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At least 235 records · Page 13

Evaluation and improvement of the parameterization of aerosol hygroscopicity in global climate models using in-situ surface measurements (Final Report)

Aerosols are tiny particles suspended on the atmosphere that can interact with incoming solar radiation and affect the Earth radiative budget. They do so by scattering and absorbing solar radiation, and these properties vary depending on the aerosol size and chemical composition. Moreover, by taking up water from the surrounding air, hygroscopic aerosol particles will grow in size and change their chemical composition, thus modifying their optical properties (scattering and absorption) and their final impact on radiative forcing calculations. An accurate knowledge of aerosol hygroscopicity is crucial for estimating the net radiative impact of aerosols. We took a three-pronged approach to improve our understanding of aerosol hygroscopicity and how it is implemented in Earth system models. In the first part of our project, we developed a benchmark dataset from existing aerosol hygroscopic growth measurements made by tandem nephelometer humidogram systems. We analyzed, using a standardized methodology, observations from 26 in-situ stations around the globe. Measurement data was collected from multiple data providers, reviewed and harmonized to create a consistent dataset of the scattering enhancement factor due to aerosol water uptake. This dataset is archived in several publicly available databases for use by interested researchers. In the second part of the project, we used the benchmark hygroscopicity dataset to perform a global study on aerosol hygroscopicity and aerosol optical properties. Measurements show a global picture of scattering enhancement with larger values for Arctic and marine sites and lower for urban and desert sites. We assessed the RH dependence of aerosol radiative forcing and showed that the overall effect of aerosol hygroscopicity on DARF is an increase in the absolute forcing effect (negative sign) by a factor of up to 4 compared to dry conditions (RH<40%). Finally, we explored using aerosol single scattering albedo (SSA) and scattering Angstrom exponent (SAE) as possible proxies for aerosol hygroscopicity. SSA showed more promise as a surrogate for the scattering enhancement factor than SAE, but neither was ideal. In the third part of the project we evaluated the output of ten Earth system models (ESMs) against the benchmark hygroscopicity dataset. ESMs utilize various schemes for aerosol hygroscopicity which had not been previously tested against observations on a global scale. We found that ESMs currently overestimate scattering enhancement due to hygroscopic growth. Model parameterizations of hygroscopicity and model chemistry are two main factors driving the observed diversity in hygroscopicity simulations among the models. In addition, our study makes several suggestions for modelers, including improving the parameterizations of organic and sea salt aerosol hygroscopicity. Future hygroscopicity model evaluation experiments should include the model data related to particles size which was not available for our study.

54 ENVIRONMENTAL SCIENCES↗

Fire, dust, air and water: Improving aerosol biogeochemistry interactions in ACME. Final report

Aerosol-biogeochemistry interactions will have important consequences for human health, ecosystem services, and climate feedbacks over the next several decades. In this proposal we seek to link how human activities on land, including direct industrial emissions and landscape fires, impact the atmosphere and the biogeochemistry of the ocean and land. Our overall goal was to complement existing work at DOE labs to improve the capability and performance of the E3SM model in short-term, high-resolution projections of climate. Projections of ocean uptake of anthropogenic carbon are highly dependent on the details of the ocean physical and biogeochemistry parameterizations. Potentially equally important are the estimates of increases in iron and soluble nitrogen deposition in aerosols to the open ocean, but there are substantial uncertainties in these feedbacks. The E3SM land model simulates natural and anthropogenic fires, but improvement is needed to more accurately simulate fire responses to climate variability as well as fire contributions to terrestrial climate feedbacks. This proposal addressed four of the six priorities within the ACME/E3SM call by improving the representation of fire, industrial combustion sources, and desert dust and adding iron and soluble iron to the atmospheric chemistry (1). Our work focused on improving ocean biogeochemistry and the response of the oceans to anthropogenic atmospheric iron and nitrogen (3). We also improved the representation of land disturbance on fires and fire mediated carbon cycle feedbacks in the land model (4). Finally we had planned to couple the land, atmosphere and ocean biogeochemical systems (6) and explore how this coupling changes the feedbacks in the climate system. Our work under this proposal was separated into the following 5 tasks: i) improve representation of fire dynamics in both boreal and tropical ecosystems, ii) improve estimates of industrial emissions of iron and phosphorus, iii) improve representation of atmospheric iron, phosphorus and nitrogen transport, chemistry and deposition, iv) improve representation of iron, phosphorus and nitrogen deposition impacts on ocean biogeochemistry, and v) couple emissions into atmosphere, to deposition onto land and ocean biogeochemistry. For all 5 tasks, we conducted offline experiments of the historical period to enable comparison with available aerosol and land surface observations. We had planned to conduct fully coupled simulations, however, these will be conducted as part of the coupling in version 3 and 4 of the E3SM model, and thus have not been completed.

