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At least 235 records · Page 13
All sourcesNASA NTRSDOE OSTI
DOE OSTI2016

Magnetic dipole interactions in crystals

The influence of magnetic dipole interactions (MDIs) on the magnetic properties of local-moment Heisenberg spin systems is investigated. A general formulation is presented for calculating the eigenvalues λ and eigenvectors μ ˆ of the MDI tensor of the magnetic dipoles in a line (one dimension, 1D), within a circle (2D) or a sphere (3D) of radius r surrounding a given moment μ → i for given magnetic propagation vectors k for collinear and coplanar noncollinear magnetic structures on both Bravais and non-Bravais spin lattices. Results are calculated for collinear ordering on 1D chains, 2D square and simple-hexagonal (triangular) Bravais lattices, 2D honeycomb and kagomé non-Bravais lattices, and 3D cubic Bravais lattices. The λ and μ ˆ values are compared with previously reported results. Calculations for collinear ordering on 3D simple tetragonal, body-centered tetragonal, and stacked triangular and honeycomb lattices are presented for c/a ratios from 0.5 to 3 in both graphical and tabular form to facilitate comparison of experimentally determined easy axes of ordering on these Bravais lattices with the predictions for MDIs. Comparisons with the easy axes measured for several illustrative collinear antiferromagnets (AFMs) are given. The calculations are extended to the cycloidal noncollinear 120 ° AFM ordering on the triangular lattice where λ is found to be the same as for collinear AFM ordering with the same k. The angular orientation of the ordered moments in the noncollinear coplanar AFM structure of GdB 4 with a distorted stacked 3D Shastry-Sutherland spin-lattice geometry is calculated and found to be in disagreement with experimental observations, indicating the presence of another source of anisotropy. Similar calculations for the undistorted 2D and stacked 3D Shastry-Sutherland lattices are reported. The thermodynamics of dipolar magnets are calculated using the Weiss molecular field theory for quantum spins, including the magnetic transition temperature T m and the ordered moment, magnetic heat capacity, and anisotropic magnetic susceptibility χ versus temperature T . The anisotropic Weiss temperature θ p in the Curie-Weiss law for T>T m is calculated. A quantitative study of the competition between FM and AFM ordering on cubic Bravais lattices versus the demagnetization factor in the absence of FM domain effects is presented. The contributions of Heisenberg exchange interactions and of the MDIs to T m and to θ p are found to be additive, which simplifies analysis of experimental data. Some properties in the magnetically-ordered state versus T are presented, including the ordered moment and magnetic heat capacity and, for AFMs, the dipolar anisotropy of the free energy and the perpendicular critical field. The anisotropic χ for dipolar AFMs is calculated both above and below the Néel temperature T N and the results are illustrated for a simple tetragonal lattice with c/a>1, c/a=1 (cubic), and c/a<1 , where a change in sign of the χ anisotropy is found at c/a=1 . Finally, following the early work of Keffer [Phys. Rev. 87, 608 (1952)], the dipolar anisotropy of χ above T N =69 K of the prototype collinear Heisenberg-exchange-coupled tetragonal compound MnF 2 is calculated and found to be in excellent agreement with experimental single-crystal literature data above 130 K, where the smoothly increasing deviation of the experimental data from the theory on cooling from 130 K to T N is deduced to arise from dynamic short-range collinear c -axis AFM ordering in this temperature range driven by the exchange interactions.

36 MATERIALS SCIENCE↗
DOE OSTI2014

North-south asymmetric solar cycle evolution: Signatures in the photosphere and consequences in the corona

