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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 235 records · Page 13
All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

Hot electron preheat effects in two-photon polymerization plastic lattice laser-driven shock-tube experiments on the OMEGA laser

We present simulations of Omega shock tube experiments designed to investigate hot electron preheat effects in 3D-printed, two-photon polymerization (2PP) plastic lattices. Preheat is inferred in the experiments from the expansion of a plastic witness disk embedded in the lattice. Using the Eulerian radiation-hydrodynamics code xRAGE, we model shock propagation and preheat from both radiative and hot electron energy sources to evaluate their relative impact. To simulate the transport of laser-generated hot electrons, the nonlocal electron heat transport model proposed by Schurtz, Nicolaï, and Busquet (SNB) is extended with a hot electron source term and an energy cascade algorithm. We explore how variations in ablator, lattice geometry, and laser drive affect the shock velocity and witness disk expansion. Simulations show that the inclusion of a 5 μm gold layer reduces shock pressure by 60% and shock speeds by 30%–40% but does not significantly reduce the hot electron preheat, and that different lattice geometries lead to enhanced shock velocities—up to 40% faster than in homogeneous foams. However, radiative and conductive preheat from classical mechanisms alone fail to match experiment. By including a hot electron source term, we reproduce experimental observables such as disk expansion rates and spatial radiographic features. We find that a hot electron population corresponding to 4%–8% of the incident laser energy with T hot = 50 keV produces expansion which agrees with the experimental data, suggesting hot electron preheat is the most plausible explanation.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Effects of Proton Irradiation on GaN Vacuum Electron Nanodiodes

Gallium nitride (GaN)-based nanoscale vacuum electron devices, which offer advantages of both traditional vacuum tube operation and modern solid-state technology, are attractive for radiation-hard applications due to the inherent radiation hardness of vacuum electron devices and the high radiation tolerance of GaN. Here, we investigate the radiation hardness of top-down fabricated n-GaN nanoscale vacuum electron diodes (NVEDs) irradiated with 2.5-MeV protons (p) at various doses. We observe a slight decrease in forward current and a slight increase in reverse leakage current as a function of cumulative protons fluence due to a dopant compensation effect. The NVEDs overall show excellent radiation hardness with no major change in electrical characteristics up to a cumulative fluence of 5E14 p/cm 2 , which is significantly higher than the existing state-of-the-art radiation-hardened devices to our knowledge. In conclusion, the results show promise for a new class of GaN-based nanoscale vacuum electron devices for use in harsh radiation environments and space applications.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

Accurate and confident prediction of electron beam longitudinal properties using spectral virtual diagnostics

Abstract Longitudinal phase space (LPS) provides a critical information about electron beam dynamics for various scientific applications. For example, it can give insight into the high-brightness X-ray radiation from a free electron laser. Existing diagnostics are invasive, and often times cannot operate at the required resolution. In this work we present a machine learning-based Virtual Diagnostic (VD) tool to accurately predict the LPS for every shot using spectral information collected non-destructively from the radiation of relativistic electron beam. We demonstrate the tool’s accuracy for three different case studies with experimental or simulated data. For each case, we introduce a method to increase the confidence in the VD tool. We anticipate that spectral VD would improve the setup and understanding of experimental configurations at DOE’s user facilities as well as data sorting and analysis. The spectral VD can provide confident knowledge of the longitudinal bunch properties at the next generation of high-repetition rate linear accelerators while reducing the load on data storage, readout and streaming requirements.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Atomic-Scale Behavior of Radiation-Resistant ZnO under High-Energy Electron Bombardment

Understanding the atomic structure and defect characteristics of ZnO thin films is crucial for optimizing their electronic properties and performance in advanced applications. Here, we investigate the atomic structure and defect characteristics of atomic layer deposition (ALD)-grown ZnO thin films by using aberration-corrected scanning transmission electron microscopy (STEM). Atomic-resolution imaging identifies prevalent stacking faults, dipole disorder, and various grain boundary types, which are believed to influence the electronic properties of ZnO. Additionally, real-time electron beam exposure experiments demonstrate structural transformations, including crystal growth and surface rearrangements. These findings provide insights into the growth mechanisms of ALD ZnO under high-energy electron irradiation conditions, an important finding for the use of polycrystalline ZnO wide bandgap semiconductors in space-like conditions. In conclusion, our results underscore the capability of STEM in directly visualizing and quantifying atomic-scale defects and beam-induced transformations in radiation-resistant ZnO.

