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NASA NTRS1994

Laboratory Comparisons of Organic Materials to Those Observed in the Interstellar Medium

Spectra of objects which lie along several lines of sight through the diffuse interstellar medium (ISM) all contain an absorption feature near 3.4 Pm which has been attributed to saturated aliphatic hydrocarbons on interstellar grains. The similarity of the absorption bands near 3.4 microns (2950 /cm) along different lines of sight reveal that the carrier of this band lies in the diffuse dust. Several materials have been proposed as "fits" to the 3.4 microns feature over the years. A comparison of these identifications is presented. A remarkable similarity between the spectrum of the diffuse dust and an organic extract from the Murchison meteorite suggests that some of the interstellar organic material may be preserved in primitive solar system bodies. Recent detections of the hydrocarbon absorption feature in external galaxies are presented. These results indicate the widespread availability of the organic material for incorporation into planetary systems. Recent detections of the X-CN absorption feature in dense molecular clouds are also presented. The preliminary results suggest that the X-CN band is only observed toward embedded sources and is not distributed throughout the molecular cloud. If so, this has profound effects on the production mechanism of this component of the organic material in space.

Pendleton, Yvonne J.↗
DOE OSTI2021

Alignment of the magnetic field in star-forming regions and why it might be difficult to observe

ABSTRACT Magnetic fields are an important component of the interstellar medium (ISM) and exhibit strongly varying field strengths and a non-trivial correlation with the gas density. Its dynamical impact varies between individual regions of the ISM and correlates with the orientation of the field with respect to the gas structures. Using high-resolution magneto-hydrodynamical simulations of the ISM, we explore the connection between the orientation of the field and the dynamical state of the gas. We find that the onset of gravitational instability in molecular gas above a density of $\rho \sim 10^{-21}\, \mathrm{g\, cm}^{-3}$$(n\sim 400\, \mathrm{cm}^{-3})$ coincides with an alignment of the magnetic field lines and the gas flow. At this transition, the gradient of the density changes from mainly perpendicular to preferentially parallel to the field lines. A connection between the three-dimensional alignment and projected two-dimensional observables is non-trivial, because of a large dispersion of the magnetic field orientation along the line of sight. The turbulent correlation lengths can be small compared to the typical integration lengths. As a consequence, the small-scale signal of the orientation can sensitively depend on the line of sight or the dynamical state of the cloud can fluctuate stochastically or be completely averaged out. With higher spatial resolution more small-scale structures are resolved, which aggravates the link between magneto-hydrodynamical quantities and projected observables.

Girichidis, Philipp (ORCID:0000000293009914)↗
NASA NTRS1993

AGB stars as a source of short-lived radioactive nuclei in the solar nebula

The purpose is to estimate the possible contribution of some short-lived nuclei to the early solar nebula from asymptotic giant branch (AGB) sources. Low mass (1 to 3 solar mass) AGB stars appear to provide a site for synthesis of the main s process component for solar system material with an exponential distribution of neutron irradiations varies as exp(-tau/tau(sub 0)) (where tau is the time integrated neutron flux with a mean neutron exposure tau(sub 0)) for solar abundances with tau(sub 0) = 0.28 mb(sup -1). Previous workers estimated the synthesis of key short-lived nuclei which might be produced in AGB stars. While these calculations exhibit the basic characteristics of nuclei production by neutron exposure, there is need for a self-consistent calculation that follows AGB evolution and takes into account the net production from a star and dilution with the cloud medium. Many of the general approaches and the conclusions arrived at were presented earlier by Cameron. The production of nuclei for a star of 1.5 solar mass during the thermal pulsing of the AGB phase was evaluated. Calculations were done for a series of thermal pulses with tau(sub 0) = 0.12 and 0.28 mb(sup -1). These pulses involve s nucleosynthesis in the burning shell at the base of the He zone followed by the ignition of the H burning shell at the top of the He zone. After about 10-15 cycles the abundances of the various nuclei in the He zone become constant. Computations of the abundances of all nuclei in the He zone were made following Gallino. The mass of the solar nebula was considered to consist of some initial material of approximately solar composition plus some contributions from AGB stars. The ratios of the masses required from the AGB He burning zone to the ISM necessary to produce the observed value of Pd-107/Pd-108 in the early solar system were calculated and this dilution factor was applied to all other relevant nuclei.

