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Temporal development of the correlation between ozone and potential vorticity in the Arctic in the winters of 1988/1989, 1989/1990, and 1990/1991

Ozone sonde data of the winters 1988/89, 1989/90, and 1990/91 from a group of Arctic stations are used in this study. The ozone mixing ratio on several isentropic surfaces is correlated to the potential vorticity (P). The P is based on the initialized analysis data from the European Center for Medium-Range Weather Forecasts. Similar investigations were made by Lait et al. (Geophys. Res. Lett., 17, 521-524, March Supplement 1990) for the AASE campaign (January and February 1989), showing how the ozone mixing ratio varies with the distance to the edge of the vortex. Their findings are confirmed and extended to the following two winters. Furthermore we have studied the temporal development of the P-ozone correlations during these winters in order to recognize any chemical ozone depletion.

Knudsen, Bjorn↗

Reconstruction of O3 and N2O fields from ER-2, DC-8, and balloon observations

Measurements of N2O and O3 during the Airborne Arctic Stratospheric Expedition have been composited using the potential vorticity and potential temperature of each measurement as coordinates. For ozone, data sources included the ER-2 and balloon ozonesonde in situ measurements, DC-8 DIAL lidar, and Stratospheric Aerosol and Gas Experiment satellite profiles. For N2O, only ER-2 data were used. These chemical composites have been reconstructed onto average meteorological fields for the mission in a latitude-altitude cross section, yielding a picture of the chemical composition of the polar vortex during this period. Tracers inside the vortex show an apparent descent of about 2 km relative to those outside, resulting in an apparent chemical edge on isentropic and isobaric surfaces.

Schoeberl, Mark R.↗

Column measurements of stratospheric trace species over Are, Sweden in the winter of 1991-1992

Total vertical column amounts of stratospheric HCl, HF, ClONO2 and HNO3 are reported from high resolution infrared solar absorption spectra taken during the European Arctic Stratospheric Ozone Experiment (EASOE) in the winter of 1991-1992. These ground based measurements were made near Are in North Sweden (63.4 deg N, 13.1 deg E) at an altitude of 800 m using a Fourier transform spectrometer and tunable diode laser heterodyne spectrometer. On 9th January 1992 the HCl vertical column dropped to 1.2 x 10(exp 15) molecules/sq cm from a November average of 3.6 x 10(exp 15) molecules/sq cm. The HCl drop occurred at a time when Are was below the polar vortex and the lower stratospheric ClO column above Are was elevated to approximately 2 x 10(exp 15) molecules/sq cm as measured by the Microwave Limb Sounder experiment on the Upper Atmosphere Research Satellite. These measurements indicate conversion of lower stratospheric chlorine from reservoir to chemically active forms.

Bell, W.↗

Simulation of the December 1998 Stratospheric Major Warming

Prior to 1991, major warmings (defined by increasing zonal mean temperatures and zonal mean easterly winds from 60degN to the pole at 10 hPa) typically occurred approximately once every two Arctic winters; a major warming in mid-Dec. 1998 was the first since Feb. 1991. The Dec. 1998 warming was also the second earliest on record. The earliest, and the only other major warming on record before the end of Dec. was in early Dec 1987; prior to that, the earliest was in late Dec./early Jan. 1984-85. The 1984-85 and 1987 warmings resulted in the warmest and weakest lower stratospheric polar vortices in the 20 years before 1998-99. Fig. 1 compares temperatures and vortex strength in 1998-99 with those in the previous 20 years, using the US National Center for Environmental Prediction (NCEP) record; 1987-88 and 1984-85 are also highlighted. The Dec. 1998 warming had a more pronounced effect on mid-stratospheric temperatures than the Dec. 1987 warming (Fig. 1a), although smaller than that of warmings later in winter (e.g., 1984-85). 10-hPa temperatures fell well below average again in late Jan. 1999 and remained unusually low until an early final warming began in late Feb. 840 K PV gradients (Fig. 1c) set a record minimum in Jan. 1999, but were near average in Feb before the final warming. The effect of the Dec. 1998 warming on lower stratospheric temperatures was comparable to that of other major warmings; there was a brief period of record-high minimum 46-hPa temperatures in early Jan 1999 (Fig. 1b), and temperatures then fell to near average for a short period in mid-Feb. Lower stratospheric PV gradients were the weakest on record during the 1998-99 winter (Fig. 1d). The evolution of the vortex and minimum temperatures during 1998-99 was remarkably similar to that during 1987-88, the only previous year when a major warming was observed before the end of Dec.