The heliospheric current sheet is the continuum of the coronal magnetic equator that divides the heliospheric magnetic field into two sectors (polarities). Several recent studies have shown that the heliospheric current sheet is southward shifted during approximately 3 years in the solar declining phase (the so-called bashful ballerina phenomenon). In this article we study the hemispherical asymmetry in the photospheric and coronal magnetic fields using Wilcox Solar Observatory measurements of the photospheric magnetic field since 1976 as well as the potential field source surface model. Multipole analysis of the photospheric magnetic field shows that during the late declining phase of solar cycles since the 1970s, the 'bashful ballerina phenomenon' is a consequence of the g{sub 2}{sup 0} quadrupole term, signed oppositely to the dipole moment. Surges of new flux transport magnetic field from low latitudes to the poles, thus leading to a systematically varying contribution to the g{sub 2}{sup 0}-term from different latitudes. In the case of a north-south asymmetric flux production, this is seen as a quadrupole contribution traveling toward higher latitudes. When the quadrupole term is largest, the main contribution comes from the polar latitudes. At least during the four recent solar cycles, the g{sub 2}{sup 0}-term arises because the magnitude of the southern polar field is larger than the magnitude found in the north in the declining phase of the cycle. In the heliosphere this hemispheric asymmetry of the coronal fields is seen as a southward shift of the heliospheric current sheet by about 2°.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1995

Bounce-Averaged Hamiltonian for Charged Particles in an Axisymmetric but Nondipolar Model Magnetosphere

In order to facilitate bounce-averaged guiding center simulations of geomagnetically trapped particles, we express the kinetic energy of a particle with magnetic coordinates (L,phi) as an analytic function of the first two adiabatic invariants (M, J) and the L value of the field line. The magnetic field model is axisymmetric, consisting of a dipolar B field plus a uniform southward magnetic field parallel to the dipole moment mu(sub E). This model magnetosphere is surrounded by a circular equatorial neutral line whose radius b is an adjustable parameter. The L value of a field line is (by definition) inversely proportional to the flux enclosed by the corresponding magnetic shell of equatorial radius r(sub 0), and the L value at the neutral line (r(sub 0) = b) is denoted L*. The azimuthal coordinate phi measures magnetic local time. The best functional representation found for the normalized difference (L(exp 3)a(exp 3)/mu(sub E))(B(sub m) - B(sub 0)) between mirror-point field B(sub m) and equatorial field B(sub 0) along any field line is a 5-term expansion in powers (2/3 through 6/3) of the quantity X equivalent to (La/mu(sub E))(exp 1/2)K, where K equivalent to (J(exp 2)/8m(sub 0)M)(exp 1/2) is an adiabatically conserved quantity independent of particle energy, m(sub 0) is the rest mass of the particle, and a is the radius of the Earth. This functional form is motivated by results for limiting cases in which particles mirror very near and very far from the magnetic equator. Expansion coefficients corresponding to various powers of X are obtained from least squares fits to numerically computed results for X as a function of L and B(sub m). These are accurately expressible as fourth-order polynomials in (r(sub 0)/b)(exp 3), hence indirectly as functions of L/L* = 3La/2b. This representation, which leads (except for a manageably small region of parameter space) to better than 1% accuracy in the specification of B(sub m) as a function of K and L, allows bounce-averaged guiding center simulations to be performed without actually tracing the bounce motions of individual particles. Bounce-averaged drifts L' (meridional) and phi' (azimuthal) are proportional to derivatives of the Hamiltonian H (sum of kinetic and potential energies) with respect to phi and L, respectively. Our formulation thus provides a computationally efficient method for tracing the bounce-averaged adiabatic motion (conserving all three invariants) and nonadiabatic transport (violating the third invariant while conserving the first two invariants) of geomagnetically trapped particles in the model magnetosphere.

Schulz, Michael↗
DOE OSTI2017

First determination of ground state electromagnetic moments of Fe 53

Here, the hyperfine coupling constants of neutron deficient 53 Fe were deduced from the atomic hyperfine spectrum measured using the bunched-beam collinear laser spectroscopy technique. The low-energy 53 Fe beam was produced by projectile-fragmentation reactions followed by gas stopping, and used for the first time for laser spectroscopy. Ground state magnetic-dipole and electric-quadrupole moments were determined as μ= –0.65(1)μ N and Q=+35(15)e 2 fm 2 , respectively. The multiconfiguration Dirac-Fock method was used to calculate the electric field gradient to deduce Q from the quadrupole hyperfine coupling constant, since the quadrupole coupling constant has not been determined for any Fe isotopes. Both experimental values agree well with nuclear shell model calculations using the GXPF1A effective interaction performed in a full fp shell model space, which support the soft nature of the 56 Ni nucleus.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Group of Quantum Bits Acting as a Bit Using a Single-Domain Ferromagnet of Uniaxial Magnetic Ions