Wasserburg, G. J.↗
NASA NTRS2014

High-Energy X-Ray Detection of G359.89-0.08 (SGR A-E): Magnetic Flux Tube Emission Powered by Cosmic Rays?

We report the first detection of high-energy X-ray (E (is) greater than 10 keV) emission from the Galactic center non-thermal filament G359.89−0.08 (Sgr A−E) using data acquired with the Nuclear Spectroscopic Telescope Array (NuSTAR). The bright filament was detected up to approximately 50 keV during a NuSTAR Galactic center monitoring campaign. The featureless power-law spectrum with a photon index gamma approximately equals 2.3 confirms a non-thermal emission mechanism. The observed flux in the 3-79 keV band is F(sub X) = (2.0 +/- 0.1) × 10(exp -12)erg cm(-2) s(-1) , corresponding to an unabsorbed X-ray luminosity L(sub X) = (2.6+/-0.8)×10(exp 34) erg s(-1) assuming a distance of 8.0 kpc. Based on theoretical predictions and observations, we conclude that Sgr A−E is unlikely to be a pulsar wind nebula (PWN) or supernova remnant-molecular cloud (SNR-MC) interaction, as previously hypothesized. Instead, the emission could be due to a magnetic flux tube which traps TeV electrons. We propose two possible TeV electron sources: old PWNe (up to (is) approximately 100 kyr) with low surface brightness and radii up to (is) approximately 30 pc or MCs illuminated by cosmic rays (CRs) from CR accelerators such as SNRs or Sgr A*.

X-rays: individual↗
NASA NTRS1995

Interstellar Dust Connections to Interplanetary Dust

The organic component of the interstellar medium, which has revealed itself through the ubiquitous 3.4 micrometer hydrocarbon absorption feature, is widespread throughout the disk of our galaxy and has been attributed to dust grains residing in the diffuse interstellar medium. The absorption band positions near 3.4 micrometers are characteristic of C-H stretching vibrations in the -CH3 and -CH2- groups of saturated aliphatic hydrocarbons associated with perturbing chemical groups. The production of complex molecules is thought to occur within dense molecular clouds when ice- mantled grains are processed by various energetic mechanisms. Studies of the processing of interstellar ices and the subsequent production of organic residues have relevance to studies of interplanetary dust, because primitive solar system bodies are likely reservoirs of organic material, either preserved from the interstellar medium or produced in situ. A comparison of the interstellar organics and the Murchison meteorite illustrates the importance of probing the interstellar connection to the solar system, because although the carbonaceous meteorites are undoubtedly highly processed, they do retain specific interstellar signatures (such as diamonds, SiC grains, graphite and enriched D/H). The organic component, while not proven interstellar, has a remarkable similarity to the interstellar organics observed in over a dozen sightlines through our galaxy. This paper compares spectra from laboratory organics produced through the processing of interstellar ice analog materials with the high resolution infrared observations of the interstellar medium in order to investigate the mechanisms (such as ion bombardment, plasma processing, and UV photolysis) that may be producing the organics in the ISM. Comparisons to interplanetary dust particles, comets, and meteorites are discussed.

Pendleton, Y. J.↗
NASA NTRS2013

On the Ubiquity of Molecular Anions in the Dense Interstellar Medium

Results are presented from a survey for molecular anions in seven nearby Galactic star-forming cores and molecular clouds. The hydrocarbon anion C6H(−) is detected in all seven target sources, including four sources where no anions have been previously detected: L1172, L1389, L1495B, and TMC-1C. The C6H(−) /C6H column density ratio is approx. > 1.0% in every source, with a mean value of 3.0% (and standard deviation 0.92%). Combined with previous detections, our results show that anions are ubiquitous in dense clouds wherever C6H is present. The C6H(−)/C6H ratio is found to show a positive correlation with molecular hydrogen number density, and with the apparent age of the cloud.We also report the first detection of C4H(−) in TMC-1 (at 4.8 sigma confidence), and derive an anion-to-neutral ratio C4H(−) /C4H = (1.2 +/- 0.4)×10(exp −5)(= 0.0012% +/- 0.0004%). Such a low value compared with C6H(−) highlights the need for a revised radiative electron attachment rate for C4H. Chemical model calculations show that the observed C4H(−) could be produced as a result of reactions of oxygen atoms with C5H(−) and C6H(−).

