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$\mathrm{UPDATED}$ $\mathrm{U3SI2}$ thermal creep model and sensitivity analysis of the $\mathrm{U3SI2-SIC}$ accident tolerant $\mathrm{FUEL}$

U 3 Si 2 is a candidate accident tolerant fuel (ATF) replacement for UO 2 . U 3 Si 2 ’s high uranium density and high thermal conductivity are favorable properties in steady-state and accident conditions. Low power performance of this U3Si2-SiC concept fuel is compared to that of UO 2 -Zr4 fuels by implementing models that describe the properties of U 3 Si 2 and SiC-SiC into Idaho National Laboratory's (INL) fuel performance code, BISON. Included in these material models is a thermal creep model for U 3 Si 2 based on compressive creep data. The simulated results are in keeping with community knowledge that the U 3 Si 2 -SiC concept fuel may serve as a replacement for UO 2 -Zr4 fuels during steady-state operation, provided the mSiC layer remains under compression. Through a moderate power history and three 24-month fuel cycles, the mSiC layer remains under compressive stress through a burnup of 80 MWd/kgU. During low power operation, failure of the mSiC layer generally occurs prior to significant thermal creep in U 3 Si 2 . Generally, U 3 Si 2 creep is temperature sensitive and of little importance at the temperatures and stresses simulated during steady operation and during fuel-to-cladding contact. A parameter variation study including 11,520 individual simulations with variations in nominal fuel thermal creep rate, cladding thermal conductivity, cladding irradiation creep and swelling, cladding gap size, and cladding thickness demonstrated that research priorities for this ATF should revolve around reducing cladding thickness as a means to minimize cladding failure. Generally, despite advances in SiC-SiC compliance, the brittle nature of mSiC excludes U 3 Si 2 -SiC for use where fuel cladding contact may occur.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

2022 Bioenergy Industry Status Report

This report provides a snapshot of the bioenergy industry status at the end of 2022. The report compliments other annual market reports from the Department of Energy's (DOE's) Office of Energy Efficiency and Renewable Energy (EERE) offices and is supported by DOE's Bioenergy Technologies Office (BETO). The 2022 Bioenergy Industry Status Report focuses on past year data covering multiple dimensions of the bioenergy industry and does not attempt to make future market projections. The report provides a balanced and unbiased assessment of the industry and associated markets. It is openly available to the public and is intended to compliment International Energy Agency and industry reports with a focus on DOE stakeholder needs.

09 BIOMASS FUELS↗

ANS Winter 2024 Summary: Optimizing the ATF-2Ramp Power Profile

When the Halden Boiling Water Reactor closed down in 2018, a need to restore the capability for in-reactor power ramp testing arose. Such testing is valuable for studying pellet-clad interaction phenomena in nuclear fuels. The data from these studies is of great interest to a number of research programs, including the accident-tolerant fuel (ATF) program at Idaho National Laboratory (INL). In 2022, Woolstenhulme et al. proposed several power ramp testing ideas using facilities at INL, including irradiation in the Transient Reactor Test Facility (better known as TREAT) and the Advanced Test Reactor (ATR) [1]. Worrall et al. [2] and Labossiere-Hickman et al. [3] subsequently performed feasibility studies for the ATR testing options in 2023. This summary further investigates the three-pin trefoil design (Fig. 1) for the proposed ATF-2Ramp Experiment discussed in Labossiere-Hickman et al. [3]. ATF-2Ramp is designed to operate in the center flux trap (CFT) of the ATR during a powered axial locator mechanism (PALM) cycle: a short, variable-powered cycle with an asymmetric power distribution. Previously, it was shown that tailoring the thickness of the hafnium (Hf) neutron shields (“mini-shrouds”) surrounding each pin offered a degree of control sufficient to achieve the programmatic linear heat generation rate (LHGR) targets for ATF-2Ramp during the high-power period of a PALM cycle. New work involves shortening the experiment test train for consistency with the fuel pins in ATF-2D [4] and then shaping the axial power profile of the three test pins.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Fuel performance uncertainty quantification and sensitivity analysis in the presence of epistemic and aleatoric sources of uncertainties