54 ENVIRONMENTAL SCIENCES↗

Non-contact Current-Voltage (I-V) Tracer for Photovoltaics

This report presents a non-contact approach to simultaneously obtain current-voltage (I-V) curves of photovoltaic (PV) substrings and modules in a string without the need of disconnecting the individual modules from the string. There are two types of I-V curve tracers currently available in the marketplace, capacitor-based and electronic load-based. The primary requirement of these conventional I-V tracers is the disconnection of individual modules in the string so the individual modules contacted through the connectors of the individual modules. These contact-tracers have three major limitations in the utility scale power plants: First limitation – Weather and Accuracy: The mass-produced commercial contact-tracers cannot obtain the I-V curves of both string and its modules (as high as 30 modules), almost simultaneously (within about 5 minutes) at, practically, a single irradiance level, a single module temperature, a single spectrum and a single AOI (angle of incidence). This inability of the contact-tracers forces the testing personnel to wait for an extended or multiple sunny (>800 W/m 2 ) duration(s) of a cloudy day. This is a serious limitation as waiting for the sunny conditions or days is a huge practical challenge in almost all locations, except desert locations. Also, since the I-V curves are obtained at different prevailing weather conditions, it becomes critical to translate all the measured I-V curves of 30 modules in the string to a single test condition, for example STC (standard test conditions), so the underperforming modules can be identified. The accuracy of translation equations is heavily influenced by the irradiance level and temperature, spectral and AOI ranges; Second limitation - Safety: The second limitation is related to the high voltage electrical safety of the test personnel during disconnecting and reconnecting of individual modules or cable connectors from the string under daylight conditions and damaging of the original module connectors (especially the field aged connectors) during the disconnecting and reconnecting process; Third limitation – Labor: The third limitation is related to the enormous amount of time and hardship for the test personnel under prevailing (often harsh) protracted field conditions. This project was executed by Arizona State University in collaboration with its industry partner, PV Measurements Inc. (PVM). To mitigate all the three challenges of the state-of-the-art equipment indicated above, we utilized a non-contact I-V (NCIV) tracer approach. In this approach, we utilized an electrostatic voltmeter (ESV) and voltage sensor/probe combination to obtain I-V curves. The ESV units are extensively used in the high voltage industry but not in the PV industry. To obtain the simultaneous I-V curves of the substrings and modules within a string, we utilized multiple commercial ESV-Probe sets. In this approach, we utilized a non-contact voltage sensor (called, Probe) placed on the glass surface of the module (above the last cell of the module). This probe senses the module voltage (with respect to ground) through measured capacitance which is dictated by the surface charges (which in turn is dictated by the module voltage) and transmits the sensed voltage to the voltmeter (called, ESV or NCV, non-contact voltmeter). The current is sensed by a non-contact hall sensor. In a 30-module string, the 30th probe obtains the entire string I-V along with the string I-V obtained by the electronic load. so that the I-V curves of the substrings and modules can be obtained by NCIV without the need of disconnecting the individual modules in the string. The string I-V curves obtained by the electronic load and NCIV can be compared for the accuracy determination. One can use 30 ESV units and 30 Probes to obtain 30 I-V curves of a 30-module string or use just 5 ESV units and 30 Probes in conjunction with 5 six-channel switchboxes (called, 6:1 switchboxes). To reduce the equipment cost, we utilized the 6:1 switchbox approach so the number of ESV units is reduced from 30 to 5. The approaches, achievements and challenges of this project are detailed in this report.

