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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 235 records · Page 13

Determination of Multimode Motional Quantum States in a Trapped Ion System

Trapped atomic ions are a versatile platform for studying interactions between spins and bosons by coupling the internal states of the ions to their motion. Measurement of complex motional states with multiple modes is challenging, because all motional state populations can only be measured indirectly through the spin state of ions. Here we present a general method to determine the Fock state distributions and to reconstruct the density matrix of an arbitrary multimode motional state. Further, we experimentally verify the method using different entangled states of multiple radial modes in a five-ion chain. This method can be extended to any system with Jaynes-Cummings-type interactions.

74 ATOMIC AND MOLECULAR PHYSICS↗

Atom Interferometry with Floquet Atom Optics

Floquet engineering offers a compelling approach for designing the time evolution of periodically driven systems. We implement a periodic atom-light coupling to realize Floquet atom optics on the strontium 1 S 0 - 3 P 1 transition. These atom optics reach pulse efficiencies above 99.4% over a wide range of frequency offsets between light and atomic resonance, even under strong driving where this detuning is on the order of the Rabi frequency. Moreover, we use Floquet atom optics to compensate for differential Doppler shifts in large momentum transfer atom interferometers and achieve state-of-the-art momentum separation in excess of 400 ℏ⁢k. In conclusion, this technique can be applied to any two-level system at arbitrary coupling strength, with broad application in coherent quantum control.

74 ATOMIC AND MOLECULAR PHYSICS↗

Multidimensional Coherent Spectroscopy of Molecular Polaritons: Langevin Approach

We present a microscopic theory for nonlinear optical spectroscopy of N molecules in an optical cavity. Using the Heisenberg-Langevin equation, an analytical expression is derived for the time- and frequency-resolved signals accounting for arbitrary numbers of vibrational excitations. We identify clear signatures of the polariton-polaron interaction from multidimensional projections of the signal, e.g., pathways and timescales. Cooperative dynamics of cavity polaritons against intramolecular vibrations is revealed, along with a crosstalk between long-range coherence and vibronic coupling that may lead to localization effects. Our results further characterize the polaritonic coherence and the population transfer that is slower.

74 ATOMIC AND MOLECULAR PHYSICS↗

New Polarizability Functions for Calculating Atomic Hydrogen S State Spectral Lines in Exact Agreement with NIST Measurements

This paper presents a new approach to calculating atomic hydrogen energy levels which is simple, fast and accurate. One advantage of this new approach is the ability to explicitly incorporate the polarizability resulting from a scattering event between a hydrogen atom and a photon. The polarizability effect is small but significant, producing exact S state spectral energies. The general calculational approach is applicable to both atomic hydrogen and multi-electron energy levels. Although motivated by the multi-electron case for chemistry applications, the focus of this paper will be calculations that are specific to atomic hydrogen which include the polarizability.

74 ATOMIC AND MOLECULAR PHYSICS↗

New PHENIX Results on Mid-Rapidity Bottom and Charm Production in Au+Au collisions at $\sqrt{s_{NN}}$= 200 GeV

Energy loss of quarks in the hot and dense medium has been studied for decades. Both the experimental and theoretical efforts have hinted that the energy loss is quark mass dependent. Although experiments at the Relativistic Heavy Ion Collider (RHIC) and the Large Hadron Collider (LHC) have found that the electrons from heavy quarks are less or similarly suppressed compared to the light hadrons, the mass ordering of the suppression between charm and bottom quarks is not yet clear due to large experimental uncertainties. We have fully exploited the events recorded at mid-rapidity in Au+Au collisions at center-of-mass energy of 200 GeV by the PHENIX experiment at RHIC to study the invariant yield of electrons from open heavy flavors. Latest results on the nuclear modification factors for charm and bottom separated heavy flavor electrons are reviewed in this proceeding. The implications of these results on the understanding of the quark mass and medium size dependence of the energy loss are also discussed.

74 ATOMIC AND MOLECULAR PHYSICS↗

Robust Optimized Pulse Schemes for Atomic Fountain Interferometry

The robustness of an atomic fountain interferometer with respect to variations in the initial velocity of the atoms and deviations from the optimal pulse amplitude is examined. We numerically simulate the dynamics of an interferometer in momentum space with a maximum separation of and map out the expected signal contrast depending on the variance of the initial velocity distribution and the value of the laser field amplitude. We show that an excitation scheme based on rapid adiabatic passage significantly enhances the expected signal contrast, compared to the commonly used scheme consisting of a series of and pulses. We demonstrate further substantial increase of the robustness by using optimal control theory to identify splitting and swapping pulses that perform well on an ensemble average of pulse amplitudes and velocities. Our results demonstrate the ability of optimal control to significantly enhance future implementations of atomic fountain interferometry.

74 ATOMIC AND MOLECULAR PHYSICS↗

The Spin-Orbit Interaction: A Small Force with Large Implications

The spin-orbit interaction is quite small compared to electrostatic forces in atoms. Nevertheless, this small interaction can have large consequences. Several examples of the importance of the spin-orbit force in atomic photoionization are presented and explained.