Fuel performance modeling and simulation includes many uncertain parameters from models to boundary conditions, manufacturing parameters and material properties. These parameters exhibit large uncertainties and can have an epistemic or aleatoric nature, something that renders fuel performance code-to-code and code-to-measurements comparisons for complex phenomena such as the pellet cladding mechanical interaction (PCMI) very challenging. Additionally, PCMI and other complex phenomena found in fuel performance modeling and simulation induce strong discontinuities and non-linearities that can render difficult to extract meaningful conclusions form uncertainty quantification (UQ) and sensitivity analysis (SA) studies. In this work, we develop and apply a consistent treatment of epistemic and aleatoric uncertainties for both UQ and SA in fuel performance calculations and use historical benchmark-quality measurement data to demonstrate it. More specifically, the developed methodology is applied to the OECD/NEA Multi-physics Pellet Cladding Mechanical Interaction Validation benchmark. A cold ramp test leading to PCMI is modeled. Two measured quantities of interest are considered: the cladding axial elongation during the irradiations and the cladding outer diameter after the cold ramp. The fuel performance code used to perform the simulation is FAST. The developed methodology involves various steps including a Morris screening to decrease the number of uncertain inputs, a nested loop approach for propagating the epistemic and aleatoric sources of uncertainties, and a global SA using Sobol indices. The obtained results indicate that the fuel and cladding thermal conductivities as well as the cladding outer diameter uncertainties are the three inputs having the largest impact on the measured quantities. More importantly, it was found that the epistemic uncertainties can have a significant impact on the measured quantities and can affect the outcome of the global sensitivity analysis.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Destructive Examination of a FeCrAl-UO 2 Irradiation Test

Several destructive postirradiation examinations were performed on an irradiation specimen that coupled an early iron-chromium-aluminum (FeCrAl) candidate alloy cladding with UO2 pellets. This irradiation test was designed to investigate the early life performance and compatibility of the FeCrAl-UO 2 cladding-fuel system under prototypic light water reactor neutronic conditions. Additionally, these tests were expected to provide neutron irradiated samples for severe accident testing of this fuel system. The irradiation studied in this work was part of the ATF-1 series of drop-in style irradiations performed in the Idaho National Laboratory Advanced Test Reactor. The rodlet studied in this work is one of three similar rodlets irradiated in ATF-1 that had approximately 7.6 cm of cladding machined from a wrought FeCrAl alloy and fueled with a 6.1 cm stack of UO 2 pellets. The outer diameter of the cladding was ~0.94 cm and the inner diameter was ~0.83 cm. After irradiation and non-destructive examination in Idaho this rodlet was shipped to the Oak Ridge National Laboratory hot-cells for further examination. The irradiated rodlet was sectioned into several samples for microstructural, micromechanical, and severe accident testing. During sectioning, it was noted that the fuel was not firmly bonded to the cladding and could be readily removed from small cladding slices. Microstructural characterization of fuel cross sections also revealed no significant interaction between the fuel and the cladding. Samples were also prepared for microhardness testing. To prepare for high temperature oxidation testing, the fuel was dissolved from segments of the cladding. High temperature oxidation testing of cladding segments was performed at 1200°C and 1300°C in a steam environment. Comparisons between the oxidation of this FeCrAl alloy in its neutron irradiated state, as-fabricated state, and the oxidation of Zircaloy-2 are made. The oxidation testing will be followed by ring compression testing to evaluate ductility. The microstructure of the samples after oxidation and ring compression testing will also be analyzed.

Harp, Jason↗

Energy-based break-even transportation distance of biomass feedstocks

The distance a solid biomass feedstock could be used to transport the feedstock when used as biobased fuel is critical information for transportation analysis. However, this information is not available. The break-even transportation distance (BTD) of various fuels from biomass feedstocks and fossil sources was analyzed for truck, rail, and ship transport modes based on bulk density, moisture content, and specific energy. Fourteen different biomass feedstocks, such as crop residues (e.g., corn stover), woody biomass (e.g., wood chips), including thermally pretreated (torrefied) and densified forms (pellets), cattle feedlot compost, and three standard fossil fuels, namely, coal, lignite, and diesel, were considered for BTD analysis and comparison. The BTD values were derived by comparing the energy content of biomass feedstocks with the energy expended in transporting the fuels through selected transportation modes. For ready reference, an alternative derivation of BTD equations and example calculations were also presented. Among the biomass feedstocks, torrefied pellets had the highest BTD (4.16 × 10 4 , 12.47 × 10 4 , and 54.14 × 10 4 km), and cattle feedlot compost had the lowest BTD (1.29 × 10 4 , 3.88 × 10 4 , and 9.23 × 10 4 km), respectively, for truck, rail, and ship. Higher bulk density and higher specific energy of the biomass feedstocks increased the BTD for all modes of transport. Transport is most efficient when mass-limited. Biomass feedstock bulk densities where transportation becomes mass-limited are 223, 1,480, and 656 kg/m 3 for truck, rail, and ship, respectively. Truck transport is typically mass-limited (payload limit restriction; increased BTD), whereas rail transport is entirely volume-limited (cargo space restriction; decreased BTD), and ship transport is mostly volume-limited for biomass feedstocks and mass-limited for densified biomass feedstocks. Ship transport is the most efficient, followed by rail and truck; on average for the materials (17) studied, rail is 3.1 times and ship is 9.2 times the truck's BTD. Based on the bulk density and higher specific energy of the biomass feedstocks, regardless of the refinery location, interstate truck transport of these feedstocks is not a limiting factor in the bio-refining process., with the studied biomass feedstock BTD per truckload representing between 0.89 and 2.88 times the US perimeter.