Manney, G. L.↗

Wintertime Arctic Oscillation and North Atlantic Oscillation and their impacts on the Northern Hemisphere climate in E3SM

The characteristics of the wintertime Arctic Oscillation (AO) and North Atlantic Oscillation (NAO) and their impacts on climate variability over the Northern Hemisphere are important metrics for evaluating a climate system model. Observational analyses reveal that the horizontal and vertical structures in the AO and NAO exhibit a meridional dipole and a large-scale barotropic pattern between the Arctic and mid-latitudes. Historical model simulations from the Energy Exascale Earth System Model (E3SM-HIST) are used to identify how well it captures these major climate modes. It is found that the simulated AO and NAO modes have spatial structures similar to the observed features. In addition, the observed frequency bands in the AO and NAO-related time variability are captured well in the E3SM-HIST simulation. Associated with the positive phase in wintertime AO and NAO, zonal flow and warm advection in mid-latitude continents are enhanced, along with stronger cold flow from enhanced northerly winds over high latitudes. These features are linked to the atmospheric circulation pattern reflected by lower SLP anomalies over the Arctic and higher SLP anomalies over the mid-latitudes. In E3SM-HIST, these spatial associations and main structural features are analogous to those in observations. In the time-height evolution related to winter AO and NAO modes, it can also be seen that the simulations reproduce the downward propagating patterns in observations. Nevertheless, the vertical structures associated with AO and NAO in E3SM-HIST exhibit substantial biases in the lower stratosphere. The cause of these stratospheric biases is investigated using the strength of climatological stratospheric polar vortex (SPV) and wave activity fluxes. The results herein suggest that E3SM-HIST has a reasonable skill in reproducing the observed characteristics related to the winter AO and NAO, although there exist systematic biases in the associated climate variability.

54 ENVIRONMENTAL SCIENCES↗

Aircraft measurements of the atmospheric electrical global circuit during the period 1971-1984

This report will update an investigation of the global circuit conducted over the last 14 years through aircraft measurements of the variation of ionospheric potential and associated parameters. The data base included electric field, conductivity, and air-earth current density profiles from the tropics (25 deg N) to the Arctic (79 deg N). Almost all of the data have been obtained over the ocean to reduce noise associated with local generators, aerosols, and convection. Recently, two aircraft have been utilized to obtain, for the first time, quasi-periodic sets of simultaneous ionospheric potential (VI) soundings at remote locations and extending over time spans sufficiently long so that the universal time diurnal variation (Carnegie curve) could be observed. In additon, these measurements provided the first detection of the modulation of electric fields in the troposphere caused by the double vortex ionospheric convection pattern. Besides summarizing these measurements and comparing them to similar data obtained by other groups, this report discusses meteorological sources of error and criteria for determining if the global circuit is being measured rather than variations caused by local meteorological processes.

Markson, R.↗

Arctic polar stratospheric cloud observations by airborne lidar

Lidar observations obtained from January 24 to February 2, 1989, during the Airborne Arctic Stratospheric expedition (AASE) mission further support the existence of two distinct classes (Types 1 and 2) of polar stratospheric clouds (PSCs). Most of the Type 1 PSCs observed were formed by rapid adiabatic cooling and exhibited very low depolarization ratios and low-to-intermediate scattering ratios. Type 2 PSCs were observed in regions of lowest temperature and showed much larger depolarization and scattering ratios, as would be expected from larger ice crystals. PSCs with low scattering ratios but moderate depolarization ratios were observed near the center of the vortex on one flight. These may have been either sparse Type 2 PSCs or Type 1 PSCs formed by less rapid cooling.