74 ATOMIC AND MOLECULAR PHYSICS↗

Configuration–Interaction Perturbation Theory Calculations of Pu II

Configuration–interaction perturbation theory (CI–PT) is applied to calculations of low-energy states of Pu II. This ion is quite challenging due to a large number of possible determinants arising from seven valence electrons and strong relativistic effects. The CI–PT calculations agree with experiments for the energies and g-factors for many low-energy states that allowed positive identification of the theoretical levels. Isotope shifts were also used to aid in identification, and, in case of the odd states, fitting with three independent parameters was used to match theoretical isotope shifts to the experimental values with good accuracy. The CI–PT approach tested here on the Pu II ion can be generally used to calculate properties of many complex atoms, including U I that can find application in fundamental and applied science.

74 ATOMIC AND MOLECULAR PHYSICS↗

Relativistic Configuration-Interaction and Perturbation Theory Calculations for Heavy Atoms

Heavy atoms present challenges to atomic theory calculations due to the large number of electrons and their complicated interactions. Conventional approaches such as calculations based on Cowan’s code are limited and require a large number of parameters for energy agreement. One promising approach is relativistic configuration-interaction and many-body perturbation theory (CI-MBPT) methods. We present CI-MBPT results for various atomic systems where this approach can lead to reasonable agreement: La I, La II, Th I, Th II, U I, Pu II. Among atomic properties, energies, g-factors, electric dipole moments, lifetimes, hyperfine structure constants, and isotopic shifts are discussed. While in La I and La II accuracy for transitions is better than that obtained with other methods, more work is needed for actinides.

74 ATOMIC AND MOLECULAR PHYSICS↗

Modeling Competing Line-broadening Mechanisms in Neutron Star Atmospheres: Interference between Motional Stark and Ion Broadening

Neutron star surfaces have extremely high magnetic fields. In the atmosphere, the broadening of spectral lines will be substantial from the dense plasma as well as from the magnetic field. One broadening mechanism of note is due to the motional Stark effect (MSE)—an additional electric field that arises from the motion of the atom in the magnetic field. However, approximate formulae are often used to construct atmosphere models, and the MSE is assumed to be the dominant line-broadening mechanism even in ions. Detailed pressure-broadening models in these extreme magnetic fields are now currently being developed. In these more detailed models, it was suggested that the MSE may not be as large as previously predicted. If correct, this hypothesis implies that neutron star line widths might be dominated by pressure broadening rather than by motional Stark broadening. We find that, in the absence of plasma perturbations, for typical magnetic fields (B = 10 12 G), mid-Z elements, such as oxygen, have motional Stark widths of order 1 eV for transitions between dipole-allowed transitions from the ground state, though higher temperatures and transitions to higher-energy states are expected to have more broadening. The MSE also breaks down selection rules, giving rise to forbidden transitions, which have much larger widths. When plasma perturbations are included, we find that the plasma perturbation and motional Stark processes are not independent and, as a result, the spectral lines become narrow in a nontrivial way and display harmonics of the ion cyclotron frequency.

74 ATOMIC AND MOLECULAR PHYSICS↗

Opacity on NIF: Anchor 2 Iron (Level 2 Milestone 7118 Report)

In FY2020 we fulfilled the exit criteria of milestone 7118. We fielded iron opacity experiments at higher densities and temperatures approaching anchor 2 conditions and made good progress on overcoming the problems that we found. This report describes in detail the progress that has been made. We presented the results in a LANL seminar on August 10 and we gave two talks on our results to the National Opacity Workshop Series, one on July 9 and the other on September 14. Before discussing the anchor 2 measurements, we present an update of the NIF anchor 1 data. We did a new analysis of the anchor 1 data and compared the results to a series of calculations using the LANL ATOMIC code. Figures 1 and 2 compare the data with the best-fit to calculations. This result is significantly improved over the result published in Atoms. The differences are small for the iron quasi-continuum between 8-9.5 Å and for the Mg Heα and Lyα lines. The opacities near the centers of the iron bound-bound features also match fairly well in the 9.5-12.5 Å range. However, the opacity windows between the large iron bound-bound features are deeper in the Atomic predictions than the measurement. Furthermore, large discrepancies exist for the Mg He β, γ, and δ lines and for the short-wavelength quasicontinuum. The experiment and analysis refinements described below have set the stage for unraveling these discrepancies. Specifically, we can repeat the Anchor 1 experiments using improved backlighter, hohlraum, and spectrometers to obtain reduced backgrounds and better spectral resolution. Exploiting the AlMg calibration experiments and repeating the Anchor 1 measurements multiple times will enable formal and rigorous uncertainty determination. This well-defined path gives us confidence that high quality opacity data can be obtained on NIF.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Spectroscopy of atoms in an optical dipole trap using spectrally selective heating by a probe laser field

Spectral properties of atoms localised in an optical dipole trap are studied using the method of spectrally selective heating by a probe field. The method is based on measuring the number of atoms in a trap after they interact with a probe field. The dependence of the number of atoms on the frequency of the probe field fully characterises the shift and width of the spectral absorption line of trapped atoms. (paper)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