09 BIOMASS FUELS↗

Study of solid molecular deuterium D 2 growth under gas pressure

The injection of high-speed cryogenic pellets made of frozen hydrogen-isotopes, represents to date the most effective method to fuel magnetically confined thermonuclear fusion plasmas. Additionally, the injection of very large pellets composed of cryogenic solid of some suitable impurity (typically a noble-gas such as H 2 , Ne, or H 2 /Ne, D 2 /Ne mixtures), shattered in relatively small fragments just before entering the plasma, seems to be the most promising method to reduce the damage risks for the plasma-facing components in case of a plasma disruption. This technology, known as "Shattered Pellet Injection" (SPI), allows to spread out the plasma energy and mitigate possible damage to the in-vessel components, as well as to densify the plasma to suppress the formation of runaway electrons, and/or dissipate their energy. Several techniques to produce and launch cryogenic pellets have been investigated in the past decades. "Pipe gun" injectors are reliable and relatively simple devices are still commonly used today. They make use of single- or two-stage pneumatic light-gas guns to accelerate the pellet at high speeds. In these injectors, the cryogenic pellets are formed “ in situ ” (i.e., inside the launching barrel), by de-sublimating them directly from the gas phase, i.e., at temperatures and pressures below those of the triple point. The simplest case is pure deuterium pellets ($\mathcal{T}$ < 18.7 K, $\mathcal{P}$ < 171.3 hPa). The production of good quality solid deuterium, capable of withstanding the mechanical stress during the acceleration of the pellets, is a key issue. To this end the phase transition of deuterium from gas to solid (and vice versa) is modeled with extensive molecular-dynamics (MD) simulations. Furthermore, the solid growth from the gas phase is simulated in an ample range of temperatures and pressures, to find the best compromise between growth velocity and mechanical properties of the resulting solid system.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Development of advanced vacuum technologies for extending plasma pulse duration on EAST

Advanced vacuum technologies, including pumping, fueling and wall conditioning, have been successfully developed or upgraded to efficiently control the fuel and impurity particles to extend the plasma pulse duration in the experimental advanced superconducting tokamak (EAST). To improve the particle exhaust rate cryopumps with a 60% increase in pumping speed and ∼2 times increase in saturation capacity have been developed, and molecular pumps with a ∼30% increase in pumping speed have been upgraded. In order to monitor the molecular pump status while avoiding bearing faults and overload accidents, a fault detection system has been built which can offer an early warning to avoid more losses within the fusion device. A series of fueling technologies have been developed including gas injection system, supersonic molecular beam injector, pellet injector (PI), massive gas injector and shattered pellet injector, installed at the midplane and divertor positions at different ports to improve fueling uniformity and efficiency. Meanwhile, routine wall conditioning such as electric and hot N 2 baking, ion cyclotron wall conditioning and glow discharge cleaning have been successfully developed to remove the impurity particles from the inner component and materials. The low Z material wall coating and real-time powder injection during plasma discharge are also designed and applied to further improve particle control capability. Finally, by using these advanced vacuum related technologies, good vacuum (<2 × 10 −6 Pa) and wall conditions are realized, and the fuel and impurity particles can be effectively and stably controlled, which promotes the achievement of the record plasma of ∼1056 s pulse duration with the line-averaged electron density of 1.8 × 10 19 m −3 on EAST. They provide a very important reference for vacuum system design and operation for future fusion devices.