ISM↗
NASA NTRS2012

Transformation of Graphitic and Amorphous Carbon Dust to Complex Organic Molecules in a Massive Carbon Cycle in Protostellar Nebulae

More than 95% of silicate minerals and other oxides found in meteorites were melted, or vaporized and recondensed in the Solar Nebula prior to their incorporation into meteorite parent bodies. Gravitational accretion energy and heating via radioactive decay further transformed oxide minerals accreted into planetesimals. In such an oxygen-rich environment the carbonaceous dust that fell into the nebula as an intimate mixture with oxide grains should have been almost completely converted to CO. While some pre-collapse, molecular-cloud carbonaceous dust does survive, much in the same manner as do pre-solar oxide grains, such materials constitute only a few percent of meteoritic carbon and are clearly distinguished by elevated D/H, N-15/N-16, C-13/C-12 ratios or noble gas patterns. Carbonaceous Dust in Meteorites: We argue that nearly all of the carbon in meteorites was synthesized in the Solar Nebula from CO and that this CO was generated by the reaction of carbonaceous dust with solid oxides, water or OH. It is probable that some fraction of carbonaceous dust that is newly synthesized in the Solar Nebula is also converted back into CO by additional thermal processing. CO processing might occur on grains in the outer nebula through irradiation of CO-containing ice coatings or in the inner nebula via Fischer-Tropsch type (FTT) reactions on grain surfaces. Large-scale transport of both gaseous reaction products and dust from the inner nebula out to regions where comets formed would spread newly formed carbonaceous materials throughout the solar nebula. Formation of Organic Carbon: Carbon dust in the ISM might easily be described as inorganic graphite or amorphous carbon, with relatively low structural abundances of H, N, O and S . Products of FTT reactions or organics produced via irradiation of icy grains contain abundant aromatic and aliphatic hydrocarbons. aldehydes, keytones, acids, amines and amides.. The net result of the massive nebular carbon cycle is to convert relatively inert carbonaceous dust from the ISM into the vital organic precursors to life such as amino acids and sugars intimately mixed with dust and ice in primitive planetesimals. Since the number of carbon atoms entering the Solar Nebula as dust exceeds the number of atoms entering the nebula as oxide grains. the formation of large quantities of complex organic molecules may represent the largest single chemical cycle in the nebula.

Nuth, Joseph A., III↗
NASA NTRS2004

Small-scale Interstellar Structure Toward the Open Cluster Chi Persei; Program ID: BO29 (Cycle 2)

The primary objective of this program was to obtain FUSE observations of the interstellar H2 absorption toward six early-type stars in the core of the open star cluster Chi Persei. High resolution optical observations of the interstellar Na I absorption toward these stars and others in the core of Chi Per have revealed a rich variety of small-scale diffuse ISM structure in both the distant Perseus and more local Orion spiral arms. At the 1 arc minute angular scales typically probed by the separations of these stars, this structure corresponds to respective physical length scales of 0.6 and 0.15 pc in the Perseus and Orion arm gas. The principal scientific goal of the FUSE observations was to determine if this small-scale Na I structure toward the core of Chi Per was reflected in the abundance and/or excitation of interstellar H2. In September 2001, we obtained FUSE observations of the Chi Per stars BD +56 563, BD +56 571, BD +56 573, BD +56 574, BD +56 575, and BD +56 578 for this program. The data reveal that the Perseus arm gas exhibits significant small-scale variations in the strength of its molecular hydrogen absorption while the Orion arm H2 absorption is relatively uniform. We presented these results at the January 2003 American Astronomical Society meeting in Seattle, WA (points, Meyer, Lauroesch, Nguyen, and Friedman 2002, Bulletin of the American Astronomical Society, 34,1229). Since Na I is not a dominant ion in H I clouds, the variations detected in the Perseus arm Na I line profiles could be due to spatial differences in either the physical structure or the physical conditions in the gas. Although many of the H2 absorption profiles are too saturated or too weak to be definitive in this regard, it is clear that small-scale variations are present in H2 gas with excitation as high as the J=4 rotational level. In contrast, lower spatial resolution H I 21 cm studies of the Perseus arm gas across the face of the h and Chi Per double cluster have shown smoother, continuous variations on the larger scale. In order to investigate if the global velocity structure of H2 toward h and Chi Per more closely follows the chaotic structure seen in interstellar Na I absorption or the smoother, continuous H I structure, we have expanded our FUSE study with a Cycle 4 program (D902, PI: Points) to survey the H2 absorption toward a number of other stars across the face of the double cluster. We have obtained FUSE spectra of 14 additional h and Chi Per stars through this program and are now combining all of the data into a comprehensive study that will be submitted for publication next year.