Defects↗
DOE OSTI2024

Experimental validation of a collision-radiation dataset for molecular hydrogen in plasmas

Quantitative spectroscopy of molecular hydrogen has generated substantial demand, leading to the accumulation of diverse elementary process data encompassing radiative transitions, electron-impact transitions, predissociations, and quenching. However, their rates currently available are still sparse, and there are inconsistencies among those proposed by different authors. In this study, we demonstrate an experimental validation of such a molecular dataset by composing a collisional-radiative model (CRM) for molecular hydrogen and comparing experimentally obtained vibronic populations across multiple levels. From the population kinetics of molecular hydrogen, the importance of each elementary process in various parameter space is studied. In low-density plasmas (electron density ne≲1017 m−3) the excitation rates from the ground states and radiative decay rates, both of which have been reported previously, determine the excited state population. The inconsistency in the excitation rates affects the population distribution the most significantly in this parameter space. However, in higher density plasmas (ne≳1018 m−3), the excitation rates from excited states become important, which have never been reported in the literature, and may need to be approximated in some way. In order to validate these molecular datasets and approximated rates, we carried out experimental observations for two different hydrogen plasmas; a low-density radio frequency heated plasma (ne≈1016 m−3) and the Large Helical Device (LHD) divertor plasma (ne≳1018 m−3). The visible emission lines from EF1Σg+, HH¯1Σg+, D1Πu±, GK1Σg+, I1Πg±, J1Δg±, h3Σg+, e3Σu+, d3Πu±,g3Σg+, i3Πg±, and j3Δg± states were observed simultaneously and their population distributions were obtained from their intensities. We compared the observed population distributions with the CRM prediction, in particular the CRM with the rates compiled by Janev et al., Miles et al., and those calculated with the molecular convergent close-coupling (MCCC) method. The MCCC prediction gives the best agreement with the experiment, particularly for the emission from the low-density plasma. However, the population distribution in the LHD divertor shows a worse agreement with the CRM than those from low-density plasma, indicating the necessity of the precise excitation rates from excited states. We also found that the rates for the electron attachment is inconsistent with experimental results. This requires further investigation.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Dose-Weighted Radiographic Source-Spot Size

The spatial resolution of a flash radiograph is determined by the time-integrated size of the radiation source. Since the radiation pulse includes the beam head and tail, which may be substantially larger than the beam body, the radiation source is larger than the focused flattop of the electron beam pulse. Moreover, the radiation dose rate is weighted by both beam current and electron energy, and it is the radiation dose that forms the radiograph image. Therefore, in order to estimate radiographic resolution from computer simulations of a focused electron beam, one should use a dose weighted moment analysis of the radiation source distribution. This approach is used to show that, in the absence of beam effects other than space-charge and emittance, radiographic resolution for Scorpius exceeds requirements, regardless of reasonable timing options for current and gap-voltage pulses.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Development of spatially and temporally resolved electron density measurements for the assessment of radiation hydrodynamics simulations of laboratory X-ray photoionized plasmas

The photoionized plasma gas cell experiment is an established platform we use to make at-parameter (ξ > > 1 ergs cm s –1 ) measurements of plasma properties with application to high-energy astrophysical systems. We model the experiments with 1D radiation hydrodynamics simulations using the HELIOS-CR code to inform our understanding and assist in the interpretation of results. The simulations predict that the bulk of the plasma is in a quasi-uniform and hydrodynamically unperturbed state throughout the duration of the experiment. To evaluate this prediction, we introduced a photonic Doppler velocimetry (PDV) diagnostic to measure spatially and temporally resolved plasma electron density. The initial measurements were successful but had limitations that made model-data comparisons challenging. To address this, we re-designed the gas cell PDV diagnostic and doubled the number of measurement locations to sample across two thirds of the depth of the cell. We also present a comparison of the results from the upgraded PDV diagnostic to the HELIOS-CR simulations for the first time. As a result, the experimental data confirms the prediction of an unperturbed region in the bulk of the plasma but reveals discrepancies in the time evolution and spatial distribution of the simulated electron density.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