14 SOLAR ENERGY↗

Mother's Day tribute: Remembering mom of baby 'Trinity'

For Elizabeth “Diz” Graves, the summer months of 1945 were a symbolic intersection of her personal and professional lives. As a physicist with the then-secret lab in Los Alamos, Elizabeth participated in the Trinity test - the successful detonation of the world’s first nuclear weapon, which took place in the remote New Mexico desert on July 16, 1945. Her role was to observe the explosion that advanced science into the Atomic Age, according to records in the National Security Research Center (NSRC). This is the Lab’s classified library, which also houses unclassified legacy materials. And, Elizabeth was seven months pregnant.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

Phase II Geochemical and Isotopic Evaluation of Groundwater Flow in the Pahute Mesa–Oasis Valley Flow System, Nevada

This report presents the results of the Phase II geochemical evaluation for the Pahute Mesa CAUs. The evaluation was performed by multiple organizations including Los Alamos National Laboratory (LANL), Desert Research Institute (DRI), Lawrence Livermore National Laboratory (LLNL), and Navarro. Section 1.0 presents the introduction and describes the objectives for the Phase II geochemical evaluation. Section 2.0 presents the hydrologic setting, including average annual precipitation and net infiltration, hydraulic-head gradients, geology, and hydrostratigraphy of the PM-OV flow system.

54 ENVIRONMENTAL SCIENCES↗

How did the world’s first atomic bomb get its name? Looking back on the Trinity test on its 76th anniversary

The world’s first-ever atomic bomb is called The Gadget. It was detonated in the New Mexico desert on July 16,1945 during the Trinity test, verifying that an implosion-type plutonium bomb would be successful when released above Nagasaki just weeks later. That atomic bomb was called Fat Man and it was a weaponized version of the Trinity device of The Gadget. According to the longtime lore, the bulbous-looking Fat Man bomb’s name was inspired by British Prime Minister Winston Churchill. After the Thin Man bomb, whose moniker was inspired by the U.S. President Franklin Roosevelt, didn’t come to fruition, the gun-type uranium atomic bomb named Little Boy was developed. It was likely dubbed as such because it was smaller in size.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

Plutonium and poetry: Where Trinity and Oppenheimer's reading habits met Literary inspirations, correcting misinterpretation of his famous quote

The Lab’s first director, J. Robert Oppenheimer, was a man of sonnets and scientific synthesis. Oppenheimer’s work at Los Alamos was defined not only by physics and administrative skill, but also by a life philosophy inspired, in part, by literature. The Trinity test, which took place 76 years ago on July 16th in the New Mexico desert, epitomizes this. Known as one of the greatest scientific achievements ever, the successful detonation of the world’s first nuclear weapon marked the dawn of the Atomic Age. Created in just 27, albeit harrowing, months, Oppenheimer and his team at the Los Alamos Lab worked nonstop on this clandestine effort to help end World War II. As he had done throughout his life, Oppenheimer continued to foster his love of literature during the Manhattan Project. Two of his influences were John Donne and the Hindu scripture Bhagavad-Gita. Oppenheimer recalled both during the Trinity test.

96 KNOWLEDGE MANAGEMENT AND PRESERVATION↗

Update of Erosion Conditions and Assessment of Mitigation Options for the L-Bar Site