EAST↗

FCIC DFO--Moisture Management and Optimization in Municipal Solid Waste Feedstock through Mechanical Processing

The project goal is to produce densified product, focusing on characteristics of bulk density, durability, and moisture content, to reduce the cost of preprocessing. The objective of the project is to efficiently manage and handle the properties of MSW feedstock through INL-developed fractional milling, high moisture pelleting, and low temperature drying preprocessing technologies .

09 BIOMASS FUELS↗

Mechanical Response of Cr-Coated Zircaloy-4 Cladding to Pellet-Cladding Interactions

Chromium-coated zircaloy is a promising accident tolerant fuel (ATF) cladding design which can help mitigate high temperature oxidation. The mechanical response of the cladding during and after loading may be altered by the Cr coating throughout anticipated operational and accident occurrences such as a pellet-cladding interaction (PCI). In this work, the mechanical behavior of Cr-coated and uncoated cold worked stress-relieved (CWSR) Zircaloy-4 (Zry-4) cladding to PCI loading conditions are studied. Stress relaxation tests are performed on CWSR Zry-4 cladding using full-tube axial tension and internal pressurization to investigate mechanical anisotropy and rate-limiting deformation mechanisms of the uncoated Zry-4. These results are compared to internal pressure testing results of similar cladding with physical vapor deposition (PVD) Cr-coating to reveal how the Cr-coating affects the cladding mechanical response. Findings are discussed in the context of ATF cladding performance during operation and storage.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Biochemical Conversion of Herbaceous Biomass to Renewable Diesel: Biorefinery Marginal Air Quality Impacts and Comparison to Feedstock Production

This study assesses the air quality impacts of an advanced biorefinery that produces renewable diesel blendstock (RDB) from lignocellulosic biomass via aerobic respiration (Davis et al. 2022) by estimating fine particulate matter (PM2.5) impacts from biorefinery emissions. It continues a prior analysis that used a geospatial assessment to identify source regions for biomass feedstocks and studied the impact of feedstock production emissions on air quality (Thind et al. 2022). Thind et al. (2022) identified RDB biorefineries that can use corn stover feedstocks of 2,000; 5,200; and 9,100 dry metric tons per day (DMT/day), based in Iowa, and suggested 7 unique counties can serve as hosts for a biorefinery that draws biomass feedstock from neighboring counties. Given 13 unique county-biorefinery size combinations and two waste lignin end uses at the biorefinery (lignin as a fuel for electricity generation and lignin for pellet production), the air-quality-related sustainability aspects of each of these 26 scenarios are assessed by estimating the annual average impacts of biorefinery emissions on the dispersion and formation of secondary PM2.5 in the atmosphere using a novel reduced-complexity air quality model called the Intervention Model for Air Pollution (InMAP). The 26 biorefinery design combinations help capture how a biorefinery's emissions of air pollutants and their resulting impact on local and regional air quality are influenced by the magnitude of production scale, lignin utilization strategy, and location of a proposed biorefinery. Methods developed in Thind et al. (2022) are applied to estimate the constraints on primary PM2.5 and secondary PM2.5 precursor emissions based on compliance with U.S. Environmental Protection Agency's (EPA's) annual primary National Ambient Air Quality Standard (NAAQS) of PM2.5 (i.e.12.0 micrograms per cubic meter (microgram/m3)) at downwind receptors of a biorefinery. Incremental PM2.5 concentrations caused by the emission of biorefining corn stover into RDB are assessed and compared to those of corn stover production. To illuminate which upstream supply chain stage of renewable diesel production contributes most to air quality impacts, marginal PM2.5 concentrations are compared between both stages at multiple downwind air quality monitor locations. In addition, through a hotspot analysis, we identify the primary contributing factors of emissions within the feedstock production and biorefinery stage operations. In doing so, we provide insights for improving the air pollutant emission-related sustainability of advanced lignocellulosic biofuel production.