Read/write operations with individual quantum bits (i.e., qbits) are a demanding concern to solve in quantum computing. To alleviate this difficulty, we considered the possibility of using a group of qbits that act collectively as a bit (hereafter, a group bit or a gbit, in short). A promising candidate for a gbit is a single-domain ferromagnet (SDF) independent of its size, which can be prepared as a magnet of well-separated uniaxial magnetic ions (UMIs) at sites of no electric dipole moment with their uniaxial axes aligned along one common direction. When magnetized, the UMIs of such a magnet have a ferromagnetic (FM) arrangement and the resulting SDF becomes a gbit with its two opposite moment orientations representing the |0&rang; and |1&rang; states of a bit. Here, we probed the requirements for such magnets and identified several 2H-perovskites as materials satisfying these requirements.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2014

Alkali-vapor magnetic resonance driven by fictitious radiofrequency fields

We demonstrate an all-optical {sup 133}Cs scalar magnetometer, operating in nonzero magnetic field, in which the magnetic resonance is driven by an effective oscillating magnetic field provided by the AC Stark shift of an intensity-modulated laser beam. We achieve a projected shot-noise-limited sensitivity of 1.7fT/√(Hz) and measure a technical noise floor of 40fT/√(Hz). These results are essentially identical to a coil-driven scalar magnetometer using the same setup. This all-optical scheme offers advantages over traditional coil-driven magnetometers for use in arrays and in magnetically sensitive fundamental physics experiments, e.g., searches for a permanent electric dipole moment of the neutron.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2024

Improved stellarator permanent magnet designs through combined discrete and continuous optimizations

A common optimization problem in the areas of magnetized plasmas and fusion energy is the design of magnets to produce a given three-dimensional magnetic field distribution to high precision. When designing arrays of permanent magnets for stellarator plasma confinement, such problems have tens of thousands of degrees of freedom whose solutions, for practical reasons, should be constrained to discrete spaces. We perform a direct comparison between two algorithms that have been developed previously for this purpose, and demonstrate that composite procedures that apply both algorithms in sequence can produce substantially improved results. One approach uses a continuous, quasi-Newton procedure to optimize the dipole moments of a set of magnets and then projects the solution onto a discrete space. The second uses an inherently discrete greedy optimization procedure that has been enhanced and generalized for this work. Further, the approaches are both applied to design arrays cubic rare-Earth permanent magnets to confine a quasi-axisymmetric plasma with a magnetic field on axis of 0.5 T. The first approach tends to find solutions with higher field accuracy, whereas the second can find solutions with substantially (up to 30%) fewer magnets. When the approaches are combined, they can obtain solutions with magnet quantities comparable to the second approach while matching the field accuracy of the first.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

Nuclear relaxation in an electric field enables the determination of isotropic magnetic shielding

It is shown that in contrast to the case of nuclear relaxation in a magnetic field B, simultaneous application of the magnetic field B and an additional electric field E causes transverse relaxation of a spin-1/2 nucleus with the rate proportional to the square of the isotropic part of the magnetic shielding tensor. This effect can contribute noticeably to the transverse relaxation rate of heavy nuclei in molecules that possess permanent electric dipole moments. Relativistic quantum mechanical computations indicate that for {sup 205}Tl nucleus in a Pt-Tl bonded complex, Pt(CN){sub 5}Tl, the transverse relaxation rate induced by the electric field is of the order of 1 s{sup −1} at E = 5 kV/mm and B = 10 T.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2015