The L-Bar former uranium milling site was remediated and closed per regulations and is now under the long-term stewardship of the U.S. Department of Energy, Office of Legacy Management (DOE/LM). Since assuming stewardship in 2004, DOE/LM has observed erosion and sedimentation processes at the L-Bar Site that will challenge meeting the design closure criteria in the long term, and therefore erosion control structures were installed in several areas. Portions of these structures were subsequently damaged by summer convective storm events and they are being redesigned. At the request of DOE/LM, Desert Research Institute (DRI) reviewed the proposed redesign plans of the erosion control structures. The purpose of this review is to support DOE/LM decisions regarding mitigation of ongoing erosion processes, including assessing possible repair of the existing erosion control structures, as well as plan for effective long-term site management. This design review is performed in reference to the Uranium Mill Tailings Radiation Control Act (UMTRCA) standards contained in 40 CFR 192.02 that require containment of residual radioactive material be effective for up to 1,000 years (if achievable, but certainly for 200 years), limit radon release, protect groundwater, and minimize future maintenance. The erosion control structures under review are not subject to the UMTRCA standard directly, but they contribute to the performance of the overall containment system by virtue of their relationship with the large diversion channels bounding the disposal cell. The 11 design drawings included in “Erosion Control Alternatives Analysis, L-Bar, New Mexico, Disposal Site, LTS-111-0043-08-002,” dated January 11, 2019, and listed in Appendix A, and supporting calculations in Weston (2019) are the focus of the review. Additionally, DOE/LM provided supporting data such as a 2018 photogrammetry-based digital elevation model of the site, precipitation records collected from an on-site weather station, and sedimentation records collected at an on-site basin. This assessment includes review of the proposed design to mitigate current site conditions but also addresses site changes between the initial erosion assessment report (Miller et al., 2012) and current conditions. The analysis is at a predesign engineering level and does not include development of hydraulic or sediment transport models. Site precipitation data are included in Miller et al. (2012). The natural conditions of the site, the design of site diversion systems, observed erosion at the site, and predesign engineering analysis are used to develop a holistic view of the challenges to L-Bar Site stability and possible responsive actions.

54 ENVIRONMENTAL SCIENCES↗

The Architecture of Area 12 Camp - Nevada's Atomic Ghost Town. An Architectural Survey of Area 12 Camp, Nevada National Security Site, Nye County, Nevada

The U.S. Department of Energy, National Nuclear Security Administration Nevada Field Office (NNSA/NFO) plans to demolish 10 buildings and one structure in Area 12 Camp at the Nevada National Security Site (NNSS) in Nye County, Nevada, to meet current and future National Weapons Science, Global and Homeland Security Program, and Environmental Management mission requirements and to reduce dangers to site workers from some of these resources. These demolitions constitute an undertaking subject to review under Title 54 U.S.C. § 306108, commonly known as Section 106 of the National Historic Preservation Act, Title 54 U.S.C. § 300101, et seq., and its implementing regulations, 36 C.F.R. Part 800. These resources were recorded and evaluated as individually ineligible for the National Register of Historic Places (National Register or NRHP) by Menocal and Shaw (2019). Upon review by the Nevada State Historic Preservation Office (SHPO) and internal review by Desert Research Institute (DRI) and NNSA/NFO staff, it was determined that these resources needed to be rerecorded and evaluated in relation to what appeared to be a National Register-eligible Historic District made up of the entirety of Area 12 Camp. Based on preliminary information, it appeared that all 11 resources would likely be contributing elements of that historic district. With that assumption in mind, recording of the entire proposed Area 12 Camp Historic District was done for three purposes. First, it would result in a definitive significance evaluation of the 11 resources in question. Second, recording of the entire camp would be offered as an appropriate mitigation measure for the demolition of these resources. Third, it would present an essential background for future management of resources within the district boundaries. Prior to the present survey, Area 12 Camp had not yet been systematically recorded; therefore, DRI surveyed an area of approximately 229 acres for architectural resources. This effort resulted in the identification, recording, and evaluation of the Area 12 Camp Historic District (SHPO Resource No. D372), including the identification of its contributing components. This district is recommended eligible for the National Register of Historic Places under Criteria A and C. It is unevaluated under Criteria B and D. The Area 12 Historic District contains 71 Principal Resources, which include landscapes, buildings, and structures. Of these resources, 69 (including 10 of the 11 resources to be removed) are recommended as contributing elements of the historic district during its period of significance corresponding to nuclear testing from 1960 through 1992. During most of the Cold War, the government reservation now called the NNSS was named the Nevada Test Site (NTS).

54 ENVIRONMENTAL SCIENCES↗

Photographic Mitigation Documentation Related to the Engine Assembly and Disassembly Facility, Area 25, Nevada National Security Site, Nye County, Nevada