Meyer, David M.↗
NASA NTRS1994

The Orion OB1 association. 1: Stellar content

Walfraven photometry of established and probable members of the Orion OB1 association is presented. Effective temperature, surface gravity, luminosity and mass are derived for all stars, using atmosphere model by Kurucz (1979). Absolute magnitudes are calculated using the Straizys and Kuriliene (1981) tables. Distance moduli and visual extinctions are determined. A comparison of the visual extinctions to IRAS 100 micrometers data shows that the near edge of the Orion A and B clouds lies at a distance of approximately 320 pc, while the far edge is at approximately 500 pc. A method for deriving the ages of the subgroups by comparing theoretical isochrones to the observations in the log g, log T(sub eff) plane is presented. The derived ages suggest, contrary to earlier studies, that subgroup 1b is younger than 1c, which can possibly be explained by past geometries of the system of stars and gas. The initial mass function for Orion OB1 is derived with the aid of the Kolmogorov-Smirnoff test. Through extensive simulations, we show that it is very difficult to derive accurately the Initial Mass Function (IMF) from the available data. To within somewhat weak limits the IMF is found to be of the form xi(log M) = AM(exp -1.7 +/- 0.2) for all subgroups. The energy output of the subgroups in the form of stellar winds and supernovae is calculated and compared to the observed size and expansion velocity of the Orion-Eridanus bubble. It is shown that the energy output of the association can account for the morphology and kinematics of the interstellar medium (ISM).

Brown, A. G. A.↗
NASA NTRS1995

Processing Mechanisms for Interstellar Ices: Connections to the Solar System

The organic component of the interstellar medium, which has revealed itself through the ubiquitous 3.4 micrometers hydrocarbon absorption feature, is widespread throughout the disk of our galaxy and has been attributed to dust grains residing in the diffuse interstellar medium. The absorption band positions near 3.4 micrometers are characteristic of C-H stretching vibrations in the -CH3 and -CH2- groups of saturated aliphatic hydrocarbons associated with perturbing chemical groups. The production of complex molecules is thought to occur within dense molecular clouds when ice-mantled grains are processed by various energetic mechanisms. Studies of the processing of interstellar ices and the subsequent production of organic residues have relevance to studies of ices in the solar system, because primitive, icy solar system bodies such as those in the Kuiper belt are likely reservoirs of organic material, either preserved from the interstellar medium or produced in situ. Connections between the interstellar medium and the early solar nebula have long been a source of interest. A comparison of the interstellar organics and the Murchison meteorite illustrates the importance of probing the interstellar connection to the solar system, because although the carbonaceous meteorites are undoubtedly highly processed, they do retain specific interstellar signatures (such as diamonds, SiC grains, graphite and enriched D/H). The organic component, while not proven interstellar, has a remarkable similarity to the interstellar organics observed in over a dozen sightlines through our galaxy. This paper compares spectra from laboratory organics produced through the processing of interstellar ice analog materials with the high resolution infrared observations of the interstellar medium in order to investigate the mechanisms (such as ion bombardment, plasma processing, and UV photolysis) that may be producing the organics in the ISM.

Pendleton, Y. J.↗
NASA NTRS2016

The Formation of Nucleobases from the Irradiation of Purine in Astophysical Ices and Comparisons with Meteorites.

N-heterocycles have been identified in meteorites and their extraterrestrial origins are suggested by isotopic ratio measurements. Although small N- heterocycles have not been detected in the interstellar medium (ISM), recent experiments in our lab have shown that the irradiation of the aromatic molecules like benzene (C6H6) and naphthalene (C10H8) in mixed molecular ices leads to the formation of O- and N-heterocyclic molecules. Among the class of N-heterocycles are the nucleobases, which are of astrobiological interest because they are the information bearing units of DNA and RNA. Nucleobases have been detected in meteorites [3-5], with isotopic signatures that are also consistent with an extraterrestrial origin. Three of the biologically relevant nucleobases (uracil, cytosine, and guanine) have a pyrimidine core structure while the remaining two (adenine and guanine) possess a purine core. Previous experiments in our lab have demonstrated that all of the bio-logical nucleobases (and numerous other molecules) with a pyrimidine core structure can be produced by irradiating pyrimidine in mixed molecular ices of several compositions [6-8]. In this work, we study the formation of purine-based molecules, including the nucleobases adenine, and guanine, from the ultraviolet (UV) irradiation of purine in ices consisting mixtures of H2O and NH3 at low temperature. The experiments are designed to simulate the astrophysical conditions under which these species may be formed in dense molecular clouds, protoplanetary disks, or on the surfaces of icy bodies in planetary systems.