Electron-mirror duality and thermality

Classical electromagnetic radiation from moving point charges is foundational, but the thermal dynamics responsible for classical acceleration temperature are poorly understood. We investigate the thermal properties of classical electromagnetic radiation in the context of the correspondence between accelerated electrons and moving mirrors, focusing on three trajectories with asymptotically infinite (Davies–Fulling), asymptotically zero (Walker–Davies), and eternally uniform acceleration. The latter two are argued not to be thermal, while the former is found to emit thermal photons with a temperature that depends on the electron’s speed. Thermal radiation occurs in the absence of jerk.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2026

Electron energy loss spectroscopy study of ceria sinters and nanoparticles irradiated with swift heavy ions

The electronic energy loss spectra of ceria (CeO 2 ) irradiated with swift heavy ions (27 MeV Xe and 946 MeV Au) in the electronic slowing down regime were measured for bulk sintered samples and nanoparticles by using a double Cs-corrected transmission electron microscope. The low-loss region as well as the core-loss region, including the oxygen K-edge and cerium M 4, 5 white lines, were recorded. No strong lattice disorder was found in the low-loss peaks for both types of samples showing the same bulk oxygen plasmon loss peak at about 15 eV. However, there is a clear evidence of cerium reduction to the trivalent oxidation state after irradiation for the sintered samples as shown by the K-edge shape of oxygen and decrease of the Ce M 4 /M 5 intensity ratio. A similar change of the M 4 /M 5 intensity ratio was observed for the irradiated nanoparticles with respect to the virgin sample owing to the high energy input inside the nanograin. The effect of radiation damage on electron energy loss spectroscopy data is analyzed for both types of samples and irradiation conditions.

Crystallographic defects↗
DOE OSTI2020

Response to Comment on “Radiation-Belt Remediation Using Space-Based Antennas and Electron Beams” by G. Ganguli and C. Crabtree

Ganguli and Crabtree have written a comment about a recent article by the authors listed above on radiation-belt remediation. They have objected to our evaluation of the Naval Research Laboratory’s chemical release concept which states that this concept may be impractical due to an apparently low overall efficiency. In their comment, they provide a scientific argument and refer to the published literature to counter our statement. Here, in this response, we provide more details on our numerical calculations and experimental results which led to this evaluation.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Ultrafast time-resolved 2D imaging of laser-driven fast electron transport in solid density matter using an x-ray free electron laser

High-power, short-pulse laser-driven fast electrons can rapidly heat and ionize a high-density target before it hydrodynamically expands. The transport of such electrons within a solid target has been studied using two-dimensional (2D) imaging of electron-induced Kα radiation. However, it is currently limited to no or picosecond scale temporal resolutions. Here, we demonstrate femtosecond time-resolved 2D imaging of fast electron transport in a solid copper foil using the SACLA x-ray free electron laser (XFEL). An unfocused collimated x-ray beam produced transmission images with sub-micron and ~10 fs resolutions. The XFEL beam, tuned to its photon energy slightly above the Cu K-edge, enabled 2D imaging of transmission changes induced by electron isochoric heating. Time-resolved measurements obtained by varying the time delay between the x-ray probe and the optical laser show that the signature of the electron-heated region expands at ~25% of the speed of light in a picosecond duration. Time-integrated Cu Kα images support the electron energy and propagation distance observed with the transmission imaging. The x-ray near-edge transmission imaging with a tunable XFEL beam could be broadly applicable for imaging isochorically heated targets by laser-driven relativistic electrons, energetic protons, or an intense x-ray beam.