09 BIOMASS FUELS↗

Fuel Behavior Implications of Reactor Design Choices in Pressurized Water SMRs

Small pressurized water reactors (PWRs) can feature boron free operation, natural circulation mode, reduced height assemblies and/or long refueling cycles. This paper attempts to explore core design optimization for each of these design evolutions. In consequence, five core design layouts are developed incorporating boron free operation with continuous control rods insertion, natural circulation with low burnup/low power density design, natural circulation with high burnup/low power density design, forced circulation with standard core power density design, and forced circulation with high power density design. These cores’ performance is compared to a standard 4-loop PWR. The design process aims to improve the fuel cycle cost under safety constraints through core design optimization using CASMO4E/SIMULATE3 reactor physics codes and FRAPCON4.1 fuel performance assessment tool. Core modeling assumes standard 17x17 PWR fuel assemblies loaded with low enriched uranium (LEU) up to 5wt% or LEU+ (i.e., below 10wt% enrichment) pellets with gadolinium oxide (Gd2O3) as the burnable poison. Satisfactory core and fuel performances are obtained for all the designed cores under steady state and considered overpower transients. For low power density operation, long cycle lengths are achieved reaching a 2.5- and a 5-year cycles and peak rod-average burnup is pushed to 83 MWd/kgU. Other cycle lengths are maintained at 18 months. Boron free operation exhibits the ability to achieve longer cycle lengths at the cost of higher peaking factors leading to high local power and fuel temperatures which prevents sizable power uprates and is deemed uneconomical. Fuel assembly height reduction allows coolant velocity retrofit which enables higher core power density without violating structural integrity of the fuel assembly. As a result, a core power density of 123 kW/l is reached where total cladding hoop strain becomes the limiting parameter.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Portuguese Wood Pellets Market: Organization, Production and Consumption Analysis

Wood pellets are a form of energy that can be seen as an alternative to fossil fuels, thus contributing to the reduction of greenhouse gas emissions. In other words, wood pellets can be considered a solution contributing to the mitigation of climate change. The use of wood pellets has grown significantly in recent years, with different markets emerging, such as Portugal, both from production and consumption perspectives. The wood pellet industry in Portugal began its development about 15 years ago, with the companies installed in the country initially almost exclusively dedicated to the production of wood pellets for export to central and northern European markets. However, over the years, the domestic market, initially considered insignificant, began to develop; it recently reached a considerable consuming share of the national production. This study presents an analysis of the Portuguese wood pellet market using data collected on the sector, and specifically on producers and consumers. The information was gathered using surveys presented directly to consumers and producers and through interviews with other stakeholders in the sector. From the analysis of the information, it was possible to understand the market’s dynamics, its current evolution and its prospects for the upcoming years, since it can already be considered mature and consolidated.

Nunes, Leonel J. R. (ORCID:0000000154048163)↗

Fuel Performance Calculations of Tagged UO 2 MiniFuel Disks

Isotopic taggants are being considered as a novel form of forensic identifiers for nuclear fuels. As part of this effort, eighteen tagged MiniFuel disks were irradiated in the High Flux Isotope Reactor at Oak Ridge National Laboratory. In this work, the BISON fuel performance code was used to recreate the pellets and predict their behavior and their post-irradiation material properties. These predictions are to serve as a baseline to help investigators identify results of interest during post-irradiation examination of actual MiniFuel disks. The simulation methodology and models are described herein, along with the individual disk predictions. Several general trends were identified in this analysis. Based on the models, it is predicted that the pellets’ internal temperatures will rise over time, fission gas release will remain constant at around 1%, regardless of the burnup, and no grain growth will occur in any of the disks. The reasons for these predictions are discussed below. Probable shortcomings in the BISON predictions are addressed, and future work is proposed.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

High temperature mechanical properties of fluorite crystal structured materials (CeO 2 , ThO 2 , and UO 2 ) and advanced accident tolerant fuels (U 3 Si 2 , UN, and UB 2 )

The mechanical interaction between the fuel and cladding that occurs during operation of a nuclear reactor is important to understand as it can lead to cladding failures and release of radioactive material into the coolant. Additionally, in order to develop better models of the pellet-clad mechanical interactions, the mechanical properties of the fuel at relevant operating temperatures, like the elastic moduli, are needed for current and advanced accident tolerant fuels (ATFs). In this work, elevated temperature nanoindentation and resonant ultrasound spectroscopy were used to measure the moduli and hardness of several fluorite materials (CeO 2 , ThO 2 , UO 2 ) and several ATF candidates (ATF) (U 3 Si 2 , UN, UB 2 ). In addition, a comparison of the two techniques was performed in this study to independently validate the mechanical properties.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Detailed characterization of a PWR fuel rod at high burnup in support of LOCA testing