Astrochemistry↗
NASA NTRS1993

The ISM in the M82 starburst

We have observed (O 1) (63 microns) and (Si 2) (35 microns) in the central 700 pc of the starburst galaxy M82. The luminosities in these transitions are 7.1 x 10(exp 7) solar luminosity and 6.2 x 10(exp 7) solar luminosity, respectively, which are each approx. 0.15% of the bolometric luminosity from this region. The ratios of (O 1) line luminosity to (O 3), (Si 2) (35 microns), and to bolometric luminosities in M82 are similar to those in M42, M17, and Sgr A. These similarities, and the association of the bulk of the (O 1) and (Si 2) emission with the ionized emission, suggest that the dominant emission mechanism for (O 1) and (Si 2) in M82 is the same as in these Galactic regions, namely warm gas photodissociated by UV flux from the OB stars responsible for the nearby H 2 regions. We argue that shock or x ray heated gas or H 2 plasma is a minor contributor to the intensities of these fine structure lines. Both the (O 1) (53 microns) and the (Si 2) (35 microns) spectrum show an asymmetric line profile indistinguishable in shape from those of the (O 3) (52 and 88 microns) and (N 3) (57 microns) lines and similar to that of the more extended (C 2) 158 micron line measured previously in M82. We detect two distinct velocity components, which we attribute to emission from two regions at either end of the central bar, where the bar connects to an orbiting torus of neutral gas seen in H 1 and CO J = 1-0. We model separately the two velocity components and derive the physical conditions in these two regions. The clouds in these regions are small, R approx. 1-2 pc, have warm neutral gas surfaces, T approx. 200 K, and are concentrated with volume filling factors of approx. 0.02 and area filling factors of 1-5. The entire central region (R approx. 700 pc) is characterized by a large number, approx. 5 x 10(exp 4), of 2 x 10(exp 3) solar mass clouds with surface densities of approx. 3 x 10(exp 4) cm(exp -3), illuminated by FUV fluxes 10(exp 4) times the average local interstellar value for the Milky Way. These clouds reside in the harsh conditions of a starburst nucleus, with photoevaporation times of 10(exp 6) yr, and collision timescales only about an order of magnitude longer.

Lord, Steven↗
NASA NTRS1990

Starburst outflows from nearby galaxies

Starburst outflows from NGC 5461, 1569 and M82 are discussed. The Sc I galaxy, M101, is reknowned for the kpc-size superassociations of star clusters and HII regions that dominate its spiral arms. NGC 5461 is one of the brightest of these superassociations, rivaling the Large Magellanic Cloud in H alpha luminosity. The NGC 5461 superassociation is dominated by a single unresolved HII region of outstanding luminosity (approx. 1000 Orion nebulae). Detailed examination of corresponding continuum images indicates that only the southern plume has any sort of stellar counterpart. The other plumes are clearly diffuse with no underlying hot stars. An image of NGC 1569 is discussed. Besides showing the peculiar arm noted by Zwicky (1971) and the filamentary extensions to the North and South (as noted by Hodge 1974), this image also reveals two arc-like features of diffuse ionized gas to the South. Both arcs are concentric with the bright center of the galaxy - where the super star clusters, A and B are located. The inner arc (Arc 1) appears to follow the same curve as the SW arm thus suggesting that the two features represent limb-brightened fragments of vast superbubble that was blown out by a central starburst sometime in the past. As the classic starburst galaxy, M82 displays all the luminous hallmarks of intense high-mass star formation and outflow activity. The diffuse H alpha and x ray emitting gas along the minor axis provides especially good evidence for a bipolar outflow of hot gas which is shock heating the swept-up interstellar medium (ISM) to temperatures of approx. 10(exp 4) K. An image shows the H alpha emission within the disk and along the minor axis. Another image shows the same field in the light of near-infrared. Both figures are based on charge coupled device images taken with the McGraw-Hill 1.3 m telescope (Waller 1989). The longer wavelength emission clearly shows a more extended morphology along the major axis. The morphological discrepancy is most likely due to the greater obscuration by dust suffered by the H alpha photons. A third image shows the map of visual extinction that researchers derive from a pixel-by-pixel comparison of the (SIII) and H alpha fluxes. The greatest extinctions are evident along an arc that includes two especially obscured regions on opposite sides of the bursting nucleus.