This letter report provides documentation in partial fulfillment of the mitigation of adverse effects to the Engine Maintenance Assembly and Disassembly (E-MAD) facility, a major component of the Nuclear Rocket Development Station (NRDS) Historic District located in Area 25 of the Nevada National Security Site (NNSS). Construction of the E-MAD facility began in 1962 for the purpose of disassembling and maintaining nuclear-powered rocket engines. Once the building was complete in 1967, the E-MAD facility remained in continuous operation until the nuclear rocket program was terminated in 1973. The mothballed facility was repurposed in 1977 for spent nuclear fuel handling and packaging activities. By the mid-1980s, all activities at the E-MAD facility had ceased (Reno et al. 2019). This submission is intended to comply with Stipulation III.D.1 of the Memorandum of Agreement DE-GM58-20NA25534 between the U.S. Department of Energy and the Nevada State Historic Preservation Officer Regarding Corrective Action Activities and Demolition of the Engine Maintenance Assembly and Disassembly Facility and the Test Cell C Historic District, Major Components of the Nuclear Rocket Development Station Historic District Located in Area 25 at the Nevada National Security Site Nye County (hereafter referred to as the MOA). Stipulation III.D.1 states the U.S. Department of Energy (DOE) will submit the existing supplementary collection of the large-format, black-and-white photographic prints taken during the 1996 Historic American Engineering Record (HAER) documentation of the E-MAD facility to the Nuclear Testing Archive (NTA), located on the second floor of the Rogers Building at Desert Research Institute (DRI) in Las Vegas, Nevada.

54 ENVIRONMENTAL SCIENCES↗

Buster-Jangle

Buster-Jangle changed the working relationship between the AEC and the DoD. Beginning with Trinity and continuing through Greenhouse, the military was the logistical hub of nuclear testing, supplying men and material to carry out the myriad of mostly non-technical tasks. With the inclusion of the two Jangle tests and the Desert Rock exercises, that relationship became more symbiotic driven by the growing requirements for tactical weapons and their possible battlefield use. At Buster-Jangle, as well, the first use of a jet bomber was evidence that the military technology was evolving, requiring closer cooperation between the two agencies to match weapons and delivery systems.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

A shared mission: U.S. Navy members visit Los Alamos

During the week of Veteran’s Day (Nov. 8–11), Santa Fe was full of something we don’t see a lot here in the high desert — sailors! In honor of Santa Fe Navy Week, sailors and personnel from a number of U.S. Navy vessels, commands, and other programs visited Northern New Mexico to give residents an opportunity to learn about the U.S. Navy and its importance to national security. On Nov. 8, the Associate Laboratory Directorate of Weapons Production (ALDWP) invited a group of the U.S. Navy visitors up to Los Alamos to honor our shared mission.

99 GENERAL AND MISCELLANEOUS↗

Compilation and Evaluation of Data from Groundwater Impounded within the U12n and U12t Tunnels, Rainier and Aqueduct Mesas, Nevada National Security Site

The Department of Defense (DOD) Defense Threat Reduction Agency (DTRA) and the U.S. Department of Energy (DOE) Office of Environmental Management Nevada Program (EM NV) conducted routine physical and geochemical monitoring of water impounded behind impermeable structures placed within the U12n and U12t tunnels on the Nevada National Security Site (NNSS) (formerly the Nevada Test Site [NTS]). Desert Research Institute (DRI) conducted a semiquantitative evaluation of pressure data to determine the extent to which the tunnels have been inundated and a qualitative evaluation of monitored geochemical parameters to determine if trends exist that were indicative of hydrologic and/or geochemical processes operating behind the tunnel plugs. Data were also evaluated to determine if monitored radiological parameters exceeded primary standards associated with the Environmental Protection Agency’s (EPA) Safe Drinking Water Act (SDWA) (40 C.F.R. § 141.66).

54 ENVIRONMENTAL SCIENCES↗

Section 110 Documentation of a Douglas AD-2 Skyraider Crash Site, Area 1, Nevada National Security Site, Nye County, Nevada

The National Nuclear Security Administration, Nevada Field Office has undertaken a Section 110 current condition assessment of the unanticipated discovery of an aviation crash site in Nye County, Nevada. Because no undertaking is planned, an area of potential effect (APE) was not defined. A study area of 0.55 acres was established to delineate the general extent of the debris scatter and establish a boundary for the cultural resource documentation of the site by Desert Research Institute (DRI). The Douglas AD-2 Skyraider drone crash site (26NY17011) is recommended eligible for the National Register of Historic Places (NRHP) under Significance Criterion A, as a physical remnant of Project 5.1 “Atomic Weapons Effects on AD Type Aircraft in Flight,” one of the series of military effects studies conducted as part of Shot Simon during Operation Upshot-Knothole in 1953. Furthermore, the site is eligible under Criterion D because closer examination of the debris could address research questions concerning the Type 1 Remote Control Equipment developed by the Naval Air Experimental Station that was onboard to remotely pilot the aircraft.