Helicon waves in uniform plasmas. II. High m numbers

Helicons are whistler modes with azimuthal wave numbers. They have been studied in solids and plasmas where boundaries play a role. The present work shows that very similar modes exist in unbounded gaseous plasmas. Instead of boundaries, the antenna properties determine the topology of the wave packets. The simplest antenna is a magnetic loop which excites m = 0 or m = 1 helicons depending on whether the dipole moment is aligned parallel or perpendicular to the ambient background magnetic field B{sub 0}. While these low order helicons have been described by J. M. Urrutia and R. L. Stenzel [“Helicon modes in uniform plasmas. I. Low m modes,” Phys. Plasmas 22, 092111 (2015)], the present work focuses on high order modes up to m = 8. These are excited by antenna arrays forming magnetic multipoles. Their wave magnetic field has been measured in space and time in a large and uniform laboratory plasma free of boundary effects. The observed wave topology exhibits m pairs of unique field line spirals which may have inspired the name “helicon” to this mode. All field lines converge into these nested spirals which propagate like corkscrews along B{sub 0}. The field lines near the axis of helicons are perpendicular to B{sub 0} and circularly polarized as in parallel whistlers. Helical antennas couple to these transverse fields but not to the spiral fields of helicons. Using a circular antenna array of phased m = 0 loops, right or left rotating or non-rotating multipole antenna fields are generated. They excite m < 0 and m > 0 modes, showing that the plasma supports both modes equally well. The poor excitation of m < 0 modes is a characteristic of loops with dipole moment across B{sub 0}. The radiation efficiency of multipole antennas has been found to decrease with m.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS2012

Statistical Theory of the Ideal MHD Geodynamo

A statistical theory of geodynamo action is developed, using a mathematical model of the geodynamo as a rotating outer core containing an ideal (i.e., no dissipation), incompressible, turbulent, convecting magnetofluid. On the concentric inner and outer spherical bounding surfaces the normal components of the velocity, magnetic field, vorticity and electric current are zero, as is the temperature fluctuation. This allows the use of a set of Galerkin expansion functions that are common to both velocity and magnetic field, as well as vorticity, current and the temperature fluctuation. The resulting dynamical system, based on the Boussinesq form of the magnetohydrodynamic (MHD) equations, represents MHD turbulence in a spherical domain. These basic equations (minus the temperature equation) and boundary conditions have been used previously in numerical simulations of forced, decaying MHD turbulence inside a sphere [1,2]. Here, the ideal case is studied through statistical analysis and leads to a prediction that an ideal coherent structure will be found in the form of a large-scale quasistationary magnetic field that results from broken ergodicity, an effect that has been previously studied both analytically and numerically for homogeneous MHD turbulence [3,4]. The axial dipole component becomes prominent when there is a relatively large magnetic helicity (proportional to the global correlation of magnetic vector potential and magnetic field) and a stationary, nonzero cross helicity (proportional to the global correlation of velocity and magnetic field). The expected angle of the dipole moment vector with respect to the rotation axis is found to decrease to a minimum as the average cross helicity increases for a fixed value of magnetic helicity and then to increase again when average cross helicity approaches its maximum possible value. Only a relatively small value of cross helicity is needed to produce a dipole moment vector that is aligned at approx.10deg with the rotation axis.

Shebalin, J. V.↗
NASA NTRS1991

The magnetic field and magnetospheric configuration of Uranus

A significant and unique planetary magnetic field discovered by Voyager 2 is presented. A large tilt of 58.6 deg of the magnetic-dipole axis from the rotation axis was found. Combined with a large offset of 0.3 RU of the magnetic dipole from the center of the planet, the moment of 0.23 gauss-RU3 leads to field magnitudes at the surface which vary widely between 0.1 and 1.0 gauss. A simple diagram illustrating the offset tilted dipole of Uranus and some field lines is shown. A more exact and accurate spherical-harmonic model of the planetary field, which includes both dipole and quadrupole moments, is derived. There exists a well-developed bipolar magnetic tail on the night side of the planet which rotates daily about the extended planet-sunline with Uranus because of the large obliquity of the Uranian rotation axis.