Mccormick, M. P.↗

Airborne lidar measurements of ozone during the 1989 airborne Arctic stratospheric expedition

The NASA/NOAA Airborne Arctic Stratospheric Expedition (AASE) was conducted during the winter to study the conditions leading to possible ozone (O3) destruction in the wintertime Arctic stratosphere. As part of this experiment, the NASA-Langley airborne differential absorption lidar (DIAL) system was configured for operation on the NASA-Ames DS-8 aircraft to make measurements of O3 profiles from about 1 km above the aircraft to altitudes of 22 to 26 km. The airborne DIAL system remotely sensed O3 above the DC-8 by transmitting two laser beams at 10 Hz using wavelengths of 301.5 and 311 nm. Large scale distributions of O3 were obtained on 15 long range flights into the polar vortex during the AASE. Selected data samples are presented of O3 observed during these flights, general trends observed in O3 distributions, and correlations between these measurements and meteorological and chemical parameters. The O3 distribution observed on the first flight of the DC-8 into the polar vortex on Jan. 6 reflected the result of diabatic cooling of the air inside the vortex during the winter compared to the warmer air outside the vortex. On a potential temperature surface, the O3 mixing ratio generally increases when going from outside to inside the vortex.

Browell, Edward V.↗

Meteorological atlas of the Northern Hemisphere lower stratosphere for January and February 1989 during the Airborne Arctic Stratospheric Expedition

Northern Hemisphere meteorological data for the months of January and February 1989 in the lower stratosphere are shown. National Meteorological Center (NMC) data, and Total Ozone Mapping Spectrometer (TOMS) data are used to display polar stereographic projections of 100-mb temperatures, 50-mb temperatures, 50-mb geopotential heights, total ozone, and Ertel's potential vorticity (Epv) on both 400 K and 460 K isentropic surfaces. In addition, latitude/height cross sections at 10 E of balanced wind isotachs, wind vectors, potential temperature, and temperature are also shown. Horizontal traces of NASA ER-2 and DC-8 flight tracks are also included. Vertical profiles of NMC temperatures following flight paths of both aircraft are shown. In addition, vertical profiles of wind speed are contoured following the ER-2 for estimating the lateral penetration into the polar vortex, while vertical profiles of Ertel's potential vorticity are included for estimating the vertical penetration of the DC-8 into the stratosphere.

Newman, Paul A.↗

Airborne Arctic Stratospheric Expedition 2: Air Parcel Trajectories

An overview of Airborne Arctic Stratospheric Expedition 2 is given. Effects of Pinatubo aerosol on stratospheric ozone at mid-latitudes, in situ measurements of ClO and ClO/HCl ratio, balloon-borne measurements of ClO, NO, and O3 in a volcanic cloud, and new observations of the NO(y)/N2O correlation in the lower stratosphere are discussed. Among other topics addressed are the following: in situ tracer correlations of methane, nitrous oxide, and ozone as observed aboard the DC-8, in situ measurements of changes in stratospheric aerosol and the N2O-aerosol relationship inside and outside of the polar vortex, measurements of halogenated organic compounds near the tropical tropopause, and airborne brightness measurements of the polar winter troposphere.

Source record↗

Polar Vortex Conditions During the 1995-96 Artic Winter: Meteorology and MLS Ozone

The 1995-96 northern hemisphere (NH) winter was colder than any of the previous 17 NH winters, with temperatures continuously below the type 1 polar stratospheric cloud (PSC) threshold for over 2 1/2 months; upper tropospheric ridges in late Feb and early Mar 1996 led to the lowest observed NH winter lower stratospheric temperatures, and the latest observation of HN temperatures below the type 2 PSC threshold.