54 ENVIRONMENTAL SCIENCES↗

Report Series: Evaluation, Finding of Effect, and Mitigation Documentation for the Main Gate (23-GS100), Mercury, Area 23, Nevada National Security Site, Nye County, Nevada

The U.S. Department of Energy (DOE) National Nuclear Security Administration Nevada Field Office (NNSA/NFO) plans to replace the existing guard shack at the Main Gate (23-GS100, Nevada State Historic Preservation Office [SHPO] Resource No. S1758) to the Nevada National Security Site (NNSS) in Nye County, Nevada. The purpose of the project is to improve security. The project is considered an undertaking subject to review under Title 54 of United States Code (USC) § 306108, commonly known as Section 106 of the National Historic Preservation Act, Title 54 USC § 300101, et seq., and its implementing regulations, Title 36 of the Code of Federal Regulations (36 CFR) Part 800. In 2018, Desert Research Institute (DRI) completed an architectural survey of the town of Mercury. This effort resulted in the identification, recordation, and evaluation of the Mercury Historic District (MHD, SHPO Resource No. D230), including the identification of its contributing elements (Reno et al. 2018). The MHD was recommended eligible for listing in the National Register of Historic Places (NRHP, National Register) under the Secretary of the Interior’s (SOI) Significance Criteria A and C, as defined in 36 CFR Part 60.4, as a significant concentration of buildings and structures with a direct and important association with Cold War-era nuclear testing from 1951 through 1992. It has not been evaluated under Criteria B and D to date. As part of a larger modernization program for Mercury, the NNSA/NFO and the SHPO executed the 2018 Programmatic Agreement between the National Nuclear Security Administration Nevada Field Office and the Nevada State Historic Preservation Officer regarding Modernization and Operational Maintenance of the Nevada National Security Site, at Mercury in Nye County, Nevada (Mercury PA). The Mercury PA includes streamlined Section 106 procedures for undertakings in the MHD based on contributing element categories. The Main Gate is identified in Appendix C of the Mercury PA as a Category I contributing element, indicating that it might be individually eligible for the NRHP. It is a historic property for the purposes of Section 106 compliance and subject to the stipulations of the Mercury PA. Per Stipulation VI of the Mercury PA, when the Area of Potential Effect (APE) for an undertaking includes Category I elements, the NNSA/NFO must evaluate the Category I elements for individual NRHP eligibility under all of the SOI Significance Criteria, prior to initiating any activity that may affect the elements. Thus, the purpose of this report is to evaluate the Main Gate as a potential individually eligible historic property in fulfillment of Stipulation VI of the Mercury PA. The evaluation detailed herein concludes that the Main Gate is individually eligible for listing in the NRHP under SOI Significance Criterion A at the national level of significance for its direct, important association with Cold War-era nuclear testing from 1965 (the date the current Main Gate was constructed) through 1992 (when critical nuclear testing on the NNSS ceased).

23-GS100↗

Big Hole Drilling Support for Nuclear Testing, 1985-1992: An Architectural Survey of the Area 1 Subdock, Nevada National Security Site, Nye County, Nevada

The U.S. Department of Energy, National Nuclear Security Administration Nevada Field Office (NNSA/NFO) planned to demolish two buildings at the Area 1 Subdock at the Nevada National Security Site (NNSS) in Nye County, Nevada, to meet environmental management mission requirements. A review was conducted under Title 54 United States Code (USC) § 306101 (commonly known as Section 106 of the National Historic Preservation Act) and its implementing regulations, 36 Code of Federal Regulations (CFR) Part 800. As a result, a Memorandum of Agreement (MOA) was developed to mitigate the effects of the building demolitions. Stipulation III.B of the MOA requires an architectural survey of the Area 1 Subdock. Prior to this survey, the Subdock had not been systematically recorded. Therefore, an area of approximately 33 hectares (81 acres) was surveyed for historic properties by Desert Research Institute personnel. This effort resulted in the identification, recording, and evaluation of the potential Area 1 Subdock Historic District (SHPO Resource No. D377), including the identification of its contributing components. This district is recommended as eligible for the National Register of Historic Places (NRHP) under Criteria A and C. It contains 14 primary resources which include individual buildings, structures, storage yards, and infrastructure. Of these resources, all except one are recommended as elements that contribute to the district during its period of significance corresponding to nuclear testing from 1985 through 1992. Four of the resources (B18847, B18848, S2772, S2773) are recommended as individually eligible for the NRHP.