Ness, Norman F.↗
DOE OSTI2019

Ground-state electromagnetic moments of Ca 37

The hyperfine coupling constants of neutron deficient 37 Ca were deduced from the atomic hyperfine spectrum of the 4 s 2 S 1/2 ↔ 4 p 2 P 3/2 transition in Ca II , measured using the collinear laser spectroscopy technique. The ground-state magnetic-dipole and spectroscopic electric-quadrupole moments were observed for the first time as μ=+0.7453(72)μ N and Q = -15(11) e 2 fm 2 , respectively. The experimental values agree well with nuclear shell-model calculations using the universal sd model-space Hamiltonians versions A and B (USDA/B) in the sd -model space with a 95% probability of the canonical nucleon configuration. It is demonstrated that the magnetic moment of 39 Ca requires a larger non- sd -shell component than that of 37 Ca for good agreement with the shell-model calculation, suggests a more robust closed subshell structure of 36 Ca at the neutron number N =16 than 40 Ca. The results are also compared to valence-space in-medium similarity renormalization group calculations based on chiral two- and three-nucleon interactions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Single-ion properties of the S eff = 1 2 XY antiferromagnetic pyrochlores Na A ' Co 2 F 7 ( A ' = Ca 2 + , Sr 2 + )

The antiferromagnetic pyrochlore material NaCaCo 2 F 7 is a thermal spin liquid over a broad temperature range (≈140 K down to T F =2.4 K), in which magnetic correlations between Co 2+ dipole moments explore a continuous manifold of antiferromagnetic XY states. The thermal spin liquid is interrupted by spin freezing at a temperature that is ~2% of the mean-field interaction strength, leading to short-range static XY clusters with distinctive relaxation dynamics. Here we report the low-energy inelastic neutron scattering response from the related compound NaSrCo 2 F 7 , confirming that it hosts the same static and dynamic spin correlations as NaCaCo 2 F 7 . We then present the single-ion levels of Co 2+ in these materials as measured by inelastic neutron scattering. An intermediate spin-orbit coupling model applied to an ensemble of trigonally distorted octahedral crystal fields accounts for the observed transitions. The single-ion ground state of Co 2+ is a Kramers doublet with a strongly XY-like g tensor ( gxy/gz ~3). The local disorder inherent from the mixed pyrochlore A sites (Na + /Ca 2+ and Na + /Sr 2+ ) is evident in these measurements as exaggerated broadening of some of the levels. A simple model that reproduces the salient features of the single-ion spectrum produces approximately 8.4% and 4.1% variation in the z and xy components of the g tensor, respectively. In conclusion, this study confirms that an S eff = 1/2 model with XY antiferromagnetic exchange and weak exchange disorder serves as a basic starting point in understanding the low-temperature magnetic behavior of these strongly frustrated magnets.

36 MATERIALS SCIENCE↗
DOE OSTI2015

Search for exotic short-range interactions using paramagnetic insulators

We describe a proposed experimental search for exotic spin-coupled interactions using a solid-state paramagnetic insulator. The experiment is sensitive to the net magnetization induced by the exotic interaction between the unpaired insulator electrons with a dense, nonmagnetic mass in close proximity. An existing experiment has been used to set limits on the electric dipole moment of the electron by probing the magnetization induced in a cryogenic gadolinium gallium garnet sample on application of a strong electric field. With suitable additions, including a movable source mass, this experiment can be used to explore “monopole-dipole” forces on polarized electrons with unique or unprecedented sensitivity. As a result, the solid-state, nonmagnetic construction, combined with the low-noise conditions and extremely sensitive magnetometry available at cryogenic temperatures could lead to a sensitivity over 10 orders of magnitude greater than exiting limits in the range below 1 mm.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2016

Pulsar magnetospheres: beyond the flat spacetime dipole

Most studies of the pulsar magnetosphere have assumed a pure magnetic dipole in flat spacetime. However, recent work suggests that the effects of general relativity are in fact of vital importance and that realistic pulsar magnetic fields will have a significant nondipolar component. We introduce a general analytical method for studying the axisymmetric force-free magnetosphere of a slowly rotating star of arbitrary magnetic field, mass, radius, and moment of inertia, including all the effects of general relativity. We confirm that spacelike current is generically present in the polar caps (suggesting a pair production region), irrespective of the stellar magnetic field. We show that general relativity introduces a ∼60% correction to the formula for the dipolar component of the surface magnetic field inferred from spindown. Finally, we show that the location and shape of the polar caps can be modified dramatically by even modestly strong higher moments. This can affect emission processes occurring near the star and may help explain the modified beam characteristics of millisecond pulsars.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