47 OTHER INSTRUMENTATION↗
DOE OSTI2024

Photonuclear Physics in SCALE

Radiation shielding modeling involves a wide range of applications, such as power reactors, critical experiments, portable sources, linear accelerators, and fusion systems. Particle energy ranges vary from thermal energies to fast energy spectra. MAVRIC, as the radiation shielding sequence of the SCALE code system [1] developed and maintained by Oak Ridge National Laboratory, is capable of modeling both neutron and photon interactions in matter and is widely used by the US Nuclear Regulatory Commission, Department of Energy, the National Nuclear Security Administration, and radiation shielding practitioners all around the world. Although most applications don’t involve highly energetic photons that can cause photonuclear reactions and create coupled chains of high energy, ionized electrons and bremsstrahlung radiation within a material medium, when present, these reactions can have a significant impact upon the downstream particle fluxes from incident photons above 20 MeV. For example, linear accelerators used for medical isotope production are examples of applications in which high-energetic photons are generated and used for driving or controlling other components of a complex facility. Radiation shielding analyses of such a facility would require accounting for any and all significant sources of radiation. Unfortunately, MAVRIC included no data and methods to model either photonuclear reactions or the bremsstrahlung photons until this work, which enabled accounting for both. Photonuclear reaction cross sections were imported from the Evaluated Nuclear Data File libraries, and corresponding methods were implemented in the SCALE code system; see Section 2 for how the nuclear data are imported and used. Bremsstrahlung photons were modeled by assuming thick-target approximation whereby all generated electrons and positrons due to photon interactions are assumed to be absorbed within the same material in which they were born, yielding a quick particle transport simulation method by using fast lookup tables for generating subsequent gammas; see Section 4 for details. A suite of verification models was used to test implemented methods and associated data. Tests yielded satisfactory results for the new features. Enhancements will be released as part of the next major SCALE release (v7.0), which is anticipated to be deployed in 2025, with beta releases available in the interim.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Characterization of sub-picosecond laser-produced fast electrons by modeling angularly resolved bremsstrahlung measurements with 3D hybrid particle-in-cell code

Hard x-rays produced by intense laser-produced fast electrons interacting with solids are a vital source for producing radiographs of high-density objects and implosion cores for inertial confinement fusion. Accurate calculation of hard x-ray sources requires a three-dimensional (3D) simulation geometry that fully models the electron transport dynamics, including electron recirculation and the generation of absolute photon yields. To date, 3D simulations of laser-produced bremsstrahlung photons over tens of picoseconds and code benchmarking have not been performed definitively. In this study, we characterize sub-picosecond laser-produced fast electrons by modeling angularly resolved bremsstrahlung measurements for refluxing and non-refluxing targets using the 3D hybrid particle-in-cell (PIC), Large Scale Plasma code. Bremsstrahlung radiation and escaped electron data were obtained by focusing a 50-TW Leopard laser (15 J, 0.35 ps, 2 × 10 19 W/cm 2 ) on a 100-μm-thick Cu foil and a Cu with a large plastic backing (Cu–CH target). Data for both the Cu and Cu–CH targets were reproduced for simulations with a given set of electron parameters. Comparison of the simulations revealed that the hard x-ray emission from the Cu target was significantly longer in duration than that from the Cu–CH target. Here, the benchmarked hybrid PIC code could prove to be a powerful tool in the design and optimization of time- and angular-dependent bremsstrahlung sources for flash x-ray and gamma-ray radiography.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Optical Properties of Wigglers for EIC Ring Electron Cooler

Electron Ion Collider (EIC) requires cooling of protons at top energy (275 GeV) to achieve the average design luminosity. Such a cooler must be capable of counteracting an IBS-driven emittance growth in proton bunches. The Ring Electron Cooler (REC) is a candidate for the EIC top energy cooler. The REC is a non-magnetized RF-based 150 MeV electron cooler, in which electrons are kept in the storage ring and re-utilized for several million turns. The REC is equipped with 18 damping wigglers, which keep electrons’ emittance constant by counteracting both electrons’ IBS and a proton electron beam-beam scattering happening in the cooling section. These wigglers operate at a relatively low energy but must have a rather high field to provide the required radiation cooling of electrons. As a result of this unique range of parameters, the wigglers’ optics exhibits interesting features The actual design parameters of the wigglers will be finalized in the REC lattice optimization.