arctic↗

Aerosols and polar stratospheric clouds measurements during the EASOE campaign

Preliminary results of observations performed using two different lidar systems during the EASOE (European Arctic Stratospheric Ozone Experiment), which has taken place in the winter of 1991-1992 in the northern hemisphere lattitude regions, are presented. The first system is a ground based multiwavelength lidar intended to perform measurements of the ozone vertical distribution in the 5 km to 40 km altitude range. It was located in Sodankyla (67 degrees N, 27 degrees E) as part of the ELSA experiment. The objectives of the ELSA cooperative project is to study the relation between polar stratospheric cloud events and ozone depletion with high vertical resolution and temporal continuity, and the evolution of the ozone distribution in relation to the position of the polar vortex. The second system is an airborne backscatter lidar (Leandre) which allows for the study of the 3-D structure and the optical properties of polar stratospheric clouds. The Leandre instrument is a dual-polarization lidar system, emitting at 532 nm, which allows for the determination of the type of clouds observed, according to the usual classification of polar stratospheric clouds. More than 60 hours of flight were performed in Dec. 1991, and Jan. and Feb. 1992 in Kiruna, Sweden. The operation of the Leandre instrument has led to the observation of the short scale variability of the Pinatubo volcanic cloud in the high latitude regions and to several episodes of polar stratospheric clouds. Preliminary analysis of the data is presented.

Haner, D.↗

Arctic polar stratospheric cloud measurements by means of a four wavelength depolarization lidar

A four wavelength depolarization backscattering lidar has been operated during the European Arctic Stratospheric Ozone Experiment (EASOE) in Sodankyl, in the Finnish Arctic. The lidar performed measurements during the months of December 1991, January, February and March 1992. The Finnish Meteorological Institute during the same period launched regularly three Radiosondes per day, and three Ozone sondes per week. Both Mt. Pinatubo aerosols and Polar Stratospheric Clouds were measured. The use of four wavelengths, respectively at 355 nm, 532 nm , 750 nm, and 850 nm permits an inversion of the lidar data to determine aerosol particle size. The depolarization technique permits the identification of Polar Stratospheric Clouds. Frequent correlation between Ozone minima and peaks in the Mt. Pinatubo aerosol maxima were detected. Measurements were carried out both within and outside the Polar Vortex.

Stefanutti, L.↗

Analysis of stratospheric ozone, temperature, and minor constituent data

The objective of this research is to use available satellite measurements of temperature and constituent concentrations to test the conceptual picture of stratospheric chemistry and transport. This was originally broken down into two sub-goals: first, to use the constituent data to search for critical tests of our understanding of stratospheric chemistry and second, to examine constituent transport processes emphasizing interactions with chemistry on various time scales. A third important goal which has evolved is to use the available solar backscattered ultraviolet (SBUV) and Total Ozone Mapping Spectrometer (TOMS) data from Nimbus 7 to describe the morphology of recent changes in Antarctic and global ozone with emphasis on searching for constraints to theories. The major effort now being pursued relative to the two original goals is our effort as a theoretical team for the Arctic Airborne Stratospheric Expedition (AASE). Our effort for the AASE is based on the 3D transport and chemistry model at Goddard. Our goal is to use this model to place the results from the mission data in a regional and global context. Specifically, we set out to make model runs starting in late December and running through March of 1989, both with and without heterogeneous chemistry. The transport is to be carried out using dynamical fields from a 4D data assimilation model being developed under separate funding from this task. We have successfully carried out a series of single constituent transport experiments. One of the things demonstrated by these runs was the difficulty in obtaining observed low N2O abundances in the vortex without simultaneously obtaining very high ozone values. Because the runs start in late December, this difficulty arises in the attempt to define consistent initial conditions for the 3D model. To accomplish a consistent set of initial conditions, we are using the 2D photochemistry-transport model of Jackman and Douglass and mapping in potential temperature, potential vorticity space as developed by Schoeberl and coworkers.

Stolarski, Richard S.↗

A Golden Era of PSC Observations From the A-Train By CALIOP and MLS

The fundamental role of polar stratospheric clouds (PSCs) in the depletion of stratospheric ozone is well established. Heterogeneous reactions on PSCs convert the stable chlorine reservoirs HCl and ClONO2 to chlorine radicals that destroy ozone catalytically. PSCs also prolong ozone depletion by delaying chlorine deactivation through the removal of gas-phase HNO3 and H2O by sedimentation of large PSC particles. There has been substantial recent progress in our understanding of PSC processes due to the long-term, vortex-wide observations from the CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) lidar on the CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations) satellite and the MLS (Microwave Limb Sounder) on the Aura satellite. The CALIOP observations provide unprecedented high spatial resolution information on particulate aerosol/PSC morphology and composition, while MLS provides complementary collocated measurements of gas-phase HNO3 and H2O, the major constituents of all PSC particles. The combined analyses of these datasets have enabled better PSC composition discrimination and provided valuable new insight into PSC formation processes and particle growth kinetics. The more than 17 years of CALIOP and MLS data have uniquely captured the primary aspects of the seasonal and multi-year variability of PSCs in the Arctic and Antarctic, enabling the development of a state-of-the-art reference PSC data record and climatology. In this presentation, we highlight the significant advances in our understanding achieved during this golden era of spaceborne PSC observations and identify remaining gaps in our knowledge that future spaceborne lidar missions may help resolve.