Experimental investigations of the fuel microstructure and volatile fission products along the pellet of a high burnup specimen (local burnup 76 GWd/tHM) have been conducted to support future transient testing. Detailed microscopy examinations have been carried out at different length scales. Transmission electron microscopy has highlighted a significant amount of damage across the entire radius with the formation of networks of dislocations. The optical and scanning electron microscopy determined the formation of three zones in the pellet with different characteristics. An intermediate region with no grain subdivision, lower porosity than the central zone porosity and high retained fission gas in nanometric bubbles and in the matrix was present between r/r0 ˜ 0.55 and 0.8. The high retention of gas in this region might suggest that the region will be prone to fine fragmentation, in addition to the HBS. An abrupt transition in the structure was observed at mid radius, with a third region developing from the mid radius to the pellet center. In this part of the pellet, metallic and grey phases with size between hundreds of nanometers and a few micrometers have formed at grain boundaries. The majority of fission gas has been released from the grain matrix and the original grains have polygonised, forming sub-grain domains separated by low-angle grain boundaries. No final explanation can be given for the polygonization occurring in the center, but on the basis of the irradiation history and the analysis of all the post irradiation examination (PIE) data, it is postulated that the polygonization within the original grains is an effect of dynamic recovery occurring at high temperature in the fuel center.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Report on RIA Relevant Modified Burst Testing of ATF Cladding Materials

The mechanical performance of accident-tolerant fuel (ATF) cladding candidates in light-water reactors (LWRs) must be similar to or better than that of current conventional nuclear fuel claddings to reduce dose to the public and ensure a that the core coolable geometry is maintained during a postulated reactivity-initiated accident (RIA) in light-water reactors (LWRs). During an RIA event, the rapid thermal expansion of nuclear fuel can deform the cladding once the fuel–cladding gap closes. In some cases, the pellet–cladding mechanical interaction (PCMI) can induce mechanical failure in ATF candidates. Thus, the mechanical response of ATF cladding must be investigated by mimicking the conditions of RIA and potentially performing Transient Reactor Test (TREAT) experiments to establish or verify the safety envelope. The work presented in this report investigated the failure behavior of as-received, hydrided, and chromium-coated (Cr-coated) Zircaloy-4 (Zry-4) cladding tube under strain-driven mechanical conditions, mimicking postulated RIA loading conditions. Mechanical testing was performed at 300°C via modified burst test (MBT) equipment with pulse width control previously developed under the Department of Energy’s (DOE’s) Advanced Fuel Campaign (AFC). The mechanical strains were determined using 2D digital image correlation (DIC) techniques. The base Zry-4 acquired by Cameco Inc. was in stress-relieved annealed (SRA) condition. Because of the observed large deformation of the cladding tubes, the failure strain definition was updated for the MBT, which can also be applied to other tube tests where significant bulging (out-of-plane deformation) is present. The failure strain was determined to be affected by the speed of the test or the RIA event. As the RIA-like event duration decreased from 75 to 15 ms, the failure strain decreased 5, 7 and 1% for as-received, hydrided, and Cr-coated specimens, respectively. Fractography on the Cr-coated specimens indicated the presence of two failure mechanisms: (i) crenulation at the outer surface of the coating due to the tensile tractional forces along with coatings grain microstructure and (ii) formation of critical defect at the coating/cladding interface that initiated coating rupture after severe plastic deformation of the Zry- 4 substrate. Based on the MBT results and fractography observations, performing mechanical property testing at high strain rates—in particular on Cr-coated tubes—and semi-integral TREAT experiments are required future efforts to ensure ATF cladding performance during transients. The testing recommended would also inform the development of long-term generalized cladding technologies.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Transient fuel performance analysis for the preliminary fuel concept of general atomics fast modular reactor

This study investigates the transient fuel performance of General Atomics Fast Modular Reactor (GA-FMR) during accident scenarios, focusing on the behavior of its innovative fuel system that combines high-assay low enriched uranium dioxide (HALEUO2) fuel with SiGA® ceramic matrix composite silicon carbide cladding. The preliminary fuel design’s response was analyzed during reactivity-initiated accidents (RIA) and loss of coolant accidents (LOCA) using BISON fuel performance analysis code, which included both the diffusion enhanced and BISON-FASTGRASS coupled UO 2 models. The RIA analysis demonstrated that effective reactivity control reduced fuel temperature, though with transient fission gas release resulting in additional tensile stress state on the cladding. LOCA simulations revealed differing predictions between the two models: the BISON UO 2 model showed more transient fission gas release but minimal pellet expansion, while the BISON-FASTGRASS UO 2 model predicted less pronounced fission gas release but more fuel swelling and thermal expansion, potentially leading to pellet-cladding mechanical interaction. Here, these findings highlight critical areas for fuel design optimization and identify knowledge gaps requiring further experimental and computational investigation to advance GA-FMR fuel development.

Lee, Soon K. [Argonne National Laboratory (ANL), A↗