43 PARTICLE ACCELERATORS↗
DOE OSTI2025

Coherent frequency combs from electrons colliding with a laser pulse

Highly coherent and powerful light sources capable of generating soft x-ray frequency combs are essential for high precision measurements and rigorous tests of fundamental physics. In this work, we derive the analytical conditions required for the emission of coherent radiation from an electron beam colliding with a laser pulse, modeled as a plane wave. These conditions are applied in a series of numerical simulations, where we show that a soft x-ray frequency comb can be produced if the electrons are regularly-spaced and sufficiently monoenergetic. High quality beams of this kind may be produced in the near future from laser-plasma interactions or linear accelerators. Furthermore, we highlight the advantageous role of employing few-cycle laser pulses in relaxing the stringent monoenergeticity requirements for coherent emission. The conditions derived here can also be used to optimize coherent emission in other frequency ranges, such as the terahertz domain.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Traveling wakefield tube: THz source powered by nonrelativistic electron beam

High peak power, tunable, narrowband terahertz emitters are becoming sought after given their portability, efficiency, and ability to be deployed in the field for industrial, medical, and military applications. The use of accelerator systems producing THz frequencies via Cherenkov radiation, generated by passing an electron beam through a slow-wave wakefield structure, is a promising method to meet future THz requirements. To date, efforts have been dedicated to analysis and design of sources utilizing laser seeded bunched electron beam drivers with relativistic energies beyond 5 MeV. Presented here is a wakefield THz generation scheme based on passing a long quasi-dc nonrelativistic beam (200 keV) through a dielectric loaded travelling wave structure. Reduced energy allows for compactness and portability of the accelerator as the size and weight of the dielectric slow wave structure is vanishingly small compared to the accelerator unit. The presented scheme can serve as a tunable high peak power THz source operated between 0.4-1.6 THz and produces power gain by a factor of five with an average efficiency of 6.8%

43 PARTICLE ACCELERATORS↗
DOE OSTI2023

Energy Characterization of the UMD Electron Accelerator

Multiple different groups at Los Alamos National Laboratory have a cited interest in understanding the effects of ionizing radiation in materials. Of especial interest to the ISR division is understanding the effects in materials that are used in the space environment, where radiation is omnipresent and impossible to fully shield from. Development is under way to simulate the effects of radiation damage in detectors and electronics, primarily with particle transport codes such as Geant4 and RAMPART, a code that provides a user friendly interface to Geant4. However, these simulations need benchmarking to experimental tests, some of which have been performed at a variety of small electron accelerator facilities. One of these facilities is the Linear Electron Accelerator at the University of Maryland Radiation Facilities. This facility can provide electron beams on the order of 100 mA delivered in tight macropulse bunches, which allows for experiments where the behavior of electronics is monitored as a function of pulse number. While the beam rates per macropulse of this accelerator is monitored during an experiment via a current pick-off connected to a large graphite beamstop, the energy distribution of this electron beam is not measured during the experiment and has not been well characterized. The energy distribution of the beam is pertinent for these types of experiments, since dose is directly related to energy deposited in a medium. Further, these experiments are performed in open air and sample placement in the room can dictate what dose rate they receive per macropulse. We have created simulated dosemaps for the UMD vault room, but these simulations assume a given energy of the beam, both for calculating the dose and to simulate how much the beam diverges in the air. There have been two attempts now to characterize this accelerator beam energy with a plate type spectrometer, including the most recent experiment earlier this year to quantify the beam energy distribution. These results will also be compared to a dosimetry experiment performed by collaborators at the UMD facility, the details of which are described in Reference. Understanding the electron beam energy is important for future experiments, because the energy directly impacts the dose and radiation damage given to a sample and is important for properly simulating the electron beam when comparing simulation to experiment.

43 PARTICLE ACCELERATORS↗
DOE OSTI2026

Uranium Doped Gallium Nitride Epitaxial Thin Films

Gallium nitride (GaN) is near ubiquitous in modern day technologies, forming the backbone of solid-state lighting and high-power electronics. Engineering the physical properties of GaN has been investigated to some degree by the incorporation or doping of most of the elements of the periodic table, but the actinides remain unexplored. Molecular beam epitaxy is used to demonstrate uranium doping of GaN single crystals. High structural quality of the host matrix is maintained despite partial elemental segregation of the uranium dopant into 1D structures at the levels presented here. Electronic transport measurements reveal relatively high conductivity, which persists down to cryogenic temperature and is characterized by the formation of narrow gaps in the electronic band structures very close to the Fermi level. Photoluminescence measurements reveal that the U-doped GaN exhibits optical behavior similar to that of the GaN substrate. The addition of actinide materials to a non-centrosymmetric, optically active, radiation-hard, and electronically tunable host matrix opens a world of possibilities for investigating and leveraging elements with high electron correlations in the pursuit of novel devices.

36 - MATERIALS SCIENCE↗