polar stratospheric clouds↗

What Controls the Arctic Lower Stratosphere Temperature?

The temperature of the Arctic lower stratosphere is critical for understanding polar ozone levels. As temperatures drop below about 195 K, polar stratospheric clouds form, which then convert HCl and ClONO2 into reactive forms that are catalysts for ozone loss reactions. Hence, the lower stratospheric temperature during the March period is a key parameter for understanding polar ozone losses. The temperature is basically understood to be a result of planetary waves which drive the polar temperature away from a cold "radiative equilibrium" state. This is demonstrated using NCEP/NCAR reanalysis calculations of the heat flux and the mean polar temperature. The temperature during the March period is fundamentally driven by the integrated impact of large scale waves moving from the troposphere to the stratosphere during the January through February period. We will further show that the recent cold years in the northern polar vortex are a result of this weakened wave driving of the stratosphere.

Newman, Paul A.↗

Field and Satellite Observations of the Formation and Distribution of Arctic Atmospheric Bromine Above a Rejuvenated Sea Ice Cover

Recent drastic reduction of the older perennial sea ice in the Arctic Ocean has resulted in a vast expansion of younger and saltier seasonal sea ice. This increase in the salinity of the overall ice cover could impact tropospheric chemical processes. Springtime perennial ice extent in 2008 and 2009 broke the half-century record minimum in 2007 by about one million km2. In both years seasonal ice was dominant across the Beaufort Sea extending to the Amundsen Gulf, where significant field and satellite observations of sea ice, temperature, and atmospheric chemicals have been made. Measurements at the site of the Canadian Coast Guard Ship Amundsen ice breaker in the Amundsen Gulf showed events of increased bromine monoxide (BrO), coupled with decreases of ozone (O3) and gaseous elemental mercury (GEM), during cold periods in March 2008. The timing of the main event of BrO, O3, and GEM changes was found to be consistent with BrO observed by satellites over an extensive area around the site. Furthermore, satellite sensors detected a doubling of atmospheric BrO in a vortex associated with a spiral rising air pattern. In spring 2009, excessive and widespread bromine explosions occurred in the same region while the regional air temperature was low and the extent of perennial ice was significantly reduced compared to the case in 2008. Using satellite observations together with a Rising-Air-Parcel model, we discover a topographic control on BrO distribution such that the Alaskan North Slope and the Canadian Shield region were exposed to elevated BrO, whereas the surrounding mountains isolated the Alaskan interior from bromine intrusion.

Nghiem, Son V.↗

The January 30, 1989 Arctic polar stratospheric clouds (PSC) event - Evidence for a mechanism of dehydration

In-situ particle measurements made aboard the NASA ER-2 in the Arctic on 890130 (YYMMDD) show Type 1 PSC particles over much of the flight, with instances of embedded Type 2 PSCs. The Type 2 particles were observed at temperatures warmer than the local frost-point temperature of water; extended up to the upper size cutoff of the instrument (about 24-micron diameter); and are shown to contain too large a volume to be primarily NAT. Based on measured vertical temperature profiles, it is concluded that the Type 2 particles observed on this day were formed above the aircraft in a region where saturation with respect to ice was achieved and were sufficiently large to have fallen into the path of the ER-2. Although the amount of material in the particles, expressed as water, is small by comparison to the total (vapor + aerosol) water concentration, the flux of water from the falling particles is of sufficient magnitude, if sustained, to lead to dehydration of the source region. These observations verify the mechanism for dehydration of polar vortex air masses by precipitation of ice particles.

Gandrud, B. W.↗