54 ENVIRONMENTAL SCIENCES↗

Connecting the Radiative Influences of Aerosol upon the Mass Flux Profiles of Shallow Cumuli across the Southeast Atlantic Ocean Basin and its Boundaries (Final Report)

The Atlantic Ocean covers approximately 25% of Earth’s surface and the atmosphere above it is home to a complex array of clouds and aerosols that have important influences on regional and global weather and climate. These influences must be accurately depicted in short range, medium range, seasonal, and climate forecast models. Conditions over the tropical Atlantic are particularly complex due to continental scale plumes of dust from the Sahara Desert and smoke from agricultural burning in Africa that drift across the Atlantic Ocean basin toward the Americas. These plumes are often found meandering in the lower atmosphere above shallow tropical clouds that form above the ocean surface, presumably mingling with these clouds on occasion due to convective mixing processes. Elevated dust and smoke particles absorb incoming sunlight and substantially warm the marine atmosphere in the layer in which they are present. This warming may alter the thermal stability of the marine atmosphere and may throttle or enhance the development of clouds, change their internal structure and the rate at which they precipitate. Alternatively, it may isolate the lower atmosphere from drier layers above enabling water vapor to accumulate near the ocean surface potentially leading to the development of deeper convection. Our study was organized around the principal concept of determining the impact of African smoke and dust plumes upon cloud development at ASI and understanding how a popular shallow convection parameterization used in models responds to the presence of this aerosol. We analyzed observations collected during the US Department of Energy (DOE) Layered Atlantic Smoke Interactions with Clouds (LASIC) campaign using the Atmospheric Radiation Measurement Program’s Mobile Facility #1 (AMF-1), which was deployed to Ascension Island (ASI) in Southeastern Atlantic for a one-year period. Ascension Island is immediately downwind from an African source of these plumes, but far enough removed to enable the lower atmosphere to have reacted to their presence. A main goal of our study was to compute radiative heating rate profiles over Ascension Island and along the trajectory from the biomass burning regions along coastal Africa to Ascension Island. To compute the radiative heating rate due to aerosols and clouds, we employed observed profiles of temperature, humidity, and clouds from LASIC alongside aerosol optical properties from the Modern-era Retrospective analysis for Research and Applications Version 2 (MERRA-2), as input for the Rapid Radiation Transfer Model (RRTM). Radiative heating was also assessed across the southeast Atlantic Ocean using an ensemble of back trajectories from the Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model. We were successful in this effort and the resulting publication is already being cited despite its relatively short lifetime in the literature. The second part of our study involved the process-level representation of the clouds observed over the Southeastern Atlantic in models. Our initial task, upon which the balance of this portion of the study depended, was to evaluate the representativeness of the clouds observed by AMF-1. What orographic influence did Ascension Island have on the measured cloud structure? We set out to answer this question by trying to separate observations that were clearly indicative of orographic forcing from those that were representative of open ocean. The siting of AMF-1, which was 340-m above sea-level on the slope of a steep escarpment, proved demonstrably problematic for cloud process measurements. Despite considerable effort using multiple approaches including artificial intelligence (AI), we were unable to successfully compensate for the orographic forcing present at the AMF-1 site on ASI and, hence, produce process-level summaries of the convective mass flux representative of open ocean over the Southeastern Atlantic. Even though the project has officially ended, we are making a final attempt using two new types of clustering algorithm (i.e., AI) on the recommendation of a former student, who is an expert in this area. Since we have only recently begun to test these new AI schemes, the recommendations from the second part of our project outlined below are based on our experience at the time of this report.

54 ENVIRONMENTAL SCIENCES↗