Optical activity of solids from first principles

Within the framework of independent particle approximation, the optical activity tensor of solids is formulated as from different contributions: the magnetic dipole, electric quadrupole, and band dispersion terms. The first two terms have similar counterparts in the theory of finite systems, whereas the last term is unique for crystals. Further, the magnetic dipole and electric quadrupole transition moments are calculated with a sum-over-states formulation. We apply the formulation to calculate and analyze the optical rotation of elemental tellurium and the circular dichroism of the (6,4) carbon nanotube. Decomposed optical activity into different contributions is discussed. The calculated spectra agree well with experiments. As a showcase of achiral crystals, we calculate the optical activity of wurtzite GaN.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Lifetime measurements of states of S 35 , S 36 , S 37 , and S 38 using the AGATA γ -ray tracking spectrometer

Lifetimes or lifetime limits of a small number of excited states of the sulfur isotopes with mass numbers A = 35 , 36, 37, and 38 have been measured using the differential recoil-distance method. The isotopes of sulfur were populated in binary grazing reactions initiated by a beam of 36 S ions of energy 225 MeV incident on a thin 208 Pb target which was mounted in the Cologne plunger apparatus. The combination of the PRISMA magnetic spectrometer and an early implementation of the AGATA γ-ray tracking array was used to detect γ rays in coincidence with projectile-like nuclear species. Lifetime measurements of populated states were measured within the range from about 1 to 100 ps. The number of states for which lifetime measurements or lifetime limits were possible was limited by statistics. For 35 S, the lifetime was determined for the first 1/2 + state at 1572 keV; the result is compared with a previous published lifetime value. The lifetime of the 3 - state of 36 S at 4193 keV was determined and compared with earlier measurements. No previous lifetime information exists for the (6 + ) state at 6690 keV; a lifetime measurement with large associated error was made in the present work. For 37 S, the states for which lifetime limits were established were those at 646 keV with J π = 3/2 - and at 2776 keV with J π = 11/2 - ; there are no previously published lifetime values for excited states of 37 S. Finally, a lifetime limit was established for the J π =(6 + ) state of 38 S at 3675 keV; no lifetime information exists for this state in the literature. Measured lifetime values were compared with the results of state-of-the-art shell-model calculations based on the PSDPF, SDPF-U, and FSU effective interactions. In addition, nuclear magnetic-dipole and electric-quadrupole moments, branching ratios, mixing ratios, and electromagnetic transition rates, where available, have been compared with shell-model values. The current work suffers from poor statistics; nevertheless, lifetime values and limits have been possible, allowing a useful discussion of the ability of state-of-the-art shell-model calculations to reproduce the experimental results.

electromagnetic transitions↗
NASA NTRS1976

High resolution spectral analyses of the Jovian decametric radiation. I - Burst morphology and drift rates

Morphological analyses of high-resolution spectral recordings of Jovian decametric radiation show a regime of phenomena not seen at lower resolutions. Observed emissions range from narrow-band (50 kHz) simple quasi-periodic bursts to wide-band emissions (extending over a 500-kHz passband) exhibiting complex structural detail. Assuming gyroemission from electrons in a dipole field for which the magnetic moment is 10 Gauss Jupiter-radius-cubed, drift-rate measurements of the bursts indicate that the source size is of the order of 600 km and its location is near 1.3 Jupiter radii at a colatitude of 27.3 deg. The measurements suggest that the emitting electrons belong to a population having a very specific equatorial pitch angle near 3.5 deg. This study concludes that it may be possible to verify gyroemission as the mechanism responsible for the decametric radiation.

Krausche, D. S.↗