Waller, William H.↗
DOE OSTI2022

Differences in chemical evolution between isolated and embedded prestellar cores

Models of prestellar cores often assume that the cores are isolated from their environment – material outside the core boundary plays no role in the subsequent evolution. This is unlikely to be the case in reality, where cores are located within hierarchically substructured molecular clouds. Here, we investigate the dynamical and chemical evolution of prestellar cores, modelled as Bonnor–Ebert spheres, and show that the density of the ambient medium has a large impact on the resulting chemical properties of the cores. Models embedded in high-density, low-temperature surroundings have greatly enhanced abundances of several molecules, such as CO and CS, compared to models with more diffuse surroundings, corresponding to relatively isolated cores. The predicted intensities and profile shapes of molecular lines are also affected. The density of the ambient medium has a stronger effect on the chemical evolution than whether the cores are initially in or out of equilibrium. This suggests that the impact of environment cannot be neglected when modelling chemistry in prestellar cores; the results of these models are highly sensitive to the assumptions made about the core surroundings.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2014

Interstellar Organics, the Solar Nebula, and Saturn's Satellite Phoebe

The diffuse interstellar medium inventory of organic material (Pendleton et al. 1994, Pendleton & Allamandola 2002) was likely incorporated into the molecular cloud in which the solar nebula condensed. This provided the feedstock for the formation of the Sun, major planets, and the smaller icy bodies in the region outside Neptune's orbit (transneptunian objects, or TNOs). Saturn's satellites Phoebe, Iapetus, and Hyperion open a window to the composition of one class of TNO as revealed by the near-infrared mapping spectrometer (VIMS) on the Cassini spacecraft at Saturn. Phoebe (mean diameter 213 km) is a former TNO now orbiting Saurn. VIMS spaectral maps of PHoebe's surface reveal a complex organic spectral signature consisting of prominent aromatic (CH) and alophatic hydrocarbon (CH2, CH3) absorption bands (3.2-3.6 micrometers). Phoebe is the source of a huge debris ring encircling Saturn, and from which particles (approximately 5-20 micrometer size) spiral inward toward Saturn. They encounter Iapetus and Hperion where they mix with and blanket the native H2O ice of those two bodies. Quantitative analysis of the hydrocarbon bands on Iapetus demonstrates that aromatic CH is approximately 10 times as abundant as aliphatic CH2+CH3, significantly exceeding the strength of the aromatic signature in interplanetary dust particles, comet particles, ad in carbonaceous meteorites (Cruikshank et al. 2013). A similar excess of aromatics over aliphatics is seen in the qualitative analysis of Hyperion and Phoebe itself (Dalle Ore et al. 2012). The Iapetus aliphatic hydrocarbons show CH2/CH3 approximately 4, which is larger than the value found in the diffuse ISM (approximately 2-2.5). In so far as Phoebe is a primitive body that formed in the outer regions of the solar nebula and has preserved some of the original nebula inventory, it can be key to understanding the content and degree of procesing of the nebular material. There are other Phoebe-like TNOs that are presently beyond our ability to study in the organic spectral region, but JWST will open that possibility for a number of objects. We now need to explore and understand the connection of this organic-bearing Solar System material to the solar nebula the the inventory of ISM materials incorporated therein.

