challenges with low, inconsistent, or imbalanced flow rates; high electricity consumption; and—of greatest concern—outdoor air short-circuiting or not being delivered to occupied spaces at all. Most ERVs are designed to operate with their own duct system; they are not designed as an add-on to much larger heating, ventilating, and air-conditioning (HVAC) systems. The ventilation-integrated comfort system (VICS) is expressly designed to integrate with low-capacity, efficient, ducted heating and cooling systems. Overall, the latest VICS prototype consumed 40–75 watts (W), including the air handler power, to deliver 50–120 cfm of whole-dwelling ventilation. The large, cross-flow ERV core performed to match manufacturer values (73% winter sensible effectiveness, 64% summer total effectiveness), but further improvements are possible. The VICS system researched and tested during this project will provide efficient, controllable, balanced energy recovery ventilation that is integrated with heating and cooling systems. The integration reduces space and ductwork needed for separate ventilation systems, and there are no compromises to heating, cooling, or ventilation performance. The integrated nature of the device also reduces risks for improper installation and commissioning. Even when using the air handler blower to distribute outdoor air, the total power consumption is lower than that of most available ERV products in the same airflow range. This system has the potential to offer very high-performance ventilation with much smoother and simpler installation than conventional systems.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

DOE OSTI2021

Research and Development of a Ventilation-Integrated Comfort System

29 ENERGY PLANNING, POLICY, AND ECONOMY↗

DOE OSTI2020

Environmental, Health and Safety Assessment Application of a Heat Integrated, Post-combustion CO2 Capture System Using Monoethanolamine and Hitachi H3-1 Solvent at the E.W. Brown Coal-fired Power Plant

An Environmental Health and Safety (EH&S) Assessment was completed for operation of a pilot scale carbon dioxide (CO2) capture system (CCS) at the Louisville Gas & Electric (LG&E) and Kentucky Utilities (KU) Energy, LLC (LG&E-KU) E. W. Brown Generating Station in Harrodsburg, Mercer County, Kentucky. The pilot system was evaluated using two CO2 capture solvents, monoethanolamine (MEA) and Hitachi’s H3-1 solvent. The purpose of the EH&S Assessment was to determine if there were any unacceptable environmental, health or safety concerns that may prevent operation or environmental permitting of a larger scale pilot scale plant. The assessment included review of process flow diagrams, input and output flow rates for primary materials, literature describing similar processes and chemicals used or created during the process, actual air emission and wastewater test data and air emission calculations. The evaluation included identification of risks related to hazardous chemicals, air emissions, wastewater discharges, solid wastes generated and employee hazards. Most potential EH&S issues that were identified are commonly found and successfully managed at large industrial facilities. No risks were identified that could not be successfully managed or would likely prevent implementation or environmental permitting of the pilot or larger scale plant. Potential exposures and resulting health risks from exposure to low concentrations of nitrosamines generated from degradation of the Hitachi H3-1 and possibly MEA solvents may be a health concern for site workers, but additional investigation is needed to accurately assess this risk. Applying the information gained from operating the pilot plant, performing air emission testing and used solvent testing to a large-scale facility at a commercial coal-fired electric generating plant suggests additional air emission control measures may be necessary to reduce potential site worker health risks and possibly community risks. Depending upon the location and regional air quality, considerable effort may be required to obtain the necessary air permit for construction and operation of a similarly configured large-scale PCCCS facility.

gas separation↗

DOE OSTI2020

Environmental, Health and Safety Assessment Application of a Heat Integrated, Post-combustion CO 2 Capture System Using Monoethanolamine and Hitachi H3-1 Solvent at the E.W. Brown Coal-Fired Power Plant

An Environmental Health and Safety (EH&S) Assessment was completed for operation of a pilot scale carbon dioxide (CO 2 ) capture system (CCS) at the Louisville Gas & Electric (LG&E) and Kentucky Utilities (KU) Energy, LLC (LG&E-KU) E. W. Brown Generating Station in Harrodsburg, Mercer County, Kentucky. The pilot system was evaluated using two CO 2 capture solvents, monoethanolamine (MEA) and Hitachi’s H3-1 solvent. The purpose of the EH&S Assessment was to determine if there were any unacceptable environmental, health or safety concerns that may prevent operation or environmental permitting of a larger scale pilot scale plant. The assessment included review of process flow diagrams, input and output flow rates for primary materials, literature describing similar processes and chemicals used or created during the process, actual air emission and wastewater test data and air emission calculations. The evaluation included identification of risks related to hazardous chemicals, air emissions, wastewater discharges, solid wastes generated and employee hazards. Most potential EH&S issues that were identified are commonly found and successfully managed at large industrial facilities. No risks were identified that could not be successfully managed or would likely prevent implementation or environmental permitting of the pilot or larger scale plant. Potential exposures and resulting health risks from exposure to low concentrations of nitrosamines generated from degradation of the Hitachi H3-1 and possibly MEA solvents may be a health concern for site workers, but additional investigation is needed to accurately assess this risk. Applying the information gained from operating the pilot plant, performing air emission testing and used solvent testing to a large-scale facility at a commercial coal-fired electric generating plant suggests additional air emission control measures may be necessary to reduce potential site worker health risks and possibly community risks. Depending upon the location and regional air quality, considerable effort may be required to obtain the necessary air permit for construction and operation of a similarly configured large-scale PCCCS facility.

gas separation↗