Interstellar↗
NASA NTRS2014

Interstellar Organics, the Solar Nebula, and Saturn's Satellite Phoebe

The diffuse interstellar medium inventory of organic material (Pendleton et al. 1994, Pendleton Allamandola 2002) was likely incorporated into the molecular cloud in which the solar nebula condensed. This provided the feedstock for the formation of the Sun, major planets, and the smaller icy bodies in the region outside Neptune's orbit (transneptunian objects, or TNOs). Saturn's satellites Phoebe, Iapetus, and Hyperion open a window to the composition of one class of TNO as revealed by the near-infrared mapping spectrometer (VIMS - Visible and Infrared Mapping Spectrometer) on the Cassini spacecraft at Saturn. Phoebe (mean diameter 213 kilometers) is a former TNO now orbiting Saturn. VIMS spectral maps of Phoebe's surface reveal a complex organic spectral signature consisting of prominent aromatic (CH) and aliphatic hydrocarbon (CH2, CH3) absorption bands (3.2-3.6 meters). Phoebe is the source of a huge debris ring encircling Saturn, and from which particles (5-20 meter size) spiral inward toward Saturn. They encounter Iapetus and Hyperion where they mix with and blanket the native H2O ice of those two bodies. Quantitative analysis of the hydrocarbon bands on Iapetus demonstrates that aromatic CH is 10 times as abundant as aliphatic CH2 plus CH3, significantly exceeding the strength of the aromatic signature in interplanetary dust particles, comet particles, and in carbonaceous meteorites (Cruikshank et al. 2013). A similar excess of aromatics over aliphatics is seen in the qualitative analysis of Hyperion and Phoebe itself (Dalle Ore et al. 2012). The Iapetus aliphatic hydrocarbons show CH2/CH3 4, which is larger than the value found in the diffuse ISM (InterStellar Matter - (2-2.5). Insofar as Phoebe is a primitive body that formed in the outer regions of the solar nebula and has preserved some of the original nebula inventory, it can be key to understanding the content and degree of processing of that nebular material. There are other Phoebe-like TNOs that are presently beyond our ability to study in the organic spectral region, but JWST (James Webb Space Telescope) will open that possibility for a number of objects. We now need to explore and understand the connection of this organic-bearing Solar System material to the solar nebula and the inventory of ISM (Interstellar Medium) materials incorporated therein.

Phoebe↗
DOE OSTI2022

The Davis–Chandrasekhar–Fermi method revisited

ABSTRACT Despite the rich observational results on interstellar magnetic fields in star-forming regions, it is still unclear how dynamically significant the magnetic fields are at varying physical scales, because direct measurement of the field strength is observationally difficult. The Davis–Chandrasekhar–Fermi (DCF) method has been the most commonly used method to estimate the magnetic field strength from polarization data. It is based on the assumption that gas turbulent motion is the driving source of field distortion via linear Alfvén waves. In this work, using MHD simulations of star-forming clouds, we test the validity of the assumption underlying the DCF method by examining its accuracy in the real 3D space. Our results suggest that the DCF relation between turbulent kinetic energy and magnetic energy fluctuation should be treated as a statistical result instead of a local property. We then develop and investigate several modifications to the original DCF method using synthetic observations, and propose new recipes to improve the accuracy of DCF-derived magnetic field strength. We further note that the biggest uncertainty in the DCF analysis may come from the linewidth measurement instead of the polarization observation, especially since the line-of-sight gas velocity can be used to estimate the gas volume density, another critical parameter in the DCF method.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2001

Organic Signature of Dust from the Interstellar Medium (ISM)

Dust in the ISM carries an "organic" signature in form of a distinct group of C-H stretching bands, both in emission and absorption, around 3.4 micrometers. These bands agree with the symmetrical and asymmetrical C-H stretching vibrations of aliphatic -CH2- entities and are thought to be associated with organic molecules on the surface of dust grains. We show that this interpretation is inconsistent with laboratory experiments. Synthetic MgO and natural olivine single crystals, grown from a CO/CO2/H2O-saturated melt, exhibit the same C-H stretching bands but those bands are clearly associated with C-H entities inside the dense mineral matrix. The multitude of C-H stretching bands suggests that the C-H bonds arise from polyatomic C(sub n) entities. We heated the MgO and olivine crystals to temperatures between 550-1000 K to pyrolyze the C-H bonds and to cause the C-H stretching bands to disappear. Upon annealing at moderate temperatures between 300-390 K the C-H stretching bands reappear within a few days to weeks. The C-H stretching band intensity increases linearly with the square root of time. Thus, while the pyrolysis broke the C-H bonds and caused the H to disperse in the mineral matrix, the H atoms (or H2 molecules) are sufficiently mobile to return during annealing and reestablish the C-H bonds. Dust grains that condense in a gas-laden environment (outflow of late-stage stars or in dense molecular clouds) probably incorporate the same type of Cn-H entities. Imbedded in and in part bonded to the surrounding mineral matrix, the Cn-H entities display C-H stretching bands in the 3.4 micrometer region, but their lower frequency librational modes are so strongly coupled to the lattice modes that they broaden excessively and thus become unobservable.

Freund, Friedemann↗